首页 | 本学科首页   官方微博 | 高级检索  
相似文献
 共查询到20条相似文献，搜索用时 31 毫秒
1.
Abstract— The isotopic compositions of Sm and Gd in seven lunar samples from the Apollo 15 deep drill core were determined to discuss the effects of neutron capture near the lunar surface. Large isotopic deviations of 150Sm/149Sm, 156Gd/155Gd, and 158Gd/157Gd derived from neutron capture effects were observed in all samples. Although neutron capture products in lunar samples were investigated extensively in the 1970s, our precise isotopic measurements resulted in several new findings. The neutron fluence in the Apollo 15 drill core is a function of depth with a symmetric peak at 190 g/cm2 depth from the surface, confirming the results of earlier investigations. Neutron fluence values calculated from the isotopic shifts by comparison to artificially irradiated standard reagents were (5.16–7.49) × 1016 n/cm2. These values are 1.3 to 1.4x larger than those previously reported. Variations of εSm/εGd with depth are interpreted as being due to variations in the neutron energy spectrum. Here εSm and εGd are defined as in previous studies of lunar neutron stratigraphy. Our data suggest that the neutron is more thermalized at the lower layers than it is at the upper layers. In addition to large isotopic shifts for 149Sm, 150Sm, 155Gd, 156Gd, 157Gd, and 158Gd, isotopic enrichments of 152Gd and 154Gd derived from neutron capture for 151Eu and 153Eu, respectively, were also observed in all samples.  相似文献   

2.
Abstract– The isotopic compositions of Sm and/or Gd of nine documented drill core samples of the Jilin H5 chondrite were determined to study the neutron capture records of individual meteorite samples. All the samples showed significant isotopic shifts of 150Sm/149Sm and/or 158Gd/157Gd corresponding to neutron fluences of (1.3–1.7) × 1015 n cm?2. Considering the short 4π irradiation age of 0.32 Ma during the second stage, the 2π irradiation of 7 Ma during the first stage is the main influence on the Sm and Gd isotopic shifts of the Jilin chondrite. Although a depth dependence of the neutron capture effects was expected from the isotopic variations of 150Sm/149Sm and 158Gd/157Gd in the Jilin chondrite core samples that were possibly drilled perpendicular to the surface of the large object with a radius of >10 m in the 2π‐geometry, no clear evidence was observed in this study. The data from the combination of the isotopic shifts between Sm and Gd defined as εSm/εGd suggest that the neutrons produced in the 2π‐geometry of the Jilin chondrite follow the similar energy spectra as the neutrons in lunar samples, although the present analytical quality is not enough to discuss a critical discussion for the thermalization of the neutron energy levels.  相似文献   

3.
  相似文献   

4.
Neutron capture effects in meteorites and lunar surface samples have been successfully used in the past to study exposure histories and shielding conditions. In recent years, however, it turned out that neutron capture effects produce a nuisance for some of the short‐lived radionuclide systems. The most prominent example is the 182Hf‐182W system in iron meteorites, for which neutron capture effects lower the 182W/184W ratio, thereby producing too old apparent ages. Here, we present a thorough study of neutron capture effects in iron meteorites, ordinary chondrites, and carbonaceous chondrites, whereas the focus is on iron meteorites. We study in detail the effects responsible for neutron production, neutron transport, and neutron slowing down and find that neutron capture in all studied meteorite types is not, as usually expected, exclusively via thermal neutrons. In contrast, most of the neutron capture in iron meteorites is in the epithermal energy range and there is a significant contribution from epithermal neutron capture even in stony meteorites. Using sophisticated particle spectra and evaluated cross section data files for neutron capture reactions we calculate the neutron capture effects for Sm, Gd, Cd, Pd, Pt, and Os isotopes, which all can serve as neutron‐dose proxies, either in stony or in iron meteorites. In addition, we model neutron capture effects in W and Ag isotopes. For W isotopes, the GCR‐induced shifts perfectly correlate with Os and Pt isotope shifts, which therefore can be used as neutron‐dose proxies and permit a reliable correction. We also found that GCR‐induced effects for the 107Pd‐107Ag system can be significant and need to be corrected, a result that is in contrast to earlier studies.  相似文献   

