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1.
In-situ cosmogenic 3He exposure ages of pyroxene phenocrysts from basalts from the Upper Neostromboli formation in southwest Stromboli date its eruption at 7.0 ± 0.3 ka (1σ, n = 3, Ginostra site) and 6.8 ± 0.2 ka (1σ, n = 10, Timpone del Fuoco site) respectively. Correlation of our new data to previous K/Ar and palaeomagnetic ages from the northwestern Neostromboli phase suggests that it erupted within a confined period between roughly 6 and 14 ka. The low uncertainty on the 3Hecos ages as well as on individual exposure ages (4.4–8.7%) demonstrates that 3Hecos exposure dating is a viable tool for dating Holocene basalt lavas. The ages compare favourably to uncertainties obtained for radiocarbon dating of similar rocks.  相似文献   

2.
《Marine pollution bulletin》2009,58(6-12):515-523
Hatched juveniles of Caprella danilevskii (Crustacea: Amphipoda) were exposed to one of two concentrations of tributyltin (TBT) (1.1 and 10.7 ng TBT L−1) for 49 d at 20 °C. These concentrations are near or below ambient levels in seawater. In both treatments and control, the survival rate was 100% at maturation, and >85% at the end of the experiments. Females reached maturation at 20 (median) to 21.5 d at instar VII, and repeated spawning 4–5 times during the experiment. The total number of juveniles per female decreased significantly from 39.5 in the control to 24.5 and 17.5 in 1.1 ng L−1 and 10.7 ng L−1 treatments, respectively. An earlier study reported that as the TBT concentration in seawater increased from a 0–10 ng L−1 regime to a 10–20 ng L−1 regime, the number of stations where Caprella spp. could be collected decreased along the coast of the Seto Inland Sea, of Japan. Thus, the present study indicates the possibility that the extremely low concentration of TBT measured in Japanese waters after 2000 lead to a reduction in reproductive success of Caprella spp.  相似文献   

3.
To investigate the interaction between cyanobacteria and heterotrophic bacteria under gradients of glucose and nitrate, a cyanobacterial strain of Microcystis aeruginosa was grown in microcosms with and without a freshwater bacterial mixture, which was collected from Lake Taihu. Concentrations of glucose (1350, 975, 600, 300, 150, and 37.5 μmol C L−1) and nitrate (150, 300, and 9000 μmol N L−1) were used in a range of combinations giving 9 different treatments of glucose:nitrate. In the microcosm without the bacterial mixture, M. aeruginosa abundance gradually increased with days in all treatments. However, M. aeruginosa had much lower density in some treatments with the bacterial mixture. The difference in M. aeruginosa growth could be explained by competition with bacteria in the cultures in which these were added. The abundance of M. aeruginosa and bacteria when grown together was nearly equal and the number of the bacterial species was highest in the treatment with 300 μmol C L−1 and 150 μmol N L−1. Our results suggest that at this glucose:nitrate ratio M. aeruginosa and the bacterial mixture maintain a balance, and bacteria maintain diversity. In conclusion, we propose that dissolved organic carbon and nitrate availability fundamentally affects the structure as well as stoichiometry of pelagic associations.  相似文献   

4.
《Marine pollution bulletin》2009,58(6-12):575-586
Irgarol 1051 (2-methythiol-4-tert-butylamino-6-cyclopropylamino-s-triazine) is an algaecide commonly used in antifouling paints. It undergoes photodegradation which yields M1 (2-methylthio-4-tert-butylamino-6-amino-s-triazine) as its major and most stable degradant. Elevated levels of both Irgarol and M1 have been detected in coastal waters worldwide; however, ecotoxicity effects of M1 to various marine autotrophs such as cyanobacteria are still largely unknown. This study firstly examined and compared the 96 h toxicities of Irgarol and M1 to the cyanobacterium Chroococcus minor and two marine diatom species, Skeletonema costatum and Thalassiosira pseudonana. Our results suggested that Irgarol was consistently more toxic to all of the three species than M1 (96 h EC50 values: C. minor, 7.71 μg L−1 Irgarol vs. >200 μg L−1 M1; S. costatum, 0.29 μg L−1 Irgarol vs. 11.32 μg L−1 M1; and T. pseudonana, 0.41 μg L−1 Irgarol vs. 16.50 μg L−1 M1). Secondly, we conducted a meta-analysis of currently available data on toxicities of Irgarol and M1 to both freshwater and marine primary producers based on species sensitivity distributions (SSDs). Interestingly, freshwater autotrophs are more sensitive to Irgarol than their marine counterparts. For marine autotrophs, microalgae are generally more sensitive to Irgarol than macroalgae and cyanobacteria. With very limited available data on M1 (i.e. five species), M1 might be less toxic than Irgarol; nonetheless this finding warrants further confirmation with additional data on other autotrophic species.  相似文献   

