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1.
Based on the Stratospheric Aerosol and Gas Experiment (SAGE) II and the Halogen Occultation Experiment (HALOE) ozone profiles and the Total Ozone Mapping Spectrometer (TOMS) total ozone data sets, an empirical model for estimating the vertical distribution of stratospheric ozone over China is proposed. By using this model, the vertical distribution of stratospheric (16–50 km) ozone can be estimated according to latitude, month and total ozone. Comparisons are made between the modeled ozone profiles and the ... 相似文献
2.
利用SAGE Ⅱ和HALOE臭氧垂直分布资料和TOMS臭氧总量资料, 研究我国北方(45°~55°N和35°~45°N范围), 东部(105°~135°E) 和西部(75°~105°E) 大气臭氧总量和垂直分布特征和差异。结果表明:我国北方东部冬季、春季和秋季臭氧总量明显大于西部, 主要表现在平流层臭氧极大值附近及其以下高度臭氧含量东部比西部明显偏大, 这种差异在冬、春季尤为明显; 随着纬度的降低, 冬季和秋季臭氧总量东、西部差异减小, 但春季臭氧总量东、西部差异没有明显改变; 夏季, 在45°~55°N范围, 东、西部臭氧分布没有明显差异, 但在35°~45°N范围, 臭氧分布东、西部差异较明显, 臭氧总量东、西部差异达到20.6 DU, 16 km以下臭氧柱总量东、西部差异达到12.8 DU。该文还对导致我国东、西部臭氧分布差异的原因进行了分析。 相似文献
3.
大尺度山地上空的臭氧低值及地面加热 总被引：11，自引：0，他引：11
首次利用Ｎｉｍｂｕｓ－７卫星上搭载的臭氧观测光谱仪（ＴＯＭＳ）资料,分析研究了大尺度山地（青藏高原、洛基山脉和安第斯山脉）上空臭氧总量的分布和季节变化规律,指出了大尺度山地对大气臭氧的减少作用。从全球大气臭氧总量分布和纬向偏差分布可以看出：在上述３个大尺度山地上空均存在着明显的臭氧低值扰动,该扰动区夏季强于冬季。在这３个区域中,青藏高原上空的臭氧低值扰动为最强。分析同时指出：上述大尺度山地上空臭氧季节变化的极小值在秋季,极大值在春季。但上述地区臭氧总量与同纬度其它地区臭氧总量的偏差在春季或初夏达到极小值。为分析这种大尺度山地对臭氧减少作用的原因,本文分析了青藏高原地面热源与臭氧总量的关系,指出：大尺度山地表面对大气的加热与该地区臭氧减少之间存在着良好的反相关;在地面对大气的感热加热、潜热加热和有效长波辐射加热中,以感热加热与臭氧减少的关系为最好。 相似文献
4.
An Empirical Method for Estimating Background Stratospheric Aerosol Extinction Profiles over China 
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下载免费PDF全文 YANG Jing-Mei 《大气和海洋科学快报》2012,5(2):95-101
The current paper introduces an empirical method for estimating the vertical distribution of background stratospheric aerosol extinction profiles covering the latitude bands of 50±5°N,40±5°N,30±5°N,and 20±5°N and the longitude range of 75 135°E based on Stratospheric Aerosol and Gas Experiment (SAGE) II aerosol extinction measurements at wavelengths of 1020 nm,525 nm,452 nm,and 386 nm for the volcanically calm years between 1998 2004.With this method,the vertical distribution of stratospheric aerosol extinction coefficients can be estimated according to latitude and wavelength.Comparisons of the empirically calculated aerosol extinction profiles and the SAGE II aerosol measurements show that the empirically calculated aerosol extinction coefficients are consistent with SAGE II values,with relative differences within 10% from 2 km above the tropopause to 33 km,and within 22% from 33 km to 35 km.The empirically calculated aerosol stratospheric optical depths (vertically integrated aerosol extinction coefficient) at the four wavelengths are also consistent with the corresponding SAGE II optical depth measurements,with differences within 2.2% in the altitude range from 2 km above the tropopause to 35 km. 相似文献
5.