5.
Abstract— A purely physical model based on a Monte Carlo simulation of galactic cosmic ray (GCR) particle interaction with meteoroids is used to investigate neutron interactions down to thermal energies. Experimental and/or evaluated excitation functions are used to calculate neutron capture production rates as a function of the size of the meteoroid and the depth below its surface. Presented are the depth profiles of cosmogenic radionuclides 36Cl, 41Ca, 60Co, 59Ni, and 129I for meteoroid radii from 10 cm up to 500 cm and a 2π irradiation. Effects of bulk chemical composition on n‐capture processes are studied and discussed for various chondritic and lunar compositions. The mean GCR particle flux over the last 300 ka was determined from the comparison of simulations with measured 41Ca activities in the Apollo 15 drill core. The determined value significantly differs from that obtained using equivalent models of spallation residue production.  相似文献   

6.
R-process yields for a helium layer have been calculated within a network of 6033 heavy nuclei using a steady flow approximation. The calculation of the neutron capture cross sections has been improved. The beta decay rates computed by Klapdor and his colleagues have been used in the calculation. We find that ther-process yield peaks near mass numbers 80 and 130 require a neutron number density of approximately 1020 cm?3 and a freezing time comparable to or less than 0.1 s. The peak near mass number 195 requires a neutron number density of about 1021 cm?3 and a freezing time comparable to or less than about 0.01 s. The individual yield features of the steady flowr-process depend entirely upon the neutron capture cross sections of the nuclei along the flow path and the beta decay rates, which can shift the flow path and thereby introduce inappropriate capture cross sections into the determination of the yields.  相似文献   

7.
A physical model based on the open‐source toolkit Geant4 for production rates of cosmogenic nuclei on the lunar surface is proposed and calibrated. The fluxes of proton and neutron beneath the lunar surface are obtained by simulating the physical processes between the cosmic‐ray particles and the lunar surface material. By combining the experimental proton cross sections and the a posteriori neutron cross sections, we calculate the production rate depth profiles of long‐lived nuclei (10Be, 14C, 26Al, 36Cl, and 53Mn). Through comparing experimental and theoretical data for these nuclei, we find that for all the selected nuclei, experimental and theoretical production rate depth profiles agree well with each other by introducing a single normalization factor. It means that the physical model based on Geant4 can also reproduce the depth profiles of cosmogenic nuclei, and that this model can be used by everyone worldwide. In addition, we predict the production rates of three stable nuclei (21Ne, 22Ne, and 38Ar).  相似文献   

8.
Preliminary depth relationships are presented for the Apollo 15, 16 and 17 drill core samples. For a given depth in any of these drill stems, thein situ lunar surface depth can be estimated. Ranges of uncertainty are also established, based on percent core recovery and degree of sample disturbance. The most likely explanation for the sample disturbance observed in the top three sections of the Apollo 16 drill stem is sample migration after the stem was capped on the lunar surface; essentially no sample was lost. Similar disturbance occurred in the Apollo 17 drill core, although to a lesser degree. The average original bulk densities (i.e., before any disturbance occurred) of the Apollo 15, 16 and 17 drill cores are 1.76, 1.59, and 1.87 g cm?3, respectively. The Apollo 15 and 17 values are probably close to thein situ values; but the Apollo 16 averagein situ density could be as much as 13% less than the already low density in the drill core.  相似文献   

