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M.P. Collings J.W. Dever H.J. Fraser M.R.S. McCoustra 《Astrophysics and Space Science》2003,285(3-4):633-659
The interaction of carbon monoxide (CO) with vapour-deposited water(H2O) ices has been studied using temperature programmed desorption (TPD) and Fourier transform reflection-absorption infrared
spectroscopy (FT-RAIRS) over a range of astrophysically relevant temperatures. Such measurements have shown that CO desorption
from amorphous H2Oices is a much more complex process than current astrochemical models suggest. Re-visiting previously reported laboratory
experiments (Collings et al., 2003), a rate model has been constructed to explain, in a phenomenological manner, the desorption
of CO over astronomically relevant time scales. The model presented here can be widely applied to a range of astronomical
environments where depletion of CO from the gas phase is relevant. The model accounts for the two competing processes of CO
desorption and migration, and also enables the entrapment of some of the CO in the ice matrix and its subsequent release as
the water ice crystallises and then desorbs. The astronomical implications of this model are discussed.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
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This paper reports results from an experiment designed to measure the nascent rovibrational population of H2 molecules that have formed through the heterogeneous recombination of H atoms on the surface of cosmic dust analogues under
conditions approaching those of the interstellar medium (ISM). H2 that has formed on a highly oriented pyrolytic graphite (HOPG) surface has been detected, using laser induced resonance-enhanced
multi-photon ionization (REMPI), in the v = 1 (J= 0–3) rovibrational states at surface temperatures of 30 K and 50 K. These excited product molecules display rotational temperatures
significantly higher than the target surface temperature. These first results suggest that a considerable proportion of the
binding energy released on formation of the H2 is deposited in the surface, in addition to internal excitation of the product molecules.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
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S. Lepp 《Astrophysics and Space Science》2003,285(3-4):737-744
The evolution of the universe from times after the recombination of the first atoms is controlled by chemistry. Chemistry
can also help us to learn more about the first structures. In this paper we review the chemistry and atomic physics that are
important in the time shortly after recombination, including the formation of the first structures.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
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太阳系早期的短寿期放射性核素 总被引：2，自引：0，他引：2
较详细地介绍全新的太阳系起源理论——X-wind模式,天体化学实验发现太阳系早期存在大量的短寿期放射性核素(半衰期小于100Ma),这些核素对太阳系的形成和演化有重要的影响,一种理论认为,这些核素是在恒星内部合成,并由星风注入原太阳分子云,星风产生的激波诱发分子云核的塌缩而形成原太阳,另一种理论认为,这些核素是高能粒子与原太阳分子云或太阳星云中的气体和尘埃相互作用的产物。 相似文献
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