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为了探讨冰晶核化对雷暴云闪电行为的影响,通过已有的三维对流云起、放电模式探讨对比了3种冰晶核化方案,分别为原模式中的经验公式YS方案及与气溶胶相关的DE方案和LP方案。研究表明冰晶核化方案对雷暴云内冰晶微物理发展特征、起电及放电过程均有一定影响。模拟结果显示:(1)考虑了气溶胶的两种新参数化方案中冰晶粒子在高温区(高于-13.8℃)出现,在雷暴云发展过程中DE方案和LP方案冰晶的垂直分布均大于YS方案。(2)DE方案和LP方案中高温区出现的冰晶所带电荷极性有明显的反转现象,导致雷暴云电荷结构产生差异;雷暴云发展旺盛时刻DE方案和LP方案出现三级性电荷结构,而YS方案在整个雷暴云过程都是偶极性,并且DE方案和LP方案中电荷空间分布区域更加广泛。(3)不同核化方案下雷暴云放电特征存在差异,YS方案在偶极性电荷结构背景下没有负地闪产生,而DE方案和LP方案中次正电荷区的存在促进了负地闪的发生,并且负先导出现在较低的高度范围内;DE方案和LP方案中电荷量级较大,因此云闪发生频次以及正、负先导传播次数增加明显。 相似文献
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膨胀云室可形成水汽、水面和冰面过饱和环境,是研究气溶胶粒子、人工影响天气冷暖催化剂核化过程和机理的重要实验设备。但长期以来,我国缺乏装备先进云雾粒子谱和图像测量系统的膨胀云室。2019年完成的我国自主研制的膨胀云室系统由云室主体、控制系统、通讯系统及环境和云雾测量系统4个子系统组成。该系统首次采用了国产云粒子谱仪和成像仪测量系统。测试结果表明:该云室具有良好的温度和压力控制能力,平均降温速率达到0.26℃·min-1,温度分布均匀,-40℃时舱内温差小于0.29℃;膨胀造雾过程4 min,雾可维持4 min,雾滴较小;可以实现从室温到-50℃低温环境的控制,具备压力膨胀成云雾模拟和微物理参数监测能力,解决了我国缺乏气溶胶粒子和暖云催化剂室内实验装备的状况,对验证暖云催化剂核化性能和提高暖云人工增雨科技水平有重要价值。 相似文献
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沙尘气溶胶对云和降水影响的模拟研究 总被引：9，自引：0，他引：9
采用二维分档云模式,对比背景大气气溶胶分布,讨论了扬沙和沙尘暴天气条件下矿物气溶胶对云微物理结构、光学特性以及降水形成的影响.结果表明:扬沙和沙尘暴天气增加大气中大核和巨核的浓度,促进云中水汽的活化,使降水提前出现,暖云和冷云降水量均大幅增加,但可忽略巨核增加对云光学厚度和反照率的作用;当矿物沙尘粒子同时作为有效的云凝结核和冰核参与云的发展时,冰核浓度增加使水成物有效半径减小,抑制了暖云和冷云降水,云内存留的大量冰晶增强云的光学厚度和反照率. 相似文献
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利用GRAPES模式研究气溶胶对云和降水过程的影响 总被引：5，自引：3，他引：2
在GRAPES中尺度模式的双参数微物理方案中加入了气溶胶活化参数化过程,实现了对云滴数浓度的预报。选取不同季节两个降水过程进行模拟,并分别开展了不同气溶胶背景下的两个试验进行对比分析,研究气溶胶对云和降水可能的影响。结果表明:气溶胶浓度增加后,因为活化产生了更多尺度较小的云滴,抑制了云雨的自动转化,使大气中滞留了更多的云水,暖云降水减小;另一方面,云水的增加会使冰相粒子,尤其是雪和霰通过碰并云水等过程而增大,最后融化成雨增加冷云降水,同时冰相粒子增加会释放更多的潜热,促进上升气流的发展,进一步增加冷云降水。气溶胶对降水的影响存在空间不一致性,暖云较厚的地方暖雨过程受到的抑制明显,使地面降水减小,冷云厚度相对较厚时,冷云降水的增加会大于暖云降水的抑制,使地面降水增加。同时由于在云降水发展的不同阶段冷暖云的变化,气溶胶对降水的影响也存在着时间不一致性。 相似文献
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1.引言控制对流云和地形云增雨的主要因子包括目标云和播撒(或催化)物质的特有性能.对于冷云播撤,成核剂的关键的可变因素包括核化机制、核化时间速率和产量(或成核率).在被催化的云中,有效的核化时间可能十分短促.对流云中上升气流使气溶胶粒子 相似文献
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在UWyo单组分气溶胶的绝热气块分档云模式基础上,发展了多种化学组分气溶胶的绝热气块分档云模式。利用2006年春季华北地区地面气溶胶分级采样的离子成分分析数据和同时段高空气溶胶、云微物理飞机观测资料,研究了气溶胶混合状态对暖云微物理特征的影响。模拟结果表明,华北地区气溶胶内部混合比外部混合有利于增加云凝结核数浓度、降低气块水汽最大饱和比、增加云滴数浓度。气溶胶的混合状态不同,形成的云滴谱的特征差异较大,主要体现在云滴谱的平均尺度和峰值的突出程度;云滴谱相对离散度在0.3附近变化,且随着云滴数浓度的增加,云滴谱相对离散度呈现减小的趋势。气溶胶混合状态能够影响暖云微物理特征,从而影响大气辐射和降水过程,在天气和气候变化的研究中应予以关注。 相似文献
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云模式中气溶胶物理过程参数化方案研究概述 总被引：2，自引：1，他引：2
介绍了大气气溶胶的浓度、气溶胶的谱形等物理性质对云的微物理过程造成的影响以及目前云模式中常用到的一些气溶胶物理过程的体积水、分档等参数化方案，并评述了这些参数化方案各自的特点。提出了在设计气溶胶物理过程参数化方案时需要注意和有待解决的几个问题，建议在设计气溶胶-云相互作用的模式时，要根据不同的研究目的选择合适的参数化方案。 相似文献
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《中国气象科学研究院年报》2011,(1):39-45
2011年,云降水物理与人工影响天气研究主要在暖云数值模式研制及模拟、云物理过程对降水影响、冰雹物理过程、效果检验、南方冻雨的微物理过程以及华北气溶胶特征等方面取得如下研究成果。 相似文献
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In-Jin Choi Takamichi Iguchi Sang-Woo Kim Teruyuki Nakajima Soon-Chang Yoon 《Meteorology and Atmospheric Physics》2014,123(3-4):181-194
