| Characteristics of Elemental Composition of PM_(2.5) in the Spring Period at Tongyu in the Semi-arid Region of Northeast China |
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| 作者姓名： | ZHANG Renjian FU Congbin HAN Zhiwei ZHU Chongshu |
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| 作者单位： | [1]Key Laboratory of Regional Climate-Environment Research for Temperate East Asia, Institute of Atmospheric Physics, Chinese Academy of Sciences, START Regional Center for Temperate East Asia, Beijing 100029 [2]SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi＇an 710075 |
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| 基金项目： | 国家重点基础研究发展计划(973计划)，中国科学院"百人计划"，国家自然科学基金 |
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| 摘 要： | Continuous observations of mass concentration and elemental composition of aerosol particles （PM2.5） were conducted at Tongyu, a semi-arid site in Northeast China in the spring of 2006. The average mass concentration of PM2.5 at Tongyu station was 260.9±274.4 μg m^-3 during the observation period. Nine dust events were monitored with a mean concentration of 528.0±302.7 μgm^-3. The PM2.5 level during non- dust storm （NDS） period was 111.65±63.37 μg m^-3. High mass concentration shows that fine-size particles pollution was very serious in the semi-arid area in Northeast China. The enrichment factor values for crust elements during the dust storm （DS） period are close to those in the NDS period, while the enrichment factor values for pollution elements during the NDS period are much higher than those in the DS period, showing these elements were from anthropogenic sources. The ratios of dust elements to Fe were relative constant during the DS period. The Ca/Fe ratio in dust aerosols at Tongyu is remarkably different from that observed in other source regions and downwind regions. Meteorological analysis shows that dust events at Tongyu are usually associated with dry, low pressure and high wind speed weather conditions. Air mass back-trajectory analysis identified three kinds of general pathways were associated with the aerosol particle transport to Tongyu, and the northwest direction pathway was the main transport route.
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| 关 键 词： | 粉末气溶胶 质量密度 运输路径 检测方法 |
Characteristics of Elemental Composition of PM2.5 in the Spring Period at Tongyu in the Semi-arid Region of Northeast China |
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| ZHANG Renjian,FU Congbin,HAN Zhiwei,ZHU Chongshu.Characteristics of Elemental Composition of PM_(2.5) in the Spring Period at Tongyu in the Semi-arid Region of Northeast China[J].Advances in Atmospheric Sciences,2008,25(6):922-931. |
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| Authors: | ZHANG Renjian FU Congbin HAN Zhiwei and ZHU Chongshu |
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| Institution: | Key Laboratory of Regional Climate-Environment Research for Temperate East Asia, Institute of Atmospheric Physics,
Chinese Academy of Sciences, START Regional Center for Temperate East Asia, Beijing 100029;Key Laboratory of Regional Climate-Environment Research for Temperate East Asia, Institute of Atmospheric Physics,
Chinese Academy of Sciences, START Regional Center for Temperate East Asia, Beijing 100029;Key Laboratory of Regional Climate-Environment Research for Temperate East Asia, Institute of Atmospheric Physics,
Chinese Academy of Sciences, START Regional Center for Temperate East Asia, Beijing 100029;SKLLQG, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710075 |
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| Abstract: | Continuous observations of mass concentration and elemental composition of aerosol particles (PM2.5) were conducted at Tongyu, a semi-arid site in Northeast China in the spring of 2006. The average mass concentration of PM2.5 at Tongyu station was 260.9±274.4 μg m−3 during the observation period. Nine dust events were monitored with a mean concentration of 528.0±302.7 μg m−3. The PM2.5 level during nondust storm (NDS) period was 111.65±63.37 μg m−3. High mass concentration shows that fine-size particles pollution was very serious in the semi-arid area in Northeast China.
The enrichment factor values for crust elements during the dust storm (DS) period are close to those in the NDS period, while
the enrichment factor values for pollution elements during the NDS period are much higher than those in the DS period, showing
these elements were from anthropogenic sources. The ratios of dust elements to Fe were relative constant during the DS period.
The Ca/Fe ratio in dust aerosols at Tongyu is remarkably different from that observed in other source regions and downwind
regions. Meteorological analysis shows that dust events at Tongyu are usually associated with dry, low pressure and high wind
speed weather conditions. Air mass back-trajectory analysis identified three kinds of general pathways were associated with
the aerosol particle transport to Tongyu, and the northwest direction pathway was the main transport route. |
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| Keywords: | dust aerosol mass concentration elemental composition transport pathway |
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