5.
We present a 10Be production-rate calibration derived from an early Holocene debris-flow deposit at about 1000 m above sea level in the central Southern Alps, New Zealand, in the mid-latitude Southern Hemisphere. Ten radiocarbon ages on macrofossils from a soil horizon buried by the deposit date the deposit to 9690 ± 50 calendar years before AD2008. Surface 10Be concentrations of seven large boulders partially embedded in the stable surface of the deposit are tightly distributed, yielding a standard deviation of ～2%. Conversion of the 10Be measurements to sea level/high-latitude values using each of five standard scaling methods indicates 10Be production rates of 3.84 ± 0.08, 3.87 ± 0.08, 3.83 ± 0.08, 4.15 ± 0.09, and 3.74 ± 0.08 atoms g?1 a?1, relative to the ‘07KNSTD’ 10Be AMS standard, and including only the local time-integrated production-rate uncertainties. When including a sea level high-latitude scaling uncertainty the overall error is ～2.5% (1σ) for each rate. To test the regional applicability of this production-rate calibration, we measured 10Be concentrations in a set of nearby moraines deposited before 18 060 ± 200 years before AD2008. The 10Be ages are only consistent with minimum-limiting 14C age data when calculated using the new production rates. This also suggests that terrestrial in situ cosmogenic-nuclide production did not change significantly from Last Glacial Maximum to Holocene time in New Zealand. Our production rates agree well with those of a recent calibration study from northeastern North America, but are 12–14% lower than other commonly adopted values. The production-rate values presented here can be used elsewhere in New Zealand for rock surfaces exposed during or since the last glacial period.  相似文献   

6.
Soda lakes and pans represent saline ecosystems with unique chemical composition, occurring on all continents. The purpose of this study was to identify and characterise the main environmental gradients and trophic state that prevail in the soda pans (n = 84) of the Carpathian Basin in Central Europe. Underwater light conditions, dissolved organic matter, phosphorus and chlorophyll a were investigated in 84 pans during 2009–2010. Besides, water temperature was measured hourly with an automatic sensor throughout one year in a selected pan. The pans were very shallow (median depth: 15 cm), and their extremely high turbidity (Secchi depth median: 3 cm, min: 0.5 cm) was caused by high concentrations of inorganic suspended solids (median: 0.4 g L−1, max: 16 g L−1), which was the dominant (>50%) contributing factor to the vertical attenuation coefficient in 67 pans (80%). All pans were polyhumic (median DOC: 47 mg L−1), and total phosphorus concentration was also extremely high (median: 2 mg L−1, max: 32 mg L−1). The daily water temperature maximum (44 °C) and fluctuation maximum (28 °C) were extremely high during summertime. The combination of environmental boundaries: shallowness, daily water temperature fluctuation, intermittent hydroperiod, high turbidity, polyhumic organic carbon concentration, high alkalinity and hypertrophy represent a unique extreme aquatic ecosystem.  相似文献   

7.
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8.
《Marine pollution bulletin》2012,65(12):2663-2670
This study evaluated embryotoxicity and genotoxicity of two dissolved metals copper and cadmium (Cu and Cd) and two pesticides (metolachlor and irgarol) occurring in Arcachon Bay (SW France) in Pacific oyster (Crassostrea gigas) larvae and investigated the relationship between those two endpoints. Embryotoxicity was measured by calculating the percentage of abnormal D-shaped larvae and genotoxicity was evaluated with DNA strand breaks using the comet assay. After 24 h exposure, significant increases of the percentage of abnormal D-larvae and the DNA strand breaks were observed from 0.1 μg L−1 for Cu, 10 μg L−1 for Cd and 0.01 μg L−1 for both irgarol and metolachlor in comparison with the controls. A strong positive relationship between embryotoxicity and genotoxicity was recorded for Cu, Cd and metolachlor. The current study suggests that copper, irgarol and metolachlor can induce larval abnormalities and DNA damage in a population of exposed oysters at environmentally relevant concentrations.  相似文献   

