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1.
Stable isotopic compositions (δ18O and d-excess) from 25 rivers in Thailand were analysed monthly during 2013–2015. Results indicated that monsoon precipitation fundamentally influences the river isotopes. The overland flow supplied from monsoon precipitation and human-altered flow regimes produces considerable isotopic variability. Spatial and temporal variations were observed among four principal geographical regions. The seasonality of monsoon precipitation in mountainous Thailand produced large variations in isotopic compositions because most rainfall occurred during the southwest monsoon, and dry conditions prevailed during the northeast monsoon. The northern and northeastern regions are mountainous, highland areas. Low δ18O values were found in these regions, likely because of altitude effects on precipitation. Conversely, monsoonal precipitation continually supplies rivers in southern Thailand all year round, producing higher and more consistent δ18O values than in the other regions. The Chao Phraya plain in the central region experienced enrichment of δ18O river runoff related to evaporation in irrigation systems. Larger catchment areas and longer residence times resulted in more pronounced evaporation effects, producing lower values of d-excess and local river water line slopes compared with precipitation. The isotopic differences between river waters and precipitation were utilized to determine river recharge elevations and water transit time. The methods presented here can be used to explore hydrological interactions in other tropical river basins.  相似文献   

2.
Stable isotopic compositions of precipitation (δ18Op, δ2Hp and d-excessp) and atmospheric vapour (δ18Ov, δ2Hv and d-excessv) with high spatial–temporal resolution are crucial in revealing hydrologic cycle. Based on the variation characteristics of δ18Op/δ18Ov, δ2Hp/δ2Hv and d-excessp/d-excessv in the headwaters of the Shule River (HSR) on hourly and daily scales from June to September 2018, this study analysed the relationships between δ18Op/δ2Hp and δ18Ov/δ2Hv combined with the equilibrium fractionation model, as well as δ18Op/δ18Ov and meteorological factors. The slopes of local meteoric water line (LMWL) and the δ2Hv-δ18Ov fitting equation were similar (7.96 and 7.94) with both intercepts exceeding 10, reflecting the great contribution of recycling moisture. The values of δ18Ov/δ2Hv were lower than δ18Op/δ2Hp but with consistent variation patterns throughout the period. The equilibrium simulation results suggested that precipitation and atmospheric vapour almost approached isotopic equilibrium state, especially during monsoon intrusion period. Affected by monsoon intrusion, the slopes and intercepts of the LMWLs and the δ2Hv-δ18Ov fitting equations were smaller than those during non-monsoon period and d-excess and δ18O were negatively correlated. Relative humidity had significant negative correlations with δ18Op and δ18Ov in the whole period, however, the positive correlations between δ18Op/δ18Ov and temperature were observed during non-monsoon and monsoon intrusion period, respectively. Our results demonstrated that precipitation and atmospheric vapour isotopic compositions exhibited consistency under the influence of diverse moisture sources, while more complex relationships were found between δ18Op/δ18Ov and meteorological factors. This research provided evidence for using the isotopic compositions of atmospheric vapour to indicate moisture sources, and can improve understanding of the water cycle and eco-hydrological process from the perspective of the interaction between water and gas phases of the inland river basin in northwest China.  相似文献   

3.
Stable water isotopes (δ18O and δ2H) are an important source signature for understanding the hydrological cycle and altered climate regimes. However, the mechanisms underlying atmospheric water vapour isotopes in the northeast Qinghai‐Tibetan Plateau of central Asia remain poorly understood. This study initially investigated water vapour isotopic composition and its controls during the premonsoon and monsoon seasons. Isotopic compositions of water vapour and precipitation exhibited high variability across seasons, with the most negative average δ18O values of precipitation and the most positive δ18O values of water vapour found during the premonsoon periods. Temperature effect was significant during the premonsoon period but not the monsoon period. Both a higher slope and intercept of the local meteoric water line were found during the monsoon period as compared with in the premonsoon period, suggesting that raindrops have been experienced a greater kinetic fractionation process such as reevaporation below the cloud during the premonsoon periods. The δ2H and δ18O signatures in atmospheric water vapour tended to be depleted with the occurrence of precipitation events especially during the monsoon period and probably as a result of rainout processes. The monthly average contribution of evaporation from the lake to local precipitation was 35.2%. High d‐excess values of water vapour were influenced by the high proportion of local moisture mixing, as indicated by the gradually increasing relative humidity along westerly and Asian monsoon trajectories. The daily observation (observed ε) showed deviations from the equilibrium fractionation factors (calculated ε), implying that raindrops experienced substantial evaporative enrichment during their descent. The average fraction of raindrops reevaporation was estimated to be 16.4± 12.9%. These findings provide useful insights for understanding the interaction between water vapour and precipitation, moisture sources, and help in reconstructing the paleoclimate in the alpine regions.  相似文献   

