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1.
This study explores the influence of air gaseous pollutants–aerosols and solar zenith angle (SZA) on the spectral diffuse-to-direct beam E dλ/E bλ irradiances ratio. It does so using ground-based spectroradiometric measurements taken over the Athens atmosphere during May 1995. It was found that the spectral E dλ/E bλ ratio decreases rapidly with increasing wavelength and regression curves of the form E dλ/E bλ = aλ?b fitted the experimental data. These curves are strongly modified by aerosols–air pollutants, aerosol optical properties, and SZA. The log–log plot of E dλ/E bλ versus λ reveals a significant departure from linearity, which is likely to be associated with aerosol physical properties and SZA effects. The effect of atmospheric turbidity, as expressed through the aerosol optical at 500 nm and SZA on the spectral E dλ/E bλ ratio, is investigated in detail for two discernible atmospheric conditions observed in the urban Athens atmosphere. The first case includes different atmospheric turbidity levels under the same SZA, while the second corresponds to different SZA values under the same turbidity levels. It was found that the correlation between E dλ/E bλ and spectral aerosol optical depth can be a useful tool in determining the aerosol optical properties and aerosol types composition.  相似文献   

2.
The analysis of time series of the Linke turbidity factors is performed for the atmosphere mass m = 2 (T 2) and atmospheric aerosol optical thickness for the wavelength λ0 = 0.55 μm (AOT) from the data of 14 actinometrical stations of Central Siberia and Trans-Baikal territory. It is shown that over the period from 1976 to 2006, the increased atmospheric transparency is observed in the region. Quantitative estimates of changes in multiyear mean annual variations of T 2 and AOT at different periods of averaging and for different time periods are derived.  相似文献   

3.
In-water and remote measurements of ocean color   总被引：2，自引：0，他引：2  
Spectral measurements of downwelling irradiance, E d(), above the surface, and of upwelling irradiance just below the surface, E u(), allow computation of spectral values of the diffuse reflectance R() = E u()/E d(); this yields full information about the true color and brightness of the ocean. Typical results are presented and interpreted for waters very different in turbidity and phytoplankton content. Conversely, the possibility of infering the water content from R() data at selected wavelengths is examined in terms of the respective number of equations and unknowns. The necessary use of assumptions and of empirical laws is emphasized.The magnitude of the useful signal emerging from the water, and the magnitude of the additional signals due to specular reflexion at the interface and to atmospheric scattering, are compared on the basis of spectroradiometric measurements performed within and above the sea, from different altitudes. These unwanted signals are dominant, causing a drastic change in the spectral composition of the light received by a remote sensor. The evaluation of the atmospheric effect must be very precise in order to recover the marine signal with a sufficient accuracy for a meaningful application of any kind of algorithm.This work was supported in part by the Centre National d'Exploitation des Océans (under contract CNEXO 77/1695) and in part by the Centre National de la Recherche Scientifique (RCP 247 & ERA 278).  相似文献   

4.
An 8-wavelength sun-photometer has been operated at Hefei (31.31°N, 117.17°E) to monitoroptical properties of atmospheric aerosols. Altogether 133 solar spectral extinction data were ob-tained on clear days during the period from September 1993 through September 1994, In this pa-per, the feature of the sun-photometer is briefly described. A relative aureole method is intro-duced. which can be used to monitor temporal evolution of aerosol loading during the sun-pho-tometer calibration period. Temporal variabilities of spectral aerosol optical depths and Angstromturbidity parameters are presented. Relation of these variabilities with synoptic and local meteoro-logical conditions are analyzed and discussed, From measured spectral aerosol optical depths undersome representative atmospheric conditions, columnar aerosol size distributions have been retrievedby a linearly constrained inversion method. These typical columnar aerosol size distributions are al-so presented and discussed.  相似文献   

5.
The actinic flux is the only radiometric quantity suitable for photolysisfrequency determination. It is derived from solar spectral irradiancemeasurements performed by a portable spectroradiometer in the 300–850nm wavelength range. The spectral irradiance is first divided into a directpart and a diffuse part, according to the atmospheric conditions, and thenconverted into the corresponding actinic flux quantity. As an intermediary,the ratio of diffuse actinic flux to diffuseirradiance is calculated by the spherical harmonics radiative code withrespect to wavelength, solar zenith angle, surface albedo, and aerosolproperties.The results of extensive sensitivity studies of asa function of the main atmospheric parameters are discussed and lead to theconclusion that aerosol optical depth is the major critical value for aprecise determination. The global algorithm totransform spectral irradiance into actinic flux is finally applied forphotodissociation rate calculations by convolution of the obtained actinicflux spectra with the absorption cross-sections and quantum yields of themolecule studied. Photolysis rates of different atmospheric photooxidants havebeen measured with this spectroradiometric method during the summers of 1993and 1994 in Brittany and in Portugal. The ozone and nitrogen dioxidephotodissociation rates obtained present a good agreement with thej(O3) and j(NO2) actinometerresults, for the same experimental conditions in Brittany.  相似文献   

