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1.
Flux densities of carbon dioxide were measured over an arid, vegetation-free surface by eddy covariance techniques and by a heat budget-profile method, in which CO2 concentration gradients were specified in terms of mixing ratios. This method showed negligible fluxes of CO2, consistent with the bareness of the experimental site, whereas the eddy covariance measurements indicated large downward fluxes of CO2. These apparently conflicting observations are in quantitative agreement with the results of a recent theory which predicts that whenever there are vertical fluxes of sensible or latent heat, a mean vertical velocity is developed. This velocity causes a mean vertical convective mass flux (= cw for CO2, in standard notation). The eddy covariance technique neglects this mean convective flux and measures only the turbulent flux c w. Thus, when the net flux of CO2 is zero, the eddy covariance method indicates an apparent flux which is equal and opposite to the mean convective flux, i.e., c w = – c w. Corrections for the mean convective flux are particularly significant for CO2 because cw and c w are often of similar magnitude. The correct measurement of the net CO2 flux by eddy covariance techniques requires that the fluxes of sensible and latent heat be measured as well.  相似文献   

2.
Comparison was made of the flux measurements of a closed-path CO2/H2O analyzer and an open-path H2O analyzer above a clover field and the forest floor of a Douglas-fir stand. The attenuation of the gas concentration fluctuations caused by the sampling tube of the closed-path analyzer resulted in underestimation of the H20 flux above both surfaces. The degree of underestimation above the clover field depended on wind speed, but was smaller than that calculated from the transfer function for laminar flow in a circular tube and the scalar cospectrum in the neutral and unstable surface layer. Above the forest floor CO2 fluctuations led those of H2O by 0.7s. The implications of this are discussed regarding the determination of the time delay caused by the sampling tube of the closedpath analyzer. The day-time CO2 efflux from the forest floor, averaged over three days, was 0.043 mg/(m2s).  相似文献   

3.
The commonly reported temperature coefficient of P. the equilibrium partial pressure of CO2, is (P/T) A,C ,which is about 15 ppm/°C, or 5% of the atmospheric partial pressure of CO2. This coefficient, however, applies only to deep water, not to surface water which can exchange CO2 with the atmosphere. The coefficient (P/T) A,C ,, where designates constancy of the sum of atmospheric and surface-ocean CO2, is the appropriate value for air-sea exchange. Numerical values are mass-dependent because the depth of the exchanging ocean layer must be specified. For a 100-m surface layer, the value is ca. 1.5 ppm/°C, or 0.5% of ambient CO2. Editor's Note:In view of the interdisciplinary importance of the carbon dioxide-climate problem, this note on seawater chemistry should be of interest to specialists beyond the discipline of ocean chemistry.  相似文献   

4.
We present turbulence spectra and cospectra derived from long-term eddy-covariancemeasurements (nearly 40,000 hourly data over three to four years) and the transferfunctions of closed-path infrared gas analyzers over two mixed hardwood forests inthe mid-western U.S.A. The measurement heights ranged from 1.3 to 2.1 times themean tree height, and peak vegetation area index (VAI) was 3.5 to 4.7; the topographyat both sites deviates from ideal flat terrain. The analysis follows the approach ofKaimal et al. (Quart. J. Roy. Meteorol. Soc. 98, 563–589, 1972) whose results were based upon 15 hours of measurements atthree heights in the Kansas experiment over flatter and smoother terrain. Both thespectral and cospectral constants and stability functions for normalizing and collapsingspectra and cospectra in the inertial subrange were found to be different from those ofKaimal et al. In unstable conditions, we found that an appropriate stabilityfunction for the non-dimensional dissipation of turbulent kinetic energy is of the form () = (1 - b-)-1/4 - c-, where representsthe non-dimensional stability parameter. In stable conditions, a non-linear functionGxy() = 1 + bxyc xy (cxy < 1) was found to benecessary to collapse cospectra in the inertial subrange. The empirical cospectralmodels of Kaimal et al. were modified to fit the somewhat more (neutraland unstable) or less (stable) sharply peaked scalar cospectra observed over forestsusing the appropriate cospectral constants and non-linear stability functions. Theempirical coefficients in the stability functions and in the cospectral models varywith measurement height and seasonal changes in VAI. The seasonal differencesare generally larger at the Morgan Monroe State Forest site (greater peak VAI) andcloser to the canopy.The characteristics of transfer functions of the closed-path infrared gas analysersthrough long-tubes for CO2 and water vapour fluxes were studied empirically. This was done by fitting the ratio between normalized cospectra of CO2 or watervapour fluxes and those of sensible heat to the transfer function of a first-order sensor.The characteristic time constant for CO2 is much smaller than that for water vapour. The time constant for water vapour increases greatly with aging tubes. Three methods were used to estimate the flux attenuations and corrections; from June through August, the attenuations of CO2 fluxes are about 3–4% during the daytime and 6–10% at night on average. For the daytime latent heat flux (QE), the attenuations are foundto vary from less than 10% for newer tubes to over 20% for aged tubes. Correctionsto QE led to increases in the ratio (QH + QE)/(Q* - QG) by about 0.05 to0.19 (QH is sensible heat flux, Q* is net radiation and QG is soil heat flux),and thus are expected to have an important impact on the assessment of energy balanceclosure.  相似文献   

