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Roles of sorting and chemical weathering in the geochemistry and magnetic susceptibility of Xiashu loess, East China 总被引：1，自引：0，他引：1
Fuchun Li Zhangdong Jin Changren Xie Jiayi Feng Libo Wang Yongzhao Yang 《Journal of Asian Earth Sciences》2007,29(5-6):813-822
Uncertainties in paleoenvironmental interpretations for traditional chemical analysis of bulk samples result from different grain-size sub-populations of sediments containing variable distributions of elements and minerals. Therefore, it is important to understand the elemental and mineral distribution in different grain sizes in determining the quantitative relationship between chemical weathering and climatic change. We sieved a series of Xiashu loess samples into three sub-populations of different grain sizes (<2, 2–45 and >45 μm, respectively), and then analyzed each population for rubidium (Rb), strontium (Sr), rare earth elements and magnetic susceptibility. In comparison with elemental concentrations of bulk samples, clay mineralogy and illitic crystallinity, our results show that distinct elemental distributions and magnetic susceptibilities for different grain-size sub-populations are controlled by sorting and/or chemical weathering, although we also suggest that the Xiashu loess may have the same provenance as the Central Chinese Loess. Maximum concentrations of Rb and fine-grained magnetic minerals in the less than 2 μm sub-population, coupled with our finding of maximum Sr in the larger than 45 μm fraction, indicate that Sr was lost during chemical weathering. Grain-size sub-population analysis is, therefore, an effective method for extracting paleoenvironmental information, because individual sub-populations show minimal variations in initial Rb/Sr ratios compared to bulk analysis of all sizes together. Furthermore, a negative correlation between Rb/Sr ratios and Sr concentrations for the <2 μm fraction (R2 = 0.97) may indicate that clay is a sensitive indicator of intensity of chemical weathering and is an ideal sub-population for determining Rb/Sr ratios, but not for magnetic susceptibility. 相似文献
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Rb, Sr, and magnetic susceptibility have been measured in the last interglacial–glacial loess profiles at Luochuan and Huanxian, central China. A high degree of similarity between the parameters in both profiles suggests that variations of Rb/Sr ratios in the sequence can be regarded as an indicator of East Asian summer monsoon strength. Matching the Rb/Sr record with the SPECMAP δ18O curve suggests that the Rb/Sr ratio responds sensitively to changes of the East Asian monsoon induced by global ice-volume variation. 相似文献
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本文系统地测试了陕西洛川黄土-古土壤剖面中的Rb,Sr含量和磁化率。通过对比该剖面2．50MaB．P．以来Rb／Sr曲线和磁化率曲线,发现两者的形状和变化的相位十分相似,然而两者的相对振幅却有明显的差别。Rb／Sr曲线记录了0．80MaB．P．左右一次重要的气候转型界面,揭示了黄士和古土壤内部次一级的气候波动旋回,反映了早更新世黄土高原较温暖潮湿的特点以及更新世以来气候由湿向干的变化趋势。研究表明,Rb／Sr值可以作为衡量东亚夏季风环流强度变化的较为敏感的替代性指标。 相似文献
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2.5Ma以来大陆风化强度的演变 总被引：1，自引：0，他引：1
本次研究得出了２．５ＭａＢＰ以来洛川剖面黄土－古土壤序列的酸不深物＾８７Ｓｒ／＾８６Ｓｒ、Ｒｂ／Ｓｒ、磁化率和沉积速率的变化曲线。黄土和古土壤酸不深物＾８７Ｓｒ／８６Ｓｒ、Ｒｂ／Ｓｒ和磁化率的变化具有类似的阶段性和周期性,这与晚新生代以来古气候的主要变化以及行星轨道参数相一致。研究证明,黄土和古土壤酸不深物＾８７Ｓｒ／＾８６Ｓｒ值得化学风化强度的替代指标,沉积速率是物理风化强度的替代指标。自２．５ 相似文献
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Late Cenozoic Chemical Weathering and Environmental Changes Recorded in the Co Ngoin Sediments,Central Qinghai-Tibet Plateau 总被引：1，自引：2，他引：1
