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1.
Minqiang ZHOU Qichen NI Zhaonan CAI Bavo LANGEROCK Jingyi JIANG Ke CHE Jiaxin WANG Weidong NAN Yi LIU Pucai WANG 《大气科学进展》2023,40(2):223-234
Measurements of carbon dioxide(CO2), methane(CH4), and carbon monoxide(CO) are of great importance in the Qinghai-Tibetan region, as it is the highest and largest plateau in the world affecting global weather and climate systems. In this study, for the first time, we present CO2, CH4, and CO column measurements carried out by a Bruker EM27/SUN Fourier-transform infrared spectrometer(FTIR) at Golmud(36.42°E, 94.91°N, 2808 m) in August 2021. The mean and... 相似文献
2.
Dongxu YANG Yi LIU Liang FENG Jing WANG Lu YAO Zhaonan CAI Sihong ZHU Naimeng LU Daren LYU 《大气科学进展》2021,38(9):1433-1443
Space-borne measurements of atmospheric greenhouse gas concentrations provide global observation constraints for top-down estimates of surface carbon flux.Here,the first estimates of the global distribution of carbon surface fluxes inferred from dry-air CO_2 column (XCO_2) measurements by the Chinese Global Carbon Dioxide Monitoring Scientific Experimental Satellite (Tan Sat) are presented.An ensemble transform Kalman filter (ETKF) data assimilation system coupled with the GEOS-Chem global chemistry transport model is used to optimally fit model simulations with the Tan Sat XCO_2 observations,which were retrieved using the Institute of Atmospheric Physics Carbon dioxide retrieval Algorithm for Satellite remote sensing (IAPCAS).High posterior error reduction (30%–50%) compared with a priori fluxes indicates that assimilating satellite XCO_2 measurements provides highly effective constraints on global carbon flux estimation.Their impacts are also highlighted by significant spatiotemporal shifts in flux patterns over regions critical to the global carbon budget,such as tropical South America and China.An integrated global land carbon net flux of 6.71±0.76 Gt C yr~(-1) over12 months (May 2017–April 2018) is estimated from the Tan Sat XCO_2 data,which is generally consistent with other inversions based on satellite data,such as the JAXA GOSAT and NASA OCO-2 XCO_2 retrievals.However,discrepancies were found in some regional flux estimates,particularly over the Southern Hemisphere,where there may still be uncorrected bias between satellite measurements due to the lack of independent reference observations.The results of this study provide the groundwork for further studies using current or future Tan Sat XCO_2 data together with other surfacebased and space-borne measurements to quantify biosphere–atmosphere carbon exchange. 相似文献
3.
Ke CHE Yi LIU Zhaonan CAI Dongxu YANG Haibo WANG Denghui JI Yang YANG Pucai WANG 《大气科学进展》2022,39(8):1299-1315
Measurements of column-averaged dry-air mole fractions of carbon dioxide and carbon monoxide, CO2 (XCO2) and CO (XCO), were performed throughout 2019 at an urban site in Beijing using a compact Fourier Transform Spectrometer (FTS) EM27/SUN. This data set is used to assess the characteristics of combustion-related CO2 emissions of urban Beijing by analyzing the correlated daily anomalies of XCO and XCO2 (e.g., ΔXCO and ΔXCO2). The EM27/SUN measurements were calibrated to a 125HR-FTS at the Xianghe station by an extra EM27/SUN instrument transferred between two sites. The ratio of ΔXCO over ΔXCO2 (ΔXCO:ΔXCO2) is used to estimate the combustion efficiency in the Beijing region. A high correlation coefficient (0.86) between ΔXCO and ΔXCO2 is observed. The CO:CO2 emission ratio estimated from inventories is higher than the observed ΔXCO:ΔXCO2 (10.46 ± 0.11 ppb ppm?1) by 42.54%–101.15%, indicating an underestimation in combustion efficiency in the inventories. Daily ΔXCO:ΔXCO2 are influenced by transportation governed by weather conditions, except for days in summer when the correlation is low due to the terrestrial biotic activity. By convolving the column footprint [ppm (μmol m–2 s–1)–1] generated by the Weather Research and Forecasting-X-Stochastic Time-Inverted Lagrangian Transport models (WRF-X-STILT) with two fossil-fuel emission inventories (the Multi-resolution Emission Inventory for China (MEIC) and the Peking University (PKU) inventory), the observed enhancements of CO2 and CO were used to evaluate the regional emissions. The CO2 emissions appear to be underestimated by 11% and 49% for the MEIC and PKU inventories, respectively, while CO emissions were overestimated by MEIC (30%) and PKU (35%) in the Beijing area. 相似文献
4.
