137Cs baseline levels in the Mediterranean and Black Sea: A cross-basin survey of the CIESM Mediterranean Mussel Watch programme     

《Marine pollution bulletin》2009,58(6-12):801-806

The common mussel Mytilus galloprovincialis was selected as unique biomonitor species to implement a regional monitoring programme, the CIESM Mediterranean Mussel Watch (MMW), in the Mediterranean and Black Seas. As of today, and upon standardization of the methodological approach, the MMW Network has been able to quantify ¹³⁷Cs levels in mussels from 60 coastal stations and to produce the first distribution map of this artificial radionuclide at the scale of the entire Mediterranean and Black Seas. While measured ¹³⁷Cs levels were found to be very low (usually <1 Bq kg⁻¹ wet wt) ¹³⁷Cs activity concentrations in the Black Sea and North Aegean Sea were up to two orders of magnitude higher than those in the western Mediterranean Basin. Such effects, far from representing a threat to human populations or the environment, reflect a persistent signature of the Chernobyl fallout in this area.  相似文献   

(137)Cs baseline levels in the Mediterranean and Black Sea: a cross-basin survey of the CIESM Mediterranean Mussel Watch programme     

Thébault H  Rodriguez Y Baena AM  Andral B  Barisic D  Albaladejo JB  Bologa AS  Boudjenoun R  Delfanti R  Egorov VN  El Khoukhi T  Florou H  Kniewald G  Noureddine A  Patrascu V  Pham MK  Scarpato A  Stokozov NA  Topcuoglu S  Warnau M 《Marine pollution bulletin》2008,57(6-12):801-806

The common mussel Mytilus galloprovincialis was selected as unique biomonitor species to implement a regional monitoring programme, the CIESM Mediterranean Mussel Watch (MMW), in the Mediterranean and Black Seas. As of today, and upon standardization of the methodological approach, the MMW Network has been able to quantify (137)Cs levels in mussels from 60 coastal stations and to produce the first distribution map of this artificial radionuclide at the scale of the entire Mediterranean and Black Seas. While measured (137)Cs levels were found to be very low (usually < 1 Bq kg(-1) wet wt) (137)Cs activity concentrations in the Black Sea and North Aegean Sea were up to two orders of magnitude higher than those in the western Mediterranean Basin. Such effects, far from representing a threat to human populations or the environment, reflect a persistent signature of the Chernobyl fallout in this area.  相似文献   

Geochronological reconstruction of Cs transport from the Coruh river to the SE Black Sea: comparative assessment of radionuclide retention in the mountainous catchment area     

S. B. Gulin  G. G. Polikarpov  J. -M. Martin 《Continental Shelf Research》2003,23(17-19):1811

The deposition record of ¹³⁷Cs was traced in the SE Black Sea sediments adjacent to the Coruh river mouth in comparison with the earlier studied chronology of ¹³⁷Cs deposition in front of the Danube delta (NW Black Sea). In both cases, the ¹³⁷Cs profiles showed two subsurface peaks attributable to maximum fallout of ‘bomb’ and Chernobyl radionuclides. The Coruh profile revealed a larger contribution of ‘bomb’ ¹³⁷Cs in comparison with the Chernobyl input, suggesting different coverage of NW and SE Black Sea regions with the Chernobyl fallout. The ¹³⁷Cs-derived dating showed that maximum deposition of particulate bound ¹³⁷Cs in sediments adjacent to the Coruh river mouth was delayed for 14 yr relative to date of Chernobyl accident, reflecting a buffer effect of the watershed soils. This transit time is 3 times longer than in the Danube catchment area, indicating a difference in retention processes in these mountainous (Coruh) and lowland (Danube) river basins. The ¹³⁷Cs profile in Coruh sediments showed penetration of ¹³⁷Cs to much greater depth than would be expected from ¹³⁷Cs fallout chronology, suggesting the sediment mixing rate of 1.3 cm² yr⁻¹. This value was used to evaluate deposition chronology of ¹³⁷Cs, applying the model developed for pulse fallout case. Comparing the measured and modelled data has allowed differentiation of the flood-induced discharge of the ¹³⁷Cs-containing suspended matter and the slower transit of eroded soil particles from the contaminated catchment areas. The obtained results may be used for the prediction of period when the pollutants, deposited over the river basins, can reach the Black Sea.  相似文献   

