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1.
We examine the physics of growth of water bubbles in highly viscous melts. During the initial stages, diffusive mass transfer of water into the bubble keeps the internal pressure in the bubbles close to the initial pressure at nucleation. Growth is controlled by melt viscosity and supersaturation pressure and radial growth under constant pressure is approximately exponential. At later stages, internal pressure falls, radial growth decelerates and follows the square-root of time. At this stage it is controlled by diffusion. The time of transition between the two stages is controlled by the decompression, melt viscosity and the Peclet number of the system. The model closely fit experimental data of bubble growth in viscous melts with low water content. Close fit is also obtained for new experiments at high supersaturation, high Peclet numbers, and high, variable viscosity. Near surface, degassed, silicic melts are viscous enough, so that viscosity-controlled growth may last for very long times. Using the model, we demonstrate that bubbles which nucleate shortly before fragmentation cannot grow fast enough to be important during fragmentation. We suggest that tiny bubbles observed in melt pockets between large bubbles in pumice represent a second nucleation event shortly before or after fragmentation. The presence of such bubbles is an indicator of the conditions at fragmentation. The water content of lavas extruded at lava domes is a key factor in their evolution. Melts of low water content (<0.2 wt%) are too viscid and bubbles nucleated in them will not grow to an appreciable size. Bubbles may grow in melts with 0.4 wt% water. The internal pressure in such bubbles may be preserved for days and the energy stored in the bubbles may be important during the disintegration of dome rocks and the formation of pyroclastic flows.  相似文献   

2.
Equilibrium and disequilibrium degassing of a volatile phase from a magma of K-phonolitic composition was investigated to assess its behavior upon ascent. Decompression experiments were conducted in Ar-pressurized externally heated pressure vessels at superliquidus temperature (1050 °C), in the pressure range 10–200 MPa using pure water as fluid phase. All experiments were equilibrated at 200 MPa and then decompressed to lower pressures with rates varying from 0.0028 to 4.8 MPa/s. Isobaric saturation experiments were performed at the same temperature and at 900–950 °C to determine the equilibrium water solubility in the pressure range 30–250 MPa. The glasses obtained from decompression experiments were analyzed for their dissolved water content, vesicularity and bubble size distribution. All decompressed samples presented a first event of bubble nucleation at the capsule–melt interface. Homogeneous bubble nucleation in the melt only occurred in fast-decompressed experiments (4.8 and 1.7 MPa/s), for ΔP ≅ 100 MPa. For these decompression rates high water over-saturations were maintained until a rapid exsolution was triggered at ΔP > 150 MPa. For slower rates (0.0028, 0.024, 0.17 MPa/s) the degassing of the melt took place by diffusive growth of the bubbles nucleating at the capsule–melt interface. This process sensibly reduced water over-saturation in the melt, preventing homogeneous nucleation to occur. For decompression rates of 0.024 and 0.17 MPa/s low water over-saturations were attained in the melt, gradually declining toward equilibrium concentrations at low pressures. A near-equilibrium degassing path was observed for a decompression rate of 0.0028 MPa/s. Experimental data combined with natural pumice textures suggest that both homogeneous and heterogeneous bubble nucleations occurred in the phonolitic magma during the AD 79 Vesuvius plinian event. Homogeneous bubble nucleation probably occurred at a depth of ∼ 3 km, in response to a fast decompression of the magma during the ascent.  相似文献   

