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1.
The dynamics of terrestrial ecosystems depends on interactions between carbon, nutrient and hydrological cycles. Terrestrial ecosystems retain carbon in live biomass (aboveground and belowground), decomposing organic matter, and soil. Carbon is exchanged naturally between these systems and the atmosphere through photosynthesis, respiration, decomposition, and combustion. Human activities change carbon stock in these pools and exchanges between them and the atmosphere through land-use, land-use change, and forestry.In the present study we estimated the wood (stem) biomass, growing stock (GS) and carbon stock of Indian forests for 1984 and 1994. The forest area, wood biomass, GS, and carbon stock were 63.86 Mha, 4327.99 Mm3, 2398.19 Mt and 1085.06 Mt respectively in 1984 and with the reduction in forest area, 63.34 Mha, in 1994, wood biomass (2395.12 Mt) and carbon stock (1083.69 Mt) also reduced subsequently. The Conifers, of temperate region, stocked maximum carbon in their woods, 28.88 to 65.21 t C ha−1, followed by Mangrove forests, 28.24 t C ha−1, Dipterocarp forests, 28.00 t C ha−1, and Shorea robusta forests, 24.07 t C ha−1. Boswellia serrata, with 0.22 Mha forest area, stocked only 3.91 t C ha−1. To have an idea of rate of carbon loss the negative changes (loss of forest area) in forest area occurred during 1984–1994 (10yrs) and 1991–1994 (4yrs) were also estimated. In India, land-use changes and fuelwood requirements are the main cause of negative change. Total 24.75 Mt C was lost during 1984–1994 and 21.35 Mt C during 1991–94 at a rate of 2.48 Mt C yr−1 and 5.35 Mt C yr−1 respectively. While in other parts of India negative change is due to multiple reasons like fuelwood, extraction of non-wood forest products (NWFPs), illicit felling etc., but in the northeastern region of the country shifting cultivation is the only reason for deforestation. Decrease in forest area due to shifting cultivation accounts for 23.0% of the total deforestation in India, with an annual loss of 0.93 Mt C yr−1.  相似文献   

2.
Increased Carbon Sink in Temperate and Boreal Forests   总被引:6,自引:0,他引:6  
An intense search is under way to identify the `missing sink' in the world carbon budget of perhaps 2 Pg year–1 (petagrams, or billiontonnes) of carbon, but its location and mechanism have proved elusive. Here we use a new forest inventory data set to estimate the carbon sink and the carbon pool of woody biomass in 55 countries that account for nearly all temperate or boreal forests and approximately half the world's total forest area. In each country there was a net accumulation of biomass; together, the carbon sink of woody biomass was 0.88 Pg year–1 during the 1990swith estimated uncertainty from 0.71 to 1.1 Pg year–1. Thisestimate, already about half of the missing sink, would probably be even larger if carbon accumulation in soil and detritus were also accounted for, but we are unable to quantify that additional sink. The sink is twice that estimated for the woody biomass of these forests a decade ago due to higher estimates for tree growth throughout the region and decreased timber harvests in Russia. In contrast, the new data indicate a carbon pool that is smaller than earlier estimates because of improved data for Russia and Australia.  相似文献   

3.

The expected growth in the demand for passenger and freight services exacerbates the challenges of reducing transport GHG emissions, especially as commercial low-carbon alternatives to petroleum fuels are limited for shipping, air and long-distance road travel. Biofuels can offer a pathway to significantly reduce emissions from these sectors, as they can easily substitute for conventional liquid fuels in internal combustion engines. In this paper, we assess the potential of bioenergy to reduce transport GHG emissions through an analysis leveraging various integrated assessment models and scenarios, as part of the 33rd Energy Modeling Forum study (EMF-33). We find that bioenergy can contribute a significant, albeit not dominant, proportion of energy supply to the future transport sector: in scenarios aiming to keep the temperature increase below 2 °C by the end of the twenty-first century, models project that in 2100 bioenergy can provide on average 42 EJ/yr (ranging from 5 to 85 EJ/yr) for transport (compared to 3.7 EJ in 2018), mainly through lignocellulosic fuels. This makes up 9–62% of final transport energy use. Only a small amount of bioenergy is projected to be used in transport through electricity and hydrogen pathways, with a larger role for biofuels in road passenger transport than in freight. The association of carbon capture and storage (CCS) with bioenergy technologies (BECCS) is a key determinant in the role of biofuels in transport, because of the competition for biomass feedstock to provide other final energy carriers along with carbon removal. Among models that consider CCS in the biofuel conversion process the average market share of biofuels is 21% in 2100 (ranging from 2 to 44%), compared to 10% (0–30%) for models that do not. Cumulative direct emissions from the transport sector account for half of the emission budget (from 306 to 776 out of 1,000 GtCO2). However, the carbon intensity of transport decreases as much as other energy sectors in 2100 when accounting for process emissions, including carbon removal from BECCS. Lignocellulosic fuels become more attractive for transport decarbonization if BECCS is not feasible for any energy sectors. Since global transport service demand increases and biomass supply is limited, its allocation to and within the transport sector is uncertain and sensitive to assumptions about political as well as technological and socioeconomic factors.

