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1.
The recession of bomb tritium in river discharge of large basins indicates a contribution of slowly moving water. For an appropriate interpretation it is necessary to consider different runoff components (e.g. direct runoff and ground water components) and varying residence times of tritium in these components. The spatially distributed catchment model (tracer aided catchment model, distributed; TACD) and a tritium balance model (TRIBIL) were combined to model process‐based tritium balances in a large German river basin (Weser 46 240 km2) and seven embedded sub‐basins. The hydrological model (monthly time step, 2 × 2 km2) estimated the three major runoff components: direct runoff, fast‐moving and slow‐moving ground water for the period of 1950 to 1999. The model incorporated topography, land use, geomorphology, geology and hydro‐meteorological data. The results for the different basins indicated a contribution of direct runoff of 30–50% and varying amounts for fast and slow ground water components. Combining these results with the TRIBIL model allowed us to estimate the residence time of the components. Mean residence times of 8 to 14 years were found for the fast ground water component, 21 to 93 years for the slow ground water component and 14 to 50 years for an overall mean residence time within these basins. Balance calculations for the Weser basin indicate an over‐estimation of loss of tritium through evapotranspiration (more than 60%) and decay (10%). About 28% were carried in stream‐flow where direct runoff contributed about 12% and ground water runoff 13% in relation to precipitation input over the studied 50‐year period. Neighbouring basins and nuclear power plants contributed about 1% each over this time period. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
2.
Environmental tracers, such as tritium, have generally been used to estimate aquifer recharge under natural conditions. A tritium tracer test is presented for estimating recharge under semi‐arid and irrigated conditions. The test was performed along 429 days (June 2007–August 2008) on an experimental plot located in SE Spain with drip irrigation and annual row crops (rotation of lettuce and melon), in which common agricultural practices were followed in open air. Tritiated water was sprinkled (simulated rainfall) over the plot, soil cores were taken at different depths and a liquid scintillation analyzer was used to measure tritium concentration in soil water samples. Tritium transport, as liquid or vapor phase, was simulated with the one‐dimensional numerical code SOLVEG. Simulations show that the crop water use was below potential levels, despite regular irrigation. Continuous high water content in soil promoted a great impact of rainfall events on the aquifer recharge. The results obtained from tritium tracer test have been compared with other independent recharge assessment, soil water balance method, to evaluate the reliability of the first one. Total recharge from tracer test was 476 mm for the October 2007–September 2008 period versus 561 mm from soil water balance method for the same period, which represents 37.1% and 43.7% of the applied water (1284 mm, irrigation + precipitation), respectively. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
3.
A GLUE‐based uncertainty assessment framework for tritium‐inferred transit time estimations under baseflow conditions 
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下载免费PDF全文 Francesc Gallart Maria Roig‐Planasdemunt Michael K. Stewart Pilar Llorens Uwe Morgenstern Willibald Stichler Laurent Pfister Jérôme Latron 《水文研究》2016,30(25):4741-4760
The last decade has seen major technical and scientific improvements in the study of water transfer time through catchments. Nevertheless, it has been argued that most of these developments used conservative tracers that may disregard the oldest component of water transfer, which often has transit times greater than 5 years. Indeed, although the analytical reproducibility of tracers limits the detection of the older flow components associated with the most dampened seasonal fluctuations, this is very rarely taken into account in modelling applications. Tritium is the only environmental tracer at hand to investigate transfer times in the 5‐ to 50‐year range in surface waters, as dissolved gases are not suitable due to the degassing process. Water dating with tritium has often been difficult because of the complex history of its atmospheric concentration, but its current stabilization together with recent analytical improvements open promising perspectives. In this context, the innovative contribution of this study lies in the development of a generalized likelihood uncertainty estimation‐based approach for analysing the uncertainties associated with the modelling of transit time due to both parameter identification and tracer analytical precision issues. A coupled resampling procedure allows assessment of the statistical significance of the transfer time differences found in diverse waters. This approach was developed for tritium and the exponential‐piston model but can be implemented for virtually any tracer and model. Stream baseflow, spring and shallow aquifer waters from the Vallcebre research catchments, analysed for tritium in different years with different analytical precisions, were investigated by using this approach and taking into account other sources of uncertainty. The results showed three groups of waters of different mean transit times, with all the stream baseflow and spring waters older than the 5‐year threshold needing tritium. Low sensitivity of the results to the model structure was also demonstrated. Dual solutions were found for the waters sampled in 2013, but these results may be disambiguated when additional analyses will be made in a few years. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
4.
