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1.
Root‐related rhodochrosite and concretionary siderite formation in oxygen‐deficient conditions induced by a ground‐water table rise 下载免费PDF全文
Maciej J. Bojanowski Elżbieta Jaroszewicz Adrijan Košir Maciej Łoziński Leszek Marynowski Anna Wysocka Arkadiusz Derkowski 《Sedimentology》2016,63(3):523-551
Sedimentological, mineralogical, stable carbon and oxygen isotope determinations and biomarker analyses were performed on siderite concretions occurring in terrestrial silts to understand their formation and to characterize the sedimentary and diagenetic conditions favouring their growth. High δ13C values (6·4‰ on average) indicate that siderite precipitated in an anoxic environment where bacterial methanogenesis operated. The development of anoxic conditions during shallow burial was induced by a change in sedimentary environment from flood plain to swamp, related to a rise of the ground‐water table. Large amounts of decaying plant debris led to efficient oxygen consumption within the pore‐water in the peat. Oxygen depletion, in combination with a decrease in sedimentation rate, promoted anoxic diagenetic conditions under the swamp and favoured abundant siderite precipitation. This shows how a change in sedimentary conditions can have a profound impact on the early‐diagenetic environment and carbonate authigenesis. The concretions contain numerous rhizoliths; they are cemented with calcium‐rhodochrosite, a feature which has not been reported before. The rhodochrosite cement has negative δ13C values (?16·5‰ on average) and precipitated in suboxic conditions due to microbial degradation of roots coupled to manganese reduction. The exceptional preservation of the epidermis/exodermis and xylem vessels of former root tissues indicates that the rhodochrosite formed shortly after the death of a root in water‐logged sediments. Rhodochrosite precipitated during the initial stages of concretionary growth in suboxic microenvironments within roots, while siderite cementation occurred simultaneously around them in anoxic conditions. These suboxic microenvironments developed because oxygen was transported from the overlying oxygenated soil into sediments saturated with anoxic water via roots acting as permeable conduits. This model explains how separate generations of carbonate cements having different mineralogy and isotopic compositions, which would conventionally be regarded as cements precipitated sequentially in different diagenetic zones during gradual burial, can form simultaneously in shallow burial settings where strong redox gradients exist around vertically oriented permeable root structures. 相似文献
2.
We study the mineralogical changes suffered by specimens of natural miocene red and green continental sandstones (from Pozuelos Formation and Tiomayo Formation) cropping out in the Argentine Puna that increase their bulk magnetic susceptibility and change color when thermally treated. We hypothesize that on heating siderite, which is present in small quantities as cement in the studied sandstones, would oxidize and decompose into maghemite and/or magnetite. Subsequent heating to higher temperatures sometimes would bring about the conversion of maghemite and/or magnetite to hematite. Mössbauer spectroscopy proved to be a very valuable tool for the determination of the presence of siderite in small amounts in the studied samples. The present results show that further work is needed in order to fully understand the mineralogical changes suffered by continental sandstones during heating. The characterization of such changes occurred during laboratory routines is relevant, since they can help to better understand natural processes. 相似文献
3.
A shale split in the well-studied Foord Seam (Upper Carboniferous), Stellarton Basin, Nova Scotia, provides a rare opportunity to study little known siderite concretions with anatomically preserved plants from a limnic basin. Siderite concretions occur throughout the split, commonly as sheet-like, inter-connected lepidodendrid logs, or less frequently as spherical masses; they are typically vuggy. A sample of 14 stratigraphically oriented concretions in the split shows that primary siderite varies from 45% to 80% (wt.%) due to selective replacement by 5% to 40% ferroan dolomite or ankerite in plant tissues. These two minerals show large Mg/Fe and Mg/Ca variability and are Fezoned. Clay content ranges from trace to 20%, and quartz from 5% to 10%. Partial cell-wall destruction by erosion and changeable oxic/anoxic conditions, prior to siderite permineralization, resulted in preservation mainly of the more resistant plant tissues. On average, carbon from siderite is isotopically heavier (+4.8±1.9 0/00) than that from ‘dolomite' (−7.2±1.1 0/00). The distribution of and the positive correlation between δ13C and δ18O probably reflects the two fractionation processes associated with methanogenesis and ‘dolomitization', respectively, in the genetic history of the siderite concretions in the split. Siderite concretions formed diagenetically early from bicarbonate under reducing conditions in a slightly alkaline freshwater environment that precluded calcite deposition. 相似文献
4.