Difference of mercury bioaccumulation in red mullets from the north-western Mediterranean and Black seas   总被引：1，自引：0，他引：1  

M. Harmelin-Vivien  D. Cossa  D. B?naru  C. Mellon-Duval 《Marine pollution bulletin》2009,58(5):679-321

The relationships between total mercury (Hg) concentration and stable nitrogen isotope ratio (δ¹⁵N) were evaluated in Mullus barbatus barbatus and M. surmuletus from the Mediterranean Sea and M. barbatus ponticus from the Black Sea. Mercury concentration in fish muscle was six times higher in the two Mediterranean species than in the Black Sea one for similar sized animals. A positive correlation between Hg concentration and δ¹⁵N occurred in all species. Increase in Hg concentration with δ¹⁵N was high and similar in the two Mediterranean fishes and much lower in the Black Sea species. Since this was neither related to trophic level difference between species nor to methylmercury (MeHg) concentration differences between the north-western Mediterranean and the Black Sea waters, we suggested that the higher primary production of the Black Sea induced a dilution of MeHg concentration at the base of the food webs.  相似文献   

Water mass variation in the Mediterranean and Black Seas     

《Journal of Geodynamics》2012

The mass-induced sea level variability and the net mass transport between Mediterranean Sea and Black Sea are derived for the interval between August 2002 and July 2008 from satellite-based observations and from model data. We construct in each basin two time series representing the basin mean mass signal in terms of equivalent water height. The first series is obtained from steric-corrected altimetry while the other is deduced from GRACE data corrected for the contamination by continental hydrology. The series show a good agreement in terms of annual and inter-annual signals, which is in line with earlier works, although different model corrections influence the consistency in terms of seasonal signal and trend.In the Mediterranean Sea, we obtain the best agreement using a steric correction from the regional oceanographic model MFSTEP and a continental hydrological leakage correction derived from the global continental hydrological model WaterGAP2. The inter-annual time series show a correlation of 0.85 and a root mean square (RMS) difference of 15 mm. The two estimates have similar accuracy and their annual amplitude and phase agree within 3 mm and 23 days respectively. The GRACE-derived mass-induced sea level variability yields an annual amplitude of 27 ± 5 mm peaking in December and a trend of 5.3 ± 1.9 mm/yr, which deviates within 3 mm/yr from the altimetry-derived estimate.In the Black Sea, the series are less consistent, with lower accuracy of the GRACE-derived estimate, but still show a promising agreement considering the smaller size of the basin. The best agreement is realized choosing the corrections from WaterGAP2 and from the regional oceanographic model NEMO. The inter-annual time series have a correlation and RMS differences of 0.68 and 55 mm, their annual amplitude and phase agree within 4 mm and 6 days respectively. The GRACE-derived seawater mass signal has an annual amplitude of 32 ± 4 mm peaking in April. On inter-annual time scales, the mass-induced sea level variability is stronger than in the Mediterranean Sea, with an increase from 2003 to 2005 followed by a decrease from 2006 to 2008.Based on mass conservation, the mass-induced sea level variations, river runoff and precipitation minus evaporation are combined to derive the strait flows between the basins and with the Atlantic Ocean. At the Gibraltar strait, the net inflow varies annually with an amplitude of 52 ± 10 × 10⁻³ Sv peaking end of September (1 Sv = 10⁶ m³ s⁻¹). The inflow through the Bosphorus strait displays an annual amplitude of 13 ± 3 ×10⁻³ Sv peaking in the middle of March. Additionally, an increase of the Gibraltar net inflow (3.4 ± 0.8 × 10⁻³ Sv/yr) is detected.  相似文献   

Distribution and content of different artifical radio nuclides in the water of the North Sea during the years 1977 to 1981 (complemented with some results from 1982 to 1984)     