The mean residence time (MRT) of karst groundwater in three mountainous catchments of the Western Himalaya was estimated using multiple approaches: the tritium method, the sine wave model and tracer tests. Water samples were collected from precipitation, glacier melt, streams and karst springs for δ2H and tritium analysis during 2012 and 2013. High tritium values were observed in winter precipitation and low values in summer precipitation. The variation of tritium in karst springs was similar to that of the streams, whereas glacier melt showed lower tritium values. The MRT of cold karst springs was shorter than that of warm karst springs. The tracer breakthrough curves (TBC) retrieved for different springs suggested a short travel time for groundwater and possibly conduit flow. Deterioration of water quality and variation in flux magnitude are the two main practical consequences of the short travel time of karst groundwater in the region.
EDITOR D. KoutsoyiannisASSOCIATE EDITOR K. Heal 相似文献
5.
ABSTRACT The distribution of environmental tritium, deuterium and oxygen-18 in the unsaturated zone and the underlying sandy phreatic aquifer was studied throughout 1981 in an area of high pine forests in the Rhine valley near Heidelberg. The observed vertical distribution of isotopes in the unsaturated zone can be satisfactorily explained by the combined use of a multi-cell model for moisture transport and an evapotranspiration model. The distribution in the underlying aquifer of the tracer input at the water table obtained using this method is found by replacing the total vertical diffusion coefficient in the diffusion equation with the dispersion coefficient. In this way observed tritium profiles are satisfactorily simulated for the period 1966–1981. The stable isotope profile in the unsaturated zone however remains largely unexplained due to inadequate data on the stable isotope content of precipitation over the investigated area. 相似文献
6.
Jun Shimada 《水文研究》1988,2(1):43-59
It is very interesting and meaningful to investigate the rainfall-groundwater recharge process under the humid climatic condition of Japan, where mean annual precipitation is about 1600 mm. The present study has investigated soil water movement in the unsaturated zones of a volcanic ash layer, called the ‘Kanto Loam formation’, using environmental tritium as a tracer. The site selected is a flat ground surface on a terraced upland which has a deep unsaturated zone (about 20 m) with a relatively high water content (about 70 per cent) consisting of nearly uniform Kanto Loam formation. The tritium concentrations in groundwater, soil waters having different matric potentials, precipitation, and the seepage water moving through the formation into a man-made cave were measured to characterize the rainfall-groundwater recharge process and the effect of large pore spaces in the formation mentioned by previous studies. Because of the humid climate of Japan, there appears to be a unique soil water flow characteristic which may involve percolation through large pore spaces during heavy rainfall. However, in a fine grained and high water content soil like the Kanto Loam formation, the existence of this flow through large pore spaces does not have a significant effect upon the whole recharge process. The recharge model of displacement flow with dispersion is useful in estimating the tritium concentration profile of soil water. The calculated result shows a recharge rate of 2.5 mm/day. The value obtained reflects the hydrological characteristics of the uplands covered with volcanic ash. 相似文献
7.
Tritium data in the Dead Sea for the period 1960–1979 are given. Tritium levels have increased until 1965 in the upper layers of the Dead Sea reaching a level of 170 TU, in response to the atmospheric buildup of tritium from thermonuclear testing. The levels have been decreasing ever since, both because of rapidly declining atmospheric concentrations of tritium and because of mixing of the surface layers with tritium deficient, deeper water masses. The depth of penetration of the tracer delineated the depth of meromictic stratification and successfully monitored the deepening of the pycnocline, until the overturn in 1979 homogenised the entire tritium profile. Modelling the changing tritium inventory over this period showed the predominance of the direct exchange across the air/sea interface, both in the buildup of tritium in the lake and also in its subsequent removal from it. The good fit between calculated and measured tritium inventories confirmed the evaporation estimate of 1.46 m/yr (the mean value for the period) with a precision unattained by other methods. 相似文献
8.