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4.
The soil C balance is determined by the difference between inputs (e.g., plant litter, organic amendments, depositional C) and outputs (e.g., soil respiration, dissolved organic C leaching, and eroded C). There is a need to improve our understanding of whether soil erosion is a sink or a source of atmospheric CO2. The objective of this paper is to discover the long-term influence of soil erosion on the C cycle of managed watersheds near Coshocton, OH. We hypothesize that the amount of eroded C that is deposited in or out of a watershed compares in magnitude to the soil C changes induced via microbial respiration. We applied the erosion productivity impact calculator (EPIC) model to evaluate the role of erosion–deposition processes on the C balance of three small watersheds (∼1 ha). Experimental records from the USDA North Appalachian Experimental Watershed facility north of Coshocton, OH were used in the study. Soils are predominantly silt loam and have developed from loess-like deposits over residual bedrock. Management practices in the three watersheds have changed over time. Currently, watershed 118 (W118) is under a corn (Zea mays L.)–soybean (Glycine max [L.] Merr.) no till rotation, W128 is under conventional till continuous corn, and W188 is under no till continuous corn. Simulations of a comprehensive set of ecosystem processes including plant growth, runoff, and water erosion were used to quantify sediment C yields. A simulated sediment C yield of 43 ± 22 kg C ha−1 year−1 compared favorably against the observed 31 ± 12 kg C ha−1 year−1 in W118. EPIC overestimated the soil C stock in the top 30-cm soil depth in W118 by 21% of the measured value (36.8 Mg C ha−1). Simulations of soil C stocks in the other two watersheds (42.3 Mg C ha−1 in W128 and 50.4 Mg C ha−1 in W188) were off by <1 Mg C ha−1. Simulated eroded C re-deposited inside (30–212 kg C ha−1 year−1) or outside (73–179 kg C ha−1 year−1) watershed boundaries compared in magnitude to a simulated soil C sequestration rate of 225 kg C ha−1 year−1 and to literature values. An analysis of net ecosystem carbon balance revealed that the watershed currently under a plow till system (W128) was a source of C to the atmosphere while the watersheds currently under a no till system (W118 and W188) behaved as C sinks of atmospheric CO2. Our results demonstrate a clear need for documenting and modeling the proportion of eroded soil C that is transported outside watershed boundaries and the proportion that evolves as CO2 to the atmosphere.  相似文献   

5.
The biomass carbon (C) stock of forests is one of key parameters for the study of regional and global carbon cycles. Literature reviews shows that inventory-based forest C stocks documented for major countries in the middle and high northern latitudes fall within a narrow range of 36–56 Mg C ha−1 with an overall area-weighted mean of 43.6 Mg C ha−1. These estimates are 0.40 to 0.71 times smaller than those (61–108 Mg C ha−1) used in previous analysis of balancing the global carbon budget. A statistical analysis, using the global forest biomass database, implies that aboveground biomass per hectare is proportional to forest mean height [biomass in Mg/ha = 10.63 (height in m)] in closed-canopy forests in the study regions, indicating that forest height can be a proxy of regional biomass C stocks. The narrow range of C stocks is likely a result of similar forest height across the northern regions. The lower biomass C stock obtained in this study strongly suggests that the role of the northern forests in the global carbon cycle needs to be re-evaluated. Our findings also suggest that regional estimates of biomass could be readily made from the use of satellite methods such as lidar that can measure forest canopy height over large regions.  相似文献   