3.
This study focuses on constraining bubble nucleation and H2O exsolution processes in alkalic K-phonolite melts, using “white pumice” of the 79 AD eruption of Vesuvius as starting material. The first set of experiments consisted of H2O solubility runs at 1153 to 1250 K and pressures between 50 and 200 MPa, to constrain equilibrium water concentrations along the decompression pathways. The decompression experiments were equilibrated with H2O at 150 MPa and 1173 and 1223 K, and then decompressed at 3 to 17 MPa/s before rapid quenching. Experiments nucleated bubbles within the first 50 MPa pressure drop, producing maximum bubble number densities (NV), corrected to melt volume, of 3.8 × 1014 m− 3 at 1173 K and 4.3 × 1013 m− 3 at 1223 K. Most bubbles were not visibly attached to crystals, except for a subset attached to pyroxenes primarily in the 1173 K experiments. When compared with prior bubble nucleation studies, the reduced nucleation ΔP and relatively low NV observed indicate predominantly a heterogeneous nucleation mechanism. Melt–vapor–crystal wetting angles measured in 1173 K experiments from bubbles attached to pyroxene crystals are 36 to 69°, which are similar to those measured on titanomagnetite crystals in calc-alkaline dacite melts. The 1223 K experiments have porosities and water concentrations that largely track equilibrium, despite the rapid decompression rate. The 1173 K experiments deviate strongly from equilibrium trends in both porosity and water concentration, and slower H2O diffusion rates are likely the cause of the inhibited bubble growth. Bubble number densities from 79 AD Vesuvius natural EU2 pumice are relatively high (2 to 4 × 1015 m− 3; [Gurioli, L., Houghton, B.F., Cashman, K.V., Cioni, R., 2005. Complex changes in eruption dynamics during the 79 AD eruption of Vesuvius. Bull. Volcanol. 67: 144–159.]) when corrected to vesicularity. In comparison, corrected NV's from homogeneous and heterogeneous bubble nucleation experiments from this study and prior work are at least factor of 5 lower, indicating perhaps that the natural magmas initially nucleated bubbles in the presence of CO2. The disequilibrium H2O exsolution seen in the 1173 K experiments indicates that inhibited bubble growth could lead to delayed exsolution in the conduit in cooler K-phonolite magmas.  相似文献   

4.
 Experiments on degassing of water-saturated granite melts with a pressure drop from 100 and 450 MPa to 40 and 120 MPa, respectively, at temperatures close to feldspar liquidus (750–700  °C), were carried out to determine the modality of water exsolution and vesicle formation at the liquidus temperature. Pressure-drop rates as small as approximately 100 bar/day were used. Uniform space distributions of bubbles of exsolved water were obtained with starting glass containing a small fraction (≈0.5 vol.%) of trapped air bubbles. Volume crystallization of feldspar was observed in degassed melts supplied with seeds. Bubble size distributions (BSD) measured in granite glasses after degassing are presented. Data on vesicle characteristics (number, radius, area, elongation) were acquired on images digitized with standard software, while the reconstruction of size distributions was performed with the Schwartz-Saltikov "unfolding" procedure. Bubble size distributions of size classes in the range 5–1000 μm were acquired with proper magnification and satisfactory statistical reliability of determined number densities. The BSDs of the experimental samples are compared with the results of measurements of rapidly degassed products of Mt. Etna and Vulcano Island. Many particular features of the bubble nucleation and growth can be distinguished in an individual BSD. However, the general BSD of the whole data set, including natural ones, can be relatively well described with linear regression in bilogarithmic coordinates. The slope of this regression is approximately 2.8±0.1. This dependence is in striking contrast with distributions theoretically predicted with classical nucleation models based on homogeneous nucleation of vesicles. The theoretical distribution requires the occurrence of strong maxima that are not observed in our experimental and natural samples, thus arguing for heterogeneous nucleation mechanisms. Received: 1 October 1998 / Accepted: 25 June 1999  相似文献   