9.
Abstract— The regolith evolution of the lunar meteorites Dhofar (Dho) 081, Northwest Africa (NWA) 032, NWA 482, NWA 773, Sayh al Uhaymir (SaU) 169, and Yamato (Y‐) 981031 was investigated by measuring the light noble gases He, Ne, and Ar. The presence of trapped solar neon in Dho 081, NWA 773, and Y‐981031 indicates an exposure at the lunar surface. A neon three‐isotope diagram for lunar meteorites yields an average solar 20Ne/22Ne ratio of 12.48 ± 0.07 representing a mixture of solar energetic particles neon at a ratio of 11.2 and solar wind neon at a ratio of 13.8. Based on the production rate ratio of 21Ne and 38Ar, the shielding depth in the lunar regolith of NWA 032, NWA 482, SaU 169, and Y‐981031 was obtained. The shielding depth of these samples was between 10.5 g/cm2 and >500 g/cm2. Based on spallogenic Kr and Xe, the shielding depth of Dho 081 was estimated to be most likely between 120 and 180 g/cm2. Assuming a mean density of the lunar regolith of 1.8 g/cm3, 10.5 g/cm2 corresponds to a depth of 5.8 cm and 500 g/cm2 to 280 cm below the lunar surface. The range of regolith residence time observed in this study is 100 Ma up to 2070 Ma.  相似文献   

10.
The constraints on the properties of neutron star matter from the mass of neutron star PSR J1614-2230 are examined in the framework of the relativistic mean field theory. We find that there are little differences between the σ potentials of large mass neutron star and those of canonnical mass neutron star. For potentials of ω, ρ, neutrons and electrons, the values corresponding to the large mass neutron star are larger than those to the canonnical mass neutron star as the baryon number density is more than a certain value. We also find that for the relative particle number density of electrons, muons, neutrons and protons and the pressure of the neutron star, the values corresponding to the large mass neutron star are far larger than those to the canonnical mass neutron star. For the relative particle number density of hyperons Λ, Σ?, Σ0, Σ+ and Ξ?, the values corresponding to the large mass neutron star are far smaller than those to the canonnical mass neutron star. These mean that the larger mass of neutron star is more advantageous to the production of protons but is not advantageous to the production of hyperons.  相似文献   

11.
Physical and mechanical properties of the lunar soil (a review)   总被引：1，自引：0，他引：1  
We review the data on the physical and mechanical properties of the lunar soil that were acquired in the direct investigations on the lunar surface carried out in the manned and automatic missions and in the laboratory examination of the lunar samples returned to the Earth. In justice to the American manned program Apollo, we show that a large volume of the data on the properties of the lunar soil was also obtained in the Soviet automatic program Lunokhod and with the automatic space stations Luna-16, -20, and -24 that returned the lunar soil samples to the Earth. We consider all of the main physical and mechanical properties of the lunar soil, such as the granulometric composition, density and porosity, cohesion and adhesion, angle of internal friction, shear strength of loose soil, deformation characteristics (the deformation modulus and Poisson ratio), compressibility, and the bearing capacity, and show the change of some properties versus the depth. In most cases, the analytical dependence of the main parameters is presented, which is required in developing reliable engineering models of the lunar soil. The main physical and mechanical properties are listed in the summarizing table, and the currently available models and simulants of the lunar soil are reviewed.  相似文献   

12.
The rapid neutron capture process (r-process) is one of the major nucleosynthesis processes responsible for the synthesis of heavy nuclei beyond iron. Isotopes beyond Fe are most exclusively formed in neutron capture processes and more heavier ones are produced by the r-process. Approximately half of the heavy elements with mass number A > 70 and all of the actinides in the solar system are believed to have been produced in the r-process. We have studied the r-process in supernovae for the production of heavy elements beyond A = 40 with the newest mass values available. The supernova envelopes at a temperature >109 K and neutron density of 1024 cm?3 are considered to be one of the most potential sites for the r-process. The primary goal of the r-process calculations is to fit the global abundance curve for solar system r-process isotopes by varying time dependent parameters such as temperature and neutron density. This method aims at comparing the calculated abundances of the stable isotopes with observation. We have studied the r-process path corresponding to temperatures ranging from 1.0 × 109 K to 3.0 × 109 K and neutron density ranging from 1020 cm?3 to 1030 cm?3. With temperature and density conditions of 3.0 × 109 K and 1020 cm?3 a nucleus of mass 273 was theoretically found corresponding to atomic number 115. The elements obtained along the r-process path are compared with the observed data at all the above temperature and density range.  相似文献   

