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1.
137Cs湖泊沉积年代学方法应用的局限——以Crawford湖为例   总被引：17，自引：5，他引：12  
项亮 《湖泊科学》1995,7(4):307-313
＾１３７Ｃｓ湖泊沉积年代学方法是测定现代湖泊沉积物沉积年代和沉积速率的重要同位素年代学方法之一。对加拿大Ｃｒａｗｆｏｒｄ湖采集的沉积孔柱内＾１３７Ｃｓ垂直分布的研究发现,该方法给出时的标有明显偏差。比较＾２１０Ｐｂ和纹层等年代方法的结果,其１９６３年时标蓄积峰值所在位置明显移向表层,而作为１９５４年时标的该核素出现蓄积的层位则远早于该年沉积物蓄积层位。研究还表明,孔柱中较高的间隙水含量、缺少足以吸  相似文献   

2.
210Pb- and137Cs-measurements, and varve counting have been used to date sediment cores from Lake Zurich (Switzerland). Two cores from different water depths were dated with210Pb/210Po and revealed sediment accumulation rates of (0.055±0.015) g·cm?2·y?1 and (0.09±0.03) g·cm?2·y?1, respectively. A comparable rate of (0.07±0.01) g·cm?2·y?1 has been obtained from137Cs measurements. These rates were confirmed by annual layer (varve)-counts which lead to rates of 0.07 g·cm?2·y?1. Constant210Pb activities were observed in the top 6 cm of the sediment cores. This constancy is generally explained in the literature by mixing processes caused by bioturbation and by distortion during coring operations of the uppermost water-rich fluffy sediments. However the distinct137Cs-maxima and the regular and undisturbed varve lamination of the top sediment observed in the cores of Lake Zurich contradict this assumption. In addition, measurements of7Be at the water/sediment interaces proved complete sediment core recovery and mechanically undisturbed sediments. Remobilization processes are assumed to cause the observed constant210Pb activities. Remobilization may also be the reason for an incomplete210Pb inventory in the sediments which contain only about 50% of the fallout from atmosphere. The results of the210Pb dating should therefore be considered with some care. If existent, varve counting represents the easiest and most reliable means for dating lake sediments.  相似文献   

3.
Illite clay particles with adsorbed137Cs were added as a submillimeter layer to the surface of silt-clay sediments contained in rectangular Plexiglas cells stored in a temperature-regulated aquarium, in order to trace the effect of the oligochaete, Tubifex tubifex, and the amphipod, Pontoporeia hoyi, on mass redistribution near the sediment-water interface. A well-collimated NaI gamma detector scanned each sediment column (～10 cm deep) at daily or weekly intervals for six months, depicting the time evolution of radioactivity with and without added benthos. In a cell with tubificids (～5 × 104 m?2), which feed below 3 cm and defecate on surface sediments, the labeled layer was buried at a rate of 0.052 ± 0.007 cm/day (20°C). When labeled particles entered the feeding zone,137Cs reappeared in surface sediments creating a bimodal activity profile. In time, the activity tended toward a uniform distribution over the upper 6 cm, decreasing exponentially below to undetectable levels by 9 cm. In a cell with amphipods (～1.6 × 104 m?2) uniform activity developed rapidly (～17 days) down to a well-defined depth (1.5 cm). The mixing of sediments by Pontoporeia is described by a simple quantitative model of eddy diffusive mixing of sediment solids. The value of the diffusion coefficient, 4.4 cm2/yr (7°C) was computed from a least squares fit of theoretical to observed profile broadening over time. In a cell without benthos, small but measurable migration of137Cs indicated an effective molecular diffusion coefficient of 0.02 cm2/yr.  相似文献   

4.
Lake sediments, in which abundant, continuous and high resolved signals are preserved, have the potential to recover the history of terrestrial environmental variation. The value of such paleo-environment signals depends firstly on tying them to accurate …  相似文献   

5.
210Pb is widely used for dating recent sediments in the aquatic environment; however, our experiences working in shallow coastal environments in the Pacific coast of Mexico have demonstrated that the potential of 210Pb for reliable historical reconstructions might be limited by the low 210Pb atmospheric fallout, sediment mixing, abundance of coarse sediments and the lack of 137Cs signal for 210Pb corroboration. This work discusses the difficulties in obtaining adequate sedimentary records for geochronological reconstruction in such active and complex settings, including examples of 210Pb geochronologies based on sediment profiles collected in two contrasting areas coastal areas (mudflats associated to coastal lagoons of Sinaloa State and the continental shelf of the Gulf of Tehuantepec), in which geochemical data was used to support the temporal frame established and the changes in sediment supply recorded in the sediment cores which were related to the development of land-based activities during the last century.  相似文献   