5.
Bubble growth in rhyolitic melts: experimental and numerical investigation   总被引：2，自引：0，他引：2  
 Bubble growth controlled by mass transfer of water from hydrated rhyolitic melts at high pressures and temperatures was studied experimentally and simulated numerically. Rhyolitic melts were hydrated at 150 MPa, 780–850  °C to uniform water content of 5.5–5.3 wt%. The pressure was then dropped and held constant at 15–145 MPa. Upon the drop bubbles nucleated and were allowed to grow for various periods of time before final, rapid quenching of the samples. The size and number density of bubbles in the quenched glasses were recorded. Where number densities were low and run duration short, bubble sizes were in accord with the growth model of Scriven (1959) for solitary bubbles. However, most results did not fit this simple model because of interaction between neighboring bubbles. Hence, the growth model of Proussevitch et al. (1993), which accounts for finite separation between bubbles, was further developed and used to simulate bubble growth. The good agreement between experimental data, numerical simulation, and analytical solutions enables accurate and reliable examination of bubble growth from a limited volume of supersaturated melt. At modest supersaturations bubble growth in hydrated silicic melts (3–6 wt% water, viscosity 104–106 Pa·s) is diffusion controlled. Water diffusion is fast enough to maintain steady-state concentration gradient in the melt. Viscous resistance is important only at the very early stage of growth (t<1 s). Under the above conditions growth is nearly parabolic, R2=2Dtρm(C0–Cf)/ρg until the bubble approaches its final size. In melts with low water content, viscosity is higher and maintains pressure gradients in the melt. Growth may be delayed for longer times, comparable to time scales of melt ascent during eruptions. At high levels of supersaturation, advection of hydrated melt towards the growing bubble becomes significant. Our results indicate that equilibrium degassing is a good approximation for modeling vesiculation in melts with high water concentrations (C0>3 wt%) in the region above the nucleation level. When the melt accelerates and water content decreases, equilibrium can no longer be maintained between bubbles and melt. Supersaturation develops in melt pockets away from bubbles and new bubbles may nucleate. Further acceleration and increase in viscosity cause buildup of internal pressure in the bubbles and may eventually lead to fragmentation of the melt. Received: 19 June 1995 / Accepted: 27 December 1995  相似文献   

6.
We present a visco-elastic bubble growth model, accounting for viscous and elastic deformations and for volatile mass transfer between bubbles and melt. We define the borders between previous bubble growth models accounting for incompressible viscous melt, and our new model accounting also for elastic deformation; this is done by a set of end-member analytical solutions and numerical simulations. Elastic deformation is most prominent for magma of small vesicularity, where the growth regime depends on the shear modulus. For high shear modulus, bubble growth is slow and follows an exponential law in a viscous growth regime, while for low shear modulus bubbles quickly follow a square-root diffusive solution. Our model provides all the elastic components (stresses, strains and strain rates) required for defining criteria for failure and magma fragmentation. We suggest two failure criteria, a stress related one based on the internal friction and the Mohr-Coulomb failure theory, and a strain related one based on fibre elongation experiments. We argue that both criteria are equivalent if we consider their shear modulus dependency and its effect on magma rheology. Last, we apply our model to the process of bubble nucleation. In the incompressible case, following nucleation, growth is slow and leads to long incubation times during which bubbles may be dissolved back into the melt. The elastic response in magmas with low shear modulus results in a short incubation time, increasing the probability of survival. The above effects emphasize the significance of visco-elasticity for the dynamic processes occurring in magmas during volcanic activity.  相似文献   

7.
Syn-eruptive degassing of volcanoes may lead to syn-eruptive crystallization of groundmass phases. We have investigated this process using textural and compositional analysis of dome material from Merapi volcano, Central Java, Indonesia. Samples included dome lavas from the 1986–88, 1992–93, 1994 and 1995 effusive periods as well as pyroclastic material deposited by the November 1994 dome collapse. With total crystallinities commonly in excess of 70% (phenocrysts+microlites), the liquids present in Merapi andesites are highly evolved (rhyolitic) at the time of eruption. Feldspar microlites in dome rocks consist of plagioclase cores (Ab63An29Or8) surrounded by alkali feldspar rims (Ab53An5Or42), compositional pairs which are not in equilibrium. A change in the phase relations of the ternary feldspar system caused by degassing best explains the observed transition in feldspar composition. A small proportion of highly vesicular airfall tephra grains from the 1994 collapse have less evolved glass compositions than typical dome material and contain rimless plagioclase microlites, suggesting that the 1994 collapse event incorporated less-degassed, partially liquid magma in addition to fully solidified dome rock.As decompression drives volatile exsolution, rates of degassing and resultant microlite crystallization may be governed by magma ascent rate. Microlite crystallinity is nearly identical among the 1995 dome samples, an indication that similar microlite growth conditions (PH2O and temperature) were achieved throughout this extrusive period. However, microlite number density varied by more than a factor of four in these samples, and generally increased with distance from the vent. Low vent-ward microlite number densities and greater microlite concentrations down-flow probably reflect progressively decreasing rates of undercooling at the time of crystal nucleation during extrusion of the 1995 dome. Comparison between dome extrusion episodes indicates a correlation between lava effusion rate and microlite number density, suggesting that extrusion slowed during 1995. Crystal textures and compositions in the 1992–93 and 1994 domes share the range exhibited by the 1995 dome, suggesting that transitions in crystallization conditions (i.e., rates of undercooling determined by effusion rate) are cyclic.  相似文献   