13.
Abstract— Proton‐induced production cross sections of 129I from Te and Ba are presented. Earlier assumptions that Te is the most important target element in meteoroids are confirmed. Based on this data set and the experimental production rates of 129I from thick‐target experiments, the production of 129I in stony meteoroids is modeled using a GCR flux density of 4.06 cm?2 s?1. The results of this modeling must be considered preliminary because the contribution from neutron capture on 128Te needs further investigation. We obtained modeled production rates that agree with experimental results for samples from two medium‐sized meteorites (Abee and Knyahinya). However, we find that this model does not describe 41Ca in lunar rocks well and seems to overestimate 129I production in larger bodies, such as Allende. We present elemental production rates from Te and Ba based on our modeling as well as for a model that describes neutron capture products. For 129I analysis of Knyahinya, a novel method to separate Te and analysis using ICP‐MS was used, enabling the use of experimental elemental concentrations obtained from the same meteorite to calculate 129I production.  相似文献   

14.
Abstract— We derived the cosmic‐ray and solar particle exposure history for the two lunar meteorites Elephant Moraine (EET) 96008 and Dar al Gani (DaG) 262 on the basis of the noble gas isotopic abundances including the radionuclide 81Kr. For EET 96008, we propose a model for the exposure to cosmic rays and solar particles in three stages on the Moon: an early stage ～500 Ma ago, lasting less than 9 Ma at a shallow shielding depth of 20 g/cm2, followed by a stage when the material was buried, without exposure, until it was exposed in a recent stage. This recent stage, at a shielding depth in a range of 200–600 g/cm2, lasted for ～26 Ma until ejection. This model is essentially the same as that previously found for lunar meteorite EET 87521; thus, pairing of the two Elephant Moraine lunar meteorites that were recovered on the same icefield in Antarctica is confirmed by our data. The cosmic‐ray‐produced isotopes, the trapped solar and lunar atmospheric noble gases, as well as the radionuclide 81Kr observed for the DaG 262 lunar meteorite are consistent with a one‐stage lunar exposure history. The average burial depth of the Dar al Gani material before ejection was within a range of 50–80 g/cm2. The exposure to cosmic rays at this depth lasted 500–1000 Ma. This long residence time for Dar al Gani at relatively shallow depth explains the high concentrations of implanted solar noble gases.  相似文献   

