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1.
The formation of three Loop Current Eddies, Ekman, Franklin, and Hadal, during the period April 2009 through November 2011 was observed by an array of moored current meters and bottom mounted pressure equipped inverted echo sounders. The array design, areal extent nominally 89° W to 85° W, 25° N to 27° N with 30–50 km mesoscale resolution, permits quantitative mapping of the regional circulation at all depths. During Loop Current Eddy detachment and formation events, a marked increase in deep eddy kinetic energy occurs coincident with the growth of a large-scale meander along the northern and eastern parts of the Loop Current. Deep eddies develop in a pattern where the deep fields were offset and leading upper meanders consistent with developing baroclinic instability. The interaction between the upper and deep fields is quantified by evaluating the mean eddy potential energy budget. Largest down-gradient heat fluxes are found along the eastern side of the Loop Current. Where strong, the horizontal down-gradient eddy heat flux (baroclinic conversion rate) nearly balances the vertical down-gradient eddy heat flux indicating that eddies extract available potential energy from the mean field and convert eddy potential energy to eddy kinetic energy.  相似文献   

2.
The initial discharge stages of two flashes during the Shandong Artificially Triggering Lightning Experiment (SHATLE) are analyzed based on the synchronous data of the current and close electromagnetic field. For a lightning flash, named 0503, the wire was connected, not electrically, but via a 5 m length of nylon, with the lightning rod; while for another, named 0602, the wire was connected with the rod directly. Results show that the discharge processes of the initial stage (IS) in flash 0503 are quite different from that of the usual classical-triggered flash 0602 and altitude-triggered flashes. A large pulse with a current of about 720 A resulted from the breakdown of the 5 m air gap during flash 0503, and the corresponding electric field at 60 m from the lightning rod was 0.38 kV/m. The upward positive leaders (UPLs) propagated continuously from the tip of the rocket after this breakdown. The geometric mean (GM) of the UPL peak current was 23.0 A. Vaporization of the wire occurred during the initial continuous current (ICC) stage and the largest current pulse was about 400 A. Compared with triggered flash 0503, the discharge processes of IS in flash 0602 were simple, only two large pulses similar to each other occurred before dart leader/return stroke sequences. The peak current of the first pulse was 2.1 kA and its corresponding electric field and magnetic field at a distance of 60 m from the lightning rod were 0.98 kV/m and 7.03 μT, respectively. During the second pulse, the wire disintegrated. The current decreased to the background level at the moment of the wire disintegration. The current of the second pulse in triggered flash 0602 was 2.8 kA, and the corresponding electric field and magnetic field at 60 m from the lightning rod were 1.22 kV/m and 9.01 μT, respectively.  相似文献   

3.
A mooring equipped with 200 high-resolution temperature sensors between 6 and 404 m above the bottom was moored in 1890 m water depth above a steep, about 10° slope of Mount Josephine, NE-Atlantic. The sensors have a precision of less than 0.5 mK. They are synchronized via induction every 4 h so that the 400 m range is measured to within 0.02 s, every 1 s. Thin cables and elliptical buoyancy assured vertical mooring motions to be smaller than 0.1 m under maximum 0.2 m s−1 current speeds. The local bottom slope is supercritical for semidiurnal internal tides by a factor of two. Exploring a one-month record in detail, the observations show: 1/semidiurnal tidal dominance in variations of dissipation rate ε, eddy diffusivity Kz and temperature, but no significant correlation between the records of ε and total kinetic energy, 2/a variation with time over four orders of magnitude of 100-m vertically averaged ε, 3/a local minimum in density stratification between 50 and 100 m above the bottom, 4/a gradual decrease in daily or longer averaged ε and Kz by one order of magnitude over a vertical distance of 250 m, upwards from 150 m above the bottom, 5/monthly mean values of <[ε]> = 2 ± 0.5 × 10−7 m2 s−3, <[Kz]> = 8 ± 3 × 10−3 m2 s−1 averaged over the lower 150 m above the bottom.  相似文献   