8.
Bubble and crystal textures provide information with regard to the kinetics of the vesiculation and crystallization processes. They also provide insights into the fluid mechanical behavior of magma in a conduit. We performed textural (bubble and crystal) and compositional analyses of pyroclasts that were obtained from the Tenjo pyroclastic flow, which resulted on account of the eruption in 838 A.D. on Kozu Island, about 200 km south of Tokyo, Japan. Pyroclasts in one flow unit (300∼2,060 kg/m3; average density 1330 kg/m3) can be classified into three types on the basis of vesicle textures. Type I pyroclasts have small isolated spherical bubbles with higher vesicularities (67–77 vol.%) and number density (10.8–11.7 log m−3). Type II pyroclasts have vesicularities similar to type I (61–69 vol.%), but most bubbles exhibit evidences of bubble coalescence, and lower number densities than type I (8.9–9.5 log m−3). Type III pyroclasts contain highly deformed bubbles with lower vesicularities (16–34 vol.%) and number densities (8.2–9.0 log m−3). The microlite volume fraction (DRE converted) also changes consistently across type I, type II, and type III as 0.06, 0.08, and 0.10–0.15, respectively. However, the number density of the microlites remains nearly invariant in all the pyroclast types. These facts indicate that the variation in the microlite volume fraction is controlled not by the number density (i.e., nucleation process), but by the size (i.e., growth process); the growth history of each type of microlite was different. Water content determinations show that the three types of pumices have similar H2O contents (2.6±0.2 wt%). This fact implies that all three types were quenched at nearly the same depth (35±5 MPa, assuming that the magma was water-saturated) in the conduit. If the crystal sizes are limited only by growth time, a variation in this parameter can be related to the residence time, which is attributed to the flow heterogeneity in the conduit. By assuming a laminar Poiseuille-type flow, these textural observations can be explained by the difference in ascent velocity and shearing motion across the conduit, which in turn results in the differences in growth times of crystals, degrees of deformation, and bubble coalescence. Consequently, for crystals in the inner part of the conduit, the crystal growth time from nucleation to quenching is shorter than that near the conduit wall. The vesicle texture variation of bubbles in types I, II, and III results from the difference in the deformation history, implying that the effect of degassing occurred primarily towards the conduit wall.  相似文献   

9.
Analytical models for decompressional bubble growth in a viscous magma are developed to establish the influence of high magma viscosity on vesiculation and to assess the time-scales on which bubbles respond to decompression. Instantaneous decompression of individual bubbles, analogous to a sudden release of pressure (e.g. sector collapse), is considered for two end-member cases. The infinite melt model considers the growth of an isolated bubble before significant bubble interaction occurs. The shell model considers the growth of a bubble surrounded by a thin shell and is analogous to bubble growth in a highly vesicular magmatic foam. Results from the shell model show that magmas less viscous than 109 Pa s can freely expand without developing strong overpressures. The timescales for pressure re-equilibration are shortened by increased ratios of bubble radius to shell thickness and by larger decompression. Time-scales for isolated bubbles in rhyolitic melts (infinite melt model) are significantly longer, implying that such bubbles could experience internal pressures greater than the ambient pressure for at least a few hours following a sudden release of pressure. The shell model is developed to assess bubble growth during the linear decompression of a magma body of constant viscosity. For the range of decompression rates and viscosities associated with actual volcanic eruptions, bubble growth continues at approximately the equilibrium rate, with no attendant excess of internal pressure. The results imply that viscosity does not have any significant role in preventing the explosive expansion of high viscosity foams. However, for viscosities of >109 Pa s there is the potential for a viscosity quench under the extreme decompression rates of an explosive eruption. It is proposed that the typical vesicularities of pumice of 0.7–0.8 are a consequence of the viscosity of the degassing magmas becoming sufficiently high to inhibit bubble expansion over the characteristic time-scale of eruption. For fully degassed silicic lavas with viscosities in the range 1010 to 1012 Pa s time-scales for decompression of isolated bubbles can be hours to many months.  相似文献   

