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1.
The results of microbiological, biogeochemical, and isotope geochemical studies in the Kara Sea are described. The samples for these studies were obtained during the 54th voyage of the research vessel Akademik Mstislav Keldysh in September 2007. The studied area covered the northern, central, and southwestern parts of the Kara Sea and the Gulf of Ob. The quantitative characteristics of the total bacterial population and the activity of the microbial processes in the water column and bottom sediments were obtained. The total population of the bacterioplankton (BP) varied from 250000 cells/ml in the northern water area to 3000000 cells/ml in the Gulf of Ob. The BP population depended on the content of the water suspension. The net BP production was minimal in the central water area, amounting to 0.15–0.2 μg C/(l day), and maximal (0.5–0.75 μg C/(l day)) in the Gulf of Ob. The organic material at the majority of the stations in the Ob transect predominantly contained light carbon isotopes (−28.0 to −30.18‰) of terrigenous origin. The methane content in the surface water layer varied from 0.18 to 2.0 μl CH4/l, and the methane oxidation rate changed in the range of 0.1–100 nl CH4/(l day). The methane concentration in the upper sediment layer varied from 30 to 300 μl CH4/dm3; the rate of the methanogenesis was 44 to 500 nl CH4/(dm3 day) and that of the methane oxidation, 30 to 2000 nl CH4/(dm3 day). The rate of the sulfate reduction varied from 4 to 184 μg S/(dm3 day).  相似文献   

2.
The results of an analysis of data on the total content of nitrogen dioxide in a vertical atmospheric column are given. These data have been obtained from measurements with the twilight method over a period of 25 years. The monthly and annual means (the arithmetic means of both morning and evening values) of NO2, on the whole, have increased by ～6% in spite of its rapid decrease in 1991–1995 due to the Pinatubo eruption. The linear-trend index amounts to 0.23% per year. The annual mean over the entire observation time is equal to (3.18 ± 0.05) × 1015 mol/cm2, and the amplitude of seasonal variations amounts to (2.39 ± 0.04) × 1015 mol/cm2. Spectral analysis of the experimental data has revealed compound oscillations with periods of 6 to 253 months, the values of which do not contradict published data. Most of these oscillations are nonharmonic. A simple statistical model satisfactorily describes time variations in the monthly and annual means of NO2 with rms deviations of ～4% and 1%, respectively.  相似文献   

3.
A new seafloor observatory, the gas monitoring module (GMM), has been developed for continuous and long-term measurements of methane and hydrogen sulphide concentrations in seawater, integrated with temperature (T), pressure (P) and conductivity data at the seafloor. GMM was deployed in April 2004 within an active gas-bearing pockmark in the Gulf of Patras (Greece), at a water depth of 42 m. Through a submarine cable linked to an onshore station, it was possible to remotely check, via direct phone connection, GMM functioning and to receive data in near-real time. Recordings were carried out in two consecutive campaigns over the periods April–July 2004, and September 2004–January 2005, amounting to a combined dataset of ca. 6.5 months. This represents the first long-term monitoring ever done on gas leakage from pockmarks by means of CH4+H2S+T+P sensors. The results show frequent T and P drops associated with gas peaks, more than 60 events in 6.5 months, likely due to intermittent, pulsation-like seepage. Decreases in temperature in the order of 0.1–1°C (up to 1.7°C) below an ambient T of ca. 17°C (annual average) were associated with short-lived pulses (10–60 min) of increased CH4+H2S concentrations. This seepage “pulsation” can either be an active process driven by pressure build-up in the pockmark sediments, or a passive fluid release due to hydrostatic pressure drops induced by bottom currents cascading into the pockmark depression. Redundancy and comparison of data from different sensors were fundamental to interpret subtle proxy signals of temperature and pressure which would not be understood using only one sensor.  相似文献   