Dr. Hans Kautsky 《Ocean Dynamics》1985,38(5):193-224

Summary The measured concentrations of¹³⁷Cs in the water of the North Sea gained during the years 1977 to 1982 largely confirm the results found in the preceding years (Fig. 1). After a distinct maximum in 1978 — brought about by a particularly strong influx during 1977 — the total quantity of¹³⁷Cs present in the North Sea has reced, to around half of these peak values by the year 1982 (Table 1).On the way from the Sellafield Works near the Irish Sea as far as into the North Sea, a strong shift of the¹³⁷Cs:⁹⁰Sr ratio in favour of the⁹⁰Sr can be observed.By following the temporal course of that ratio at different measurement points, a transport time can be deduced of around 3 years between the Sellafield Works and the Pentland Firth; a further year would be needed to reach into the southeastern North Sea.The ratio Cs:Sr furthermore permits, in the southeastern North Sea, a good distinction between the watermasses comming from the north into the North Sea with respect to those that come through the Channel from the South. These masses practically flow side by side until about the entrance to the Skagerrak.The vertical distribution of the¹³⁷Cs shows, as is to be expected, seasonally conditioned differences. However, effects also occur, which — on the basis of the data available to date — do not yet permit a clear explanation.The⁹⁰Sr, as well as the^239+240Pu, present in the North Sea show an analogous distribution scheme compared with that of the¹³⁷Cs. Their concentrations lie far below that of the¹³⁷Cs (⁹⁰Sr 17.5%;^239+240Pu 0.03%).Tritium, on the other hand — with essentially higher concentrations — shows a completely different distribution, because it is principly introduced via the freshwater flowing in from the land.

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Verteilung und Gehalt verschiedener künstlicher Radionuklide im Wasser der Nordsee in den Jahren 1977 bis 1981 (ergänzt durch einige Ergebnisse von 1982 bis 1984)

Zusammenfassung Die in den Jahren 1977 bis 1982 gewonnenen Meßdaten der Aktivitätskonzentrationen von¹³⁷Cs im Wasser der Nordsee bestätigen weitgehend die in den vorhergehenden Jahren gefundenen Ergebnisse (Fig. 1) Nach einem deutlichen Maximum im Jahre 1978 — hervorgerufen durch eine besonders starke Zufuhr im Jahre 1977 —ist die in der Nordsee insgesamt vorhandene Menge an¹³⁷Cs bis zum Jahre 1982 wieder auf rund die Hälfte zurückgegangen (Tab. 1).Auf dem Weg von den Sellafield Works an der Irischen See bis in die Nordsee ist eine starke Verschiebung des¹³⁷Cs:⁹⁰Sr Verhältnisses zugunsten des⁹⁰Sr zu beobachten.Aus dem zeitlichen Verlauf dieses Verhältnisses an verschiedenen Meßpunkten ergeben sich Transportzeiten zwischen den Sellafield Works und dem Pentland Firth von rund 3 Jahren; bis in die südöstliche Nordsee wird ein weiteres Jahr benötigt.Das Verhältnis Cs:Sr erlaubt außerdem in der südöstlichen Nordsee eine gute Unterscheidung der aus der Nordsee bzw. durch den Kanal von Süden kommenden Wassermassen, die praktisch nebeneinander her bis etwa zum Beginn des Skagerraks fließen.Die Vertikalverteilung des¹³⁷Cs zeigt, wie zu erwarten ist, jahreszeitlich bedingte Unterschiede. Es treten aber auch Effekte auf, die sich anhand der bisher vorliegenden Daten noch nicht eindeutig erklären lassen.Das in der Nordsee vorhandene⁹⁰Sr sowie das^239+240Pu zeigen ein analoges Verteilungsschema verglichen mit dem des¹³⁷Cs. Ihre Konzentrationen liegen weit unter der des¹³⁷Cs (⁹⁰Sr 17,5%,^239+240Pu 0,03%).Das Tritium zeigt bei wesentlich höheren Konzentrationen dagegen eine völlig andere Verteilung, da seine Hauptzufuhr im wesentlichen über das von Land her zufließende Süßwasser erfolgt.

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Distribution et teneur de differents radionucleides artificiels, dans les eaux de la Mer du Nord entre les années 1977 et 1981 (completes par quelques résultats de 1982 à 1984)