This study performed a three-dimensional regional-scale simulation of aerosol and cloud fields using a meso-scale non-hydrostatic model with a bin-based cloud microphysics. The representation of aerosols in the model has been improved to account for more realistic multi-modal size distribution and multiple chemical compositions. Two case studies for shallow stratocumulus over Northeast Asia in March 2005 were conducted with different aerosol conditions to evaluate model performance. Improved condensation nuclei (CN) and cloud condensation nuclei (CCN) are attributable to the newly constructed aerosol size distribution. The simulated results of cloud microphysical properties (cloud droplet effective radius, liquid water path, and optical thickness) with improved CN/CCN number are close to the retrievals from satellite-based observation. The effects of aerosol on the microphysical properties of shallow stratocumulus are investigated by model simulation, in terms of columnar aerosol number concentration. Enhanced aerosol number concentration results in increased liquid water path in humid case, but invariant liquid water path in dry case primarily due to precipitation occurrence. The changes of cloud microphysical properties are more predominant for small aerosol burden than for large aerosol burden with the retarded changes in cloud mass and size due to inactive condensation and collision-coalescence processes. Quantitative evaluation of sensitivity factor between aerosol and cloud microphysical properties indicates a strong aerosol-cloud interaction in Northeast Asian region. 相似文献
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2016年11月13日在北京地区上空存在持续稳定的层状云天气背景下,利用飞机开展气溶胶粒径谱、化学组成、云滴谱等参量的垂直观测,研究该个例云底气溶胶的活化能力。结果表明:探测期间北京地区为轻度污染天气,地面气溶胶浓度(0.11~3 μm)达到4600 cm-3。云层高度为800~1200 m,云底气溶胶数浓度相对于近地面大幅度降低,有效粒径显著增大(0.3~0.6 μm)。同时,近地面气溶胶中疏水性的一次有机气溶胶贡献显著,而云底气溶胶中一次有机气溶胶的贡献大幅降低,无机组分和二次有机气溶胶的贡献明显增大,造成吸湿性参数κ由0.25(地面)增大至0.32(云底)。云中气溶胶和云滴的谱分布衔接较好,且两者的数浓度之和与云底气溶胶浓度一致,可分别代表未活化和已活化的粒子。基于云底气溶胶粒径谱和吸湿性参数计算得到不同过饱和比下云凝结核的活化率,通过与云中观测结果对比,反推得到云底过饱和度约为0.048%。 相似文献
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一次秋季冷锋降水过程气溶胶与云粒子分布的飞机观测 总被引：2，自引：1，他引：1
利用机载PMS（Particle Measuring Systems）测量系统,对2008年10月4—5日石家庄地区一次冷锋降水云系的3次气溶胶和云粒子探测资料进行了分析。结果表明,冷锋过境降水前后,气溶胶粒子分布差异较大。降水发生前,气溶胶粒子平均数浓度约为103cm-3,平均直径为0.95μm;气溶胶主要集中于3000m高度以下的对流层低层,云内气溶胶数浓度明显减少。降水发生后,气溶胶粒子平均数浓度约为102cm-3,比降水前约小1个量级,平均直径为1.28μm;气溶胶主要集中于1200m以下的近地面层,其数浓度随高度增加而降低。气溶胶粒子浓度在低层云区内水平变化较小,而在无云区和云下近地层水平起伏较大。云粒子平均浓度比气溶胶小1～2个量级。气溶胶粒子平均谱主要呈双峰型,而云粒子谱主要为单峰型。 相似文献
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通过分析中国近海MODIS数据中气溶胶参数与云参数的相互关系,讨论了该区域气溶胶的间接效应及其对于云的可能影响.结果表明,在中国近海,气溶胶具有明显的间接效应,而且由于气溶胶种类和水汽的季节变化,使得气溶胶的间接作用具有很强的时间变化特征.在夏季,由于人为气溶胶占主导,它作为有效的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）有正相关、与云滴有效半径（CER）有负相关性、与云光学厚度（COT）也存在着正相关,气溶胶的间接效应明显;在春季,由于沙尘气溶胶盛行,同时沙尘并不是很好的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）的正相关减弱、与云滴有效半径（CER）则由夏季的负相关变为正相关、与云光学厚度（COT）存在弱的负相关,气溶胶的间接效应不明显. 相似文献
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K. N. Bower T. W. Choularton M. W. Gallagher R. N. Colvile K. M. Beswick D. W. F. Inglis C. Bradbury B. G. Martinsson E. Swietlicki O. H. Berg S. -I. Cederfelt G. Frank J. Zhou J. N. Cape M. A. Sutton G. G. McFadyen C. Milford W. Birmili B. A. Yuskiewicz A. Wiedensohler F. Stratmann M. Wendisch A. Berner P. Ctyroky Z. Galambos S. H. Mesfin U. Dusek C. J. Dore D. S. Lee S. A. Pepler M. Bizjak B. Divjak 《Atmospheric Research》1999,50(3-4)
