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冬季乌鲁木齐市低层大气O3垂直分布观测的个例分析 总被引：1，自引：1，他引：0
为了揭示乌鲁木齐冬季边界层O_3垂直分布特征,利用系留气艇于2008年1月11-13日在乌鲁木齐市区进行了边界层O_3观测试验。利用本次观测试验的数据并结合相关气象资料,对观测期间边界层O_3的垂直分布特征及其影响因子进行了分析。结果表明:白天近地面500～800 m高度以下O_3浓度较低,该高度以上存在O_3高浓度分布区,夜间整个观测高度范围内O_3浓度均较低;O_3浓度分布与太阳辐射、温度层结、风、相对湿度等因子密切相关,O_3高浓度分布区出现在逆温层底以上,且O_3浓度与相对湿度呈显著的反相关分布;近地面的NO_x对O_3浓度有着重要影响。由此表明乌鲁木齐冬季低层大气O_3的分布在各种因素的影响下具有明显的时空变化。 相似文献
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利用2007年12月的加密探空资料, 对高原东部及其下游地区的边界层结构和高原东部边界层变化对下游大气的影响进行了分析。结果表明, 冬季青藏高原东部夜间近地面逆温层可以发展到平均500 m的高度, 白天混合层可以发展到平均2000 m的高度。白天混合层内水汽和风速混合十分均匀, 在混合层发展成熟时存在十分深厚的逆湿层。冬季青藏高原下游的四川盆地, 边界层内温度日较差小, 夜间逆温层把大量地表水汽截留在近地层, 日出前近地层水汽容易达到饱和。白天, 混合层在中午发展成熟, 平均高度只有300 m。四川盆地对流层下部存在非常强的逆温层, 该逆温层是青藏高原抬升地表加热和冬季盛行西风气流形成的, 逆温层变化是青藏高原东部边界层温度日变化和局地西风变化的共同结果。逆温层显著改变大气动量、 热量和水汽的垂直分布。与对流层下部逆温相联系的中层云对辐射的影响是造成四川盆地温度日较差和混合层高度变化的原因。 相似文献
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基于旋翼无人机开展大气边界层观测可为气象要素和大气污染物垂直结构的研究提供具有高时空解析能力的新方法,有助于深入理解低层大气物理化学变化机制。本文详述了旋翼无人机在开展大气边界层环境气象垂直观测实验的应用及优势。基于自主研发的旋翼无人机环境气象观测平台,通过开展传感器在无人机上不同的搭载位置,以及旋翼无人机与探空气球、高塔的对比观测实验,明确了旋翼无人机对气象环境观测的影响及合理的搭载方式。研究进一步在湖北重污染天气条件下开展了0—1000 m的大气边界层垂直观测,并研发了基于旋翼无人机姿态数据的大气边界层气象要素及污染物垂直观测的订正方法。结果表明:实验获取了2—10 m垂直分辨率的高质量大气廓线数据,可精细捕捉大气边界层及其逆温层高度和污染物浓度等要素的垂直变化特征。本文旨在为无人机观测的科研应用提供一种技术可行且数据可靠的观测手段。 相似文献
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乌鲁木齐冬季大气边界层温度和风廓线观测研究 总被引：2，自引：0，他引：2
为了进一步认识乌鲁木齐冬季大气边界层的结构特征及其对大气污染的影响,为改进城市空气污染预报和污染治理提供科学依据,利用2008年1月11—13日系留气艇对乌鲁木齐市城区大气边界层过程进行观测试验的资料,分析了观测期间乌鲁木齐风、温廓线和混合层厚度的变化特征,并探讨了大气边界层结构对乌鲁木齐大气污染的影响。结果表明:观测期间乌鲁木齐近地面全天存在悬浮逆温,且有时为多层逆温,大气层结稳定;受逆温层的影响,近地面全天风速都很小,均在4m/s以下,风向随高度变化规律明显;观测期间乌鲁木齐大气混合层厚度平均为274m。乌鲁木齐冬季大气边界层风、温廓线的特征及混合层厚度,对大气污染的影响作用显著,是造成该地区冬季多污染的主要原因之一。 相似文献
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苏州东山冬季大气边界层结构特征及其对污染物浓度的影响 总被引：5，自引：1，他引：5