4.
Long-term atmospheric water vapour hydrogen (δ2H), oxygen (δ18O) and deuterium excess (d-excess) can provide unique insights into the land-atmosphere coupling processes. The in-situ measurements of atmospheric water vapour δ2H, δ18O and d-excess were conducted above a reed wetland of Liaodong Bay (2019–2020). We found significant inter-annual variations in atmospheric water vapour isotopes between the two growing (May–September) seasons. The δ2H, δ18O and d-excess of atmospheric water vapour exhibited different seasonal and diurnal cycles concerning the vertical measurement heights, especially in 2019. The isotopic differences of atmospheric water vapour among vertical measurement heights were more evident in the daytime. Rainfall events directly impacted the diurnal patterns of water vapour isotopes, and the influences depended on rainfall intensities. However, only weak correlations existed between water vapour isotopes and local meteorological factors (R2 = 0.01–0.16, p < 0.001), such as water vapour concentration (w), Relative Humidity (RH) and surface air temperature (Ta). Based on the back-air trajectory analyses, the spatial–temporal dynamics of atmospheric water vapour isotopes are highly synchronized with monsoon activities. Different water vapour sources influence the water vapour isotope in this region and the higher d-excess value is related to the intense convection brought by the monsoon. High-resolution measurements of atmospheric water vapour isotopes will improve our understanding of the hydrological cycles in coastal areas.  相似文献   

5.
To understand the moisture regime at the southern slopes of Mt. Kilimanjaro, we analysed the isotopic variability of oxygen (δ18O) and hydrogen (δD) of rainfall, throughfall, and fog from a total of 2,140 samples collected weekly over 2 years at 9 study sites along an elevation transect ranging from 950 to 3,880 m above sea level. Precipitation in the Kilimanjaro tropical rainforests consists of a combination of rainfall, throughfall, and fog. We defined local meteoric water lines for all 3 precipitation types individually and the overall precipitation, δDprec = 7.45 (±0.05) × δ18Oprec + 13.61 (±0.20), n  = 2,140, R 2 = .91, p  < .001. We investigated the precipitation‐type‐specific stable isotope composition and analysed the effects of amount, altitude, and temperature. Aggregated annual mean values revealed isotope composition of rainfall as most depleted and fog water as most enriched in heavy isotopes at the highest elevation research site. We found an altitude effect of δ18Orain = ?0.11‰ × 100 m?1, which varied according to precipitation type and season. The relatively weak isotope or altitude gradient may reveal 2 different moisture sources in the research area: (a) local moisture recycling and (b) regional moisture sources. Generally, the seasonality of δ18Orain values follows the bimodal rainfall distribution under the influences of south‐ and north‐easterly trade winds. These seasonal patterns of isotopic composition were linked to different regional moisture sources by analysing Hybrid Single Particle Lagrangian Integrated Trajectory backward trajectories. Seasonality of d excess values revealed evidence of enhanced moisture recycling after the onset of the rainy seasons. This comprehensive dataset is essential for further research using stable isotopes as a hydrological tracer of sources of precipitation that contribute to water resources of the Kilimanjaro region.  相似文献   