6.
A three-step methodology to assess the carbon sequestration and the environmental impact of afforestation projects in the framework of the Flexible Mechanisms of the Kyoto Protocol (Joint Implementation and Clean Development Mechanism) was developed and tested using a dataset collected from the Jonkershoek forest plantation, Western Cape, South Africa, which was established with Pinus radiata in former native fynbos vegetation and indigenous forest. The impact of a change in land use was evaluated for a multifunctional, a production and a non-conversion scenario. First, the carbon balance was modelled with GORCAM and was expressed as (1) C sequestration in tC ha−1 year−1 in soil, litter, and living biomass according to the rules of the first commitment period of the Kyoto Protocol, and (2) CO2 emission reductions in tC ha−1 year−1, which includes carbon sequestered in the above-mentioned pools and additionally in wood products, as well as emission reductions due to fossil fuel substitution. To estimate forest growth, three data sources were used: (1) inventory data, (2) growth simulation with a process-based model, and (3) yield tables. Second, the effects of land use change were assessed for different project scenarios using a method related to Life Cycle Assessment (LCA). The method uses 17 quantitative indicators to describe the impact of project activities on water, soil, vegetation cover and biodiversity. Indicator scores were calculated by comparing indicator values with reference values, estimated for the climax vegetation. The climax vegetation is the site-specific ecosystem phase with the highest exergy content and the highest exergy flow dissipation capacity. Third, the land use impact per functional unit of 1 tC sequestered was calculated by combining the results of step 1 and step 2. The average baselines to obtain carbon additionality are 476 tC ha−1 for indigenous forest and 32 tC ha−1 for fynbos. Results show that the influence of the growth assessment method on the magnitude of C sequestration and hence on the environmental impact per functional unit is large. When growth rate is assessed with the mechanistic model and with the yield table, it is overestimated in the early years and underestimated in the long term. The main conclusion of the scenario analysis is that the production forest scenario causes higher impacts per functional unit than the multifunctional scenario, but with the latter being less efficient in avoiding CO2 emissions. The proposed method to assess impacts on diverse components of the ecosystem is able to estimate the general tendency of the adverse and positive effects of each scenario. However, some indicators, more specifically about biodiversity and water balance, could be improved or reinterpreted in light of specific local data about threat to biodiversity and water status.  相似文献   

7.
《Climate Policy》2013,13(4):319-333
Abstract

This paper discusses the results of the BEAP linear programming model that has been developed to study the optimal use of biomass and land for greenhouse gas emission reduction, notably the competition between food production, biomass production for energy and materials and afforestation. The model results suggest up to 100 EJ biomass use in case of global policies (about 20% of global primary energy use). The biomass is used for industrial and residential heating, transportation fuels and as a feedstock for plastics. In the electricity markets competing emission reduction options are more cost-effective than biomass. In case the Kyoto protocol is continued beyond 2010 the developed countries can rely in 2020–2030 on afforestation and land use change credits from developing countries, without any major use of other emission reduction strategies. However, in case of a planning perspective of more than half a century bioenergy is preferred instead of afforestation. The results indicate a limited impact on global agricultural trade, but food demand may be affected by CO2 policies.  相似文献   

8.
The study reports estimates of above ground phytomass carbon pools in Indian forests for 1992 and 2002 using two different methodologies. The first estimate was derived from remote sensing based forest area and crown density estimates, and growing stock data for 1992 and 2002 and the estimated pool size was in the range 2,626–3,071 Tg C (41 to 48 Mg C ha???1) and 2,660–3,180 Tg C (39 to 47 Mg C ha???1) for 1992 and 2002, respectively. The second methodology followed IPCC 2006 guidelines and using an initial 1992 pool of carbon, the carbon pool for 2002 was estimated to be in the range of 2,668–3,112 Tg C (39 to 46 Mg C ha???1), accounting for biomass increment and removals for the period concerned. The estimated total biomass increment was about 458 Tg over the period 1992–2002. Removals from forests include mainly timber and fuel wood, whereby the latter includes large uncertainty as reported extraction is lower than actual consumption. For the purpose of this study, the annual extraction values of 23 million m3 for timber and 126 million m3 for fuel wood were used. Out of the total area, 10 million ha are plantation forests with an average productivity (3.2 Mg ha???1 year???1) that is higher than natural forests, a correction of 408 Tg C for the 10 year period was incorporated in total estimated phytomass carbon pool of Indian forests. This results in an estimate for the net sink of 4 Tg C year???1. Both approaches indicate Indian forests to be sequestering carbon and both the estimates are in agreement with recent studies. A major uncertainty in Indian phytomass carbon pool dynamics is associated with trees outside forests and with soil organic carbon dynamics. Using recent remote-sensing based estimates of tree cover and growing stock outside forests, the estimated phytomass carbon pool for trees outside forests for the year 2002, is 934 Tg C with a national average tree carbon density of 4 Mg C ha???1 in non-forest area, in contrast to an average density of 43 Mg C ha???1 in forests. Future studies will have to consider dynamics in both trees outside forests and soil for total terrestrial carbon dynamics.  相似文献   

