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1.
The temporal variability of the chemical composition of surface aerosol with particle diameters of 0.7–2 μm is analyzed. This analysis is based on the results of measurements of infrared transmission spectra of aerosol samples collected with the use of a cascade impactor at the Zvenigorod Scientific Station of the Institute of Atmospheric Physics (IAP) in 1999–2005. Seasonal features of the aerosol chemical composition and its dependence on the particle size are revealed. The interdiurnal variability of the aerosol composition depends on the season, and it manifests itself more strongly in winter and spring. Air-mass changes lead to changes in the relation of sulfates and nitrates in the micron fraction of aerosol. The enrichment of samples in nitrates is especially characteristic of the winter and spring seasons. Compounds containing the NO2 group are often met in the samples of aerosol with particle sizes of 0.7–1.3 μm during the cold time of the year. The estimates of the optical thickness of micron aerosol in the sulfate absorption band are obtained, and optical-thickness variations of some scales are detected. The quantitative characteristics of statistical relations between different chemical components of aerosol inside individual fractions and between chemical components of the micron and submicron fractions are obtained and analyzed.  相似文献   

2.
Asymptotics for the mass concentration of finely dispersed aerosol are obtained on the basis of in situ measurements in a desert in the Caspian region and estimates of hydrodynamic parameters in the viscous thermal boundary layer near the soil surface. In the problem under consideration, the dynamic velocity (friction speed) and the temperature drop in the thermal boundary layer are external parameters. The model of a porous soil layer, in which the air dynamics is described with the use of the Darcy equation, is considered a possible mechanism of aerosol export. The estimates of the critical parameters at which sand particles thermally roll over in soil pores are obtained.  相似文献   

3.
We studied the temperature variations of the lower air layer caused by dust content using a dust storm in Dushanbe in November 2007 as an example. Quantitative estimates of air cooling and a decrease in the diurnal temperature difference due to a diminishing horizontal visibility range are given. Observations of air temperature variations due to the dust content of the atmosphere in an arid zone are presented. The critical value of aerosol concentration for toggling between the greenhouse and antigreenhouse effects is determined. The long-term effect of dust aerosol on climate is analyzed.  相似文献   

4.
A method for reconstructing the parameters of postvolcanic stratospheric aerosol from the results of joint measurements of the aerosol backscattering coefficient with lidar systems based on the Nd:YAG laser and the aerosol extinction coefficient with the SAGE III satellite instrumentation is developed. The most informative set of optical characteristics is determined for each of the microphysical parameters under consideration (concentration, surface area, volume, and effective size of particles of the fine and coarse aerosol fractions). Multiple polynomial regressions between optical and microphysical characteristics of aerosol are obtained. These regressions make it possible to determine the microphysical characteristics of aerosol within a wide range without solving incorrect inverse problems. The results are compared with independent experimental data. The errors of reconstructing microphysical parameters of aerosol are estimated for different situations in the stratosphere. The influence of the shape of particles of the dust fraction on the results of a reconstruction of the microphysical parameters of aerosol is considered.  相似文献   

5.
利用MODIS气溶胶产品中550nm气溶胶光学厚度和小颗粒比例两个参数的关系,直接计算得到我国海域人为和沙尘气溶胶光学厚度,并对人为和沙尘气溶胶的分布进行了分析,结果表明:在我国海域,利用550nm气溶胶光学厚度和小颗粒比例的关系直接计算人为和沙尘气溶胶光学厚度是可行的;我国海域的人为和沙尘气溶胶光学厚度有明显的时空变化.人为气溶胶在春夏季最大,而在秋冬季最小;沙尘气溶胶在冬春季最大,而在夏秋季最小.在该海域人为和沙尘气溶胶光学厚度有显著的空间变化,在纬向上,人为气溶胶光学厚度在30°~45°N达到最大值,向南北递减;沙尘气溶胶光学厚度在33°~40°N最大,在其他纬度都很小.在经向上,人为气溶胶光学厚度与离岸距离有关,在沿海120°E处最大,随着经度增加而减小.沙尘作为大颗粒气溶胶,传输距离小,所以它只是在120°~123°E出现最大值,在其他经度处都很小.  相似文献   