6.
To investigate stable isotopic variability of precipitation in Singapore, we continuously analysed the δ‐value of individual rain events from November 2014 to August 2017 using an online system composed of a diffusion sampler coupled to Cavity Ring‐Down Spectrometer. Over this period, the average value (δ18OAvg), the lowest value (δ18OLow), and the initial value (δ18OInit) varied significantly, ranging from ?0.45 to ?15.54‰, ?0.9 to ?17.65‰, and 0 to ?13.13‰, respectively. All 3 values share similar variability, and events with low δ18OLow and δ18OAvg values have low δ18OInit value. Individual events have limited intraevent variability in δ‐value (Δδ) with the majority having a Δδ below 4‰. Correlation of δ18OLow and δ18OAvg with δ18OInit is much higher than that with Δδ, suggesting that convective activities prior to events have more control over δ‐value than on‐site convective activities. The d‐excess of events also varies considerably in response to the seasonal variation in moisture sources. A 2‐month running mean analysis of δ18O reveals clear seasonal and interannual variability. Seasonal variability is associated with the meridional movement of the Intertropical Convergence Zone and evolution of the Asian monsoon. El Niño–Southern Oscillation is a likely driver of interannual variability. During 2015–2016, the strongest El Niño year in recorded history, the majority of events have a δ18O value higher than the weighted average δ18O of daily precipitation. δ18O shows a positive correlation with outgoing longwave radiation in the western Pacific and the Asian monsoon region, and also with Oceanic Niño Index. During El Niño, the convection centre shifts eastward to the central/eastern Pacific, weakening convective activities in Southeast Asia. Our study shows that precipitation δ‐value contains information about El Niño–Southern Oscillation and the Intertropical Convergence Zone, which has a significant implication for the interpretation of water isotope data and understanding of hydrological processes in tropical regions.  相似文献   

7.
Little is known about the spatial and temporal variability of the stable isotopic composition of precipitation in the North Atlantic and its relationship to the North Atlantic Oscillation (NAO) and anthropogenic climate change. The islands of the Azores archipelago are uniquely positioned in the middle of the North Atlantic Ocean to address this knowledge gap. A survey of spatial and temporal variability of the stable isotope composition of precipitation in Azores is discussed using newly presented analyses along with Global Network of Isotopes in Precipitation data. The collected precipitation samples yield a new local meteoric water line (δ2H = 7.1 * δ18O + 8.46) for the Azores region and the North Atlantic Ocean. The annual isotopic mean of precipitation shows a small range for the unweighted and precipitation mass‐weighted δ18O‐H2O values. Results show an inverse relation between the monthly δ18O‐H2O and the amount of precipitation, which increases in elevation and into the interior of the island. Higher amounts of precipitation (from convective storm systems) do not correspond to the most depleted values of stable isotopes in precipitation. Precipitation shows an orographic effect with depleted δ18O‐H2O values related to the Rayleigh effect. Monthly δ18O‐H2O values for individual precipitation sampling stations show little relationship to air temperature. Results show a local source of moisture during the summer with the characteristics of the first vapour condensate. The stable isotope composition of precipitation is strongly correlated to the NAO index, and δ18O‐H2O values show a statistically significantly trend towards enrichment since 1962 coincident with the increased air temperature and relative humidity due to climate change. Results are in line with observations of increasing sea surface temperature and relative humidity.  相似文献   

8.
We report a quantitative analysis of regional differences in the the oxygen isotope composition of river water and precipitation across the USA because data are now available to undertake a more geographically and temporally extensive analysis than was formerly possible. Maps of modern, mean annual δ18O values for both precipitation (δ18OPPT) and river water (δ18ORIV) across the 48 contiguous states of the USA have been generated using latitude and elevation as the primary predictors of stable isotope composition while also incorporating regional and local deviations based on available isotopic data. The difference between these two maps was calculated to determine regions where δ18ORIV is significantly offset from local δ18OPPT. Additional maps depicting seasonal and extreme values for δ18ORIV and δ18OPPT were also constructed. This exercise confirms the presence of regions characterized by differences in δ18ORIV and δ18OPPT and specifically identifies the magnitude and regional extent of these offsets. In particular, the Great Plains has δ18ORIV values that are more positive than precipitation, while much of the western USA is characterized by significantly lower δ18ORIV values in comparison with local δ18OPPT. The most salient feature that emerged from this comparison is the ‘catchment effect’ for the rivers. Because river water is largely derived from precipitation that fell upstream of the sample locality (i.e. at higher elevations) δ18ORIV values are often lower than local δ18OPPT values, particularly in catchments with high‐elevation gradients. Seasonal patterns in the isotopic data substantiate the generally accepted notion that amplitudes of δ18O variation are greatly dampened in river water relative to those of local precipitation. Copyright © 2005 John Wiley & Sons, Ltd.  相似文献   