9.
Magnetic sector mass spectrometers dominate the field of 40Ar/39Ar geochronology. Recent advances in quadrupole mass spectrometer technology, especially improvements in resolution, have increased the performance of these instruments to the extent that they can be used for isotopic determinations. We describe a triple filter quadrupole mass spectrometer (Hiden HAL 3F Series Pulse Ion Counting Triple Filter QMS) linked to an automated furnace extraction and cleaning system dedicated to 40Ar/39Ar incremental heating experiments.The instrument produces peaks with broad flat tops and a width of 0.9 amu at 10 cps height and 0.84 amu at 500,000 cps height on a 1 million cps high peak (peak width at 0.01‰ and 50% peak height respectively). This allows measurement of ratios of the main Ar peaks in the 1‰ range. Measurements of 1.6 × 10?12 mole of air reference gas over two years yields 40Ar/36Ar = 257.9 ± 1.3 (1σ, n = 34). The ability of the instrument to produce 40Ar/39Ar ages from rocks/minerals of a wide age range, reaching into the late Quaternary, are demonstrated by a series of tests and comparison with geochronological data from other studies and an in-house MAP 215-50 magnetic sector mass spectrometer. We demonstrate that high-end quadrupole systems can be used for routine 40Ar/39Ar dating purposes.  相似文献   

10.
The Adriatic foreland of the Apennines comes ashore only in Apulia (easternmost Italy). Its southern part, our study area, lacks any structural analysis devoted to define its recent-to-active tectonics. Throughout the Quaternary, this region was affected by mild brittle deformation with rare faults, characterized by small displacement, and widespread extension joints, frequently organized in sets. Therefore, we conducted a quantitative and systematic analysis of the joint sets affecting Quaternary deposits, by applying an inversion technique ad hoc to infer the orientation and ratio of the principal stress axes, R = (σ2 ? σ3)/(σ1 ? σ3). Within a general extensional regime, we recognized three deformational events of regional significance. The oldest event, constrained to the early and middle part of the Middle Pleistocene, is characterized by variable direction of extension and R between 0.64 and 0.99. The penultimate event, dated late Middle Pleistocene, is characterized by an almost uniaxial tension, with a horizontal σ3 striking ～N43°E; R is high, between 0.85 and 0.99. The most recent event is characterized by the lowermost R values, that never exceed 0.47 and are frequently <0.30, indicating a sort of horizontal ‘radial’ extension. This event is not older than the Late Pleistocene and possibly reflects the active stress field still dominating the entire study area.  相似文献   

11.
Our study summarizes data from six small water reservoirs in West Slovakia and analyzes the occurrence of zooplankton groups in relation to physico-chemical and catchment variables. The reservoirs are in two different catchments – of the Morava and Váh rivers. A total of 103 species were identified; 64 crustaceans (in both the pelagic and littoral zones) and 39 planktonic Rotifera in the pelagic zones. Significant differences were observed in species richness, abundance and biomass of planktonic crustaceans: 48 species were characteristic of the Váh catchment, while 53 were found in the Morava catchment. The density of zooplankton in the three reservoirs of the Váh River catchment ranged from 102 ind L?1 to 21,488 ind L?1 and the zooplankton biomass ranged from 0.12 mg L?1 to 103.29 mg L?1. The density of zooplankton in three Morava River catchment reservoirs ranged from 2 ind L?1 to 3928 ind L?1 and the zooplankton biomass ranged from 0.1 mg L?1 to 27.3 mg L?1. The differences were found to be related to catchment (altitude and catchment affiliation), chemical (BOD5, DO) and biological (Chromophyta, Chlorophyta) factors. Eutrophication of reservoirs in the Váh catchment was mainly due to agriculture and fish management, resulting in high nutrient concentrations. Species richness showed an unimodal response to BOD5 and N-NH4 with near optimum low values, 4.6 and 0.19 respectively. The relationship to oxygen content reflects preferences for less eutrophic waters and species richness tended to decrease with increasing DO and to decrease with increasing nutrient content.  相似文献   