5.
From measurements in the atmospheric surface layer over a paddy field, the Kolmogorov constants for CO2 and longitudinal wind velocity were obtained. In this study, the nondimensional dissipation rate nc = (1–16 v )-1/2 for CO2 variance and = (1–16 v )-1/4 – v for turbulent energy were used, assuming the equality of the local production term and the local dissipation term, and neglecting the divergence flux term in the budget equation. The value of the constant for CO2 was consistent with recent determinations for temperature and humidity. The constant for longitudinal wind velocity showed good agreement with other recent observations.  相似文献   

6.
Summary During an expedition to the high Andes of Southern Peru in June–July 1977, measurements of direct solar radiation in four spectral bands (0.270–0.530–0.630–0.695–2.900 ) were conducted at six sites in elevations ranging from sea level to 5645 m. These measurements were evaluated in Langley plots to determine total optical depths () and irradiances at the top of the atmosphere. In addition, water vapor optical depths (wv) were calculated from the mean radiosounding over Lima during the expedition, and Rayleigh (ray) and ozone (oz) optical depths were obtained from published tabulations. Subtracting ray, oz, and wv from yielded estimates of aerosol optical depth aer. The components ray and oz decrease from the shorter towards the longer wavelength bands and from the lower towards the higher elevation sites; aer also decreases towards the higher elevations. Particularly pronounced is the decrease of aer and from the lowlands of the Pacific coast to the highlands of the interior, reflecting the effect of a persistent lower-tropospheric inversion and the contrast from the marine boundary layer to the clear atmosphere of the high Andes.With 4 Figures  相似文献   

7.
Summary The first GCM climate change projections to include dynamic vegetation and an interactive carbon cycle produced a very significant amplification of global warming over the 21st century. Under the IS92a business as usual emissions scenario CO2 concentrations reached about 980ppmv by 2100, which is about 280ppmv higher than when these feedbacks were ignored. The major contribution to the increased CO2 arose from reductions in soil carbon because global warming is assumed to accelerate respiration. However, there was also a lesser contribution from an alarming loss of the Amazonian rainforest. This paper describes the phenomenon of Amazonian forest dieback under elevated CO2 in the Hadley Centre climate-carbon cycle model.  相似文献   

8.
Several formulations and proposals to determine the value of the radiometric scalar roughness for sensible heatz 0h,r are tested with respect to their performance in the estimation of the sensible heat flux by means of the profile equations derived from Monin-Obukhov similarity theory. The equations are applied to the data set of spatially averaged surface skin temperature and profiles of wind speed and temperature observed in a pasture field during a growing season. The use of a physical model developed for a dense canopy to estimate scalar roughness for sensible heatz 0h,r produced sensible heat fluxH with a correlation coefficientr=0.884, the ratio of means being H s /H=1.19 in a comparison with reference values ofH s . In comparison, a proposal for a fixed value ofz 0h yieldedr=0.887, H s /H=0.879. In both cases, the validity ofz 0h =z 0h,r was assumed. All expressions derived to estimatez 0h,r from a multiple linear regression with such predictors as leaf area index, solar radiation and the ratio of solar radiation to extraterrestrial radiation, were found to produce a better result, withr better than 0.90 and H s /H around 1.0. However, when the constantsc andf of a linear regression equationHs=cH+f are used to evaluate the equations, a marked difference in performance of each formulation appeared. In general, equations with smaller numbers of predictors tend to produce a biased result, i.e., an overestimation ofH at largeH s . These values ofH are used in conjunction with the energy balance equation to derive values of the latent heat fluxLE, which are shown to be in good agreement with the reference valuesLE s , withr greater than 0.97.  相似文献   

