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太湖梅梁湾富营养化过程的同位素地球化学证据 总被引：4，自引：0，他引：4
以浅水湖泊太湖为研究对象,通过湖泊水体、水生生物同位素以及相应湖泊水体营养指标的比较分析,并根据梅梁湾钻孔沉积物TN,TP,TOC,C/N,δ15N,δ13C等多项指标记录,恢复了湖泊富营养化过程.研究结果表明,不同湖区植物碳、氮同位素值和水体NH4+的δ15N值变化反映了植物组成和营养水平的差异.梅梁湾水体NH4+的δ15N和水环境参数不同月份的变化反映了外部营养载荷的输入对湖泊环境有明显的影响.1950～1990年湖泊沉积物有机质碳、氮同位素同步变化的趋势说明湖泊初级生产力的增长和湖泊逐渐富营养化的过程,而1990年之后二者之间反相关关系的出现表明在富营养条件下,大量浮游植物生长对富15N的无机氮的吸收及表层沉积物有机质分解和反硝化作用,代表湖泊富营养化加剧.以同位素示踪,并结合元素地球化学指标变化,将太湖梅梁湾富营养化过程分为三阶段,以20世纪50年代和20世纪90年代为营养状态的转换时段,揭示了人类活动不断加强的影响,与近50年来的湖泊环境监测结果一致. 相似文献
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太湖梅梁湾水动力及相关过程的研究 总被引：56，自引：13，他引：43
太湖是位于长江下游的一个大型水湖泊,水动力过程和要素对浅水湖泊的环境演化有着复杂和深远的影响,本文基于１９９８年开展的有关太湖梅梁湾的水动力过程的野外调查结果,总结了梅梁湾在夏季盛行风向条件下湖流特征,发现了梅梁湾在夏季偏南风条件下,表层湖流以顺时针环流为主要特征,但在湾内靠近梁溪河口地区,流场受地形影响而有所不同,反映在叶绿素浓度和总磷、总氮浓度分布上,因受湖流影响较大而富集在梁溪河口周转,即偏 相似文献
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太湖流域水污染控制与生态修复的研究与战略思考 总被引：16，自引：2，他引：14
为了探明太湖水体中胶体磷含量,更深入认识营养盐在大型浅水湖泊中的循环过程和机理,分别从太湖的梅梁湾和贡湖湾两个不同类型的湖区采集水样,利用切向流超滤方法分离出胶体物质,对太湖水体中胶体磷含量进行了初步研究．结果表明:太湖水体春季胶体磷含量在0．017-0．029 mg／L间,其中梅梁湾藻型湖区胶体磷含量范围是0 023- 0．029 mg／L,贡湖湾草型湖区胶体磷含量在0．017-0．022 mg／L间．梅梁湾水体胶体磷占总磷比例平均为28．6%;而贡湖湾胶体磷占总磷比例平均达到39．3%．梅梁湾水体真溶解态磷含量显著高于贡湖湾水体,达贡湖湾的4倍．与澳大利亚的17个湖泊相比,太湖属胶体磷含量偏低的湖泊,但相对于海洋的研究结果,太湖胶体磷含量明显偏高． 相似文献
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太湖春季浮游动物磷释放的初步研究 总被引：3，自引：0，他引：3
浮游动物是湖泊生态系统的主要组成之一,于2004年3月至5月间调查了太湖梅梁湾、五里湖浮游动物数量,并在实验室条件下分别测定了浮游动物正磷酸盐(PO4-P)的释放率．结果表明,研究期间梅梁湾的枝角类密度都高于五里湖,五里湖的轮虫数量高于梅梁湾,两水域桡足类密度上的差异不明显;梅梁湾和五里湖浮游动物PO4-p释放率的范围分别为0．20-O．43 mg／(g(DW)·h)和0．19-0．54 mg／(g(DW)·h)．因此浮游动物营养盐释放对湖泊生态系统营养盐循环具有一定的作用． 相似文献
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新疆博斯腾湖沉积物粒度的古环境意义初探 总被引：3，自引：0，他引：3
湖泊沉积物的粒度分析是一种研究古环境变化常用的手段,但是其环境意义具有多解性,尤其是沙（荒）漠干旱区的湖泊沉积物粒度变化,代表的是沙尘天气的多寡强弱还是其它环境因素的变化值得细致研究。在对我国最大的内陆淡水湖—新疆博斯腾湖的沉积物短岩芯进行了^210Pbex,^137Cs定年的基础上,对近50多年沉积物的粒度进行分析,结果表明平均粒径与粗颗粒含量与区域最大河流—开都河大山口站的最大一天洪量、洪峰流量、天山巴音布鲁克站年降水量、湖泊水位变化以及湖泊附近焉耆站3-6月风力强度变化记录等环境因素对比发现,湖泊中部沉积物中粗颗粒含量变化主要反映的是入湖河流径流量、区域洪水强度及频率、山地降水,而并不反映大风天气或者湖泊水位的变化。对其近千年沉积岩芯的多指标分析结果表明,即使在数百年时间尺度上,博斯腾湖沉积物粒度的环境意义依然与十年时间尺度上一致。 相似文献
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南四湖现代沉积物中营养元素分布特征 总被引：25，自引：2，他引：23
对南四湖不同湖区20个表层沉积物和独山湖湖区沉积岩芯中营养元素进行了分析结果表明表层沉积物中南阳湖总磷最高,独山湖次之;独山湖总有机碳和总氮含量最高,南阳湖次之;而昭阳湖总有机碳、总氮和总磷含量较低.沉积岩芯中137Cs数据表明南四湖独山湖区柱状沉积物上部(0-18 cm)沉积速率为3.5mm/a;总有机碳、总氮和总磷含量主要集中在沉积岩芯0-8 cm内,并呈现一致的垂向分布规律,具有明显的三阶段分布特征,反映了流域社会经济的发展导致营养元素的释放量增加,造成了湖泊现代沉积物中营养元素的积累.碳氮比值处于7.6-11.4之间,有机质的选择性分解不明显,指示沉积物中有机质主要来自无纤维束的陆源植物.监测数据表明济宁市的城市生活污水、工农业废水排放进入南阳湖是南四湖有机质和TP富集的主要来源. 相似文献
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小冰期弱化学风化的湖泊沉积记录 总被引：38，自引：3，他引：38
