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1.
Sungkyun SHIN Young Min NOH Kwonho LEE Hanlim LEE Detlef MLLER Y.J.KIM Kwanchul KIM Dongho SHIN 《大气科学进展》2014,31(6):1417-1426
The vertical distribution of single scattering albedos （SSAs） of Asian dust mixed with pollutants was derived using the multi-wavelength Raman lidar observation system at Gwangju （35.10°N,126.53°E）.Vertical profiles of both backscatter and extinction coefficients for dust and non-dust aerosols were extracted from a mixed Asian dust plume using the depolarization ratio from lidar observations.Vertical profiles of backscatter and extinction coefficients of non-dust particles were input into an inversion algorithm to retrieve the SSAs of non-dust aerosols.Atmospheric aerosol layers at different heights had different light-absorbing characteristics.The SSAs of non-dust particles at each height varied with aerosol type,which was either urban/industrial pollutants from China transported over long distances at high altitude,or regional/local pollutants from the Korean peninsula.Taking advantage of independent profiles of SSAs of non-dust particles,vertical profiles of SSAs of Asian dust mixed with pollutants were estimated for the first time,with a new approach suggested in this study using an empirical determination of the SSA of pure dust.The SSAs of the Asian dust-pollutants mixture within the planetary boundary layer （PBL） were in the range 0.88-0.91,while the values above the PBL were in the range 0.76-0.87,with a very low mean value of 0.76 ± 0.05.The total mixed dust plume SSAs in each aerosol layer were integrated over height for comparison with results from the Aerosol Robotics Network （AERONET） measurements.Values of SSA retrieved from lidar observations of 0.92 ± 0.01 were in good agreement with the results from AERONET measurements. 相似文献
2.
干旱区一次春季沙尘过程的大气气溶胶垂直分布结构及其特征 总被引：2，自引：0，他引：2
采用微脉冲激光雷达(Micro-Pulse Lidar,MPL)对干旱荒漠代表站张掖站上空一次春季沙尘暴过程的边界层和自由大气的气溶胶分布和大气环境进行了观测。结果表明,气溶胶的垂直廓线可分为高、中、低3层,高层气溶胶出现在5～9km,主要是通过上风方向的高海拔区域或低层气溶胶通过对流等过程突破边界层顶进入自由大气输送而来,其分布高度在一天中随着时间的推移逐渐降低;中层气溶胶位于2.5～4.5km,其消光特性随高度的增加没有明显的变化,具有垂直混合现象;低层气溶胶在2.5km以下,其消光特性随着高度增加反而降低;中、低层气溶胶主要来源于外部源区或当地沙尘源区和沙壤土起沙。气溶胶垂直分布表现出3种形式:在大气稳定条件下,气溶胶随高度增加呈单峰型减小趋势;不稳定条件下随高度增加指数型降低;混合层中随高度增加而保持稳定。由于受边界层日变化的影响,气溶胶分布的上界出现单峰型日变化特征,具体表现为下午较高,早晨较低。 相似文献
3.
4.
In many atmospheric flows, a dispersed phase is actively suspended by turbulence, whose competition with gravitational settling ultimately dictates its vertical distribution. Examples of dispersed phases include snow, sea-spray droplets, dust, or sand, where individual elements of much larger density than the surrounding air are carried by turbulent motions after emission from the surface. In cases where the particle is assumed to deviate from local fluid motions only by its gravitational settling (i.e., they are inertialess), traditional flux balances predict a power-law dependence of particle concentration with height. It is unclear, however, how particle inertia influences this relationship, and this question is the focus of this work. Direct numerical simulations are conducted of turbulent open-channel flow, laden with Lagrangian particles of specified inertia; in this way the study focuses on the turbulent transport which occurs in the lowest few meters of the planetary boundary layer, in regions critical for connecting emission fluxes to the fluxes felt by the full-scale boundary layer. Simulations over a wide range of particle Stokes number, while holding the dimensionless settling velocity constant, are performed to understand the role of particle inertia on vertical dispersion. It is found that particles deviate from their inertialess behaviour in ways that are not easily captured by traditional theory; concentrations are reduced with increasing Stokes number. Furthermore, a similarity-based eddy diffusivity for particle concentration fails as particles experience inertial acceleration, precluding a closed-form solution for particle concentration as in the case of inertialess particles. The primary consequence of this result is that typical flux parametrizations connecting surface emission models (e.g., saltation models or sea-spray generation functions) to elevated boundary conditions may overestimate particle concentrations due to the reduced vertical transport caused by inertia in between; likewise particle emission may be underestimated if inferred from concentration measurements aloft. 相似文献
5.
