首页 | 本学科首页   官方微博 | 高级检索  
相似文献
 共查询到20条相似文献，搜索用时 109 毫秒
1.
The article presents the results of lithological and geochemical investigations of recent sediments of Lake Pusty Staw. The analysed sediments document about 300 years of the history of this lake. Historical materials indicate that significant changes in the catchment of the lake took place from the beginning of the 18th century (deforestation and afforestation) followed by 19th century tourist development, and 20th century industrialisation. The sediments were dated using the 210Pb and 137Cs method and core lithology. These made it possible to establish a reliable chronology to the year 1730. The calculated sedimentation rates ranged between 0.17 and 0.83 cm year–1. There was a period of intensified erosion caused by land clearance between 1734 and 1810, which resulted in an acceleration in sedimentation rate (0.36 cm year–1) and a change of lithological type of sediment from detritus gyttja to clayey gyttja. On the basis of Cu, Zn, Cd and Pb content in the sediments, it was determined that the beginning of pollution of the lake dates back to the 19th century and was caused probably by the existence of a health resort. A systematic increase in pollution occurred in the 20th century as a result of industrial plants. Normalised with respect to Al, the content of heavy metals in polluted sediments was from several to twenty times higher than in sediments of the preindustrial period, and a comparison of historical materials with changes of sediments in most cases made it possible to identify the direct causes of the increase in pollution.  相似文献   

2.
Paleolimnological techniques for assessing recent drainage basin disturbance are evaluated in three Moroccan lakes with catchments contrasted in terms of land-use and vegetation. Rates of sediment accumulation in the two lakes with agricultural catchments were relatively high (>1.6 cm yr-1) in the most recent past. Dilution effects prevented core dating by the 210Pb method alone and post-1953 chronologies were constructed by combining 210Pb and 137Cs data. The recent sediment accumulation rate at the currently least disturbed site, where natural Cedrus forest is still abundant, was relatively low (<0.4 cm yr-1) but has increased since the mid-19th century.Magnetic, geochemical, pollen, and diatom studies of all three lake sediment cores linked with modern field survey data show that soil erosion in the most vegetationally disturbed catchment (Dayat-er-Roumi) has been high throughout the recent past and that intensity peaks are probably associated with wetland drainage operations beginning in the 1940's. At the partially forested site (Dayat Affougah), pre-1950's woodland clearance and other land-use changes are the likely cause of past major soil erosion episodes. The site currently dominated by natural Cedrus forest (Lac Azigza) shows only minor disturbance during the past c. 150 years although a major soil erosion episode occrred in the 17th century.Paleolimnological analysis has clearly demonstrated that major landscape change has occurred at all three sites. However, only at the two sites with catchment cultivation do previously accelerated soil erosion and lake sediment accumulation rates persist to the present. Information essential for formulation of appropriate management plans is presented and the importance of paleolimnology in assessing man-induced lake-catchment disturbance is stressed.  相似文献   

3.
Phosphorus accumulation rates in depositional zone sediments of Lake Okeechobee were determined in 11 mud-zone cores and two peat-zone cores dated by 210Pb. Although difficulties were encountered in interpreting 210Pb data from some sites, reliable dating of sediments from the mud zone of this shallow lake is possible. Sediment accumulation rates in this zone have increased during the present century by an average of about twofold, and accumulation of organic sediments in the lake during pre-settlement times apparently was much slower than during the past century. Concentrations of all forms of sedimentary P but especially nonapatite inorganic-P and organic-P also have increased since pre-settlement times and especially since about 1940. Annual P accumulation rates in the lake's sediments have increased about fourfold during the 1900s, with most of the increase occurring in the past 40–50 years. The recent accumulation rate of sedimentary P (past ~ 10 years) agrees within a factor of 1.5 with the net retention of P in the lake calculated from published input-output mass balances.  相似文献   