9.
Spatial and temporal variations of the isotopic composition of precipitation over Thailand were investigated. The local meteoric water line for Thailand deviates slightly from the global meteoric water line, with lower slopes (7.62 ± 0.07, 7.59 ± 0.08) and intercepts (6.42 ± 0.39, 6.22 ± 0.42) using ordinary and precipitation weighted methods. Differences in spatial and temporal δ18O distributions between the tropical monsoon and tropical savanna climate zones were found due to differing moisture source contributions and seasonal precipitation patterns. The temporal data reveals that the northeast monsoon rains originate from isotopically-enriched local moisture with isotope values of −9.36 to −0.09‰ (mean − 3.73 ± 0.42‰), whereas the southwest monsoon clouds had a more significant rainout effect from Rayleigh distillation, with isotope values of −9.56 to −1.78‰ (mean − 5.40 ± 0.38‰). The precipitation amount at each site was negatively correlated with δ18O (−0.24 to −3.20‰ per 100 mm, R2 = 0.1–0.9). Furthermore, δ18O was negatively correlated with geography (latitude, altitude) for the southwest monsoon periods, as expected based on other observed correlations. However, an inverse correlation was seen in the northeast monsoon due to differing moisture transportation as part of the continental effect. The correlation coefficient (R) was higher in the southwest monsoon (−0.84 for latitude effect, −0.64 for altitude effect) than the northeast monsoon (0.67 for latitude effect, 0.35 for altitude effect). The spatial pattern of isotopic composition reflects the southwest monsoon more clearly than the northeast monsoon, but the two monsoons also have a cancelling impact on orographic patterns. An agreement of the δ18O and deuterium excess (d-excess) was a negative correlation and found to reflect precipitation sources and re-evaporation processes. The d-excess was slightly higher for the northeast monsoon, bringing moisture from the Pacific Ocean and travelling across the continent before reaching the observed stations. By contrast, the d-excess was relatively lower for the Indian Ocean's moisture in the southwest monsoon.  相似文献   

10.
Stable isotopes, 2Hwater, 18Owater as well as 18Osulphate and 34Ssulphate, were used to study the flow system of shallow groundwater and soil water at the base area of a former leaching heap at the uranium mining area of Ronneburg, Germany. The flow paths and water‐retention times were estimated by comparison of δ2H and δ18O values in groundwater and soil water to the δ2H and δ18O signature of precipitation, giving distinctive inputs of summer or winter precipitation. The points of measuring the groundwater were divided into three categories with different flow conditions: rapid flow, stagnant conditions and a transition zone by hierarchical cluster analysis of δ2H and δ18O values of groundwater. The transit time of groundwater in the rapid flow area is less than 6 months, whereas water in the stagnant zone is stored for at least 1 year. In soil water, a clear response to different input signals is detectable only in the 30‐cm horizon (retention time is about 6 months), whereas at deeper levels a mixing with older water is taking place. The isotopic composition of the dissolved sulphate was used to identify oxidation of sulphides as the source of sulphate. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

11.
Abstract

Stable isotopes are powerful research tools in environmental sciences and their use in ecosystem research is increasing. Stable isotope measurements allow the study of evapotranspiration fluxes, soil evaporation and leaf transpiration phenomena. Soil water and leaf water are the sources of the evapotranspiration that transfers large quantities of water from land to the atmosphere; as a result the isotopic composition of water left in the leaves is modified towards enrichment. Evaporation also changes the isotopic composition of water bodies creating a natural isotopic signal. The isotopic identity of soil water affects the oxygen isotopic signature of leaf and stem water. In this paper we present the isotopic data of bulk leaf water, showing the enrichment in isotopic value of oxygen due to evapotranspiration from leaves in conjunction with the isotopic signal of rainwater and other environmental factors such as humidity and temperature. Results suggest that the variation in the values of δ18O of Eucalyptus citriodora, Dalbergia sissoo, Melia azedarach and Pinus roxburghii is due to the seasonal changes in the δ18O of the source water for plants, i. e. rain. It is further observed that leaf water δ18O values are depleted during the months of July, August and September. This occurs due to the following reasons: (a) the sampling areas receive about 50% of the average annual rain during these months, and (b) rainfalls during these months are isotopically depleted compared with winter rains.

