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On the scavenging of organic gases by cloud and raindrops: I. A theoretical and experimental study of acetaldehyde absorption and desorption for water drops in air
Authors:J H Topalian  S Mitra  D C Montague  A Quintanar  H R Pruppacher
Institution:(1) Department of Atmospheric Sciences, University of California, 90024 Los Angeles, CA, U.S.A.
Abstract:Our previously developed theoretical models for describing the rate at which water-soluble atmospheric trace gases are scavenged by cloud and rindrops were evaluated for the case of acetaldehyde being absorbed and desorbed by water drops of radii between 250 to 2500 mgrm radius. The experimental verification of our theoretical predictions was carried out in the UCLA 33 m high precipitation shaft in which falling water drops were allowed to come to terminal velocity before passing through a chamber of variable lengths filled with air containing acetaldehyde at various partial pressures. For all drop sizes studied, the experimental results and the theoretical predictions were in reasonable agreement.
Keywords:Acetaldehyde  Air pollution  Pollution removal  Scavenging  Wet deposition
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