4.
Below-cloud aerosol scavenging is generally estimated from field measurements using advanced instruments that measure changes in aerosol distributions with respect to rainfall. In this study, we discuss various scavenging mechanisms and scavenging coefficients from past laboratory and field measurements. Scavenging coefficients derived from field measurements (representing natural aerosols scavenging) are two orders higher than that of theoretical ones for smaller particles (Dp < 2 μm). Measured size-resolved scavenging coefficients can be served as a better option to the default scavenging coefficient (e.g. a constant of 10?4 s?1 for all size of aerosols, as used in the CALPUFF model) for representing below-cloud aerosol scavenging. We propose scavenging correction parameter (CR) as an exponential function of size-resolved scavenging coefficients, winds and width in the downwind of the source–receptor system. For a wind speed of 3 m s?1, CR decrease with the width in the downwind for particles of diameters Dp < 0.1 μm but CR does not vary much for particles in the accumulation mode (0.1 < Dp < 2 μm). For a typical urban aerosol distribution, assuming 3 m s?1 air-flow in the source–receptor system, 10 km downwind width, 2.84 mm h?1 of rainfall and using aerosol size dependent scavenging coefficients in the CR, scavenging of aerosols is found to be 16% in number and 24% in volume of total aerosols. Using the default scavenging coefficient (10?4 s?1) in the CALPUFF model, it is found to be 64% in both number and volume of total aerosols.  相似文献   

5.
This study incorporates observations from Array of Real-time Geostrophic Oceanography (ARGO) floats and surface drifters to identify seasonal circulation patterns at the surface, 1000 m, 1500 m, and 2000 m in the northwest Indian Ocean, and quantify velocities associated with them. A skill comparison of the Simple Ocean Data Assimilation (SODA) reanalysis output was also performed to contribute to the understanding of the circulation dynamics in this region.Subsurface currents were quantified and validated using the ARGO float data. Surface currents were identified using surface drifter data and compared to the subsurface observations to enhance our previous understanding of surface circulations. Quantified Southwest Monsoon surface currents include the Somali Current (vmax = 179.5 cm/s), the East Arabian Current (vmax = 52.3 cm/s), and the Southwest Monsoon Current (vmax = 51.2 cm/s). Northeastward flow along the Somali coast is also observed at 1000 m (vmax = 26.1 cm/s) and 1500 m (vmax = 12.7 cm/s). Currents associated with the Great Whirl are observed at the surface (vmax = 161.4 cm/s) and at 1000 m (vmax = 16.2 cm/s). In contrast to previous studies, both ARGO and surface drifter data show the Great Whirl can form as early as the boreal Spring intermonsoon, lasting until the boreal Fall intermonsoon. The Arabian Sea exhibits eastward/southeastward flow at the surface, 1000 m, 1500 m, and 2000 m. Quantified Northeast Monsoon surface currents include the Somali Current (vmax = 97.3 cm/s), Northeast Monsoon Current (vmax = 30.0 cm/s), and the North Equatorial Current (vmax = 28.5 cm/s). Southwestward flow along the Somali coast extends as deep as 1500 m.Point-by-point vector and scalar correlations of SODA output to ARGO and surface drifter data showed that surface SODA output and surface drifter data generally produced a strong correlation attributed to surface currents strongly controlled by the monsoons, while subsurface correlations of SODA output and ARGO were mostly insignificant due to variability associated with intermonsoonal transitions. SODA output produced overall smaller velocities than both observational datasets. Assimilating ARGO velocities into the SODA reanalysis could improve subsurface velocity assimilation, especially during the boreal fall and spring when ARGO observations suggest that flow is highly variable.  相似文献   

6.
This paper presents a set of technically feasible multi-gas emission pathways (envelopes) for stabilising greenhouse gas concentration at 450, 550 and 650 ppm CO2-equivalent and their trade-offs between direct abatement costs and probabilities to meet temperature targets. There are different pathways within the envelope. Delayed response pathways initially follow the upper boundary of the emission envelope and reduce more by the end of the century. In contrast, early action pathways first follow the lower boundary and then the upper boundary. The latter require an early peak in the global emissions but keeps the option open for shifting to lower concentration targets in the future. Costs evaluations depend on the discount rate. Early action profiles have high costs early on, but learning-by-doing and smoother reduction rates over time lead to in most cases to lower costs across the century (net present value (NPV)). To achieve the 450 ppm CO2-equivalent, the global emissions need to peak before 2020. The NPV of costs increase from 0.2% of cumulative gross domestic product to 1.0% as the shift is made from 650 to 450 ppm (discount rate 5%). However, the chances of limiting global mean warming to 2 °C above pre-industrial levels are very small for peaking and stabilisation at 650 ppm (1–23%) and 550 ppm (1–48%), but increase for a peaking at 510 ppm with subsequent stabilisation 450 ppm to 14–67%.  相似文献   