6.
This paper first describes the atmospheric correction algorithm for OCTS visible band data used at NASDA/EOC. Sharing a basic structure with Gordon and Wang’s Sea WiFS algorithm, it uses 10 candidate aerosol models including the “Asian dust model” introduced in consideration of the unique feature of aerosols over the east Asian waters. Based on the observations at 670 and 865 nm bands, the algorithm selects a pair of aerosol models that account best for the observed spectral reflectances, and synthesizes the aerosol reflectance used for the atmospheric correction. Two different schemes for determining the value of the parameter for the aerosol model selection are presented and their anticipated estimation error is analyzed in terms of retrieved water reflectance at 443 nm. The results of our numerical simulation show that the standard deviation of the estimation error of the “weighted average” scheme is mostly within the permissible level of ±0.002, reducing the error by 18% on average compared to the “simple average” scheme. The paper further discusses the expected error under the old CZCS-type atmospheric correction, which assumes constant aerosol optical properties throughout the given image. Although our algorithm has a better performance than the CZCS algorithm, further analysis shows that the error induced by the assumption taken in the algorithm that the water-leaving radiance at 670 nm band is negligibly small may be large in high pigment concentration waters, indicating the necessity for future improvements.  相似文献   

7.
During a cruise aboard the R/V Hakuho-maru in the northwestern North Pacific in the summer of 1998 the particle number concentrations and the major ionic components of size fractionated aerosols were measured to investigate the aerosol produced by marine biological activity. Continuous low concentrations of nitrate (<1.8 nmol m−3), similar to the marine air background level, were found over the northwestern North Pacific (40–45°N) and the Sea of Okhotsk (44–45°N). Over the Sea of Okhotsk, a high concentration of chlorophyll-a (5.4 mg m−3) in seawater was observed, and atmospheric concentrations of non sea-salt (nss-) sulfate (44 nmol m−3), methane sulfonic acid (MSA) (1.8 nmol m−3) and particle number in the size range of 0.1 < D < 0.5 μm (199 cm−3) were found to be 9, 7, and 2 times, respectively, higher than those in the background marine air. The increase in particle number concentrations mainly in the size range of 0.2 < D < 0.3 μm was likely caused by the increase of biogenic sulfate over the high productive region of the Sea of Okhotsk. In humid air conditions (R.H. > 96%), the increased biogenic sulfate that condensed the large amount of water vapor would not have sufficient solute mass to activate as cloud condensation nuclei (CNN) and would remain as aerosol particles in the marine air with frequent sea-fogs over the high productive region. Biogenic sulfate originating from dimethyl sulfide (DMS) would gradually grow into the CCN size and continuously supply a great number of CCN to the marine air in the northwestern North Pacific. This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

8.
The Chinese desert is one of the major sources of atmospheric mineral dust transported for a long distance to the North Pacific by the atmospheric circulation. The characteristic of the aerosol in the North Pacific is smilar to that of the aerosol in North China with a considerable concentration of mineral in spring due to the large-scale dust storm occurring in North China. The study of isotope tracer indicates that the concentration of Al is significantly related to 210Pb, suggesting that the mineral aerosol in the North Pacific may origir ate from the desert in Northwest China by using air mass trajectory analysis. About 6-12×106 tons of Chinese desert mineral dust per year would be transported to the North Pacific.  相似文献   

9.
对海面目标物的目视观察，其能见距离与观测方向、海面背景光谱辐射、目标物固有光谱辐射和大气分子及气溶胶的光学参数等因素有密切关系。本文从理论上分析各种因素的影响，特别是研究了海面背景辐射对目标物光谱对比度的作用。推导出不同观测方向下目标物光谱对比度的计算公式。作为例子，给出海面上黑色物体的光谱对比度公式，也给出海面目标“被隐蔽”的条件。  相似文献   

10.
The results of a numerical simulation of the action of hygroscopic particles on a warm convective cloud with the purpose of obtaining additional precipitation are presented. The one-dimensional numerical model considered in this work describes the evolution of the cloud medium in the central part of an axisymmetric convective cloud at the specified height-variable velocity of the upward air flow which forms the cloud. Our model comprehensively describes microphysical processes in the cloud medium with the use of the kinetic equation for the size distribution of cloud droplets. This model makes it possible to obtain the spatiotemporal pattern of the cloud formation and development and to analyze regular features in the cloud evolution under the action of hygroscopic reagents. The cloud characteristics calculated with the use of this model correspond to the cloud parameters observed in natural conditions of the atmosphere. The process of precipitation stimulation by hygroscopic particles in convective clouds with vertical thicknesses of 2.5–4.5 km was analyzed on the basis of the results of numerical calculations. The results of calculations of the dependence of the intensity and total amount of precipitation on the vertical cloud thickness and parameters of particles introduced into the cloud are presented. It is shown that hygroscopic particles with root-mean-cube radii of 1–1.5 μm are the most effective for acting on warm convective clouds with the purpose of obtaining additional precipitation. In this case, the required reagent expenditure is 100–200 kg/km2. The conditions necessary for obtaining the maximal positive effect of the action are elucidated.  相似文献   