During March and April of 1995 a major international field project was conducted at the UMIST field station site on Great Dun Fell in Cumbria, Northern England. The hill cap cloud which frequently envelopes this site was used as a natural flow through reactor to examine the sensitivity of the cloud microphysics to the aerosol entering the cloud and also to investigate the effects of the cloud in changing the aerosol size distribution, chemical composition and associated optical properties. To investigate these processes, detailed measurements of the cloud water chemistry (including the chemistry of sulphur compounds, organic and inorganic oxidised nitrogen and ammonia), cloud microphysics and properties of the aerosol and trace gas concentrations upwind and downwind of the cap cloud were undertaken. It was found that the cloud droplet number was generally strongly correlated to aerosol number concentration, with up to 2000 activated droplets cm−3 being observed in the most polluted conditions. In such conditions it was inferred that hygroscopic organic compounds were important in the activation process. Often, the size distribution of the aerosol was substantially modified by the cloud processing, largely due to the aqueous phase oxidation of S(IV) to sulphate by hydrogen peroxide, but also through the uptake and fixing of gas phase nitric acid as nitrate, increasing the calculated optical scattering of the aerosol substantially (by up to 24%). New particle formation was also observed in the ultrafine aerosol mode (at about 5 nm) downwind of the cap cloud, particularly in conditions of low total aerosol surface area and in the presence of ammonia and HCl gases. This was seen to occur at night as well as during the day via a mechanism which is not yet understood. The implications of these results for parameterising aerosol growth in Global Climate Models are explored. 相似文献
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Yuan WANG Jonathan M.VOGEL Yun LIN Bowen PAN Jiaxi HU Yangang LIU Xiquan DONG Jonathan H.JIANG Yuk L.YUNG Renyi ZHANG 《大气科学进展》2018,35(2):234-247
Aerosol–cloud–radiation interactions represent one of the largest uncertainties in the current climate assessment. Much of the complexity arises from the non-monotonic responses of clouds, precipitation and radiative fluxes to aerosol perturbations under various meteorological conditions. In this study, an aerosol-aware WRF model is used to investigate the microphysical and radiative effects of aerosols in three weather systems during the March 2000 Cloud Intensive Observational Period campaign at the US Southern Great Plains. Three simulated cloud ensembles include a low-pressure deep convective cloud system, a collection of less-precipitating stratus and shallow cumulus, and a cold frontal passage. The WRF simulations are evaluated by several ground-based measurements. The microphysical properties of cloud hydrometeors, such as their mass and number concentrations, generally show monotonic trends as a function of cloud condensation nuclei concentrations.Aerosol radiative