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南大西洋沉积物中多环芳香化合物的组成特征研究
引用本文:黄鑫,曾志刚,陈帅,殷学博,王晓媛,马瑶,杨宝菊,荣坤波,舒云超,姜涛.南大西洋沉积物中多环芳香化合物的组成特征研究[J].海洋学报(英文版),2014,33(11):150-154.
作者姓名:黄鑫  曾志刚  陈帅  殷学博  王晓媛  马瑶  杨宝菊  荣坤波  舒云超  姜涛
作者单位:中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院大学, 北京 100049;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院大学, 北京 100049;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院大学, 北京 100049;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院大学, 北京 100049;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院大学, 北京 100049;中国科学院海洋研究所海洋地质与环境重点实验室, 青岛 266071;中国科学院大学, 北京 100049
基金项目:The National Key Basic Research Program of China under contract No.2013CB429700; the National Special Fund for the 12th Five Year Plan of COMRA under contract Nos DY125-12-R-02,DY125-12-R-05 and DY125-11-R-05; the National Natural Science Foundation of China under contract Nos 41325021,40830849 and 40976027; the Strategic Priority Research Program of the Chinese Academy of Sciences under contract No.XDA11030302; the Shandong Province Natural Science Foundation of China for Distinguished Young Scholars under contract No.JQ200913 Acknowledgements The authors would like to thank the crews of the COMRA cruise (DYl15-22 and DYl15-26) for their help with sampling operations, and thank Meng Qianxiang for his help with sampling analysis.
摘    要:10 samples of sediments obtained from the South Mid-Atlantic Ridge were measured for the abundances and distributions of polycyclic aromatic compounds(PAHs). The total concentrations of PAHs(∑PAHs) ranged from 2.768 to 9.826 μg/g dry sediment. The ∑PAHs was higher in sample 22V-TVG10 and sample 26V-TVG05 which were close to hydrothermal fields, with the lowest value in sample 22V-TVG14 which was farthest from hydrothermal fields, suggesting a probable hydrothermal origin of ∑PAHs of samples. Approximately nine kinds of PAHs were identified, and low molecular mass tricyclic and tetracyclic aromatic compounds were predominant in the samples. The concentrations of fluoranthene which were typical as hydrothermal alteration compounds were the highest among PAHs with dry weight between 0.913–3.157 μg/g. The phenanthrene homologue was most abundant in the samples, and the ratios between parent phenanthrene and methylphenanthrene which probably reflected the degree of hydrothermal alteration ranged from 0.097 to 1.602. The sample 22V-TVG10 possessing a maximum ratio value showed the intense influence of the hydrothermal alteration on this sample, which might further imply that PAHs in sediments were mainly derived from the hydrothermal alteration.

关 键 词:多环芳烃化合物  大西洋中脊  沉积物  芳香族化合物  热液蚀变  特性  成分  甲基菲
收稿时间:2013/1/12 0:00:00
修稿时间:2014/3/28 0:00:00

Component characteristics of polycyclic aromatic compounds in sediments of the South Mid-Atlantic Ridge
HUANG Xin,ZENG Zhigang,CHEN Shuai,YIN Xuebo,WANG Xiaoyuan,MA Yao,YANG Baoju,RONG Kunbo,SHU Yunchao and JIANG Tao.Component characteristics of polycyclic aromatic compounds in sediments of the South Mid-Atlantic Ridge[J].Acta Oceanologica Sinica,2014,33(11):150-154.
Authors:HUANG Xin  ZENG Zhigang  CHEN Shuai  YIN Xuebo  WANG Xiaoyuan  MA Yao  YANG Baoju  RONG Kunbo  SHU Yunchao and JIANG Tao
Institution:1.Key Laboratory of Marine Geology and Environment, Institute of Oceanology, Chinese Academy of Sciences, Qingdao 266071, China;University of Chinese Academy of Sciences, Beijing 100049, China2.Key Laboratory of Marine Geology and Environment, Institute of Oceanology, Chinese Academy of Sciences, Qingdao 266071, China
Abstract:10 samples of sediments obtained from the South Mid-Atlantic Ridge were measured for the abundances and distributions of polycyclic aromatic compounds (PAHs). The total concentrations of PAHs (∑PAHs) ranged from 2.768 to 9.826 μg/g dry sediment. The ∑PAHs was higher in sample 22V-TVG10 and sample 26V-TVG05 which were close to hydrothermal fields, with the lowest value in sample 22V-TVG14 which was farthest from hydrothermal fields, suggesting a probable hydrothermal origin of ∑PAHs of samples. Approximately nine kinds of PAHs were identified, and low molecular mass tricyclic and tetracyclic aromatic compounds were predominant in the samples. The concentrations of fluoranthene which were typical as hydrothermal alteration compounds were the highest among PAHs with dry weight between 0.913-3.157 μg/g. The phenanthrene homologue was most abundant in the samples, and the ratios between parent phenanthrene and methylphenanthrene which probably reflected the degree of hydrothermal alteration ranged from 0.097 to 1.602. The sample 22V-TVG10 possessing a maximum ratio value showed the intense influence of the hydrothermal alteration on this sample, which might further imply that PAHs in sediments were mainly derived from the hydrothermal alteration.
Keywords:South Mid-Atlantic Ridge  sediment  polycyclic aromatic compounds  hydrothermal activity
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