6.
The equivalent wavelength ( λ E), at which the aerosol optical depth (AOD) is equal to broadband AOD (BAOD), can change in a wide range from 0.619 μm to 1.575 μm in the usual aerosol conditions. By using the least squares technique and some empirical corrections, a parameterized relationship of λ E with BAOD, Ångström wavelength exponent ( α ), solar zenith angle ( θ 0) and H2O amount is developed. Using this relationship, and based on the strong sensitivity of BAOD on θ 0 when θ 0>70°, the broadband extinction method to derive the spectral AOD and α is further proposed. As shown in comparative simulations to retrieve AOD by the present, Molineaux et al. and Gueymard methods, the present method has the best accuracy in most simulations using Junge, MODTRAN, log‐normal and Deirmendjian aerosol models. A key question of the pyrheliometer method to determine wavelength-dependent AODs is the effect of uncertainty in the aerosol size istribution. It is found that the AOD solution around λ E is less sensitive to the uncertainty. The wavelength exponent α is derived using an assumption of the stable atmospheric turbidity. If the pyrheliometer data from θ 0=85° to 70° are used and the change of the turbidity is ±10%, the error of solution α is usually within ±0.32. If the variation of the turbidity is random, the mean value of a lot of the measurements of α would be very reasonable.  相似文献   

7.
Trend analysis of rainfall time series for Sindh river basin in India   总被引：1，自引：1，他引：0  
The main goal of this paper is to estimate a set of optimal seasonal, daily, and hourly values of atmospheric turbidity and surface radiative parameters Ångström’s turbidity coefficient (β), Ångström’s wavelength exponent (α), aerosol single scattering albedo (ωo), forward scatterance (Fc) and average surface albedo (ρg), using the Brute Force multidimensional minimization method to minimize the difference between measured and simulated solar irradiance components, expressed as cost functions. In order to simulate the components of short-wave solar irradiance (direct, diffuse and global) for clear sky conditions, incidents on a horizontal surface in the Metropolitan Area of Rio de Janeiro (MARJ), Brazil (22° 51′ 27″ S, 43° 13′ 58″ W), we use two parameterized broadband solar irradiance models, called CPCR2 and Iqbal C, based on synoptic information. The meteorological variables such as precipitable water (uw) and ozone concentration (uo) required by the broadband solar models were obtained from moderate-resolution imaging spectroradiometer (MODIS) sensor on Terra and Aqua NASA platforms. For the implementation and validation processes, we use global and diffuse solar irradiance data measured by the radiometric platform of LabMiM, located in the north area of the MARJ. The data were measured between the years 2010 and 2012 at 1-min intervals. The performance of solar irradiance models using optimal parameters was evaluated with several quantitative statistical indicators and a subset of measured solar irradiance data. Some daily results for Ångström’s wavelength exponent α were compared with Ångström’s parameter (440–870 nm) values obtained by aerosol robotic network (AERONET) for 11 days, showing an acceptable level of agreement. Results for Ångström’s turbidity coefficient β, associated with the amount of aerosols in the atmosphere, show a seasonal pattern according with increased precipitation during summer months (December–February) in the MARJ.  相似文献   

8.
Measured Spectra of Solar Ultraviolet Irradiances at Athens Basin, Greece   总被引：1，自引：0，他引：1  
Summary From a data archive of spectral energy distribution of global and diffuse solar irradiances measured in Athens during a field experiment, the impacts of changes in solar zenith angle, site altitude, and gaseous-aerosol pollutants loading, on spectral composition of ultraviolet (UV) radiation reaching the ground, has been determined for cloudless conditions. Measurements of spectral energy distribution of ultraviolet irradiance showed that in urban atmospheres there is a significant altitude effect on spectral UV irradiances which is more pronounced on shorter wavelength UVB than on longer wavelength UVA. In particular the largest attenuation in the UVB band, produced by the altitude effect, between the non-urban site of Mt. Hymettus and the urban site of Athens Museum, was about 27%; while the corresponding attenuation in the UVA band reached 20%. Correspondingly, the respective attenuation caused by altitude effect in the diffuse UVB band was 12%; whereas the altitude effect increases UVA band to as much as 9% between the summit of Mt. Hymettus and the urban site of Athens Museum. Depletion of UV irradiances by the urban atmosphere of downtown Athens was strongly related to aerosol-gaseous pollutants loading. The spectral UV measurements were found to be sensitive to both, changes in solar zenith angle and atmospheric turbidity. The spectral ratio of diffuse-to-direct irradiance critically depends on both solar zenith angle and aerosol-gaseous pollutants loading, increasing rapidly toward the shorter wavelengths. Finally, the hypothesis that the increased levels of aerosol-gaseous pollutants may act as a filter to the transfer of UV energy to the ground is supported, by the limited set of spectral measurements used in the present work. Received June 16, 1996 Revised April 18, 1997  相似文献   