陕西大西沟喷流沉积型菱铁矿矿床地质特征及矿床成因 总被引:1,自引:0,他引:1
陕西大西沟铁矿床位于秦岭造山带山-柞盆地西北部,与银洞子大型银铅矿床毗邻。矿体主要赋存在泥盆系青石垭组中上段,容矿岩石为一套海相复理石碎屑岩和碳酸盐岩建造。矿床的金属矿物主要有菱铁矿、磁铁矿、黄铁矿,其次为黄铜矿、磁黄铁矿等;非金属矿物主要是重晶石、石英、铁白云石,其次为方解石、绢云母、绿泥石、黑云母、斜长石、钠长石、堇青石等,局部地段由于表生氧化和次生富集作用而形成针铁矿、赤铁矿、蓝辉铜矿等。与矿化有关的围岩蚀变较弱,主要有硅化、绢云母化、绿泥石化和碳酸盐化。基于野外地质观察、矿物共生组合和矿石结构构造的系统研究,将大西沟铁矿床的形成划分为3期6阶段,分别是:①喷流沉积期:硅质岩-黄铁矿-菱铁矿阶段(Ⅰ)、重晶石-磁铁矿阶段(Ⅱ);②热液改造期:堇青石-黄铁矿-磁铁矿阶段(Ⅲ)、石英-碳酸盐阶段(Ⅳ)、碳酸盐-硫化物-磁铁矿阶段(Ⅴ);③表生氧化期(Ⅵ)。流体包裹体显微测温结果表明,喷流沉积期Ⅰ阶段菱铁矿完全均一温度和盐度w(NaCl_(eq))峰值区间分别为230~270℃和13%~14.5%,Ⅱ阶段重晶石中流体包裹体的完全均一温度和盐度w(NaCl_(eq))峰值区间分别为220~290℃和9%~13%;热液改造期Ⅳ阶段菱铁矿和石英中气液两相包裹体均一温度峰值区间为240~300℃,盐度w(NaCl_(eq))为2.6%~15.7%;热液改造期Ⅴ阶段菱铁矿与石英中流体包裹体,除大量气液两相包裹体外,还发育有含子矿物多相包裹体,其中,气液两相包裹体均一温度峰值区间为290~340℃,盐度w(NaCl_(eq))为5.1%~13.4%,含子矿物多相包裹体均一温度峰值区间为380~440℃,盐度w(NaCl_(eq))为40.6%~59.7%。含子晶流体包裹体可能是流体不混溶或/和高盐度流体加入的反映。矿区内不同产状碳酸盐矿物的C、O同位素组成比较均一,δ~(13)C_(PDB)值集中在-3.58‰~-1.15‰之间,δ~(18)O_(SMOW)值为21.22‰~21.82‰,均表现出海相碳酸盐或海底喷流热液溶解海相碳酸盐的特征。大西沟矿床的地质、矿化和流体特征与海底热液喷流沉积型矿床一致,可能属于典型的喷流沉积型菱铁矿床,但后期受到秦岭造山作用的影响及热液叠加改造并形成磁铁矿和少量硫化物。大西沟菱铁矿矿床与邻近的银洞子铅锌矿组成一个较完整的喷流沉积成矿系统,两者可能分别代表了喷流沉积的边缘相和中心相。 相似文献
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6.