4.
ensemble simulations with the A.M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences (IAP RAS) climate model (CM) for the 21st century are analyzed taking into account anthropogenic forcings in accordance with the Special Report on Emission Scenarios (SRES) A2, A1B, and B1, whereas agricultural land areas were assumed to change in accordance with the Land Use Harmonization project scenarios. Different realizations within these ensemble experiments were constructed by varying two governing parameters of the terrestrial carbon cycle. The ensemble simulations were analyzed with the use of Bayesian statistics, which makes it possible to suppress the influence of unrealistic members of these experiments on their results. It is established that, for global values of the main characteristics of the terrestrial carbon cycle, the SRES scenarios used do not differ statistically from each other, so within the framework of the model, the primary productivity of terrestrial vegetation will increase in the 21st century from 74 ± 1 to 102 ± 13 PgC yr−1 and the carbon storage in terrestrial vegetation will increase from 511 ± 8 to 611 ± 8 PgC (here and below, we indicate the mean ± standard deviations). The mutual compensation of changes in the soil carbon stock in different regions will make global changes in the soil carbon storage in the 21st century statistically insignificant. The global CO2 uptake by terrestrial ecosystems will increase in the first half of the 21st century, whereupon it will decrease. The uncertainty interval of this variable in the middle (end) of the 21st century will be from 1.3 to 3.4 PgC yr−1 (from 0.3 to 3.1 PgC yr−1). In most regions, an increase in the net productivity of terrestrial vegetation (especially outside the tropics), the accumulation of carbon in this vegetation, and changes in the amount of soil carbon stock (with the total carbon accumulation in soils of the tropics and subtropics and the regions of both accumulation and loss of soil carbon at higher latitudes) will be robust within the ensemble in the 21st century, as will the CO2 uptake from the atmosphere only by terrestrial ecosystems located at extratropical latitudes of Eurasia, first and foremost by the Siberian taiga. However, substantial differences in anthropogenic emissions between the SRES scenarios in the 21st century lead to statistically significant differences between these scenarios in the carbon dioxide uptake by the ocean, the carbon dioxide content in the atmosphere, and changes in the surface air temperature. In particular, according to the SRES A2 (A1B, B1) scenario, in 2071–2100 the carbon flux from the atmosphere to the ocean will be 10.6 ± 0.6 PgC yr−1 (8.3 ± 0.5, 5.6 ± 0.3 PgC yr−1), and the carbon dioxide concentration in the atmosphere will reach 773 ± 28 ppmv (662 ± 24, 534 ± 16 ppmv) by 2100. The annual mean warming in 2071–2100 relatively to 1961–1990 will be 3.19 ± 0.09 K (2.52 ± 0.08, 1.84 ± 0.06 K).  相似文献   

5.
Substantial amounts of adsorbed methane were detected in authigenic carbonate concretions recovered from sedimentary layers from depths between 245 and 1,108 m below seafloor during Ocean Drilling Program Leg 186 to ODP sites 1150 and 1151 on the deep-sea terrace of the Japan Trench. Methane contents were almost two orders of magnitude higher in the concretions (291–4,528 nmol/g wet wt) than in the surrounding bulk sediments (5–93 nmol/g wet wt), whereas methane/ethane ratios and stable carbon isotopic compositions were very similar. Carbonate content of surrounding bulk sediments (0.02–3.2 wet wt%) and methane content of the surrounding bulk sediments correlated positively. Extrapolation of the carbonate contents of bulk sediments suggests that 100 wt% carbonate would correspond to 1,886±732 nmol methane per g bulk sediment, which is similar to the average value observed in the carbonate concretions (1,321±1,067 nmol/g wet wt, n = 13). These data support the hypothesis that, in sediments, adsorbed hydrocarbon gases are strongly associated with authigenic carbonates.  相似文献   

6.
Egorov  A. V.  Ivanov  M. K. 《Geo-Marine Letters》1998,18(2):127-138
 Microbiologically produced hydrocarbon gases (HCGs) in normal pelagic sediments have lithologically controlled distribution – their content increases sharply in organic-rich sapropels. Generally, the HCG content is low (<10000 nl/l), The amount of heavy HCGs is high (up to 60%, unsaturated HCGs dominate the saturated ones, and ethylene is prevalent. The same features were found in sediment and mud breccia from inactive mud volcanoes. Thermogenic HCG was determined in active mud volcanoes and in a high salinity fluid vent. They are characterized by: high methane concentration, δ13C(CH4) =−37.1 to −57.8%, essential ethane contents (2–7%), absence of unsaturated HCG, and the prevalence of iso-over n-butane.  相似文献   

