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1.
Wheat straw burning and its associated impacts on Beijing air quality   总被引:18,自引:0,他引:18  
Based on MODIS images, large-scale flow field charts and environmental monitoring data, we thor- oughly analyzed the spatial distribution of wheat straw burning in North China, with focus on its envi- ronmental impacts on the air quality of Beijing and pollution transport paths. And we anatomized changes of air quality in Beijing under the impacts of pollution generated by wheat straw burning around. The results indicate that: (1) The North China Plain, a winter-wheat growing area, is the main source of pollutants induced by wheat straw burning in Beijing. The direction of south-west is the dominant heavy pollution transport path. (2) Impacts of wheat straw burning on air quality are mainly manifested by significantly increasing CO concentration. (3) Precursors of O3 generated by wheat straw burning, combining with favorable meteorological conditions, can induce increasing O3 concentration greatly. NO concentration will be greatly increased due to decreasing O3 concentration at night. (4) Atmospheric particles, especially the fine ones, from wheat straw burning exert considerable influ- ence on Beijing air quality. (5) Different contributions of wheat straw burning to pollutants are identified. Ratios of PM10/SO2, CO/SO2, etc., can be applied to indicate pollution extent of wheat straw burning. High ratios of PM10/SO2 and CO/SO2 show that the air quality was heavily impacted by wheat straw burning and these ratios can be employed as indicators of contribution of wheat straw burning to the degradation of Beijing air quality. (6) Randomness of wheat straw burning activities renders random outbreak of air pollution of this type. Regional and extensive wheat straw burning activities can cause serious air pollution event.  相似文献   

2.
Multiple cities in a diveloped economic area may consist of a city cluster,and the difusion and mixing of its pollutants result in the effect of pollutants plume between cities and the large-scale regional pollution diffusion phenomenon.The distant transfer and diffusion of pollutants occurs when massive aerosols are affected by the dynamic porcess of large-scale circulations.Research suggesten that the life span of aerosol particles whose diameters are about 1 um is the longest.The longevity …  相似文献   

3.
— The CSIRO Division of Atmospheric Research limited area model (DARLAM) is applied to atmospheric transport modeling of haze in southeast Asia. The 1998 haze episode is simulated using an emission inventory derived from hotspot information and adopting removal processes based on SO2.¶Results show that the model is able to simulate the transport of haze in the region. The model images closely resemble the plumes of NASA Total Ozone Mapping Spectrometer and Meteorological Service Singapore haze maps. Despite the limitation of input data, particularly for haze emissions, the three-month average pattern correlation obtained for the whole episode is 0.61. The model has also been able to reproduce the general features of transboundary air pollution over a long period of time. Predicted total particulate matter concentration also agrees reasonably well with observation.¶The difference in the model results from the satellite images may be attributed to the large uncertainties of emission, simplification of haze deposition and transformation mechanisms and the relatively coarse horizontal and vertical resolution adopted for this particular simulation.  相似文献   

4.
This paper illustrates the use of statistical techniques to standardize ground based measurements of particulate matter (PM10). Concentrations are interpolated over Western Europe using uncertain secondary information from a chemical transport model and of aerosol optical thickness from MODIS satellite observations. A consistent overview of PM10 concentrations over Europe based solely on ground based measurements is complicated by differences between countries. Different monitoring methods are used and calibrations are applied. There also is an inherent limitation to the spatial representativeness of ground based measurements. Validation showed that adding secondary information from either the chemical transport model or the satellite observations improved the PM10 mapping. The URMSE decreased from 5.14 to 4.26 and 4.58, respectively. A combination of both sources of secondary information gave the most accurate and precise predictions, with an URMSE of 3.62. This means that both external sources contain additional information on the spatial distribution of PM10 concentrations and should therefore be preferred.  相似文献   

5.
应用环境磁学方法研究了2008年奥运会前后北京市朝阳区大气降尘及对照点表土样品的磁学特征.结果表明,所有样品中载磁矿物主要为低矫顽力的亚铁磁性矿物(主要为磁铁矿).但大气降尘样品的磁性颗粒粒度较表土偏粗;磁性矿物含量高于表土样品,大气降尘除来自于自然源外,更多为来自于人为因素的结果.大气降尘磁化率与空气污染物浓度随时间...  相似文献   

