Quartz OSL sensitivity from dating data for provenance analysis of pleistocene and holocene fluvial sediments from lowland Amazonia |
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| Institution: | 1. Instituto de Geociências, Universidade Estadual de Campinas, Campinas, SP, Brazil;2. Departamento de Ciências Ambientais, Universidade Federal de São Paulo, Diadema, SP, Brazil;3. Instituto de Geociências, Universidade de São Paulo, São Paulo, SP, Brazil;4. Geological Survey of Israel, Jerusalem, Israel |
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| Abstract: | The properties of the quartz luminescence signal have been shown to be a useful tool for sediment provenance analysis. These provenance studies are based on the sensitivity of the fast optically stimulated luminescence (OSL) component, which is also used for sediment dating. Besides the widespread occurrence of quartz in terrigenous sediments, OSL sensitivity can be acquired using relatively fast and low-cost measurements compared to sediment provenance analysis methods based on accessory minerals or isotopes. Additionally, laboratories worldwide already have an extensive database of recorded quartz OSL signals primarily measured for dating studies, and these data could potentially be repurposed for provenance analysis of Quaternary sedimentary systems through OSL sensitivity calculation. Here, we investigate the use of OSL quartz signals measured in sediment dating surveys for OSL sensitivity calculation and evaluation of changes in sediment sources. The OSL sensitivity was calculated and expressed as %BOSLF, which corresponds to the percentage of the fast OSL component signal (blue stimulation) to the total OSL curve; such approach is advantageous as it does not require any normalisation of the measured signal intensity to dose or aliquot size (weight). Three sets of samples from Amazonian fluvial sediments are investigated: two sets of Holocene floodplain sediments representing different sediment sources to the Amazonian fluvial system, i.e. the Amazon craton and the Andes Mountain belt, and a set of samples from the Içá Formation, a paleo-fluvial system active during the Pleistocene whose provenance is not fully known. Results show that the quartz OSL signal derived from the first test doses (Tn) applied in dating protocols had the best performance for %BOSLF calculation when compared to results from a measurement protocol designed specifically for sediment provenance analysis. There is significant correlation (R2 = 88) between sensitivities derived from Tn and a specific OSL provenance analysis protocol. The proposed approach indicates to be appropriate for sediment provenance analysis since it is able to discriminate signal differences among samples from known sources: Brazilian cratonic quartz yield high sensitivity values (mean %BOSLF >70), in contrast to the relatively lower values from Andean quartz (mean %BOSLF <50). In general, quartz OSL sensitivities from the Içá Formation samples fall into the same range of modern sediments transported by the Içá and Japurá rivers draining the Andean Eastern Cordillera of Colombia and Ecuador. We also observe a decrease in quartz OSL sensitivity during the Holocene, notably after 4 ka, with younger deposits showing lower sensitivity. Sediment provenance variations are discussed in terms of watershed rearrangement and/or precipitation-driven changes during the Late Pleistocene and Holocene across Amazonia. |
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| Keywords: | Quartz luminescence sensitivity OSL signal Deconvolution Içá formation Solimões river Andean sediments Amazon craton sediments |
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