9.
Improving our ability to predict the impact of climate change on the carbon (C) balance of boreal forests requires increased understanding of site-specific factors controlling detrital and soil C accumulation. Jack pine (Pinus banksiana) and black spruce (Picea mariana) stands along the Boreal Forest Transect Case Study (BFTCS) in northern Canada have similar C stocks in aboveground vegetation and large woody detritus, but thick forest floors of poorly-drained black spruce stands have much higher C stocks, comparable to living biomass. Their properties indicate hindered decomposition and N cycling, with high C/N ratios, strongly stratified and depleted δ13C and δ15N values, high concentrations of tannins and phenolics, and 13C nuclear magnetic resonance (NMR) spectra typical of poorly decomposed plant material, especially roots and mosses. The thinner jack pine forest floor appears to be dominated by lichen, with char in some samples. Differences in quantity and quality of aboveground foliar and woody litter inputs are small and unlikely to account for the contrasts in forest floor accumulation and properties. These are more likely associated with site conditions, especially soil texture and drainage, exacerbated by increases in sphagnum coverage, forest floor depth, and tannins. Small changes in environmental conditions, especially reduced moisture, could trigger large C losses through rapid decomposition of forest floor in poorly drained black spruce stands in this region.  相似文献   

10.
This paper presents carbon flux estimates arising from the effect of increasing demand on harvests and management of industrial forests in a global timber market. Results are presented for specific regions and the globe. Harvests and management of forests are predicted to store an additional 184 Tg (1 Tg = 1012 grams) of carbon per year in forests and wood products over the next 50 years, with a range of 108 to 251 Tg per year. Although harvests in natural boreal and tropical forest regions will cause carbon releases, new plantation establishment in subtropical emerging regions more than offsets these losses. Unlike many existing studies, these results suggest that harvests and management of North American forests will lead to carbon emissions from that region over the next 50 years. The results are quantitatively sensitive to the assumed growth in demand although the results are qualitatively similar in the sensitivity analysis.  相似文献   

11.
Above- and below-ground biomass values for 17 types of grassland communities in China as classified by the Chinese Grasslands Resources Survey were obtained from systematic replicated sampling at 78 sites and from published records from 146 sites. Most of the systematic samples were along a 5,000-km-long transect from Hailar, Inner Mongolia (49°15′N, 119°15′E), to Pulan, Tibet (30°15′N, 81°10′E). Above-ground biomass was separated into stem, leaf, flower and fruit, standing dead matter, and litter. Below-ground biomass was measured in 10-cm soil layers to a depth of 30 cm for herbs and to 50 cm for woody plants. Grassland type mean total biomass carbon densities ranged from 2.400 kg m−2 for swamp to 0.149 kg m−2 for alpine desert grasslands. Ratios of below- to above-ground carbon density varied widely from 0.99 for tropical tussock grassland to 52.28 for alpine meadow. Most below-ground biomass was in the 0–10 cm soil depth layer and there were large differences between grassland types in the proportions of living and dead matter and stem and leaf. Differences between grassland types in the amount and allocation of biomass showed patterns related to environments, especially aridity gradients. Comparisons of our estimates with other studies indicated that above-ground biomass, particularly forage-yield biomass, is a poor predictor of total vegetation carbon density. Our estimate for total carbon storage in the biomass of the grasslands of China was 3.32 Pg C, with 56.4% contained in the grasslands of the Tibet-Qinghai plateau and 17.9% in the northern temperate grasslands. The need for further standardized and systematic measurements of vegetation biomass to validate global carbon cycles is emphasised.  相似文献   