7.
Data on the NO2 content in the vertical column of the atmosphere obtained with the Ozone Monitoring Instrument (OMI) aboard the EOS Aura satellite (United States) in the period from October 2004 to October 2007 are compared with the results of ground-based measurements at the Zvenigorod Scientific Station (55.7° N, 36.8° E). The “unpolluted”; part of the total NO2 content in the atmospheric column, which mostly represents the stratosphere, and the NO2 contents in the vertical column of the troposphere, including the lower layer, which is subject to pollution, are included in the comparison. The correlation coefficient between the results of ground-based and satellite measurements of the “unpolluted” total NO2 content is ∼0.9. The content values measured with the OMI instrument are smaller than the results of ground-based measurements (on average, by (0.30 ± 0.03) × 1015 cm−2 or by (11 ± 1)%). Therms discrepancy between the satellite and ground-based data is 0.6 × 1015 cm−2. The NO2 content in the vertical column of the troposphere from the results of satellite measurements is, on average, (1.4 ± 0.5) × 1015 cm−2, (or about 35%) smaller than from the results of ground-based measurements, and the rms discrepancy between them is about 200%. The correlation coefficient between these data is ∼0.4. This considerable discrepancy is evidently caused by the strong spatial (horizontal) inhomogeneity and the temporal variability of the NO2 field during episodes of pollution, which leads to different (and often uncorrelated) estimates of the NO2 content in the lower troposphere due to different spatial resolutions of ground-based and satellite measurements.  相似文献   

8.
Based on the experimental data obtained in 1990–1993 by the method of isotopic tracers with the help of a stable isotope of nitrogen (15N), we establish basic regularities of the formation of “new” and regeneration production in the Black Sea and reveal the factors specifying their combination. It is shown that the rates of nitrate and ammonium uptake by microplankton vary from the minimum values in winter to the maximum values in summer. In the surface layer, the uptake of nitrates corresponding to the amount of “new” production in deep-water layers is equal to ∼ 50% (in winter) and ∼ 30% (in summer) of the total uptake of inorganic nitrogen compounds by microplankton. In the zone of photosynthesis, the average fractions of nitrates are equal to 31 ± 10% in winter and 41 ± 10% in summer. The minimum values of this parameter are attained in the middle of spring and in autumn. The fraction of “new” production (f-ratio) and the integral content of nitrates in the zone of photosynthesis are connected by a hyperbolic dependence. The period of cyclic transformations of nitrates in this zone decreases from several dozens of days at the beginning of winter to 12 h in the mid-spring. In summer, this period is equal, on the average, to one day. The average period of cyclic transformations of ammonium is equal to 15 ± 4 h in winter and 5 ± 3 h in summer. __________ Translated from Morskoi Gidrofizicheskii Zhurnal, No. 6, pp. 29–43, November–December, 2006.  相似文献   

9.
We investigated changes in the global distribution of surface-layer salinity by comparing 2003–2007 Argo-float data with annual mean climatological surface-layer salinity data for 1960–1989 from the World Ocean Database 2005. The two datasets showed similar patterns, with low values in subpolar and tropical regions and higher values in the subtropics. The recent Argo data indicate that the contrast between low and high salinity has intensified in all areas except the subpolar North Atlantic. The intensified contrast of the surface layer salinity was maintaining for 2003–2007. Using a simple method, we attempted to estimate evaporation and precipitation changes on the basis of surface-layer salinity changes. The results show a high probability that the global hydrological cycle has increased in the past 30 years.  相似文献   

10.
Concentrations of dissolved methane in seawater and bottom sediments, as well as of methane emanating from gas seeps were measured at 18 stations including several small bays in the Sevastopol coastal area (Black Sea) during 2007–2008. Methane concentrations in surface waters ranged from 10 to 2,970 nmol l?1, and correlated well with values recorded for sediments. Methane concentrations in the water column were influenced by water depth, as well as by air and water temperatures. In the spring and summer of 2008, in situ CH4 saturation relative to air was in the range of 970–71,900%. Maximum saturation was in summer. CH4 fluxes to the atmosphere from the Sevastopol coastal area were estimated to vary from 190 to 1,550 μmol m?2 day?1. Gas bubbles escaping from the seepages contained about 57 vol% methane. Radiocarbon dating of the methane revealed an age not exceeding 150 years, implying a biogenic origin.  相似文献   