4.
Sediment sequences spanning the last 800 years from two small lakes in the south Swedish uplands were explored for assessment of effects of changing human population, local land-use practices and airborne pollution on lake-ecosystem functioning and resilience. Variations in nutrient cycling and deposition of lithogenic elements were studied, using a multi-proxy stratigraphic approach. Carbon and nitrogen elemental and isotopic analyses were applied in combination with records of hydrocarbons (n-alkanes) to investigate the sources and depositional conditions of sediment organic matter. Changes in fluvial and airborne delivery of inorganic matter were based on X-ray fluorescence measurements. The results reveal that population growth and related increases in land-use pressure had a major impact on catchment erosion and input of terrestrial organic matter to the lakes from the 1500s to the end of the 1800s. Evidence also exists of a brief period of catchment disturbance at ca. 1200–1300, followed by recovery, likely connected to the Black Death pandemic. At ca. 1900 synchronous shifts in most of the proxy records suggest a marked change in external forcing common to the two lakes related to a major decrease in population density and the introduction of modern forestry following the industrial revolution. Interestingly, the two sediment records exhibit generally coherent trends in C/N ratio, organic C content and δ13C, both before and after 1900, indicating broadly similar sensitivities of the lake ecosystems to human impact. In contrast, deviating trends in total N content, δ15N and lithogenic element concentrations (K, Ti, Rb and Zr) reflect site-specific responses to local disturbances during the last century due to different nutrient conditions and catchment properties. Our companion sediment records highlight the importance of understanding long-term human impact on watersheds and demonstrate how regional versus local forcing of lake ecosystems, as well as site-specific responses related to catchment characteristics can be reconstructed.  相似文献   

5.
A combined mineral magnetic and scaled chrysophyte study of lake sediments from Lake Lacawac and Lake Giles in northeastern Pennsylvania was conducted to determine the effects of land-use and sediment source changes on the variation of pH, conductivity, and alkalinity inferred from biotic changes. Ten 30–40 cm long gravity cores were collected from Lake Lacawac and three from Lake Giles. Isothermal remanent magnetizations (IRMs) were given to the lake sediments in a 1.3 T magnetic field to measure magnetic mineral concentration variations. IRM acquisition experiments were conducted to identify magnetic mineralogy. The bedrock, soils and a peat bog on the shores of Lake Lacawac were also sampled for magnetic analysis to determine possible lake sediment sources. The top 10 cm of sediment collected from Lakes Lacawac and Giles was two to four times more magnetic than deeper sediment. 210Pb dating suggests that this intensity increase commenced circa 1900. SEM images of magnetic extracts from the highly magnetic sediments indicates the presence of magnetic fly ash microspheres from fossil fuel burning electric power generation plants. The similarity in magnetic coercivity in the top 8 cm lake sediments and in the peat bog supports an atmospheric source for some of the magnetic minerals in the youngest lake sediments. The highly magnetic sediments also contain an antiferromagnetic mineral in two cores closest to Lake Lacawacs southeastern shore. This magnetic mineral is only present deep in the soil profile and would suggest erosion and significant land-use changes in the Lacawac watershed as another cause for the high magnetic intensities (concentrations) in the top 10 cm of the lake sediments. The most significant changes in the scaled chrysophyte flora occurred immediately above the 10 cm level and were used to infer a doubling of the specific conductivity between circa 1910 and 1929. These variations also support land-use changes in the Lacawac catchment at this time. A similar shift in the scaled chrysophte flora was not observed in the top of Lake Giles, however, distinct changes were found in the deeper sections of the core coupled with a smaller peak in magnetic concentration. Fourier analysis of the 210Pb-dated lake sediment magnetics indicates the presence of a 50 year period, low amplitude variation in the Lake Lacawac, Lake Giles, and Lake Waynewood (Lott et al., 1994) magnetic concentration records. After removal of the land-use/fly ash magnetic concentration peak by Gaussian filtering, the 50 year variation correlates strongly from lake to lake even though the lakes are in different watersheds separated by up to 30 km. When this magnetic variation is compared with Gaussian-filtered rainfall variations observed in New York City and Philadelphia over the past 120–250 years there is a strong correlation suggesting that magnetic concentration variations can record regional rainfall variations with an approximately 50 year period. This result indicates that magnetics could be used to document regional variations in climatic change.  相似文献   

