Anthropogenic iodine-129 in seawater along a transect from the Norwegian coastal current to the North Pole     

Alfimov V  Aldahan A  Possnert G  Winsor P 《Marine pollution bulletin》2004,49(11-12):1097-1104

Variation in the concentrations of iodine-129 (129I, T1/2=15.7 Myr), a low-level radioactive component of nuclear fuel waste, is documented in surface waters and depth profiles collected during 2001 along a transect from the Norwegian Coastal Current to the North Pole. The surface waters near the Norwegian coast are found to have 20 times higher 129I concentration than the surface waters of the Arctic Ocean. The depth profiles of 129I taken in the Arctic Ocean reveal a sharp decline in the concentration to a depth of about 300-500 m followed by a weaker gradient extending down to the bottom. A twofold increase in the 129I concentration is observed in the upper 1000 m since 1996. Based on known estimates of marine transient time from the release sources (the nuclear reprocessing facilities at La Hague, France, and Sellafield, UK), a doubling in the 129I inventory of the top 1000 m of the Arctic Ocean is expected to occur between the years 2001 and 2006. As 129I of polar mixed layer and Atlantic layer of the Arctic Ocean is ventilated by the East Greenland Current into the Nordic Seas and North Atlantic Ocean, further dispersal and increase of the isotope concentration in these regions will be encountered in the near future.  相似文献   

The Relationships between Effective Porosity,Uniaxial Compressive Strength and Sonic Velocity of Intact Borrowdale Volcanic Group Core Samples from Sellafield     

D.?C.?EntwisleEmail author  P.?R.?N.?Hobbs  L.?D.?Jones  D.?Gunn  M.?G.?Raines 《Geotechnical and Geological Engineering》2005,23(6):793-809

The effective porosity, saturated sonic velocity and saturated uniaxial compressive strength were determined on a large number of Borrowdale Volcanic Group volcaniclastic core samples from three boreholes at Sellafield, Cumbria. The work formed part of the UK Nirex Limited site investigation into whether the Sellafield area could be suitable as a repository for intermediate and low level radioactive waste. Most of the intact samples were of low to very low effective porosity, had a high sonic velocity and were very strong to extremely strong. However, a proportion of values deviated significantly from this. Bivariate analysis showed a negative relationship exists between sonic velocity and effective porosity. The cross plots of these two parameters with uniaxial compressive strength showed a wide range of strength values for samples of low effective porosity and high sonic velocity. Six failure types were identified during the uniaxial compressive strength tests. The strongest samples tended to fail through the matrix and the weakest rock samples tended to fail through haematized material or along haematized veins. Effective porosity and sonic velocity measurements could not distinguish between those samples that failed through the matrix and those that failed along discrete narrow veins. The presence of narrow haematized veins has a major effect on the intact rock strength.  相似文献   

Modelling the biological half-life and seasonality of ¹⁴C in Fucus vesiculosus from the east coast of Ireland: implications for the estimation of future trends     

Keogh SM  Cournane S  León Vintró L  McGee EJ  Mitchell PI 《Marine pollution bulletin》2011,62(4):696-700

Radiocarbon levels were recorded in Fucus vesiculosus samples collected on a monthly basis over a three-year period at a site on the east coast of Ireland. The resulting data was analysed using a numerical model which estimates the transit times from the Sellafield plant to the sampling location, and the mean availability time of ¹⁴C in seaweed. With the inclusion of a model parameter allowing for seasonal variability in uptake by the Fucus, good correlation was observed between the predicted and measured concentrations. Future temporal trends of ¹⁴C Fucus concentrations along the eastern Irish coastline were modelled with the application of three possible prospective discharge scenarios, predicting ¹⁴C Fucus concentrations to reduce to ambient background levels within 2.5-years of discharges being set to zero. Such projections may prove helpful in assessing the consequences of discharge management and policy making in the context of the OSPAR convention.  相似文献   

Modelling temporal trends of 137Cs and 99Tc concentrations in Fucus vesiculosus from the eastern Irish coastline     

Cournane S  Vintró LL  Mitchell PI  McMahon CA  Smith K  Long S 《Marine pollution bulletin》2011,62(11):2337-2344

Time series of ¹³⁷Cs and ⁹⁹Tc activity concentrations in the brown seaweed Fucus vesiculosus and seawater, gathered at three locations on the eastern Irish coastline during the period 1988-2008, have been modelled using a novel approach incorporating a variable uptake rate in the seaweed. Seasonal variations in the time series, identified using spectral analysis, were incorporated into the model which was used to determine transfer kinetic parameters and to predict ¹³⁷Cs and ⁹⁹Tc concentrations in seaweed, as influenced by levels in ambient seawater. An optimisation method combining evolutionary and grid search minimisation techniques was adopted to determine the best values for the model parameters, from which concentration factors (CF) and biological half-lives (tb_1/2) for ¹³⁷Cs and ⁹⁹Tc in F. vesiculosus were calculated. CF values of 170-179 and 1.1 × 105 l kg⁻¹ (dry weight) were obtained for ¹³⁷Cs and ⁹⁹Tc, respectively, while the corresponding tb_1/2 values were 39-47 and 32 days, respectively.  相似文献