6.
城市热岛效应和气溶胶浓度的动力、热力学分析   总被引:4,自引:0,他引:4       下载免费PDF全文
在能量平衡方程中引入气溶胶的吸收和散射作用,并与三维行星边界层运动方程组相耦合,根据温度分布显式求解运动场,探讨三维行星边界层内温度、运动、气溶胶浓度分布特征.结果表明,城市人为热释放直接决定了城市热岛效应的强度,城市面积越大,城市热岛效应的强度也越强,城市面积固定时,城市越分散,城市热岛效应的强度越弱,这为城市建设多采取卫星城的方式提供了一定的理论支撑.气溶胶的散射作用要大于吸收作用,其对城市热岛效应的强度主要起削弱作用,当气溶胶浓度较大时,吸收作用更显著一些,此时城市热岛效应的强度会有一定的增强,但是幅度不大.当城市热岛效应的强度增强时,其所驱动的环流也会增强,造成城区中心气溶胶浓度略有下降.  相似文献   

7.
Like other Asian countries, Pakistan is facing the issue of air pollution due to rapid urbanization, enormous transportation increases, and other related human activities. Moreover, continuously increasing emission sources have not only raised pollutant concentrations but also their types, thus damaging both human health and the environment. Faisalabad is the third largest megacity of Pakistan and its state of air quality is getting worse due to factors such as industrialization, high traffic volumes, and extensive fossil‐fuel‐burning activities. This review article aims to highlight the present status of air pollution in this city with special reference to particulate matter, elemental profiles, gaseous pollutants, organic–inorganic particulate contents as well as their sources. The concentration levels of these entities were also compared with other national and international cities, and related environmental standards. It is found that current levels of these pollutants are beyond safety limits as specified by various environment protection agencies and organizations. Several weak aspects and gaps are also identified along with suggestions for improvements of the present situation and directions for future research.  相似文献   

8.
Despite the existing public and government measures for monitoring and control of air quality in Bulgaria, in many regions, including typical and most numerous small towns, air quality is not satisfactory. In this paper, factor analysis and Box–Jenkins methodology are applied to examine concentrations of primary air pollutants such as NO, NO2, NOx, PM10, SO2 and ground level O3 in the town of Blagoevgrad, Bulgaria within a 1 year period from 1st September 2011 to 31st August 2012, based on hourly measurements. By using factor analysis with PCA and Promax rotation, a high multicollinearity between the six pollutants has been detected. The pollutants were grouped in three factors and the degree of contribution of the factors to the overall pollution was determined. This was interpreted as the presence of common sources of pollution. The main part of the study involves the performance of time series analysis and the development of univariate stochastic seasonal autoregressive integrated moving average (ARIMA) models with recording on a hourly basis as seasonality. The study also incorporates the Yeo–Johnson power transformation for variance stabilizing of the data and model selection by using Bayersian information criterion. The obtained SARIMA models demonstrated very good fitting performance with regard to the observed air pollutants and short-term predictions for 72 h ahead, in particular in the case of ozone and particulate matter PM10. The presented statistical approaches allow the building of non-complex models, effective for short-term air pollution forecasting and useful for advance warning purposes in urban areas.  相似文献   