10.
We investigate the interaction of thermal convection and crystallization in large aspect-ratio magma chambers. Because nucleation requires a finite amount of undercooling, crystallization is not instantaneous. For typical values of the rates of nucleation and crystal growth, the characteristic time-scale of crystallization is about 103–104 s. Roof convection is characterized by the quasi-periodic formation and instability of a cold boundary layer. Its characteristic time-scale depends on viscosity and ranges from about 102 s for basaltic magmas to about 107 s for granitic magmas. Hence, depending on magma viscosity, convective instability occurs at different stages of crystallization. A single non-dimensional number is defined to characterize the different modes of interaction between convection and crystallization.Using realistic functions for the rates of nucleation and crystal growth, we integrate numerically the heat equation until the onset of convective instability. We determine both temperature and crystal content in the thermal boundary layer. Crystallization leads to a dramatic increase of viscosity which acts to stabilize part of the boundary layer against instability. We compute the effective temperature contrast driving thermal convection and show that it varies as a function of magma viscosity and hence composition.In magmas with viscosities higher than 105 poise, the temperature contrast driving convection is very small, hence thermal convection is weak. In low-viscosity magmas, convective breakdown occurs before the completion of crystallization, and involves partially crystallized magma. The convective regime is thus characterized by descending crystal-bearing plumes, and bottom crystallization proceeds both by in-situ nucleation and deposition from the plumes. We suggest that this is the origin of intermittent layering, a form of rhythmic layering described in the Skaergaard and other complexes. We show that this regime occurs in basic magmas only at temperatures close to the liquidus and never occurs in viscous magmas. This may explain why intermittent layering is observed only in a few specific cases.  相似文献   

11.
In this study, carbon dioxide exsolution from carbonated water is directly observed under reservoir conditions (9 MPa and 45 °C). Fluorescence microscopy and image analysis are used to quantitatively characterize bubble formation, morphology, and mobility. Observations indicate the strong influence of interfacial tension and pore-geometry on bubble growth and evolution. Most of the gas exhibits little mobility during the course of depressurization and clogs water flow paths. However, a snap-off mechanism mobilizes a small portion of the trapped gas along the water flow paths. This feature contributes to the transport of the dispersed exsolved gas phase and the formation of intermittent gas flow. A new definition of critical gas saturation is proposed accordingly as the minimum saturation that snap-off starts to produce mobile bubbles. Low mobility of the water phase and CO2 phase in exsolution is explained by formation of dispersed CO2 bubbles which block water flow and lack the connectivity to create a mobile gas phase.  相似文献   

12.
This study assesses the effect of decompression rate on two processes that directly influence the behavior of volcanic eruptions: degassing and permeability in magmas. We studied the degassing of magma with experiments on hydrated natural rhyolitic glass at high pressure and temperature. From the data collected, we defined and characterized one degassing regime in equilibrium and two regimes in disequilibrium. Equilibrium bubble growth occurs when the decompression rate is slower than 0.1 MPa s–1, while higher rates cause porosity to deviate rapidly from equilibrium, defining the first disequilibrium regime of degassing. If the deviation is large enough, a critical threshold of super-saturation is reached and bubble growth accelerates, defining the second disequilibrium regime. We studied permeability and bubble coalescence in magma with experiments using the same rhyolitic melt in open degassing conditions. Under these open conditions, we observed that bubbles start to coalesce at ~43 vol% porosity, regardless of decompression rate. Coalescence profoundly affects bubble texture and size distributions, and induces the melt to become permeable. We determined coalescence to occur on a time scale (~180 s) independent of decompression rate. We parameterized and incorporated our experimental results into a 1D conduit flow model to explore the implications of our findings on eruptive behavior of rhyolitic melts with low crystal contents stored in the upper crust. Compared to previous models that assume equilibrium degassing of the melt during ascent, the introduction of disequilibrium degassing reduces the deviation from lithostatic pressure by ~25%, the acceleration at high porosities (>50 vol%) by a factor 5, and the associated decompression rate by an order of magnitude. The integration of the time scale of coalescence to the model shows that the transition between explosive and effusive eruptive regimes is sensitive to small variations of the initial magma ascent speed, and that flow conditions near fragmentation may significantly be affected by bubble coalescence and gas escape.Editorial responsibility: D. Dingwell  相似文献   