Citation Butt, S., Ali, M., Fazil, M. & Latif, Z. (2010) Seasonal variations in the isotopic composition of leaf and stem water from an arid region of Southeast Asia. Hydrol. Sci. J. 55(5), 844–848.  相似文献   

12.
A Lagrangian (Rayleigh) distillation model is used to track the evolution of stable isotopes in precipitation over mountainous terrain from the Pacific Coast of Canada to two alpine field sites in the Canadian Rocky Mountains. Precipitation δ18O at Vancouver constrains the model and air–mass back trajectories provide the water vapour pathway for 10 winter storm events. Isotopic values along storm pathways are modelled with a classical Rayleigh model that prescribes a linear decrease in temperature and pressure from initial to final conditions, and two models that account directly for orographic precipitation processes by: (i) applying an orographic rainfall model and (ii) using North American Regional Reanalysis data to calculate the change in vapour content along storm pathways. All models are significant predictors of snowpack δ18O, but the orographic model provides the best fit to precipitation‐weighted δ18O for each storm. The improvement in modelled δ18O by accounting for terrain along storm trajectories illustrates the need to account for orographically driven moisture loss when modelling vapour transport to ice core sites with mountainous upwind terrain. This finding is also applicable to isotopic studies of paleoaltimetry and source areas of groundwater recharge. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

13.
Deciduous forest covers vast areas of permafrost under severe dry climate in eastern Siberia. Understanding the water cycle in this forest ecosystem is quite important for climate projection. In this study, diurnal variations in isotopic compositions of atmospheric water vapour were observed in eastern Siberia with isotope analyses of precipitation, sap water of larch trees, soil water, and water in surface organic layer during the late summer periods of 2006, 2007, and 2008. In these years, the soil moisture content was considerably high due to unusually large amounts of summer rainfall and winter snowfall. The observed sap water δ18O ranged from ?17.9‰ to ?13.3‰, which was close to that of summer precipitation and soil water in the shallow layer, and represents that of transpired water vapour. On sunny days, as the air temperature and mixing ratio rose from predawn to morning, the atmospheric water vapour δ18O increased by 1‰ to 5‰ and then decreased by about 2‰ from morning to afternoon with the mixing ratio. On cloudy days, by contrast, the afternoon decrease in δ18O and the mixing ratio was not observed. These results show that water vapour that transpired from plants, with higher δ18O than the atmospheric water vapour, contributes to the increase in δ18O in the morning, whereas water vapour in the free atmosphere, with lower δ18O, contributes to the decrease in the afternoon on sunny days. The observed results reveal the significance of transpired water vapour, with relatively high δ18O, in the water cycle on a short diurnal time scale and confirm the importance of the recycling of precipitation through transpiration in continental forest environments such as the eastern Siberian taiga. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

14.
Over a 4‐month summer period, we monitored how forest (Pinus sylvestris ) and heather moorland (Calluna spp. and Erica spp.) vegetation canopies altered the volume and isotopic composition of net precipitation (NP) in a southern boreal landscape in northern Scotland. During that summer period, interception losses were relatively high and higher under forests compared to moorland (46% of gross rainfall [GR] compared with 35%, respectively). Throughfall (TF) volumes exhibited marked spatial variability in forests, depending upon local canopy density, but were more evenly distributed under heather moorland. In the forest stands, stemflow was a relatively small canopy flow path accounting for only 0.9–1.6% of NP and only substantial in larger events. Overall, the isotopic composition of NP was not markedly affected by canopy interactions; temporal variation of stable water isotopes in TF closely corresponded to that of GR with differences of TF‐GR being ?0.52‰ for δ2H and ?0.14‰ for δ18O for forests and 0.29‰ for δ2H and ?0.04‰ for δ18O for heather moorland. These differences were close to, or within, analytical precision of isotope determination, though the greater differences under forest were statistically significant. Evidence for evaporative fractionation was generally restricted to low rainfall volumes in low intensity events, though at times, subtle effects of liquid–vapour moisture exchange and/or selective transmission though canopies were evident. Fractionation and other effects were more evident in stemflow but only marked in smaller events. The study confirmed earlier work that increased forest cover in the Scottish Highlands will likely cause an increase in interception and green water fluxes at the expenses of blue water fluxes to streams. However, the low‐energy, humid environment means that isotopic changes during such interactions will only have a minor overall effect on the isotopic composition of NP.  相似文献   