effects do not influence the trends of cloud microphysics, except for the stratus and shallow cumulus cases where aerosol semi-direct effects are identified. The precipitation changes by aerosols vary with the cloud types and their evolving stages, with a prominent aerosol invigoration effect and associated enhanced precipitation from the convective sources. The simulated aerosol direct effect suppresses precipitation in all three cases but does not overturn the aerosol indirect effect. Cloud fraction exhibits much smaller sensitivity(typically less than 2%) to aerosol perturbations, and the responses vary with aerosol concentrations and cloud regimes. The surface shortwave radiation shows a monotonic decrease by increasing aerosols, while the magnitude of the decrease depends on the cloud type. 相似文献
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Jefferson R. Snider Jean&#;Louis Brenguier 《Tellus. Series B, Chemical and physical meteorology》2000,52(2):828-842
During the 2nd Aerosol Characterization Experiment (ACE‐2), relationships between stratocumulus cloud properties and aerosols were examined. Here, the relevant measurements including the cloud condensation nuclei (CCN) activation spectrum, updraft velocity, cloud microphysical and aerosol properties are presented. It is shown that calculations of droplet concentration based on updraft velocity and the CCN activation spectrum are consistent with direct observations. Also discussed is an apparent disparity among measurements of the CCN activation spectrum, the accumulation mode size distribution, and the composition of the submicrometric aerosol. The observed consistency between CCN, updraft and cloud droplets is a necessary refinement; however, extended analyses of the ACE‐2 data set are needed to guide improvements in model simulations of the interaction between aerosols and cloud microphysics. In particular, there is need for an examination of aerosol size spectra and chemical composition measurements with a view towards validating droplet activation schemes which relate the aerosol and cloud dynamical properties to cloud albedo. 相似文献
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对流云对大气气溶胶和相对湿度变化响应的数值模拟 总被引：6，自引：3，他引：3
利用二维面对称分档云模式研究了气溶胶颗粒物浓度和尺度谱分布对混合相对流云微物理过程和降水的影响, 并重点讨论了气溶胶效应随环境相对湿度的变化。结果表明, 在初始热力和动力条件相同的情况下, 相对清洁的海洋性云在发展和成熟阶段能更有效地产生雨滴、 冰晶和霰粒, 形成更强的雷达反射率。随着气溶胶浓度增加, 比如在本文模拟的污染大陆性云中, 气溶胶粒子数浓度的增加限制云滴增长, 不利于降水粒子的形成。模拟结果也发现, 环境相对湿度对气溶胶效应有显著影响, 即当地面相对湿度从50%增大到70%时, 所模拟的云从浅对流泡发展为深对流云; 气溶胶对云微物理特性和降水的影响在干空气中较小, 但在湿空气中表现非常显著, 这与前人结果一致。随着相对湿度的增加, 冰相粒子出现的时间提前, 增长加快, 云砧范围扩大, 但相对来说, 降水起始时间对相对湿度的变化比气溶胶更敏感。 相似文献
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N. E. Veremei Yu. A. Dovgalyuk V. Gopalakrishnan K. F. Komarovskikh P. Murugavel S. D. Pawar A. A. Sinkevich 《Russian Meteorology and Hydrology》2015,40(12):777-786