13.
The vesiculation of magma during the 1983 eruption of Miyakejima Volcano, Japan, is discussed based on systematic investigations of water content, vesicularity, and bubble size distribution for the products. The eruption is characterized by simultaneous lava effusion and explosive sub-plinian (‘dry’) eruptions with phreatomagmatic (‘wet’) explosions. The magmas are homogeneous in composition (basaltic andesite) and in initial water content (H2O = 3.9±0.9 wt%), and residual groundmass water contents for all eruption styles are low (H2O <0.4 wt%) suggestive of extensive dehydration of magma. For the scoria erupted during simultaneous ‘dry’ and ‘wet’ explosive eruptions, inverse correlation was observed between vesicularity and residual water content. This relation can be explained by equilibrium exsolution and expansion of ca. 0.3 wt% H2O at shallow level with different times of quenching, and suggests that each scoria with different vesicularity, which was quenched at a different time, provides a snapshot of the vesiculation process near the point of fragmentation. The bubble size distribution (BSD) varies systematically with vesicularity, and total bubble number density reaches a maximum value at vesicularity Φ ∼ 0.5. At Φ  ∼ 0.5, a large number of bubbles are connected with each other, and the average thickness of bubble walls reaches the minimum value below which they would rupture. These facts suggest that vesiculation advanced by nucleation and growth of bubbles when Φ < 0.5, and then by expansion of large bubbles with coalescence of small ones for Φ > 0.5, when bubble connection becomes effective. Low vesicularity and low residual water content of lava and spatter (Φ  < 0.1, H2O  < 0.1 wt%), and systematic decrease in bubble number density from scoria through spatter to lava with decrease in vesicularity suggest that effusive eruption is a consequence of complete degassing by bubble coalescence and separation from magma at shallow levels when magma ascent rate is slow.
T. ShimanoEmail:
  相似文献   

14.
This paper outlines methods for determining a bubble size distribution (BSD) and the moments of the BSD function in vesiculated clasts produced by volcanic eruptions. It reports the results of applications of the methods to 11 natural samples and discusses the implications for quantitative estimates of eruption processes. The analysis is based on a quantitative morphological (stereological) method for 2-dimensional imaging of cross-sections of samples. One method determines, with some assumptions, the complete shape of the BSD function from the chord lengths cut by bubbles. The other determines the 1st, 2nd and 3rd moments of distribution functions by measurement of the number of bubbles per unit area, the surface area per unit volume, and the volume fraction of bubbles. Comparison of procedures and results of these two distinct methods shows that the latter yields rather more reliable results than the former, though the results coincide in absolute and relative magnitudes. Results of the analysis for vesiculated rocks from eleven subPlinian to Plinian eruptions show some interesting systematic correlations both between moments of the BSD and between a moment and the eruption column height or the SiO2 content of magma. These correlations are successfully interpreted in terms of the nucleation and growth processes of bubbles in ascending magmas. This suggests that bubble coalescence does not predominate in sub-Plinian to Plinian explosive eruptions. The moment-moment correlations put constraints on the style of the nucleation and growth process of bubbles. The scaling argument suggests that a single nucleation event and subsequent growth with any kind of bubble interaction under continuous depressurization, which leads to an intermediate growth law between the diffusional growth ( ) at a constant depressurization rate and the Ostwald ripening ( ) under a constant pressure, where Rm and t are the mean radius of bubble and the effective time of diffusion respectively, occurred in the eruptions. It is emphasized that the BSD in vesiculated rocks from terrestrial volcanoes can be used to estimate quantitatively eruption processes such as the initial saturation pressure and magma ascent velocity in a volcanic conduit.  相似文献   