15.
Sample 14307,30, a gas-rich breccia (Group 1 of Warner, 1972) has been studied by coupling track method and light noble gas isotopic analysis. The breccia is made of a glassy dark matrix with embedded millimeter to sub-millimeter sized angular ligth xenoliths. These ones are breccia fragments of higher grade metamorphic facies (Group ? 2). A lighter strata (～ 0.5 cm thick) intersects the dark matrix. Noble gas analysis have shown the dark matrix (36Ar = 5.4 × 10?4 cc STP/g) to be enriched in solar type gases with respect to the light fractions (36Ar ? 2.2 × 10?4 cc STP/g). Themean value of the bulk ‘exposure age’ for different samplings is 180 ± 20 × 106 yr, as calculated from spallogenic3He,21Ne and126Xe contents, using our data and those of Bogard and Nyquist (1972). After appropriate correction for radiogenic40Ar, the ratio40Arexc/36Artr is about 5. A total of 390 crystals coming from 11 locations either in the dark matrix, the lighter strata or a light xenolith (0.25 cm diam), have been studied by track analysis using optical and scanning electron microscopy. 181 crystals were thoroughly investigated by means of the latter technique. The following results were obtained:
  1. 72 crystals (70-300µm diam) from one location (No. 12) in the matrix show aminimum track density distribution spreading over 3 orders of magnitude (from 2 × 106 up to 2 × 109 cm?2). The spectrum has at its lower edge a well defined peak (～ 50% of total crystal number) around 3 × 106 cm?2). Grains with track density variations over a factor of 3 have a low abundance as compared to average lunar soils. Moreover the mineralogy of this location is peculiar due to its large abundance in orthopyroxenes. Considering the lower edge of the track density distribution amaximum surface residence time of 5 × 106 yr can be set for rock 14307 in itspresent shape;
  2. 11 feldspars (1-15µm diam) and 22 clinopyroxenes (70-130µm) have been studied in the light xenolith. All crystals have minimum track densities larger than 108 cm?2. No spatial variation of track-densities (2.5 ± 0.5 × 109 cm?2) were found in feldspars inside a millimeter-sized polished section. Clearly these tracks were not acquired by an irradiation of the xenolith as an individual entity, but survived its own formation as a breccia of Group 2. Therefore, solar energetic iron particle tracks have not been erased despite a complex mechanical and thermal history involved by two subsequent brecciation processes;
  3. in the 10 other locations, crystals (70-200µm diam) either from the dark matrix or the lighter strata show a significant departure from the pattern observed in lunar soils; namely:
  1. the minimum track density distribution is strongly peaked at high values (～ 1-4 × 109 cm?2) for ～ 95% of the crystals, the remaining ～ 5% having low-values (0.2-1 × 107 cm?2);
  2. the abundance (2%) of crystals with track density variation over a factor of 3 is about one order of magnitude less than in average lunar soils;
  3. the magnitude of track density gradients within single crystals is small. In fact, thelargest track density variation versus depth found can be described by the relation? α D?0.5, in contrast with soil grains which generally exhibit a variation of the form? α D?1.1±0.4.
The above observations imply that the peculiar irradiation characteristics of these fossilized soils are more likely to be attributed to some wide scale process rather than to some accidental or local phenomena. Attempts to account for these findings by present solar VH particle flux and energy distribution (as determined by Crozaz and Walker, 1971; Fleischeret al., 1971b; Priceet al., 1971), current estimates of lunar fine scale erosion, accumulation and turn-over rates, have proven essentially negative. The bulk ‘exposure age’ of the breccia, rather low by lunar soil standards, makes things even worse. For lack of any better explanation, the above observations could be more easily understood by postulating a higher flux (by factors from ～ 10 up to 200) and a harder energy spectrum (at least for particles with rigidity less than 0.3 GV) for the solar cosmic rays at the time the constituents of the breccia were part as loose grains of the lunar regolith.  相似文献   

16.
The neutron capture cross-sections of124, 132, 134Xe have been measured by the activation technique at 25 keV neutron energy. These data were supplemented by calculated capture cross-sections for128, 129, 130, 131Xe via the statistical model. The complete set of capture cross-sections obtained in this way served to determine the solar xenon abundance throughs-process systematics and to study a variety of isotopic anomalies.  相似文献   

17.
Bearing load vs penetration curves have been measured on a 1.3 g sample of lunar soil from the scoop of the Surveyor 3 soil mechanics surface sampler, using a circular indentor 2 mm in diameter. Measurements were made in an Earth laboratory, in air. This sample provided a unique opportunity to evaluate earlier, remotely controlled, in-situ measurements of lunar surface bearing properties. Bearing capacity, measured at a penetration equal to the indentor diameter, varied from 0.02–0.04 N cm–2 at bulk densities of 1.15 g cm–3 to 30-100 N cm–2 at 1.9 g cm–3. Deformation was by compression directly below the indentor at bulk densities below 1.61 g cm–3, by outward displacement at bulk densities over 1.62 g cm–3. Preliminary comparison of in-situ remote measurements with those on returned material indicates good agreement if the lunar regolith at Surveyor 3 has a bulk density of 1.6 g cm–3 at 2.5 cm. depth; definitive comparison awaits both better data on bulk density of the undisturbed lunar soil and additional mechanical-property measurements on returned material.  相似文献   