6.
Use of fallout radionuclides as indicators of erosion processes   总被引：1，自引：0，他引：1  
The different depth penetration characteristics of 137Cs, 7Be and 210Pb excess in undisturbed soils can be used to identify erosion processes by analysis of sediments derived from surface erosion. Caesium-137 concentrations (half-life 30 years) typically decrease to half the surface value at between 30 and 50 mm. Beryllium-7 (half-life 53 days) has half-penetration depths of between 0.7 and 10 mm, whereas 210Pb excess (half-life 20.2 years) has half-penetration depths between 10 and 30 mm. Experiments designed to determine the applicability of these depth penetration characteristics to soil erosion studies are reported. Surface runoff was artificially generated at two locations in a grazed paddock using a rainfall simulator. Suspended sediment was extracted from runoff and analysed for natural and artificial gamma emitting radio-nuclides. Suspended sediment derived from sheet flow contained initially high values of 137Cs, 7Be and 210Pb excess. As the experiment continued 137Cs concentrations remained high, but 7Be and 210Pb excess value decreased with time. This is interpreted as indicating a change from sheet dominated erosion to rill dominated erosion. During a second experiment artificial rain was allowed to fall onto an eroded gully wall. The derived suspended sediment contained no detectable 137Cs, 7Be or 210Pb excess. Overland flow from above the gully wall was then allowed to run down the gully face and mix with the water falling directly onto the gully wall. There was no detectable change in the radionuclide signature, showing that the gully wall was the predominant source of sediment. This was tested independently by mass balance and 226Ra to 232Th ratios. The good correlation between 210Pb excess and 7Be at this site suggests that the differential technique described here may be applicable over time-scales longer than are possible with 7Be. It may therefore be practical to examine catchment erosion history through analysis of 210Pb excess and 137Cs in sediment cores.  相似文献   

7.
On two short sediment cores from Lake Łazduny (northeastern Poland) different methods for age estimation were applied including varve counting, 210Pb, 137Cs and OSL dating. The investigated sediment consists of finely laminated, organic-rich calcareous gyttja interrupted by a sand layer. For 210Pb we tested the CFCS, CIC, CRS and SIT models and compared the results with the established varve chronology and the 137Cs distribution. The total 210Pb activity distribution is consistent between cores and shows a regular decrease with depth. However, the total inventory of unsupported 210Pb was significantly different and indicates varying rates of sediment focusing. Our results show that all 210Pb dating models used in this study produced different results, while the SIT model performed best in comparison with varve counts and 137Cs peaks. The CFCS model produced a realistic age-depth trend but obtained ages were too old compared to the varve time scale. The age estimates provided by the CRS model were too old as well with an increasing offset downcore and the CIC model failed completely by producing an unrealistic chronology with age inversions. This confirms that only systematic testing of different 210Pb dating models and routine validation using independent time markers produces reliable 210Pb chronologies. OSL dating of two samples from the sand layer provided much too old results which indicate incomplete bleaching during deposition of the analyzed quartz grains. This multiple dating approach demonstrates the considerable potential but also potential pitfalls of dating such young sediments.  相似文献   

