Recommended Values of ²³⁹Pu, ²⁴⁰Pu and ^239+240Pu Concentrations in Reference Material IAEA-315 (Marine Sediment) Estimated by Thermal Ionisation Mass Spectrometry, Inductively Coupled Plasma-Mass Spectrometry and Alpha Spectrometry     

Taeko Shinonaga  Helmuth Aigner  Dilani Klose  Peter Spinder  Heinz Fröschl  David Donohue 《Geostandards and Geoanalytical Research》2008,32(1):93-101

The recommended concentrations of ²³⁹Pu, ²⁴⁰Pu and ^239+240Pu in reference material IAEA‐315 (marine sediment) were estimated by three analytical methods: isotope dilution thermal ionisation mass spectrometry (TIMS), isotope dilution inductively coupled plasma‐mass spectrometry (ICP‐MS) and alpha spectrometry. The determination of ²³⁹Pu and ²⁴⁰Pu (^239+240Pu by alpha spectrometry) was carried out with samples from randomly selected bottles using each method. Plutonium‐238 was also measured by alpha spectrometry. A plutonium‐242 reference material was used as a spike for the quantitative analysis. The influence of ²⁴²Pu in the samples was therefore calculated; however, this contribution was less than the range of uncertainty and did not influence the final results. The obtained data were statistically analysed using variance component analysis and paired comparison. The combined standard uncertainties from “method/measurement”, “bottle” and “sub‐sample” were in the order of 3 to 6%. The main contributions to the uncertainty were from the material heterogeneity and from systematic differences between methods. Based on this study with twenty‐seven analyses using 10–14 g sample mass, concentrations of (38 ± 3) Bq kg^?1, (28 ± 3) Bq kg^?1 and (66 ± 4) Bq kg^?1 are proposed as recommended values for ²³⁹Pu, ²⁴⁰Pu and ^239+240Pu, respectively, and (9.5 ± 0.4) Bq kg^?1 for ²³⁸Pu as an information value in reference material IAEA‐315. In mass concentration units, these amount to (16.4 ± 1.2) ng kg^?1, (3.3 ± 0.4) ng kg^?1 and (0.015 ± 0.003) ng kg^?1 for ²³⁹Pu, ²⁴⁰Pu and ²³⁸Pu, respectively. The certified reference materials NIST 4350B and NIST 4354 were also analysed by TIMS for quality assurance of the method used in this study.  相似文献   

陕西小秦岭地区太华群的重新厘定   总被引：2，自引：0，他引：2  

陈陇刚  王北颖  薛煜洲 《陕西地质》1997,(1)

陕西小秦岭地区太华群变质岩与国内外许多高级片麻岩区类似，存在大量的深成花岗质片麻岩体，它们经过多期变质变形作用，形成具不同基础岩石类型的多相片麻岩。本文在吸收前人研究成果的基础上，依据区内岩石组合的岩石学、岩石地球化学等特征，将原划太华群重新厘定为太华岩群、翁岔铺片麻岩套、太峪岭片麻岩套、佛头崖单元、罗斑花岗伟晶岩及葫芦沟变砂岩，并首次在本区建立了相应的构─岩石单位体系。  相似文献   

Profondeur d'extraction racinaire et signature isotopique de l'eau prélevée par les racines des couverts végétaux     

Zakaria Boujamlaoui  Thierry Bariac  Philippe Biron  Laurent Canale  Patricia Richard 《Comptes Rendus Geoscience》2005,337(6):589-598

We seek to identify the depth to which water is extracted by the roots in the soil. Indeed, in an isotopic steady-state condition of leaf water, transpiration introduces into the atmosphere a vapour whose isotopic signature is identical to that of root water. In the isotopic models of atmospheric general circulation, it is classically allowed that the signature of transpiration belongs to the meteoric water line. This supposes that the water taken by the roots has escaped with the evaporation of the soil and comes thus from the deep layers of the soil. At the time of experimentation carried out on maize plants (Nemours, Seine-et-Marne, France), this extraction depth was inferred from the comparison between the signature of the water measured on the level of the first internode of the stems of the plants and the isotopic profile of water in the soil. When the flow of transpiration reaches a maximum value, the plant uptakes water resulting from precipitations and which preserves its non-evaporating character after having quickly infiltrated in the deep layers of the soil. This relates to only 55% of the flux transpired by the canopy, the remainder presenting an evaporating character more or less marked according to ambient conditions. This experiment invalidates the classical hypothesis used in isotopic models of general atmospheric circulation in temperate regions. In fact, only half the amount of water vapour transpired by the canopy during the day presents a signature similar to that of the rainwater sampled in deep soil layers. To cite this article: Z. Boujamlaoui et al., C. R. Geoscience 337 (2005).  相似文献   

