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1.
Continuous Measurement of Number Concentrations and
Elemental Composition of Aerosol Particles
for a Dust Storm Event in Beijing 总被引：1，自引：0，他引：1
A continuous measurement of number size distributions and chemical composition of aerosol particles was conducted in Beijing in a dust storm event during 21-26 March 2001. The number concentration of coarse particles （ 〉2μm） increased more significantly than fine particles （ 〈2μm） during the dust storm due to dust weather, while the anthropogenic aerosols collected during the non-dust-storm period tended to be associated with fine particles. Elemental compositions were analyzed by using proton-induced X-ray emission （PIXE）. The results show that 20 elements in the dust storm were much higher than in the non-dust-storm period. The calculated soil dust concentration during the dust storm was, on average, 251.8μg m^-3, while it was only 52.1μg m^-3 on non-dust-storm days. The enrichment factors for Mg, A1, P, K, Ca, Ti, Mn, Fe, C1, Cu, Pb, and Zn show small variations between the dust storm and the non-dust-storm period, while those for Ca, Ni and Cr in the dust storm were much lower than those in the non-dust-storm period due to significant local emission sources. A high concentration and enrichment factor for S were observed during the dust storm, which implies that the dust particles were contaminated by aerosol particles from anthropogenic emissions during the long-range transport. A statistical analysis shows that the elemental composition of particles collected during the dust storm in Beijing were better correlated with those of desert soil colleted from desert regions in Inner Mongolia. Air mass back-trajectory analysis further confirmed that this dust storm event could be identified as streaks of dust plumes originating from Inner Mongolia. 相似文献
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2004年北京秋季大气颗粒物的化学组分和来源特征 总被引：1，自引：0，他引：1
2004年9月在北京城区进行了大气颗粒物采样,样品用PIXE方法进行了分析,得到了20种元素的浓度及其谱分布。并对北京颗粒物的谱分布、富集因子和来源进行了分析研究。发现K元素浓度分布呈细粒态单峰谱分布,细粒态K富集因子较高,表明了生物质燃烧的主要贡献。因子分析结果还表明,土壤尘、生物质燃烧、煤烟尘、工业源和汽车尾气排放源对秋季北京局地排放源有明显贡献。 相似文献
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西藏恰功铁矿岩浆演化序列及斑岩出溶流体特征 总被引：6，自引：1，他引：5
谢玉玲 李应栩 Zhaoshan CHANG David R. COOKE Chris G. RYAN Jamie LAIRD 白劲松 刘云飞 李光明 张丽 《地质学报》2009,83(12):1869-1886
冈底斯成矿带是碰撞造山过程形成的最重要的成矿带,恰功矽卡岩铁(铜)矿床即位于冈底斯成矿带中部.本文在详细的野外地质填图和室内研究基础上确定了恰功铁矿与成矿有关的斑岩体为二长花岗斑岩,锆石的U-Pb定年结果为68.8±2.2 Ma,明显早于冈底斯东部与后碰撞伸展有关的斑岩型矿床和主碰撞期形成的矽卡岩型矿床,其应代表了冈底斯一次尚未被充分认识到的成矿事件.通过对成矿斑岩的岩石学、岩石化学、岩浆出溶流体的包裹体岩相学、显微测温分析及包裹体成分的LRM、LA-ICP-MS和PIXE分析,本文探讨了与该矽卡岩矿床有关的斑岩的岩浆起源、斑岩侵位机制及出溶流体特征.结果表明,成矿斑岩为矿区最早的侵入岩单元,具有壳幔源混源特征,其常量元素组成与冈底斯东部斑岩铜矿带的埃达克质岩相近,但稀土和微量元素组成与东部斑岩明显不同,为地幔物质上涌并诱发角闪岩相下地壳熔融的产物,岩体侵位深度大(>7 km)、剥蚀程度高.早期岩浆出溶的流体为高温、高压、高盐度流体,其中富含Fe、Pb、Zn、Cu等成矿金属,与世界其他斑岩铜矿床相比,相对富铁、铅而贫铜.流体的沸腾作用发生于钾硅化阶段,形成了一套富气、高盐、高固相和气液包裹体组合,不同于早期出溶流体的包裹体组合.从岩浆起源和出溶流体性质可以看出,该斑岩具有形成与斑岩有关的铁铅多金属矿床的成矿潜力,但从该矿区地表出露的蚀变和包裹体测压结果可以看出,该斑岩体目前剥蚀深度较大,对斑岩型矿床保存不利,对该斑岩体及与成矿关系的认识对理解该区内的矿床成因和指导区域找矿具有重要的指示意义. 相似文献
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满洲里-新巴尔虎右旗斑岩系列矿床石英流体包裹体液相组分的PIXE分析和地质应用 总被引：1，自引：0，他引：1
ＰＩＸＥ（质子感应Ｘ射线分析）方法是目前国际上新的流体包裹体成分分析方法。在前人工作的基础上,尝试用ＰＩＸＥ方法分析了满洲里－新巴尔虎右旗斑岩系列多金属矿床石英流体包裹体的液相多元素化学组分,其结果反映了地质矿化规律。该方法对于多金属矿床石英流体包裹体成分研究非常有用。结合其他包裹体研究,提出甲乌拉与直干布拉根矿床流体组分和成矿物理化学条件均不同,初步认为不存在同一矿化中心;还提出了查干布拉根矿床西矿段深部可能存在乌奴格吐山式斑岩型Ｃｕ矿床,应引起注意。 相似文献
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K. Slezakova M. C. Pereira M. A. Reis M. C. Alvim-Ferraz 《Journal of Atmospheric Chemistry》2007,58(1):55-68
Epidemiological studies initially considered the impact of total solid particles on human health, but according to the acquired
knowledge about the worse effect of smaller particles, those studies turned to consider the impact of PM10. However, for the last decade PM2.5 began to be more important, once as they are smaller they can penetrate deeper in the lungs, being possible their trapping