15.
The 79 AD eruption of Vesuvius included 8 eruption units (EU1–8) and several complex transitions in eruptive style. This study focuses on two important transitions: (1) the abrupt change from white to gray pumice during the Plinian phase of the eruption (EU2 to EU3) and (2) the shift from sustained Plinian activity to the onset of caldera collapse (EU3 to EU4). Quantification of the textural features within individual pumice clasts reveals important changes in both the vesicles and groundmass crystals across each transition boundary. Clasts from the white Plinian fall deposit (EU2) present a simple story of decompression-driven crystallization followed by continuous bubble nucleation, growth and coalescence in the eruptive conduit. In contrast, pumices from the overlying gray Plinian fall deposit (EU3) are heterogeneous and show a wide range in both bubble and crystal textures. Extensive bubble growth, coalescence, and the onset of bubble collapse in pumices at the base of EU3 suggest that the early EU3 magma experienced protracted vesiculation that began during eruption of the EU2 phase and was modified by the physical effects of syn-eruptive mingling-mixing. Pumice clasts from higher in EU3 show higher bubble and crystal number densities and less evidence of bubble collapse, textural features that are interpreted to reflect more thorough mixing of two magmas by this stage of the eruption, with consequent increases in both vesiculation and crystallization. Pumice clasts from a short-lived, high column at the onset of caldera collapse (EU4) continue the trend of increasing crystallization (enhanced by mixing) but, unexpectedly, the melt in these clasts is more vesicular than in EU3 and, in the extreme, can be classified as reticulite. We suggest that the high melt vesicularity of EU4 reflects strong decompression following the partial collapse of the magma chamber.Editorial responsibility: D.B. Dingwell  相似文献   

16.
This article describes the simulation of three-dimensional buoyancy-driven bubble rise using a phase-field-based incompressible Lattice Boltzmann model. The effect of the Cahn–Hilliard mobility parameter, which is the rate of diffusion relaxation from non-equilibrium toward equilibrium state of chemical potential, is evaluated in detail. In contrast with previous work that pursues a high density ratio of binary fluids in the hydrodynamic equation, we apply a large dynamic viscosity ratio, together with a matched density pair and a separate compensating gas phase buoyant force, and the numerical results fit previous experimental results well. Through analysis, it is noted that for cases with moderate Reynolds number, a large value of mobility keeps a relatively sharp interface, while smaller values of mobility would result in diffusive interfacial regions. Moreover, for cases with large Reynolds number, small bubbles at the tail tend to separate more easily when the value of mobility is larger. This article offers some potentially useful details for performing phase-field-based simulations.  相似文献   

17.
Plinian/ignimbrite activity stopped briefly and abruptly 16 and 45 h after commencement of the 1912 Novarupta eruption defining three episodes of explosive volcanism before finally giving way after 60 h to effusion of lava domes. We focus here on the processes leading to the termination of the second and third of these three episodes. Early erupted pumice from both episodes show a very similar range in bulk vesicularity, but the modal values markedly decrease and the vesicularity range widens toward the end of Episode III. Clasts erupted at the end of each episode represent textural extremes; at the end of Episode II, clasts have very thin glass walls and a predominance of large bubbles, whereas at the end of Episode III, clasts have thick interstices and more small bubbles. Quantitatively, all clasts have very similar vesicle size distributions which show a division in the bubble population at 30 μm vesicle diameter and cumulative number densities ranging from 107–109 cm–3. Patterns seen in histograms of volume fraction and the trends in the vesicle size data can be explained by coalescence signatures superimposed on an interval of prolonged nucleation and free growth of bubbles. Compared to experimental data for bubble growth in silicic melts, the high 1912 number densities suggest homogeneous nucleation was a significant if not dominant mechanism of bubble nucleation in the dacitic magma. The most distinct clast populations occurred toward the end of Plinian activity preceding effusive dome growth. Distributions skewed toward small sizes, thick walls, and teardrop vesicle shapes are indicative of bubble wall collapse marking maturation of the melt and onset of processes of outgassing. The data suggest that the superficially similar pauses in the 1912 eruption which marked the ends of episodes II and III had very different causes. Through Episode III, the trend in vesicle size data reflects a progressive shift in the degassing process from rapid magma ascent and coupled gas exsolution to slower ascent with partial open-system outgassing as a precursor to effusive dome growth. No such trend is visible in the Episode II clast assemblages; we suggest that external changes involving failure of the conduit/vent walls are more likely to have effected the break in explosive activity at 45 h.  相似文献   