利用2015年1月15—27日在苏州东山气象观测站系留气艇观测数据以及细颗粒物浓度观测资料,对东山大气边界层结构特征及其对污染物垂直结构分布的影响进行分析研究。结果表明:苏州东山地区冬季空气污染过程的边界层结构演变比较典型,夜间稳定边界层高度约为200 m,白天最大边界层高度可达1 000 m。边界层内污染物垂直结构分布易受边界层高度的影响,较低的大气边界层高度可使细颗粒物在近地层持续累积;反之,边界层高度较高,湍流发展旺盛,颗粒物垂直分布均匀。夜间大气边界层稳定,逆温结构多发,导致近地面出现细颗粒物堆积。风的垂直结构对细颗粒物空间分布也存在显著影响,在风速较小的低空层细颗粒分布较多,而风速较大的中高层的分布较少。 相似文献
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利用先进的WRF中尺度模式中3种边界层参数化方案(YSU、MYJ和ACM2),模拟了2005年1月25~28日兰州市冬季地面温度和风速的变化,并与同期系留探空和自动气象站的实测资料进行了对比分析。结果表明:对兰州冬季大气边界层地面温度日变化的模拟,局地闭合的MYJ方案优于非局地闭合的YSU和ACM2方案;3种方案模拟的夜间位温廓线较好,白天的较差;在边界层低层,考虑局地和非局地闭合的ACM2方案模拟的位温廓线与观测值比较一致;在边界层上部,局地闭合的MYJ方案则更适合于描述大气湍流对位温垂直分布的影响;3种边界层参数化方案模拟的兰州地区冬季温度场空间分布特征相似,但MYJ方案模拟的夜间温度低于YSU和ACM2方案,白天则高于YSU和ACM2方案。 相似文献
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四川盆地作为我国一个特殊的大气气溶胶污染区域,亟待厘清其大气污染时空变化与独特盆地地形影响相关机理。本文综述了近年来一系列相关研究成果,包括:（1）揭示了四川盆地大气环境变化中大地形影响作用,青藏高原东侧区域气溶胶空间分布“避风港”效应,以及大地形热力强迫对盆地空气质量变化的“气候调节”影响; （2）探明了四川盆地大气边界层结构对大气气溶胶变化的影响,冬季重霾期间大气边界层垂直结构变化特征及其相关PM2.5物理化学特性;（3）明晰了大气气溶胶在四川盆地暴雨过程中的重要作用机理,以及四川盆地气溶胶高污染分布导致的降水分布型态的气候变化。这些研究提升了四川盆地气溶胶污染形成机理及大地形对大气环境变化影响效应的科学认识,并表明未来应该深入研究四川盆地地形背景下独特大气边界层结构,人为与自然源排放和环境大气物理-化学过程变化。 相似文献
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复杂地形城市冬季边界层气溶胶扩散和分布模拟 总被引：1，自引：5，他引：1
着眼于城市冬季气溶胶扩散特征问题,针对地形复杂的兰州市及周边地区,开发了WRF模式,使之与包含了大气气溶胶辐射效应和气溶胶粒子扩散的综合大气边界层数值模式嵌套,以模拟城市冬季边界层气溶胶的扩散和分布规律。通过一个个例的模拟结果分析,揭示了兰州冬季气溶胶的扩散分布的如下特征;市区盆地内100 m以下存在东、西两个浓度高值中心,中心值为0.6~3.0 mg.m-3,往上浓度递减,1000 m高度处仅为0.02 mg.m-3。受排放源强、源高、气象场等因素的共同影响,白天盆地内气溶胶浓度随高度和时间的变化强烈,白天浓度随时间最大变化幅度为1.0 mg.m-3。气溶胶输送扩散高度可达到600~800 m,此高度以上浓度值很小。代表性测点上模拟的气溶胶浓度廓线表明,中午浓度达到最高,垂直扩散最强。这些结果与以往的烟雾层高度观测和气溶胶光学厚度观测结果吻合。夜间,盆地内气溶胶浓度随高度和时间的变化减弱,气溶胶输送扩散高度在400~500m,夜间浓度随时间变化平均幅度为0.05 mg.m-3。 相似文献
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This study estimated the largely unstudied downward transport and modification of tropospheric ozone associated with tropical
moist convection using a coupled meteorology-chemistry model. High-resolution cloud resolving model simulations were conducted
for deep moist convection events over West Africa during August 2006 to estimate vertical transport of ozone due to convection.
