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春秋季南黄海二甲基硫(DMS)与二甲巯基丙酸(DMSP)的浓度分布研究
引用本文:杨剑,杨桂朋,张洪海,张生辉.春秋季南黄海二甲基硫(DMS)与二甲巯基丙酸(DMSP)的浓度分布研究[J].海洋学报(英文版),2016,35(2):76-87.
作者姓名:杨剑  杨桂朋  张洪海  张生辉
作者单位:中国海洋大学 化学化工学院, 海洋化学理论与工程技术教育部重点实验室, 山东 青岛, 266100;中国科学院 烟台海岸带研究所, 山东省海岸带环境工程技术研究中心, 山东 烟台, 264003,中国海洋大学 化学化工学院, 海洋化学理论与工程技术教育部重点实验室, 山东 青岛, 266100,中国海洋大学 化学化工学院, 海洋化学理论与工程技术教育部重点实验室, 山东 青岛, 266100,中国海洋大学 化学化工学院, 海洋化学理论与工程技术教育部重点实验室, 山东 青岛, 266100
摘    要:Temporal distributions of dimethylsulfide(DMS) and dimethylsulfoniopropionate(DMSP) were studied in the southern Yellow Sea(SYS) during April and September 2010. The mean concentrations(range) of DMS, dissolved and particulate DMSP(DMSPd and DMSPp) in the surface waters in spring are 1.69(0.48–4.92), 3.18(0.68–6.75)and 15.81(2.82–52.33) nmol/L, respectively, and those in autumn are 2.80(1.33–5.10), 5.45(2.19–11.30) and 30.63(6.24–137.87) nmol/L. On the whole, the distributions of DMS and DMSP in spring are completely different from those in autumn. In the central part of the SYS, the concentrations of DMS and DMSP in spring are obviously higher than those in autumn, but the opposite situation is found on the south of 34°N, which can be attributed to the differences in nutrients and phytoplankton biomass and composition between spring and autumn. Besides,the seasonal variations of water column stability and the Changjiang diluted water also have significant impact on the distributions of DMS and DMSP in spring and autumn on the south of 34°N. DMS and DMSPp concentrations coincide well with chlorophyll a(Chl a) levels in the spring cruise, suggesting that phytoplankton biomass may play an important role in controlling the distributions of DMS and DMSPp in the study area. Annual DMS emission rates range from 0.015 to 0.033 Tg/a(calculated by S), respectively, using the equations of Liss and Merlivat(1986) and Wanninkhof(1992). This result implies a significant relative contribution of the SYS to the global oceanic DMS fluxes.

关 键 词:二甲基硫  二甲巯基丙酸  叶绿素a  海-气通量  南黄海
收稿时间:2014/7/30 0:00:00
修稿时间:2015/2/26 0:00:00

Temporal variations of dimethylsulfide and dimethylsulfoniopropionate in the southern Yellow Sea in spring and autumn
YANG Jian,YANG Guipeng,ZHANG Honghai and ZHANG Shenghui.Temporal variations of dimethylsulfide and dimethylsulfoniopropionate in the southern Yellow Sea in spring and autumn[J].Acta Oceanologica Sinica,2016,35(2):76-87.
Authors:YANG Jian  YANG Guipeng  ZHANG Honghai and ZHANG Shenghui
Institution:Key Laboratory of Ministry of Education for Marine Chemistry Theory and Technology, College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China;Coastal Environment Engineering Technology Research Center of Shandong Province, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences, Yantai 264003, China,Key Laboratory of Ministry of Education for Marine Chemistry Theory and Technology, College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China,Key Laboratory of Ministry of Education for Marine Chemistry Theory and Technology, College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China and Key Laboratory of Ministry of Education for Marine Chemistry Theory and Technology, College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China
Abstract:Temporal distributions of dimethylsul.de (DMS) and dimethylsulfoniopropionate (DMSP) were studied in the southern Yellow Sea (SYS) during April and September 2010. The mean concentrations (range) of DMS, dissolved and particulate DMSP (DMSPd and DMSPp) in the surface waters in spring are 1.69 (0.48-4.92), 3.18 (0.68-6.75) and 15.81 (2.82-52.33) nmol/L, respectively, and those in autumn are 2.80 (1.33-5.10), 5.45 (2.19-11.30) and 30.63 (6.24-137.87) nmol/L. On the whole, the distributions of DMS and DMSP in spring are completely different from those in autumn. In the central part of the SYS, the concentrations of DMS and DMSP in spring are obviously higher than those in autumn, but the opposite situation is found on the south of 34°N, which can be attributed to the differences in nutrients and phytoplankton biomass and composition between spring and autumn. Besides, the seasonal variations of water column stability and the Changjiang diluted water also have significant impact on the distributions of DMS and DMSP in spring and autumn on the south of 34°N. DMS and DMSPp concentrations coincide well with chlorophyll a (Chl a) levels in the spring cruise, suggesting that phytoplankton biomass may play an important role in controlling the distributions of DMS and DMSPp in the study area. Annual DMS emission rates range from 0.015 to 0.033 Tg/a (calculated by S), respectively, using the equations of Liss and Merlivat (1986) and Wanninkhof (1992). This result implies a signi.cant relative contribution of the SYS to the global oceanic DMS fluxes.
Keywords:dimethylsulfide  dimethylsulfoniopropionate  chlorophyll a  sea-to-air flux  the southern Yellow Sea
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