18.
 Dacite tephras produced by the 1991 pre-climactic eruptive sequence at Mt. Pinatubo display extreme heterogeneity in vesicularity, ranging in clast density from 700 to 2580 kg m–3. Observations of the 13 surge-producing blasts that preceded the climactic plinian event include radar-defined estimates of column heights and seismically defined eruptive and intra-eruptive durations. A comparison of the characteristics of erupted material, including microlite textures, chemical compositions, and H2O contents, with eruptive parameters suggests that devolatilization-induced crystallization of the magma occurred to a varying extent prior to at least nine of the explosive events. Although volatile loss progressed to the same approximate level in all of the clasts analyzed (weight percent H2O=1.26-1.73), microlite crystallization was extremely variable (0–22%). We infer that syn-eruptive volatile exsolution from magma in the conduit and intra-eruptive separation of the gas phase was facilitated by the development of permeability within magma residing in the conduit. Correlation of maximum microlite crystallinity with repose interval duration (28–262 min) suggests that crystallization occurred primarily intra-eruptively, in response to the reduction in dissolved H2O content that occurred during the preceding event. Detailed textural characterization, including determination of three-dimensional shapes and crystal size distributions (CSD), was conducted on a subset of clasts in order to determine rates of crystal nucleation and growth using repose interval as the time available for crystallization. Shape and size analysis suggests that crystallization proceeded in response to lessening degrees of feldspar supersaturation as repose interval durations increased. We thus propose that during repose intervals, a plug of highly viscous magma formed due to the collapse of vesicular magma that had exsolved volatiles during the previous explosive event. If plug thickness grew proportionally to the square root of time, and if magma pressurization increased during the eruptive sequence, the frequency of eruptive pulses may have been modulated by degassing of magma within the conduit. Dense clasts in surge deposits probably represent plug material entrained by each subsequent explosive event. Received: 4 December 1997 / Accepted: 13 September 1998  相似文献   

19.
The evolution of bubble size distributions in volcanic eruptions   总被引：1，自引：0，他引：1  
We review observations of bubble size distributions (BSDs) generated during explosive volcanic eruptions and laboratory explosions, as inferred from vesicle size distributions found in the end products. Unimodal, polymodal, exponential and power law BSDs are common, even in the absence of coalescence, and both power law and exponential distributions have been generated in the same eruption. To date theoretical models have proposed incompatible mechanisms for producing the various distributions. We here present a unifying mechanism. Data from our laboratory analogue experiments suggest that power law distributions are associated with highly non-equilibrium degassing. A numerical model is developed in which bubbles nucleate repeatedly and grow in the spaces between those of previous generations, where, in a non-equilibrium degassing scenario, the volatile concentration remains high. This process causes the BSD to evolve from unimodal, through exponential, into a power law. The exponent of the power law is a measure of the number of nucleation events, or the duration of the nucleation period compared with the timescale of bubble growth. The mathematical inevitability of the evolution from unimodal (Poissonian) to power law is discussed. The findings may resolve the apparent contradiction between the equilibrium degassing conduit flow models and the non-equilibrium degassing conditions derived from bubble growth models of explosive volcanic eruptions. The process of ongoing nucleation is the mechanism whereby the volcanic system maintains near-equilibrium in the case of rapid depressurisation and slow volatile diffusion.  相似文献   

20.
The Fontana Lapilli deposit is one of very few examples of basaltic Plinian eruptions discovered so far. Juvenile clasts have uniform chemical composition and moderate ranges of density and bulk vesicularity. However, clast populations include two textural varieties which are microlite-poor and microlite-rich respectively. These two clast types have the same clast density range, making a distinction impossible on that base alone. The high bubble number density (～ 107 cm? 3) and small bubble population of the Fontana clasts suggest that the magma underwent coupled degassing following rapid decompression and fast ascent rate, leading to non-equilibrium degassing with continuous nucleation as it is common for silicic analogues. The Fontana products have lower microlite contents (10–60 vol.%) with respect to the other documented basaltic Plinian eruptions suggesting that the brittle fragmentation, implied for the other basaltic Plinian deposits, does not apply to the Fontana products and another fragmentation mechanism led the basaltic magma to erupt in a Plinian fashion.  相似文献   

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