12.
Nanoparticle contamination in freshwater habitat leads to the drastic reduction in the population of freshwater micro crustaceans. Both Ceriodaphnia cornuta and Moina micrura were considered as the potential biological bio-tracers of freshwater ecosystem. This study describes the chemical synthesis of zinc oxide nanoparticles (ZnO NPs) using zinc nitrate as the starting material. The physico-chemical characterization of ZnO NPs was made by UV–Vis spectroscopy, X-Ray Diffraction (XRD), Fourier Transform Infra Red (FTIR) and Transmission Electron Microscopy (TEM). ZnO NPs elicited 100% and 76% mortality of freshwater crustaceans, Ceriodaphnia cornuta and Moina micrura at 160 μg L−1 respectively. The accumulation of ZnO NPs in the intestine and loss of antennae and carapace were clearly visualized through light microscopy. The exposure of C. cornuta and M. micrura neonates at 160 μg L−1 of ZnO NPs showed abnormal swimming behaviour after 12 h. However, chitosan significantly reduced the mortality and enhanced the survival of C. cornuta and M. micrura at 100 μg ml−1. This study concludes the protective effect of chitosan against the hazardous effect of ZnO NPs in C. cornuta and M. micrura.  相似文献   

13.
The single backscattering model was used to estimate total attenuation of coda waves (Qc) of local earthquakes recorded on eight seismological stations in the complex area of the western continental Croatia. We estimated Q0 and n, parameters of the frequency dependent coda-Q using the relation Qc = Q0fn. Lapse time dependence of these parameters was studied using a constant 30 s long time window that was slid along the coda of seismograms. Obtained Qc were distributed into classes according to their lapse time, tL. For tL = 20–50 s we estimated Q0 = 45–184 and n = 0.49–0.94, and for tL = 60–100 s we obtained Q0 = 119–316 and n = 0.37–0.82. There is a tendency of decrease of parameter n with increasing Q0, and vice versa. The rates of change of both Q0 and n seem to decrease for lapse times larger than 50–80 s, indicating an alteration in rock properties controlling coda attenuation at depths of about 100–160 km. A very good correlation was found between the frequency dependence parameter n and the Moho depths for lapse times of 50, 60 and 70 s.  相似文献   

14.
《Marine pollution bulletin》2012,65(12):2650-2655
In the present work, fat, skin, liver and muscle samples from Leptonychotes weddellii (Weddell seal, n = 2 individuals), Lobodon carcinophagus (crabeater seal, n = 2), Arctocephalus gazella (Antarctic fur seal, n = 3) and Mirounga leonina (southern elephant seal, n = 1) were collected from King George Island, Antarctica, and analysed for POPs (PCBs, organochlorine pesticides and PBDEs) and stable isotopes (δ13C and δ15N in all tissues but fat). PBDEs could be found in only one sample (L. weddellii fat). Generally, PCBs (from 74 to 523 ng g−1 lw), DDTs (from 14 to 168 ng g−1 lw) and chlordanes (from 9 to 78 ng g−1 lw) were the prevailing compounds. Results showed a clear stratification in accordance with ecological data. Nonetheless, stable isotope analyses provide a deeper insight into fluctuations due to migrations and nutritional stress. Correlation between δ15N and pollutants suggests, to some degree, a considerable ability to metabolize and/or excrete the majority of them.  相似文献   

15.
Growth, stem morphology and some biochemical parameters were studied of one completely submerged (Myriophyllum spicatum) and two floating leaved macrophytes (Nymphoides peltata and Trapa japonica) under different turbulence velocities. The root mean square velocities of the high, medium and low amount of turbulence that was generated for the experiment were 2.18 ± 0.66, 1.48 ± 0.26 and 0.70 ± 0.07 cm s−1, respectively, in the microcosm. All three experimental plants survived exposed to all turbulence conditions provided, although a decrease in shoot elongation rate was associated with an increase in turbulence. Acceleration of tissue H2O2 generation and MDA content increased during the study period in all plant species. Oxidative enzymatic activities (POD, IAA and CKX) increased with time in plants under medium and high turbulence velocities. The shoot elongation rate, stem and leaf diameter, chlorophyll content and carbohydrate fractionations were found to be affected by this abiotic stress. It is evident from this study that high turbulence velocity inhibits normal metabolic activities of all three plants, while low to medium turbulence does not harm the floating leaved plants. Moreover, floating leaved plants were found to possess highly capable strategies to cope with this mechanical stress than completely submerged species.  相似文献   