6.
赣北黄茅潭湖泊沉积记录的240年以来古洪水事件   总被引：1，自引：1，他引：0  
古洪水研究是近几十年来全球变化研究的一个热点,同时也是难点。本文利用赣北黄茅潭的湖泊沉积,建立了小冰期以来全球变暖背景下的区域洪水记录。采用210Pb和137Cs方法厘定了地层年代,基于粒度与元素地球化学指标的对比分析,揭示了器测记录(1950年)以来指标记录的特点与区域日降水超过50 mm天数的关系,认为黄茅潭HMT-01孔粒度(包括粗粉砂+砂/粘土比值、平均粒径)和Zr/Rb、Ti/Rb、Zr/Fe比值可作为洪水指标记录,共识别出1950-2010年期间记载的13次洪水事件中的11次。基于这些指标记录及指标特点,共识别1769-1950年间由历史文献记录的31次洪水事件中的23次,识别率达74.2%。研究表明：①湖泊沉积中Zr/Rb、Ti/Rb、Zr/Fe比值和粒度参数(平均粒径、粗粉砂+砂/粘土)作为洪水指标,对洪水事件沉积有较好的指示作用,且Zr/Rb比值对洪水事件的检出率较高;②黄茅潭流域洪水发生频率暖期高于冷期;③年代际尺度上,1820s-1840s,1860s-1870s为19世纪冷期黄茅潭洪水高频期,这两个阶段对应东亚夏季风偏强,长江中下游地区降雨较多;20世纪赣北黄茅潭洪水基本随1920s-1940s,1980s-1990s两个变暖阶段而高频出现,与长江中下游大洪水演变特点基本一致。研究结果为利用湖泊沉积记录反演过去的洪水变化,延长洪水序列、认识洪水规律提供了一定的科学依据。  相似文献   

7.
The post-glacial history of Lake Pieni-Kuuppalanlampi, western Lake Ladoga region, was studied by means of stratigraphic pollen and diatom analyses. Diatoms were analysed to track the isolation history of the basin and the limnological effects of the early land-use phases indicated by pollen analysis. Chrysophycean stomatocysts and Isoëtes spores were also employed in the limnological reconstructions. Sediment dating was provided by six conventional radiocarbon dates.The lower part of the 370-cm long sediment sequence represents early Holocene, large lake conditions: the (freshwater) Yoldia and Ancylus stages of the Baltic basin, with a short-term lagoonal or isolation phase at the end of Yoldia. The basin was isolated due to Ancylus lake regression at 9785 cal B.P. For the small-lake sequence (0–250 cm) we used diatom inferences (WA-method) for hindcasting water chemistry. The post-isolation limnology of Pieni-Kuuppalanlampi reflects the development of vegetation on its small hill-top catchment. In its early development, the lake was mesotrophic, but became more acidic (pH about 6) and oligotrophic after the decline of temperate hardwood trees and the spread of spruce to the area after around 5000 B.P. The lake ecosystem appears to have reacted sensitively to agricultural land-use in the catchment from AD 400–800 onwards: inferred total phosphorus levels and pH both rise during these periods.  相似文献   

8.
We present a palaeolimnological study encompassing five centuries of trophic-state change of the dike-breach lake De Waay located on the Rhine-Meuse delta (the Netherlands). Diatom-inferred total phosphorus (TP) concentrations indicate hypertrophic epilimnetic conditions (>300 μg l−1 TP) since the formation of the lake in the fifteenth century until the end of the eighteenth century. Cladocera data support the reconstructed trophic state and indicate turbid conditions in lake De Waay during this period. High inferred TP concentrations as well as the amount of Ti in the sediment reflect numerous flooding events. From the nineteenth century onwards reconstructed TP concentrations decreased to 40–150 μg l−1 due to improvements in sewage and dike systems that considerably diminished direct river flooding and seepage-derived nutrients. As a consequence, the increased stability of littoral habitats led to an increased diversity of the Cladocera assemblages. The most significant decrease in TP concentrations to ~40 μg l−1 occurred between about 1900 and 1930. This mesotrophic phase was a consequence of the isolation of the lake from catchment drainage and the introduction of a highly elaborate flood control during this period. However, since the mid twentieth century a eutrophication trend is preserved in the record, likely related to increased agricultural activity in the vicinity of the lake. Our results emphasize that land-use and trophic-state history must be taken into account when evaluating the ecological status of lakes for water management and protection actions, especially for lakes in landscapes that are strongly modified by human action.  相似文献   