封闭湖泊沉积物的低Sr含量、低磁化率和高Rb/Sr比记录了单一湖泊流域在以冷干为特征的小冰期气候环境下经历的弱化学风化过程. 由于Rb, Sr在表生环境下不同的地球化学行为, 内陆湖泊沉积物中Rb/Sr比值是沉积记录中具有明确气候意义的有效指标. 与热带气候和现代温湿环境下化学风化受降水控制不同, 湖泊沉积岩芯的磁化率、Sr含量与冰芯δ18O一致的变化趋势揭示了小冰期最盛期极弱的化学风化过程是受气温控制的. 而随着气温的升高, 化学风化强度逐渐受降水的制约. 相似文献
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Current study presents the application of chemometric techniques to comprehend the interrelations among sediment variables whilst identifying the possible pollution source at Langat River,Malaysia.Surface sediment samples（0-10 cm）were collected at 22 sampling stations and analyzed for total metals（~（48）Cd,~（29）Cu,~（30）Zn,~（82）Pb）,pH,redox potential（Eh）,salinity,electrical conductivity（EC）,loss on ignition（LOI）and cation exchange capacity（CEC）.The principal component analysis（PCA）scrutinized the origin of environmental pollution by various anthropogenic and natural activities：four principal components were obtained with 86.34%（5 cm）and88.34%（10 cm）.Standard,forward and backward stepwise discriminant analysis effectively discriminate 2variables（84.06%）indicating high variation of heavy metals accumulation at both depth.The cluster analysis accounted for high input of Zn and Pb at LA8,LA 10,LA 11 and LA 12 that mergers three（5 cm）and four（10cm）into clusters.This is consistent with the contamination factor（C_1）that shows high Cd（LA 1）and Pb（LA 7,LA 8,LA 10,LA 11 and LA 12）contaminations at 5cm.These indicate that Pb and Zn are the most bioavailable metals in the sediment with significant positive linear relationship at both sediment depths.Therefore,this approach is a good indication of environmental pollution status that transfers new findings on the assessment of heavy metals by interpreting large complex datasets and predicting the fate of heavy metals in the sediment. 相似文献
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长江中下游不同湖泊沉积物中重金属污染物的累积及其潜在生态风险评价 总被引：21，自引：4，他引：17
利用富集因子和Hakanson潜在生态风险指数法,结合年代学结果,对长江中下游湖泊太白湖、龙感湖、巢湖和西氿沉积物中重金属元素Co、Cr、Cu、Ni、Pb、Zn的富集程度进行了评价,并比较分析了上述重金属的潜在生态风险.结果表明,太白湖和龙感湖沉积物中各重金属富集程度均较低;巢湖沉积物中Co、Cr、Ni的富集程度接近中等水平,而Cu、Pb、Zn的富集已经达到中等水平;西氿沉积物中Co的富集非常低,Cr、Ni富集水平较低,Pb达到中等富集,Cu、Zn达到较高的富集水平.对4个湖泊沉积物中重金属的综合污染程度进行比较:巢湖西氿龙感湖太白湖.各湖泊沉积物中单一元素的潜在生态风险都较低,但是,根据多元素潜在生态评价指数,各湖泊沉积物中重金属存在明显不同的潜在生态风险:巢湖西氿龙感湖太白湖.总体上看,太白湖和巢湖沉积物重金属污染以及潜在生态风险自1965年以来一直在加重,而龙感湖和西氿沉积物在表层有下降的趋势.这种差异与各个湖泊流域内人类活动的方式和强度密切相关.巢湖和西氿流域内城市化、工业化发展迅速,人类活动导致大量重金属元素进入湖泊,给湖泊带来明显的污染;而龙感湖和太白湖流域人类活动主要以农业活动为主,人类活动对重金属的贡献相对较小. 相似文献
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Trace metals distribution pattern in floodplain sediments of a lowland river in relation to contemporary valley bottom morphodynamics 