7.
This work analyzes some physical and microphysical properties of Mesoscale Convective Systems (MCSs) and cloud-to-ground lightning. Satellite data from the GOES-10 infrared and NOAA-18 and TRMM microwave channels and lightning information from the Brazilian lightning detection network (BrasilDAT) were utilized for the period from 2007 to 2009. Based on an automatic MCSs detection method, 720 MCSs life cycles were identified during the period and in the region of study, with a lightning detection efficiency of over 90%. During the diurnal cycle, maximum electrical activity occurred close to the time of maximum convective cloud fraction (18 UTC), and 3 h after the maximum normalized area expansion rate. Diurnal cycles of both properties were modulated by diurnal heating, and thus could be used to monitor diurnal variability of lightning occurrence. The electrical activity was more intense for the widest (Pearson’s correlation of 0.96) and deeper (Pearson’s correlation of 0.84) clouds, which reached 390 km size and 17 km maximum cloud top height. Area growth during the initial phase of MCSs exerted a strong influence on their size and duration, and thus also showed a potential for defining the possibility of electrical activity during their life cycle. The average lightning life cycle exhibited a maximum close to MCSs maturation, while the maximum average lightning density occurred in the MCSs initial life cycle stage. The growth rate of electrical activity during the early stages can indicate the strength of convection and the possible duration of systems with lightning occurrence. Strong condensation processes and mass flux during the growth phase of the systems can provide favorable conditions for cloud electrification and lightning occurrence. A comparison of high microwave frequencies with lightning data showed a strong relationship of vertically integrated ice content and particle size with lightning occurrence, with Pearson's correlation of 0.86 and 0.96, respectively. The polarization difference in the 85 GHz channel showed that electrical activity increases linearly with polarization reduction, associated with a high value of Pearson's correlation coefficient (above 0.90). This suggests that regions with more intense electrical activity are predominantly located in areas with a high concentration of larger ice particles that are vertically oriented, due to the existence of intense updrafts and the electric field. These results demonstrate the potential use of thermodynamic, dynamic and microphysical characteristics for analyzing thunderstorms severity, and as additional information for nowcasting and monitoring electrical activity over large regions that lack ground-based lightning sensors.  相似文献   

8.
Mixing states of cloud interstitial particles between water-soluble and insoluble materials apparently differ under various cloud-forming conditions. To study the mixing states of cloud interstitial particles, we made observations at Mt. Tateyama, Japan (2300 m a.s.l.) during June 2007 using fog (> 10 μm)-cut inlets. Number concentrations of dried particles (0.3–0.5 μm diameter) selected for less-grown (LG) particles (particles smaller than 0.56 μm diameter at 88% relative humidity) were used to quantify tendencies of the growth characteristics of cloud interstitial particles. Size-segregated soot mass concentrations (< 0.4 and < 1.1 μm) were also measured for cloud interstitial particles. Three samples of cloud interstitial LG particles at 88% RH were investigated for water-soluble and insoluble components using dialysis (extraction) of water-soluble materials with transmission electron microscopy (TEM). For one TEM sample with high fractions of the LG particles and high soot mass concentrations under high precipitation (2–6 mm/h), most particles (0.1–0.5 μm) were found to be water insoluble. More than half of the water-insoluble particles were considered to be soot particles showing chain aggregations of electron-opaque spherules. Regarding the other two TEM samples with low fractions of the LG particles under less intense precipitation (ca. 1 mm/h), most particles were partly water soluble. The scavenging process in the precipitating cloud can change the population of particles left behind, preferentially leaving insoluble particles according to cloud formation conditions.  相似文献   

