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1.
Low magnetic susceptibility, low Sr content and hence high Rb/Sr ratio in the lake sediment sequence indicate a weak chemical
weathering process under arid and cold climate of the Little Ice Age in a single closed lake watershed. According to different
geochemical behavior between rubidium and strontium in earth surface processes, variation of Rb/Sr ratios in the lake sediment
sequence can be used as an effective geochemical proxy with definite climatic significance of chemical weathering in watershed.
Unlike chemical weathering process in tropic zone and modern temperate-humid climate, concordant changes in both Sr content
and magnetic susceptibility with δ18O values of Dunde ice core suggest that the weak chemical weathering was controlled by air temperature during the Little Ice
Age maximum. After the Little Ice Age, chemical weathering intensity was controlled also gradually by precipitation with increasing
in temperature. 相似文献
2.
Variation in the rubidium to strontium (Rb/Sr) ratio of the loess–palaeosol sequences has been proposed to reflect the degree of pedogenesis and weathering in the northwestern region of China. To characterize the Rb/Sr ratio of the dissolved loads of a single catchment, we analysed a 12·08 m sediment core from Daihai Lake in Inner Mongolia, north China. Dating control was provided by 210Pb, 137Cs and AMS‐14C. Sequential extraction experiments were conducted to investigate the concentrations of Rb and Sr on various chemical fractions in the lake sediments. Down‐core variation in the Rb/Sr ratios provides a record of Holocene weathering history. From 9 to 3·5 ka bp , accelerated chemical weathering was experienced throughout the Daihai catchment under mainly warm and humid conditions, and this reached a maximum at c. 5 ka bp . However, weathering was reduced between c. 8·25 and 7·90 ka bp , which may reflect the global 8·2 ka cooling event. After c. 2·5 ka bp , increased Rb/Sr ratios with higher frequency of fluctuations indicate reduced weathering within the Daihai catchment. The highest Rb/Sr ratios in the Little Ice Age lake sediments indicate the weakest phase of Holocene chemical weathering, resulting from a marked reduction in Sr flux into the basin. The Rb/Sr record also shows an enhancement of chemical weathering under today's climate, but its intensity is less than that of the Medieval Warm Period. Increased Rb/Sr in lake sediment corresponding to reduced catchment weathering is in striking contrast to Rb/Sr decrease in the glacial loess layers in the loess–palaeosol sequence. Copyright © 2005 John Wiley & Sons, Ltd. 相似文献
3.
湖泊沉积物中元素相态的连续提取分析—以岱海为例 总被引：7，自引：1，他引：6
如何利用湖泊/海洋沉积物地球化学代用指标有效地指示环境很大程度取决于元素的来源及其在沉积物中赋存形态的确定.对位于半干旱区的内蒙古岱海14个沉积物样品的连续提取实验及18个元素在水可溶态、可交换态、碳酸盐结合态、铁锰氧化物结合态、有机物结合态及残留态等六种赋存相态中含量变化进行了测试和研究,结合沉积物的矿物组成,结果表明在岱海流域内只经历了较弱的化学风化过程,除了Ca和Sr外,其他元素主要赋存于残留态中,只发生了很小程度的活化溶解.受元素亲合性和湖水物理化学状态的制约,出溶的Sr与Ca的赋存相态基本一致,而出溶的Pb、Be、Co、Cu、K、Mn、Fe等元素则与自生碳酸盐、有机质表现出一定的亲合性.元素在不同赋存相态中分布为地球化学环境代用指标的提取和解释提供了机理性的实验依据. 相似文献
4.
岱海的"中世纪暖期" 总被引：30，自引：1，他引：29
内蒙古岱海沉积物近2200a来Rb/Sr比值、CaCO3和有机碳含量的变化展现了包括中世纪暖期（MWP）及小冰期（LIA）等典型气候事件在内的环境演化过程,总体表现为暖期的沉积物Rb/Sr比值低,冷期的则高：CaCO3和有机碳含量则相反。这里,以单一流域化学风化记录表明我国北方存在明显的中世纪暖期,发生时间约900－1200aB.P..主要环境特征表现为流域化学风化的显著增强（低Rb/Sr比值）、生物生产力逐步提高（高有机碳）、湖泊水位大幅度抬升的湖泊沉积记录,其间经历的化学风化是近两千年内最强的,并且其发生时间与全球其他地区基本一致。 相似文献
5.