Résumé Les mesures de concentration du Césium 137 dans les eaux de la Mer du Nord, acquises entre les années 1977 et 1982, confirment largement les résultats obtenus au cours des années précédentes. Après un net maximum en 1978 — occassionné par un apport particulièrement fort en 1977 — la quantité totale de Césium 137 présent en Mer du Nord a régressé,jusqu'en 1982, aux alentours de la moitié de ces valeurs maximales.Il a pu être observé une modification importante du rapport Césium 137/Strontium 90, en faveur du Strontium 90, sur le trajet de Sellafield Works prés de la Mer d'Irlande jusqu'à la Mer du Nord.En suivant l'évolution temporelle de la valuer de ce rapport en différents points de mesure, on peut en déduire une durée de transport d'environ 3 ans entre Sellafield Works et Pentland Firth; une année supplémentaire est ensuite nécessaire pour pénétrer en Mer du Nord Sud-orientale.En Mer du Nord Sud-orientale, le rapport Césium/Strontium permet en outre d'effectuer une nette distinction entre les masses d'eau pénétrant respectivement par le Nord dans la Mer du Nord et celles pénétrant par le Sud et venant de la Manche. Ces masses d'eau s'écoulent pratiquement côte à côte jusqu'à l'entrée du Skagerrak.Comme l'on pouvait s'y attendre, la distribution verticale du Césium est différente suivant les saisons. Cependant il apparaît également des effects qui, sur la base des données disponibles à ce jour, ne s'expliquent pas encore clairement.Le Strontium 90 aussi bien que le Plutonium 239+240 présent dans la Mer du Nord, montrent une distribution comparable, analogue à celle du Césium 137. Leurs concentrations sont bien inférieures à celle du Césium 137 (Strontium 90 17,5%; Plutonium 239+240 0,03%).Le tritium d'autre part, — avec des concentrations significativement plus fortes —montre une distribution complètement différente, due principalement au fait qu'il est introduit par l'intermédiaire de l'écoulement d'eau douce provenant de la terre.

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Elevated sedimentation in lake records linked to agricultural activities in the Ishikari River floodplain,northern Japan     

Young Sang Ahn  Futoshi Nakamura  Toshikazu Kizuka  Yugo Nakamura 《地球表面变化过程与地形》2009,34(12):1650-1660

The purpose of this study was to examine the historical change in sedimentation rates in lakes that have been impacted by river regulation and agricultural activities in the Ishikari River floodplain. We dated sediment cores using caesium‐137 (¹³⁷Cs) dating and tephrochronology, and we estimated sediment sources from ¹³⁷Cs concentrations in the topsoil of representative land covers. We found that, between 1739 and 1963, the distance between the lake and the main river channel and whether or not the lake was connected to the river affected the sedimentation rates. After 1963, agricultural drainage systems were established in the Ishikari River floodplain. The average sedimentation rate before and after the construction of drainage ditches varied between 1–66 and 87–301 mg cm^–2 a^–1, respectively. The increase in the sedimentation rate after 1963 was caused by the construction of a number of drainage networks, as well as extensive cultivation activity and/or fragmentation of the swamp buffers surrounding the lakes. The ¹³⁷Cs activities at the surfaces of the lake as well as the catchment‐derived ¹³⁷Cs contributions and ¹³⁷Cs inventory in the lake profiles were used to examine the sediment influx from the various drainage areas after the establishment of the drainage system. Our results indicate that the majority of the lake sediments were derived from cultivated areas, and therefore the catchment‐derived ¹³⁷Cs contribution in the lakes was strongly correlated with the sedimentation rate. The ¹³⁷Cs inventory across all of the lake profiles was also significantly greater than the atmospheric fallout. We identified a negative correlation between the ¹³⁷Cs lake profile inventory and the sedimentation rate. This is because the sediment originating from the drainage areas contained low ¹³⁷Cs concentrations, which diluted the overall concentration of ¹³⁷Cs in the lake sediment. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

Distribution of local Cs anomalies on the seafloor near the Fukushima Dai-ichi Nuclear Power Plant     

Blair Thornton  Seiki Ohnishi  Tamaki Ura  Naoteru Odano  Shun Sasaki  Tsuneo Fujita  Tomowo Watanabe  Kaoru Nakata  Tsuneo Ono  Daisuke Ambe 《Marine pollution bulletin》2013

An estimated 3.5 ± 0.7 × 10¹⁵ Bq of ¹³⁷Cs is thought to have been discharged into the ocean following the melt down at Fukushima Dai-ichi Nuclear Power Plant (F1NPP). While efforts have been made to monitor seafloor radiation levels, the sampling techniques used cannot capture the continuous distribution of radionuclides. In this work, we apply in situ measurement techniques using a towed gamma ray spectrometer to map the continuous distribution of ¹³⁷Cs on the seafloor within 20 km of the F1NPP. The results reveal the existence of local ¹³⁷Cs anomalies, with levels of ¹³⁷Cs an order of magnitude higher than the surrounding seafloors. The sizes of the anomalies mapped in this work range from a few meters to a few hundreds of meters in length, and it is demonstrated that the distribution of these anomalies is strongly influenced by meter scale features of the terrain.  相似文献   