9.
Broadband solar irradiance data obtained in the spectral range 400–940 nm at Kwangju, South Korea from 1999–2000 have been analyzed to investigate the effects of cloud cover and atmospheric optical depth on solar radiation components. Results from measurements indicate that the percentage of direct and diffuse horizontal components of solar irradiance depend largely on total optical depth (TOD) and cloud cover. During summer and spring, the percentages of diffuse solar irradiance relative to the global irradiance were 5.0% and 4.9% as compared to 2.2% and 3.0% during winter and autumn. The diffuse solar irradiance is higher than the direct in spring and summer by 24.2%, and 40.6%, respectively, which may largely be attributed to the attenuation (scattering) of radiation by heavy dust pollution and large cloud amount. In cloud-free conditions with cloud cover ≤2/10, the fraction of the direct and diffuse components were 66.0% and 34.0%, respectively, with a mean daily global irradiance value of 7.92±2.91 MJ m−2 day−1. However, under cloudy conditions (with cloud cover ≥8/10), the diffuse and direct fractions were 97.9% and 2.2% of the global component, respectively. The annual mean TOD under cloudless conditions (cloud cover≤2/10) yields 0.74±0.33 and increased to as much as 3.15±0.67 under cloudy conditions with cloud amount ≥8/10. An empirical formula is derived for estimating the diffuse and direct components of horizontal solar irradiance by considering the total atmospheric optical depth (TOD). Results from statistical models are shown for the estimation of solar irradiance components as a function of TOD with sufficient accuracy as indicated by low standard error for each solar zenith angle (SZA).  相似文献   

10.
曹丽青  高国栋 《气象科学》2004,24(2):185-192
本文采用太阳短波辐射分光谱模式计算了我国太阳辐射收支各分量。模式中主要考虑及计算了大气中各种成份在不同谱区对太阳辐射的吸收和衰减作用。如水汽、均匀混和气体的红外吸收，紫外和可见光区的臭氧吸收、雷利散射及大气气溶胶的削弱作用等。给出了大气中各种成份在不同波段对太阳辐射的削弱。并且分析了我国太阳辐射收支各分量1月、7月的分布特征。模式误差在4％～10％，比较理想。为无辐射观测的高原、沙漠、海洋等地区提供了一种较好的计算方法。  相似文献   

11.
Summary ¶Aerosol optical depth (a) is the most comprehensive variable to characterize aerosol, assess atmospheric pollution and make atmospheric corrections to satellite remotely sensed data from ground-based instruments. The aerosol optical properties in Korea peninsula observed at both Kwangju and Anmoyondo during the Asian dust period (March–May) have been presented in this study. Aerosol optical depths at all wavelengths showed a sharp increase during major dust outbreak in spring when compared with the average for the season. For example at Kwangju, aerosol optical depths increase from the spring average value of 0.43±0.02 at 501nm to values >0.70 during major dust event days in 1999 and 2001. Daily mean Ångström exponents () computed at both sites show dramatic changes from high values to low values on dust day periods with a sharp increase in the single scattering albedo. The study also revealed that the observed direct normal solar irradiance and diffuse horizontal irradiance during days with increased dust pollution levels is capable of reducing direct solar radiation by as much as 28% and a corresponding increase of 14% in diffuse solar irradiance during cloudless and windless days.  相似文献   

12.
太阳直接辐射的分光测量   总被引：2，自引：1，他引：2  
利用热电式相对日射表和八种有色玻璃滤光片,于1975—1978年先后在我国七个地区(共十个测点)进行了太阳分光辐射的测量,获得了2698组资料。根据这些资料,分析了太阳高度、季节、地理纬度和海拔高度以及气溶胶和水汽等大气成份对各波段的太阳分光辐射的影响。最后,用大气质量、浑浊度系数和地面绝对湿度三个物理量作参数,以表格的形式列出了各波段分光辐射的相对通量值。  相似文献   