WENSHOU TIAN MARTYN CHIPPERFIELD QIAN HUANG 《Tellus. Series B, Chemical and physical meteorology》2008,60(4):622-635
The relatively low total column ozone (TCO) above the Tibetan Plateau (TP) observed in summer is only partly due to the thinness of the atmospheric column. In this paper the effect of the TP on the TCO is further investigated using satellite data [Total Ozone Mapping Spectrometer (TOMS) ozone column and Stratospheric Aerosol and Gas Experiment II (SAGE II) ozone profiles], ECMWF ERA-40 reanalysis data and a 3-D chemistry-climate model (CCM). It is found that the low TCO over the TP is also closely related to large-scale uplift and descent of isentropic surfaces implied by seasonal and longitudinal variations in the tropopause height. The variations in tropopause height, with a maximum in summer, can be driven by various processes including convective activity, air expansion as well as the monsoon system. While previous studies have showed an important role of troposphere-to-stratosphere transport in contributing to the observed low ozone column over the TP, the mechanism revealed in this study is an alternative amendment to the causes of the TCO low over the TP. It is also found that the monsoon anticyclone circulation induces an isentropic transport of trace gases from high latitudes towards the TP in the lower stratosphere and hence modifies tracer distributions. For the vertical distribution of ozone, the modulation by the TP is most significant below ∼20 km, that is, in the upper troposphere and lower stratosphere (UTLS). The smaller differences in NO x between Eastern TP and TP compared to large dynamically caused differences in ozone and methane imply the TCO low over the TP is mainly due to transport processes rather than chemistry. 相似文献
6.
青藏高原平流层臭氧和气溶胶的变化趋势研究 总被引：2，自引：1，他引：2
通过分析SAGEⅡ资料,发现青藏高原平流层臭氧存在递减趋势,15—50 km臭氧的变化对臭氧总量变化贡献最大,其中25—50 km和15—25 km两层的贡献大致相当。通过青藏高原和中国东部地区平流层臭氧变化的对比,清楚地看出:两地臭氧总量变化的差异主要是由于在15—25 km臭氧变化不同所致。5—7月臭氧变化趋势的情况与年平均的变化类似,两地臭氧变化的差异主要在平流层低层,即15—25 km。青藏高原平流层气溶胶面密度的时间变化序列显示:大的火山喷发对青藏高原平流层气溶胶具有重要影响,其影响可持续6年左右。从1997年至今,青藏高原18—25 km气溶胶面密度增加,最大的增长出现在23 km,每年大约增长4%—5%。而在16—17 km气溶胶的面密度出现减少趋势。与此同时,在37 km以下,青藏高原的温度出现递减的趋势,而且其递减速度比中国东部地区快;在37—50 km,温度出现增加的趋势,青藏高原的增温也比中国东部地区快。青藏高原平流层低层气溶胶的增加和温度的降低都将增强该区域非均相反应的作用。 相似文献
7.
Temporal Variations in the Vertical Distribution of Stratospheric Ozone over Obninsk from Lidar Data
The results of lidar measurements of ozone profiles over Obninsk in the altitude range of 12–35 km in 2012–2016 are presented. Temporal variations in total ozone in the above altitude range and seasonal variations in the vertical distribution of ozone are considered. Basic attention is paid to the analysis of ozone profile variations on the daily and weekly scales. The backtrajectory analysis demonstrated that in most cases the formation of layers with low or high ozone values is explained by the direction of meridional advection. Cross-correlation coefficients for the variations in ozone and temperature relative to the current monthly mean variations are calculated. Rather high values of correlation coefficients (~0.4–0.6) are obtained for summer in the low stratosphere (100 and 160 hPa) and for winter in the upper troposphere (50 and 20 hPa). In general, variations in ozone profiles are consistent with available climatologic data. 相似文献
8.
S. Yonemura S. Kawashima H. Matsueda Y. Sawa S. Inoue H. Tanimoto 《Theoretical and Applied Climatology》2008,92(1-2):47-58
Summary The application of principal components and cluster analysis to vertical ozone concentration profiles in Tsukuba, Japan, has
been explored. Average monthly profiles and profiles of the ratio between standard deviation and the absolute ozone concentration
(SDPR) of 1 km data were calculated from the original ozone concentration data. Mean (first) and gradient (second) components
explained more than 80% of the variation in both the 0–6 km tropospheric and 11–20 km troposphere–stratosphere (interspheric)
layers. The principal components analysis not only reproduced the expected inverse relationship between mean ozone concentration
and tropopause height (r
2 = 0.41) and that in the tropospheric layer this is larger in spring and summer, but also yielded new information as follows.