CHEN Shiyue JIN Zhangdong WANG Sumin SHEN Ji Nanjing Institute of Geography Limnology Chinese Academy of Sciences Nanjing Jiangsu School of Environment Planning Liaocheng University Liaocheng Shandong Institute of Earth Environment Chinese Academy of Sciences Xi’an Shaanxi 《《地质学报》英文版》2005,79(3):384-391
A series of faulted inland basins were developed in the central Qinghai-Tibet Plateau, among which the Co Ngoin Basin containing thick lacustrine sediments is located in the peripheral area of the Indian monsoon. In this paper, we present the weathering history and paleoclimatic changes in the last 2.8 Ma based on studies of high-resolution temporal distributions of Sr, Rb and Zr concentrations, Rb/Sr and Zr/Rb ratios and δ ^13C and TOC for the Co Ngoin sediments, in combination with the sediment properties, grain size distribution and clay mineralogy. The sedimentary records indicate three environmental stages in the last 2.8Ma. At the core depth of 197-170m (about 2.8-2.5Ma), low-intensity chemical weathering in the Co Ngoin catchment was experienced under warm-dry to cool-wet climate conditions with relatively low Sr concentration and high Rb/Sr and Zr/Rb ratios. The sudden occurrence of both subalpine coniferous forest and coarses and and gravel sediments in the Co Ngoin core reflects a strong tectonic uplift. The high Sr concentrations and low Rb/Sr and Zr/Rb ratios reflect a relatively strong chemical weathering between 2.5Ma and 0.8Ma (at the core depth of 170-38.5m) under a temperate/cool and wet climate, characterized by mud and silt with fine sand, probably indicating a stable process of denudation and planation of the plateau. Above the depth of 38.5m (about 0.8-0Ma), the coarsening of sediments indicates a strong tectonic uplift and a relatively low intensity of chemical weathering as supported by the record of sediments having relatively low Sr concentrations and high Rb/Sr and Zr/Rb ratios. Since then, the plateau has taken the shape of the modern topographic pattern above 4000m a.s.l. 相似文献
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青藏高原中部2.8Ma以来的化学风化与环境演化的湖泊沉积记录 总被引：2，自引：0，他引：2
对采自青藏高原中部错鄂湖泊钻孔近200m以上深处、形成于2.8Ma以来的沉积岩岩芯中Sr,Rb,Zr含量变化及Rb/Sr,Zr/Rb比进行了研究,并结合其岩性、粒度、粘土矿物组成,分析了该地区2.8Ma来化学风化的相对强度和古环境演化过程。研究表明,2.8Ma来青藏高原中部的环境经历了3个演化阶段：在深约197－170m(2.8-2.5Ma)岩性段,低Sr含量,高Rb/Sr和Zr/Rb比揭示的是较弱的化学风化过程,反映了与当时强烈的高原隆升运动有关;在约170－38.5m（约2.5-0.8Ma)段,高Sr含量,低Rb/Sr和Zr/Rb比记录的是该流域较强的化学风化阶段,与高原在稳定期中部总体处于温湿或凉湿的环境下的结论吻合;在38.5-0m（约0.8-0Ma)段,总体Sr含量处于相对低值,Rb/Sr比相对较高,化学风化相对较弱,表明高原中部处于较寒冷的环境之中,高原整体已隆升到4000m以上。 相似文献
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Major and trace elemental compositions of loess samples collected from the Jingyuan section in the northwestern Chinese Loess Plateau (CLP) were analyzed to investigate the potential impacts of grain size sorting and chemical weathering on the loess geochemistry and to extract appropriate geochemical indices for better evaluating the East Asian monsoon variability. Based on variations of major and trace elements in different grain size fractions, seventeen elements were classified into three types: (1) Si and Na display higher contents with the increased particle sizes; (2) Al, Fe, Mg, K, Mn, Zn, Rb, Cr, V are mainly enriched in fine size fractions; (3) Ti, Ba, Zr, P, Ca and Sr show irregular variations among different size fractions. Comparison of Al-normalized elemental ratios with Zr/Rb and Rb/Sr ratios (two commonly employed indicators for grain size sorting and pedogenic weathering) indicates that Si/Al, Zr/Al, Ti/Al variations match well with Zr/Rb and grain size results, whilst Ca/Al, Sr/Al, P/Al ratios display similar variability as that of Rb/Sr ratio. Comparison of loess based proxies (e.g., elemental ratios, magnetic susceptibility, grain size) of Jingyuan section with speleothem and ice-core records confirms that elemental ratios of high-resolution loess sequences developed in the northwestern CLP can be employed to address fluctuations of the winter monsoon-induced grain size sorting and summer monsoon-related weathering and pedogenesis at glacial–interglacial and millennial timescales. 相似文献
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Rb and Sr Geochemical Characterization of the Chinese Loess Stratigraphy and Its Implications for Palaeomonsoon Climate 总被引：1，自引：0，他引：1
CHEN JunDepartment of Earth Sciences Nanjing University Nanjing WANG Yongjin Department of Geography Nanjing Normal University Nanjing CHEN Yang LIU Lianwen JI Junfeng Department of Earth Sciences Nanjing University Nanjing LU Huayu Xi ''an State Key Laboratory of Loess Quaternary Geology Chinese Academy of Sciences Xi ''an 《《地质学报》英文版》2000,74(2):279-288
Concentrations and distributions of Rb and Sr in loess and palaeosol samples from the Luochuan profile have been studied, in grain-size fractions and chemical forms. Results show that Rb is quite rich in the fraction of less than 2μm, and exits only in the residual phase, while Sr is distributed in sand and silt fractions, occurring in the residual and carbonate phases. Therefore, variations of the concentrations of Rb and Sr in loess and palaeosols are closely related not only to dustfall compositions depending on winter monsoon wind strength but also to summer monsoon-induced pedogenic intensity. This indicates that variations of Rb/Sr ratio in Chinese loess sequences represent cyclic alternations of East Asian summer and winter monsoon climates on the orbital time-scale. Variations in Sr concentrations along the sequence bear a high similarity to the oxygen isotope record of the deep sea sediments over the past 2.5 Ma, whereas variations in Rb concentrations are in good agreement with the record of 相似文献
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The magnetic properties of the late Quaternary hemipelagic sediment from piston core BS77-15 taken in the Tyrrhenian Sea were investigated and the results compared with palaeoclimatic records. The magnetic mineralogy of the sediment was studied and the magnetic carriers were identified by their spectra of coercivity and unblocking temperature. Investigations of rock magnetic parameters such as the Natural Remanent Magnetization (NRM), the low-field magnetic susceptibility χ, the frequency-dependent susceptibility χ fd , the acquisition of Anhysteretic Magnetization (ARM) and Isothermal Magnetization (IRM) and the Median Destructive Field (MDF) have established the downcore variations in terms of magnetic mineralogy, grain size and coercivity in the sediments. The rock magnetic parameters were compared with an alternative climatic record from the same core based on the faunal association of planktonic foraminifera. A significant correlation was found between faunal climatic record and χ fd . Together with the magnetic properties of the sediment this suggests that a palaeoclimatic signal is recorded by a fine-grained low-coercivity fraction of the magnetic minerals. 相似文献