9.
The geochemistry of lake (Renstradträsket) and estuarine (Pieni Pernajanlahti Bay) sediment was investigated in a medium sized watershed draining to the Gulf of Finland, Baltic Sea. Catchment land-use types were compared and found similar. Sediment cores were dated using 210Pb- and 137Cs-chronologies and analyzed for Al, K, Cu, Zn, Fe, Mn, phosphorus fractions, TN, TC and biogenic silica (BSi). Differences between the sediment cores were studied by using linear regression analysis and principal components analysis (PCA). Despite similarities in catchment land-use and history, the sediment geochemical profiles of the sites varied significantly. Some of the differences could be related to differences in chemical sedimentation environment (lacustrine versus estuarine). TP concentration was found to be positively correlated with sediment iron content in estuarine sediment but negatively correlated with Fe in lake sediment. In the estuarine core sedimentary iron was not correlated to lithogenic potassium and aluminum but in the lake core the iron seemed to be lithogenic in origin, as suggested by the strong positive correlations (r 2 = 0.95–0.96) between these three variables. Most similarities among the cores were found in Al concentrations. Estuarine nutrient profiles appeared relatively monotonous compared to the lake core. This is probably due to more vigorous mixing of the sediments that may ensure more rapid and complete consumption of the organic matter deposited on the bottom of the estuary. Therefore the lake sediment appeared to preserve the historical record of eutrophication better. Biologically less active and more particle-bound materials like the trace metals Cu and Zn seemed to retain good records of anthropogenic impact also in the estuarine core. The study highlights the need to take the sedimentation environment into account when interpreting geochemical record.  相似文献   

10.
Detailed stratigraphic analyses of sediments deposited in Lake Botjärnen, a small boreal forest lake in the shield terrain of central Sweden, clearly reflect progressively increasing human impact on terrestrial and aquatic ecosystems following settlement and establishment of an iron industry in the 17th century. Rising frequencies of pollen and spores from light-demanding plants provide evidence of extensive forest clearance for charcoal and timber production, which peaked in the early 20th century. An associated increase in catchment erosion is reflected by changing carbon and nitrogen elemental content and carbon–isotope composition of sediment organic matter and by increased magnetic susceptibility of the sediments. Records of air-borne pollutants (lead, zinc and sulphur) can be correlated to the development of local and regional mining and metal industry as inferred from historical accounts. Rapid recession of the iron industry led to re-forestation and recovery of the aquatic nutrient status to pre-industrial conditions over the past 100 years. The chronology of the sediment succession, which is based on 210Pb and 137Cs radionuclide data in combination with radiocarbon dating, is confirmed by historical lead pollution trends established for the region.  相似文献   

11.
This paper raises fundamental questions about the sole use of paleolimnological techniques to identify sediment sources and develop catchment management plans. The concept of an integrated lake: catchment framework was established 30 years ago, yet paleolimnologists occasionally fail to appreciate the dynamics of the contributing catchment. This is especially critical when the predominant source of sediment accumulating in a lake is allochthonous. In this paper we argue that a detailed appraisal of catchment sources and investigation of historical documentary evidence is needed to identify and evaluate the relative significance of sediment sources. We used such an approach at Aqualate Mere, Shropshire, UK. Mineral magnetic and radionculide signatures of potential catchment sources and accumulating lake sediments were compared in an attempt to match the sources to sediments deposited in the Mere. Dated lake sediments indicate there has been an increase in sedimentation rate and the relative amount of minerogenic material delivered to the Mere over the last 200 years. In contrast to a previous study at the same site, there is no evidence to attribute this increase to an overspill from a nearby canal. Other catchment disturbances include landscaping in parkland surrounding the Mere in the early nineteenth century and drainage systems installed to improve catchment agriculture over the last ca. 150 years. Both activities may explain the change in sedimentation rates and types, independent of the hypothesized canal origin. Although our results exclude the canal as a major sediment source, identifying the contribution of other potential catchment sources remains problematic. 137Cs inventories for the lake are similar to those recorded at a local reference site, suggesting little influx of 137Cs-bearing topsoil, yet 137Cs activities remain high in the upper 20–30 cm of the lake sediment profile, indicating a topsoil origin. Combined radionuclide and mineral magnetic signatures proved to be relatively poor discriminators of potential sources, and the high atmospheric pollution load from the West Midland conurbation has probably altered recent lake sediment signatures. Although further research is required to identify the origins of recent (last ca. 200 years) minerogenic sediment inputs to the Mere, we suggest that the combined lake: catchment approach offers a more rigorous method for understanding the impact of catchment disturbance than analysis of the paleolimnological record alone.  相似文献   