The X-ray fluorescence(XRF)core-scanned Rb/Sr ratios of lake sediments have been widely used as a proxy for chemical weathering intensity and past climate change.However,some factors could affect Rb/Sr ratios,causing misinterpretation and limiting its application.In this study,we present a high-resolution XRF core-scanned Rb/Sr record of core ZB13-C1 from the Zoige Basin in the eastern Tibetan Plateau.To validate its application,we correlated this record with the chemical index of alteration(CIA)and other paleoclimatic proxies.Our results showed that(1)the core-scanned Rb/Sr ratios and CIA were reliable proxies of chemical weathering intensity in fine-grained sedimentary sequences;(2)the low values of corescanned Rb/Sr ratios and CIA were significantly correlated with high total organic carbon content,arboreal pollen content,carbonate content,and C/N ratios,confirming its reliability as a proxy for the Asian summer monsoon intensity;(3)the corescanned Rb/Sr ratios at core depths of 25–0.3 and 56–47 m were unable to reliably reflect chemical weathering intensity due to both the grain-size effect and the low test accuracy.Our study highlights the need for mutual verification of multiple indicators before accurately applying Rb/Sr as a paleoclimatic proxy in other similar study areas. 相似文献
6.
Mohammad Nuruzzama Waliur Rahaman Gyana R. Tripathy Rahul Mohan Shramik Patil 《水文研究》2020,34(11):2351-2364
Dissolved major ions, Sr concentrations and 87Sr/86Sr ratios of 10 coastal lakes from the Larsemann Hills, East Antarctica have been studied to constrain their solute sources, transport and glacial weathering patterns in their catchments. In absence of perennial river/streams, lakes serve as only reliable archive to study land surface processes in these low-temperature regions. The lake water chemistry is mostly Na-Cl type and it does not show any significant depth variations. Sr isotope compositions of these lakes vary from 0.7110 to 0.7211 with an average value of 0.7145, which is higher than modern seawater value. In addition to oceanic sources, major ions and Sr isotopic data show appreciable amount of solute supply from chemical weathering of silicate rocks in lake catchments and dissolution of Ca-Mg rich salts produced during the freezing of seawaters. The role of sulphide oxidation and carbonate weathering are found to be minimal on lake hydro-chemistry in this part of Antarctica. Inverse model calculations using this chemical dataset provide first-order estimates of dissolved cations and Sr; they are mostly derived from oceanic (seawater + snow) sources (cations approximately 76%) and (Sr approximately 92%) with minimal supplies from weathering of silicates (cations approximately 15%); (Sr approximately 2%) and Ca-rich minerals (cations approximately 9%); (Sr approximately 7%). The silicate weathering rate and its corresponding atmospheric CO2 consumption rate estimates for Scandrett lake catchment (3.6 ± 0.3 tons/km2/year and 0.5 × 105 moles/km2/year), are lower than that of reported values for the average global river basins (5.4 tons/km2/year and 0.9 × 105 tons/km2/year) respectively. The present study provides a comprehensive report of chemical weathering intensity and its role in atmospheric CO2 consumption in low-temperature pristine environment of Antarctica. These estimates underscore the importance of Antarctica weathering on atmospheric CO2 budget, particularly during the past warmer periods when the large area was exposed and available for intense chemical weathering. 相似文献
7.