in alveoli and worse effects on human health. Therefore, more information on PM2.5 should be provided namely concerning the levels and elemental composition. Considering the relevance of traffic on the emission
of particles of small sizes, this work included the detailed characterization of PM10 and PM2.5, sampled at two sites directly influenced by traffic, as well as at two reference sites, aiming a further evaluation of the
influence of PM10 and PM2.5 on public health. The specific objectives were to study the influence of traffic emission on PM10 and PM2.5 characteristics, considering concentration, size distribution and elemental composition. PM10 and PM2.5 samples were collected using low-volume samplers; the element analyses were performed by particle induced X-ray emission
(PIXE). At the sites influenced by traffic emissions PM10 and PM2.5 concentrations were 7–9 and 6–7 times higher than at the background sites. The presence of 17 elements (Mg, Al, Si, P, S,
Cl, K, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn and Pb) was determined in both PM fractions; particle metal contents were 3–44 and
3–27 times higher for PM10 and PM2.5, respectively, than at the backgrounds sites. The elements originated mostly from anthropogenic activities (S, K, V, Mn,
Ni, Zn and Pb) were predominantly present in PM2.5, while the elements mostly originated from crust (Mg, Al, Si and Ca) predominantly occurred in PM2.5–10. The results also showed that in coastal areas sea salt spray is an important source of particles, influencing PM concentration
and distributions (PM10 increased by 46%, PM2.5/PM10 decreased by 26%), as well as PM compositions (Cl in PM10 was 11 times higher). 相似文献
9.
Monika A. Kusiak Kazuhiro Suzuki Daniel J. Dunkley Janusz Lekki Nonna Bakun-Czubarow Mariusz Paszkowski Bartosz Budzy&#x; 《Gondwana Research》2008,14(4):675
Chemical Th–U–total Pb (CHIME) dating of monazite by electron probe microanalyzer (EPMA) and proton microprobe (PIXE) was carried out on felsic granulites from Stary Gierałtów, Poland, which represent part of the Orlica-Śnieżnik Dome in the NE Bohemian Massif. Analyzed monazite is characterized by mosaic zoning rather than simple core-to-rim growth, and strontium contents of up to 750ppm. An isochron age of 347 ± 13Ma represents timing of amphibolite-facies metamorphism, in agreement with previously published estimates. 相似文献
10.
Fluid inclusions in quartz from miarolitic cavities, pegmatites, and quartz veins in Miocene biotite-granite plutons, Kofu, Japan, were analyzed by particle-induced X-ray emission to examine chemistries and behaviors of granite-derived fluids in island-arc granite. Most inclusions are aqueous two-phase inclusions, and halite-bearing polyphase inclusions are also observed in quartz veins in the upper part of the plutons. From element contents of fluid inclusions in the miarolitic cavities, the original fluid released from the granite plutons during solidification is inferred to have concentrations of Mn, Fe, Cu, Zn, Ge, Br, Rb, Pb, and Ba of several tens to hundreds of parts per million by weight (ppm) and a salinity of about 10 wt% NaCl equivalent. We estimated the formation conditions of the fluid to have been at about 1.3–1.9 kb and 530–600°C on the basis of the homogenization temperatures of the inclusions and the solidification conditions of the plutons. The polyphase inclusions probably originated from hypersaline fluid by boiling of part of the released fluid during its ascent in the plutons. The polyphase inclusions contain several hundreds to tens of thousands of ppm of Fe and Mn, and tens to several hundreds of ppm of Cu, Zn, Br, Rb, and Pb. The salinities are about 35 wt% NaCl equivalent. Compositional variations in two-phase inclusions from the miarolitic cavities and quartz veins are primarily explained by mineral precipitation with dilution by surface water exerting a secondary influence. Thus, chemistries and behaviors of the granite-derived fluids in the plutons can be explained by mineral precipitation, boiling, and dilution of the originally released fluid. 相似文献