12.
Koltjärnen and Nylandssjön are two closely situated lakes (<2 km apart) in northern Sweden. During the past century, distinct varved sediments have formed in these lakes. Nylandssjön has two varved, deep basins. Since lake and catchment characteristics superficially appear very similar for the two lakes and they are exposed to the same climate, one would expect the sediment varves to be similar. This investigation compares the varves in the two deep basins of Nylandssjön, and in the two lakes. The comparison of basins of Nylandssjön shows that varve thickness, water content and annual accumulation rates of organic matter and nitrogen are correlated for the period (1970–2003). The grey-scale curves are only clearly similar in about 50% of the varves. In the between-lake comparison varve thickness, water content and annual accumulation rates of organic matter and nitrogen are correlated for the period (1950–1996). However, the annual accumulation rates of dry mass, minerogenic matter and biogenic silica differ between the lakes, as well as within-varve successions in grey-scale. A general explanation to the differences is that the prerequisites for varve formation are not totally similar because of differences in catchment size, catchment- to-lake material fluxes, lake productivity and land-use influence. This study illustrates the complex relationships that exist between a lake, its catchment, in-lake productivity and formation of sediment varves. As a consequence, we must not apply a too simplistic view of the potential of varves as past climatic indicators, especially if the lakes are affected by land-use.  相似文献   

13.
Environmental change in Lake Taihu and its catchment since the early to middle part of the twentieth century has left a clear geochemical record in the lake sediments. The human activities in the lake and its catchment responsible for the change include agriculture, fishery, urbanisation, sewage and industrial waster disposal. Sediment cores were collected from Meilian Bay of northern Lake Taihu to investigate the record of anthropogenic impacts on the lake’s ecosystem and to assess its natural, pre-eutrophication baseline state. Two marked stratigraphic sediment units were identified on the basis of total phosphorus concentration (TP), pigments, total organic carbon (TOC)/total nitrogen (TN), δ13C and δ15N corresponding to stages in the lake history dominated by phytoplankton, and by aquatic macrophytes. Results show that as TP loading increased from the early 1950s the lake produced sediments with increasing amounts of organic matter derived from phytoplankton. In the early 1950s, the first evidence for eutrophication at the Meilian Bay site is recorded by an increase in C/N values and in sediment accumulation rate, but there is little change in phosphorus concentrations, pigments, δ13C and δ15N at this time. After 1990 a more rapid increase in trophic status took place indicated by increased levels of phosphorus, pigments, δ15N and by decreased δ13C and TOC/TN values in the lake sediments. The first increase in trophic status of the early 1950s results mainly from agricultural development in the catchment. In contrast, the acceleration from ca. 1990 originates from the recent development of fisheries and the urbanisation and industrialisation of the catchment.  相似文献   

14.
We use Cladocera remains in the sediments to reconstruct the longterm history of Lake Orta, a lake which experienced severe pollution from copper and ammonium sulphate, and started to recover during the last 15 years. Both human and natural impacts were detected over almost 400 years. Pollution was manifested by a dramatic decrease in the number of remains, in the planktonic/littoral (P/L) ratio, and in chydorid species diversity. Most species, even those most tolerant to stress, disappeared. The recolonization of biota was initially sustained by one species of chydorid,Chydorus sphaericus, which had a three-fold increase at the beginning of the 1980s, when studies on plankton recorded the development of a pelagic population. This fact, and the appearance in the sediments ofAlona quadrangularis, attest to the development of filamentous algae which was reported in studies on the plankton. The colonization of the lake by pelagic species came only in the last twelve years and was manifested also as a stabilization of the P/L ratio. Two other periods of disturbance were detected in the sediments: the first, at the end of the 19th century, was related to the introduction of exotic fish species; the second occurred during the second half of the 17th century. This event probably cannot be ascribed to human impact, but may be related to a decrease in temperature in that period (the Maunder Minimum).  相似文献   

15.
Frozen sediment cores from Lake Pupuke in Auckland City, New Zealand, contain a high resolution decadal to annual scale record of changing lake paleoenvironments and geochemistry that reflects changing landuse and hydrology in the catchment over the past c. 190 years. A reliable chronology is available from AMS 14C and 210Pb dating of the sediments, with the timing of the older part of the record supported by the first appearance of pollen of introduced Pinus and Plantago lanceolata associated with European settlement of Auckland in the early 1840s. Diatom stratigraphy, sediment elemental and carbon isotope geochemistry reflect changes in sediment sources and lake conditions commensurate with European development of the Lake Pupuke catchment, in particular enhanced algal productivity controlled by the influx of nutrients after c. 1920 AD. Attempts to prevent nuisance algal blooms in 1933, 1934 and 1939 using CuSO4 addition produced Cu spikes in the sediment that allowed confirmation of the accuracy of the 210Pb chronology. Hence, the elemental and isotopic composition of the Lake Pupuke sediments reflect the timing of significant anthropogenic activities, rather than climatic variations, that have occurred within the watershed over the past c. 190 years. The comparison of records of land use change in the catchment with the multi-proxy record of changes in the sediments usually allowed unambiguous identification of the signatures of change and their causes.  相似文献   