9.
We present the first application of a multi-stage impactor to study volcanic particle emissions to the troposphere from Masaya volcano, Nicaragua. Concentrations of soluble SO4 2–,Cl–, F–, NO3 –, K+, Na+,NH4 +, Ca2+ and Mg2+ were determined in 11 size bins from 0.07 m to >25.5 m. The near-source size distributions showed major modes at 0.5m (SO4 2–, H+,NH4 +); 0.2 m and 5.0 m (Cl–) and 2.0–5.0 m(F–). K+ and Na+ mirrored the SO4 2– size-resolvedconcentrations closely, suggesting that these were transported primarily asK2SO4 and Na2SO4 in acidic solution, while Mg2+ andCa2+ presented modes in both <1 m and >1 m particles. Changes in relative humidity were studied by comparing daytime (transparent plume) and night-time (condensed plume) results. Enhanced particle growth rates were observed in the night-time plume as well as preferential scavenging of soluble gases, such as HCl, by condensed water. Neutralisation of the acidic aerosol by background ammonia was observed at the crater rim and to a greater extent approximately 15 km downwind of the active crater. We report measurements of re-suspended near-source volcanic dust, which may form a component of the plume downwind. Elevated levels ofSO4 2–, Cl–, F–,H+, Na+, K+ and Mg2+ were observed around the 10 m particle diameter in this dust. The volcanic SO4 2– flux leaving the craterwas 0.07 kg s–1.  相似文献   

10.
Recent studies suggest that the destruction of methane by Cl in the marine boundary layer could be accounted for as another major sink besides the methane destruction by OH. High level ab initio molecular orbital calculations have been carried out to study the CH4+Cl reaction, the carbon Kinetic Isotope Effect (KIE) is calculated using Conventional Transition-State Theory (CTST) plus Wigner and Eckart semiclassical tunneling corrections. The calculated KIE is around 1.026 at 300 K and has a small temperature variation. This is by far the largest KIE among different processes involving atmospheric methane destruction (e.g., OH, soil). A calculated mass balance of atmospheric methane including the KIE for the CH4+Cl reaction is found to favor those methane budgets with enhanced biological methane sources, which have relatively lighter carbon isotope composition.  相似文献   

11.
Parameterization of evaporation from a non-plant-covered surface is very important in the hierarchy strategy of modelling land surface processes. One of the representations frequently used in its computation is the resistance formulation. The performance of the evaporation schemes using the , , and their combination resistance approaches to parameterize evaporation from bare soil surfaces is discussed. For that purpose, the nine schemes, based on a different dependence of and on volumetric soil moisture content and its saturated value, are used.The tests of performances of the considered schemes are based on time integrations by the land surface module (BARESOIL) using observed data. The 23 data sets at a bare surface experimental site in Rimski anevi, Yugoslavia on chernozem soil, were used for the resistance algorithm evaluation. The quality of the schemes was compared with the observed values of the latent heat flux using several statistical parameters.  相似文献   

