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1.
We examined nutrient flux, uptake, and transformation along a spring-fed stream in the Ozark region of Missouri, USA, over the year 2006. Water in Mill Creek originates from several springs, with a single spring contributing over 90% of the stream discharge during much of the year of study. Soluble reactive phosphate concentrations were usually low (<10 μg L−1) along Mill Creek, but peaked during high discharge. Concentrations of dissolved inorganic nitrogen (DIN) were relatively high in the spring water, mainly as nitrate, but usually declined across a small pond and the 10-km length of Mill Creek. During low flows in summer and early autumn, the stream removed over 300 μg L−1 of DIN over its 10-km length, or about 80% of the initial amount. DIN retention along the stream, as a percentage of the DIN upstream, was related mainly to discharge, with higher flows having much higher DIN concentrations. The net uptake rate of DIN uptake was 0.91 μg m−2 s−1 in the stream during summer baseflow. The uptake rate declined downstream for different reaches and was closely related to DIN concentration. In experimental channels, uptake by epilithic algae was one significant sink for nitrate-N in Mill Creek. In 2006, inorganic nutrient export during a single day after a spring storm was similar to export during 40–100 days of low flow conditions in summer and early autumn. Our results suggest that significant nutrient retention can occur during baseflow periods via biological uptake, whereas substantial export occurs during high flow conditions.  相似文献   

2.
Streams can be classified as stable or unstable, depending on the stage of channel evolution. Many streams of the southern Piedmont in United States have high sediment loads and are listed as impaired under the total maximum daily load (TMDL) program and may be unstable. It is not clear as to what the target (reference) load or remediation measures should be for unstable streams. The objective of this study was to determine the relative channel stability for a typical southern Piedmont stream using rapid geomorphic assessments (RGAs) and sediment yield analysis. The results were supported through a sediment fingerprinting analysis. RGAs were performed along 52 reaches on the North Fork Broad River (NFBR) main stem and two tributaries. Annual sediment yields were calculated and compared with yields in the southern Piedmont for stable streams that are resilient to degradation or aggradation and unstable streams that are susceptible to such disturbances. Majority of the NFBR main stem was found to be unstable with signs of geomorphic instability in the form of degradation and aggradation. The estimated average annual sediment yield was 0·78 T ha?1 year?1. By comparison, the median annual yield is 0·20 T ha?1 year?1 for stable streams and 0·48 T ha?1 year?1 for unstable streams in the Piedmont ecoregion with comparable drainage basin size. We conclude that the NFBR is in an unstable stage of channel evolution. Sediment fingerprinting proved that majority of the stream‐suspended sediment emanated from eroding stream channels. The methods outlined in this study have implications for the reference condition and remediation efforts related to stream turbidity and stream channel restoration. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

3.
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4.
Despite the known importance of water temperature for river ecosystems, the thermal regime of streams and rivers can be heavily modified by afforestation. Although the nature of the heat budget affecting streams in forested catchments shows high variability in space and time, most of the studies of stream temperature response to afforestation have lacked replication among streams. This study examined the impacts of coniferous forest plantations on stream water temperature at six sites (three forested and three open moorland) in the Yorkshire Dales, northern England. Our aim was to test the hypothesis that afforestation would alter the thermal regime of streams, leading to reduced year‐round thermal variability, and cooler summer/warmer winter water temperatures, relative to streams flowing across open moorland. Data collected from April 2007 to March 2009 showed similar thermal dynamics among all six streams over the study period, although variability in forested streams was markedly lower as expected. Mean and maximum daily water temperatures were significantly higher in open moorland streams for much of the year but while some forested streams were warmer than individual moorland streams during winter months (November to February), there was considerable overlap in water temperature between moorland and forest streams. Most stream temperature records showed evidence of low/no winter flow and freezing. These results contrast with many previous studies that have reported warmer temperatures in forested versus open moorland streams during winter, a finding that most likely reflects site‐specific hydrological, geomorphological and climatological influences on water temperature in addition to afforestation. This study demonstrates the need for replication of hydrological monitoring when examining the effects of basin‐scale management practices and provides further evidence for changes in stream thermal regime following afforestation, a practice that is likely to increase in future due to growing demands for increased forest cover in the UK uplands. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