Mole fractions of atmospheric CO_2(XCO_2) have been continuously measured from October 2014 to March 2016 at the Guangzhou Panyu Atmospheric Composition Site(23.00°N,113.21°E;140 m MSL) in the Pearl River Delta(PRD)region using a cavity ring-down spectrometer.Approximately 66.63%,19.28%,and 14.09% of the observed values were filtered as background,pollutant source,and sink due to biospheric uptake,respectively,by applying a robust local regression procedure.Their corresponding mean values were 424.12±10.12 ppm(×10~(-6) mol mol~(-1)),447.83±13.63 ppm,and 408.83±7.75 ppm.The background XCO_2 levels were highest in spring and winter,moderate in autumn,and lowest in summer.The diurnal XCO_2 was at a minimum from 1400-1600 LST(Local Standard Time) and a maximum at 0500 LST the next day.The increase of XCO_2 in spring and summer was mainly associated with polluted air masses from south coastal Vietnam,the South China Sea,and the southeast Pearl River Estuary.With the exception of summer,airflow primarily from marine regions southeast of Taiwan that passed over the Pearl River Estuary had a greater impact on XCO_2,suggesting an important potential source region. 相似文献
5.
Christian Azar Kristian Lindgren Michael Obersteiner Keywan Riahi Detlef P. van Vuuren K. Michel G. J. den Elzen Kenneth M?llersten Eric D. Larson 《Climatic change》2010,100(1):195-202
The United Nations Framework Convention on Climate Change (UNFCCC 1992) calls for stabilization of atmospheric greenhouse gas (GHG) concentrations at a level that would prevent dangerous anthropogenic
interference with the climate system. We use three global energy system models to investigate the technological and economic
attainability of meeting CO2 concentration targets below current levels. Our scenario studies reveal that while energy portfolios from a broad range of
energy technologies are needed to attain low concentrations, negative emission technologies—e.g., biomass energy with carbon
capture and storage (BECCS)—significantly enhances the possibility to meet low concentration targets (at around 350 ppm CO2). 相似文献
6.
全球农作物对大气CO2及其倍增的吸收量估算 总被引：15，自引：0，他引：15
根据农作物产量资料（ＦＡＯ１９９２年），计算出中国和全球各种作物对ＣＯ２的吸收总量分别为５．５×１０８ｔ／ａＣ和２８．９×１０８ｔ／ａＣ。同时以不同ＣＯ２浓度下小麦、玉米、大豆等全生育期光合速率实验数据直接计算的Ｃ吸收量为对照，与相应的中国产量资料计算结果比较，两者相差２．６％。从而进一步依据作物对ＣＯ２倍增反应诊断实验结果，推算出大气ＣＯ２浓度比目前倍增（７００ｐｐｍ）条件下，中国和全球农作物吸收ＣＯ２总量将增长２１％－２６％，分别为６．６×１０８ｔ／ａ—６．９×１０８ｔ／ａ和３４．１×１０８ｔ／ａ—３６．２×１０８ｔ／ａＣ。研究还表明，单位面积作物年吸Ｃ量全球（３．２ｔ／（ｈｍ２·８））比中国（４．２ｔ／（ｈｍ２·ａ））低２５．４％，而且Ｃ４作物普遍高于同类Ｃ３作物。 相似文献
7.
目前温室气体清单的编制主要基于IPCC方法,该方法用于特定城市或区域清单编制时可能会引起较大的不确定性,而目前对城市/区域尺度清单的不确定性的分析还存在很大的欠缺。本文通过南京市和长三角温室气体排放因子甄选,应用IPCC方法计算了2009年南京市和长三角的人为温室气体排放量,并以其为个例利用蒙特卡洛方法开展城市和区域尺度的温室气体人为排放清单不确定性的初步探究。研究结果表明:南京市CH4和CO2排放量的95%的概率分布范围分别为(1.08~1.86)×105t和(6.50~7.41)×107t,不确定性分别为-21.74%~34.78%和-7.01%~5.87%;长三角CH4和CO2排放量的95%的概率分布范围分别为(4.07~5.89)×106t和(1.62~1.82)×109t,不确定性分别为-15.60%~22.24%和-6.04%~5.34%。 相似文献
8.