8.
An experiment was designed to assess the relative importance of sediment accumulation and bioturbation in determining the vertical distribution of nuclides in estuarine sediments. A diver-collected core, 120 cm long, was raised from central Long Island Sound and analyzed down its length for:210Pb and226Ra;239, 240Pu; and Mn, Zn, Cu, and Pb. Sampling for chemical analysis was guided by X-radiography of the core. Excess210Pb (relative to226Ra) is roughly homogeneous in the top 2–4 cm of the core, then decreases quasi-exponentially to zero at (or above) 15 cm.239, 240Pu and excess Zn, Cu, and Pb, relative to background values at greater depths in the core, are distributed like excess210Pb in the top 10–15 cm. The absence of Mn enrichment at the top of the core, in contrast to other cores raised from this station, suggests that 1–3 cm of sediment was lost by erosion at the site of this core sometime prior to sampling. Below 15 cm excess210Pb and excess Zn, Cu, and Pb are found only in the bulk sample from 25 to 30 cm and in clearly identifiable burrow fillings dissected from 70 cm and 115 cm depth. Infilling of large burrows, excavated and then abandoned by crustaceans, is therefore a mechanism for transfer of surficial material to depth in these sediments.The bioturbation rate in the top several centimeters at this station has been determined previously using234Th (24-day half-life). The distribution of239, 240Pu can be used to estimate a bioturbation rate for the underlying layer (to ～10 cm depth); this rate is found to be 1–3% of the maximum mixing rate for the top 2–3 cm. Using these two mixing rates in a composite-layer, mixing + sedimentation model, the distribution of excess210Pb in the top 15 cm was used to constrain the sediment accumulation rate, ω. While the apparent rate of sediment accumulation (assuming no mixing below 2–4 cm) is 0.11 cm/yr, the model requires ω < 0.05 cm/yr. Thus in an area of slow sediment accumulation, a low rate of bioturbation below the surficial zone of rapid mixing causes an increase of at least a factor of two in apparent accumulation rate.  相似文献   

9.
A large number of sediment cores collected during 2005-2010 from the Taiwan Strait were analyzed for radionuclides (210Pb, 137Cs and 7Be) to elucidate sedimentation dynamics in this all-important gateway linking two largest marginal seas in the western Pacific (namely, the South China Sea and the East China Sea). Apparent sediment accumulation rates derived from 210Pb and 137Cs profiles vary from <0.1 to >2 cm/yr, averaging ∼0.4 cm/yr and showing a spatial pattern closely related to hydrodynamics and sediment source-to-sink pathways. Spatial-temporal variation of 7Be activity in surface sediments off Taiwan’s west coast indicates episodic deposition of flood layers and their mobility from river estuaries toward the north. In conjunction with particle size distribution in surface sediments and the structure of sediment strata revealed by sub-bottom echo images; the radionuclide data can be used to outline three different sediment source-to-sink dispersal systems. Based on sediment loads of surrounding rivers and the distribution of sediment accumulation rates, lateral transport is required to account for the budget and size distribution of sediments in the strait.  相似文献   

10.
The radionuclides137Cs,210Pb and7Be have been examined in the alpine Rhoˆne watershed (Switzerland) during a period of two years in order to evaluate their usefulness as tracers of the removal and transport rate of top-soil particles and particle-reactive contaminants of atmospheric origin. The specific activities of the radionuclides in fluvial suspension show a distinct seasonal pattern which depends on the hydrologic regime of the stream and the sources of the suspended matter. Input-output budgets based on the atmospheric deposition and fluvial removal of three radionuclides in the alpine Rhoˆne watershed are used to estimate their erosional residence times. The simplest one box model yields mean residence times of about 800 and 1400 years for137Cs and210Pb, respectively. The removal rate of short-lived7Be suggests that a part of the watershed (0.6–2.3% of the total surface) is exposed to a rapid erosion, in which the mean residence time of the radionuclides is in the range of 1–220 days. This has little influence on the calculated residence time of137Cs but increases the estimated residence time of210Pb in soil to over 1800 years. The use of210Pb-7Be pair in fluvial output may be very helpful in the assessment of the impact of atmospheric pollutants on the water quality in rivers and lakes.  相似文献   

11.
Vertical profiles of the activities of 137Cs and 210Pb were measured on floodplain sediment cores and upland soil cores along the Soda Butte Creek and the Yellowstone River to determine floodplain sedimentation rates. The position of mine tailings from a 1950 impoundment failure was used as a stratigraphic marker to estimate the sedimentation rates and to make comparisons with rates provided by radionuclide‐based methods. Mass accumulation (sedimentation) rates calculated from the position of the mine tailings ranged from 0·00 to 0·17 g cm?2 yr?1 and were in good agreement with sedimentation rates calculated from the inventories of 137Cs and 210Pb. Sedimentation rates calculated from the position of the 137Cs peak generally overestimated the sedimentation rates, probably because of increased downward migration of 137Cs caused by the low pH of water moving through the mine tailings or the high permeability of floodplain sediments relative to upland reference soils. This study demonstrates that the 137Cs and 210Pb inventory methods for determining sedimentation rates can be applied to an alpine floodplain where sedimentation events are episodic and where orographic effects on precipitation generate strong downstream gradients in the delivery of atmospheric radionuclides. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