Studied are the effects of severe aerosol pollution of the atmosphere on the parameters of a cumulonimbus cloud (including its charge structure) and on precipitation. Considered is the example of the cloud that developed on May 11, 2009 near the town of Kharagpur (India) under conditions of severe aerosol pollution of the atmosphere due to dust transport from the desert. The in situ observations of the evolution of the cumulonimbus cloud of large vertical and horizontal extent and of its electric conditions were carried out on that day. It is found that the distribution of electric charges in the cloud was characterized by inverted polarity (i.e., the main positive charge is in the bottom of the cloud and the negative one is in the upper part of the cloud that contradicts usually observed cases). Using the small-dimension numerical model conducted are numerical experiments on the simulation of aerosol effects produced on the evolution of dynamic, microphysical, and electric structure of the cloud under study, namely, the cloud development under background conditions and in case of high aerosol concentration. It is assumed that aerosol particles possess ice-forming properties. It is obtained that the dynamic, microphysical, and electric structures of the cloud are significantly transformed under the influence of high aerosol concentrations; precipitation generation also significantly intensifies; polarity in the distribution of electric charge varies that agrees with the data of in situ observations. 相似文献
20.
Frank Drewnick Johannes Schneider Silke S. Hings Nele Hock Kevin Noone Admir Targino Silke Weimer Stephan Borrmann 《Journal of Atmospheric Chemistry》2007,56(1):1-20
The Aerodyne aerosol mass spectrometer (Q-AMS) was coupled with a counterflow virtual impactor (CVI) for the first time to measure cloud droplet residuals of warm tropospheric clouds on Mt. Åreskutan in central Sweden in July 2003. Operating the CVI in different operational modes generated mass concentration and species-resolved mass distribution data for non-refractory species of the ambient, interstitial, and residual aerosol. The ambient aerosol measurements revealed that the aerosol at the site was mainly influenced by long-range transport and regional photochemical generation of nitrate and organic aerosol components. Four different major air masses were identified for the time interval of the experiment. While two air masses that approached the site from northeastern Europe via Finland showed very similar aerosol composition, the other two air masses from polar regions and the British Islands had a significantly different composition. During cloud events the larger aerosol particles were found to be activated into cloud droplets. On a mass basis the activation cut-off diameter was approximately 150 nm for nitrate and organics dominated particles and 200 nm for sulfate dominated particles. Generally nitrate and organics were found to be activated into cloud droplets with higher efficiency than sulfate. While a significant fraction of the nitrate in ambient particles was organic nitrates or nitrogen-containing organic species, the nitrate found in the cloud droplet residuals was mainly ammonium nitrate. After passage of clouds the ambient aerosol size distribution had shifted to smaller particle sizes due to the predominantly activation of larger aerosol particles without a significant change in the relative composition of the ambient aerosol. 相似文献