Robert L. Michel 《Journal of Hydrology》1992,130(1-4):367-378
The US Geological Survey has maintained a network of stations to collect samples for the measurement of tritium concentrations in precipitation and streamflow since the early 1960s. Tritium data from outflow waters of river basins draining 4500–75000 km2 are used to determine average residence times of water within the basins. The basins studied are the Colorado River above Cisco, Utah; the Kissimmee River above Lake Okeechobee, Florida; the Mississippi River above Anoka, Minnesota; the Neuse River above Streets Ferry Bridge near Vanceboro, North Carolina; the Potomac River above Point of Rocks, Maryland; the Sacramento River above Sacramento, California; the Susquehanna River above Harrisburg, Pennsylvania. The basins are modeled with the assumption that the outflow in the river comes from two sources—prompt (within-year) runoff from precipitation, and flow from the long-term reservoirs of the basin. Tritium concentration in the outflow water of the basin is dependent on three factors: (1) tritium concentration in runoff from the long-term reservoir, which depends on the residence time for the reservoir and historical tritium concentrations in precipitation; (2) tritium concentrations in precipitation (the within-year runoff component); (3) relative contributions of flow from the long-term and within-year components. Predicted tritium concentrations for the outflow water in the river basins were calculated for different residence times and for different relative contributions from the two reservoirs. A box model was used to calculate tritium concentrations in the long-term reservoir. Calculated values of outflow tritium concentrations for the basin were regressed against the measured data to obtain a slope as close as possible to 1. These regressions assumed an intercept of zero and were carried out for different values of residence time and reservoir contribution to maximize the fit of modeled versus actual data for all the above rivers. The final slopes of the fitted regression lines ranged from 0.95 to 1.01 (correlation coefficient > 0.96) for the basins studied. Values for the residence time of waters within the basins and average relative contributions of the within-year and long-term reservoirs to outflow were obtained. Values for river basin residence times ranged from 2 years for the Kissimmee River basin to 20 years for the Potomac River basin. The residence times indicate the time scale in which the basin responds to anthropogenic inputs. The modeled tritium concentrations for the basins also furnish input data for urban and agricultural settings where these river waters are used. 相似文献
9.
Tritium concentrations are used to trace water circulation in the Urumqi and Turfan basins in the Xinjiang, western China. Tritium analyses were made for 77 water samples of river waters, groundwaters, spring waters, lake waters and glacier ice collected in summers in 1992 and 1994. The tritium concentrations in the waters are in a wide range from 0 to 125 TU, most of which are considerably high compared with those of most waters in Japan, because tritium levels in precipitation in the area are over ten times as high as those in Japan. River waters originating in glacier regions contain melt glacier, the proportion of which is over 0.5 to river water. The mean resi-dence time of circulating meteoric water in the mountain regions is estimated to be about 15 years. Most groundwaters and spring waters in the flat regions are mainly derived from river waters originating in glacier regions. The groundwater of greatest tritium concentrations in wells in Urumqi City is derived from Urumqi River about 25 years ago. It takes several ten years for river water to pass the underground to many springs. Some groundwaters and spring waters have taken a long time more than 40 years to travel under the ground. Enrichment of tritium in lake water by evaporation is considered to estimate the contribution of groundwater flow to the recharge of lake. Various contributions of groundwater to lakes are inferred for the various type of salinity in closed or semi-closed lakes. The inflow rates of groundwater to salt lakes are small as against fresh water lakes. 相似文献
10.