16.
The ～ 14 km diameter Jänisjärvi impact structure is located in Svecofennian Proterozoic terrain in the southeastern part of the Baltic shield, Karelia, Russia. Previous radioisotopic dating attempts gave K/Ar and 40Ar/39Ar ages of 700 ± 5 Ma and 698 ± 22 Ma, respectively, with both results being difficult to interpret. Recent paleomagnetic results have challenged these ages and proposed instead ages of either 500 Ma or 850–900 Ma. In order to better constrain the age of the Jänisjärvi impact structure, we present new 40Ar/39Ar data for the Jänisjärvi impact melt rock. We obtained five concordant isochron ages that yield a combined isochron age of 682 ± 4 Ma (2σ) with a MSWD of 1.2, P = 0.14, and 40Ar/36Ar intercept of 475 ± 3. We suggest that this date indicates the age of the impact and therefore can be used in conjunction with existing paleomagnetic results to define the position of the Baltica paleocontinent at that time. Argon isotopic results imply that melt homogenization was achieved at the hundred-micrometer scale certainly, because of the low-silica content of the molten target rock that allows fast 40Ar? diffusion in the melt. However, the large range of F(40Ar?inherited) (4.1% to 11.0%) observed for seven grains shows that complete isotopic homogenization was not reached at the centimeter and perhaps the millimeter scale. The F(40Ar?inherited) results are also in good agreement with previous Rb and Sr isotopic data.  相似文献   

17.
Carbonatites are mantle-derived, intraplate magmas that provide a means of documenting isotopic variations of the Earth's mantle through time. To investigate the secular Li isotopic evolution of the mantle and to test whether Li isotopes document systematic recycling of material processed at or near the Earth's surface into the mantle, we analyzed the Li isotopic compositions of carbonatites and spatially associated mafic silicate rocks. The Li isotopic compositions of Archean (2.7 Ga) to Recent carbonatites (δ7Li = 4.1 ± 1.3 (n = 23, 1σ)) overlap the range typical for modern mantle-derived rocks, and do not change with time, despite ongoing crustal recycling. Thus, the average Li isotopic composition of recycled crustal components has not deviated greatly from the mantle value (~ + 4) and/or Li diffusion is sufficiently fast to attenuate significant heterogeneities over timescales of 108 years. Modeling of Li diffusion at mantle temperatures suggests that limited δ7Li variation in the mantle through time reflects the more effective homogenization of Li in the mantle compared to radiogenic isotope systems. The real (but limited) variations in δ7Li that exist in modern mantle-derived magmas as well as carbonatites studied here may reflect isotopic fractionation associated with shallow-level processes, such as crustal assimilation and diffusive isotopic fractionation in magmatic systems, with some of the scatter possibly related to low-temperature alteration.  相似文献   

18.
We have evaluated all parameters for the calculation of cosmogenic 36Cl production rates and thus surface exposure ages in dolomite and limestone. We found that we can use either of both published negative muon stopping rates until more information is available. The largest uncertainty of the age estimation in the upper meter of rock comes from the 36Cl production rate from Ca spallation and, in the case of 50–100 ppm Cl content, from the production rate of epithermal neutrons, which we estimate at 760 ± 150 neutrons/g_air/yr (1σ). For a sample with representative amounts of Ca and Cl (20 wt% Ca and 50 ppm Cl, or 40 wt% Ca and 100 ppm Cl), the age can be calculated with a precision of 7–10% in the top 1.5 m of the depth profile. Further improvement of 36Cl calculations depends on new calibration of 36Cl production from Ca spallation, re-evaluation of 36Cl production by low-energy neutron capture on 35Cl, as well as of the muon flux and muon capture based on the most recent measurement data.  相似文献   