12.
Bat guano deposits are increasingly used as records of past environmental changes, an approach that requires a precise chronology of the guano layers. This paper presents a comparison between the well-established 14C dating method and methods based on natural 210Pb excesses, (210Pb)ex, and artificial radionuclides 137Cs and 241Am. The studied example is a bat guano deposit from a cave in SW France (the Brantites III cave), which is currently investigated for paleo-environmental reconstructions using stable isotopes. 14C data show that the upper part of the guano deposit accumulated during the last 150 years with a marked increase in accumulation rates after around 1960 AD. While the incorporation of atmospheric 14C in guano is a well-understood process, the origin of 210Pb excesses is more complex. Based on consideration of 137Cs and (210Pb)ex inventories recorded in undisturbed soils in France, and the measured inventories in the guano deposit, we suggest that most of the 210Pb excess is produced by 222Rn decay in the cave air and then adsorbed onto the guano. As Radon concentrations in caves can vary significantly on both short and long-term timescales, one needs to be cautious before applying the often-used CRS (constant rate of supply of 210Pb excess) model to guano dating. Our (210Pb)ex data are best interpreted by two successive periods of roughly constant, but widely different accumulation rates (0.3 cm/y and 2.6 cm/y before and after 1960, respectively) and (210Pb)ex fluxes. We suggest that these relatively abrupt variations result from a change in cave ventilation leading to a more favourable shelter for bats after 1960. The upper 40 cm of the deposit shows evidence of 210Pb mobility, adding a further complexity to the interpretation of (210Pb)ex profiles in guano deposits. However, the existence of well-defined 137Cs and 241Am peaks allows a precise identification of the year of maximum atmospheric fallouts (∼1963–1964). When the ages provided by artificial radionuclides are combined with the 210Pb-derived accumulation rates, an age model can be built, which is in good agreement with the 14C age model. This example shows that the (210Pb)ex method, when associated with 137Cs (241Am) data, can be used to date recent guano deposit, although its application is not as straightforward as the 14C method.  相似文献   

13.
The vertical distributions of210Pb and226Ra in the Santa Barbara Basin have been measured. The210Pb/226Ra activity ratio is close to unity in surface water, but ranges from 0.2 to 0.6 in deep water with a mean value of 0.3 (d > 250m), suggesting rapid removal of210Pb from the water column. The210Pb concentrations in the particulate phase at different water depths indicate that the removal of210Pb is due to adsorption on settling particles.It is estimated that the particulate210Pb contributes about 50–70% of the total210Pb measured on unfiltered water samples of the Santa Barbara Basin. The fate of210Pb (and Pb) in the water column is thus strongly controlled by the settling particles, which have a mean residence time of one year or less in the basin. Material balance calculation for210Pb in the basin suggests that there is an external source supplying about 70–80% of the210Pb observed in particulate material or sediments. This excess210Pb is most likely provided by particles entering the basin loaded already with210Pb.  相似文献   

14.
Particle-reactive radionuclides were determined in sediments from the inner New York Bight to trace transport and storage of fine-grained sediments and associated reactive materials. Seven sediment ? cores 20–50 cm in length were analyzed for water content, loss on ignition (LOI) and excess210Pb; three of these were also analyzed for239,240Pu. Excepting some depth horizons in a core from a dredge-spoil dumpsite, every sample analyzed contained excess210Pb. Variations in the concentration of excess210Pb with depth in the sediment at all stations correlated strongly with LOI, which apparently traces that fraction of the sediment which is active in removing reactive elements from the water column. In the cores analyzed for239,240Pu, every sample contained finite Pu, and Pu concentrations correlated strongly with excess210Pb.The radionuclide distributions may be simply viewed as products of steady-state sediment accumulation or of mixing. Geochemically reasonable accumulation rates are very high (0.5–2.6 g/cm2 y) and could probably only be sustained by offshore transport of dumped materials. At the other extreme the relationships between excess210Pb and LOI are compatible with rapid mixing of a210Pb carrier phase (traced by LOI) into the pre-existing substrate with little or no actual accumulation. Other non-steady-state processes, such as sediment gravity flow, could also explain the observed distributions.Measured sediment inventories (dpm/cm2) of excess210Pb and Pu at these stations are greatly in excess of those supportable by direct atmospheric deposition: lateral supply is required. Incorporation of sedimentary fines into the sand substrate could make the inner New York Bight an important repository of reactive materials.  相似文献   