15.
We present the results of a 3‐year monitoring programme of the stable isotope composition of lake water and precipitation at Taozi Lake, in the East Asian monsoon region of China. Our aims were to reveal the spatiotemporal pattern of variation of stable isotopes in a small closed‐basin lake and to quantitatively determine the impacts of precipitation and evaporation on the stable isotope composition of lake water under a humid monsoon climate. In the time domain, the stable oxygen isotopic ratio of the lake water (δ18OL) exhibited substantial seasonal and interannual variations, but the isotope variations between different precipitation events substantially exceeded seasonal and interannual variations. Compared with the stable isotopes in precipitation, δ18OL was substantially positive and dL was negative. In the space domains, the lake water was homogeneously mixed. Indicated by statistic analyses, precipitation plays a dominant role in dynamic of the lake stable isotope during precipitation events of relatively large magnitude, whereas the effect of evaporation is dominant during smaller precipitation events. Results advance our understanding of the stable isotope change rule in the process of lake water evaporation, and it is helpful to identify the climatic significance recorded in stable isotopic compositions of lake bottom sediments.  相似文献   

16.
Recharge areas of the Guarani Aquifer System (GAS) are particularly sensitive and vulnerable to climate variability; therefore, the understanding of infiltration mechanisms for aquifer recharge and surface run‐off generation represent a relevant issue for water resources management in the southeastern portion of the Brazilian territory, particularly in the Jacaré‐Pepira River watershed. The main purpose of this study is to understand the interactions between precipitation, surface water, and groundwater using stable isotopes during the strong 2014–2016 El Niño Southern Oscillation event. The large variation in the isotopic composition of precipitation (from ?9.26‰ to +0.02‰ for δ18O and from ?63.3‰ to +17.6‰ for δ2H), mainly associated with regional climatic features, was not reflected in the isotopic composition of surface water (from ?7.84‰ to ?5.83‰ for δ18O and from ?49.7‰ to +33.6‰ for δ2H), mainly due to the monthly sampling frequency, and groundwater (from ?7.04‰ to ?7.76‰ for δ18O and from ?49.5‰ to ?44.7‰ for δ2H), which exhibited less variation throughout the year. However, variations in deuterium excess (d‐excess) in groundwater and surface water suggest the occurrence of strong secondary evaporation during the infiltration process, corresponding with groundwater level recovery. Similar isotopic composition in groundwater and surface water, as well as the same temporal variations in d‐excess and line‐conditioned excess denote the strong connectivity between these two reservoirs during baseflow recession periods. Isotopic mass balance modelling and hydrograph separation estimate that the groundwater contribution varied between 70% and 80%, however, during peak flows, the isotopic mass balance tends to overestimate the groundwater contribution when compared with the other hydrograph separation methods. Our findings indicate that the application of isotopic mass balance methods for ungauged rivers draining large groundwater reservoirs, such as the GAS outcrop, could provide a powerful tool for hydrological studies in the future, helping in the identification of flow contributions to river discharge draining these areas.  相似文献   

17.
Characterization of spatial and temporal variability of stable isotopes (δ18O and δ2H) of surface waters is essential to interpret hydrological processes and establish modern isotope–elevation gradients across mountainous terrains. Here, we present stable isotope data for river waters across Kyrgyzstan. River water isotopes exhibit substantial spatial heterogeneity among different watersheds in Kyrgyzstan. Higher river water isotope values were found mainly in the Issyk‐Kul Lake watershed, whereas waters in the Son‐Kul Lake watershed display lower values. Results show a close δ18O–δ2H relation between river water and the local meteoric water line, implying that river water experiences little evaporative enrichment. River water from the high‐elevation regions (e.g., Naryn and Son‐Kul Lake watershed) had the most negative isotope values, implying that river water is dominated by snowmelt. Higher deuterium excess (average d = 13.9‰) in river water probably represents the isotopic signature of combined contributions from direct precipitation and glacier melt in stream discharge across Kyrgyzstan. A significant relationship between river water δ18O and elevation was observed with a vertical lapse rate of 0.13‰/100 m. These findings provide crucial information about hydrological processes across Kyrgyzstan and contribute to a better understanding of the paleoclimate/elevation reconstruction of this region.  相似文献   