9.
基于三维时域有限差分数值算法（3D-FDTD）建立了雷击高建筑物电磁场传播模型,研究了负地闪击中不同高度建筑物时回击垂直电场、角向磁场以及水平电场沿地表的传播规律。模拟结果表明:建筑物的高度对雷电电场峰值的影响显著,如当建筑物高度从100 m增加至600 m时,在距离d=100 m位置的垂直电场峰值减小了63%,水平电场正极性峰值的增加比例为84%、负极性峰值的绝对值增加比例高达130%;观测位置不变时,角向磁场峰值和水平电场正极性峰值均会随着建筑物高度的增加而增大;对于距离d=100 m,300 m时,垂直电场的峰值随着建筑物高度的增加而减小,而d=500 m时,垂直电场峰值随着建筑物高度的增加呈现出先增大后减小的趋势;此外,建筑物高度会影响垂直电场峰值对距离的敏感程度,建筑物越低（高）,相应的垂直电场峰值随着观测距离增大衰减越快（慢）。该文研究结果能够为现代化城市中高建筑物附近线缆、室外设备等的雷电防护方案设计提供参考。  相似文献   

10.
In this study, total suspended particles (TSP) and size-segregated atmospheric aerosol samples were measured on Qianliyan Island in the Yellow Sea in spring (April–May), summer (July–August) and fall (October–November) of 2006 and in water (January–February) of 2007. The mass concentration of the TSP varied from 75.6 to 132.0 μg/m3. The average concentration were 9.37 ± 7.56 μg/m3 and 5.32 ± 4.25 μg/m3 for nitrate and ammonium in the TSP, respectively. TSP concentration showed a significant correlation with those of nitrate (n = 27, r = 0.73) and ammonium (n = 27, r = 0.60). The mass-size distribution of atmospheric particles exhibited two modes with an accumulation mode at 0.43–1.1 μm and a coarse mode at 3.3–4.7 μm throughout the sampling months. A bi-modal size distribution of nitrate in concentration occurred in the April–May, October–November and January–February, but a uni-modal size distribution occurred in the August. The uni-modal size distribution of ammonium at 0.43–0.65 μm was observed throughout the sampling months. The average of inorganic nitrogen in mass concentration accounted for 4.0% of the total mass of aerosol particles while ammonium-N was the dominant fraction of TIN (Total Inorganic Nitrogen), contributing to 62–71% of the TIN.  相似文献   

11.
A new methodology is proposed to estimate the strength of the South Atlantic Anticyclone (SAA), using the gridded sea level pressure (SLP) of the National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) Reanalysis data. The top quartile (1017.3 hPa) of the SLP data was found a reasonable criterion to delimit the SAA area. Consequently, we defined the SAA area as the quadrangle containing 80% of the observations with pressure >1017.3 hPa. In this quadrangle, an area weighted pressure gradient (AWPG) was computed for the whole area and for the north–south and west–east halves. When compared with maximum pressure, the AWPG showed a better correlation with the significant wave height (SWH) and wind speed (WS) derived from altimetry. The mean value of the AWPG was 8 × 10−4 Pa/m, with representative values of 9.1 × 10−4 Pa/m and 7.4 × 10−4 Pa/m for austral winter and summer, respectively. The phase difference between the monthly AWPG in the north and south sub-quadrangles accounts for the evolution of the spatial pattern of the anticyclone throughout a year. This quantitative approach proved to be a useful estimate of the strength of South Atlantic Anticyclone. Further improvements of this approach are discussed.  相似文献   

12.
The character of turbulent overturns in a weakly stratified deep-sea is investigated in some detail using 144 high-resolution temperature sensors at 0.7 m intervals, starting 5 m above the bottom. A 9-day, 1 Hz sampled record from the 912 m depth flat-bottom (<0.5% bottom-slope) mooring site in the central-north Alboran Sea (W-Mediterranean) demonstrates an overall conservative temperature range of only 0.05 °C, a typical mean buoyancy period as large as 3 h and a 1 Hz-profile-vertically-averaged turbulence dissipation rate maximum of only 10−8 m2 s−3. Nonetheless, this ‘boundary layer’ varies in height between <6 and >104 m above the bottom and is thus not homogeneous throughout; the temperature variations are seldom quiescent and are generally turbulent in appearance, well exceeding noise levels. The turbulence character is associated with small-scale internal waves; examples are found of both shear- and convection-driven turbulence; particular association, although not phase-locked, is found between turbulence variations and tidal rather than with inertial motions; the mean buoyancy frequency of a few times the inertial frequency implies the importance of ‘slantwise convection’ in the direction of the earth rotational vector rather than in the direction of gravity. Such convection is observed both in near-homogeneous and weakly stratified form.  相似文献   