We present a microphysical model for the surface layer marine and coastal atmospheric aerosols that is based on long-term observations of size distributions for 0.01–100 µm particles. The fundamental feature of the model is a parameterization of amplitudes and widths for aerosol modes of the aerosol size distribution function (ASDF) as functions of fetch and wind speed. The shape of ASDF and its dependence on meteorological parameters, height above sea level (H), fetch (X), wind speed (U) and relative humidity (RH), are investigated. At present, the model covers the ranges H = 0–25 m, U?=?3–18 km s?1, X?≤?120 km and RH?=?40–98%. The latest version of the Marine Aerosol Extinction Profiles model (MaexPro) is described and applied to the computation and analysis of the spectral profiles of aerosol extinction coefficients α(λ) in the wavelength band λ?=?0.2–12 µm. MaexPro is based on the aforementioned aerosol model assuming spherically shaped aerosol particles and the well-known Mie theory. The spectral profiles of α(λ) calculated by MaexPro are in good agreement with observational data and the numerical results obtained from the Navy Aerosol Model (NAM) and the Advanced Navy Aerosol Model (ANAM). Moreover, MaexPro was found to be an accurate and reliable tool for investigating the optical properties of atmospheric aerosols. 相似文献
6.
Ｉ．ＩＮＴＲＯＤＵＣＴＩＯＮＡｅｒｏｓｏｌｃｏｍｐｏｓｉｔｉｏｎｉｓａｐｉｅｃｅｏｆｉｍｐｏｒｔａｎｔｉｎｆｏｒｍａｔｉｏｎｆｏｒｒａｄｉａｔｉｏｎｔｒａｎｓｆｅｒ．Ｔｗｏｐａｒａｍｅｔｅｒｓ,ｎａｒｎｅｌｙ,ｔｏｔａｌｌｏａｄｉｎｇａｎｄｃｈｅｍｉ... 相似文献
7.
Aerosol samples, collected daily were analyzed with electron microscopy for particle concentration and size distribution. The chemical compositions of individual particles were determined with X-ray energy spectrometry and specific morphological tests. The results demonstrated clear and significant dependencies of aerosol properties on air trajectories computed from a backtrack model. Air parcels, such as American air pollution and Sahara dust, were identified. Their physical mixing and chemical reactions with marine aerosols as well as aerosol wet deposition are discussed. 相似文献
8.
This study conducted meteorological simulations in northern Colombia by analyzing different planetary boundary layer (PBL) schemes available in the numerical Weather Research and Forecasting (WRF) model. The study area included three nested domains with horizontal resolutions of 18 km, 6 km, and 2 km, with 38 vertical levels. The evolution and structure of the PBL were analyzed during the driest months (March, April, and May 2016) and in regions with the highest particulate matter concentrations. Sensitivity analysis of the WRF model was performed with two local and two non-local PBL schemes. The results were validated using observations of the surface air temperature, relative humidity, and surface wind speed collected from three meteorological stations in the area. The PBL heights were experimentally determined using radiosonde data provided by a station located in the center of the study area. Variations in PBL heights were estimated using linear regression methods and minimization of statistical errors for the bulk Richardson number, as well as analysis of vertical temperature and wind profiles. The WRF model reliably reproduced the daily values and diurnal cycles of temperature, relative humidity, and wind speed within the PBL and accounted for the influence of topography and sea breezes. Horizontal heat advection dominates the upwelling of air masses when sea breezes are active. The onshore wind direction starts to change from east to northwest, implying a decay in the land breeze regime. All schemes overestimate the mixing height and tend to underestimate surface air temperature values at night. All show wetter conditions and underestimate wind speed. Although the non-local Yonsei University (YSU) scheme shows the best performance, it also shows the largest sources of errors when determining the behavior of the surface layer during stable conditions. Relative humidity and wind speed estimates provided by the local Mellor‐Yamada‐Nakanishi‐Niino (MYNN) scheme were closer to those recorded at the meteorological stations. 相似文献
9.