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《Chemie der Erde / Geochemistry》2014,74(4):571-576
Rubidium (Rb) and strontium (Sr) contents and ratios were analyzed in 197 sediment samples collected from the CGS1 segment of the Chagelebulu Section in the Badain Jaran Desert of China to study millennial scale climate change during the Holocene. The results showed that the Rb and Sr contents and Rb/Sr ratios were low in the samples of dune sands and loess (Mz < 5.64Φ), and those values were high in the samples of loess (Mz > 5.64Φ) and paleosols, these data displayed 11 changing cycles in alternation of peaks and valleys in the chart. In addition, the Rb contents were positively correlated with Mz (mean particle diameter) and clay contents. While the correlations were weaker, Sr contents also showed a tendency to increase with increases in the Mz and clay contents. Based on a comprehensive analysis of the distribution of Rb and Sr within the CGS1 segment, it appears that the observed Rb and Sr contents and ratios varied in accordance with fluctuations of the East Asian winter and summer monsoons. In terms of timing and climate, low values (C1–C11) resulting from winter monsoons had a strong correlation with cold events in the North Atlantic: the period C1 corresponded to times ranging from 400 a to 1400 a and the periods C2, C3, C4, C7, C9, C10, and C11 corresponded to times of 3000 a, 4000 a, 5900 a, 8200 a, 9400 a, 10,300 a, and 11,000 a, respectively. The cold event C5 (6200 a) was also discovered in the North Atlantic in recent; and C6 (7100 a), C8 (8700 a) were discovered in some other places of China. These cold events indicated by Rb and Sr contents and ratios in the Chagelebulu Section of the Badain Jaran Desert recorded the regional response of global climate change during the Holocene. 相似文献
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David Alan Spears 《Geochimica et cosmochimica acta》1974,38(2):235-244
The RbSr age dating method has been applied to a sequence of Carboniferous shales for which some geochemical information was already available. In the marine shales, the Rb/Sr ratio is higher than in the non-marine and brackish water shales. Although the range of values can be attributed to depositional processes, the range of Rb/Sr values is too small to give a depositional isochron, and thus the age of deposition can not be determined. If samples with a variable mineralogy had been selected for the isotope study, the range of Rb/Sr could have been extended. Only by chance, however, would the depositional age have been obtained.A comparison of the RbSr isotope values in the Carboniferous shales with those in probable source rocks shows that a reduction in the Sr87/Sr86 ratio relative to the Rb87/Sr86 ratio may have taken place. Such a reduction could have occurred on the Carboniferous land-mass during the formation of the clay minerals. 相似文献
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Typical Geochemical Elements in Loess Deposit in the Northeastern Tibetan Plateau and Its Paleoclimatic Implication 总被引：2，自引：0，他引：2
TAN Hongbing MA Haizhou ZHANG Xiying LU Huayu WANG Jianguo 《《地质学报》英文版》2006,80(1):110-116