16.
This study assesses Little Ice Age (LIA) lake sediment morphological and geochemical records and moraine chronologies in the upper Fraser River watershed, British Columbia, Canada, to resolve differences in paleoenvironmental interpretation and to clarify sediment production and sediment delivery processes within alpine geomorphic systems. Moose Lake (13.9 km2), situated at 1032 m a.s.l., contains a partially varved record indicating variable rates of accumulation during the last millennium that, in general, coincide with previously documented LIA glacial advances in the region and locally. Dendrochronological assessment of forefield surfaces in the headwaters of the catchment (Reef Icefield) shows that periods of moraine construction occurred just prior to ad 1770, ad 1839 and ad 1883, and some time before ad 1570. Taken collectively, increases in varve thickness within eight Moose Lake sediment cores coincide with documented glacier advances over the twelfth through fourteenth centuries, the eighteenth century, and nineteenth through twentieth centuries. Glacial activity during the sixteenth century is also indicated. While varve thickness variations in proximal and distal sediments clearly reflect glacial activity upstream of Moose Lake, the intermediate varve record is relatively insensitive to these decadal and longer‐term catchment processes. Variations in Ca and related elements derived from glaciated carbonate terrain within the Moose River sub‐catchment (including Reef Icefield) indicate gradually increasing delivery from these sources from the twelfth through twentieth centuries even where the varve thickness record is unresponsive. Elevated carbonate concentrations confirm glacial activity c. ad 1200, ad 1500, ad 1750, and ad 1900.  相似文献   

17.
The geochemistry of lake sediments was used to identify anthropogenic factors influencing aquatic ecosystems of sub-alpine lakes in the western United States during the past century. Sediment cores were recovered from six high-elevation lakes in the central Great Basin of the United States. The proxies utilized to examine the degree of recent anthropogenic environmental change include spheroidal carbonaceous particle (SCP), mercury (Hg), and sediment organic content estimated using loss-on-ignition. Chronologies for the sediment cores, developed using 210Pb, indicate the cores span the twentieth century. Mercury flux varied between lakes but all exhibited increasing fluxes during the mid-twentieth century. The mean ratio of modern (post-A.D. 1985) to preindustrial (pre-A.D. 1880) Hg flux was 5.2, which is comparable to the results from previous studies conducted in western North America. Peak SCP flux for all lakes occurred between approximately A.D. 1940 and A.D. 1970, after which time the SCP flux was greatly reduced. The reduction in SCP input is likely due to better controls on combustion sources. Measured Hg concentrations and calculated sedimentation rates suggest atmospheric Hg flux increased in the early 1900s, from A.D. 1920 to A.D. 1990, and at present. Atmospheric deposition is the primary source of the anthropogenic inputs of Hg and SCPs to these high elevation lakes. The input of SCPs, which is largely driven by regional sources, has declined with the implementation of national pollution control regulations. Mercury deposition in the Great Basin has most likely been influenced more by regional inputs.  相似文献   

18.
Sediments in Marshall and Hidden Lakes in the Uinta Mountains of northeastern Utah contain records of atmospheric mineral-dust deposition as revealed by differences in mineralogy and geochemistry of lake sediments relative to Precambrian clastic rocks in the watersheds. In cores spanning more than a thousand years, the largest changes in composition occurred within the past approximately 140 years. Many elements associated with ore deposits (Ag, As, Bi, Cd, Cu, In, Mo, Pb, S, Sb, Sn, and Te) increase in the lake sediments above depths that correspond to about AD 1870. Sources of these metals from mining districts to the west of the Uinta Mountains are suggested by (1) the absence of mining and smelting of these metals in the Uinta Mountains, and (2) lower concentrations of most of these elements in post-settlement sediments of Hidden Lake than in those of Marshall Lake, which is closer to areas of mining and the densely urbanized part of north-central Utah that is termed the Wasatch Front, and (3) correspondence of Pb isotopic compositions in the sediments with isotopic composition of ores likely to have been smelted in the Wasatch Front. A major source of Cu in lake sediments may have been the Bingham Canyon open-pit mine 110 km west of Marshall Lake. Numerous other sources of metals beyond the Wasatch Front are likely, on the basis of the widespread increases of industrial activities in western United States since about AD 1900. In sediment deposited since ca. AD 1945, as estimated using 239+240Pu activities, increases in concentrations of Mn, Fe, S, and some other redox-sensitive metals may result partly from diagenesis related to changes in redox. However, our results indicate that these elemental increases are also related to atmospheric inputs on the basis of their large increases that are nearly coincident with abrupt increases in silt-sized, titanium-bearing detrital magnetite. Such magnetite is interpreted as a component of atmospheric dust, because it is absent in catchment bedrock. Enrichment of P in sediments deposited after ca. AD 1950 appears to be caused largely by atmospheric inputs, perhaps from agricultural fertilizer along with magnetite-bearing soil.  相似文献   