15.
Four cores recovered within the framework of the INTERPOL Project have been analysed for their grain size and geochemistry; sediment accumulation rates (SARs) were also determined from 210Pb and 137Cs profiles. Two cores are representative of the Axios and Aliakmon Rivers depositional environment, whilst the third core represents the Pinios River province; the fourth core represents an environment of outer shelf relict sands. Apparent SARs ranged between 0.667 g cm−2 yr−1 (Axios and Aliakmon Rivers) and 0.414 g cm−2 yr−1 (Pinios River). Trawling activities and biomixing are critical processes that may be responsible for the mixing of the surface sediments, as observed from the excess 210Pb profiles. The thickness of the surface mixed layer was 4.5 cm in the vicinity of Axios and Aliakmon Rivers and in the area of Pinios River, 3.75 cm on the outer shelf and 1 cm in the area where no trawling was observed. Sediment accumulation appeared to be regulated by variations in the riverine discharge, shelf transport pathways and winnowing processes. Major element variations, such as Si, Al, Ti, V and Ni, were dominated by terrigenous supply as aluminosilicate minerals and quartz, whereas most Ca and Sr were biogenic. Si/Al and Ca/Al ratios have been used to express changes in sediment accumulation and winnowing. Redox processes were depicted by Mn, which showed an increase in the depth of its redoxcline, from 1 cm in inshore stations to 2 cm on the outer shelf. Si/Al ratios follow the Ca/Al ratios and can be used to assess percentage winnowing in the sediment. Increases in these ratios indicate a decrease in sediment input rates and are seen in the upper parts of most of the cores. Anthropogenic or ‘excess’ metal contents have been calculated from Zn/V and Pb/V ratios. Their distributions in the cores showed that by far the highest contamination is associated with the Axios River output, whilst sediments influenced by the Pinios River were relatively uncontaminated.  相似文献   

16.
Cores taken at Burrinjuck Reservoir in southeastern New South Wales have been dated using the first appearance of 137Cs, charcoal/bushfire correlations, and annual grass pollen peaks. None of the main 210Pb dating models reproduced the ‘known’ chronology. Correlation analysis shows no significant relationship between original 210Pb (unsupp.) concentration and grain-size, sedimentation rate or loss on ignition. Differences in sediment source may explain the variations in 210Pb. A simple provenance model has been used to interpret the ratio of original 210Pb (unsupp.)/226Ra as a tracer of topsoils and subsoils. High ratios in the reservoir sediments probably indicate eroded topsoils and low ratios eroded subsoils.  相似文献   

17.
Anthropogenic radionuclides have reached the Hudson estuary as global fallout from nuclear weapons testing and through local releases from commercial nuclear reactors. Significant activities of238Pu and239,240Pu (fallout-derived),134Cs and60Co (reactor-released), and137Cs (derived from both sources), have accumulated in the sediments throughout the estuary, with the primary zone of accumulation near the downstream end of the system in New York harbor. The estuary appears to have trapped nearly all of the239,240Pu delivered as fallout, and consequently, ocean dumping of dredged harbor sediment is currently the primary means for the net transport of these nuclides to coastal waters. In contrast, only 10–30% of the137Cs,134Cs and60Co delivered to the estuary have been retained on the fine particles which accumulate at a rapid rate in the harbor.The primary factors which have governed the distribution of anthropogenic radionuclides in Hudson sediments are: (1) spread of fine particles labeled with both fallout and reactor nuclides throughout the axis of the estuary, (2) differences in timing of the peak fallout years (1962–1964) and years of maximum reactor releases (1971–1972), (3) large variations in sediment accumulation rates, ranging from a few millimeters per year or less to many tens of centimeters per year, (4) appreciable desorption of137Cs and134Cs from particles at higher salinities, and (5) possible enhanced desorption of60Co at higher salinities (relative to134Cs and137Cs) which may be associated with the release of reduced manganese from the harbor sediments.  相似文献   