尺度转换视角下易武斗茶会的构建与变迁     

唐雪琼  徐海妙  尹铎 《地理科学》2022,42(1):136-142

选取易武斗茶会为研究案例,以尺度转换为理论分析工具,通过参与式观察法和半结构化访谈法,深入分析易武斗茶会的发展历程并展示推动其发展演变的多元社会主体的不同行动与实践。研究发现：① 易武斗茶会的演变过程中存在2种尺度转换的方式,一种是为迎合普洱茶市场细分而进行的尺度下推,另一种是根据地方发展需求而进行的尺度上推。② 易武斗茶会尺度转换是在地方政府的推动、茶企的支持、茶农的配合以及茶客的偏好下共同驱动的。③ 多元主体的行动在推动易武斗茶会尺度转换的过程中满足了各自群体的利益诉求,地方依凭茶叶经济实现了本土发展。从节事的角度对中国茶文化进行深入分析研究,为茶村如何通过地方性节事活动实现本土发展提供理论依据与案例借鉴。  相似文献   

Primary vs. secondary curved fold axes: Deciphering the origin of the Aït Attab syncline (Moroccan High Atlas) using paleomagnetic data     

《Journal of Structural Geology》2015

The Aït Attab syncline, located in the Central High Atlas, displays a curved geometry in plan view, and is considered as one of the most spectacular fold shapes in the Central High Atlasic belt. We conducted a paleomagnetic study in Jurassic-Cretaceous red beds to investigate the origin of this geometry. The Natural Remanent Magnetization (NRM) is dominated by a secondary magnetization carried by haematite with unvarying normal polarity that has been dated at about 100 Ma. The regional fold test performed in both limbs of the syncline is positive and the paleomagnetic vectors (after tectonic correction) are parallel throughout the curvature, indicating a negative oroclinal bending test. These results are inconsistent with previous works that consider the bent geometry of this syncline to result from subsequent distortion of originally NE–SW trending structures by rotation about a vertical axis. We interpret the NRM data to demonstrate that the changing trend of the Aït Attab syncline is a primary feature, resulting from the influence of pre-existing, NE–SW and E-W-striking extensional faults that developed during a strike-slip regime. Paleomagnetic results also reveal that the tilting observed in the sampled red beds is post Albian, probably linked to the Cenozoic inversion of the High Atlasic belt.  相似文献   

基于BPSO-NBayes的雷暴释用预报技术研究   总被引：1，自引：1，他引：0  

刘亚杰  胡邦辉  王学忠  王举  黄泓 《气象科学》2018,38(3):370-377

提出了一种新的雷暴预报法,即二进制粒子群-朴素贝叶斯分类器(Binary Particle Swarm Optimization-Naive Bayesian Classifiers,BPSO-NBayes)方法,以福州、连城、宁波3站为例,对使用T511数值预报产品站点的雷暴释用预报技术进行研究。利用2010—2014年T511数值预报产品和单站观测资料,使用BPSO-NBayes方法,建立了0~72 h雷暴预报模型,并与Fisher判别准则和Bayes判别准则进行比较。预报结果表明,BPSO-NBayes模型临界成功指数都在0.29以上,平均值达到0.33以上,是3种方法中最好的,空报率都在0.59以下,漏报率在0.60以下,而且变化幅度很小。BPSO-NBayes模型明显优于Fisher判别准则和Bayes判别准则,具有良好的稳定性和预报能力。  相似文献   

Rapid decrease of soil erosion rates with soil formation and vegetation development in periglacial areas     

Alessandra Musso  Michael E. Ketterer  Konrad Greinwald  Clemens Geitner  Markus Egli 《地球表面变化过程与地形》2020,45(12):2824-2839

High mountainous areas are geomorphologically active environments which are strongly shaped by redistribution of sediments and soils. With the projected climate warming in the twenty-first century and the continued retreat of glaciers, the area of newly exposed, highly erodible sediments and soils will increase. This presents a need to better understand and quantify erosion processes in young mountainous soils, as an increase in erodibility could threaten human infrastructure (i.e. hydroelectric power, tourist installations and settlements). While soil development is increasingly well understood and quantified, a coupling to soil erosion rates is still missing. The aim of this study was, therefore, to assess how soil erosion rates change with surface age. We investigated two moraine chronosequences in the Swiss Alps: one in the siliceous periglacial area of Steingletscher (Sustenpass), with soils ranging from 30 a to 10 ka, and the other in the calcareous periglacial area of Griessgletscher (Klausenpass) with surfaces ranging from age of 110 a to 13.5 ka. We quantified the erosion rates using the ^239+240Pu fallout radionuclides and compared them to physical and chemical soil properties and the vegetation coverage. We found no significant differences between the two parent materials. At both chronosequences, the erosion rates were highest in the young soils (on average 5−10 t ha^-1 a^-1 soil loss). Erosion rates decreased markedly after 3−5 ka of soil development (on average 1−2.5 t ha^-1 a^-1 soil loss) to reach a more or less stable situation after 10−14 ka (on average 0.3–2 t ha^-1 a^-1). Climate change not only causes glacier retreat, but also increased sediment dynamics. Depending on the relief and vegetational development, it takes up to at least 10 ka to reach soil stability. The establishment of a closed vegetation cover with dense root networks seems to be the controlling factor in the reduction of soil erodibility. © 2020 John Wiley & Sons, Ltd.  相似文献   