选用2007年1月8—30日期间8个无云天的激光雷达资料进行分析。基于Fernald方法反演得到气溶胶消光系数廓线,结合无线电探空资料分析了边界层内气溶胶时空分布,并将反演的激光雷达最低观测高度处(180 m)的气溶胶消光系数与地面PM10、能见度资料进行对比分析。结果表明：冬季大连市区气溶胶主要分布在2 km以下区域,早晨和夜间在0.5 km以下区域经常存在一个气溶胶层;气溶胶消光系数廓线与探空资料较吻合;反演激光雷达最低观测高度处(180 m)的气溶胶消光系数与地面的PM10浓度呈正相关,与能见度呈负相关,相关性较好。 相似文献
10.
The importance of specifying realistic lateral boundary conditions in the regional modeling of mineral aerosols has not been examined previously. This study examines the impact of assigning values for mineral aerosol (dust) concentrations at the lateral boundaries of Regional Climate Model version 3 (RegCM3) and its aerosol model over Southwest Asia. Currently, the dust emission module of RegCM3 operates over the interior of the domain, allowing dust to be transported to the boundaries, but neglecting any dust emitted at these points or from outside the domain. To account for possible dust occurring at, or entering from the boundaries, mixing ratios of dust concentrations from a larger domain RegCM3 simulation are specified at the boundaries of a smaller domain over Southwest Asia. The lateral boundary conditions are monthly averaged concentration values (μg of dust per kg of dry air) resolved in the vertical for all four dust bin sizes within RegCM3’s aerosol model. RegCM3 simulations with the aerosol/dust model including lateral boundary conditions for dust are performed for a five year period and compared to model simulations without prescribed dust concentrations at the boundaries. Results indicate that specifying boundary conditions has a significant impact on dust loading across the entire domain over Southwest Asia. More specifically, a nearly 30% increase in aerosol optical depth occurs during the summer months from specifying realistic dust boundary conditions, bringing model results closer to observations such as MISR. In addition, smaller dust particles at the boundaries have a more important impact than large particles in affecting the dust loading within the interior of this domain. Moreover, increases in aerosol optical depth and dust concentrations within the interior domain are not entirely caused by inflow from the boundaries; results indicate that an increase in the gradient of concentration at the boundaries causes an increase of diffusion from the boundaries. Lastly, experiments performed using a climatology of dust concentrations yield similar results to those using actual monthly values. Therefore, using a climatology of dust mixing ratios is sufficient in implementing lateral boundary conditions for mineral aerosols. In short, this work concludes that realistic specification of lateral boundary conditions for mineral aerosols can be important in modeling the dust loading over arid regional climates such as Southwest Asia. 相似文献
11.
The dispersion of heavy particles subjected to a turbulent forcing is often simulated with Lagrangian stochastic models. Although
these models have been employed successfully over land, the implementation of traditional LS models in the marine boundary
layer is significantly more challenging. We present an adaptation of traditional Lagrangian stochastic models to the atmospheric
marine boundary layer with a particular focus on the representation of the scalar turbulence for temperature and humidity.
In this new model, the atmosphere can be stratified and the bottom boundary is represented by a realistic wavy surface that
moves and deforms. Hence, the correlation function for the turbulent flow following a particle is extended to the inhomogenous,
anisotropic case. The results reproduce behaviour for scalar Lagrangian turbulence in a stratified airflow that departs only
slightly from the expected behaviour in isotropic turbulence. When solving for the surface temperature and the radius of evaporating
heavy water droplets in the airflow, the modelled turbulent forcing on the particle also behaves remarkably well. We anticipate
that this model will prove especially useful in the context of sea-spray dispersion and its associated sensible heat, latent
heat, and gas fluxes between spray droplets and the atmosphere. 相似文献
12.