Inorganic carbon and nutrient fluxes on the Arctic Shelf     

《Continental Shelf Research》2007,27(10-11):1584-1599

Historic data from the Russian-American Hydrochemical Atlas of Arctic Ocean together with data from the TRANSDRIFT II 1994 and TUNDRA 1994 cruises have been used to assess the spatial and inter-annual variability of carbon and nutrient fluxes, as well as air–sea CO₂ exchange in the Laptev and western East Siberian Seas during the summer season. Budget computations using summer data of dissolved inorganic phosphate (DIP), dissolved inorganic nitrogen (DIN) and dissolved inorganic carbon (DIC) gives that the Laptev Sea shelf is a net sink of DIP and DIN of 2.5×10⁶, 23.2×10⁶ mol d⁻¹, respectively, while it is a net source of DIC (excluding air–sea exchange) of 1249×10⁶ mol d⁻¹. In the East Siberian Seas the budget computations give 0.5×10⁶, −11.4×10⁶ and −173×10⁶ mol d⁻¹ (minus being a sink) for DIP, DIN, and DIC, respectively. In summers, the Laptev Sea Shelf is net autotrophic while the East-Siberian Sea Shelf is net heterotrophic, and both systems are weak net denitrifying. The Laptev Sea Shelf takes up 2.1 mmol CO₂ m⁻² d⁻¹ from atmosphere, whereas the western part of the East-Siberian Sea Shelf loose 0.3 mmol CO₂ m⁻² d⁻¹ to the atmosphere. The variability of DIP, DIN and DIC fluxes during summer in the different regions of the Laptev and East Siberian Seas depends on bottom topography, river runoff, exchange with surrounding seas and wind field.  相似文献   

The application of caesium‐137 measurements to investigate floodplain deposition in a large semi‐arid catchment in Queensland,Australia: a low‐fallout environment     

Kathryn J. Amos  Jacky C. Croke  Heiko Timmers  Philip N. Owens  Celia Thompson 《地球表面变化过程与地形》2009,34(4):515-529

Floodplains comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of large dryland floodplains is not well understood. Processes occurring on such floodplains are often difficult to observe, and techniques used to investigate smaller perennial floodplains are often not practical in these environments. This study assesses the utility of ¹³⁷Cs inventory and depth‐profile techniques for determining relative amounts of floodplain sedimentation in the Fitzroy River, northeastern Australia; a 143 000 km² semi‐arid river system. Caesium‐137 inventories were calculated for floodplain and reference location bulk soil cores collected from four sites. Depth profiles of ¹³⁷Cs concentration from each floodplain site and a reference location were recorded. The areal density of ¹³⁷Cs at reference locations ranged from 13 to 978 Bq m^–2 (0–1367 Bq m^–2 at the 95% confidence interval), and the mean value ± 2 (standard error of the mean) was 436 ± 264 Bq m^–2, similar to published data from other Southern Hemisphere locations. Floodplain inventories ranged from 68 to 1142 Bq m^–2 (0–1692 Bq m^–2 at the 95% confidence interval), essentially falling within the range of reference inventory values, thus preventing calculation of erosion or deposition. Depth‐profiles of ¹³⁷Cs concentration indicate erosion at one site and over 66 cm of deposition at another since 1954. Analysis of ^239+240Pu concentrations in a depositional core substantiated the interpretation made from ¹³⁷Cs data, and depict a more tightly constrained peak in concentration. Average annual deposition rates range from 0 to 15 mm. The similarity between floodplain and reference bulk inventories does not necessarily indicate a lack of erosion or deposition, due to low ¹³⁷Cs fallout in the region and associated high measurement uncertainties, and a likely influence of gully and bank eroded sediments with no or limited adsorbed ¹³⁷Cs. In this low‐fallout environment, detailed depth‐profile data are necessary for investigating sedimentation using ¹³⁷Cs. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

ENAA Studies of pollution in anoxic Black Sea sediments     

Octavian G. Duliu  Carmen Cristache  Otilia A. Culicov  Marina V. Frontasyeva 《Marine pollution bulletin》2009,58(6):827-831