The responses of the climate system to increase of atmospheric carbon dioxide(CO2)arestudied by using a new version of the Bureau of Meteorological Research Centre(BMRC)globalcoupled general circulation model(CGCM).Two simulations are run:one with atmospheric CO2concentration held constant at 330 ppm,the other with a tripling of atmospheric CO2(990 ppm).Results from the 41-year control coupled integration are applied to analyze the mean state,seasonal cycle and interannual variability in the model.Comparisons between the greenhouseexperiment and the control experiment then provide estimations of the influence of increased CO2on climate changes and climate variability.Especially discussed is the question on whether theclimate changes concerned with CO2 inerease will impact interannual variability in tropical Pacific,such as ENSO. 相似文献
9.
East China (23.6°–38.4°N, 113.6°–122.9°E) is the largest developed region in China. Based on CO2 products retrieved from the Greenhouse Gases Observing Satellite (GOSAT), the spatial and temporal distributions of CO2 mixing ratios in East China during 2014–17 are discussed, and the retrieved CO2 from AIRS (Atmospheric Infrared Sounder) and OCO-2 (Orbiting Carbon Observatory-2), as well as WLG (Waliguan) background station observations, are compared with those of GOSAT. The annual CO2 retrieved from GOSAT in East China ranged from 398.96 ± 0.24 ppm in 2014 to 407.39 ± 0.20 ppm in 2017, with a growth rate of 2.82 ± 0.15 ppm yr?1, which were higher than in other regions of China. The seasonal cycle presented a maximum in spring and a minimum in summer or autumn. Higher values were mainly concentrated in the coastal areas of Zhejiang Province, and lower values were concentrated in Jiangxi and the north of Fujian Province. CO2 observed in Fujian and parts of Jiangxi increased by less than 1.0 ppm during 2014–15, but enhanced significantly by more than 5.0 ppm during 2015–16, perhaps influenced by local emissions and global impacts. We calculated year-to-year CO2 enhancements in the Yangtze River Delta region during 2014–17 that were relatively low and stable, due to the region’s carbon emissions control and reduction policies. The annual and seasonal amplitudes of CO2 retrieved from AIRS were lower than those from GOSAT in East China, probably owing to the CO2 retrieved from AIRS better reflecting the characteristics of the mid-troposphere, while GOSAT is more representative of near-surface CO2. The spatial and temporal distribution characteristics of CO2 retrieved from OCO-2 were close to those from GOSAT in East China. 相似文献
10.
A three-dimensional ocean carbon cycle model which is a general circulation model coupled with simple biogeochemical processes is used to simulate CO2 uptake by the ocean.The OGCM used is a modified version of the Geophysical Fluid Dynamics Laboratory modular ocean model(MOM2).The ocean chemistry and a simple ocean biota model are included.Principal variablesare total CO2,alkalinity and phosphate.The vertical profile of POC flux observed by sediment traps is adopted,the rain ratio,a ratio of production rate of calcite against that of POC,and the bio-production efficiency should be 0.06 and 2 per year,separately.The uptake of anthropogenic CO2 by the ocean is studied.Calculated oceanic uptake of anthropogenic CO2 during the 1980s is 2.05×1015g(Pg)per year.The regional distributions of global oceanic CO2 are discussed. 相似文献
11.
长江三角洲地区净生态系统二氧化碳通量及浓度的数值模拟 总被引：1，自引：0，他引：1
净生态系统碳通量(NEE)的计算对于准确模拟区域碳通量和大气CO2浓度的时空变化至关重要。本文利用中尺度大气-温室气体耦合模式WRF-GHG(Weather Research and Forecasting Model with Greenhouse Gases Module),对2010年7月28日至2010年8月2日期间影响长江三角洲地区大气CO2浓度及时空分布的各种过程进行了详尽模拟。结果表明,植被光合呼吸模型(VPRM)能模拟不同植被下垫面NEE的日变化;WRF-GHG模拟的大气CO2浓度日变化与观测相吻合,但低估了大气CO2浓度5~15 ppm(ppm表示10-6),这可能与人为排放源的低估、VPRM参数的不确定性以及气象场模拟的不准确性有关。太湖和植被覆盖较好的地区如浙江北部山区是该地区的主要碳汇,而城市为CO2的主要排放源。太湖和陆地生态系统对区域内碳循环起到一定的调节作用,减缓区域大气CO2浓度的升高。此外,局地气象条件如湖陆风对太湖周边地区大气CO2浓度有显著影响。 相似文献
12.