12.
Sea level rise (SLR) is among the climate-change-related problems of greatest concern, threatening the lives and property of coastal residents and generating far-reaching economic and ecological impacts. We project that SLR will lead to an increase in the rate of new housing construction to replace destroyed structures, impact global wood products supply and demand conditions, and cause changes in global forest sector carbon mitigation potential. Findings indicate that 71 million new units will be built by 2050 to accommodate the SLR-affected global population. More than two-thirds of these new units are projected to be in Asia. The estimated extra wood products needed to build these new residential units is 1,659 million m3, assuming that all these structures would be built mainly with wood, representing a 4 % increase in total wood consumption, compared to projected reference level global wood products consumption. Increased timber removals to meet this higher construction wood demand (alternative scenario) is shown to deplete global forest carbon by 2 % by 2050 compared to the reference scenario. However, all such projected declines in forest biomass carbon could be more than offset by increased carbon sequestration in harvested wood products, avoided emissions due to substitution of wood for non-wood materials in construction, and biomass regrowth on forestland by 2050, with an estimated net emissions reduction benefit of 0.47 tCO2e/tCO2e of extra wood used in SLR-related new houses over 30 years. The global net emissions reduction benefit increased to 2.13 tCO2e/tCO2e of extra wood when price-induced changes in forest land area were included.  相似文献   

13.
This study investigates the use of bioenergy for achieving stringent climate stabilization targets and it analyzes the economic drivers behind the choice of bioenergy technologies. We apply the integrated assessment framework REMIND-MAgPIE to show that bioenergy, particularly if combined with carbon capture and storage (CCS) is a crucial mitigation option with high deployment levels and high technology value. If CCS is available, bioenergy is exclusively used with CCS. We find that the ability of bioenergy to provide negative emissions gives rise to a strong nexus between biomass prices and carbon prices. Ambitious climate policy could result in bioenergy prices of 70 $/GJ (or even 430 $/GJ if bioenergy potential is limited to 100 EJ/year), which indicates a strong demand for bioenergy. For low stabilization scenarios with BECCS availability, we find that the carbon value of biomass tends to exceed its pure energy value. Therefore, the driving factor behind investments into bioenergy conversion capacities for electricity and hydrogen production are the revenues generated from negative emissions, rather than from energy production. However, in REMIND modern bioenergy is predominantly used to produce low-carbon fuels, since the transport sector has significantly fewer low-carbon alternatives to biofuels than the power sector. Since negative emissions increase the amount of permissible emissions from fossil fuels, given a climate target, bioenergy acts as a complement to fossils rather than a substitute. This makes the short-term and long-term deployment of fossil fuels dependent on the long-term availability of BECCS.  相似文献   

14.
In this study, an improved and complete secondary organic aerosols (SOA) chemistry scheme was implemented in the CHIMERE model. The implementation of isoprene chemistry for SOA significantly improves agreement between long series of simulated and observed particulate matter concentrations. While simulated organic carbon concentrations are clearly improved at elevated sites by adding the SOA scheme, time correlation are impaired at low level sites in Portugal, Italy and Slovakia. At several sites a clear underestimation by the CHIMERE model is noticed in wintertime possibly due to missing wood burning emissions as shown in previous modeling studies. In Europe, the CHIMERE model gives yearly average SOA concentrations ranging from 0.5 μg m  − 3 in the Northern Europe to 4 μg m  − 3 over forested regions in Spain, France, Germany and Italy. In addition, our work suggests that during the highest fire emission periods, fires can be the dominant source of primary organic carbon over the Mediterranean Basin, but the SOA contribution from fire emissions is low. Isoprene chemistry has a strong impact on SOA formation when using current available kinetic schemes.  相似文献   

15.
Aerosol and rain samples were collected between 48°N and 55°S during the KH-08-2 and MR08-06 cruises conducted over the North and South Pacific Ocean in 2008 and 2009, to estimate dry and wet deposition fluxes of atmospheric inorganic nitrogen (N). Inorganic N in aerosols was composed of ~68% NH4+ and ~32% NO3 (median values for all data), with ~81% and ~45% of each species being present on fine mode aerosol, respectively. Concentrations of NH4+ and NO3 in rainwater ranged from 1.7–55 μmol L−1 and 0.16–18 μmol L−1, respectively, accounting for ~87% by NH4+ and ~13% by NO3 of total inorganic N (median values for all data). A significant correlation (r = 0.74, p < 0.05, n = 10) between NH4+ and methanesulfonic acid (MSA) was found in rainwater samples collected over the South Pacific, whereas no significant correlations were found between NH4+ and MSA in rainwater collected over the subarctic (r = 0.42, p > 0.1, n = 6) and subtropical (r = 0.33, p > 0.5, n = 6) western North Pacific, suggesting that emissions of ammonia (NH3) by marine biological activity from the ocean could become a significant source of NH4+ over the South Pacific. While NO3 was the dominant inorganic N species in dry deposition, inorganic N supplied to surface waters by wet deposition was predominantly by NH4+ (42–99% of the wet deposition fluxes for total inorganic N). We estimated mean total (dry + wet) deposition fluxes of atmospheric total inorganic N in the Pacific Ocean to be 32–64 μmol m−2 d−1, with 66–99% of this by wet deposition, indicating that wet deposition plays a more important role in the supply of atmospheric inorganic N than dry deposition.  相似文献   