9.
The spatial structure and multi-scale feature of the atmospheric pollution influence domain of Beijing and its peripheral areas (a rapidly developed city agglomeration) is dissected and analyzed in this paper on the basis of the atmospheric pollution dynamic-chemical process observation data of the urban building ensemble boundary layer of the Beijing City Air Pollution Observation Experiment (BECAPEX) in winter (February) and summer (August) 2003, and relevant meteorological elements and satellite retrieval aerosol optical depth (AOD), etc. comprehensive data with the dynamic-statistical integrated analysis of "point-surface" spatial structure. Results show that there existed significant difference in the contribution of winter/summer different pollution emission sources to the component character of atmospheric pollution, and the principal component analysis (PCA) results of statistical model also indicate that SO2 and NOX dominated in the component structure of winter aerosol particle; instead, CO and NOX dominated in summer. Surface layer atmospheric dynamic and thermal structures and various pollutant species at the upper boundary of building ensembles at urban different observational sites of Beijing in winter and summer showed an "in-phase" variation and its spatial scale feature of "influence domain". The power spectrum analysis (PSA) shows that the period spectrum of winter/summer particle concentration accorded with those of atmospheric wind field: the longer period was dominative in winter, but the shorter period in summer, revealing the impact of the seasonal scale feature of winter/summer atmospheric general circulation on the period of atmospheric pollution variations. It is found that from analyzing urban area thermal heterogeneity that the multiscale effect of Beijing region urban heat island (UHI) was associated with the heterogeneous expansion of tall buildings area. In urban atmospheric dynamical and thermal characteristic spatial structures, the turbulent scale feature of the urban boundary layer (UBL) of architectural complexes had important impact on the multi-scale feature of urban atmospheric pollution. The comprehensive analyses of the variational analysis field of Moderate Resolution Imaging Spectroradiometer (MODIS) AOD-surface PM10 under the condition of clear sky and the correlation resultant wind vector field for pollution source-tracing suggest that the emission sources for winter Beijing atmospheric pollution aerosols particle might be remotely traced to the south peripheral greater-scale spatial range of Hebei, Shandong, Tianjin, etc., and the spatial distribution of the high value area of AOD was associated with that of the high value area of resident family number (heating surface source). The backward trajectory feature of winter/ summer air particles exhibits analogous multi-scale feature, and depicts the difference in the scale feature of the pollution sources spatial distribution in different seasons. The peripheral source trajectory paths of urban atmospheric pollution (UAP) mainly come from the fixed industrial surface source or heating surface source in the outskirt of Beijing, and the diffusion and transport distance of peripheral sources in winter is larger than one in summer. The above conclusions depict the multi-scale spatial influence domain and seasonal features caused by UAP source influence and atmospheric dynamical structure. The high value area of the winter Total Ozone Mapping Spectrometer (TOMS) AOD lay in the Beijing region and its south peripheral area, an S-N zonal pattern, which reflects the dynamical effect of peripheral topographic pattern on the diffusion of regional scale atmospheric pollution sources. Study suggests that the extent of winter atmospheric pollution within the "valley" megarelief in Beijing and periphery was close related with the pollution emission sources of the south peripheral area; and the significant "anti-phase" variation feature of winter AOD and sunshine duration in Beijing and its peripheral areas, and regional scale correlation of low cloud cover, fog days, and aerosols reflects the local climatic effect of aerosol influence in this region. Besides, analysis of the impacts of atmospheric dry/wet deposition distributions within a valley-scale on the regional water body of Miyun reservoir also reveals the possible influence of the multi-scale spatial structure of summer water, soil and atmospheric pollution sources on the water quality of Miyun reservoir.  相似文献   

10.
VIIRS(Visible Infrared Imaging Radiometer Suite)作为MODIS(The MODerate resolution Imaging Spectroradiometer)的后继传感器,可在全球范围内实现对气溶胶的连续时空监测.卫星反演的气溶胶光学厚度(Aerosol Optical Depth,AOD)是研究地球能量收支平衡、气候效应和空气质量的重要大气参数.但在中国重污染天气情况下,现有的VIIRS陆地气溶胶产品存在一定不足.因此,本研究改进云识别方法,优化像元筛选,约束气溶胶类型选择,实现重污染情况下AOD的反演.基于地基AERONET(AErosol RObotic NETwork)的验证结果表明,相比NOAA(National Oceanic and Atmospheric Administration)产品,改进后的反演结果克服了反演值偏低的问题,且表现出更好的相关性,RMSE从0.236下降到0.219.为验证在重污染条件下改进算法的适用性和准确性,本文对比了两种污染条件下的反演结果(0.61).统计结果表明,在较重污染天气条件下(AODAERONET>1),相比NOAA的AOD产品,本文结果的反演率从32.3%提升为68.8%,回归分析的斜率提高为0.80,相关系数达到0.76,均方根误差为0.307,在增加反演量的同时保证了反演的精度.  相似文献   