Variations in chemical compositions of the eolian dust in Chinese Loess Plateau over the past 2.5 Ma and chemical weathering in the Asian inland 总被引：5，自引：0，他引：5
Major and trace elements as well as strontium isotopic composition have been analyzed on the acid-insoluble (AI) phase of
the loess-paleosol sequence from Luochuan, Shaanxi Province, China. Results show that the chemical composition of AI phase
of loess and paleosols is distinctive to the average composition of upper continental crust (UCC), characterized by depletion
of mobile elements Na, Ca and Sr. The distribution pattern of elements in AI phase reveals that initial dust, derived from
a vast area of Asian inland, has suffered from Na- and Ca-removed chemical weathering compared to UCC. Some geochemical parameters
(such as CIA values, Na/K, Rb/Sr and87Sr/86Sr ratios) display a regular variation and evolution, reflecting that the chemical weathering in the source region of loess
deposits has decreased gradually since 2.5 Ma with the general increase of global ice volume. This coincidence reflects that
the aridity of Asian inland since the Quaternary is a possible regional response to the global climate change. 相似文献
8.
The Sr isotopic systematics in the weathering profiles of biotite granite and granite porphyry in southern Jiangxi Province were investigated. The results showed that during the chemical weathering of granites, remarked fractionation occurred between Rb and Sr. During the early stages of chemical weathering of granites, the released Sr/Si and Sr/Ca ratios are larger than those of the parent rocks, and the leaching rate of Sr is higher than those of Si, Ca, K, Rb, etc. Dynamic variations in relative weathering rates of the main Sr-contributing minerals led to fluctuation with time in87Sr/86Sr ratios of inherent and released Sr in the weathering crust of granite. Successive weathering of biotite, plagioclase and K-feldspar made87Sr/86Sr ratios in the weathering residues show such a fluctuation trend as to decrease first, increase, and then decrease again till they maintain stable. This work further indicates that when Sr isotopes are used to trace biogeochemical processes on both the catchment and global scales, one must seriously take account of the preferential release of Sr from dissolving solid phase and the fluctuation of87Sr/86Sr ratios caused by the variations of relative weathering rates of Sr-contributing minerals. 相似文献
9.
Distribution of Rb and Sr in the Luochuan loess- paleosol sequence of China during the last 800 ka 总被引：4，自引：0，他引：4
The concentrations of Rb and Sr, and magnetic susceptibility in loess and paleosol samples from the Luochum profile have been
measured. The loess units deposited in different geological periods display a very similar pattern of Rb and Sr distribution
while paleosol units exhibit a dramatic increase in the Rb/Sr ratio, ranging from 20% to 120% in increase amplitude. Owing
to different geochemical behavior of the two elements, Rb appears to be immobile while Sr appears to be mobile in the processes
of weathering and pedogenesis. So variations of the Rb/Sr ratio in the loess-paleosol sequences could reflect intensities
of weathering and pedogenesis, thus recording the relative wind strength of the East Asian summer monsoon circulation. This
could be supported by the high degree of cornlation between the Rb/Sr ratio and the magnetic susceptibility. A continuous
record of the Rb/Sr ratio in the Luochuan profile over the last 800 ka bears a striking resemblance to the δ18 O curve of the deep sea sediments and is in accordance with the SPECMAP chronology. Such similarity between the terrestrial
and the deep sea records suggests that variability in global ice volume is a primary dynamic factor controlling long-term
changes of the East Asian summer monsoon intensity.
Project supported by the National Natural Science Foundation of China (Grant No. 49725307). 相似文献
10.