The partitioning of rainfall into surface runoff and infiltration influences many other aspects of the hydrologic cycle including evapotranspiration, deep drainage and soil moisture. This partitioning is an instantaneous non-linear process that is strongly dependent on rainfall rate, soil moisture and soil hydraulic properties. Though all rainfall datasets involve some degree of spatial or temporal averaging, it is not understood how this averaging affects simulated partitioning and the land surface water balance across a wide range of soil and climate types. We used a one-dimensional physics-based model of the near-surface unsaturated zone to compare the effects of different rainfall discretization (5-min point-scale; hourly point-scale; hourly 0.125° gridded) on the simulated partitioning of rainfall for many locations across the United States. Coarser temporal resolution rainfall data underpredicted seasonal surface runoff for all soil types except those with very high infiltration capacities (i.e., sand, loamy sand). Soils with intermediate infiltration capacities (i.e., loam, sandy loam) were the most affected, with less than half of the expected surface runoff produced in most soil types when the gridded rainfall dataset was used as input. The impact of averaging on the water balance was less extreme but non-negligible, with the hourly point-scale predictions exhibiting median evapotranspiration, drainage and soil moisture values within 10% of those predicted using the higher resolution 5-min rainfall. Water balance impacts were greater using the gridded hourly dataset, with average underpredictions of ET up to 27% in fine-grained soils. The results suggest that “hyperresolution” modelling at continental to global scales may produce inaccurate predictions if there is not parallel effort to produce higher resolution precipitation inputs or sub-grid precipitation parameterizations. 相似文献
11.
Wolfgang Roether 《Earth and Planetary Science Letters》1974,23(1):108-115
Tritium and14C data of the “GOGO I” station at 28.5°N, 121.6°W in November 1971 are reported. The tritium decline between 150 and 350 m depth is as pronounced as was observed on a previous occupation of the same position, station “Geosecs I” in September 1969, and the tritium concentrations below 200 m are unchanged.14C data from the depth range of tritium decline are corrected for fallout14C contribution. The correcting procedure requires simultaneous measurements of14C, ΣCO2, and tritium. It is concluded that the natural absolute14C concentration attains a maximum near 400 m depth, of 7.5% excess over that of surface water. 相似文献
12.
13.
H. GöteÖstlund H. Gorman Dorsey Claës G. Rooth 《Earth and Planetary Science Letters》1974,23(1):69-86
Radiocarbon data for 11 stations and tritium data for 16 stations in the North Atlantic Ocean from 74°N to 3°N are presented. For radiocarbon, normal errors inΔ14C are± 4‰, and in tritium,± 0.09TU or± 3%, whichever is larger. There is a remarkable, but not simply linear, correlation between oceanic bomb transients in14C and3H. The deep convective mixing in the Greenland Sea is reflected in substantial bomb tracer penetration to all depths, with residence time for the deep, cold core water that seems to be 20 to 30 years. The outflow in the bottom layer southward over the sills of the Denmark Strait and Faroe Passage carries significant tritium concentration, at least to 40°N. Complicated, but coherent, profile structures in the subtropical Atlantic suggest effects of large-scale lateral advection. In particular, a pronounced minimum in both14C and3H might be associated with the Antarctic intermediate water. 相似文献
14.
Evapotranspiration (ET) is the largest term after precipitation in terrestrial water budgets. Accurate estimates of ET are
needed for numerous agricultural and natural resource management tasks and to project changes in hydrological cycles due to
potential climate change. We explore recent methods that combine vegetation indices (VI) from satellites with ground measurements
of actual ET (ETa) and meteorological data to project ETa over a wide range of biome types and scales of measurement, from local to global estimates. The majority of these use time-series
imagery from the Moderate Resolution Imaging Spectrometer on the Terra satellite to project ET over seasons and years. The
review explores the theoretical basis for the methods, the types of ancillary data needed, and their accuracy and limitations.