基于飞机和MODIS观测的华北地区气溶胶标高分析 总被引：1，自引：0，他引：1
为研究华北地区的气溶胶分布情况,利用2012—2014年飞机观测资料和MODIS卫星资料,对石家庄等地的气溶胶标高进行了分析。结果表明:(1)与飞机观测资料对比后认为可以利用MODIS光学厚度和常规能见度资料计算气溶胶标高;(2)华北地区春夏季气溶胶标高一般大于秋冬季;6个主要城市中,位于平原地区的城市气溶胶标高较低,西北山区城市标高较高;(3)在不进行飞行探测,仅使用地面资料和卫星资料,通过计算得到气溶胶垂直分布是可行的,尤其是在对流层中层的结果比底层更可信;(4)分别使用观测资料与拟合数据计算光学厚度,分析其误差后,确认在计算光学厚度的过程中可以使用气溶胶数密度指数递减假设。 相似文献
13.
The main goals of this work are climatological analysis of characteristics of vertical wind in the stratosphere and estimation of potential opportunities of its influence on stratospheric aerosol particles. High-altitude, temporal, and latitude dependences of zonal mean vertical wind velocity for the period of 1992?C2006 from the UKMO atmospheric general circulation model are analyzed. It is shown that monthly averaged amplitudes of the vertical wind are approximately ±5?mm/s, while annual averaged ones are ±1?mm/s. The upward wind can provide the vertical lifting against gravity for sufficiently large (up to 3?C5???m) aerosol particles with a density up to 1.0?C1.5?g/cm3 at stratospheric and mesospheric altitudes. The vertical wind, probably, is a substantial factor for particle motion up to altitudes of 30?C40?km and can change essentially the sedimentation velocities and the residence times of stratospheric aerosols. The structure of the averaged fields of vertical wind supposes the opportunity of formation of dynamically stable aerosol layers in the middle stratosphere. With the problem regarding the action of a permanent source of monodisperse particles near the stratopause taken as an example, it is shown that if the action of the averaged vertical component is taken into account along with the gravitational sedimentation and turbulent diffusion, the standard vertical profiles of the relative concentration of particles change cardinally. Estimations for the levitation heights for particles of different densities and sizes in the stratosphere under action of gravity and vertical wind pressure are presented. 相似文献
14.
In this study a moderate-sized alfalfa field was downwind of a large dry region. Measured vertical profiles of temperature, humidity and wind at upwind and downwind sides of the field were used to calculate the short-term evaporation rate, as well as the contribution of horizontally transported or advected heat energy to the evaporation. The vertical profiles must be measured at least to the height at which air is modified by the new surface. In this case that height was as large as 18 m over a several hundred meter long traverse.Evaporation rates calculated by such an approach were in very close agreement to surface fluxes measured by an eddy correlation system near the surface. The difference between calculated and measured values averaged 9.5%. The reduction in sensible heat content of the air of the control volume was substantial during passage over the field. If all this energy was assumed to have been used in evaporation, then the advection of heat contributed from 35 to 86% of the total evaporation rate.It appears that for an inhomogeneous surface, knowledge of the distortion of some properties of local boundary layers can yield reliable estimates of local evaporation. The approach has little empiricism as it is based on simple conservation laws. 相似文献
15.
G. Pavese F. De Tomasi M. Calvello F. Esposito M.R. Perrone 《Atmospheric Research》2009,92(4):489-504
Measurements from July 4 to July 8, 2005 by a high resolution visible radiometer, a Raman lidar, a ground particulate matter sampler, and ground meteorological sensors have been combined in synergy to infer the intrusion over south-east Italy, of air masses from north-west Sahara, the Atlantic Ocean, and the continental Europe. It is shown that backscatter coefficient, depolarization-ratio, and lidar ratio vertical profiles represent the best tools to detect the intrusion of long range transported air masses and to monitor their effects on the vertical distribution of aerosol optical and microphysical properties. High resolution radiometers are instead important tools to monitor changes on columnar aerosol properties and size distributions.Backscatter coefficient, depolarization-ratio, and lidar ratio vertical profiles have revealed that aerosol optical and microphysical properties significantly changed with time and space during African dust outbreaks: the intrusion of dust particles that at first occurred above 2 km of altitude extending up to 6 km, affected the all aerosol load down to ground within few hours. Aerosol size distributions showed during dust events a clear bimodality with an accumulation mode maximum at 0.24 µm and a coarse mode maximum at 0.94 μm. Conversely, we have found that during the advection of air masses from the Atlantic and continental Europe, aerosol particles were mainly located below 2 km, their optical and microphysical properties were affected by smaller changes in time and space, and were characterized by depolarization ratios rather close to those due to a pure molecular atmosphere. In this case bimodal size distributions with an accumulation mode showing two sub-modes at 0.16 μm and 0.24 μm, respectively and a coarse mode centred at 0.94 μm have also been observed. 相似文献
16.