5.
The American cranberry (Vaccinium macrocarpon Ait.) is an important part of the cultural heritage and economy of Southeastern Massachusetts, yet water quality concerns and wetland protection laws challenge its commercial production. Here, we report inputs and outputs of water, nitrogen (N), and phosphorus (P) for a 2.12‐ha cranberry bed over a 2‐year period from 2013 to 2015. Water‐budget analysis indicated that precipitation contributed 40%, floodwater 37%, irrigation 15%, and groundwater 8% of water inputs to the cranberry bed. Minor annual variation in surface water discharge (~90 mm·year?1 or 3%) contrasted with large decreases in net (= outputs ? inputs) nutrient export, from 16.2 to 9.1 kg N·ha?1·year?1 for total (dissolved + suspended particulate) nitrogen (TN) and from 3.34 to 1.47 kg P·ha?1·year?1 for total phosphorus (TP) between Years 1 and 2. Annual variation in net TN and TP export was tied to decreases in spring and summer nutrient export and controlled by the combined effects of fertilizer management, soil biogeochemistry, and hydrology. The relatively high spring TN export in Year 1 was associated with coincident increases in soil temperature and rainfall. A second factor was the timing of fertilizer application, which occurred 1 day prior to a major summer storm (i.e., third largest daily rainfall since 1926) and was responsible for up to 15% and 9% of the Year 1 TN and TP export, respectively. Nutrient budgets, which balanced water and fertilizer inputs with water, fruit, and vegetative outputs, were consistent with the burial of 21.6 kg N·ha?1·year?1 and 7.27 kg P·ha?1·year?1. Field measurements indicated that burial would increase TN and TP in the shallow (0–5 cm) rooting zone by 14% and 6%, respectively, which seemed plausible based on the relatively young age of the bed (4–5 years) and new root growth patterns in Vaccinium plants.  相似文献   

6.
A reliable and economical method for the estimation of nutrient export (e.g. phosphorus) in stream flow from catchments is necessary to quantify the impact of land use or land use change upon aquatic systems. The transport of phosphorus (P) from soil to water is known to impact negatively on water quality. A key observation from studies is that most P export occurs during high stream flow. However, it is not yet clear how flood-antecedent conditions affect the P export during flood events. In this study, the P loss from soil to water as represented by soluble reactive phosphorus (SRP) in stream waters from three different catchments, varying in land use, scale and location in Ireland was monitored over 1 year. This study examined the role of antecedent stream flow conditions on SRP export and identifies a catchment-specific relationship between SRP flood event load (EL) and a flow ratio (FR). The FR is defined as the ratio of the flood event volume (EV) to the pre-event volume (PEV). The latter is the cumulative flow volume for a number of days preceding the event. This PEV period was found to be longer (average 81 days) in the grassland catchments which were known to be saturated with soil P than in the forested catchments (average 21 days) with minimal soil P. This FR ratio is a measure of the antecedent hydrological state (wet or dry) of the catchment. For SRP for each catchment, a specific relationship between SRP EL and FR was identified. The annual SRP export was estimated, using this ratio and compared with the concentration/discharge (C/Q) method. The new flow ratio method was used with data from 12 flood events during the year to estimate an annual export of SRP. For the two grassland catchments in the study, using the FR method, we estimated an SRP export of 1.77 and 0.41 kg ha−1 yr−1. Using the C/Q method, for the same sites, our estimate of SRP export was 1.70 and 0.50 kg ha−1 yr−1 respectively. The C/Q method used SRP concentrations covering 40% of the year while the FR method used only 12 flood events covering less than 2% of the year. This new method which takes account of the antecedent flow state of the river is an alternative to and may be more promising than the traditional C/Q method, particularly when short duration or flood sampling of water quality is carried out.  相似文献   

7.
Abstract

The chemistry of streamwater, bulk precipitation, throughfall and soil waters has been studied for three years in two plantation forest and two moorland catchments in mid-Wales. Na and CI are the major ions in streamwater reflecting the maritime influence on atmospheric inputs. In all streams, baseflow is characterised by high pH waters enriched in Ca, Mg, Si and HCO3. Differences in baseflow chemistry between streams reflect the varying extent of calcite and base metal sulphide mineralization within the catchments. Except for K, mean stream solute concentrations are higher in the unmineralized and mineralized forest catchments compared with their respective grassland counterparts. In the forest streams, storm flow concentrations of H+ are approximately 1.5 times and Al four times higher than in the moorland streams. Annual catchment losses of Na, Cl, SO4, NO3, Al and Si are greatest in the forest streams. In both grassland and forest systems, variations in stream chemistry be explained by mixing waters from different parts of the catchment, although NO3 concentrations may additionally be controlled by N transformations occurring between soils and streams. Differences in stream chemistry and solute budgets between forest and moorland catchments are related to greater atmospheric scavenging by the trees and changes in catchment hydrology consequent on afforestation. Mineral veins within the catchment bedrock can significantly modify the stream chemical response to afforestation.  相似文献   