11.
Based on analysis of the air pollution observational data at 8 observation sites in Beijing including outer suburbs during the period from September 2004 to March 2005, this paper reveals synchronal and in-phase characteristics in the spatial and temporal variation of air pollutants on a city-proper scale at deferent sites; describes seasonal differences of the pollutant emission influence between the heating and non-heating periods, also significantly local differences of the pollutant emission influence between the urban district and outer suburbs, i.e. the spatial and temporal distribution of air pollutant is closely related with that of the pollutant emission intensity. This study shows that due to complexity of the spatial and temporal distribution of pollution emission sources, the new generation Community Multi-scale Air Quality (CMAQ) model developed by the EPA of USA produced forecasts, as other models did, with a systematic error of significantly lower than observations, albeit the model has better capability than previous models had in predicting the spatial distribution and variation tendency of multi-sort pollutants. The reason might be that the CMAQ adopts average amount of pollutant emission inventory, so that the model is difficult to objectively and finely describe the distribution and variation of pollution emission sources intensity on different spatial and temporal scales in the areas, in which the pollution is to be forecast. In order to correct the systematic prediction error resulting from the average pollutant emission inventory in CMAQ, this study proposes a new way of combining dynamics and statistics and establishes a statistically correcting model CMAQ-MOS for forecasts of regional air quality by utilizing the relationship of CMAQ outputs with corresponding observations, and tests the forecast capability. The investigation of experiments presents that CMAQ-MOS reduces the systematic errors of CMAQ because of the uncertainty of pollution emission inventory and improves the forecast level of air quality. Also this work employed a way of combining point and area forecasting, i.e. taking the products of CMAQ for a center site to forecast air pollution for other sites in vicinity with the scheme of model products "reanalysis" and average over the "area".  相似文献   

12.
In the assessment of air quality, regional distribution and dispersion with distance are important, together with the variations of pollutants in time. On this occasion, the point cumulative semi-variogram (PCSV) method is used in order to find simply regional distribution of pollutants of Erzurum urban centre. This method is based simply on the summation of square differences in air pollutant concentrations between different sites. Monthly regional variation maps of Erzurum are constructed by finding radius of influence (for SO2, from 1000 m to 3500 m and, for TSP, 1000–2000 m) and PCSV scattering diagram data at different levels by using monthly average sulphur dioxide (SO2) and total suspended particulate (TSP) matter concentrations in 2001–2002 winter season. Consequently, the air pollution distribution of Erzurum is assessed.  相似文献   

13.
近年来水体富营养化呈扩张趋势,蓝藻水华不仅在太湖等大型湖泊频发,水面面积较小的天津于桥水库等也形势严峻,亟需加强卫星遥感监测.但是,以往在太湖等业务化使用非常成功的MODIS等卫星数据(约500 m),由于空间分辨率较低,难以满足小型水体的监测要求;而Landsat-8等空间分辨率较高的卫星数据(30 m),通常重返周期较长,无法满足水华高频监测需求.本文以天津市于桥水库(面积约80 km2)为研究区,针对常用的卫星数据,从空间、时间、光谱范围和数据可获取性共4个方面,评价不同卫星数据蓝藻水华监测能力和算法,同时对不同卫星监测结果一致性进行评估.结果表明:(1)筛选出国产HJ-1A\B CCD、GF-1 WFV和美国Landsat-8 OLI这3种卫星波段合适,空间分辨率较高,适用于桥水库蓝藻水华监测,但考虑到其重返周期较长,建议多星联合观测;(2)各个卫星监测结果与卫星影像目视解译结果基本一致,均方根误差和相对误差均分别控制在0.78 km2和4.9%以内;(3)不同卫星监测结果一致性良好,一致性精度达到99.5%;(4)根据历史影像结果,发现于桥水库2016年水质开始呈富营养化,藻华现象在夏、秋两季最为严重.研究表明,针对小型水面水体蓝藻水华监测,利用较高分辨率数据联合监测,是一种有效的替代策略,今后可在更多小型水域推广.  相似文献   

