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1.
Abstract— The cosmogenic radionuclide 60Fe (T1/2 = 1.49 Ma) was measured in two iron meteorites as well as in the magnetic fractions of a stony-iron and a stony meteorite by means of accelerator mass spectrometry (AMS). The measured 60Fe/Fe ratios range from 1.5 × 10-14 to 6.3 × 10-14 and show a significant correlation to the respective concentrations of Ni, which is the main target element. The resulting 60Fe specific activities correspond to production rates in meteorites in the order of 1 dpm/kg Ni. In addition, model calculations of depth- and size-dependent 60Fe production rates were performed. Although there are no experimental data for the production cross sections, our measurements are in surprisingly good agreement with the theoretical predictions using production cross sections that were determined by computer model calculations.  相似文献   

2.
Cadmium is a highly volatile element and its abundance in meteorites may help better understand volatility‐controlled processes in the solar nebula and on meteorite parent bodies. The large thermal neutron capture cross section of 113Cd suggests that Cd isotopes might be well suited to quantify neutron fluences in extraterrestrial materials. The aims of this study were (1) to evaluate the range and magnitude of Cd concentrations in magmatic iron meteorites, and (2) to assess the potential of Cd isotopes as a neutron dosimeter for iron meteorites. Our new Cd concentration data determined by isotope dilution demonstrate that Cd concentrations in iron meteorites are significantly lower than in some previous studies. In contrast to large systematic variations in the concentration of moderately volatile elements like Ga and Ge, there is neither systematic variation in Cd concentration amongst troilites, nor amongst metal phases of different iron meteorite groups. Instead, Cd is strongly depleted in all iron meteorite groups, implying that the parent bodies accreted well above the condensation temperature of Cd (i.e., ≈650 K) and thus incorporated only minimal amounts of highly volatile elements. No Cd isotope anomalies were found, whereas Pt and W isotope anomalies for the same iron meteorite samples indicate a significant fluence of epithermal and higher energetic neutrons. This observation demonstrates that owing to the high Fe concentrations in iron meteorites, neutron capture mainly occurs at epithermal and higher energies. The combined Cd‐Pt‐W isotope results from this study thus demonstrate that the relative magnitude of neutron capture‐induced isotope anomalies is strongly affected by the chemical composition of the irradiated material. The resulting low fluence of thermal neutrons in iron meteorites and their very low Cd concentrations make Cd isotopes unsuitable as a neutron dosimeter for iron meteorites.  相似文献   

3.
Abstract— We measured with a secondary ion mass spectrometer Mn/Cr ratios and Cr isotopes in individual grains of Mn-bearing sulfides (i.e., sphalerites, ZnS; alabandites, MnS; and niningerites, MgS) in nine unequilibrated enstatite chondrites (UECs). The goals were to determine whether live 53Mn (half-life ～3.7 Ma) was incorporated in these objects at the time of their isotopic closure and to establish whether Mn-Cr systematics in sulfides in UECs can be used as a high-resolution chronometer to constrain formation time differences between these meteorites. Sulfide grains analysed in four of these UECs, MAC 88136 (EL3), MAC 88184 (EL3), MAC 88180 (EL3), and Indarch (EH4), have clear 53Cr excesses. These 53Cr excesses can be very large (δ53Cr/52Cr ranges up to ～18,400%, the largest 53Cr excess measured so far) and, in some grains, are well correlated with the Mn/Cr ratios. Thus, they were most likely produced by the in situ decay of 53Mn in the meteorite samples. In the remaining five meteorites, no detectable excesses of 53Cr were found, and only upper limits on the initial 53Mn/55Mn ratios could be established. The four meteorites with 53Cr excesses show variations in the inferred 53Mn/55Mn ratios in various sulfide grains of the same meteorite. The Mn-Cr systematics in these sulfides were disturbed (during and/or after the decay of 53Mn) by varying degrees of reequilibration. Provided 53Mn was homogeneously distributed in the region of the early solar system where these objects formed, the data suggest that the time of the last isotopic equilibration of sulfides in EL chondrites occurred at least 3 Ma after a similar episode in EH chondrites.  相似文献   