11.
The results of simultaneous investigations of atmospheric aerosol in two large megalopolises—Moscow and Beijing—are presented. The purpose of these investigations was to compare parameters and reveal common characteristics of urban aerosols. Aerosol parameters were measured in the megalopolises simultaneously from October 23, 2007, through November 2, 2007. The mass concentrations of aerosols were measured continuously with a nephelometer (Mosscow) and discretely with the use of aspiration samplers according to the weight method (Moscow, Beijing). The number concentration and the particle size distribution function were determined with analyzers of the size spectrum in the interval 0.15–15.0 μm and were measured synchronously with sampling for elementary analysis. The elementary compositions of samples were determined by mass spectrometry, which made it possible to identify 60 chemical elements.  相似文献   

12.
The solar radiation flux incident on the land surface and aerosol radiative forcing are calculated from measurements carried out under clear skies during the summers of 2004 and 2005 at the Zvenigorod Scientific Station (ZSS) of the A.M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences. In these calculations, the following five models of aerosol optical parameters are used: a standard model of continental aerosol, a semiempirical model based on measurement data, and three models obtained from calculations on the basis of the Mie scattering theory for the mean size distribution of aerosol particles (which is retrieved from aureole measurements). A study of the sensitivity of the flux and forcing to the choice of aerosol model has shown that the relative error related to the model choice is not large (<5%) for the incident radiation flux and reaches 120% for aerosol forcing at the atmospheric upper boundary. The aerosol radiative forcing at the atmospheric upper boundary is also estimated and, according to our calculations, varies from −15 to −2 W/m2. The use (in calculations) of the values of the albedo of single-scattering and the factor of scattering-indicatrix asymmetry at a wavelength of 550 nm, which were obtained for each of the observation periods, has made it possible to significantly refine the value of aerosol radiative forcing (compared to that calculated for the means of these parameters over all the periods). An even more accurate determination of aerosol radiative forcing is possible only when data on the size-distribution of aerosol particles and their chemical composition for a certain situation under analysis are available. As a result of this study, two models of the optical parameters of background aerosol have been proposed for use in radiation calculations: a semiempirical model and a mean model obtained from the calculations based on the theory of scattering. Both models use the values of the albedo of single scattering and the factor of asymmetry (at a wavelength of 550 nm) retrieved from the measurements for each of the observation periods.  相似文献   

13.
Measurement results of downward longwave radiation (DLR) in a wavelength range of 3.5?C50 ??m are considered which have been obtained with the use of a precision IR radiometer (Eppley pyrgeometer) of the PIR model at the Meteorological Observatory of Moscow State University in 2008?C2010. The influence of air temperature and atmospheric moisture content on the DLR values has been analyzed; correlations between DLR and the above parameters have been found. The effect of clouds on DLR has been estimated: DLR increases by about 30% in daytime and by 25% in nighttime under overcast low clouds. The annual average DLR in Moscow is 305 W/m2, with a minimum in December?CMarch and a maximum in July?CAugust. Variations in DLR throughout a year can exceed 250 W/m2. The daily average amplitude is 18?C33 W/m2 in summer and 6?C13 W/m2 in winter. An increase in DLR by about 40 W/m2 is noted under conditions of haze from forest and peat-bog fires and an aerosol optical depth of about 4 at a wavelength of 500 nm.  相似文献   

14.
The results of an analysis of intraweek differences in surface temperature precipitation, and optical aerosol thickness (τ550) in Moscow and in the vertical profiles of air temperature and wind over central Russia within the 2000–2009 period are given. The relation between the weekly cycles of the meteorological parameters and those of anthropogenic pollutions and dynamic processes is studied.  相似文献   

15.
Variations in the surface aerosol over the arid steppe zone of Southern Russia have been measured. The parameters of atmospheric aerosol (mass concentration, both dispersed and elemental compositions) and meteorological parameters were measured in Tsimlaynsk raion (Rostov oblast). The chemical composition of aerosol particles in the atmospheric surface layer has been determined, and the coefficients of enrichment of elements with respect to clarkes in the Earth’s crust have been calculated. It is shown that, in summer, arid aerosols are transported from both alkaline and sandy soils of Kalmykia to the air basin over the observation zone. Aerosol particles in the surface air layer over this region have been found to contain the products of combustion of oil, coal, and ethylized fuel. These combustion products make a small contribution to the total mass concentration of atmospheric aerosol; however, they are most hazardous to the health of people because of their sizes and heavy-metal contents. A high concentration of submicron sulfur-containing aerosol particles of chemocondensation nature has been recorded. Sources of aerosol of both natural and anthropogenic origins in southern Russia are discussed.  相似文献   