12.
Zusammenfassung An einem Material von 100 Fällen eindeutig gesicherten Herztodes, die im Institut für Gerichtliche und Soziale Medizin in Frankfurt am Main aus einem bestimmten Bereich — Raum Frankfurt am Main — und einer bestimmten zeit—Kalenderjahre 1948 bis 1950—zur Autopsie gelangten, einerseits und den bioklimatischen Daten für den gleichen Raum und die gleiche Zeit anderseits, wurde der Zusammenhang von Herztodesfällen und Wettervorgängen mit der Wahrscheinlichkeitsüberlegung, dem Wahrscheinlichkeitsintegral und formalstatistischen Methoden überprüft. Die Auswertung ergab, daß eine starke Abhängigkeit des Herztodes vom Wettergeschehen besteht. Die Häufung der Herztodesfälle konnte für die Sammelgruppe Wetterstörungen, für labiles Aufgleiten, Warmfront mit Aufgleiten und Kaltfront mit Turbulenz ebenso eindeutig gesichert werden, wie die Verminderung der Herztodesfälle in störungsfreien Zeiten. Die hohe Wahrscheinlichkeit einer Beziehung besteht ferner für Kaltfront mit Aufgleiten und in geringerem Maße auch für Föhndurchbruch. Während bei Okklusion das Material zu einem abschließenden Urteil zu gering war, konnte bei allen übrigen Wetterlagen eine Beziehung zum plötzlichen Herztod nicht nachgewiesen werden. Auch für die Gruppen, bei denen eine enge Beziehung statistisch gesichert werden konnte, sei betont, daß die Wettervorgänge nicht die alleinige Ursache des plötzlichen Herztodes, sondern nur ein auslösendes Moment bei schon vorher schwer geschädigten Herzen darstellen.
Summary On the basis of 100 ascertained cases of cardiac death from a certain region—province Frankfort on-the-Main—and a certain period—calendar years 1948 to 1950—, submitted to autopsy in the Institute for Legal and Social Medicine at Frankfort on-the-Main, and of bioclimatic data from the same region and period, the relation between cardiac death and meteorological phenomena was examined by means of probability considerations, the probability integral, and methods of formal statistics. Evaluation of this material showed cardiac death to be strongly dependent on weather conditions. Increase of frequency of cardiac death could be established without any doubt for the collective groups weather disturbances, unstable ascending motion, warm front with ascending motion, cold front with turbulence, whereas decrease of frequency was found in undisturbed periods. Furthermore, high probability of an existing relation was found for cold front with ascending motion and, to a lesser degree, also for foehn invasion. As to occlusion no definite conclusions could be drawn for scarcity of observations. For all the other weather types no relation to sudden cardiac death could be proved. Meteorological phenomena are by no means the only cause of sudden cardiac death, not even for the groups in which a close relation could be established statistically. They have but an initiatory effect in case of prior severe heart diseases.
Résumé Disposant d'un matériel médical de 100 cas de mort cardiaque qui ont fait l'objet d'autopsies à l'Institut de médecine légale et sociale de Francfort sur le Mein (région de Francfort et période de 1948 à 1950), et disposant d'autre part pour la même région et pour la même période d'observations bioclimatologiques, l'auteur a étudié la relation de ces décès avec les phénomènes météorologiques à l'aide des méthodes modernes de statistique, de l'intégrale de probabilité etc. Le résultat montre une étroite dépendance centre les cas de mort cardiaque et les conditions météorologiques. On a pu vérifier sans doute possible l'augmentation des décès lors de «perturbations», d'«ascendances labiles», de «fronts chauds avec glissement ascendant», de «fronts froids avec turbulence», de même que leur diminution lors de périodes non troublées. La forte corrélation subsiste avec les «fronts froids avec ascendance» et à un moindre degré avec «l'invasion du foehn». Tandis que pour les «occlusions» le matériel disponible était trop restreint pour aboutir à une conclusion, l'examen des situations autres que les précédentes n'a pas conduit à une relation intime. Il convient de remarquer que pour tous les groupes de météores ayant donné une corrélation statistique très nette, les phénomènes météorologiques n'ont joué qu'un rôle déclancheur chez des malades déjà gravement atteints.

Mit 2 Textabbildungen.  相似文献   

13.
Surface-Layer Fluxes in Stable Conditions   总被引：2，自引：2，他引：0  
Micrometeorological tower data from the Microfronts experiment are analyzed. Scale-dependencies of the flux and flux sampling error are combined to automatically determine Reynolds turbulence cut-off time scales for computing fluxes from time series. The computed downward heat flux at the 3 m height averaged over nine nights with 7.3 hours each night is 20% greater than the downward heat flux computed at the 10 m height. In contrast, there is only a 1.2% difference between 3 m and 10 m heat fluxes averaged over daytime periods, and there is less than a 2% difference between 3 m and 10 m momentum fluxes whether averaged over nighttime or daytime periods.Stability functions, M(z/L) and H(z/L) are extended to z/L up to 10, where z is the observational height and L is the Obukhov length. For 0.01 < z/L < 1 the estimated functions generally agree with Businger-Dyer formulations, though the H estimates include more scatter compared to the M estimates. For 1 < z/L < 10, the flux intermittency increases, the flux Richardson number exceeds 0.2, and the number of flux samples decreases. Nonetheless the estimates of the stability function M based on 3-m fluxes are closer to the formula proposed by Beljaars and Holtslag in 1991 while the M functions based on 10-m fluxes appears to be closer to the formula proposed by Businger et al. in 1971. The stability function H levels off at z/L = 0.5.  相似文献   