Mineral weathering rates and a forest macronutrient uptake stoichiometry were determined for the forested, metabasaltic Hauver Branch watershed in north‐central Maryland, USA. Previous studies of Hauver Branch have had an insufficient number of analytes to permit determination of rates of all the minerals involved in chemical weathering, including biomass. More equations in the mass‐balance matrix were added using existing mineralogic information. The stoichiometry of a deciduous biomass term was determined using multi‐year weekly to biweekly stream‐water chemistry for a nearby watershed, which drains relatively unreactive quartzite bedrock. At Hauver Branch, calcite hosts ~38 mol% of the calcium ion (Ca2+) contained in weathering minerals, but its weathering provides ~90% of the stream water Ca2+. This occurs in a landscape with a regolith residence time of more than several Ka (kiloannum). Previous studies indicate that such old regolith does not typically contain dissolving calcite that affects stream Ca2+/Na+ ratios. The relatively high calcite dissolution rate likely reflects dissolution of calcite in fractures of the deep critical zone. Of the carbon dioxide (CO2) consumed by mineral weathering, calcite is responsible for approximately 27%, with the silicate weathering consumption rate far exceeding that of the global average. The chemical weathering of mafic terrains in decaying orogens thus may be capable of influencing global geochemical cycles, and therefore, climate, on geological timescales. Based on carbon‐balance calculations, atmospheric‐derived sulfuric acid is responsible for approximately 22% of the mineral weathering occurring in the watershed. Our results suggest that rising air temperatures, driven by global warming and resulting in higher precipitation, will cause the rate of chemical weathering in the Hauver Branch watershed to increase until a threshold temperature is reached. Beyond the threshold temperature, increased recharge would produce a shallower groundwater table and reduced chemical weathering rates. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
11.
艾比湖水化学演化的初步研究 总被引：10，自引：0，他引：10
本文通过野外地质调查和大量样品的分析测试结果,从以下三个方面对艾比湖湖水的水化学特征进行论述:(1)湖水的矿化度和pH;(2)湖水的化学组成;(3)湖水化学组分的侧向分布。初步揭示了湖水水化学变化和主要化学元素迁移和富集的规律。艾比湖沉积物中碳酸盐矿物组成及其地球化学性质反映湖水化学组成的变动。这种变动明显受气候环境变化的影响。因此,CK4孔和湖底沉积物中的碳酸盐沉积,提供了许多信息作为湖水化学演化和古气候波动的标志,根据其碳酸盐含量、方解石含量、方解石格架中MgCO_3mol.％、Sr含量和Sr×1000/Ca比值,最后结合碳酸盐的沉积特征、地球化学演化和古沙嘴的演变,进一步阐明了湖水化学演化的趋势。 相似文献
12.
Humid Little Ice Age in arid central Asia documented by Bosten Lake, Xinjiang, China 总被引：15，自引：0，他引：15
J. A. Holmes 《中国科学D辑(英文版)》2006,49(12):1280-1290
Short sediment cores retrieved from Bosten Lake, the largest inland freshwater lake in China, were used to explore humidity and precipitation variations in arid central Asia during the past millennium. The chronology of the cores was established using 137Cs, 210Pb and AMS 14C dating re- sults. Multi-proxy high-resolution analysis, including pollen ratios of Artemisia and Chenopodiaceae (A/C), carbonate content and grain size, indicates that the climate during the past millennium can be divided into three stages: a dry climate between 1000―1500 AD, a humid climate during the Little Ice Age (LIA) (c. 1500―1900 AD), and a warm dry period after 1900 AD. On centennial timescales, the climate change in northwestern China during the past 1000 years is characterized by oscillations between warm-dry and cold-humid climate conditions. All the proxies changed significantly and indi- cate increased precipitation during the LIA, including increased pollen A/C ratios and pollen concen- trations, decreased carbonate content and increased grain size. The humid period during the LIA re- corded by the Bosten Lake sediments is representative of arid central Asia and is supported by nu- merous records from other sites. During the LIA, the water runoff into the Keriya River and Tarim River in the Tarim Basin increased, while the ice accumulation in the Guliya ice core increased. Additionally, the lake levels of the Aral and Caspian Sea also rose, while tree-ring analysis indicates that precipita- tion increased. We hypothesize that both the lower temperature within China and the negative anomalies of North Atlantic Oscillation (NAO) during this period may have contributed to the humid climate within this area during LIA. 相似文献
13.