A Lagrangian Stochastic Model for Heavy Particle Dispersion in the Atmospheric Marine Boundary Layer
The dispersion of heavy particles and pollutants is often simulated with Lagrangian stochastic (LS) models. Although these
models have been employed successfully over land, the free surface at the air-sea interface complicates the implementation
of traditional LS models. We present an adaptation of traditional LS models to the atmospheric marine boundary layer (MBL),
where the bottom boundary is represented by a realistic wavy surface that moves and deforms. In addition, the correlation
function for the turbulent flow following a particle is extended to the anisotropic, unsteady case. Our new model reproduces
behaviour for Lagrangian turbulence in a stratified air flow that departs only slightly from the expected behaviour in isotropic
turbulence. When solving for the trajectory of a heavy particle in the air flow, the modelled turbulent forcing on the particle
also behaves remarkably well. For example, the spectrum of the turbulence at the particle location follows that of a massless
particle for time scales approximately larger than the Stokes’ particle response time. We anticipate that this model will
prove especially useful in the context of sea-spray dispersion and its associated momentum, sensible and latent heat, and
gas fluxes between spray droplets and the atmosphere. 相似文献
17.
Stefaan Hoornaert Ricardo Henrique Moreton Godoi René Van Grieken 《Journal of Atmospheric Chemistry》2003,46(3):271-293
In the framework of the 2nd Aerosol Characterization Experiment (ACE-2), in June and July 1997, size segregated samples were collected for single particle analysis on the island of Tenerife, in both the marine boundary layer (MBL) and the free troposphere (FT), to study the characteristics of the North Atlantic aerosol. A systematic assessment was made of the aerosol under background conditions and when the environment was perturbed by European emissions and/or Saharan dust. The aerosol particles were analysed by automated and manual SEM-EDX, followed by cluster analysis to identify the different particle types and their abundance. Basing on back trajectory calculations, particle numbers and volume concentrations, different periods can be identified regarding the origin of the sampled air masses. In the FT, the air masses were classified as clean Atlantic, Saharan dust from Africa or pollution from Europe. In the MBL, air masses were classified as clean, polluted or perturbed by emissions from Europe. For both the FT and MBL samples, the main changes in chemical composition were observed between the fine and coarse mode aerosol. The FT fine mode aerosol is dominated by S-poor aluminosilicates (62%) in the event of the dust samples or sulphates, carbonaceous particles (20%) and S-rich aluminosilicates (46%) in the polluted samples. For the larger fractions, a strong decreasing trend was observed for the sulphates (less than 20%) and carbonaceous particles (10%) in the polluted samples. The MBL fine mode was completely dominated by S-rich particles (polluted 55% and perturbed 59%), and to a lesser extent, carbonaceous and aged sea salt particles. In the coarse mode, the polluted air mass is dominated by sea salt particles (62%). Contrary to the fine fraction, the polluted air mass in the coarse fraction contained 5.3% of S-rich particles. The combined interpretation of the data from the analysis of size-fractioned particles and the calculated backward trajectories for air masses coming from Europe, Africa and the Atlantic, results in better insights on aerosol chemistry, especially for the comparison of the particle composition in the FT and the MBL. 相似文献
18.