OBSERVATION AND INVESTIGATION OF VARIABILITIES OF BASELINE CO2 CONCENTRATION OVER WALIGUAN MOUNTAIN IN QINGHAI PROVINCE OF CHINA* 
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下载免费PDF全文 In-situ measurement of atmospheric CO2 was made at the top of the Waliguan Mountain(36°17'N,100°54'E,3816 m asl).where the air is not directly affected by the local anthropogenic and natural sources,by using a nondispersive infrared(NDIR)analyzer and following the procedures proposed by WMO.The CO2 in the flask samples collected on the mountain was also analyzed in a laboratory.The measurements uncover the daily,monthly and seasonal variabilities and the baseline level of the CO2 in the air over the "clean" area of Chinese hinterland.Results suggest that the CO2 concentration over the East Asia continent has evident periodical variation,similar to that of global distribution.In 1992,an annual mean baseline CO2 concentration of 356.4 ppm over the continent was obtained.The annual mean value was 357.2 ppm for 1993.Some relationships between the CO2 concentration at Waliguan and the weather conditions,especially,wind speed and direction are found through the observation. 相似文献
13.
利用瓦里关和上甸子大气本底站观测的月平均CO2浓度数据对GOSAT卫星反演的CO2浓度数据进行验证,结果表明GOSAT产品与台站观测数据有较好的一致性.利用2009年6月—2011年5月GOSAT反演的CO2浓度数据,分析了江苏地区CO2浓度的时空变化特征,结果表明:1)975 hPa高度层CO2浓度高于850 hPa高度层,CO2浓度的水平变化要小于垂直变化;2)在季节变化上,CO2浓度冬季最高,夏季最低,这可能与植被光合作用的强弱变化有关;比较前后两年的CO2浓度数据,夏季和秋季的增速较快,冬季和春季的增速较慢;3)在日变化上,发现徐州和南京站02时CO2浓度最高,14时CO2浓度最低,这可能也与植被光合作用的强弱有关. 相似文献
14.
Ground-based visible differential absorption spectrometry during twilight has been used for NO2 total column observations at the Antarctica Peninsula, Marambio Base (64S, 56W), during the austral spring of 1989 (9 September to 25 November).Results show moderate NO2 vertical column levels of 1.5 to 2.5×1015 molec cm-2 in the morning and 2 to 3×1015 molec cm-2 in the evening until middle October, highly modulated by planetary wave activity. From that date until the end of the period, a steady increase occurs which is associated with the rising of lower stratosphere temperature as the vortex weakens, reaching values of 5×1015 molec cm-2 in late November, with small a.m.-p.m. differences. NO2 is found to be positively correlated to both total ozone and 50 hPa temperature during the entire spring. However, when analyzing the departures from linear trends, a highly negative correlation has been observed from day 301 onwards. 相似文献
15.
在“双碳”目标背景下，从国家层面到地方层面，区域、城市、行业企业都在制定和实施双碳目标行动计划。CO2模拟因其客观性和高时空分辨率等优势，在城市碳排放研究中深受重视。本研究以京津冀地区为研究区域，采用Picarro仪器高精度观测的2019—2020年CO2数据，利用WRF模式进行CO2传输模拟，分析了CO2浓度变化的季节特征，评估了模式在城区中心、城郊及背景3个观测站点的模拟效果，并对边界层高度及化石燃料碳排放等可能影响CO2浓度的因素进行了研究。3个观测站点分别为北京中国科学院大气物理研究所325 m气象塔观测站（北京站）、河北香河观测站（香河站）和上甸子区域本底观测站（上甸子站）。模拟结果表明：上甸子站优于香河站，香河站优于北京站，在冬季尤其明显；CO2浓度的高值区主要分布在城区、电厂和工业区，尤其是唐山、石家庄和邯郸地区，大量交通、工业排放导致CO2浓度明显上升，且高值区的范围在冬季最大；就日平均变化和日变化而言，边界层高度与CO2浓度存在相反变化趋势；3个站点的化石燃料碳排放（FFECO2）与近地面总CO2浓度存在正相关关系，冬春季的相关性高于夏秋季，且FFECO2的占比从大到小依次为北京站、香河站、上甸子站；CO2传输模拟的不确定性存在空间差异和季节变化。 相似文献
16.
