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Polychlorinated dibenzo-p-dioxins (PCDDs) and polychlorinated dibenzofurans (PCDFs) are persistent organic pollutants (POPs) that are formed and released unintentionally from anthropogenic sources. The high persistence of PCDD/Fs results in the concentrations of these contaminants in environment decreasing only very slowly. Two transport pathways, air and water, carry PCDD/Fs into all regions of the world. Recently, more frequent extreme weather events, such as storms and floods, have been projected to occur as a result of global warming. Extreme weather events have a documented impact on the remobilization and subsequent bioavailability of POPs. In this study, three specific episodes, namely winter monsoon, southeast biomass burning and tropical cyclone (typhoon) events, which influence the environmental fate and transport of PCDD/Fs in Taiwan, were evaluated based on a climate change scenario. During the winter (northeast) monsoon period, the temperature and relative humidity observed in northern Taiwan decreases sharply. During this time, the quantity of PCDD/Fs adsorbed onto suspended particles, as observed at background sites, was found to increase from 300 ± 127 to 630 ± 115 pg I-TEQ g-TSP−1, which is even higher than that measured in Taipei City (438 ± 80 pg I-TEQ g-TSP−1). Hence, the winter monsoon not only brings cold air but also transports air pollutants and dust over long distances from mainland China to Taiwan. During the 2010 Southeast Asia biomass burning events (2010/3/22–3/28), the level of atmospheric PCDD/Fs were measured in central Taiwan (Mt. Lulin) and in the source region of northern Thailand (Chiang Mai); this revealed that the variations in atmospheric PCDD/F concentrations at these two sites followed a similar pattern. On 25 March 2010, the atmospheric PCDD/F concentration increased dramatically from 1.43 to 6.09 fg I-TEQ m−3 at Mt. Lulin and from 7.64 to 12.1 fg I-TEQ m−3 in northern Thailand. However, the atmospheric PCDD/F concentration decreased dramatically 1 day after the biomass burning event. Based on the measurements from a dated sediment core collected at a reservoir in northern Taiwan, the sharp increases in input fluxes of PCDD/Fs and mineral-derived elements levels in 1990 (20 ng I-TEQ m−2 year−1), 2001 (17 ng I-TEQ m−2 year−1), 2004 (16 ng I-TEQ m−2 year−1) and 2005 (15 ng I-TEQ m−2 year−1) seem to be a result of a deep turbid layer formed upstream due to landslides and/or mud flows during the typhoon season. This finding demonstrates the effect of typhoon events on the long-term remobilization of PCDD/Fs as well as supporting the hypothesis that such events would have the potential to remobilize pollutants that have been deposited previously. 相似文献
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Hazardous electric arc furnace dust containing dioxins/furans and heavy metals is blended with harbor sediment, fired at 950–1100 °C to prepare lightweight aggregates. Dust addition can lower the sintering temperature by about 100 °C, as compared to a typical industrial process. After firing at 950 °C and 1050 °C, more than 99.85% of dioxins/furans originally present in the dust have been removed and/or destructed in the mix containing a dust/sediment ratio of 50:100. The heavy metals leached from all fired mixes are far below Taiwan EPA legal limits. The particle density of the lightweight aggregates always decreases with increasing firing temperature. Greater addition of the dust results in a considerably lower particle density (mostly <2.0 g cm−3) fired at 1050 °C and 1100 °C. However, firing at temperatures lower than 1050 °C produces no successful bloating, leading to a denser particle density (>2.0 g cm−3) that is typical of bricks. 相似文献
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Elevated frequencies of abnormal embryos in female eelpout Zoarces viviparus have been demonstrated in Danish, Swedish and German monitoring programmes at certain geographic locations with high levels of anthropogenic input. Pollutants present in areas with high malformation frequencies were selected and tested in a controlled laboratory experiment for their potential to induce abnormalities among eelpout embryos upon injection into pregnant eelpout. Tributyltin, 2,3,7,8-tetrachlorodibenzo-p-dioxin, pyrene, nonylphenol, 2,2′,4,4′-tetrabromophenylether and heptadecafluorooctanesulfonic acid were tested, either individually or combined. Generally, the chemicals were transferred to eggs and/or embryos. Some of the exposures increased the proportion of broods with more than 10% abnormal or 5% malformed embryos, although the average percentages of abnormal development were not affected. Spinal, cranial and eye deformities were evident, similarly to what is seen in nature. Some of the exposures resulted in increased percentages of females with as well a low reproductive capacity as embryos with a low condition index. 相似文献
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