8.
Anders Malmer 《水文研究》2004,18(5):853-864
In 1998 a wild fire struck a paired catchment research area under long‐term monitoring of hydrological and nutrient budgets. Streamwater quality as concentrations of dissolved and suspended particulate matter was monitored during 1·5–2·5 years after the fire in streams from seven different catchments. As the catchments, due to earlier experimental treatments, had different vegetations, varying effects related to different fire intensities were observed. The highest, mean stormflow, suspended sediment concentrations resulted from intensive fire in secondary vegetation that had experienced severe soil disturbance in previous treatments (crawler tractor timber extraction 10 years earlier). Stormflow concentrations were typically still about 400 mg l?1 in 1999 (10–21 months after the fire), which was about the maximum recorded concentration in streams during initial soil disturbance in 1988. Forest fire in natural forest resulted in less than half as high stormflow concentrations. For dissolved elements in streamwater there was a positive relation between fuel load (and fire intensity) and concentration and longevity of effects. Stream baseflow dissolved nutrient concentrations were high in the months following the fire. Mean baseflow K concentrations were 8–15 mg l?1 in streams draining catchments with intensive fire in secondary vegetation with large amounts of fuel. After controlled fire for forest plantation establishment in 1988 corresponding concentrations were 3–5 mg l?1, and after forest fire in natural forest in this study about 2 mg l?1. This study shows differences in response from controlled fire for land management, forest fire in natural forests and wild fires in manmade vegetations. These differences relate to resistance and resilience to fire for the involved ecosystems. There is reason to believe that wild fires and repeated wild fires during or after droughts, in successions caused by human influence, may lead to larger losses of ecosystem nutrient capital from sites compared with forest fires in natural forests. As fire in the humid tropics becomes more common, in an increasingly spatially fragmented landscape, it will be important to be aware of these differences. Copyright © 2004 John Wiley & Sons, Ltd.  相似文献   

9.
Solute concentrations and fluxes in rainfall, throughfall and stemflow in two forest types, and stream flow in a 90 ha catchment in southern Chile (39°44′S, 73°10′W) were measured. Bulk precipitation pH was 6·1 and conductivity was low. Cation concentrations in rainfall were low (0·58 mg Ca2+ l?1, 0·13 mg K+ l?1, 0·11 mg Mg2+ l?1 and <0·08 mg NH4–N l?1), except for sodium (1·10 mg l?1). Unexpected high levels of nitrate deposition in rainfall (mean concentration 0·38 mg NO3–N l?1, total flux 6·3 kg NO3–N ha?1) were measured. Concentrations of soluble phosphorous in bulk precipitation and stream flow were below detection limits (<0·09 mg l?1) for all events. Stream‐flow pH was 6·3 and conductivity was 28·3 μs. Stream‐water chemistry was also dominated by sodium (2·70 mg l?1) followed by Ca, Mg and K (1·31, 0·70 and 0·36 mg l?1). The solute budget indicated a net loss of 3·8 kg Na+ ha?1 year?1, 5·4 kg Mg2+ ha?1 year?1, 1·5 kg Ca2+ ha?1 year?1 and 0·9 kg K+ ha?1 year?1, while 4·9 kg NO3–N ha?1 year?1 was retained by the ecosystem. Stream water is not suitable for domestic use owing to high manganese and, especially, iron concentrations. Throughfall and stemflow chemistry at a pine stand (Pinus radiata D. Don) and a native forest site (Siempreverde type), both located within the catchment, were compared. Nitrate fluxes within both forest sites were similar (1·3 kg NO3–N ha?1 year?1 as throughfall). Cation fluxes in net rainfall (throughfall plus stemflow) at the pine stand generally were higher (34·8 kg Na+ ha?1 year?1, 21·5 kg K+ ha?1 year?1, 5·1 kg Mg2+ ha?1 year?1) compared with the secondary native forest site (24·7 kg Na+ ha?1 year?1, 18·9 kg K+ ha?1 year?1 and 4·4 kg Mg2+ ha?1 year?1). However, calcium deposition beneath the native forest stand was higher (15·9 kg Ca2+ ha?1 year?1) compared with the pine stand (12·6 kg Ca2+ ha?1 year?1). Copyright © 2002 John Wiley & Sons, Ltd.  相似文献   