14.
Characteristics of observed trace gaseous pollutants in the Yangtze Delta   总被引:3,自引:1,他引:2  
The significant impacts on air quality and natural resources, such as land and forest, have taken place in Yangtze Delta in the last two decades, resulting from rapidly economic develop-ment in this region. The Yangtze Delta contains many cities and towns…  相似文献   

15.
The Multiangle Imaging SpectroRadiometer (MISR) launched by NASA in late 1999 has a unique multiangle design, which points nine cameras at fixed angles along the satellite flight track and collects reflected solar radiation simultaneously. This design allows the retrieval of a rich dataset of particle abundance, shape and composition over both land and ocean. Some of its capabilities have not been seen by any currently operating satellite aerosol sensors. Since MISR is sensitive to fine particles, it provides a new data source to study the spatial and temporal characteristics of air quality over large geographical regions. We first briefly introduce the MISR instrument, the retrieval and structure of MISR aerosol data, and then review the applications of MISR aerosol data in various aspects of air quality research since its launch. These include the spatial distributions of particle pollution events such as dust storms, wild fires, and urban pollution. Because of the high quality of MISR aerosol data, they can be used as quantitative indicators of particle pollution levels. We review the current modeling studies of surface level particle concentrations. Next, we introduce research results using MISR’s advanced data such as the plume heights, and particle microphysical properties. In the discussion, we compare MISR research with current MODIS research to the best of our ability as MODIS data have been more extensively explored by the Chinese scientific community. Finally, we summarize the advantages and disadvantages of MISR data related to its applications to the air quality research. Given the highly quantitative measurements and comprehensive aerosol information MISR can provide, we believe that it will provide great values to advance our understanding of the particle air pollution in China. Supported by Harvard-EPA Center on Particle Health Effects (Grant Nos. R-827353 and R-832416), NASA’s Climate and Radiation Research and Analysis Program, the EOS-MISR Instrument Project and the National High Technology Research and Development Program of China (Grant No. 2006AA06A305).  相似文献   

16.
施晓晖  徐祥德 《地球物理学报》2012,55(10):3230-3239
针对2011年12月初北京及华北持续近一周的严重大雾天气这一热点事件,从城市群大雾过程气溶胶区域影响的视角,基于"973"项目"北京及周边地区大气-水-土环境污染机理与调控原理"的研究工作,就北京及周边地区大雾天气与大气气溶胶区域影响的关系等方面进行了讨论.研究表明,北京城市大雾前低空SO2和NO2浓度存在"积聚"与"突增"现象.北京及周边地区冬季雾日数和气溶胶光学厚度则呈正相关,并具有"同位相"的年际变化趋势.研究同时发现北京及其南部周边的冬季气溶胶高值区呈南北向带状分布,其与北京周边居民户数高值区有所吻合,反映了冬季北京城市气溶胶颗粒物的远距离影响源区及大尺度输送效应.统计分析指出,冬季北京气溶胶颗粒物PM10、PM2.5主要影响成分是SO2和NOX,且有关研究也表明,电厂、采暖和工业面源是SO2的三大本地排放源,而机动车、电厂、工业为NOX的三大本地排放源,上述大气PM10、PM2.5主成分污染源亦与雾水样本化学分析结果相吻合,即冬季由于燃煤在生活能源中的比例较大,北京雾水中硫元素和碳元素的含量都较高.因此,北京冬季大雾不仅与北京城区气溶胶及其污染排放影响存在相关关系,而且与北京周边天津、河北、山东等地气溶胶及大气污染物的远距离输送和气溶胶区域影响效应有着重要的联系.因此,北京雾霾天气及相关大气污染的治理工作首先要着眼于局地污染物的减排,但同时如何做好区域大气污染的协同治理也是不容忽视的问题.  相似文献   