湖泊沉积物的磁化率、频率磁化率及其古气候意义—以青海湖、岱海近代沉积为例 总被引：28，自引：9，他引：28
湖泊沉积物的磁性参数是古气候、古环境的重要代用指标。通过对青海湖QI5孔和岱海DH32孔短岩心的磁化率、频率磁化率的研究,并与地球化学参数等其它资料对比,探讨了以上两个湖区历史时期古气候变化规律;论证了用磁化率、频率磁化率作为古气候、古环境指标的可靠性和敏感性;并对其变化机制进行了初步探讨。 相似文献
14.
湖泊沉积物的磁化率、频率磁化率及其古气候意义—以青海湖、岱海近代沉积为例 总被引：15，自引：3，他引：12
湖泊沉积物的磁性参数是古气候、古环境的重要代用指标。通过对青海湖QI_5孔和岱海DH_(32)孔短岩心的磁化率、频率磁化率的研究,并与地球化学参数等其它资料对比,探讨了以上两个湖区历史时期古气候变化规律;论证了用磁化率、频率磁化率作为古气候、古环境指标的可靠性和敏感性;并对其变化机制进行了初步探讨。 相似文献
15.
A 14.7 Ka record of earth surface processes from the arid‐monsoon transitional zone of China 
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下载免费PDF全文 Selvaraj Kandasamy Shengqian Chen Chengling Xie Qiaomei Chen Baozhi Lin Kaifeng Yu Qinghai Xu Victor M. Velasco Fahu Chen 《地球表面变化过程与地形》2018,43(3):723-734
The stability of Earth's critical zone is intimately linked with erosion, weathering and vegetation type and density. Therefore, it affects global biogeochemical processes which in turn affect the global climate by absorbing and reflecting solar radiation, and by altering fluxes of heat, water vapour, carbon dioxide and other trace gases through various feedback mechanisms. However, there is a lack of knowledge about how Earth's critical zone processes have changed over time and their link with past monsoon variability, especially in Asia. The study of lake sediments, which contain a suite of inorganic elemental and isotopic proxies, may facilitate the understanding of the Earth's critical zone processes on millennial timescales. Here we reconstruct the history of erosion–weathering–vegetation interactions since ~14.7 ka using geochemical records from a radiocarbon‐dated sediment core from Lake Gonghai in the monsoon‐arid transitional zone of north China. Detrital (Al, Ti, K, Rb) and authigenic (Ca, Sr) elemental records reveal distinct, millennial‐scale, late deglacial‐Holocene erosion and weathering patterns and transitions with the former (latter) elements showing higher (lower) values in warm intervals and vice versa. Chemical Index of Alteration (CIA) molar, a humidity proxy, suggests low humidity during the late deglacial ~11.5–14.7 ka, high humidity during the early‐mid Holocene ~11.5–3.2 ka, and intermediate humidity during the late Holocene interval since ~3.2 ka. The results of cross‐spectral analysis and comparison of our records with other climate reconstructions also suggest a pattern of orbitally‐phased humidity changes in north China. Overall, our results provide evidence for the solar‐forcing of Earth's surface processes in mid‐latitude China under natural climatic conditions. Copyright © 2017 John Wiley & Sons, Ltd. 相似文献
16.
Quantitative measurements on the paleo-weathering intensity of the loess-soil sequences and implication on paleomonsoon 总被引：2，自引：0，他引：2
The loess-soil sequences in northern China provide a near continuous record of Quaternary paleoclimate. The pedogenetic intensity
of the sequences is closely linked with the variations of the East Asian summer monsoon. In this study, 2181 samples from
the Changwu and Xifeng loess sections are analyzed and two high-resolution paleo-weathering timeseries of the last 1.2 Ma
are generated, using the ratio of CBD extractable free Fe2O3 (FeD) versus the total iron (FeT). This new index is compared with micromorphological features, low-frequency magnetic susceptibility,
frequency-dependent magnetic susceptibility, and the Rb/Sr ratio[5,6]. The results suggest that the FeD/FeT ratio is able to better reflect the degree of soil development. Since the chemical
weathering of loess in the Loess Plateau region mainly depends upon the summer precipitation and temperature under modern
climate condition, which are closely associated with strength of summer monsoon, and the chemical weathering intensity of
loess primarily reflects the variations of the summer monsoon circulation. 相似文献
17.