Coefficients of determination between modeled ETa and measured ETa are in the range of 0.45–0.95, and root mean square errors are in the range of 10–30% of mean ETa values across biomes, similar to methods that use thermal infrared bands to estimate ETa and within the range of accuracy of the ground measurements by which they are calibrated or validated. The advent of frequent-return
satellites such as Terra and planed replacement platforms, and the increasing number of moisture and carbon flux tower sites
over the globe, have made these methods feasible. Examples of operational algorithms for ET in agricultural and natural ecosystems
are presented. The goal of the review is to enable potential end-users from different disciplines to adapt these methods to
new applications that require spatially-distributed ET estimates. 相似文献
15.
Gudrun Massmann Jürgen Sültenfuß Uwe Dünnbier Andrea Knappe Thomas Taute Asaf Pekdeger 《水文研究》2008,22(6):788-801
Berlin relies on induced bank filtration from a broad‐scale, lake‐type surface water system. Because the surface water contains treated sewage, wastewater residues are present in surface water and groundwater. Multiple environmental tracers, including tritium and helium isotopes (3H, 3He, 4He), stable isotopes (δ18O and δ2H) and a number of persistent sewage indicators, such as chloride, boron and a selection of pharmaceutical residues (phenazone‐type analgesics and their metabolites, carbamazepine and anthropogenic gadolinium, Gdexcess), were used to estimate travel times from the surface water to individual production and observation wells at two sites. The study revealed a strong vertical age stratification throughout the upper aquifer, with travel times varying from a few months to several decades in greater depth. Whereas the shallow bank filtrate is characterized by the reflection of the time‐variant tracer input concentrations and young 3H/3He ages, the deeper, older bank filtrate displays no tracer seasonality, 3H/3He ages of a few years to decades and strongly deviating concentrations of several pharmaceutical residues, reflecting concentrations of the source surface water over time. The phenazone‐type pharmaceuticals persist in the aquatic environments for decades. Bank filtration in Berlin is only possible at the sandy lakeshores. In greater water depth, impermeable lacustrine sapropels inhibit infiltration. The young bank filtrate originates from the nearest shore, whereas the older bank filtrate infiltrates at more distant shores. This paper illustrates the importance of using multiple tracer methods, capable of resolving a broad range of residence times, to gain a comprehensive understanding of time‐scales and infiltration characteristics in a bank filtration system. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
16.
Tritium in the Arctic Ocean and East Greenland Current 总被引：1，自引：0，他引：1
High concentrations of tritium are found in the surface water of the Arctic Ocean (up to 50 TU) and in the East Greenland Current (up to 70 TU). These high tritium values are a direct result of atmospheric testing of nuclear weapons in the early 1960's. A box model with a time-dependent input of highly tritiated precipitation predicts that high tritium concentrations are to be expected in the surface layer of the Arctic Ocean and its various outflows. We suggest that a few tritium stations in the Arctic Ocean would provide a powerful analytical tool for assigning time scales to exchange processes. 相似文献
17.
Mean annual rates of tritium input into the ocean averaged over 5° latitude bands are presented for the major oceans, for the period 1952–1975. The rates are obtained by converting tritium concentrations in marine precipitation into net oceanic tritium input, by means of a hydrological model. The tropospheric tritium pattern is specified on the basis of available observations, and climatological means from the literature are used for the rates of evaporation and precipitation and for the relative humidity in ship's height, that enter the model. Tritium input by water vapor exchange exceeds that by precipitation about three-fold. Tritium input by river runoff and by net tropospheric tritium outflow from the continents is also accounted for. This contribution is small except for the northern Indian Ocean and the North Atlantic.The inputs have hemispheric maxima near 50° latitude. The northern hemisphere inputs were strongly peaked in 1963–1964, whereas temporal changes in the southern hemisphere were much more gradual. By 1972, about 75% of the total oceanic input had been received by the northern ocean. For the Pacific, the computed total input agrees with the actual tritium inventory within the limits of uncertainty (about ±20%). The global tritium inventory is estimated at 1.9 GCi in 1972, which corresponds to an average tritium yield of 0.9 kg tritium per megaton TNT equivalent of nuclear fusion. 相似文献
18.