14.
Parameterizing turbulent diffusion through the joint probability density   总被引：3，自引：3，他引：0  
The convective mass flux parameterization often used in meteorological modeling expresses the vertical flux of a transported scalar as proportional to the product of the difference in mean values of the scalar in updrafts and downdrafts and their characteristic velocity. The proportionality factor is a constant to be specified. We show that this proportionality factor also appears in the relaxed eddy accumulation technique of Businger and Oncley. That associates the surface-layer flux of a scalar with the product of the standard deviation of vertical velocity and the mean concentration difference between updrafts and downdrafts.We show that this constant (b) is determined uniquely by the joint probability density (jpd) of vertical velocity and the scalar. Using large-eddy simulation, we generate this jpd for a conservative scalar diffusing through a convective boundary layer. It has quite different forms in top-down and bottom-up diffusion geometries. The bottom-up jpd is fairly well represented by a jointly Gaussian form and implies b ~ 0.6, in good agreement with the surface-layer value reported by Businger and Oncley. The top-down jpd is strikingly non-Gaussian and gives b ~ 0.47. Updrafts carry the bulk of the scalar flux - 70% in the bottom-up case, 60% in the top-down case.The National Center for Atmospheric Research is sponsored by the National Science Foundation.  相似文献   

15.
Summary The influence of agricultural management on the CO2 budget of a typical subalpine grassland was investigated at the Swiss CARBOMONT site at Rigi-Seebodenalp (1025m a.s.l.) in Central Switzerland. Eddy covariance flux measurements obtained during the first growing season from the mid of spring until the first snow fall (17 Mai to 25 September 2002) are reported. With respect to the 10-year average 1992–2001, we found that this growing season had started 10 days earlier than normal, but was close to average temperature with above-normal precipitation (100–255% depending on month). Using a footprint model we found that a simple approach using wind direction sectors was adequate to classify our CO2 fluxes as being controlled by either meadow or pasture. Two significantly different light response curves could be determined: one for periods with external interventions (grass cutting, cattle grazing) and the other for periods without external interventions. Other than this, meadow and pasture were similar, with a net carbon gain of –128±17g Cm–2 on the undisturbed meadow, and a net carbon loss of 79±17g Cm–2 on the managed meadow, and 270±24g Cm–2 on the pasture during 131 days of the growing season, respectively. The grass cut in June reduced the gross CO2 uptake of the meadow by 50±2% until regrowth of the vegetation. Cattle grazing reduced gross uptake over the whole vegetation period (37±2%), but left respiration at a similar level as observed in the meadow.  相似文献   

16.
The aerodynamic classification of the resistance laws above solid surfaces is based on the use of a so-called Reynolds roughness number Re s =h s u */, whereh s is the effective roughness height, -viscosity,u *-friction velocity. The recent experimental studies reported by Toba and Ebuchi (1991), demonstrated that the observed variability of the sea roughness cannot be explained only on the basis of the classification of aerodynamic conditions of the sea surface proposed by Kitaigorodskii and Volkov (1965) and Kitaigorodskii (1968) even though the latter approach gains some support from recent experimental studies (see for example Geernaertet al. 1986). In this paper, an attempt is made to explain some of the recently observed features of the variability of surface roughness (Toba and Ebuchi, 1991; Donelanet al., 1993). The fluctuating regime of the sea surface roughness is also described. It is shown that the contribution from the dissipation subrange to the variability of the sea surface can be very important and by itself can explain Charnock's (1955) regime.  相似文献   

17.
Wind and temperature profiles in the stable boundary layer were analyzed in the context of MoninObukhov similarity. The measurements were made on a 60-m tower in Kansas during October 1999 (CASES-99). Fluxprofile relationships, obtained from these measurements in their integral forms, were established for wind speed and temperature. Use of the integral forms eliminates the uncertainty and accuracy issues resulting from gradient computations. The corresponding stability functions, which were nearly the same for momentum and virtual sensible heat, were found to exhibit different features under weakly stable conditions compared to those under strongly stable conditions. The gradient stability functions were found to be linear, namely m = 1+ 5.8 and h = 1 + 5.4 up to a limit of the MoninObukhov stability parameter = 0.8; this is consistent with earlier findings. However, for stronger stabilities beyond a transition range, both functions were observed gradually to approach a constant, with a value of approximately 7. To link these two distinct regimes, a general but pliable functional form with only two parameters is proposed for the stability functions, covering the entire stability range from neutral to very stable conditions.  相似文献   

