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The distribution of acetaldehyde in the lower troposphere during TROPOZ II
Authors:D W Arlander  D Brüning  U Schmidt  D H Ehhalt
Institution:(1) Institut für Atmosphärische Chemie, Forschungszentrum Jülich GmbH, Postfach 1913, D-52425 Jülich, Germany;(2) Present address: Institutet för Vatten- och Luftvardforskning, P.O. Box 47086, S-40258 Göteborg, Sweden;(3) Present address: Institut für Meteorologie und Geophysik, Johann Wolfgang Goethe-Universität, Postfach 11 19 32, 60054 Frankfurt, Germany
Abstract:A series of 72 measurements of the acetaldehyde (CH3CHO) mixing ratio were made in the lower troposphere during TROPOZ II. These measurements are the first ever made of the background level of this trace gas in the free troposphere. The data show a vertical decrease of the CH3CHO mixing ratio with increasing altitude and indicate higher CH3CHO concentrations in the Northern Hemisphere — in general agreement with a model-derived average CH3CHO distribution. Deviations of the observed CH3CHO mixing ratios from the modelled mean distribution are correlated with similar deviations in the corresponding HCHO mixing ratios.
Keywords:acetaldehyde  background troposphere  concentration distribution  aircraft  sampling technique
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