The larger gradient component score in summer for the interspheric layer points to the seasonal variation of the troposphere–stratosphere
exchange. The minimum SDPR was at about 3 km in the tropospheric layer and the maximum was at about 17 km in the interspheric
layer. The tropospheric SDPR mean component score was larger in summer, possibly reflecting the mixing of Pacific maritime
air masses with urban air masses. The cluster analysis of the monthly ozone profiles for the 1970s and 2000s revealed different
patterns for winter and summer. The month of May was part of the winter pattern in the 1970s but part of the summer pattern
during the 2000s. This statistically detected change likely reflects the influence of global warming. Thus, these two statistical
analysis techniques can be powerful tools for identifying features of ozone concentration profiles.
Authors’ addresses: S. Yonemura, S. Kawashima, S. Inoue, National Institute for Agro-Environmental Sciences, 3-1-3 Kannondai,
Tsukuba, Ibaraki 305-0031, Japan; H. Matsueda, Y. Sawa, Meteorological Research Institute, 1-1 Nagamine, Tsukuba, Ibaraki
305-0052, Japan; H. Tanimoto, National Institute for Environmental Studies, 16-2 Onogawa, Tsukuba, Ibaraki 305-8506, Japan. 相似文献
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11.
北京冬季低层大气O3垂直分布观测结果的研究 总被引：17，自引：7，他引：17
给出了2001年2月26～28日在北京市方庄小区用系留气艇观测大气边界层O3垂直分布的结果.结合相关资料,对边界层O3的变化机制进行了初步分析.研究表明,冬季边界层O3主要受边界层气象条件、尤其是逆温层的影响比较大.在逆温层以下O3都维持极低值分布,超过仪器所能观测的最低极限.在逆温层向自由大气过渡的高度区域,O3浓度明显的梯度变化与风速垂直切变有关.观测还表明冬季城市市区大量排放的氮氧化物、水汽参与的化学反应是影响边界层O3变化的重要因素. 相似文献
12.
1998年青藏高原臭氧低值中心异常及其背景环流场的分析 总被引：4，自引：1，他引：3
采用TOMS和SAGE II臭氧卫星观测资料,对1998年青藏高原臭氧低值中心异常变化的过程和垂直结构进行了分析。为了探讨1998年这个低值中心出现异常的原因,利用NCEP/NCAR再分析资料,通过1998年高原附近上空位势场和位温的变化,分析了1998年臭氧低值中心异常期间高原上空对流层上层到平流层下层的流场和垂直运动的变化特征。结果表明,1998年11月,青藏高原上空对流顶比正常年份高,无论是对流层上层还是平流层下层,上升运动都比正常年份强。同时高原上空南亚高压也比正常年份强,于是使得1998年高原上空的强臭氧低值中心一直维持到11月。 相似文献
13.
1. IntroductionOzone is one of the trace gases in the atmosphere distributed in 10--50 km altitude withthe maximum in 20--28 km. Ozone is significant in the following three aspects impacting theclimate and environment: 1) Ozone absorbs harmful solar ultra--violet radiation for protecting the ecological system on the Earth; 2) ozone heats the stratosphere and forces the circulation systems in this layer; 3) ozone variation in the stratosphere can change the incomingradiation at the surface leve… 相似文献
14.