Future use of tritium in mapping pre-bomb groundwater volumes 总被引：2，自引：0，他引：2
The tritium input to groundwater, represented as volume-weighted mean tritium concentrations in precipitation, has been close to constant in Tucson and Albuquerque since 1992, and the decrease in tritium concentrations at the tail end of the bomb tritium pulse has ceased. To determine the future usefulness of tritium measurements in southwestern North America, volume-weighted mean tritium levels in seasonal aggregate precipitation samples have been gathered from 26 sites. The averages range from 2 to 9 tritium units (TU). Tritium concentrations increase with site latitude, and possibly with distance from the coast and with site altitude, reflecting local ratios of combination of low-tritium moisture advected from the oceans with high-tritium moisture originating near the tropopause. Tritium used alone as a tool for mapping aquifer volumes containing only pre-bomb recharge to groundwater will become ambiguous when the tritium in precipitation at the end of the bomb tritium pulse decays to levels close to the analytical detection limit. At such a time, tritium in precipitation from the last one to two decades of the bomb pulse will become indistinguishable from pre-bomb recharge. The threshold of ambiguity has already arrived in coastal areas with a mean of 2 TU in precipitation and will follow in the next three decades throughout the study region. Where the mean tritium level is near 5 TU, the threshold will occur between 2025 and 2030, given a detection limit of 0.6 TU. Similar thresholds of ambiguity, with different local timing possible, apply globally. 相似文献
19.
A modified global model for predicting the tritium concentration in precipitation has been developed using the dataset of International Atomic Energy Agency/the World Meteorological Organization (IAEA/WMO) over the period from 1960 to 2005. The tritium concentration in precipitation and its history can be estimated at any location using the model. The modified global model of tritium in precipitation (MGMTP) here presented has higher accuracy than the global model of tritium in precipitation (GMTP) developed by Doney et al. ( 1992 ). The new model is not only more appropriate for a particular station but also applicable for the un‐normalized observations directly. Another advantage of MGMTP is that it can estimate a longer history (from 1960 to 2005) of tritium content in precipitation than GMTP (from 1960 to 1986). The seasonal cycle of tritium in precipitation has also been modelled in the form of a simple cosine function with five parameters. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
20.
Audrey Douinot Doerthe Tetzlaff Marco Maneta Sylvain Kuppel Hubert Schulte‐Bisping Chris Soulsby 《水文研究》2019,33(16):2174-2191
We used the new process‐based, tracer‐aided ecohydrological model EcH2O‐iso to assess the effects of vegetation cover on water balance partitioning and associated flux ages under temperate deciduous beech forest (F) and grassland (G) at an intensively monitored site in Northern Germany. Unique, multicriteria calibration, based on measured components of energy balance, hydrological function and biomass accumulation, resulted in good simulations reproducing measured soil surface temperatures, soil water content, transpiration, and biomass production. Model results showed the forest “used” more water than the grassland; of 620 mm average annual precipitation, losses were higher through interception (29% under F, 16% for G) and combined soil evaporation and transpiration (59% F, 47% G). Consequently, groundwater (GW) recharge was enhanced under grassland at 37% (~225 mm) of precipitation compared with 12% (~73 mm) for forest. The model tracked the ages of water in different storage compartments and associated fluxes. In shallow soil horizons, the average ages of soil water fluxes and evaporation were similar in both plots (~1.5 months), though transpiration and GW recharge were older under forest (~6 months compared with ~3 months for transpiration, and ~12 months compared with ~10 months for GW). Flux tracking using measured chloride data as a conservative tracer provided independent support for the modelling results, though highlighted effects of uncertainties in forest partitioning of evaporation and transpiration. By tracking storage—flux—age interactions under different land covers, EcH2O‐iso could quantify the effects of vegetation on water partitioning and age distributions. Given the likelihood of drier, warmer summers, such models can help assess the implications of land use for water resource availability to inform debates over building landscape resilience to climate change. Better conceptualization of soil water mixing processes and improved calibration data on leaf area index and root distribution appear obvious respective modelling and data needs for improved simulations. 相似文献