10.
Though high rates of nitrate (NO3−) leaching from forests are undesirable, the factors significantly regulating stream NO3− concentration is not clarified yet. In Japan, not only near metropolitan areas but also the Japan Sea-side area with heavy snowfall is well known for receiving more than 10 kg-N ha−1 year−1 of nitrogen (N) deposition. However, NO3− concentration in stream water is relatively low in the Japan Sea-side area compared with its concentration in other areas. We examined important environmental factors regulating stream NO3− concentrations at baseflow condition in a large region of Japan, the Kinki region (KIN) including a part of Japan Sea-side (JSK) using Random Forest regression. The amounts of N deposition and precipitation were common regulating factors for stream NO3− concentration at baseflow condition. Random forest showed the significant correlation between the factors related to ecosystem N retention and stream NO3− concentration at baseflow condition, and it suggests that large N deposited during the growing season was incorporated into the ecosystem in the entire KIN. Heavy rain and snow flush N and wash out N accumulated in the surface soil, causing small N accumulation in forests. Also, large precipitation dilute NO3− concentration in baseflows. These things lowered stream NO3− concentration at baseflow condition. Especially in JSK, most of N deposed with the heavy snow flushed out during the snowmelt period. We provided the first statistical confirmation using Random Forest regression that N accumulation and cycling in forest ecosystems were related to NO3− leaching from forests into streams.  相似文献   

11.
Agricultural, forestry-impacted and natural catchments are all vectors of nutrient loading in the Nordic countries. Here, we present concentrations and fluxes of total nitrogen (totN) and phosphorus (totP) from 69 Nordic headwater catchments (Denmark: 12, Finland:18, Norway:17, Sweden:22) between 2000 and 2018. Catchments span the range of Nordic climatic and environmental conditions and include natural sites and sites impacted by agricultural and forest management. Concentrations and fluxes of totN and totP were highest in agricultural catchments, intermediate in forestry-impacted and lowest in natural catchments, and were positively related %agricultural land cover and summer temperature. Summer temperature may be a proxy for terrestrial productivity, while %agricultural land cover might be a proxy for catchment nutrient inputs. A regional trend analysis showed significant declines in N concentrations and export across agricultural (−15 μg totN L−1 year−1) and natural (−0.4 μg NO3-N L−1 year−1) catchments, but individual sites displayed few long-term trends in concentrations (totN: 22%, totP: 25%) or export (totN: 6%, totP: 9%). Forestry-impacted sites had a significant decline in totP (−0.1 μg P L−1 year−1). A small but significant increase in totP fluxes (+0.4 kg P km−2 year−1) from agricultural catchments was found, and countries showed contrasting patterns. Trends in annual concentrations and fluxes of totP and totN could not be explained in a straightforward way by changes in runoff or climate. Explanations for the totN decline include national mitigation measures in agriculture international policy to reduced air pollution and, possibly, large-scale increases in forest growth. Mitigation to reduce phosphorus appears to be more challenging than for nitrogen. If the green shift entails intensification of agricultural and forest production, new challenges for protection of water quality will emerge possible exacerbated by climate change. Further analysis of headwater totN and totP export should include seasonal trends, aquatic nutrient species and a focus on catchment nutrient inputs.  相似文献   