13.
This study presents an analysis of a severe weather case that took place during the early morning of the 2nd of November 2008, when intense convective activity associated with a rapidly evolving low pressure system affected the southern coast of Catalonia (NE Spain). The synoptic framework was dominated by an upper level trough and an associated cold front extending from Gibraltar along the Mediterranean coast of the Iberian Peninsula to SE France, which moved north-eastward. South easterly winds in the north of the Balearic Islands and the coast of Catalonia favoured high values of 0–3 km storm relative helicity which combined with moderate MLCAPE values and high shear favoured the conditions for organized convection. A number of multicell storms and others exhibiting supercell features, as indicated by Doppler radar observations, clustered later in a mesoscale convective system, and moved north-eastwards across Catalonia. They produced ground-level strong damaging wind gusts, an F2 tornado, hail and heavy rainfall. Total lightning activity (intra-cloud and cloud to ground flashes) was also relevant, exhibiting several classical features such as a sudden increased rate before ground level severe damage, as discussed in a companion study. Remarkable surface observations of this event include 24 h precipitation accumulations exceeding 100 mm in four different observatories and 30 minute rainfall amounts up to 40 mm which caused local flash floods. As the convective system evolved northward later that day it also affected SE France causing large hail, ground level damaging wind gusts and heavy rainfall.  相似文献   

14.
Identifying the sources of reactive nitrogen (N) and quantifying their contributions to groundwater nitrate concentrations are critical to understanding the dynamics of groundwater nitrate contamination. Here we assessed groundwater nitrate contamination in China using literature analysis and N balance calculation in coupled human and natural systems. The source appointment via N balance was well validated by field data via literature analysis. Nitrate was detected in 96% of groundwater samples based on a common detection threshold of 0.2 mg N L?1, and 28% of groundwater samples exceeded WHO's maximum contaminant level (10 mg N L?1). Groundwater nitrate concentrations were the highest beneath industrial land (median: 34.6 mg N L?1), followed by urban land (10.2 mg N L?1), cropland (4.8 mg N L?1), and rural human settlement (4.0 mg N L?1), with the lowest found beneath natural land (0.8 mg N L?1). During the period 1980–2008, total reactive N leakage to groundwater increased about 1.5 times, from 2.0 to 5.0 Tg N year?1, in China. Despite that the contribution of cropland to the total amount of reactive N leakage to groundwater was reduced from 50 to 40% during the past three decades, cropland still was the single largest source, while the contribution from landfill rapidly increased from 10 to 34%. High reactive N leakage mainly occurred in relatively developed agricultural or urbanized regions with a large population. The amount of reactive N leakage to groundwater was mainly driven by anthropogenic factors (population, gross domestic product, urbanization rate and land use type). We constructed a high resolution map of reactive N source appointment and this could be the basis for future modeling of groundwater nitrate dynamics and for policy development on mitigation of groundwater contamination.  相似文献   

15.
Concentrations and flux densities of methane were determined during a Lagrangian study of an advective filament in the permanent upwelling region off western Mauritania. Newly upwelled waters were dominated by the presence of North Atlantic Central Water and surface CH4 concentrations of 2.2 ± 0.3 nmol L−1 were largely in equilibrium with atmospheric values, with surface saturations of 101.7 ± 14%. As the upwelling filament aged and was advected offshore, CH4 enriched South Atlantic Central Water from intermediate depths of 100–350 m was entrained into the surface mixed layer of the filament following intense mixing associated with the shelf break. Surface saturations increased to 198.9 ± 15% and flux densities increased from a mean value over the shelf of 2.0 ± 1.1 μmol m−2 d−1 to a maximum of 22.6 μmol m−2 d−1. Annual CH4 emissions for this persistent filament were estimated at 0.77 ± 0.64 Gg which equates to a maximum of 0.35% of the global oceanic budget. This raises the known outgassing intensity of this area and highlights the importance of advecting filaments from upwelling waters as efficient vehicles for air-sea exchange.  相似文献   