北极臭氧垂直分布和天气尺度变化的观测研究 总被引：2，自引：0，他引：2
北极地区臭氧对北极气候和环境系统起着重要作用。研究其分布和变化有助于了解北极的气候和环境及其对全球气候系统的影响,有助于气候和环境变化的数值预报。中国北极科学探测1999在北冰洋楚可奇海域成功的进行了大气臭氧观测。通过在中国“雪龙”号破冰船甲板上（于1999年8月18-24日在75°N,160°W附近处）释放大气臭氧探空仪获得了高分辨率的大气垂直结构和臭氧分布资料,可以进行大气尺度的大气臭氧变化研究。分析大气监测资料、TOMS臭氧总量资料和NCEP大气环流资料表明,大气臭氧总量随着对流层顶的低一高一低变化呈高一低一高的变化过程。研究还表明,大气柱的臭氧总量与13公里以下的大气臭氧含量关系密切,而在约20公里处的大气臭氧浓度最大值的变化与整个气柱臭氧的关系不大。500 hPa天气形势图上一个弱一强一弱的西南天气型造成的弱臭氧平流可能是这次臭氧变化的主要原因。 相似文献
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Klaus Wege 《Journal of Atmospheric Chemistry》1991,12(4):381-390
On 1 February 1989, -83.5°C was recorded in 27.8 hPa over Hohenpeißenberg, the lowest temperature in the 22-year series. This was measured together with a very low total ozone amount of 266 DU. This may be compared with nearly twice this amount on 27 February 1989. The situation was very unusual: following an extremely cold winter in the Arctic stratosphere, the stratospheric cold pole was located over southern Scandinavia on 1 February in a very southerly position. The analyzed temperatures of -92 °C in 30 hPa were also unusual. Even though the low ozone amounts over Hohenpeißenberg were probably dynamically caused, an additional very small ozone decrease due to heterogeneous reactions in altitudes from 23–28 km, where the temperatures lie below -80 °C, cannot be ruled out. Extinction measurements by the orbitting SAGE II instrument indeed show polar stratospheric clouds over Europe near 50° N during the period 31 January–2 February. Also, polar stratospheric clouds were previously observed over Kiruna at similarly low temperatures and signs of a corresponding small ozone decrease were noted there. 相似文献
17.
R. D. Bojkov E. Kosmidis J. J. DeLuisi I. Petropavlovskikh V. E. Fioletov S. Godin C. Zerefos 《Meteorology and Atmospheric Physics》2002,79(3-4):127-158
Summary Umkehr observations taken during the 1957–2000 period at 15 stations located between 19 and 52° N have been reanalyzed using
a significantly improved algorithm-99, developed by DeLuisi and Petropavlovskikh et al. (2000a,b). The alg-99 utilizes new
latitudinal and seasonally dependent first guess ozone and temperature profiles, new vector radiative transfer code, complete
aerosol corrections, gravimetric corrections, and others. Before reprocessing, all total ozone values as well as the N-values
(radiance) readings were thoroughly re-evaluated. For the first time, shifts in the N-values were detected and provisionally
corrected. The re-evaluated Umkehr data set was validated against satellite and ground based measurements. The retrievals
with alg-99 show much closer agreement with the lidar and SAGE than with the alg-92. Although the latitudinal coverage is
limited, this Umkehr data set contains ∼ 44,000 profiles and represent the longest (∼ 40 years) coherent information on the
ozone behavior in the stratosphere of the Northern Hemisphere. The 14-months periods following the El-Chichon and the Mt.
Pinatubo eruptions were excluded from the analysis. Then the basic climatological characteristics of the vertical ozone distribution
in the 44–52° N and more southern locations are described. Some of these characteristics are not well known or impossible
to be determined from satellites or single stations. The absolute and relative variability reach their maximum during winter–spring
at altitudes below 24 km; the lower stratospheric layers in the middle latitudes contain ∼ 62% of the total ozone and contribute
∼ 57% to its total variability. The layer-5 (between ∼ 24 and 29 km) although containing 20% of the total ozone shows the
least fluctuations, no trend and contributes only ∼ 11% to the total ozone variability. Meridional cross-sections from 19
to 52° N of the vertical ozone distribution and its variability illustrate the changes, and show poleward-decreasing altitude
of the ozone maximum. The deduced trends above 33 km confirm a strong ozone decline since the mid-1970s of over 5% per decade
without significant seasonal differences. In the mid-latitude stations, the decline in the 15–24 km layer is nearly twice
as strong in the winter-spring season but much smaller in the summer and fall. The effect of including 1998 and 1999 years
with relatively high total ozone data reduces the overall-declining trend. The trends estimated from alg-99 retrievals are
statistically not significantly different from those in WMO 1998a; however, they are stronger by about 1% per decade in the lower stratosphere and thus closer to the estimates by sondes.
Comparisons of the integrated ozone loss from the Umkehr measurements with the total ozone changes for the same periods at
stations with good records show complete concurrence. The altitude and latitude appearances of the long-term geophysical signals
like solar (1–2%) and QBO (2–7%) are investigated.
Received April 12, 2001 Revised September 19, 2001 相似文献
18.