Model simulations realistically reproduced the characteristics of deep convection as revealed by the estimated spatial distribution
of temperature, moisture, cloud reflectivity, and vertical profiles of temperature and moisture. Also, results indicated that
vertical transport reduced ozone by 50% (50 parts per billion by volume, ppbv) in the upper atmosphere (12–15 km) and enhanced
ozone by 39% (10 ppbv) in the lower atmosphere (<2 km). Field observations confirmed model results and indicated that surface
ozone levels abruptly increased by 10–30 ppbv in the area impacted by convection due to transport by downdrafts from the upper
troposphere. Once in the lower troposphere, the lifetime of ozone decreased due to enhanced dry deposition and chemical sinks.
Ozone removal via dry deposition increased by 100% compared to non-convective conditions. The redistribution of tropospheric
ozone substantially changed hydroxyl radical formation in the continental tropical boundary layer. Therefore, an important
conclusion of this study is that the redistribution of tropospheric ozone, due to deep convection in non-polluted tropical
regions, can simultaneously reduce the atmospheric loading of ozone and substantially impact the oxidation capacity of the
lower atmosphere via the enhanced formation of hydroxyl radicals. 相似文献
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BECAPEX科学试验城市建筑群落边界层大气环境特征及其影响 总被引：9，自引：1，他引：9
20 0 1～ 2 0 0 3年在北京实施了大气边界层动力、热力、化学综合观测试验 (BECAPEX ,BeijingCityAtmosphericPollutionObservationFieldExperiment) ,获取了北京城市大气动力和大气化学三维结构图像。综合观测试验分析研究发现 ,城市区域呈非均匀次生尺度热岛分布 ,并伴随着城市次生尺度环流 ,影响了局地空气污染物分布特征。MODIS卫星遥感 地面观测资料经过变分分析 ,可发现北京城市空气污染与周边区域影响源有密切关系 ,并影响城市群落环境气候特征 ,导致该区域日照、雾日、低云量和能见度呈显著年代际变化趋势。 相似文献
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Summary Numerous tethered balloon soundings which measured meteorological parameters and ozone concentration during the POLLUMET field experiments are investigated. They give indications of the influence of ozone conservation in the nocturnal residual layer (RL) on the development of the near surface ozone concentration of the next day. Mixing down from the RL to the surface is simulated by a simple model based on transilient turbulence theory, using measured profiles as initial values or model verification. The cases investigated show that the ozone mixed down from the RL contributes 50–70% to the maximum concentration near the surface on the following day, the rest coming from chemical production and possibly advection. Various features of exchange characteristics between the RL and the nocturnal boundary layer, (NBL) are described by the analysis of the soundings. It can be shown that the vertical exchange situation during the night can have a considerable influence on the ozone concentration of the following day. 相似文献
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D. H. Lenschow A. C. Delany B. B. Stankov D. H. Stedman 《Boundary-Layer Meteorology》1980,19(2):249-265
A fast-response chemiluminescent ozone sensor was mounted in an aircraft instrumented for air motion and temperature measurements. Measurements of the vertical flux of ozone by the eddy correlation technique were obtained after correcting for time delay and pressure sensitivity in the ozone sensor output. The observations were taken over eastern Colorado for two days in April, one a morning and the other an afternoon flight. Since the correlation coefficient of ozone and vertical velocity is small compared to, for example, temperature and vertical velocity in the lower part of the convective boundary layer, an averaging length of the order of 100 km was required to obtain a reasonably accurate estimate of the ozone flux. The measured variance of ozone appeared to be too large, probably mainly due to random noise in the sensor output, although the possibility of the production of ozone fluctuations by chemical reactions cannot be dismissed entirely. Terms in the budget equation for ozone were estimated from the aircraft measurements and the divergence of the ozone flux was found to be large compared to the flux at the surface divided by the boundary-layer height.Part of this work was carried out while a visitor at Risø National Laboratory, Denmark.The National Center for Atmospheric Research is sponsored by the National Science Foundation. 相似文献