The vertical distributions of five potential pollutants - Zn, As, Br, Sn, and Sb - were determined via epithermal neutron activation in the upper 50 cm of unconsolidated sediments from the Black Sea, which were collected 600 m below sea surface. This analysis demonstrated increasing concentrations towards the upper limits of sediments, which were greater than alert concentrations in the case of As and Br, and in accordance with Romanian Environment Regulations. The utilization of Chernobyl ¹³⁷Cs as a time marker allowed for dating of this region to the last 100 years.  相似文献   

Decadal scale variability of sea surface temperature in the Mediterranean Sea in relation to atmospheric variability     

Nikolaos Skliris  Sarantis Sofianos  Athanasios Gkanasos  Anneta Mantziafou  Vasilis Vervatis  Panagiotis Axaopoulos  Alex Lascaratos 《Ocean Dynamics》2012,62(1):13-30

Twenty-four years of AVHRR-derived sea surface temperature (SST) data (1985–2008) and 35 years of NOCS (V.2) in situ-based SST data (1973–2008) were used to investigate the decadal scale variability of this parameter in the Mediterranean Sea in relation to local air–sea interaction and large-scale atmospheric variability. Satellite and in situ-derived data indicate a strong eastward increasing sea surface warming trend from the early 1990s onwards. The satellite-derived mean annual warming rate is about 0.037°C year^–1 for the whole basin, about 0.026°C year^–1 for the western sub-basin and about 0.042°C year^–1 for the eastern sub-basin over 1985–2008. NOCS-derived data indicate similar variability but with lower warming trends for both sub-basins over the same period. The long-term Mediterranean SST spatiotemporal variability is mainly associated with horizontal heat advection variations and an increasing warming of the Atlantic inflow. Analysis of SST and net heat flux inter-annual variations indicates a negative correlation, with the long-term SST increase, driving a net air–sea heat flux decrease in the Mediterranean Sea through a large increase in the latent heat loss. Empirical orthogonal function (EOF) analysis of the monthly average anomaly satellite-derived time series showed that the first EOF mode is associated with a long-term warming trend throughout the whole Mediterranean surface and it is highly correlated with both the Eastern Atlantic (EA) pattern and the Atlantic Multidecadal Oscillation (AMO) index. On the other hand, SST basin-average yearly anomaly and NAO variations show low and not statistically significant correlations of opposite sign for the eastern (negative correlation) and western (positive correlation) sub-basins. However, there seems to be a link between NAO and SST decadal-scale variations that is particularly evidenced in the second EOF mode of SST anomalies. NOCS SST time series show a significant SST rise in the western basin from 1973 to the late 1980s following a large warming of the inflowing surface Atlantic waters and a long-term increase of the NAO index, whereas SST slowly increased in the eastern basin. In the early 1990s, there is an abrupt change from a very high positive to a low NAO phase which coincides with a large change in the SST spatiotemporal variability pattern. This pronounced variability shift is followed by an acceleration of the warming rate in the Mediterranean Sea and a change in the direction (from westward to eastward) of its spatial increasing tendency.  相似文献   

One century sedimentary record of Hg and Pb pollution in the Sagua estuary (Cuba) derived from Pb and Cs chronology     

M. Díaz-Asencio  C.M. Alonso-Hernndez  Y. Bolanos-lvarez  M. Gmez-Batista  V. Pinto  R. Morabito  J.I. Hernndez-Albernas  M. Eriksson  J.A. Sanchez-Cabeza 《Marine pollution bulletin》2009,59(4-7):108

The vertical distribution of Hg and Pb were determined in a sediment core collected from the Sagua estuary (North Cuba) that receives input from the Sagua river, one of the most polluted rivers discharging into the Cuban coastal environment. Depth profiles of metal concentrations were converted to time-based profiles using the ²¹⁰Pb dating method and confirmed with the ¹³⁷Cs fallout peak. The mean mass accumulation rate was estimated to be 0.17 ± 0.04 g cm⁻² y⁻¹ (mean sediment accumulation rate 0.52 ± 0.13 cm y⁻¹) and the core bottom was estimated to date back about 130 years. The historical sedimentary record showed a strong enrichment of mercury concentrations in the past decades, caused by the incomplete treatment of industrial wastes from a chlor-alkali plant with mercury-cell technology in the Sagua river basin. Lead fluxes to sediments showed a gradual increase from the 1920s to present, which agrees with a population increase in Sagua la Grande City. Fluxes of both metals have increased the past 25 years, with values reaching a maximum of 0.5 and 3.9 μg cm⁻² y⁻¹ for Hg and Pb, respectively.  相似文献   