12.
Abstract

This study presents an analysis of three hydrological years (2007/08, 2008/09 and 2009/10) of precipitation, runoff and sediment yield collected from a small (669.7 ha) semi-arid watershed in southeastern Spain (Lanjarón). At the watershed outlet the runoff, suspended sediment concentration, total solute concentrations and dissolved nutrients (N-NO3, N-NH4, H2PO4 and K) in streamflow were continuously monitored. The runoff was highly variable, ranging between 53.4 and 154.7 mm year?1, with an average of 97.6 mm year?1. In contrast, sediment yields were more regular, averaging 1.8 Mg ha?1 year?1. The hydrological response of the watershed depended mainly on rainfall intensity. Formerly, 32% of the watershed was forested and runoff was more regular, despite the typical Mediterranean rainfall cycle; however, due to forest area reduction to 17% and the increase in abandoned farmland area (18%) in recent decades, the runoff variability has increased. Greater amounts of solutes (32.7 Mg ha?1 year?1) were exported, so that this water is considered as poor for irrigation use. The temporal nutrient export was related to seasonal discharge fluctuations as well as daily concentrations. In addition, the nutrient concentrations of the water discharged were lower than threshold limits cited in water-quality standards for agricultural use and for potable water, with the exception of K (65.9 mg L?1), which may degrade surface waters as well as irrigated soils. Thus, hydrological and erosive processes depended on the watershed features, but also on prior conditions in combination with the characteristics of rainfall episodes.

Citation Durán, Z.V.H., Francia, M.J.R., Garcia, T.I., Rodríguez, P.C.R., Martínez, R.A., and Cuadros, T.S., 2012. Runoff and sediment yield from a small watershed in southeastern Spain (Lanjarón): implications for water quality. Hydrological Sciences Journal, 57 (8), 1610–1625.  相似文献   

13.
In 2002–2004 we undertook six sampling campaigns during representative hydrological stages in a 901 km2 Estonian lowland catchment to quantify the spatial and seasonal variability of in‐stream dissolved inorganic nitrogen (DIN) and dissolved reactive phosphorus (DRP) concentrations and to identify the influence of land cover and landscape structure. Using a synoptic approach we mapped concentrations in all stream orders. Using linear regression, the relations between the share of agricultural land and log‐transformed in‐stream concentrations were explored. Both the share of agricultural land in the entire ‘area of influence’ upstream from a sampling location, as well as the share in a 150‐m buffer around the stream were used as linear regression input variables. Log‐transformed DIN and DRP concentration variability was highest for lower order streams, while it averaged out in higher order streams during all seasons. Between‐season variation in export can mainly be attributed to discharge variation. In extremely dry periods, there are no significant relations between land cover/structure and in‐stream ln(DIN) concentrations and only weak relations for ln(DRP) concentrations. In other seasons, the share of agricultural land in the upstream area can explain concentrations in higher order streams better than in lower order streams. The prediction of ln(DIN) concentrations in lower order streams can be improved by using the share of agricultural land in a 150‐m buffer as an input variable. This indicates that hydrological connectivity must be taken into account for lower order streams, while land cover shares are enough to explain concentrations for higher order streams. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

14.
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15.
A. Malmer  H. Grip 《水文研究》1994,8(3):195-209
Streamwater chemistry was monitored for five years in six streams in a paired catchment experiment in Mendolong, Sabah, Malaysia, comparing the effects of different ways to establish forest plantations with Acacia mangium. At the start of the monitoring in 1985 three catchments were covered with selectively logged rain forest (W4-W6) and three with secondary vegetation after forest fire (W1-W3). The treatments were: (1) clearing of secondary vegetation, burning and planting (W1 and W2); (2) clear-felling, crawler tractor extraction, burning and planting (W5); and (3) clear-felling, manual extraction, no burning and planting (W4). W3 and W6, with no treatment, were monitored as control catchments. Reference monitoring at all streams was for two years and was followed by treatments which lasted for nine months before the full establishment of a new vegetation cover. This paper covers monitoring for a further 2.5 years. The soil types of the catchments were Orthic Acrisol in W3, Gleyic Podsol in W6 and a mix of both soil types in the other catchments. The effect of treatments on streamwater chemistry was clear at both base- and stormflows. Concentrations of major plant nutrients (N, P and K.) became positively correlated to streamflow during treatments. The response of leaching from slash at clear-felling was fast and larger from the clear-felling residues (W4 and W5) than the cleared secondary vegetation (W1 and W2). The intense response to burning was more marked. The stormflow period mean nutrient concentrations were approximately 10-fold for N and K and 10-100 fold for P after burning compared with baseflow mean concentrations over the same period. Significant differences in baseflow concentrations in treated streams generally lasted one year for most elements, but elevated concentrations were still detectable after three years. The first large pulse of leaching was related to mineralization after tree-felling and particularly burning. The longer lasting elevated concentrations in baseflow were associated with the loss of weathering products. The amounts of nutrients lost, calculated by regression analysis as the effect of treatment compared with control, were found to be higher with the degree of vegetation killed and with increased soil disturbance. Consequently, normal forestry practices, with crawler tractor extraction and burning before planting, created the largest leaching losses. The total calculated effect of losses in total N, P and K were (i) W1 + W2 0.5, 1.8, 83.9; (ii) W4 0.8, 0.8, 105.6; and (iii) W5 1.3, 1.3, 189.4 kg ha?1 for the period of 33 months during and after treatment. With normal forestry practice using crawler tractors and with burning before planting (W5), the treatment-induced loss of K was equivalent to 86% of the content of easily decomposed parts of the biomass (leaves, twigs, fine roots and ground vegetation) of the old forest, or larger than K removed by harvest. Exhaustion effects of lowered leaching after repeated burning (forest fire and pre-planting fire) was observed for several elements, indicating possible nutrient deficiencies.  相似文献   