11.
Data from satellite altimeters and from a 13-month deployment of in situ instruments are used to determine an empirical relationship between sea-level anomaly difference (SLA) across the Kuroshio in the East China Sea (ECS-Kuroshio) and net transport near 28°N. Applying this relationship to the altimeter data, we obtain a 12-year time series of ECS-Kuroshio transport crossing the C-line (KT). The resulting mean transport is 18.7 ± 0.2 Sv with 1.8 Sv standard deviation. This KT is compared with a similarly-determined time series of net Ryukyu Current transport crossing the O-line near 26°N southeast of Okinawa (RT). Their mean sum (24 Sv) is less than the mean predicted Sverdrup transport. These KT and RT mean-flow estimates form a consistent pattern with historical estimates of other mean flows in the East China Sea/Philippine Basin region. While mean KT is larger than mean RT by a factor of 3.5, the amplitude of the KT annual cycle is only half that of RT. At the 95% confidence level the transports are coherent at periods of about 2 years and 100–200 days, with RT leading KT by about 60 days in each case. At the annual period, the transports are coherent at the 90% confidence level with KT leading RT by 4–5 months. While the bulk of the Kuroshio enters the ECS through the channel between Taiwan and Yonaguni-jima, analysis of satellite altimetry maps, together with the transport time series, indicates that the effect of mesoscale eddies is transmitted to the ECS via the Kerama Gap southwest of Okinawa. Once the effect of these eddies is felt by the ECS-Kuroshio at 28°N, it is advected rapidly to the Tokara Strait.  相似文献   

12.
We describe the specific features of the summer 2010 emergency conditions in the European part of the Russian Federation, when an anomalous heat wave (the monthly mean temperatures in the summer months were 5–9°C higher than those for 2002–2009) and prolonged blocking anticyclones led to large wildfires. We analyze their causes and consequences. The features of the satellite system for operational fire monitoring (constructed at the Aerospace Scientific Center) and examples of its application in summer 2010 are presented. On the basis of the results of processing of satellite images of low (250–1000 m), medium (∼30–50 m), and high (∼6 m) resolutions, we found that the total area covered by fire from March to November of 2010 amounted to approximately 10.9 million hectares for the entire territory of the country and and 2.2 million hectares for its European part. Daily histograms of areas covered by fire in the summer months of 2010 were constructed. On the basis of these data and empirical models, we estimate the daily emissions of carbon monoxide (CO) from wildfires in the summer months of 2010 for the European part of Russia and Moscow oblast. On some days in August 2010, these emissions reached 15000–27000 t for the European part of Russia and 3000–7500 t for Moscow oblast. On the basis of analysis of data from the AIRS spectrometer (Aqua satellite), we derived the spatial distribution of CO concentrations at heights of 2 to 10 km above the territory of the Eastern and Central Europe. Moscow was shown to have been most severely affected by smoke from wildfires occurring on August 6–9, 2010, when the concentrations of harmful gases (CO2, CO, CH4, and O3) and aerosols in the air significantly exceeded both the daily and the one-hour maximum allowable concentrations.  相似文献   

13.
The monthly average values of the anomalies of the ocean level (according to the satellite data for 1992–2002) and the annual average dynamic heights (hydrological data) are used to compute the seasonal cycle of geostrophic currents on the surface of the Atlantic Ocean. It is shown that the west and east currents are intensified with a phase difference of several months. At the same time, their latitudinal displacements are quasisynchronous. A delay of the seasonal signal in the east-west direction of about 2–3 months (on the average) is typical of currents in the tropical zone of the Northern Hemisphere. On the contrary, in the South Atlantic, the seasonal signal propagates in the west-east direction and its phase delay can be as large as almost six months. __________ Translated from Morskoi Gidrofizicheskii Zhurnal, No. 3, pp. 60–71, May–June, 2006.  相似文献   

14.
Natural marine gas hydrate was discovered in Korean territorial waters during a 2007 KIGAM cruise to the central/southwestern Ulleung Basin, East Sea. The first data on the geochemical characterization of hydrate-bound water and gas are presented here for cold seep site 07GHP-10 in the central basin sector, together with analogous data for four sites (07GHP-01, 07GHP-02, 07GHP-03, and 07GHP-14) where no hydrates were detected in other cores from the central/southwestern sectors. Hydrate-bound water displayed very low concentrations of major ions (Cl−, SO42−, Na+, Mg2+, K+, and Ca2+), and more positive δD (15.5‰) and δ18O (2.3‰) signatures compared to seawater. Cl– freshening and more positive isotopic values were also observed in the pore water at gas hydrate site 07GHP-10. The inferred sulfate–methane interface (SMI) was very shallow (<5 mbsf) at least at four sites, suggesting the widespread occurrence of anaerobic oxidation of methane (AOM) at shallow sediment depths, and possibly high methane flux. Around the SMI, pore water alkalinity was very high (>40 mM), but the carbon isotopic ratios of dissolved inorganic carbon (δ13CDIC) did not show minimum values typical of AOM. Moreover, macroscopic authigenic carbonates were not observed at any of the core sites. This can plausibly be explained by carbon with high δ13C values diffusing upward from below the SMI, increasing alkalinity via deep methanogenesis and eventually escaping as alkalinity into the water column, with minor precipitation as solid phase. This contrasts, but is not inconsistent with recent reports of methane-fuelled carbonate formation at other sites in the southwestern basin sector. Methane was the main hydrocarbon component (>99.85%) of headspace, void, and hydrate-bound gases, C1/C2+ ratios were at least 1,000, and δ13CCH4 and δDCH4 values were in the typical range of methane generated by microbial reduction of CO2. This is supported by the δ13CC2H6 signatures of void and hydrate-bound gases, and helps clarify some contradictory interpretations existing for the Ulleung Basin as a whole. In combination, these findings suggest that deep biogenic gas and pore waters migrate upward through pathways such as hydrofractures, and measurably influence the shallow carbon cycle. As a result, cation-adjusted alkalinity/removed sulfate diagrams cannot always serve to estimate the degree of alkalinity produced by sulfate reduction and AOM in high methane flux areas.  相似文献   