4.
Abstract— Aqueous activity on meteorite parent bodies is indicated by the presence of carbonates. High spatial resolution ion microprobe analyses of nine individual carbonate grains (four dolomites, five breunnerites) from the Orgueil meteorite reveal linear correlations between 53Cr excesses and Mn/Cr ratios in all grains, indicative of in situ decay of radioactive 53Mn (half‐life 3.7 million years). The well‐defined isochrons appear to have chronological significance. If this is the case, then 53Mn/55Mn ratios between 2.1 and 4.7 × 10?6 are inferred for the time of carbonate formation and absolute ages of between 4561 and 4565 Ma are calculated (systematic uncertainty of ±2 Ma). Dolomites tend to have formed slightly earlier than the breunnerites. Our data imply extensive aqueous activity on the Orgueil parent body over a period of several million years, starting ～3–4 Myr after formation of the solar system, that most likely was the result of impact heating and latent heat from the decay of radioactive 26Al and 60Fe.  相似文献   

5.
Abstract— Mn‐Cr systematics in phosphates (sarcopside, graftonite, beusite, galileiite, and johnsomervilleite) in IIIAB iron meteorites were investigated by secondary ion mass spectrometry (SIMS). In most cases, excesses in 53Cr are found and δ53Cr is well correlated with Mn/Cr ratios, suggesting that 53Mn was alive at the time of IIIAB iron formation. The inferred Mn‐Cr “ages” are different for different phosphate minerals. This is presumably due to a combined effect of the slow cooling rates of IIIAB iron meteorites and the difference in the diffusion properties of Cr and Mn in the phosphates. The ages of sarcopside are the same for the IIIAB iron meteorites. Johnsomervilleite shows apparent old ages, probably because of a gain of Cr enriched in 53Cr during the closure process. Apparently, old Mn‐Cr ages reported in previous studies can also be explained in a similar way. Therefore, the IIIAB iron meteorites probably experienced identical thermal histories and thus derived from the core of a parent body. Thermal histories of the parent body of IIIAB iron meteorites that satisfy the Mn‐Cr chronology and metallographic cooling rates were constructed by computer simulation. The thermal history at an early stage (<10 Ma after CAI formation) is well determined, though later history may be more model‐dependent. It is suggested that relative timing of various events in the IIIAB parent body may be estimated with the aid of the thermal history. There is a systematic difference in Mn and Cr concentrations in various minerals (phosphates, sulfide, etc.) among the IIIAB iron meteorites, which seems to be mainly controlled by redox conditions.  相似文献   

6.
Neutron capture effects in meteorites and lunar surface samples have been successfully used in the past to study exposure histories and shielding conditions. In recent years, however, it turned out that neutron capture effects produce a nuisance for some of the short‐lived radionuclide systems. The most prominent example is the 182Hf‐182W system in iron meteorites, for which neutron capture effects lower the 182W/184W ratio, thereby producing too old apparent ages. Here, we present a thorough study of neutron capture effects in iron meteorites, ordinary chondrites, and carbonaceous chondrites, whereas the focus is on iron meteorites. We study in detail the effects responsible for neutron production, neutron transport, and neutron slowing down and find that neutron capture in all studied meteorite types is not, as usually expected, exclusively via thermal neutrons. In contrast, most of the neutron capture in iron meteorites is in the epithermal energy range and there is a significant contribution from epithermal neutron capture even in stony meteorites. Using sophisticated particle spectra and evaluated cross section data files for neutron capture reactions we calculate the neutron capture effects for Sm, Gd, Cd, Pd, Pt, and Os isotopes, which all can serve as neutron‐dose proxies, either in stony or in iron meteorites. In addition, we model neutron capture effects in W and Ag isotopes. For W isotopes, the GCR‐induced shifts perfectly correlate with Os and Pt isotope shifts, which therefore can be used as neutron‐dose proxies and permit a reliable correction. We also found that GCR‐induced effects for the 107Pd‐107Ag system can be significant and need to be corrected, a result that is in contrast to earlier studies.  相似文献   