文章主要介绍太湖地区富铁质棍状结核体的原始直立产状、分布特征、外形特征,内部胶体结构及其矿物学组合特征,进而讨论棍状结核体的成因模式。棍状结核体横向上广泛分布于太湖及其周边地区,产于一层标志性泥质层中;纵向上,棍状结核体在不同高度,从湖底到山边的田地,山麓下的沟槽里都有发现。原始层位可见新鲜棍状结核体,外表颜色为钢灰色,断面灰色。扰动层位的棍状体多为表面磨损的短柱状,表面风化后出现灰褐色或黄褐色。棍状结核体原始产状为直立插于标志性泥质层中,头部向下,尾部向上;头部多为具有发散螺纹的半圆球。棍状结核体可细分为短柱状和长棍状。其中,短柱状直径0.5~1 cm,长度10 cm以内;长棍状直径1~2 cm,长度15~80 cm。太湖地区棍状结核体多含外壳,厚0.1~0.2 cm。棍状结核体表面多具螺旋纹,螺旋纹上多粘有细小球粒结核。棍状结核体内部包裹大量棱角分明、磨圆度差、分选差的石英晶屑,及少量岩屑及粉尘,主要胶结物为微米级自形程度高的菱铁矿晶体。结核内部局部区域包含大量小球粒集合体,小球粒是由菱铁矿微晶加少量晶屑组成。棍状结核体较密实,孔隙度小于20%。棍状结核体的原始直立产状说明其不是下伏硬黄土层的淘洗物,不会老于标志性泥质层的年龄(7 ka B.P.)。两种成因模式可以解释棍状结核体的成因,其一是水底淤泥中的胶体结核沉积生长成因模式;其二是空爆气柱中的合成与回落成因模式,结核体在气柱中合成,自空中落下,插入已有的泥质层或与泥质层一起落下。空爆气柱回落物的假说可以合理解释棍状菱铁矿结核体的产状及分布特征,也可解释其独特的外形和内部特征。 相似文献
7.
DAVID B. LOOPE RICHARD M. KETTLER KARRIE A. WEBER NATHAN L. HINRICHS DEREK T. BURGESS 《Sedimentology》2012,59(6):1769-1781
Iron‐bearing concretions are valuable records of oxidation states of subsurface waters, but the first concretions to form can be altered drastically during later diagenetic events. Distinctive concretions composed of heavy rinds of iron oxide that surround iron‐poor, mud‐rich cores are common along bases of fluvial cross‐bed sets of the Cretaceous Dakota Formation, Nebraska, USA. Concretion rinds thicken inward and cores contain 46 to 89% void space. Millimetre‐scale spherosiderites are abundant in palaeosols that developed in floodplain facies. Evolution of rinded concretions began when intraformational clasts were eroded from sideritic soils, transported, abraded and deposited in river channels. Alteration of siderite and formation of rinds occurred much later, perhaps in the Quaternary when sandstone pore waters became oxic. Dakota concretions are analogous to ‘rattlestones’ in Pleistocene fluvial channels of The Netherlands, and their rinded structure is analogous to that of iron‐rich concretions in the aeolian Navajo Sandstone of Utah. In all three deposits, rinded concretions formed when pre‐existing, siderite‐cemented concretions were oxidized within a sand matrix. Unlike fluvial examples, siderite in the Navajo Sandstone was autochthonous and of late diagenetic origin, having precipitated from carbon dioxide and methane‐enriched waters moving through folded and jointed strata. Iron‐rich rinds formed in all these strata because concretion interiors remained anaerobic, even as oxygen accumulated in the pore waters of their surrounding, permeable matrix. Iron oxide first precipitated at redox boundaries at concretion perimeters and formed an inward‐thickening rind. Acid generated by the oxidation reaction drove siderite dissolution to completion, creating the iron‐poor core. Iron‐oxide rinds are indicators of the former presence of siderite, a mineral that forms only under reducing conditions, during either early or late diagenesis. Siderite is vulnerable to complete oxidation upon exposure, so the distinctive rinded concretions are valuable clues that aid in deciphering diagenetic histories and for recognizing methanic floodplain palaeoenvironments and wet palaeoclimate. 相似文献
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9.
论龙永煤田童子岩组菱铁矿及其岩相意义 总被引:1,自引:0,他引:1
从岩 矿 镜下 鉴定 资 料入 手,分析 了龙 永 煤田 童子 岩 组菱 铁矿 的 形态 特征 和 赋存 状 况。 在 此 基 础上 研 究 了 菱铁矿 的成 因 和岩 相意 义 。 相似文献