Active faulting in the frontal Rif Cordillera (Fes region,Morocco): Constraints from GPS data     

《Journal of Geodynamics》2014

The southern Rif cordillera front, between Fes and Meknes, is formed by the Prerif Ridges, which constitute a thrust and fold belt, in contact with the Saïss foreland basin. Geological evidence and regional GPS network data support recent and active tectonics of this Alpine cordillera, with a top-to-the-S-SW motion with respect to stable Africa. A local non-permanent GPS network was installed in 2007 around Fes to constrain the present-day activity of the mountain front. Six GPS sites are located in the Prerif mountain front (jbel Thratt and jbel Zalarh), the Saïss basin and the foreland constituted by the tabular Middle Atlas. Measurements of the GPS network in 2007, 2009 and 2012, over a five year span, seem to indicate that this region is tectonically active and is subjected to significant horizontal motions: (i) a regional displacement toward the SW with respect to stable Africa, showing an average rate of 2 mm/yr; (ii) a southwestward convergent motion between the jbel Thratt with respect to the Saïss basin and the eastern Zalarh ridge, with an average rate of about 4 mm/yr; and (iii) moderate NNE–SSW divergent dextral motion between the Saïss basin and the northern front of the tabular Middle Atlas with an average rate of about 1–2 mm/yr. The regional southwestward motion is related to the activity of the NE–SW sinistral North Middle Atlas-Kert fault zone, which follows the Moroccan Hot Line. Convergence between the Prerif ridges, located at the southern edge of the Rif, and the Saïss basin is accommodated by ENE–WSW striking northward dipping reverse sinistral faults and south vergent folds. In addition, increasing deformation toward the western ridges is in agreement with the stepped mountain front and the development of the arched structures of the Prerif ridges. Normal faults located south of the Saïss basin are responsible for local extension. Whereas the most active deformation occurs in the southern front of the jbel Thratt near Fes, the Saïss foreland basin and the Middle Atlas foreland have only moderate to low tectonic activity, as evidenced by geological and GPS data.  相似文献   

New Early Cretaceous shrimp (Decapoda) from the Sidi Aïch Formation of the Northern Chotts Range,southern Tunisia: Taxonomy,biostratigraphy, and palaeoenvironmental implications     

《Cretaceous Research》2017

The fossil dendrobranchiate shrimp Macropenaeus was originally described from the Upper Cretaceous (Cenomanian) limestones of Hadjoula, northwest Lebanon. A new species, M. sidiaichensis sp. nov., was recovered from the Sidi Aïch Formation in the Northern Chotts Range, southern Tunisia. The Barremian occurrence of the genus in Tunisia suggests that Macropenaeus most likely originated in northern Africa and then migrated to Arabia in the Cenomanian. The association of the fossil shrimp with conchostracans, plant fragments, and fish indicates the interaction of freshwater and marine conditions that characterized the northern African margin as part of widespread coastal complex, paralic environments during the Barremian.  相似文献   

Concentrations of 137Cs, 90Sr, 108m Ag, 239+240 Pu and atom ratio of 240Pu/239Pu in tanner crabs, Chionoecetes japonicus and Chionoecetes opilio collected around Japan     

Morita T  Ohtsuka Y  Fujimoto K  Minamisako Y  Iida R  Nakamura M  Kayama T 《Marine pollution bulletin》2010,60(12):2311-2322

The anthropogenic radionuclides, ¹³⁷Cs, ⁹⁰Sr, ^108mAg, ^239+240Pu, were measured in two Chionoecetes species, red queen crab (Chionoecetes japonicus) and snow crab (Chionoecetes opilio) collected around Japan during 1996–2007. There was no increase in the concentrations of these radionuclides and no large variation of the atom ratio of ²⁴⁰Pu/²³⁹Pu during this research period. These results indicated that the source of the radionuclides was not the radioactive wastes dumped by the former USSR and Russia and originated from past nuclear weapon tests. The higher atom ratio in the crab species than that from global fallout would be contributed by the Pacific Proving Grounds close-in fallout. The variability of the concentration of radionuclides in the crab species would result from the variability of the composition and quantity in the diet. However, the decrease in the concentration of radionuclides with sampling depth would depend on the concentration in the seawater and diet.  相似文献