13.
The present study deals with the aerosol optical properties which are assessed during the period 2007 to 2009 over Mohal (31.9oN, 77.12oE) in the northwestern Indian Himalaya, using ground-based measurements and multi-satellite data. The daily average value of aerosol optical depth (AOD) at 500?nm, ?ngstr?m exponent and turbidity coefficient are 0.24?±?0.08, 1.02?±?0.34 and 0.13?±?0.05, respectively. The comparative study of satellite and ground-based measurements reveals that the percentage retrieval for daily AOD at 550?nm over Mohal within the expected accuracy (???? p?? ?=?±0.05?±?0.15?? p?? ) is around 87%, with a significant correlation coefficient of 0.76. The present study suggests that the retrieval of AOD through satellite data is able to characterise the distribution of AOD over Mohal. However, further efforts are needed in order to eliminate systematic errors in the existing Moderate Resolution Imaging Spectroradiometer (MODIS) algorithm. The transport of desert dust and anthropogenic aerosol during high aerosol loading days caused a significant reduction in surface-reaching solar radiation by 149 and 117%, respectively. This large reduction in surface-reaching solar radiation increased the atmospheric heating rate by 0.93 and 0.72?K?day?1, respectively. This study indicates significant climatic implications due to the transport of aerosols in the northwestern Indian Himalaya.  相似文献   

14.
Ice samples from the 905 m deep Dome C core (East Antarctica) were studied in terms of insoluble microparticle contents. Various techniques were used: right angle light scattering, nephelometer (multiangle light scattering), Coulter counter and microscope analyses, in order to make a thorough study of the physical and optical properties of microparticles and their variations over the last 30000 years. Because of the possible effect of atmospheric turbidity on the earth-atmosphere radiation balance, optical parameters of climatic importance were estimated for insoluble microparticles. The detailed profile of total microparticle mass concentrations shows a drastic (factor of 17 ± 13) difference between high Last Glacial Maximum (LGM) and low Holocene concentrations. The optical scattering properties of 18000 BP continental dust do not indicate a significant difference with respect to Holocene dust in terms of particle size distribution and complex refractive index. The number to log radius size distribution of microparticles for the entire 30 000 yr period can be fitted by a log-normal distribution with two parameters (modal radius 0.25 ± 0.08 μm; geometric standard deviation 2.2. ± 0.2). However, for the smallest particles a better adjustment between experimental and theoretical scattering diagrams is obtained by adding to the observed size distribution another log-normal distribution (modal radius = 0.025 μm, σ g = 2). The complex refractive index is 1.53 to 1.56 for the real part and 0.005 ± 0.005 for the imaginary part at the wavelength used (λ= 546 nm). During the LGM stage, over the whole of Antarctica, the change in the total optical depth due to the drastic change in the insoluble aerosol loading is small because insoluble impurities are not the dominant aerosol component. It may have produced a slight warming of the snow surface (≈ 2 K). In the dust source regions, the optical depth would have been a maximum of 2 to 4 times the present value. The possible warming of the atmosphere in these regions is estimated at 3 K per day and should therefore be taken into account in paleoclimate reconstruction models.  相似文献   

15.
临安与龙凤山辐射数据质量及初步结果比较   总被引：1，自引：1，他引：0       下载免费PDF全文
采用国际通用的辐射数据质量评估方法对2005—2011年浙江临安、黑龙江龙凤山两个区域大气本底站辐射观测资料进行质量评估与比较分析。结果表明:两站辐射数据通过物理可能限制检验与极端罕见限制检验的百分比均超过99.5%,但通过相关要素比较限制检验的百分比上,临安与龙凤山站分别降至97.9%与95.9%;双轴定位追踪太阳出现偏差是造成直接辐射与散射辐射数据精度降低的主要原因。CM21表的热偏移在-5 W·m-2以内,而其进行热偏移订正可以显著提高数据的通过率。对应同一太阳天顶角,临安站晴空总辐射与直接辐射均低于龙凤山站,散射辐射则相反,其原因是临安的大气透明系数较低,大气浑浊度较高。2006—2011年,临安站的大气向下长波辐射呈下降趋势,达到了0.01的显著性水平,且其多年平均值 (363.7±59.3 W·m-2) 显著高于龙凤山站 (274.9±77.6 W·m-2);龙凤山站晴空太阳总辐射呈增加趋势,达到了0.1的显著性水平。  相似文献   