16.
Using a single drop experiment, the uptake of NO3 radicals on aqueous solutions of the dye Alizarin Red S and NaCl was measured at 293 K. Uptake coefficients in the range (1.7–3.1) ⋅ 10− 3 were measured on Alizarin Red S solutions. The uptake coefficients measured on NaCl solutions were in the range of (1.1–2.0) ⋅ 10−3 depending on the salt concentration. Both experiments lead to a consistent result for the mass accommodation coefficient of αNO3 = (4.2− 1.7+2.2)⋅ 10−3. The product H(Dl kClII)0.5 for the NO3 radical was determined to be (1.9 ± 0.2) M atm− 1 cm s−0.5 M−0.5 s−0.5 by fitting the uptake data for the NaCl solutions to the so-called resistance model. The yield of the chemical NO3 radical source was characterized using UV-VIS and FT-IR spectroscopy. The amount of gas-phase NO3 radicals measured at elevated humidities was less than expected. Instead, a rise of the gas-phase HNO3 concentration was found indicating a conversion of gas-phase NO3 radicals to gas-phase HNO3 on the moist reactor walls.  相似文献   

17.
The characteristics of net radiation (Rn)(0.3--10 μm) in Lhasa and Haibei in the Tibetan Plateau were analyzed based on long-term in-situ measurements of surface radiation data. The monthly average of daily Rn reached a minimum during the winter period followed by an increase until May and then a decline until January. This variation is consistent with solar activity. The annual mean daily total Rn values were 0.92 MJ m-2 d-1 and 0.66 MJ m-2d-1 in Lhasa and Haibei, respectively. A relationship between Rn and broadband solar radiation (Rs) was demonstrated by a good linear correlation at the two sites. Rn can be an accurate estimate from Rs. The estimated Rn values were similar to the observed values, and the relative deviations between the estimates and measurements of Rn were 2.8% and 3.8% in Lhasa and Haibei, respectively. The application of the Rn estimating model to other locations showed that it could provide acceptable estimated Rn values from the Rs data. Furthermore, we analyzed the influence of clouds on Rn by different clear index (Ks), defined as the ratio of Rs to the extraterrestrial solar irradiance on a horizontal surface. The results indicate that more accurate results are associated with increased cloudy conditions. The influence of the albedo was also considered, but its inclusion in the model resulted in only a slight improvement. Because surface albedo is not usually measured, an expression based solely on global solar radiation could be of more extensive use.  相似文献   

18.
Increased precipitation during the vegetation periods was observed in and further predicted for Inner Mongolia. The changes in the associated soil moisture may affect the biosphere-atmosphere exchange of greenhouse gases. Therefore, we set up an irrigation experiment with one watered (W) and one unwatered plot (UW) at a winter-grazed Leymus chinensis-steppe site in the Xilin River catchment, Inner Mongolia. UW only received the natural precipitation of 2005 (129 mm), whereas W was additionally watered after the precipitation data of 1998 (in total 427 mm). In the 3-hour resolution, we determined nitrous oxide (N20), methane (CH4) and carbon dioxide (CO2) fluxes at both plots between May and September 2005, using a fully automated, chamber-based measuring system. N20 fluxes in the steppe were very low, with mean emissions (±s.e.) of 0.9-4-0.5 and 0.7-4-0.5 μg N m^-2 h^-1 at W and UW, respectively. The steppe soil always served as a CH4 sink, with mean fluxes of -24.1-4-3.9 and -31.1-4- 5.3 μg C m^-2 h^-1 at W and UW. Nighttime mean CO2 emissions were 82.6±8.7 and 26.3±1.7 mg C m^-2 h^-1 at W and UW, respectively, coinciding with an almost doubled aboveground plant biomass at W. Our results indicate that the ecosystem CO2 respiration responded sensitively to increased water input during the vegetation period, whereas the effects on CH4 and N2O fluxes were weak, most likely due to the high evapotranspiration and the lack of substrate for N2O producing processes. Based on our results, we hypothesize that with the gradual increase of summertime precipitation in Inner Mongolia, ecosystem CO2 respiration will be enhanced and CH4 uptake by the steppe soils will be lightly inhibited.  相似文献   