18.
MESSENGER Neutron Spectrometer (NS) observations of cosmic-ray-generated thermal neutrons provide the first direct measurements of Mercury’s surface elemental composition. Specifically, we show that Mercury’s surface is enriched in neutron-absorbing elements and has a measured macroscopic neutron-absorption cross section of 45-81 × 10−4 cm2/g, a range similar to the neutron absorption of lunar basalts from Mare Crisium. The expected neutron-absorbing elements are Fe and Ti, with possible trace amounts of Gd and Sm. Fe and Ti, in particular, are important for understanding Mercury’s formation and how its surface may have changed over time through magmatic processes. With neutron Doppler filtering - a neutron energy separation technique based on spacecraft velocity - we demonstrate that Mercury’s surface composition cannot be matched by prior models, which have characteristically low abundances of Fe, Ti, Gd, and Sm. While neutron spectroscopy alone cannot separate the relative contributions of individual neutron-absorbing elements, these results provide strong new constraints on the nature of Mercury’s surface materials. For example, if all the measured neutron absorption were due to the presence of an Fe-Ti oxide and that oxide were ilmenite, then Mercury’s surface would have an ilmenite content of 7-18 wt.%. This result is in general agreement with the inference from color imaging and visible-near-infrared spectroscopy that Mercury’s overall low reflectance is consistent with a surface composition that is enriched in Fe-Ti oxides. The incorporation of substantial Fe and Ti in oxides would imply that the oxygen fugacity of basalts on Mercury is at the upper range of oxygen fugacities inferred for basalts on the Moon.  相似文献   

19.
A study on the distribution of neutron exposures in a low-mass asymptotic giant branch (AGB) star is presented, according to the s-process nucleosynthesis model with the 12C(α, n)16O reaction occurred under radiative conditions in the interpulse phases. The model parameters, such as the over- lap factor r of two successive convective thermal pulses, the mass ratio q of the 13C shell with respect to the He intershell, and the effective mass of 13C in the 13C shell, vary with the pulse number. Considering these factors, a calculating method for the distribution of neutron exposures in the He intershell has been presented. This method has the features of simplicity and universality. Using this method, the exposure distribution for the stellar model of a star with the mass of 3 M? and the solar metallicity has been calculated. The results suggest that under the reasonable assumption that the number density of neutrons is uniform in the 13C shell, the ?nal exposure distribution approaches to an exponential distribution. For a stellar model with the de?nite initial mass and metallicity, there is a de?nite relation between the mean neutron exposure τ0 and the neutron exposure Δτ of each pulse, namely τ0 = 0.434λ(q1, q2, …, qmmax +1, …, r1, r2, …, rmmax +1)Δτ, where mmax is the total number of thermal pulses with the third dredge-up episode, and the proportional coeffcient λ(q1, q2, …, qmmax +1, …, r1, r2, …, rmmax +1) can be determined by an exponential curve ?tting to the ?nal exposure distribution. This new formula quantitatively uni?es the classical model with the s-process nu- cleosynthesis model by means of neutron exposure distribution, and makes the classical model continue to offer guidance and constraints to the s-process nu- merical calculations of stellar models.  相似文献   

20.
We analyzed noble gases in nine individual chondrules, an assemblage of small chondrules, and four whole‐rock samples of the Allende CV3 chondrite. Major elements were also determined for five chondrules. The cosmic ray exposure ages are calculated from cosmogenic 3He to be 5.17 ± 0.38 and 5.15 ± 0.25 Myr for the averages of the chondrules and whole rocks, respectively, showing no significant pre‐exposure evidence for the studied chondrules. Large amounts of 36Ar, 80,82Kr, and 128Xe produced by neutron capture are observed in most samples; the abundances of these nuclides are correlated among the samples. The epithermal neutron flux and neutron slowing down density are calculated based on [80Kr]n, from which a sample depth of about 30 cm can be calculated. The measured chondrules contain variable amounts of radiogenic 129Xe. The abundance ratios of radiogenic 129Xe to neutron capture–produced 128Xe are rather constant among the studied chondrules; four chondrules give more precise ratios at the high‐temperature fractions, ranging from 1920 ± 80 to 2280 ± 140, which corresponds to a time difference of 3.9 ± 2.4 Myr. It is noticeable that most chondrules also contain 244Pu‐derived fission Xe. The average 244Pu/238U ratio for nine chondrules is 0.0069 ± 0.0018, which agrees well with the preferred ratio reported for chondrites.  相似文献   

设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号