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Radon and radium isotopes as tracers of submarine groundwater discharge – Results from the Ubatuba,Brazil SGD assessment intercomparison
Authors:William C Burnett  Richard Peterson  Willard S Moore  Joselene de Oliveira
Institution:1. Department of Oceanography, Florida State University, Tallahassee, FL 32306, USA;2. Department of Geological Sciences, University of South Carolina, Columbia, SC 20208, USA;3. Departamento de Radiometria Ambiental, Instituto de Pesquisas Energéticas e Nucleares, Travessa R, 400 Cidade Universitária São Paulo, SP CEP 05508-900, Brazil
Abstract:We determined groundwater flow rates shortly after the wet season into an embayment near Ubatuba, Brazil as part of an international intercomparison experiment for submarine groundwater discharge (SGD) assessment techniques. Our estimated rates were determined by the combined use of continuous radon measurements and assessment of radium isotope patterns. The spatial distribution of the short-lived radium isotopes (223Ra and 224Ra) provided the means for independent evaluations of radon losses by mixing and atmospheric evasion. We were thus able to construct a well-constrained mass balance for radon that included a groundwater flux term. Our results showed that the groundwater discharge into this embayment from the fractured crystalline rock aquifer is not steady-state but varies with tidal modulation and rain-induced forcing. Tidally modulated and rain-induced flow rates were comparable during this period. The SGD rates estimated from radon ranged from 1 cm/day to 29 cm/day (cm3/cm2 day) with a mean and standard deviation of 13 ± 6 cm/day. These estimates were mostly similar to a dye-dilution automatic seepage meter (15 ± 19 cm/day) and were within the broad ranges estimated by manual and continuous heat seepage meters but lower than indicated by an artificial tracer test performed nearshore.
Keywords:groundwater  discharge  radon  radium isotopes  Brazil
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