7.
Abstract— Here we present the first purely physical model for cosmogenic production rates in iron meteorites with radii from 5 cm to 120 cm and for the outermost 1.3 m of an object having a radius of 10 m. The calculations are based on our current best knowledge of the particle spectra and the cross sections for the relevant nuclear reactions. The model usually describes the production rates for cosmogenic radionuclides within their uncertainties; exceptions are 53Mn and 60Fe, possibly due to normalization problems. When an average S content of about 1 ± 0.5% is assumed for Grant and Carbo samples, which is consistent with our earlier study, the model predictions for 3He, 21Ne, and 38Ar are in agreement. For 4He the model has to be adjusted by 24%, possibly a result of our rather crude approximation for the primary galactic α particles. For reasons not yet understood the modeled 36Ar/38Ar ratio is about 30–40% higher than the ratio typically measured in iron meteorites. Currently, the only reasonable explanation for this discrepancy is the lack of experimentally determined neutron induced cross sections and therefore the uncertainties of the model itself. However, the new model predictions, though not yet perfect, enable determining the radius of the meteoroid, the exposure age, the sulphur content of the studied sample as well as the terrestrial residence time. The determination of exposure ages is of special interest because of the still open question whether the GCR was constant over long time scales. Therefore we will discuss in detail the differences between exposure ages determined with different cosmogenic nuclides. With the new model we can calculate exposure ages that are based on the production rates (cm3STP/(gMa)) of noble gases only. These exposure ages, referred to as noble gas exposure ages or simply 3,4He, 21Ne, or 36,38Ar ages, are calculated assuming the current GCR flux. Besides calculating noble gas ages we were also able to improve the 41K‐40K‐and the 36Cl‐36Ar dating methods with the new model. Note that we distinguish between 36Ar ages (calculated via 36Ar production rates only) and 36Cl‐36Ar ages. Exposure ages for Grant and Carbo, calculated with the revised 41K‐40K method, are 628 ± 30 Ma and 841 ± 19 Ma, respectively. For Grant this is equal to the ages obtained using 3He, 21Ne, and 38Ar but higher than the 36Ar‐ and 36Cl‐36Ar ages by ?30%. For Carbo the 41K‐40K age is ?40% lower than the ages obtained using 3He, 21Ne, and 38Ar but equal to the 36Ar age. These differences can either be explained by our still insufficient knowledge of the neutron‐induced cross sections or by a long‐term variation of the GCR.  相似文献   

8.
We present results of laboratory near-infrared reflectance studies of a set of calcic pyroxenes with comparable calcium contents (Wo45-50) but variable iron content and oxidation states. This new dataset complements earlier published data (Cloutis and Gaffey, 1991, J. Geophys. Res. 96, 22809-28826, and references therein). In particular, our new spectra extend the scarce available spectral data on chemically analyzed Fe-rich high-Ca clinopyroxenes. We attempted to interpret the spectral behavior of our samples in terms of chemistry and coordination site occupancies. Tentatively, we conclude that Fe-rich calcic pyroxenes have very low contents of Fe2+ in the M2 sites and belong to the spectral type A lacking the 2-μm band. This may be due to high Ca and Mn contents in these pyroxenes. Fe-poor high-Ca pyroxenes are more spectrally variable. In general, they tend to belong to the spectral type B with two major bands near 1 and 2 μm, unless the samples have high Fe3+/Fe2+ ratios or are rich in Mn and Ca. Some of them (including unusual meteorite Angra dos Reis) are of type B despite very high Ca contents. We applied the Modified Gaussian Model (MGM) to characterize three major Fe2+ absorption bands in the 1-μm region of the spectra of Ca-rich pyroxenes. Only the band due to Fe2+ in the M1 coordination site near 1.15 μm may be potentially useful to estimate the Fe content in calcic pyroxenes on remotely-sensed surfaces of Solar System bodies. The spectral variability of basaltic meteorites (angrites) that are rich in calcic pyroxenes is also discussed. The presence of spectral type A calcic pyroxenes in these meteorites complicates unambiguous identification of olivine in asteroid spectra.  相似文献   

9.
Abstract– We measured the concentrations and isotopic ratios of the cosmogenic noble gases He, Ne, and Ar in the very large iron meteorite Xinjiang (IIIE). The 3He and 4He data indicate that a significant portion of the cosmogenic produced helium has been lost via diffusion or in a recent impact event. High 22Ne/21Ne ratios indicate that contributions to the cosmogenic 21Ne from sulfur and/or phosphorous are significant. By combining the measured nuclide concentrations with model calculations for iron meteorites we were able to determine the preatmospheric diameter of Xinjiang to 260–320 cm, which corresponds to a total mass of about 70–135 tons. The cosmic‐ray exposure age of Xinjiang is 62 ± 16 Ma, i.e., relatively short compared to most of the other iron meteorites. With the current database we cannot firmly determine whether Xinjiang experienced a complex irradiation history. The finding of 3He and 4He losses might argue for a recent impact event and therefore for a complex exposure.  相似文献   