秸秆焚烧导致的江苏持续雾霾天气过程分析 总被引：3，自引：2，他引：1
利用常规观测资料和NCEP再分析资料,从污染情况、环流背景、地面气象要素特征、水汽、热力及动力条件等几个方面对江苏2012年6月中上旬持续雾霾天气进行了分析。结果表明:江苏及周边省市秸秆焚烧造成大量的气溶胶粒子悬浮于空中,是造成江苏出现持续不同程度的霾天气的主要原因,同时也为雾滴形成提供了丰富的凝结核;中高层冷空气强度未能完全破坏底层相对稳定的层结,较小的风速和较大的湿度有利于雾霾的发展,重度霾或雾风速多在3 m/s以下,且相对湿度在80%以上。频繁的弱降水过程对雾的形成和霾的加重起到了重要的作用;低层的逆温或近中性层结的维持,为雾霾持续存在提供了有利的层结条件,且浓雾形成主要有辐射贴地逆温和平流逆温两种形式;垂直上升运动与雾霾的发展之间有着互相影响的紧密联系,在具备一定的水汽条件时,底层弱的上升运动有利于雾体的向上发展从而促进雾的加浓。后向轨迹模拟雾霾相对较严重的6月10日污染轨迹表明沿江和苏南地区污染物浓度上升除了本地悬浮颗粒物外,安徽境内的污染物的输送也是一个重要因素,而北部地区更多还是本地的污染源。 相似文献
19.
Beat Schmid John M. Livingston Philip B. Russell Philip A. Durkee Haflidi H. Jonsson Donald R. Collins Richard C. Flagan John H. Seinfeld Santiago Gassó Dean A. Hegg Elisabeth Öström Kevin J. Noone Ellsworth J. Welton Kenneth J. Voss Howard R. Gordon Paola Formenti Meinrat O. Andreae 《Tellus. Series B, Chemical and physical meteorology》2000,52(2):568-593
We report on clear‐sky column closure experiments (CLEARCOLUMN) performed in the Canary Islands during the second Aerosol Characterization Experiment (ACE‐2) in June/July 1997. We present CLEARCOLUMN results obtained by combining airborne sunphotometer and in‐situ (optical particle counter, nephelometer, and absorption photometer) measurements taken aboard the Pelican aircraft, space‐borne NOAA/AVHRR data and ground‐based lidar and sunphotometer measurements. During both days discussed here, vertical profiles flown in cloud‐free air masses revealed 3 distinctly different layers: a marine boundary layer (MBL) with varying pollution levels, an elevated dust layer, and a very clean layer between the MBL and the dust layer. A key result of this study is the achievement of closure between extinction or layer aerosol optical depth (AOD) computed from continuous in‐situ aerosol size‐distributions and composition and those measured with the airborne sunphotometer. In the dust, the agreement in layer AOD (λ=380–1060 nm) is 3–8%. In the MBL there is a tendency for the in‐situ results to be slightly lower than the sunphotometer measurements (10–17% at λ=525 nm), but these differences are within the combined error bars of the measurements and computations. 相似文献
20.
Francesca Barnaba Ferdinando De Tomasi Gian Paolo Gobbi Maria Rita Perrone Anna Tafuro 《Atmospheric Research》2004,70(3-4):229-259
Functional relationships linking at λ0=351 nm aerosol extinction αλ0aer and backscatter coefficient βλ0aer of maritime and desert type aerosols are determined to allow for inversion of the single-wavelength lidar signals. Such relationships are derived as mean behavior of 20,000 extinction versus backscatter computations, performed for aerosol size distributions and compositions whose describing parameters are randomly chosen within the naturally observed variability. For desert-type aerosols, the effect of the particle non-sphericity is considered and it is shown that the extinction to backscatter ratio of non-spherical dust particles can be up to 60% larger than the values obtained for spherical particles. Aerosol extinction and backscatter coefficient profiles obtained inverting the single-wavelength lidar signal with the modeled relationships are then compared to the same profiles measured by a combined elastic-Raman lidar operating at 351 nm. Analytical back trajectories and satellite images are used to characterize advection patterns during lidar measurements and to properly choose the modeled functional relationship. A good accordance between the two techniques is found for advection patterns over the lidar site typical of maritime and dust conditions. Maximum differences between the model-based αλ0aer and βλ0aer vertical profiles and the corresponding ones measured by the combined elastic-Raman lidar technique are of 30% and 40% in maritime and desert dust conditions, respectively. The comparison of elastic-Raman lidar measurements and model-based results also reveals that particle non-sphericity must be taken into account when mineral dust-type aerosols are directly advected over the measurement site. 相似文献