19.
Although lake sediment archives are widely used for reconstructing historical records of atmospherically delivered pollutants, the quantitative relationship between fallout levels and their record in the sediments is complex and not well known. The original input signal from the atmosphere can be significantly distorted by mediating transport processes in the catchment, through the water column and within the sediments themselves. Since these processes also affect the fallout radionuclide 210Pb commonly used to date sediments, a better understanding of their impact is also important to improving the accuracy and reliability of sediment dating. Blelham Tarn has been the subject of a number of palaeolimnological investigations using radiometric dating techniques since the early 1970s. More recently it was the site of a major study carried out within the EU Transuranics project concerning the long-term fate of fallout radionuclides in catchment/lake systems. This paper reviews the radiometric data from this study and uses the results to determine mass balances for fallout 210Pb, 137Cs and 239+240Pu in Blelham Tarn, and their spatial distribution over the bed of the lake. Atmospheric fluxes were determined by measuring concentrations in rainwater and cumulative inventories in soil cores from non-eroding sites. Sediment records in a grid of 16 cores were used to determine the spatial distribution over the bed of the lake, and net inputs from the catchment. Mass balance calculations indicate that c. 47% of 210Pb in the sediments derives from erosive inputs from the catchment. For 239+240Pu the figure rises to 61%. Reduced amounts of 137Cs in the sediments are attributed to greater losses of this radionuclide from the water column via the outflow due to its greater solubility. Inputs of radionuclides from the catchment are concentrated near one of the major input streams. Away from this part of the lake the sediment record is dominated by direct atmospheric fallout, though the detailed pattern is influenced by sediment focussing. A one parameter catchment/lake transport model is developed that incorporates the assumption that transport rates will decline with time as fallout on the catchment diffuses into the soil and becomes less available for removal. Values of the transport parameter were calculated for 210Pb and 239+240Pu and found to be comparable. The results suggest that it will take c. 11000 years to remove 50% of 239+240Pu from the catchment to the lake.  相似文献   

20.
Pollen and plant macrofossils were analysed at Sägistalsee (1935 m asl), a small lake near timber-line in the Swiss Northern Alps. Open forests with Pinus cembra and Abies alba covered the catchment during the early Holocene (9000–6300 cal. BP), suggesting subcontinental climate conditions. After the expansion of Picea abies between 6300 and 6000 cal. BP the subalpine forest became denser and the tree-line reached its maximum elevation at around 2260 m asl. Charcoal fragments in the macrofossil record indicate the beginning of Late-Neolithic human impact at ca. 4400 cal. BP, followed by a extensive deforestation and lowering of the forest-limit in the catchment of Sägistalsee at 3700 cal. BP (Bronze Age). Continuous human activity, combined with a more oceanic climate during the later Holocene, led to the local extinction of Pinus cembra and Abies alba and favoured the mass expansion of Picea and Alnus viridis in the subalpine area of the Northern Alps. The periods before 6300 and after 3700 cal. BP are characterised by high erosion activity in the lake's catchment, whereas during the phase of dense Picea-Pinus cembra-Abies forests (6300–3700 cal. BP) soils were stable and sediment-accumulation rates in the lake were low. Due to decreasing land-use at higher altitudes during the Roman occupation and the Migration period, forests spread beween ca. 2000 and 1500 cal. BP, before human impact increased again in the early Middle Ages. Recent reforestation due to land-use changes in the 20th century is recorded in the top sediments. Pollen-inferred July temperature and annual precipitation suggest a trend to cooler and more oceanic climate starting at about 5500 cal. BP.  相似文献   

设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号