10.
Abstract– The isotope fractionation of Zn in meteorites has been measured for the first time using thermal ionization mass spectrometry and a double spiking technique. The magnitude of δZn ranged from ?0.29 to +0.38‰ amu?1 for five stone meteorites whereas the iron meteorite Canyon Diablo displays δZn of 1.11 ± 0.11‰ amu?1. The results for chondrites in this work can be divided into positive and negative δZn, supporting a previous proposal that chondrites are a mixture of materials from two different temperature sources. The Zn isotope fractionation present in meteorites may represent a primordial heterogeneity formed in the early solar system. An anomalous isotopic composition of Zn obtained for the Redfields iron meteorite suggests large‐scale inherited isotope heterogeneity of the protosolar nebula, or the presence of a parent body that has formed within its own isotopically anomalous reservoir. These anomalies are in the same direction but smaller than nuclear field shift effects observed in chemical exchange reactions. The isotope dilution mass spectrometry (IDMS) technique was used to measure Zn concentration, yielding a range from 20.1 μg g?1 to 302 μg g?1 in five stone meteorites and from 0.019 to 26 μg g?1 in seven iron meteorites. The IDMS‐measured abundance of Zn in Orgueil is 302 ± 14 μg g?1 and should be considered for future compilations of the abundance of Zn in the solar system.  相似文献   

11.
Abstract— A purely physical model is presented describing the depth- and size-dependence of the production of cosmogenic nuclides in meteoroids with radii up to 85 cm and in planetary surfaces by galactic cosmic ray protons. The model is based on Monte Carlo calculations of the intra- and internuclear cascades, by which depth- and size-dependent spectra of primary and secondary protons and of secondary neutrons are derived, and on experimental and theoretical thin-target cross sections of the underlying nuclear reactions. Model calculations are presented for production rates of 53Mn, 26Al, 22Ne, and 21Ne in H- and L-chondrites and of 53Mn and 26Al in lunar surface material and compared with experimental data. From the analysis of 53Mn and 26Al in the Apollo 15 lunar drill core and in the L-chondrite Knyahinya GCR p-spectra and integral particle fluxes at 1 A.U. and in the meteoroid orbits averaged over the last 10 Ma are derived. An analysis of experimental depth profiles in four H- and L-chondrites demonstrates, that the new model is well capable of describing depth- and size-dependences of production rates of cosmogenic nuclides. Moreover, it is possible to determine exposure ages for these meteorites on the basis of the theoretical 21Ne production rates. The model calculations further explain the depth- and size-dependence of 22Ne/21Ne-ratios and the dependences on these ratios of 21Ne, 26Al and 53Mn production rates. The future requirements for model calculations of cosmogenic nuclide production rates in extraterrestrial matter are outlined.  相似文献   

12.
Abstract— We measured nickel isotopes via multicollector inductively coupled plasma mass spectrometry (MC‐ICPMS) in the bulk metal from 36 meteorites, including chondrites, pallasites, and irons (magmatic and non‐magmatic). The Ni isotopes in these meteorites are mass fractionated; the fractionation spans an overall range of ～0.4‰ amu?1. The ranges of Ni isotopic compositions (relative to the SRM 986 Ni isotopic standard) in metal from iron meteorites (～0.0 to ～0.3‰ amu?1) and chondrites (～0.0 to ～0.2‰ amu?1) are similar, whereas the range in pallasite metal (～–0.1 to 0.0‰ amu?1) appears distinct. The fractionation of Ni isotopes within a suite of fourteen IIIAB irons (～0.0 to ～0.3‰ amu?1) spans the entire range measured in all magmatic irons. However, the degree of Ni isotopic fractionation in these samples does not correlate with their Ni content, suggesting that core crystallization did not fractionate Ni isotopes in a systematic way. We also measured the Ni and Fe isotopes in adjacent kamacite and taenite from the Toluca IAB iron meteorite. Nickel isotopes show clearly resolvable fractionation between these two phases; kamacite is heavier relative to taenite by ～0.4‰ amu?1. In contrast, the Fe isotopes do not show a resolvable fractionation between kamacite and taenite. The observed isotopic compositions of kamacite and taenite can be understood in terms of kinetic fractionation due to diffusion of Ni during cooling of the Fe‐Ni alloy and the development of the Widmanstätten pattern.  相似文献   