19.
Generally, it is assumed that UV-light, high temperature or reactive molecules like O3 and OH are needed to activate gas reactions in air. In consequence, the catalytic activity on natural materials such as sand and soil on the earth's surface is assumed to be insignificant. We have measured O2-dissociation rates on natural quartz sand at 40˚C and compared these with O2-dissociation rates near 500˚C on materials with well-known catalytic activity. In terms of probabilities for dissociation of impinging O2-molecules the measured rates are in the 10−12–10−4 range. We have also measured dissociation rates of H2 and N2, water-formation from H2 and O2 mixtures, exchange of N between N2, NO x and a breakdown of HNO3, NO2 and CH4 on natural quartz sand at 40˚C. The measured rates together with an effective global land area have been used to estimate the impact of thermodynamically driven reactions on the earth's surface on the global atmospheric budgets of H2, NO2 and CH4. The experimental data on natural quartz sand together with data from equilibrium calculations of air suggest that an expected increase in anthropogenic supply of air pollutants, such as NO x or other “reactive” nitrogen compounds, hydrogen and methane, will be counter-acted by catalysis on the earth's surface. On the other hand, at Polar Regions and boreal forests where the “reactive” nitrogen concentration is below equilibrium, the same catalytic effect activates formation of bio-available nitrogen compounds from N2, O2 and H2O.  相似文献   

20.
Rainfall variability and kinetic energy in Southern Nigeria   总被引:1,自引:1,他引:0  
A decreasing trend of rainfall has been observed in West Africa, where rainfall erosivity is also considered to be high. Therefore, this study was carried out to evaluate the variability of rainfall and its erosivity in two contrasting zones in southern Nigeria between 1977 and 1999 to understand the implications of climate variability on rainfall erosivity. The study sites were Ibadan, a sub-humid zone, and Port-Harcourt, a humid zone. Time of occurrence of rainfall, rainfall amount (A), intensity (I 15 and I 30), kinetic energy (E) and rainfall erosivity factor (R), were evaluated. Kinetic energy was estimated with Brown–Foster (BF) equation, making the rainfall erosivity (product of kinetic energy and intensity) to be designated as EI 30-BF and EI 15-BF. The frequency of rainfall during daylight (06:00–18:00 h) was 48% for Ibadan and 69% for Port-Harcourt. There were time-specific differences in daily rainfall occurrence between the zones, suggesting a strong influence of local effects on rainfall generation, such as, relief in Ibadan and proximity to the sea in Port-Harcourt. Annual E was 213 MJ ha−1for Ibadan and 361 MJ ha−1 for Port-Harcourt. Ibadan had a significantly higher daily E than Port-Harcourt because of higher intensity while Port-Harcourt had significantly higher annual E than Ibadan because of higher annual rainfall amount. Annual erosivity at Ibadan using the EI 30-BF was 9,742 MJ mm ha−1 h−1 whereas it was 15,752 MJ mm ha−1 h−1 at Port-Harcourt. Using the EI 15-BF, Ibadan had an annual value of 14,806 MJ mm ha−1 h−1 while Port-Harcourt had 20,583 MJ mm ha−1 h−1. Thus, annual rainfall erosivity was significantly higher in the humid than the sub-humid zone because of higher amount of rainfall but the reverse was the case with daily erosivity because of higher intensities in the sub-humid zone. Rainfall intensity was, therefore, a key measure of erosivity. There was a strong positive relationship between rainfall erosivity and rainfall amount. Between 1977 and 1988, 50–88% of the 12 years had rainfall erosivity which exceeded the long-term average but rainfall erosivity was less than the long-term average between 1989 and 1999. This suggested a decreasing trend in erosivity due to the decreasing trend in rainfall amount in West Africa. However, the trend did not imply lesser soil erosion and environmental degradation risks.  相似文献   

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