16.
中国气象局雷电野外科学试验基地开展的人工触发闪电试验是研究闪电电磁辐射效应的有效手段,利用架设在试验场地周边的多套磁场天线所获取的高灵敏度磁场数据,针对初始连续电流阶段的中低频磁场特征开展研究。得益于磁场天线带宽的拓展,首次解析出了相对平静期内的磁场脉冲,单个脉冲的平均宽度约为1 μs,平均脉冲间隔约为14 μs,对应了该阶段中上行先导的小尺度击穿发展形式;在近、远距离磁场测量中均观测到了与先导通道头部击穿放电相关的爆发式磁场脉冲,其平均脉冲间隔(约为24.5 μs)明显大于平静期脉冲的统计值,而且在爆发式脉冲期间通道底部电流逐步增大到几十至上百安培,表明此时电场条件更加有利于上行先导的发展;此外,高灵敏磁场天线能够直观地呈现出初始连续电流脉冲(initial continuous current pulse,ICCP)的电荷传输过程,且ICCP期间观测到的规则磁场脉冲的脉冲间隔比其他类型的磁场脉冲小一个量级,可能体现了正极性击穿和负极性击穿的特征差异。  相似文献   

17.
Rainfall characteristics of the Madden–Julian oscillation (MJO) are analyzed primarily using tropical rainfall measuring mission (TRMM) precipitation radar (PR), TRMM microwave imager (TMI) and lighting imaging sensor (LIS) data. Latent heating structure is also examined using latent heating data estimated with the spectral latent heating (SLH) algorithm.The zonal structure, time evolution, and characteristic stages of the MJO precipitation system are described. Stratiform rain fraction increases with the cloud activity, and the amplitude of stratiform rain variation associated with the MJO is larger than that of convective rain by a factor of 1.7. Maximum peaks of both convective rain and stratiform rain precede the minimum peak of the outgoing longwave radiation (OLR) anomaly which is often used as a proxy for the MJO convection. Stratiform rain remains longer than convective rain until ∼4000 km behind the peak of the mature phase. The stratiform rain contribution results in the top-heavy heating profile of the MJO.Associated with the MJO, there are tri-pole convective rain top heights (RTH) at 10–11, ∼7 and ∼3 km, corresponding to the dominance of afternoon showers, organized systems, and shallow convections, respectively. The stratiform rain is basically organized with convective rain, having similar but slightly lower RTH and slightly lags the convective rain maximum. It is notable that relatively moderate (∼7 km) RTH is dominant in the mature phase of the MJO, while very tall rainfall with RTH over 10 km and lightning frequency increase in the suppressed phase. The rain-yield-per flash (RPF) varies about 20–100% of the mean value of ∼2–10 × 109 kg fl−1 over the tropical warm ocean and that of ∼2–5 × 109 kg fl−1 over the equatorial Islands, between the convectively suppressed phase and the active phase of MJO, in the manner that RPF is smaller in the suppressed phase and larger in the active phase.  相似文献   

18.
In August 2009, Typhoon Morakot caused massive flooding and devastating mudslides in the southern Taiwan triggered by extremely heavy rainfall (2777 mm in 4 days) which occurred during its passage. It was one of the deadliest typhoons that have ever attacked Taiwan in recent years. In this study, numerical simulations are performed for the storm surge and ocean surface waves, together with dynamic meteorological fields such as wind, pressure and precipitation induced by Typhoon Morakot, using an atmosphere–waves–ocean integrated modelling system. The wave-induced dissipation stress from breaking waves, whitecapping and depth-induced wave breaking, is parameterized and included in the wave–current interaction process, in addition to its influence on the storm surge level in shallow water along the coast of Taiwan. The simulated wind and pressure field captures the characteristics of the observed meteorological field. The spatial distribution of the accumulated rainfall within 4 days, from 00:00 UTC 6 August to 00:00 UTC 10 August 2009, shows similar patterns as the observed values. The 4-day accumulated rainfall of 2777 mm at the A-Li Shan mountain weather station for the same period depicted a high correlation with the observed value of 2780 mm/4 days. The effects of wave-induced dissipation stress in the wave–current interaction resulted in increased surge heights on the relatively shallow western coast of Taiwan, where the bottom slope of the bathymetry ranges from mild to moderate. The results also show that wave-breaking has to be considered for accurate storm surge prediction along the east coast of Taiwan over the narrow bank of surf zone with a high horizontal resolution of the model domain.  相似文献   