16.
This study presents input–output budgets of total dissolved nitrogen (TDN), dissolved organic N (DON) and dissolved inorganic N (DIN) for a reservoir in a peatland catchment in the south Pennines (UK). This site receives high levels of atmospheric inorganic N deposition, in the range of 26 kg N ha?1 yr?1. The results show that the reservoir retains ~21 to 31% of the annual TDN input (8806 ± 741 kg N). Approximately 39 to 55% of DON (3782 ± 653 kg N) and 6 to 13% of DIN (5024 ± 349 kg N) were retained/processed. A long water retention time (104 days), average annual pH of 6.5, high concentrations of DIN in the reservoir water and a deep water column suggest that denitrification is potentially a key mechanism of N retention/removal. The results also demonstrate that DON is potentially photodegraded and utilized within the reservoir, particularly during the summer season when 58 to 80% of DON input (682 ± 241 kg N) was retained, and a net export of DIN (~34 kg N) was observed. The findings therefore suggest that DON may play a more crucial role in the biogeochemistry of peat‐dominated acid sensitive upland freshwater systems than previously thought. Reservoirs, impoundments and large lakes in peatland catchments may be important sites in mediating downstream N transport and speciation. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

17.
Waterborne carbon (C) export from terrestrial ecosystems is a potentially important flux for the net catchment C balance and links the biogeochemical C cycling of terrestrial ecosystems to their downstream aquatic ecosystems. We have monitored hydrology and stream chemistry over 3 years in ten nested catchments (0.6–15.1 km2) with variable peatland cover (0%–22%) and groundwater influence in subarctic Sweden. Total waterborne C export, including dissolved and particulate organic carbon (DOC and POC) and dissolved inorganic carbon (DIC), ranged between 2.8 and 7.3 g m–2 year–1, representing ~10%–30% of catchment net ecosystem exchange of CO2. Several characteristics of catchment waterborne C export were affected by interacting effects of peatland cover and groundwater influence, including magnitude and timing, partitioning into DOC, POC, and DIC and chemical composition of the exported DOC. Waterborne C export was greater during the wetter years, equivalent to an average change in export of ~2 g m–2 year–1 per 100 mm of precipitation. Wetter years led to a greater relative increase in DIC export than DOC export due to an inferred relative shift in dominance from shallow organic flow pathways to groundwater sources. Indices of DOC composition (SUVA254 and a250/a365) indicated that DOC aromaticity and average molecular weight increased with catchment peatland cover and decreased with increased groundwater influence. Our results provide examples on how waterborne C export and DOC composition might be affected by climate change. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

18.
Changes in stream chemistry were studied for 4 years following large wildfires that burned in Glacier National Park during the summer of 2003. Burned and unburned drainages were monitored from December 2003 through August 2007 for streamflow, major constituents, nutrients, and suspended sediment following the fires. Stream‐water nitrate concentrations showed the greatest response to fire, increasing up to tenfold above those in the unburned drainage just prior to the first post‐fire snowmelt season. Concentrations in winter base flow remained elevated during the entire study period, whereas concentrations during the growing season returned to background levels after two snowmelt seasons. Annual export of total nitrogen from the burned drainage ranged from 1·53 to 3·23 kg ha?1 yr?1 compared with 1·01 to 1·39 kg ha?1 yr?1 from the unburned drainage and exceeded atmospheric inputs for the first two post‐fire water years. Fire appeared to have minimal long‐term effects on other nutrients, dissolved organic carbon, and major constituents with the exception of sulfate and chloride, which showed increased concentrations for 2 years following the fire. There was little evidence that fire affected suspended‐sediment concentrations in the burned drainage. Sediment yields in subalpine streams may be less affected by fire than in lower elevation streams because of the slow release rate of water during spring snowmelt. Published in 2008 by John Wiley & Sons, Ltd.  相似文献   