15.
We report some main results of multidisciplinary investigations carried out within the framework of the Indian National Gas Hydrate Program in 2002–2003 in the Krishna–Godavari Basin offshore sector, east coast of India, to explore indicators of likely gas hydrate occurrence suggested by preliminary multi-channel seismic reflection data and estimates of gas hydrate stability zone thickness. Swath bathymetry data reveal new evidence of three distinct geomorphic units representing (1) a delta front incised by several narrow valleys and mass flows, (2) a deep fan in the east and (3) a WNW–ESE-trending sedimentary ridge in the south. Deep-tow digital side-scan sonar, multi-frequency chirp sonar, and sub-bottom profiler records indicate several surface and subsurface gas-escape features with a highly resolved stratification within the upper 50 m sedimentary strata. Multi-channel seismic reflection data show the presence of bottom simulating reflections of continuous to discrete character. Textural analyses of 76 gravity cores indicate that the sediments are mostly silty clay. Geochemical analyses reveal decreasing downcore pore water sulphate (SO4 2−) concentrations (28.7 to <4 mM), increasing downcore methane (CH4) concentrations (0–20 nM) and relatively high total organic carbon contents (1–2.5%), and microbial analyses a high abundance of microbes in top core sediments and a low abundance of sulphate-reducing bacteria in bottom core sediments. Methane-derived authigenic carbonates were identified in some cores. Combined with evidence of gas-escape features in association with bottom simulating reflections, the findings strongly suggest that the physicochemical conditions prevailing in the study area are highly conducive to methane generation and gas hydrate occurrence. Deep drilling from aboard the JOIDES Resolution during 2006 has indeed confirmed the presence of gas hydrate in the Krishna–Godavari Basin offshore.  相似文献   

16.
Methane in the western North Pacific   总被引：7，自引：0，他引：7  
The concentration of methane in about 400 seawater samples collected in the western North Pacific, mostly from 40°N to 5°S along 165°E was determined. While the concentration of methane in the surface water was slightly greater in the high-latitudes, it did not widely vary with a standard deviation of 0.29 n mol/l for a mean value of 2.49 n mol/l. The 90% confidence limit of the mean was 0.08 n mol/l. The degree of oversaturation in 1991 (31±4%) was not different from that in circa 1970. If we assume that this degree of oversaturation occurs in the entire oceans, the annual flux of methane becomes 6×1012g CH4. Both the concentrations of methane and chlorophylla were higher in the surface 100 m layer. However, the correlation between them was not well in the entire surface waters. This may indicate that the production of methane is not directly related to the photosynthetic process. The concentration of methane decreased gradually with increasing depth down to 1000 m. Its horizontally and vertically uniform concentration in the abyssal water suggests that the turnover time of methane in the oxic pelagic water is in the range between a few years and a few hundred years.  相似文献   

17.
The results of measurements of the CO content in the atmospheric thickness by the method of solar molecular-absorption spectroscopy are presented. Over 87 months of observations, the annual mean CO content decreased by ～19% at a mean rate of changes equal to ?(0.14 ± 0.02) atm cm per year. Maxima and minima of seasonal variations most often fall on February and September, respectively. The mean overall amplitude of changes in the CO content during the annual cycle is about 50% of the mean value. The Fourier analysis revealed variations in the CO composition with periods from 3 to 84 months. A simple statistical model satisfactorily describes time changes in the CO content in the atmospheric thickness. The results of measurements of the CO content in the atmospheric thickness are compared with the data of CO measurements in samples of surface air at stations of the Global Atmospheric Watch.  相似文献   