Caesium-137: Its accumulation in a littoral community     

M.J. Broom  P.D. Grimwood  E.G. Bellinger 《Marine pollution bulletin》1975,6(2):24-26

The low-level radioactive liquid wastes which arise at the U.K. nuclear fuel reprocessing plant at Windscale on the Cumbria coast are discharged into the Irish Sea. These wastes are initially dispersed but they can also become reconcentrated in marine organisms. The present work discusses the concentrations of ¹³⁷Cs relative to those of potassium in the various stages of marine food chains and shows that discrimination occurs in favour of ¹³⁷Cs over potassium during the transfer between the different trophic levels.  相似文献   

Transport of the environmental radionuclides in an alpine watershed     

J. Dominik  D. Burrus  J.-P. Vernet 《Earth and Planetary Science Letters》1987,84(2-3)

The radionuclides¹³⁷Cs,²¹⁰Pb and⁷Be have been examined in the alpine Rhoˆne watershed (Switzerland) during a period of two years in order to evaluate their usefulness as tracers of the removal and transport rate of top-soil particles and particle-reactive contaminants of atmospheric origin. The specific activities of the radionuclides in fluvial suspension show a distinct seasonal pattern which depends on the hydrologic regime of the stream and the sources of the suspended matter. Input-output budgets based on the atmospheric deposition and fluvial removal of three radionuclides in the alpine Rhoˆne watershed are used to estimate their erosional residence times. The simplest one box model yields mean residence times of about 800 and 1400 years for¹³⁷Cs and²¹⁰Pb, respectively. The removal rate of short-lived⁷Be suggests that a part of the watershed (0.6–2.3% of the total surface) is exposed to a rapid erosion, in which the mean residence time of the radionuclides is in the range of 1–220 days. This has little influence on the calculated residence time of¹³⁷Cs but increases the estimated residence time of²¹⁰Pb in soil to over 1800 years. The use of²¹⁰Pb-⁷Be pair in fluvial output may be very helpful in the assessment of the impact of atmospheric pollutants on the water quality in rivers and lakes.  相似文献   

The potential for reference site resampling in estimating sediment redistribution and assessing landscape stability by the caesium-137 method     

Ross A. Sutherland 《水文研究》1998,12(7):995-1007

The objective of this study was to examine a new resampling methodology for estimating reference levels of ¹³⁷Cs in uneroded locations. Accurate and precise measurement of ¹³⁷Cs is required from reference locations to estimate long-term (c. 40 years) sediment redistribution (SRD) and landscape stability. Without reliable long-term, quantitative erosion data it is extremely difficult for land managers to make optimal decisions to ensure landscape sustainability. To determine the influence of ¹³⁷Cs reference site sampling, particularly under-sampling, on SRD and landscape stability, two statistical approaches were applied to a grid-based data set. Caesium-137 inventories in the reference location (n=36) indicated that data were normally distributed, with a mean inventory of 2150±130 Bq m⁻² (±95% confidence band) and a coefficient of variation of 18%. The two approaches used to determine the effect of under sampling included: (1) one-time random subsampling from the total sample collected, subsamples ranged from n=3 to n=30; from these data means and parametric confidence bands were calculated; and (2) random subsamples (n=3 to n=36) were selected from the total ¹³⁷Cs reference sample, and each subsample was in turn resampled 1000 times with replacement to establish a sampling distribution of means. Thus, an empirically derived mean and 95% confidence bands were established. Caesium-137 activities determined from each approach were input into equations to estimate SRD from two cultivated fields. Results indicate that the one-time random sampling approach for subsamples of size ≤12 significantly over- or under-estimated net SRD, particularly from the gently sloping agricultural field. Computer-intensive resampling produced significantly better estimates of net SRD when compared with the random one-sample approach, especially when a subsample of size three was used. Landscape stability, based on partitioning the agricultural fields into areas exhibiting erosion, stability and deposition, was better approximated for both fields by applying resampling. © 1998 John Wiley & Sons, Ltd.  相似文献   

Modelling temporal trends of 137Cs and 99Tc concentrations in Fucus vesiculosus from the eastern Irish coastline     

Cournane S  Vintró LL  Mitchell PI  McMahon CA  Smith K  Long S 《Marine pollution bulletin》2011,62(11):2337-2344