Widespread and thick loess deposit in the northeastern Tibetan Plateau records paleoclimatic changes over the Quaternary period. In this study, we investigate a loess section located in a high terrace of the Huangshui River in the Xining Basin, and collect samples at 20-cm intervals by digging a well of 16-m depth （including paleosol S1 and SO and several loess interlayers over the last glacial-interglacial cycle and the Holocene）. Concentration of some active elements （Sr and Ca） and inert elements （Rb, Zr, Ti） in these loess samples are measured. The results show that ratios of those elements （oxide）, such as Rb/Sr, Ti/Sr, and Zr/CaO ratios, would indicate sensitively paleoclimatic changes, especially the history of precipitation over the last glacial-interglacial and the Holocene. Moreover, the curves of Rb/Sr, Ti/Sr, and Zr/CaO ratios had almost the same variable trends from the bottom to the top and also closely correlated with values of magnetic susceptibility and the global marine δ^18O record. But compared with the curves of magnetic susceptibility, the changes of ratios of these elements （oxide） are clearer and easy to understand. Therefore, the ratios of these typical chemical elements in the loess deposit may be used as an excellent index to investigate the history of paleoclimate, particularly precipitation changes in the northeastern Tibetan Plateau. 相似文献
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黄土高原西部高分辨率黄土序列开展的多代用指标研究,有助于揭示轨道-亚轨道尺度上东亚冬、夏季风的变化特征及动力机制。但针对同一地质记录提取冬、夏季风多代用指标进行对比和敏感性分析的工作尚不多见,因此制约了对季风快速变化特征和机理的理解。本文利用甘肃临夏85 m黄土岩芯开展高分辨率的粒度、磁化率和元素扫描分析,发现在轨道尺度上粒度和Zr/Rb比值显示的大幅冰期-间冰期波动与深海氧同位素记录有很好的对应关系,表明东亚冬季风的波动响应于北半球高纬冰量的变化。但在千年尺度上,粒度能更敏感地响应冬季风的快速变化;Rb/Sr比值和磁化率均能很好记录轨道尺度上的东亚夏季风波动,但在亚轨道尺度上Rb/Sr的敏感性明显高于磁化率。粒度、Zr/Rb和Rb/Sr所指示的东亚季风快速变化表现出较强的岁差信号,与石笋和北纬65°夏季太阳辐射有较好的对应关系,表明东亚季风变化也受到岁差直接驱动的夏季太阳辐射变的控制。在最后两个冰期-间冰期旋回中(即末期冰期旋回和倒数第二次冰期旋回)Rb/Sr及Zr/Rb比值和粒度记录分别可以辨别出与石笋相同数量级的变暖事件,但粒度记录的暖事件明显要多于Rb/Sr及Zr/Rb比值,且这些暖事件并不能一一对应。粒度及元素比值记录显著变冷的千年尺度的Heinrich(H)事件与石笋记录的夏季风明显减弱的事件有很好的对应关系,但其发生频率明显高于海洋记录。这些指标记录的千年尺度上波动信号的不一致性主要归因指标对不同气候要素敏感性的差异。未来需要进一步开展高分辨率多代用指标敏感性分析,选取对季风快速变化的敏感指标,有助于我们理解季风快速变化的特征(如周期和幅度等)和分析季风快速变化的时空差异性。 相似文献
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1IntroductionGlobal change studies on the decennial and cen-tennial timescales,which can help put together the in-formation from long timescale study and meteorologicalstudy,is crucial for predicting future global changes(Hegerl,1998;Wang Pinxian and Jian Zhimin,1999;Wang Sumin et al.,1998).Lacustrine sedi-ments characterized by their continuity,major sedi-mentation rate,and high resolution can provide usefulinformation for reconstructing the past global changes(Steven,1996;Wang Sumin and … 相似文献
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DECOUPLED SUMMER AND WINTER MONSOON IN NORTHEAST TIBET AND NORTHWEST LOESS PLATEAU DURING THE LAST INTERGLACIATIONtheNationalKeyProjectforBasicResearchonTibetPlateau (G19980 4 80 0 )andtheNationalNaturalSci
encesFoundationofChina (No.4 990 相似文献
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太行山脉武安白云石热分解机理 总被引：8，自引：0，他引：8
对太行山白云石热分解机理进行研究,发现其分解过程分为三个阶段、两步反应。第一步反应开始是界面收缩控速机理,后变为扩散控速机理,ＣＯ＾２－３的扩散为控速步骤。第一步分解产物ＭｇＯ是直接生成的,而不是ＣａＯ再碳化的产物,第二步反应是被ＭｇＯ包围着的ＣａＣＯ３的分解反应,ＣＯ２的扩散是控速步骤。 相似文献
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对大别山北麓0.78 Ma以来的黄土-古土壤样品的磁化率及Rb和Sr的地球化学特征研究表明,相对高的w(Rb)和w(Rb)/w(Sr)值及低w(Sr)值指示夏季风占优势的湿润时期,对应古土壤层;相对低的w(Rb)和w(Rb)/w(Sr)值及高w(Sr)值指示冬季风占优势的干旱期,磁化率相对较低,对应黄土层。剖面的w(Rb)/w(Sr)值自下至上降低反映大别山北麓地区的风化作用逐渐减弱,也揭示自0.78 Ma以来气候具有由湿向干的趋势;磁化率与w(Rb)/w(Sr)值的对比分析表明,它们的变化曲线存在显著不同,原因可能是由于磁化率在古土壤中的增强机制比较复杂所致,w(Rb)/w(Sr)值作为气候替代指标比磁化率更灵敏。与洛川剖面相比,大别山黄土-古土壤的w(Rb)较高而w(Sr)较低及Rb、Sr较强的分异能力特征反映了大别山气候整体较为温湿,沉积物遭受的风化程度更强。 相似文献