16.
The shortwave radiative forcings of smoke aerosol in the cloudless atmosphere during the summer fires of 2010 in European Russia were quantitatively estimated for the land surface and the atmospheric upper boundary from measurement data obtained at the Zvenigorod Scientific Station of the Obukhov Institute of Atmospheric Physics (OIAP ZSS), Russian Academy of Sciences. Variations in the temperature of the surface air layer due to the smoke-induced attenuation of incoming solar radiation were estimated. The most intensive smoke generation in the atmosphere was observed on August 7–9, 2010, when the maximum aerosol optical thickness amounted to more than 4.0 at a wavelength of 550 nm. In this case, the albedo of single aerosol scattering amounted to ∼0.95–0.96 and the asymmetry factor amounted to ∼0.69–0.70. The maximum shortwave radiative forcing of aerosol amounted to about −360 W/m2 for the land surface and almost −150 W/m2 for the atmospheric upper boundary. During the period of intensive smoke generation, the cooling of the atmospheric surface layer over daylight hours (12 h) amounted, on average, to ∼6°C. The power character of the dependence of the shortwave radiative forcing of aerosol for the land surface on aerosol optical thickness up to its values exceeding 4.0, which was revealed earlier on the basis of data on aerosol optical thickness (up to 1.5) obtained at the OIAP ZSS during the summer forest and peatbog fires of 2002 in the region of Moscow, was supported.  相似文献   

17.
Determining ‘photosynthetically active radiation’ (PAR) is a key part of calculating phytoplankton productivity in a biogeochemical model. We explore the daily and seasonal variability in the ratio of PAR irradiance to total irradiance that occurred at Ieodo Ocean Research Station (IORS) in the East China Sea under clear-sky conditions in 2004 using a simple radiative transfer model (RTM). Meteorological data observed at IORS and aerosol optical properties derived from Aerosol Robotic Network observations at Gosan are used for the RTM. Preliminary results suggest that the use of simple PA R irradianceratio values is appropriate in calculating phytoplankton productivity as follows: an average of 0.44 (±0.01) in January to an average of 0.48 (±0.01) in July, with average daily variabilities over these periods of about 0.016 (±0.008) and 0.025 (±0.008), respectively. The model experiments demonstrate that variations in the major controlling input parameters (i.e. solar zenith angle, precipitable water vapor and aerosol optical thickness) cause PAR irradiance ratio variation at daily and seasonal timescales. Further, increases (>0.012) in the PAR irradiance ratio just below the sea-surface are positively correlated with high solar zenith angles and strong wind stresses relative to those just above the sea-surface.  相似文献   

18.
The results of studies of aerosol optical thickness (AOT) in Dushanbe conducted from July 2010 to March 2011 within the AERONET program are discussed. The statistical characteristics of AOT have been shown to significantly vary during dust intrusions. The seasonal variations in the dustiness of the atmosphere have been analyzed.  相似文献   

19.
The aerosol longwave radiative forcing of the atmosphere and heating rate of the near-surface aerosol layer are estimated for the extreme smoke conditions in the Moscow region in summer 2010. Thermal radiation fluxes in the atmosphere are determined using the integral transmission function and semiempirical aerosol model developed on the basis of standard aerosol models and measurements at the Zvenigorod Scientific Station, Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences. The aerosol radiative forcing reached 33 W/m2 at the lower atmospheric boundary and ranged between–1.0 and 1.0 W/m2 at the upper atmospheric boundary. The heating rate of the 10-m atmospheric layer near surface was up to 0.2 K/h during the maximum smoke conditions on August 7–9. The sensitivity of the aerosol longwave radiative forcing to the changes in the aerosol absorption coefficient and aerosol optical thickness are estimated.  相似文献   

20.
The South China Sea(SCS) and the Arabian Sea(AS) are both located roughly in the north tropical zone with a range of similar latitude(0°–24°N). Monsoon winds play similar roles in the upper oceanic circulations of the both seas. But the distinct patterns of chlorophyll a(Chl a) concentration are observed between the SCS and the AS.The Chl a concentration in the SCS is generally lower than that in the AS in summer(June–August); the summer Chl a concentration in the AS shows stronger interannual variation, compared with that in the SCS; Moderate resolution imaging spectroradiometer(MODIS)-derived data present higher atmospheric aerosol deposition and stronger wind speed in the AS. And it has also been found that good correlations exist between the index of the dust precipitation indicated by aerosol optical thickness(AOT) and the Chl a concentration, or between wind and Chl a concentration. These imply that the wind and the dust precipitation bring more nutrients into the AS from the sky, the sub-layer or coast regions, inducing higher Chl a concentration. The results indicate that the wind velocity and the dust precipitation can play important roles in the Chl a concentration for the AS and the SCS in summer. However aerosol impact is weak on the biological productivity in the west SCS and wind-induced upwelling is the main source.  相似文献   

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