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1.
To better understand the mechanisms relating to hydrological regulations of chemical weathering processes and dissolved inorganic carbon (DIC) behaviours, high-frequency sampling campaigns and associated analyses were conducted in the Yu River, South China. Hydrological variability modifies the biogeochemical processes of dissolved solutes, so major ions display different behaviours in response to discharge change. Most ions become diluted with increasing discharge because of the shortened reactive time between rock and water under high-flow conditions. Carbonate weathering is the main source of major ions, which shows strong chemostatic behaviour in response to changes in discharge. Ions from silicate weathering exhibit a significant dilution effect relative to the carbonate-sourced ions. Under high temperatures, the increased soil CO2 influx from the mineralisation of organic material shifts the negative carbon isotope ratios of DIC (δ13CDIC) during the high-flow season. The δ13CDIC values show a higher sensitivity than DIC contents in response to various hydrological conditions. Results from a modified isotope-mixing model (IsoSource) demonstrate that biological carbon is a dominant source of DIC and plays an important role in temporal carbon dynamics. Furthermore, this study provides insights into chemical weathering processes and carbon dynamics, highlighting the significant influence of hydrological variability to aid understanding of the global carbon cycle. 相似文献
2.
Steven R. Beaupr Ellen R.M. Druffel 《Deep Sea Research Part I: Oceanographic Research Papers》2009,56(10):1717-1726
This study extends the 1991-1995 records of marine dissolved organic carbon (DOC) concentrations and Δ14C values at hydrographic Station M (34°50′N, 123°00′W) with new measurements from a frozen (-20 °C) archive of samples collected between April 1998 and October 2004. The magnitudes and synchronicity of major Δ14C anomalies throughout the time-series imply transport of DOC from the surface ocean to depths of at least 450 m on the timescale of months. Keeling plots of all measurements at Station M predict a continuum of possible background DOC compositions containing at least 21 μM of -1000‰ (i.e., ≥57,000 14C years) DOC, but are more consistent with mean deep DOC (38 μM, -549‰; i.e., 6,400 14C years). These results and coral records of surface dissolved inorganic carbon (DIC) Δ14C were used to estimate pre-bomb DOC Δ14C depth profiles. The combined results indicate that bomb-14C has penetrated the DOC pool to depths of ≥450 m, though the signal at that depth is obscured by short-term variability. 相似文献
3.
Dissolved inorganic carbon (DIC) and its carbon isotopic composition in sediment pore waters from the Shenhu area,northern South China Sea 总被引：2，自引：0，他引：2
Tao Yang Shao-Yong Jiang Jing-Hong Yang Ge Lu Neng-You Wu Jian Liu Dao-Hua Chen 《Journal of Oceanography》2008,64(2):303-310
The Shenhu area is one of the most favorable places for the occurrence of gas hydrates in the northern continental slope of
the South China Sea. Pore water samples were collected in two piston cores (SH-A and SH-B) from this area, and the concentrations
of sulfate and dissolved inorganic carbon (DIC) and its carbon isotopic composition were measured. The data revealed large
DIC variations and very negative δ
13C-DIC values. Two reaction zones, 0–3 mbsf and below 3 mbsf, are identified in the sediment system. At site SH-A, the upper
zone (0–3 mbsf) shows relatively constant sulfate and DIC concentrations and δ
13C-DIC values, possibly due to bioturbation and fluid advection. The lower zone (below 3 mbsf) displays good linear gradients
for sulfate and DIC concentrations, and δ
13C-DIC values. At site SH-B, both zones show linear gradients, but the decreasing gradients for δ
13C-DIC and SO4
2− in the lower zone below 3 mbsf are greater than those from the upper zone, 0–3 mbsf. The calculated sulfate-methane interface
(SMI) depths of the two cores are 10.0 m and 11.1 m, respectively. The depth profiles of both DIC and δ
13C-DIC showed similar characteristics as those in other gas hydrate locations in the world oceans, such as the Blake Ridge.
Overall, our results indicate an anaerobic methane oxidation (AMO) process in the sediments with large methane flux from depth
in the studied area, which might be linked to the formation of gas hydrates in this area. 相似文献
4.
Zhang Xuecheng 《中国海洋大学学报(自然科学版)》2000,30(Z1):173-178
碳源对于进行光合作用的各种藻类是必不可少的。螺旋藻的生 态习性是在高pH环境下生长,因此螺旋藻碳代谢的研究有特殊的意义。文中报道了螺旋藻对 无机碳的吸收利用以及与其生长的关系,结果表明螺旋藻培养基中碳酸氢钠的浓度50～100mm ol/dm3时,不仅可以满足螺旋藻生长的需要,而且有助于保持藻体生长的pH值。结果还表 明适当添加碳酸氢氨有利于螺旋藻的生长。 相似文献
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6.