17.
Riverine freshwater plumes are the major transport mechanism for nutrients, sediments and pollutants into the Great Barrier Reef (GBR) lagoon and connect the land with the receiving coastal and marine waters. Knowledge of the variability of the freshwater extent into the GBR lagoon is relevant for marine park management to develop strategies for improving ecosystem health and risk assessments. In this study, freshwater extent has been estimated for the entire GBR lagoon area from daily satellite observations of the Moderate Resolution Imaging Spectroradiometer (MODIS) between 2002 and 2010. To enable a reliable mapping of freshwater plumes we applied a physics-based coastal ocean colour algorithm, that simultaneously retrieves chlorophyll-a, non-algal particulate matter and coloured dissolved organic matter (CDOM), from which we used CDOM as a surrogate for salinity (S) for mapping the freshwater extent.  相似文献   

18.
We simulated geostationary satellite observations to assess the potential for high spatial-and temporal-resolution monitoring of air pollution in China with a focus on tropospheric ozone(O_3), nitrogen dioxide(NO_2), sulfur dioxide(SO_2), and formaldehyde(HCHO). Based on the capabilities and parameters of the payloads onboard sun-synchronous satellites, we simulated the observed spectrum based on a radiative transfer model using a geostationary satellite model. According to optimal estimation theory, we analyzed the sensitivities and retrieval uncertainties of the main parameters of the instrument for the target trace gases. Considering the retrieval error requirements of each trace gas, we determined the major instrument parameter values(e.g., observation channel, spectral resolution, and signal-to-noise ratio). To evaluate these values, retrieval simulation was performed based on the three-dimensional distribution of the atmospheric components over China using an atmospheric chemical transportation model. As many as 90% of the experiments met the retrieval requirements for all target gases. The retrieval precision of total-column and stratospheric O_3 was 2%. In addition, effective retrieval of all trace gases could be achieved at solar zenith angles larger than 70°. Therefore, the geostationary satellite observation and instrument parameters provided herein can be used in air pollution monitoring in China. This study offers a theoretical basis and simulation tool for improving the design of instruments onboard geostationary satellites.  相似文献   

19.
Coarse-resolution satellite albedo products are important for climate change and energy balance research because of their capability to characterize the spatiotemporal patterns of land surface parameters at both the regional and global scales. The accuracy of coarse-resolution products is usually assessed via comparison with in situ measurements. The key issue in the comparison of remote sensing observations with in situ measurements is scaling and uncertainty. This paper presents a strategy for validating 1-km-resolution remote sensing albedo products using field measurements and high-resolution remote sensing observations. Field measurements were collected to calibrate the high-resolution(30 m) albedo products derived from HJ-1a/b images. Then, the calibrated high-resolution albedo maps were resampled(i.e., upscaled) to assess the accuracy of the coarse-resolution albedo products. The samples of field measurements and high-resolution pixels are based on an uncertainty analysis. Two types of coarse-resolution albedo datasets, from global land surface satellite(GLASS) and moderate-resolution imaging spectroradiometer(MODIS), are validated over the middle reaches of the Heihe River in China. The results indicate that the upscaled HJ(Huan Jing means environment in Chinese and this refers to a satellite constellation designed for environment and disaster monitoring by China) albedo, which was calibrated using field measurements, can provide accurate reference values for validating coarse-resolution satellite albedo products. However, the uncertainties in the upscaled HJ albedo should be estimated, and pixels with large uncertainties should be excluded from the validation process.  相似文献   

20.
— To examine the spatial scales associated with atmospheric pollutants such as ozone (O3) and fine particulate matter (PM2.5), we employ the following five techniques: (1) Analysis of the persistence of high O3 concentrations aloft; (2) spatial and lag correlations between the short-term components (i.e., weather-induced variations) in the time series of O3 and PM2.5 throughout the eastern United States; (3) analysis of mixed-layer forward trajectories compiled at different locations on a climatological basis to identify the potential region covered in 1-day of atmospheric transport; (4) analysis of three-dimensional Lagrangian trajectories of tracer particles for three high-O3 episode events in the summer of 1995; and (5) analysis of the spatial extent over which emissions have an impact through photochemical model simulations. Regardless of the method chosen, the results demonstrate that pollutants such as O3 and PM2.5 have the potential to affect regions having spatial scales of several hundred kilometers. This finding has implications to regulatory policies for addressing the pollution problem, and for optimally designing monitoring networks for such pollutants.  相似文献   

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