18.
Turbulence measurements performed in a stable boundary layer over the sloping ice surface of the Vatnajökull in Iceland are described. The boundary layer, in which katabatic forces are stronger than the large-scale forces, has a structure that closely resembles that of a stable boundary layer overlying a flat land surface, although there are some important differences. In order to compare the two situations the set-up of the instruments on an ice cap in Iceland was reproduced on a flat grass surface at Cabauw, the Netherlands. Wind speed and temperature gradients were calculated and combined with flux measurements made with a sonic anemometer in order to obtain the local stability functions m and h as a function of the local stability parameter z/L. Unlike the situation at Cabauw, where m was linear as a function of z/L, in the katabatically forced boundary layer, the dependence of m on stability was found to be non-linear and related to the height of the wind maximum. Thermal stratification and the depth of the stable boundary layer however seem to be rather similar under these two different forcing conditions.Furthermore, measurements on the ice were used to construct the energy balance. These showed good agreement between observed melt and components contributing to the energy balance: net radiation (supplying 55% of the energy), sensible heat flux (30%) and latent heat flux (15%).Local sources and sinks in the turbulent kinetic energy budget are summed and indicate a reasonable balance in near-neutral conditions but not in more stable situations. The standard deviation of the velocity fluctuations u, v, and w, can be scaled satisfactorily with the local friction velocity u* and the standard deviation of the temperature fluctuation with the local temperature scale *.  相似文献   

19.
Cloud water and interstitial aerosol samples collected at Mt. Sonnblick (SBO) were analyzed for sulfate and aerosol carbon to calculate in-cloud scavenging efficiencies. Scavenging efficiencies for sulfate (SO) ranged from 0.52 to 0.99 with an average of 0.80. Aerosol carbon was scavenged less efficiently with an average value (AC) of 0.45 and minimum and maximum values of 0.14 and 0.81, respectively. Both SO and AC showed a marked, but slightly different, dependence on the liquid water content (LWC) of the cloud. At low LWC, SO increased with rising LWC until it reached a relatively constant value of 0.83 above an LWC of 0.3 g/m3. In the case of aerosol carbon, we obtained a more gradual increase of AC up to an LWC of 0.5 g/m3. At higher LWCs, _ remained relatively constant at 0.60. As the differences between SO and A varied across the LWC range observed at SBO, we assume that part of the aerosol carbon was incorporated into the cloud droplets independently from sulfate. This hypothesis is supported by size classified aerosol measurements. The differences in the size distributions of sulfate and total carbon point to a partially external mixture. Thus, the different chemical nature and the differences in the size and mixing state of the aerosol particles are the most likely candidates for the differences in the scavenging behavior.  相似文献   

20.
A new, biogeochemical model of ice age cycles is developed and applied which explains major features of climate variations in the late Quaternary —rapid ice age terminations, large glacial-interglacial amplitudes and 100-kyr cycles — in a way consistent with the paleorecord. Existing models which invoke non-linear, ice-sheet-earth-crust dynamics to explain ice age cycles are not consistent with simultaneous terminations in both hemispheres and other phase relationships implied by the paleorecord. The present model relates climate change to oscillations of oceanic primary (new) production controlled by the availability of inorganic nitrogen. Large oscillations follow shelf erosion events triggered by small sea-level drops. These drops are due to glacial buildup associated with a minimum in Northern Hemisphere insolation. Rapid global warming at terminations is initiated by open ocean denitrification events leading to new production crashes and rapid modification of atmospheric trace gas concentrations (CO2, DMS, N2O). Other feedbacks of the land-ice-atmosphere-ocean system control the rest of the climate cycle. 100-kyr cycles derive from orbital pacemaking of the strong, low-frequency model response. Results suggest that the climate regime transition near 800 kyr B.P. may be related to changes in the continental shelf slope, that existing chronologies based on orbital tuning may need to be revised and that temporary increases in atmospheric N2O concentrations at terminations, due to the denitrification events, may have caused significant greenhouse warming. A spike of elevated N2O concentration at terminations may be recorded in polar ice.  相似文献   

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