18.
To date, only a few coral proxy studies have investigated coral growth as an indicator of climate variability. This study presents the first extension-rate record (Porites lutea) from the Maldives (NW Indian Ocean), inferred from skeletal δ18O chronology for the lagoon of Rasdhoo Atoll (4°N/73°W) in the central area of the Maldives, influenced by the Indian monsoon. The record spans 90 years over the period 1917–2007. The mean annual extension over this period was 9.9 mm/year, and an increase of annual extension rates until 1990 by 3 mm/year can be explained by a rise of 0.7°C in sea surface temperature (SST) in this region. After 1990, the extension rates do no continue increasing, possibly due to ecological stress caused by progressive ocean warming and acidification. The correlation between annual extension rates and SSTs is thus significant and strong in the lower part of the record until 1955 (r = +0.69, p < 0.0001), but weaker thereafter (r = +0.44, p < 0.001). The extension rates yield a distinct interannual variability of 3–4 years, caused by interannual SST fluctuations driven by the El Ni?o-Southern Oscillation. A variability of 8–9 years is likely driven by SST variations endemic to the Indian Ocean. Spectral peaks between 18–19 years and 6–7 years cannot be explained by SST fluctuations, but by variations in the strength of the SW monsoon currents. It is suggested that during phases of stronger monsoon activity, the coral sacrificed coral extension in favor of a denser, more robust skeleton. The geomorphology of the atoll may strengthen the potential of this new coral archive to track climate variability.  相似文献   

19.
The intensity of the processes of organic matter (OM) destruction in the deep-water part of the Arctic Basin is considered in terms of the activities of hydrolytic enzymes (alkaline phosphatase and proteases) and of redox enzymes of the electron transport system (ETS). High concentrations of mineral phosphorus are shown to cause low phosphatase activity (0.000–0.005 μM P/l h). The average time of the phosphate recycling amounted to about 240 h. The ranges of the total and specific activity of protease are 0.000–0.192 mg of azocasein/(l h) and 0.00–3.57 mg of azocasein/h mg of protein, respectively. It is found that the microplankton production of exo- and endopeptidase in the Arctic Basin is controlled by the concentration of nitrates in the water. The values of the total and the specific activities of the ETS enzymes vary within 0.27–8.96 μl O2/(l h) and 8.4–583 μl O2/mg of protein h, respectively. It is shown that the maximum values of the total activities of the hydrolytic and redox enzymes are characteristic for the photic layer. The vertical fluxes of organic carbon from the photic layer, being calculated by the activity of the ETS enzymes, amounted to 220–600 g of Corg/year m2. The presence of ice intensifies the redox processes by factors of 2–15.  相似文献   

20.
Spatial distribution of the carbon and nitrogen content and their isotopic enrichment in suspended matter and sediments were measured in the Godavari estuary to identify the sources and transformation mechanism of organic matter. Significant variability in isotopic distribution was found over the entire length of the Godavari estuary, suggesting multiple sources of organic matter. The mean isotopic ratios (δ13Csed −25.1 ± 0.9, δ13Csus −24.9 ± 1, δ15Nsed 8.0 ± 2 and δ15Nsus 6.5 ± 0.9‰) and elemental concentrations (Csed 0.45 ± 0.2%, Csus 0.9 ± 0.7%, Nsed 0.07 ± 0.05% and Nsus 0.16 ± 0.1%) support a predominantly terrigenous source. Significant enrichment in the isotopic ratios of δ13C from the upper to lower estuary in both suspended (−27.5 and −24.3‰, respectively) and sedimentary (−26.2 and −24.9‰, respectively) phases indicates a decrease in the influence of terrigeneous material toward the mouth of the estuary. A significant positive relationship exists between the δ13C of suspended and sediment, which indicates that these two organic carbon pools are likely coupled in the form of a significant exchange between the two phases. A positive relationship exists between chlorophyll a and suspended organic matter, which may mean that a significant source of organic carbon is the in situ produced phytoplankton. But, applying a simple mixing model to our isotopes, data yielded about 46% as the contribution of the terrestrial source to suspended matter, which may support the excessive heterotrophic activity in the Godavari estuary reported earlier.  相似文献   

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