18.
The δ2H and δ18O composition of 77 precipitation samples collected between January 2014 and April 2019 from two sites across the Guadalquivir Basin, SW Spain, were analysed. The first site is located in an urban area of Seville at 100 km distance to the Atlantic coast and the second site is located in a dune area of the Doñana National Park a few kilometres from the coast. Sampling was performed within intervals of at least 14 days if rain occurred but frequently intervals were longer according to the rainfall incidence. Samples from both sites are available for the period February 2016 to June 2018 with six samples containing identical rain events at both locations. Precipitation weighted averages and local meteoric water lines produced by weighting and non-weighting regression methods are presented for its use in hydrological applications. Results show a remarkably high variability in δ2H and δ18O values and precipitation weighted average d-excess values of 11.8‰ and 13‰ at the sites Plaza de España and Doñana, respectively. Temperature and amount effects were found to be weak. A significant influence of secondary evaporation for single rainfall events during summer was identified by enriched isotopic signatures with reduced d-excess values plotting close or below the global meteoric water line. Backward trajectory analysis of 115 days with daily rainfall above 3 mm yield a predominant Atlantic Ocean vapour source with negligible Mediterranean influence and therefore, d-excess variability is attributed to the different ocean surface conditions of relative humidity and sea surface temperature. Parallel sampling indicate very similar isotopic signatures at both sites and point to the existence of thermal effects of the Plaza de España site in Seville city during the summer season.  相似文献   

19.
A numerical model is proposed that describes the interaction between raindrops and water vapour near the planetary boundary layer to explain the “amount effect”. This model relates the intensity to the isotopic composition of precipitation. The model resolves raindrop sizes, and explicitly includes: (1) the isotopic equilibration time of raindrops that is drop‐size dependent; (2) raindrop transit times through the atmosphere; and (3) the evolution of the isotopic composition of vapour at various rain rates. At high rain rate, the precipitation through a layer is less equilibrated with the vapour because the isotopic equilibration time is long compared to the fast transit time, and there is a preponderance of large drops, which take longer to equilibrate. The δ18O of vapour in the lower atmosphere becomes lower as a result of the interaction with these raindrops of low δ18O, and the degree of depletion of 18O is higher when precipitation rates are high. The model reproduces time‐series observations of isotopic composition of precipitation in Japan, and a vapour replenishment rate is inferred by either advection or evaporation of about 5% of the precipitation rate. The results could be the basis for a new parameterization of the isotopic equilibration for different precipitation types and rates in General Circulation Models (GCMs). When the model is applied to a GCM, this parameterization is important for places where precipitation occurs at cold temperatures (<15 °C). Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

20.
A systematic study of the chemo-isotopic characteristics and origin of the groundwater was carried out at six major qanats in the hyper-arid Gonabad area, eastern Iran. These qanats as a sustainable groundwater extraction technology have a long history, supporting human life for more than a thousand years in this region. The Gonabad qanats are characterized by outlet electrical conductivity (EC) values of 750 to 3900 µS/cm and HCO3-Na-Mg and Cl-Na water types. The Gonabad meteoric water line (GnMWL) was drawn at the local scale as δ2H = 6.32×δ18O + 8.35 (with R2 = 0.90). It has a lower slope and intercept than the global meteoric water line due to different water vapor sources and isotope kinetic fractionation effects during precipitation in this arid region. The altitude effects on isotopic content of precipitation data were derived as δ18O = (−0.0031 × H(m.a.s.l))−1.3). The δ2H and δ18O isotopes signatures demonstrate a meteoric origin of the groundwater of these qanats. The shift of the qanat's water samples from the local meteoric water line (LMWL) in a dry period with higher temperatures is most probably due to evaporation during the infiltration process and water movement in qanat gallery. Based on the isotopic results and mass balance calculations, the qanats are locally recharged from an area between 2000 to 2400 m.a.s.l of nearby carbonate formations and coarse alluvial sediments. The dissolution of evaporate interlayers in Neogene deposits deteriorates the groundwater quality, especially in Baidokht qanat.  相似文献   

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