19.
The samples of water-soluble inorganic ions (WSIs), including anions (F?, Cl?, SO42?, NO3?) and cations (NH4+, K+, Na+, Ca2+, Mg2+) in 8 size-segregated particle matter (PM), were collected using a sampler (with 8 nominal cut-sizes ranged from 0.43 to 9.0 μm) from October 2008 to September 2009 at five sites in both polluted and background regions of a coastal city, Xiamen. The results showed that particulate matters in the fine mode (PM2.1, Dp < 2.1 μm) comprised large part of mass concentrations of aerosols, which accounted for 45.56–51.27%, 40.04–60.81%, 42.02–60.81%, and 40.46–57.07% of the total particulate mass in spring, summer, autumn, and winter, respectively. The water-soluble ionic species in the fine mode at five sampling sites varied from 15.33 to 33.82 (spring), 14.03 to 28.06 (summer), 33.47 to 72.52 (autumn), and 48.39 to 69.75 μg m? 3 (winter), respectively, which accounted for 57.30 ± 6.51% of the PM2.1 mass concentrations. Secondary pollutants of NH4+, SO42? and NO3? were the dominant contributors of WSIs, which suggested that pollutants from anthropogenic activities, such as SO2, NOx were formed in aerosols by photochemical reactions. The size distributions of Na+, Cl?, SO42? and NO3? were bimodal, peaking at 0.43–0.65 μm and 3.3–5.8 μm. Although some ions, such as NH4+ presented bimodal distributions, the coarse mode was insignificant compared to the fine mode. Ca2+ and Mg2+ exhibited unimodal distributions at all sampling sites, peaking at 2.1–3.3 μm, while K+ having a bimodal distributions with a major peak at 0.43–0.65 μm and a minor one at 3.3–4.7 μm, were used in most of samples. Seasonal and spatial variations in the size-distribution profiles suggested that meteorological conditions (seasonal patterns) and sampling locations (geographical patterns) were the main factors determining the formation of secondary aerosols and characteristics of size distributions for WSIs.  相似文献   

20.
The Water vapour Strong Lines at 183 GHz (183-WSL) fast retrieval method retrieves rain rates and classifies precipitation types for applications in nowcasting and weather monitoring. The retrieval scheme consists of two fast algorithms, over land and over ocean, that use the water vapour absorption lines at 183.31 GHz corresponding to the channels 3 (183.31 ± 1 GHz), 4 (183.31 ± 3 GHz) and 5 (183.31 ± 7 GHz) of the Advanced Microwave Sounding Unit module B (AMSU-B) and of the Microwave Humidity Sounder (MHS) flying on NOAA-15-18 and Metop-A satellite series, respectively.The method retrieves rain rates by exploiting the extinction of radiation due to rain drops following four subsequent steps. After ingesting the satellite data stream, the window channels at 89 and 150 GHz are used to compute scattering-based thresholds and the 183-WSLW module for rainfall area discrimination and precipitation type classification as stratiform or convective on the basis of the thresholds calculated for land/mixed and sea surfaces. The thresholds are based on the brightness temperature difference Δwin = TB89 ? TB150 and are different over land (L) and over sea (S): cloud droplets and water vapour (Δwin < 3 K L; Δwin < 0 K S), stratiform rain (3 K < Δwin < 10 K L; 0 K < Δwin < 10 K S), and convective rain (Δwin > 10 K L and S). The thresholds, initially empirically derived from observations, are corroborated by the simulations of the RTTOV radiative transfer model applied to 20000 ECMWF atmospheric profiles at midlatitudes and the use of data from the Nimrod radar network. A snow cover mask and a digital elevation model are used to eliminate false rain area attribution, especially over elevated terrain. A probability of detection logistic function is also applied in the transition region from no-rain to rain adjacent to the clouds to ensure continuity of the rainfall field. Finally, the last step is dedicated to the rain rate retrieval with the modules 183-WSLS (stratiform) and 183WSLC (convective), and the module 183-WSL for total rainfall intensity derivation.A comparison with rainfall retrievals from the Goddard Profiling (GPROF) TRMM 2A12 algorithm is done with good results on a stratiform and hurricane case studies. A comparison is also conducted with the MSG-based Precipitation Index (PI) and the Scattering Index (SI) for a convective-stratiform event showing good agreement with the 183-WSLC retrieval. A complete validation of the product is the subject of Part II of the paper.  相似文献   

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