西藏扎布耶湖ZK91-2钻孔沉积特征与气候环境演化 总被引：6，自引：0，他引：6
扎布耶盐湖位于西藏高原腹地,１９９１年在其南部干盐滩中钻取了２０Ｍ深湖相沉积,以５～１０ＣＭ／个的密度进行高分辨率取样,详细探讨了沉积标志,矿物组合（尤其Ｍｇ,Ｃａ,Ｌｉ碳酸盐）、干旱与潮湿两种气候类型的元素组合等气候环境指标,推导了晚更新世以来该湖区湖面涨缩,水质咸淡及气温高低变化。 相似文献
18.
Analyses of rim-to-interior samples of fresh tholeiitic pillow basalts, deuterically altered holocrystalline basalts, and older, weathered tholeiitic basalts from the deep sea indicate that 87Sr/86Sr ratios of the older basalts are raised by low temperature interaction with strontium dissolved in sea water. 87Sr/86Sr correlates positively with H2O in these basalts; however, there is little detectable modification of the strontium isotope composition in rocks with H2O contents less than 1%. The isotope changes appear to be a function of relatively long-term, low-temperature weathering, rather than high-temperature or deuteric alteration. Strontium abundance and isotopic data for these rocks suggest that strontium content is only slightly modified by interaction with sea water, and it is a relatively insensitive indicator of marine alteration. Average Rb-Sr parameters for samples of apparently unaltered basalt are: Rb= 1.11ppm; Sr= 132ppm; 87Sr/86Sr= 0.70247. 相似文献
19.
The clay mineralogy of Tulare Lake sediment was examined to investigate hydroclimatic and environmental changes in the southern Sierra Nevada Mountains (SNM) since the most recent glacial maximum. Evolution of clay mineral assemblages elucidates significant changes in weathering, erosion, and hydroclimatic condition in the catchment. During the last glacial period (24.4–15.1 cal ka BP), low illite content implies less physical erosion of the granitic batholith rocks and a cold and arid environment in the southern SNM. Abrupt increases of illite content at 21.8–20.8 and 17.6 cal ka BP resulted from the glacier advances to the ablation zone and illite-rich glacier flour was transported down to the lake. The gradual increase of smectite induced by progressive depletion of illite-rich glacier flour from 17.6 cal ka BP toward the end of this period indicates climate was beginning to get warm and wet. From 11.9 to 5.3 cal ka BP, two warm and wet periods (10.7–9.4 and 8.2–5.2 cal ka BP) were characterized by high smectite/illite content ratios and low illite crystallinity values, suggesting intensive rainfall precipitation and more physical erosion in the highland and lowland catchment as well as more smectite formation in the terrace soils. Since the last glacial period, physical erosion, in comparison to the chemical weathering, was the dominant process responding to the hydroclimatic change in the Tulare Lake catchment. Moderate to weak chemical weathering was signified by the mostly low illite chemical weathering index of the core sediments. Such results suggest that vegetation cover in the southern SNM was low and limited. 相似文献
20.
K, Rb and Sr concentrations and Sr isotopic compositions were determined for the Dai granitic rocks of trondhjemitic composition occurring in a serpentinite mass in the Nagato tectonic zone formed in the Late Paleozoic era, and for the granitic rocks of quartz dioritic composition recently dredged from the seamount of the Kyushu-Palao Ridge. Both granitic rocks are characterized by low abundances of K and Rb, low K2O/Na2O ratios, high K/Rb ratios, low Rb/Sr ratios and low initial87Sr/86Sr ratios. These characteristics suggest that strong similarities may exist between the Dai granitic rocks and the dredged granitic rocks, and that the Dai granitic rocks may be classified as oceanic plagiogranite. These oceanic plagiogranites may plausibly represent single-stage mantle-derived granites, possibly from the suboceanic mantle. 相似文献