19.
In general, the rate and timing of calcite precipitation is in part affected by variations in cave air CO2 concentrations. Knowledge of cave ventilation processes is required to quantify the effect variations in CO2 concentrations have on speleothem deposition rates and thus paleoclimate records. In this study we use radon-222 (222Rn) as a proxy of ventilation to estimate CO2 outgassing from the cave to the atmosphere, which can be used to infer relative speleothem deposition rates. Hollow Ridge Cave, a wild cave preserve in Marianna, Florida, is instrumented inside and out with multiple micro-meteorological sensor stations that record continuous physical and air chemistry time-series data. Our time series datasets indicate diurnal and seasonal variations in cave air 222Rn and CO2 concentrations, punctuated by events that provide clues to ventilation and drip water degassing mechanisms. Average cave air 222Rn and CO2 concentrations vary seasonally between winter (222Rn = 50 dpm L? 1, where 1 dpm L? 1 = 60 Bq m? 3; CO2 = 360 ppmv) and summer (222Rn = 1400 dpm L? 1; CO2 = 3900 ppmv). Large amplitude diurnal variations are observed during late summer and autumn (222Rn = 6 to 581 dpm L? 1; CO2 = 360 to 2500 ppmv).We employ a simple first-order 222Rn mass balance model to estimate cave air exchange rates with the outside atmosphere. Ventilation occurs via density driven flow and by winds across the entrances which create a ‘venturi’ effect. The most rapid ventilation occurs 25 m inside the cave near the entrance: 45 h? 1 (1.33 min turnover time). Farther inside (175 m) exchange is slower and maximum ventilation rates are 3 h? 1 (22 min turnover time). We estimate net CO2 flux from the epikarst to the cave atmosphere using a CO2 mass balance model tuned with the 222Rn model. Net CO2 flux from the epikarst is highest in summer (72 mmol m? 2 day? 1) and lowest in late autumn and winter (12 mmol m? 2 day? 1). Modeled ventilation and net CO2 fluxes are used to estimate net CO2 outgassing from the cave to the atmosphere. Average net CO2 outgassing is positive (net loss from the cave) and is highest in late summer and early autumn (about 4 mol h? 1) and lowest in winter (about 0.5 mol h? 1). Modeling of ventilation, net CO2 flux from the epikarst, and CO2 outgassing to the atmosphere from cave monitoring time-series can help better constrain paleoclimatic interpretations of speleothem geochemical records.  相似文献   

20.
Tektites are terrestrial natural glasses produced during a hypervelocity impact of an extraterrestrial projectile onto the Earth's surface. The similarity between the chemical and isotopic compositions of tektites and terrestrial upper continental crust implies that the tektites formed by fusion of such target rock. Tektites are among the driest rocks on Earth. Although volatilization at high temperature may have caused this extreme dryness, the exact mechanism of the water loss and the behavior of other volatile species during tektite formation are still debated. Volatilization can fractionate isotopes, therefore, comparing the isotope composition of volatile elements in tektites with that of their source rocks may help to understand the physical conditions during tektite formation.For this study, we have measured the Zn isotopic composition of 20 tektites from four different strewn fields. Almost all samples are enriched in heavy isotopes of Zn compared to the upper continental crust. On average, the different groups of tektites are isotopically distinct (listed from the isotopically lightest to the heaviest): Muong-Nong type indochinites (δ66/64Zn = 0.61 ± 0.30‰); North American bediasites (δ66/64Zn = 1.61 ± 0.49‰); Ivory Coast tektites (δ66/64Zn = 1.66 ± 0.18‰); the Australasian tektites (others than the Muong Nong-type indochinites) (δ66/64Zn = 1.84 ± 0.42‰); and Central European moldavites (δ66/64Zn = 2.04 ± 0.19‰). These results are contrasted with a narrow range of δ66/64Zn = 0–0.7‰ for a diverse spectrum of upper continental crust materials.The elemental abundance of Zn is negatively correlated with δ66/64Zn, which may reflect that isotopic fractionation occurred by evaporation during the heating event upon tektite formation. Simple Rayleigh distillation predicts isotopic fractionations much larger than what is actually observed, therefore, such a model cannot account for the observed Zn isotope fractionation in tektites. We have developed a more realistic model of evaporation of Zn from a molten sphere: during its hypervelocity trajectory, the molten surface of the tektite will be entrained by viscous coupling with air that will then induce a velocity field inside the molten sphere. This velocity field induces significant radial chemical mixing within the tektite that accelerates the evaporation process. Our model, albeit parameter dependent, shows that both the isotopic composition and the chemical abundances measured in tektites can be produced by evaporation in a diffusion-limited regime.  相似文献   

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