Time series of ¹³⁷Cs and ⁹⁹Tc activity concentrations in the brown seaweed Fucus vesiculosus and seawater, gathered at three locations on the eastern Irish coastline during the period 1988-2008, have been modelled using a novel approach incorporating a variable uptake rate in the seaweed. Seasonal variations in the time series, identified using spectral analysis, were incorporated into the model which was used to determine transfer kinetic parameters and to predict ¹³⁷Cs and ⁹⁹Tc concentrations in seaweed, as influenced by levels in ambient seawater. An optimisation method combining evolutionary and grid search minimisation techniques was adopted to determine the best values for the model parameters, from which concentration factors (CF) and biological half-lives (tb_1/2) for ¹³⁷Cs and ⁹⁹Tc in F. vesiculosus were calculated. CF values of 170-179 and 1.1 × 105 l kg⁻¹ (dry weight) were obtained for ¹³⁷Cs and ⁹⁹Tc, respectively, while the corresponding tb_1/2 values were 39-47 and 32 days, respectively.  相似文献   

Review of heat flow data from the eastern Mediterranean region     

Yoram Eckstein 《Pure and Applied Geophysics》1978,117(1-2):150-159

Heat flow data from the eastern Mediterranean region indicates an extensive area of low heat flow, spreading over the whole basin of the Mediterranean east of Crete (Levantine Sea), Cyprus, and northern Egypt. The average of the marine heat flow measurements in the Levantine Sea is 25.7±8.4 mW/m², and the heat flow on Cyprus is 28.0±8.0 mW/m². The estimated values of heat flow in northern Egypt range from 38.3±7.0 to 49.9±9.3 mW/m², apparently with no consistent trend. To the east, on the coast of Israel, the heat flow values increase, ranging from 36.6±22.4 to 56.7±14.2 mW/m² along a SSE trend. The trend apparently correlates with an increase in crustal thickness, which is about 23 km at the north-west base of the Nile-Delta-cone, and close to 40 km beneath Israel.Contribution No. 157, Department of Geology, Kent State University, Kent, Ohio, USA.  相似文献   

The use of 137Cs as a tracer in an erosion study in south limburg (the Netherlands) and the influence of chernobyl fallout     

A. P. J. De Roo 《水文研究》1991,5(2):215-227

The ¹³⁷Cs radioactivity of soils was used as a tracer of soil erosion in a catchment in the Netherlands: 143 samples were analysed to map the ¹³⁷Cs redistribution using geostatistical interpolation methods. Caesium-137 activities on grassland are significantly higher than on arable land. Also, ¹³⁷Cs activities on waning slopes are higher and activities on steep slopes are lower. The soil erosion estimates, derived from the ¹³⁷Cs data, are used to validate the USLE erosion model. The recent Chernobyl nuclear accident also contributed to the ¹³⁷Cs activity. However, the Chernobyl input of ¹³⁷Cs, with a constant ratio of 1.765:1 to ¹³⁴Cs, cannot be used as a tracer of soil erosion. Because of the rapid decay of ¹³⁴Cs, we will not be possible to separate the sources of ¹³⁷Cs in the near future in areas significantly influenced by Chernobyl fallout and in these areas ¹³⁷Cs can no longer be used as a soil erosion tracer.  相似文献   

Animal-sediment relationships: Evaluating the ‘Pearson-Rosenberg paradigm’ in Mediterranean coastal lagoons     

P. Magni  D. Tagliapietra  L. Balthis  S. Como  G. Giordani  F. Maltagliati  A. Rismondo  P. Tomassetti 《Marine pollution bulletin》2009,58(4):478-337

We investigated the applicability of the Pearson-Rosenberg (P-R) conceptual model describing a generalized pattern of response of benthic communities in relation to organic enrichment to Mediterranean Sea coastal lagoons. Consistent with P-R model predictions, benthic diversity and abundance showed two different peaks at low (>2.5-5 mg g⁻¹) and high (>25-30 mg g⁻¹) total organic carbon (TOC) ranges, respectively. We identified TOC thresholds indicating that risks of reduced benthic diversity should be relatively low at TOC values < about 10 mg g⁻¹, high at TOC values > about 28 mg g⁻¹, and intermediate at values in-between. Predictive ability within these ranges was high based on results of re-sampling simulation. While not a direct measure of causality, it is anticipated that these TOC thresholds should serve as a general screening-level indicator for evaluating the likelihood of reduced sediment quality and associated bioeffects in such eutrophic systems of the Mediterranean Sea.  相似文献