18.
Floodplains comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of large dryland floodplains is not well understood. Processes occurring on such floodplains are often difficult to observe, and techniques used to investigate smaller perennial floodplains are often not practical in these environments. This study assesses the utility of 137Cs inventory and depth‐profile techniques for determining relative amounts of floodplain sedimentation in the Fitzroy River, northeastern Australia; a 143 000 km2 semi‐arid river system. Caesium‐137 inventories were calculated for floodplain and reference location bulk soil cores collected from four sites. Depth profiles of 137Cs concentration from each floodplain site and a reference location were recorded. The areal density of 137Cs at reference locations ranged from 13 to 978 Bq m–2 (0–1367 Bq m–2 at the 95% confidence interval), and the mean value ± 2 (standard error of the mean) was 436 ± 264 Bq m–2, similar to published data from other Southern Hemisphere locations. Floodplain inventories ranged from 68 to 1142 Bq m–2 (0–1692 Bq m–2 at the 95% confidence interval), essentially falling within the range of reference inventory values, thus preventing calculation of erosion or deposition. Depth‐profiles of 137Cs concentration indicate erosion at one site and over 66 cm of deposition at another since 1954. Analysis of 239+240Pu concentrations in a depositional core substantiated the interpretation made from 137Cs data, and depict a more tightly constrained peak in concentration. Average annual deposition rates range from 0 to 15 mm. The similarity between floodplain and reference bulk inventories does not necessarily indicate a lack of erosion or deposition, due to low 137Cs fallout in the region and associated high measurement uncertainties, and a likely influence of gully and bank eroded sediments with no or limited adsorbed 137Cs. In this low‐fallout environment, detailed depth‐profile data are necessary for investigating sedimentation using 137Cs. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

19.
The Earth's surface erodes by processes that occur over different spatial and temporal scales. Both continuous, low‐magnitude processes as well as infrequent, high‐magnitude events drive erosion of hilly soil‐mantled landscapes. To determine the potential variability of erosion rates we applied three independent, field‐based methods to a well‐studied catchment in the Marin Headlands of northern California. We present short‐term, basin‐wide erosion rates determined by measuring pond sediment volume (40 years) and measured activities of the fallout nuclides 137Cs and 210Pb (40–50 years) for comparison with long‐term (>10 ka) rates previously determined from in situ‐produced cosmogenic 10Be and 26Al analyses. In addition to determining basin‐averaged rates, 137Cs and 210Pb enable us to calculate point‐specific erosion rates and use these rates to infer dominant erosion processes across the landscape. When examined in the context of established geomorphic transport laws, the correlations between point rates of soil loss from 137Cs and 210Pb inventories and landscape morphometry (i.e. topographic curvature and upslope drainage area) demonstrate that slope‐driven processes dominate on convex areas while overland flow processes dominate in concave hollows and channels. We show a good agreement in erosion rates determined by three independent methods: equivalent denudation rates of 143 ± 41 m Ma?1 from pond sediment volume, 136 ± 36 m Ma?1 from the combination of 137Cs and 210Pb, and 102 ± 25 m Ma?1 from 10Be and 26Al. Such agreement suggests that erosion of this landscape is not dominated by extreme events; rather, the rates and processes observed today are indicative of those operating for at least the past 10 000 years. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

20.
湖泊沉积记录研究对了解流域侵蚀、揭示区域气候环境变化及人类活动影响、建立外生地球化学循环模式等均具有重要意义.放射性同位素~(210)Pb和~(137)Cs组合定年法是百年尺度湖泊沉积记录研究的首选方法,在过去几十年中得到了广泛应用,大力推动了湖泊沉积记录的高分辨率气候环境变化研究的开展.然而,如何理解和选择适用的计算模式来尽可能地提高定年准确度目前仍存在争议,这在一定程度上限制了该方法的应用.鉴于上述问题,本文基于本实验室近年来从青藏高原获取的若干支代表性湖芯的定年结果,从样品前处理、仪器及测试、数据分析及计算等全过程对~(210)Pb、~(137)Cs定年原理和方法进行了较为系统的阐述;在此基础上,提出了~(210)Pb定年样品封装原则,探讨了高纯锗γ谱仪在放射性活度测量中的影响因素,并建立了准确有效的比活度校正方法;明确指出了恒定初始浓度模式(constant initial concentration,CIC)可用于计算沉积物每层的年龄,而不是部分研究中认为的平均沉积速率,这对于深刻理解该定年模式并提供准确的定年结果具有重要的参考意义.同时,通过对比两种放射性核素的分布特征发现,相对于~(210)Pb而言,~(137)Cs更容易发生垂向迁移进而影响其时标准确性,这需引起研究者的充分重视,因此,当二者定年结果出现明显差异时,建议以~(210)Pb定年结果为准.  相似文献   

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