13.
A parent body of the Lovina meteorite underwent processes which yielded dentritic structures of taenite in phosphide-sulfide-metal matrix unusual for iron meteorites. Similar dendritic structures can be found also in IIE meteorites as microinclusions but are unknown in other iron meteorites. The similarity between dendritic structures in the Lovina meteorite and metal-phosphide inclusions in IIE iron meteorites implies similar processes which led to their crystallization from molten materials in chambers of various sizes. Studying physical and chemical crystallization parameters of metal-phosphide inclusions in the Elga meteorite (IIE) makes it feasible to estimate the p-T conditions required for the unique Lovina meteorite to have formed. It is shown that dendrites in the Lovina meteorite may have been crystallized from molten materials close in composition to P-FeNi and P-S-FeNi that are produced when phosphides and sulfides melt locally in metals as a result of impact events with subsequent fast cooling. The temperature of homogeneous melting is likely to have been more than 1450°C, and the starting temperature of crystallization of such molten materials is estimated to have been between 1050 and 1150°C. The cooling rate of inclusions can be estimated to be 10−3 °C s−1, based on the structural and chemical concordance between samples obtained experimentally (Chabot et al., 2000) and metal-phosphide inclusions (P-FeNi and P-S-FeNi) in the Elga meteorite. Large-sized dendrites in the Lovina meteorite imply cooling rates that are considerably less than 10−3 °C s−1.  相似文献   

14.
Abstract– High‐precision Cu isotopic compositions have been measured for the metal phase of 29 iron meteorites from various groups and for four terrestrial standards. The data are reported as the δ65Cu permil deviation of the 65Cu/63Cu ratio relative to the NIST SRM 976 standard. Terrestrial mantle rocks have a very narrow range of variations and scatter around zero. In contrast, iron meteorites show δ65Cu approximately 2.3‰ variations. Different groups of iron meteorites have distinct δ65Cu values. Nonmagmatic IAB‐IIICD iron meteorites have similar δ65Cu (0.03 ± 0.08 and 0.12 ± 0.10, respectively), close to terrestrial values (approximately 0). The other group of nonmagmatic irons, IIE, is isotopically distinct (?0.69 ± 0.15). IVB is the iron meteorite group with the strongest elemental depletion in Cu and samples in this group are enriched in the lighter isotope (δ65Cu down to ?2.26‰). Evaporation should have produced an enrichment in 65Cu over 63Cu (δ65Cu >0) and can therefore be ruled out as a mechanism for volatile loss in IVB meteorites. In silicate‐bearing iron meteorites, Δ17O correlates with δ65Cu. This correlation between nonmass‐dependent and mass‐dependent parameters suggests that the Cu isotopic composition of iron meteorites has not been modified by planetary differentiation to a large extent. Therefore, Cu isotopic ratios can be used to confirm genetic links. Cu isotopes thus confirm genetic relationships between groups of iron meteorites (e.g., IAB and IIICD; IIIE and IIIAB); and between iron meteorites and chondrites (e.g., IIE and H chondrites). Several genetic connections between iron meteorites groups are confirmed by Cu isotopes, (e.g., IAB and IIICD; IIIE and IIIAB); and between iron meteorites and chondrites (e.g., IIE and H chondrites).  相似文献   

15.
Abstract— Thirteen new meteorites and three meteorite inclusions have been analyzed. Their results have been incorporated into earlier published data for a comprehensive reference to all analyzed meteorites at the Smithsonian Institution. The six tables facilitate a convenient overlook of meteorite data. Table 1 presents an alphabetical list of analyzed meteorites, Table 2 chemical analyses of stony meteorites, Table 3 chemical analyses of iron meteorites, Table 4 elemental composition of stony meteorites, Table 5 average composition of carbonaceous chondrites and achondrites (falls and finds), and Table 6 presents average composition of H, L, LL, and Antarctic chondrites (falls and finds). The tables are available online at the journal's Web site http:meteoritics.org .  相似文献   

16.
Abstract The radioactivities Be10, Al26, Cl36, Mn53, Ni59, and Co60 and the rare gas isotopes were measured in a sample taken from the surface of the Hoba meteorite. The spallation-produced radioactivities indicate that the sample was at a depth of 35 to 40 cm when the body was in space. The Ni59 activity indicates that the terrestrial age of Hoba is less than 80,000 years. Its Cl36-Ar36 exposure age is 263±40 million years. The Cl36 and rare-gas isotopes were also measured in the Deelfontein meteorite; its Cl36-Ar36 exposure age is 400±40 million years. The Cl36 and the Ni59 were also measured in a sample of Sikhote-Alin. In both Hoba and Sikhote-Alin the Ni59, which is a neutron-produced isotope, is higher than would be expected from the Cl36 content. This indicates that solar flares contributed to the neutron-produced isotopes in these iron meteorites.  相似文献   