A Tibetan ozone low was found in the 1990s after the Antarctic ozone hole.Whether this ozone low has been recovering from the beginning of the 2000s following the global ozone recovery is an intriguing topic.With the most recent merged TOMS/SBUV(Total Ozone Mapping Spectrometer/Solar Backscatter Ultra Violet) ozone data,the Tibetan ozone low and its long-term variation during 1979-2010 are analyzed using a statistical regression model that includes the seasonal cycle,solar cycle,quasi-biennial oscillation(QBO),ENSO signal,and trends.The results show that the Tibetan ozone low maintains and may become more severe on average during 1979-2010,compared with its mean state in the periods before 2000,possibly caused by the stronger downward trend of total ozone concentration over the Tibet.Compared with the ozone variation over the non-Tibetan region along the same latitudes,the Tibetan ozone has a larger downward trend during 1979-2010,with a maximum value of-0.40±0.10 DU yr 1 in January,which suggests the strengthening of the Tibetan ozone low in contrast to the recovery of global ozone.Regression analyses show that the QBO signal plays an important role in determining the total ozone variation over the Tibet.In addition,the long-term ozone variation over the Tibetan region is largely affected by the thermal-dynamical proxies such as the lower stratospheric temperature,with its contribution reaching around 10% of the total ozone change,which is greatly different from that over the non-Tibetan region. 相似文献
19.
Formation of the Summertime Ozone Valley over the Tibetan Plateau: The Asian Summer Monsoon and Air Column Variations 总被引：3，自引：0，他引：3
The summertime ozone valley over the Tibetan Plateau is formed by two influences,the Asian summer monsoon(ASM) and air column variations.Total ozone over the Tibetan Plateau in summer was ～33 Dobson units(DU) lower than zonal mean values over the ocean at the same latitudes during the study period 2005-2009.Satellite observations of ozone profiles show that ozone concentrations over the ASM region have lower values in the upper troposphere and lower stratosphere(UTLS) than over the non-ASM region.This is caused by frequent convective transport of low-ozone air from the lower troposphere to the UTLS region combined with trapping by the South Asian High.This offset contributes to a ～20-DU deficit in the ozone column over the ASM region.In addition,along the same latitude,total ozone changes identically with variations of the terrain height,showing a high correlation with terrain heights over the ASM region,which includes both the Tibetan and Iranian plateaus.This is confirmed by the fact that the Tibetan and Iranian plateaus have very similar vertical distributions of ozone in the UTLS,but they have different terrain heights and different total-column ozone levels.These two factors(lower UTLS ozone and higher terrain height) imply 40 DU in the lower-ozone column,but the Tibetan Plateau ozone column is only ～33 DU lower than that over the non-ASM region.This fact suggests that the lower troposphere has higher ozone concentrations over the ASM region than elsewhere at the same latitude,contributing ～7 DU of total ozone,which is consistent with ozonesonde and satellite observations. 相似文献
20.
The impact of cut-off lows on ozone in the upper troposphere and lower stratosphere over Changchun from ozonesonde observations 总被引：1，自引：0，他引：1
In situ measurements of the vertical structure of ozone were made in Changchun(43.53?N, 125.13?E), China, by the Institute of Atmosphere Physics, in the summers of 2010–13. Analysis of the 89 validated ozone profiles shows the variation of ozone concentration in the upper troposphere and lower stratosphere(UTLS) caused by cut-off lows(COLs) over Changchun. During the COL events, an increase of the ozone concentration and a lower height of the tropopause are observed.Backward simulations with a trajectory model show that the ozone-rich airmass brought by the COL is from Siberia. A case study proves that stratosphere–troposphere exchange(STE) occurs in the COL. The ozone-rich air mass transported from the stratosphere to the troposphere first becomes unstable, then loses its high ozone concentration. This process usually happens during the decay stage of COLs. In order to understand the influence of COLs on the ozone in the UTLS, statistical analysis of the ozone profiles within COLs, and other profiles, are employed. The results indicate that the ozone concentrations of the in-COL profiles are significantly higher than those of the other profiles between ±4 km around the tropopause. The COLs induce an increase in UTLS column ozone by 32% on average. Meanwhile, the COLs depress the lapse-rate tropopause(LRT)/dynamical tropopause height by 1.4/1.7 km and cause the atmosphere above the tropopause to be less stable. The influence of COLs is durable because the increased ozone concentration lasts at least one day after the COL has passed over Changchun. Furthermore, the relative coefficient between LRT height and lower stratosphere(LS) column ozone is-0.62,which implies a positive correlation between COL strength and LS ozone concentration. 相似文献