19.
This 2‐year study (2000, 2001) reports annual nutrient (phosphorus, nitrate) export from a first‐order agricultural watershed in southern Ontario based on an intensive monitoring programme. The importance of storm and melt events in annual export estimates is demonstrated and the temporal variability in nutrient loading during events is related to processes occurring within the catchment. The feasibility of predicting event‐related nutrient export from hydrometric data is explored. The importance of sampling frequency throughout events is also shown. Export of total phosphorus (TP), soluble reactive phosphorus (SRP) and nitrate ( ) for 2000 and 2001 averaged 0·35 kg ha?1 year?1, 0·09 kg ha?1 year?1, and 35 kg ha?1 year?1 (as N) respectively. Approximately 75% of annual TP export, 80% of annual SRP export and 70% of annual export occurred during 28 events per year. A small number of large‐magnitude events (>34 mm) accounted for 18–42% of annual TP export, 0–61% of annual SRP export and 13–33% of annual NO export. Our results show that temporal variability in nutrient export is largely governed by discharge in this basin, and export can be predicted from discharge. SRP and TP export can also be predicted from discharge, but only for events that are not large in magnitude. The sampling interval throughout events is important in obtaining precise estimates of nutrient export, as infrequent sampling intervals may over‐ or under‐estimate nutrient export by ± 45% per event for P. This study improves our understanding of and P export patterns and our ability to predict or model them by relating temporal variability in event nutrient export to discharge and processes occurring within the basin, and also by exploring the significance of sampling interval in the context of the importance of individual events, season and temporal variability during events. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

20.
The impact of intensive farming on chemical weathering in the Critical Zone is still an open question. Extensively instrumented and monitored over the last 50 years, the Orgeval Critical Zone Observatory (CZO) in France is an observation site impacted by intensive farming since the 1960s. The Orgeval observatory represents an ideal place to study the response and resilience capability of the Critical Zone under agricultural stress. This paper investigates the chemical composition of different water bodies in two nested catchments of the Orgeval CZO, including rainfall, springs, rivers, and rocks, over one and half hydrological year. We show that elemental and strontium isotopic ratios are powerful to constrain the origin of the elements. The results show that the river chemistry at the outlet of the two nested catchments is dominated by rain inputs (particularly atmospheric dust dissolution) and the chemical weathering of limestone and gypsum. Fertilizer input is clearly visible, although the distinction between gypsum dissolution and fertilizer inputs needs more investigation. The mixtures of water masses inferred from our data are in good agreement with the hydrological context of the watershed, that is, a multilayered aquifer structure. At the main outlet of the CZO, we estimate that the input of ocean‐derived solutes through rainfall represents 7 t km?2 year?1, on the same order of magnitude as the net fertilizer input (10 t km?2 year?1), and that rock weathering releases 50 t km?2 year?1. Including previously published physical erosion rates, we estimate that the total denudation rate (physical and chemical) of the Orgeval CZO is 20 mm (1,000 year)?1, which, along with the entire Seine watershed, is among the lowest chemical denudation rates for carbonate terrains under temperate climate. Chemical denudation is about 10 times higher than physical erosion in the Orgeval CZO. The consumption of CO2 by rock weathering is estimated to be between 265.103 and 360.103 molC km2 year?1, similar for the two nested catchments. Compared with the rivers, the springs show a higher CO2 consumption rate that suggests, as pointed out earlier, a enhancement of carbonate dissolution linked to nitrification and thus fertilizer application. The hyporheic zone appears to be a hot spot in the carbon cycle at the Orgeval CZO. This study sheds light on the complex, anthropocenic, interplay between geology, climate, and human activities that characterize and that take place in intensive agriculture regions.  相似文献   

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