17.
Abstract— A set of iron meteorites was investigated for Re-Os isotopes and provides a well-defined isochron age of 4.624 ± 0.017 Ba and an initial 187Os/188Os ratio of 0.095636 ± 0.00009. Actual ages may be a few percent lower due to uncertainty on the 187Re decay constant. Within the small sample number presented here, there is no evidence for age differences between classes. A more detailed study of the meteorite Kodaïkanal shows that the metal reservoir of this meteorite formed approximately at the same time as the other iron meteorites, in contrast with the silicate inclusions which display a formation age of 3.67 Ba with all other chronometers. A collisional origin is in agreement with the data on this meteorite. Major secondary events do not affect the Re-Os system at the bulk rock scale in metal as it is the sole significant reservoir of these two elements. A Re-Os and Rb-Sr investigation of meteoritic troilite exhibits disturbed chronometric systems, which we attribute to the terrestrial history of the meteorite.  相似文献   

18.
Vagn Buchwald (Fig.  1 ) was born in Copenhagen where he attended school and college. Then after 18 months of military service, he assumed a position at the Technical University of Copenhagen. A few years later, he was presented with a piece of the Cape York meteorite, which led to an interest in iron meteorites. Through a campaign of informed searching, Vagn found the 20 ton Agpalilik meteorite (part of the Cape York shower) on 31st July 1963 and by September 1967 had arranged its transport to Copenhagen. After sorting and describing the Danish collection, which included application of the Fe‐Ni‐P phase diagram to iron meteorite mineralogy, Vagn was invited to sort and describe other iron meteorite collections. This led to a 7 yr project to write his monumental Handbook of Iron Meteorites. Vagn spent 3 yr in the United States and visited most of the world's museums, the visit to Berlin being especially important since the war had left their iron meteorites in bad condition and without labels. During a further decade or more of iron meteorite research, he documented natural and anthropomorphic alterations experienced by iron meteorites, discovered five new minerals (roaldite, carlsbergite, akaganeite, hibbingite, and arupite); had a mineral (buchwaldite, NaCaPO4) and asteroid (3209 Buchwald 1982 BL1) named after him; and led expeditions to Chile, Namibia, and South Africa in search of iron meteorites and information on them. Vagn then turned his attention to archeological metal artifacts. This work resulted in many papers and culminated in two major books on the subject published in 2005 and 2008, after his retirement in 1998. Vagn Buchwald has received numerous Scandinavian awards and honors, and served as president of the Meteoritical Society in 1981–1982.  相似文献   

19.
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20.
Abstract— Cosmic‐ray‐produced (cosmogenic) nuclides were studied in fragments of the Brenham pallasite, a large stony iron meteorite. The contents of light noble gases (He, Ne, and Ar) and long‐lived radionuclides (10Be, 26Al, 36Cl, and 53Mn), produced by nuclear reactions with cosmic rays, were measured in the separated metal and olivine phases from numerous samples representing a wide range of shielding conditions in the meteoroid. The distribution of cosmogenic nuclide concentrations in the metal follows patterns similar to that observed in large iron meteorites. Shielding effects were estimated from the relative proportions of low‐ and high‐energy reaction products. The production rates varied, from surface to interior, by a factor of more than several hundred. The 36Cl‐36Ar cosmic‐ray exposure age of Brenham is 156 ± 8 Myr. This determination is based on a multiple nuclide approach that utilizes cosmogenic nuclide pairs. This approach not only yields a “shielding independent” exposure age but also demonstrates that the production of cosmogenic nuclides occurred in a single stage. The depth profiles of 10Be in the stone phase and 53Mn in the metal phase are shown superimposed on corresponding profiles from the Apollo 15 long drill core. Surprisingly low abundances of lithophile elements, such as K, U, and Th, provided a unique opportunity to examine the production systematics of those nuclides whose inventories typically have significant contributions from non‐cosmogenic sources, particularly radiogenic contributions. The U and Th contents of the olivine samples are extremely low, allowing detection of cosmogenic 4He production from oxygen, magnesium, silicon, and iron.  相似文献   

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