为了解岩溶区控制溪流中溶解无机碳(DIC)和NO_3~-昼夜变化的生物地球化学过程以及DIC和NO_3~-日变化量,于2014-07-22~2014-07-24期间,在广西壮族自治区融安县官村溪流中包括地下河出口(CK)和下游雷崖村(LY)设置两个监测点同时对水体物理化学参数以及C、N同位素(δ~(13) CDIC、δ~(15) N-NO_3~-和δ~(18) O-NO_3~-)展开了为期2d的高分辨率昼夜监测采样工作。结果发现CK点各物理化学参数没有表现出昼夜变化,但是LY点Ca2+、DIC以及PCO2表现出明显的昼夜变化规律,即白天下降夜间上升且与DO和pH表现出明显的负相关关系。相对于CK点,在白天水生光合生物光合作用导致LY点DIC下降的同时δ~(13) CDIC上升,而在夜间呼吸作用导致LY点DIC上升的同时δ~(13) CDIC下降且部分时间段要低于CK点δ~(13) CDIC值。溪流中的NH4+在监测期间基本上都在下降而NO_3~-离子在夜间和上午时间段都在上升,δ~(15) N-NO_3~-却表现出下降的趋势,且比较接近δ~(15) N-NO_3~-初始值,而NO_3~-离子在下午时间段出现下降的趋势。结果表明溪流中DIC昼夜变化主要受到水生植物的光合作用和呼吸作用控制,且通过质量平衡方程计算得知溪流中由于光合作用吸收无机碳而转为有机碳的量为0.94kgC/d,这部分有机碳可以形成相对长期稳定的自然C汇。溪流在夜间和上午时间段发生了N的硝化作用,增长量为2.08kgN/d,但在下午时间段(12:00~18:00)发生了N的同化作用,损失量为0.42kgN/d。溪流输出的NO_3~--N的量为1.66kgN/d,表明在富碳、富钙的岩溶溪流中,有利于水生光合生物的生长,促进N的同化作用的发生,从而减少溪流输出NO_3~--N的量,说明岩溶区溪流N的生物地球化学过程可能在昼夜尺度上改变水质。 相似文献
7.
简要论述了典型热液裂隙充填钨—铋—钼石英脉矿床地质及其以黑钨矿—辉铋矿—辉钼矿为主的矿物组合纵向逆分带现象。重点测量研究了黑钨矿晶体的宏观形态特征和微形貌,及其成因演化机制。以现代光学微分干涉(DIC)显微镜观察测量了黑钨矿端面(102)等的螺旋生长及[010]晶带等的层生长现象。提出黑钨矿晶体的螺—层混合生长概念。 相似文献
8.
硫酸侵蚀碳酸盐岩对长江河水DIC循环的影响 总被引：26，自引：0，他引：26
对长江及其主要支流河水水化学和溶解无机碳（DIC）同位素组成（δ13GDIC）进行了研究。河水阳离子组成以Ca^2＋、Mg^2＋为主,阴离子以HCO3-、SO4^2-为主,水化学组成主要受流域碳酸盐岩矿物的化学侵蚀控制。DIC含量为0．3～2．5mmol／L,从上游到河口逐渐降低。δ13CDIC值为-12．0‰-3．4‰,与DIC含量具有相似的变化趋势。H2CO3溶解碳酸盐岩是控制河水DIC来源及其占δGDIC组成的主要机制。H2SO4溶解碳酸盐岩加剧了流域碳酸盐岩的化学侵蚀,一方面导致了河水的DIC含量增加,另一方面也使河水的δ13GDIC值升高。 相似文献
9.
群锚是常见的基础形式应用较为广泛,由于群锚之间的相互作用,群锚上拔过程中锚周土体的变形破坏机制比较复杂。采用非接触式数字图像相关方法（DIC）对群锚上拔过程开展模型试验研究,分析了群锚上拔过程中上拔力-位移关系曲线特征和锚周土体变形破坏机制。试验结果表明,密实度和埋深对群锚上拔力-位移关系曲线特征具有显著影响,在相同密实度、相同埋深率下浅埋与深埋群锚与同条件下的单锚具有相似的上拔力-位移关系曲线特征;群锚抗拔承载力具有明显的叠加效应,且砂土密实度、埋深和锚间距等参数因素对群锚效应具有显著影响。通过变形场的研究,得出了砂土密实度、埋深以及锚间距对群锚效应的影响规律。 相似文献
10.
为认识水利工程建设对岩溶库区温室气体排放的影响,本文对岩溶区水利工程破坏岩溶水体DIC的稳定性、增加温室气体排放以及水利工程建设所带来的水体富营养化问题进行了初步总结。结果表明,水利工程不仅打破了岩溶水体DIC的自身稳定性,加速水体无机CO2逸出过程,导致CaCO3发生沉淀,而且还通过改变岩溶水动力条件、加速温室气体排放等途径来提高岩溶水体的碳储存、转移、形成与分解过程。与此同时作者还建议:(1)尽快开展岩溶水体温室气体排放的定性分析与定量计算工作,并与不同排放源的温室气体释放效应进行对比;(2)温室气体排放的估算须建立在岩溶碳循环研究基础上,从时间和空间尺度上分析影响岩溶水体温室气体排放过程的关键因素,并把岩溶水体温室气体排放纳入整个岩溶生态系统的生命周期中进行考虑。 相似文献