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利用WRF-Chem模式,采用3种边界层参数化方案 (YSU, MYJ和ACM2),针对1个晴空、静稳日 (2013年8月26日20:00—27日20:00(北京时)) 进行模拟,着重分析不同边界层参数化方案对夜间残留层形成及日出前后O3浓度垂直分布形式的模拟效果,并与固城站地面及垂直同步观测资料进行对比。结果表明:3种边界层参数化方案均能够模拟出温度及风速的区域分布形式以及风温垂直结构的变化特征;相比之下,MYJ方案模拟的夜间边界层高度较YSU方案和ACM2方案明显偏高,该对比结果可能是导致近地面污染物浓度模拟差异的重要原因;在夜间稳定层结至日出后稳定状态打破的边界层结构演变过程中,采用YSU方案和ACM2方案模拟的温度和风速垂直扩线形式与观测结果更为接近;同样采用非局地闭合的YSU方案和同时考虑局地和非局地闭合的ACM2方案,对于边界层高度内O3浓度垂直分布形式的模拟效果具有明显优势。 相似文献
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BOUNDARY LAYER GROWTH AND LAPSE RATE CHANGES DETERMINED BY LIDAR AND SURFACE HEAT FLUX IN SOFIA 
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下载免费PDF全文 In this study the results from a boundary layer experiment,conducted in autumn 1991 over a flat,build-up urbanarea in Southeast Sofia,together with some models for mixed layer growth rates are used to investigate the layered struc-ture of the vertical atmospheric stability distribution in the Sofia Valley.Lidar measurements of aerosol layer heightsand morning boundary layer development are combined with surface eddy correlation measurements of kinematic heatand moisture fluxes,profiles of temperature and humidity,wind speed and wind direction.A diagnostic method is pres-ented for determining vertical lapse rates using surface meteorological measurements and lidar returns observed duringthe transition from nighttime stable stratification to daytime convective boundary layer after the sunrise. 相似文献
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BOUNDARY LAYER GROWTH AND LAPSE RATE CHANGES DETERMINED BY LIDAR AND SURFACE HEAT FLUX IN SOFIA* 下载免费PDF全文
下载免费PDF全文 In this study the results from a boundary layer experiment,conducted in autumn 1991 over a flat,build-up urban area in Southeast Sofia,together with some models for mixed layer growth rates are used to investigate the layered structure of the vertical atmospheric stability distribution in the Sofia Valley.Lidar measurements of aerosol layer heights and morning boundary layer development are combined with surface eddy correlation measurements of kinematic heat and moisture fluxes,profiles of temperature and humidity,wind speed and wind direction.A diagnostic method is presented for determining vertical lapse rates using surface meteorological measurements and lidar returns observed during the transition from nighttime stable stratification to daytime convective boundary layer after the sunrise. 相似文献
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利用ACTIVE（aerosol and chemical transport in tropical convection）试验资料,取2006年1月20日澳大利亚北部达尔文岛附近发生的一次飑线强对流天气的AE17航次和2006年1月27日无对流天气的AE21航次飞行路径中的探测资料,对澳大利亚达尔文地区夏季风盛行期间发生的有无强对流发生时O3和CO浓度垂直分布变化进行对比,考察强对流性天气发生对O3和CO浓度垂直输送作用。深对流云内强烈的垂直上升运动将O3和CO等化学气体携带输送至对流层上部并在对流层顶堆积,从而在对流层上部产生浓度峰值。当有强对流发生,飞机进入对流云上层时,O3浓度和CO浓度升高,O3和CO浓度变率增大,在对流层上部浓度出现峰值;当飞机飞出对流云时,O3和CO浓度相对较低,在对流云外出现谷值。在无对流发生的条件下O3和CO浓度相对较小,浓度变率也较小,无峰值产生。分析表明:O3和CO浓度分布不仅与强对流的垂直输送作用关系密切,且与气象要素垂直和水平分布以及动力输送过程密切相关。 相似文献
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Urs Neu 《Boundary-Layer Meteorology》1995,73(1-2):189-193
The reduction of ozone in the nocturnal residual layer by vertical mixing to the surface was investigated for several summer smog episodes on the Swiss plateau in the years 1990 and 1991. Using a limited data set of SODAR measurements and surface ozone concentrations, a parameterization of the ozone depletion in the nocturnal residual layer due to vertical mixing to the ground is proposed. This model is not intended to be physically complete but is rather simple with limited input information required. The nocturnal ozone reduction within the whole planetary boundary layer (nocturnal boundary layer plus residual layer) over the complex terrain of the Swiss plateau for the days investigated is between 20 and 50%. 相似文献