Uptake and Storage of Anthropogenic CO2 in the Pacific
Ocean Estimated Using Two Modeling Approaches
A basin-wide ocean general circulation model(OGCM) of the Pacific Ocean is employed to estimate the uptake and storage of anthropogenic CO 2 using two different simulation approaches.The simulation(named BIO) makes use of a carbon model with biological processes and full thermodynamic equations to calculate surface water partial pressure of CO 2,whereas the other simulation(named PTB) makes use of a perturbation approach to calculate surface water partial pressure of anthropogenic CO 2.The results from the two simulations agree well with the estimates based on observation data in most important aspects of the vertical distribution as well as the total inventory of anthropogenic carbon.The storage of anthropogenic carbon from BIO is closer to the observation-based estimate than that from PTB.The Revelle factor in 1994 obtained in BIO is generally larger than that obtained in PTB in the whole Pacific,except for the subtropical South Pacific.This,to large extent,leads to the difference in the surface anthropogenic CO 2 concentration between the two runs.The relative difference in the annual uptake between the two runs is almost constant during the integration processes after 1850.This is probably not caused by dissolved inorganic carbon(DIC),but rather by a factor independent of time.In both runs,the rate of change in anthropogenic CO 2 fluxes with time is consistent with the rate of change in the growth rate of atmospheric partial pressure of CO 2. 相似文献
17.
海洋对人为CO2吸收的三维模式研究 总被引：1，自引：0，他引：1
文中用包含海洋化学过程和一个简单生物过程的三维碳循环模式模拟了海洋对大气CO2的吸收,并分析了碳吸收的纬度分布。模拟工业革命以来海洋对大气CO2的吸收表明:海洋碳吸收再加上大气CO2的增加只占由化石燃料燃烧、森林砍伐和土地利用的变化而释放到大气中的CO2的2/3。1980～1989年期间海洋年平均吸收2.05GtC。海洋人为CO2的吸收有明显的纬度特征。模式计算的海洋CO2的吸收在总量与纬度分布上与观测结果比较相符。 相似文献
18.
基于典型城市站太原站2018年3月—2019年2月的大气CO2在线观测资料,利用筛分法(Meteorological filtering method, MET)和黑碳示踪法(Black Carbon tracer, BC)进行本底/非本底的筛分,得到了本底浓度的变化特征。结果表明,太原大气CO2浓度季均值冬季最高,夏季最低;不同季节呈“单峰型”日变化特征,日振幅均在26.0×10-6以上;4个季节CO2浓度与地面风速存在显著负相关关系;CO2浓度抬升区域主要受当地工业布局的影响,最大抬升幅度在秋季达17.4×10-6;使用气象筛分法(MET)得到年均本底浓度为(431.4±19.9)×10-6,人为排放等对其影响为23.5×10-6,年振幅比同纬度其它本底站大,为34.5×10-6;黑碳示踪法(BC)得到冬季季均本底浓度为(445.0±22.9)×10-6,比MET筛... 相似文献
19.
G. T. Amanatidis A. F. Bais A. G. Kelessis C S. Zerefos I. C. Ziomas 《Journal of Atmospheric Chemistry》1989,9(4):435-446
A programme of ground-based stratospheric and total NO2 column measurements was instituted at the Laboratory of Atmospheric Physics (40.5° N, 22.9° E) in August 1985. We present here the results of the first two years of measurements with a modified Canterbury filter photometer, details of which are given in the text. The stratospheric NO2 column, obtained at twilight during low local NO2 levels, shows the seasonal variation with monthly mean values of about 6×10-15 molec. cm-2 in the summertime to about 2.2×10-15 molec. cm-2 in the wintertime. These measurements compare well with measurements obtained with different instruments by other groups at similar latitudes (about 40° N) but in different places. Also, the asymmetry of the evening-to-morning stratospheric NO2 over Thessaloniki was found to be on the average equal to 1.58. Total NO2 column over Thessaloniki has a pronounced seasonal variation with amplitude of 0.68 matm. cm which can be explained partly from measured local NO2 sources which discharge in the mixing layer and partly from photolysis of the NO2 reservoir species. 相似文献
20.
Various climate protocol proposals oblige different industrialized countries to reduce CO2 and other greenhouse gas emissions. In principle, the total costs of these obligations could be substantially reduced if emission reductions are implemented in regions with low marginal costs for CO2 reduction. This has been difficult to quantify because of lack of models with suitable regional and sectoral detail. In this paper we perform these calculations by taking advantage of the capability of the IMAGE 2 model to compute regional emissions and costs. Two main options are examined for allocating emission reductions required of industrialized regions in a cost effective manner: (1) allocating them among industrialized regions (2) allocating them among all world regions. The cost savings for each of these options are presented. The main conclusions are that (a) it is of great importance for the cost comparisons of protocols to use a well defined baseline scenario and clearly formulated targets, and (b) large economic benefits, in the order of 35–65%, can accrue from joint-implementation agreements which allocate investments on the basis of net marginal costs of CO2 emission reduction. 相似文献