16.
This paper deals with the atmospheric concentrations of PM5 and PM2.5 particulate matter and its water soluble constituents along with the size distribution of ions and spatial variation at three different residential environments in a semiarid region in India. Samples were collected from the indoors and outdoors of urban, rural and roadside sites of Agra during October 2007–March 2008. The mean concentrations of PM2.5 indoors and outdoors were 178 μgm−3 and 195 μgm−3 while the mean concentrations of PM5 indoors and outdoors were 231.8 μgm−3 and 265.2 μgm−3 respectively. Out of the total aerosol mass, water soluble constituents contributed an average of 80% (33% anions, 50% cations) in PM5 and 70% (29% anions, 43% cations) in PM2.5. The indoor–outdoor ratio of water soluble components suggested additional aerosol indoor sources at rural and roadside sites. Indoor–outdoor correlations were also determined which show poor relationships among concentrations of aerosol ions at all three sites. Univariate Pearson correlation coefficients among water soluble aerosols were determined to evaluate the relationship between aerosol ions in indoor and outdoor air.  相似文献   

17.
我国的大气透明状况   总被引：4，自引：1，他引：4  
王炳忠  潘根娣 《气象学报》1982,40(4):443-452
根据全国65个甲种日射站自建站起至1978年9:30,12:30,15:30各时次直接辐射的观测资料,计算了大气透明系数。为了便于各地间的比较和绘制全国分布图,所有各时次的资料都统一订正到M=2的情况下,计算中太阳常数取值S_0=1.98卡厘米~(-2)分~(-1)。 就我国的具体情况而论,地势对大气透明度的影响最为显著,直接的结果是:高原为透明度高值区,盆地为低值区。 分析了影响大气透明度的两个重要因子——水汽和气溶胶的分布特点,以及它们之间的比例关系。水汽对辐射的吸收系根据探空资料求得的整层大气的含水量按Mugge和Muller的公式计算的。  相似文献   

18.
Summary Using the HITRAN database from 2003, the absorption of solar and thermal radiation by the atmosphere is calculated. The results are presented in the form of spectral densities of absorption yield of the atmosphere and its components, and fractions of absorbed energy of the solar radiation and thermal radiation in the atmosphere by each of its components separately and together. Finally, the obtained results are discussed in the context of the lately published model of Earth’s radiation budget-MAP 85(4), 275–281 (2004). The shares of atmospheric components in the greenhouse effect and in the absorption of solar radiation are calculated. The percentage contributions of the more important atmospheric components in the greenhouse effect are as follows: clouds 66, water vapor 25, CO2 6.7, N2O 0.7, CH4 0.7.  相似文献   

19.
Summary In addition to global solar radiationE g , the hourly diffuse componentE d incident on a horizontal surface has been measured from February 1993 to January 1995 at a meteorological station in tropical West Africa. The measured diffuse solar irradiance data was corrected for shadow band effects. The monthly mean diurnal variations of diffuse solar irradiance obtained for identical months in the two years have been compared and found to be generally consistent. The corresponding monthly mean hourly values ofE d for identical months in 1993 and 1994 agreed to within 9% while yielding correlation coefficients greater than 0.960. In addition, the monthly mean daily totals ofE d for identical months were found to agree mostly to within 6% and showed virtually the same annual variations in both years. The monthly mean daily total values of diffuse solar radiation for most months in the two years ranged between 7.94 MJm–2d–1 and 10.50 MJm–2d–1. The monthly mean of daily hourly maximum values ofE d obtained for identical months in the two years have been discussed in relation to the dominant atmospheric conditions during these months. The results been presented here have been compared with those of some investigators within and outside the Africa region.With 8 Figures  相似文献   

20.
This study aims at evaluating the variability of the optical properties of chromophoric dissolved organic matter (CDOM) of rainwater during the cold season, specifically between Autumn and Winter periods. The spectroscopic characteristics of rainwater samples collected at a town (Aveiro) in western Portugal were assessed by UV-Vis absorbance and three-dimensional excitation-emission matrix (EEM) fluorescence spectroscopies. Rainwater samples showed similar characteristics to those of natural humic substances when analysed by UV-Vis absorbance spectroscopy, but a significant difference was observed in the volume weight average (VWA) of absorbances between Autumn and Winter. In general, the EEM fluorescence spectra of the Autumn and Winter samples disclosed the presence of six fluorophores with different VWA specific fluorescence intensities: three humic-like (λ excitation/λ emission ≈ 230/415 nm; 290/415 nm; and 340/415 nm) and three protein-like (λ excitation/λ emission ≈ 230/350 nm; 280/340 nm; and 225/300 nm), but one of the humic-like peaks (≈340/415 nm) does not always appear in the EEM fluorescence spectra of the Winter samples. During the cold season, chromophoric compounds are important constituents of rainwater dissolved organic matter and the presence of these highly absorbing and fluorescing compounds may exert a determining effect in atmospheric absorption of solar radiation.  相似文献   

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