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下载免费PDF全文 The distribution of trace metals in alluvial sediments depends on their natural background concentrations, and on the dynamics of contemporary depositional and erosional (mainly flood‐induced) processes. Geological and geochemical investigations were carried out in the valley of Vistula River near Magnuszew (central Poland). Sediment samples were collected from a depth of 35 cm and comprise sediments of all defined geomorphological features. Identification and geological interpretation of the morphodynamic sediment features was supported by aerial photographs and high‐resolution satellite images. These studies revealed that the distribution of trace metals is closely linked to the morphogenesis of the alluvial floodplain. The highest concentrations of Cu, Co, Zn, V, Cr and Ni were observed in crevasse‐splays deposits. By contrast, Sr, Pb and As were concentrated in deposits which fill oxbow lakes (partly infilled with organic deposits). The lowest concentrations of trace metals were detected in flood sediments deposited within erosional troughs. The geomorphological and sedimentological history of the fluvial features explains the pattern of heavy metal distribution on the current floodplain surface. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献
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Feridon GHADIMI 《国际泥沙研究》2014,29(2):159-170
Five sediment zones（20 samples） were collected in Mighan Lake,near Arak city in Markazi province,and were analyzed to reveal element sources and assess the quality of metal contamination.Both anthropogenic and natural origins were identified by correlation,factor,and cluster analyse.According to the enrichment factors（EF） of trace metals（Ba,Co,Cr,Cu,Ni,Pb,Rb,Sr,Zr,and Zn）,three groups were identified.Enriched trace elements included：Ni,Zn,and Sr.Comparisons with contamination degree and benchmark sediment quality criteria and guidelines showed that Mighan Lake has potential for adverse effects on aquatic biota because of Ni,Zn,and Cr. 相似文献
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Alexis Castillo Jorge Valdés Abdel Sifeddine Sue-Ellen Vega Javier Díaz-Ochoa Yery Marambio 《国际泥沙研究》2019,34(2):178-190
Upwelling coastal systems can be used to understand how dissolved oxygen and biological productivity control the accumulation of redox-sensitive metals in marine sediments. The aluminium (Al), cadmium (Cd), iron (Fe), nickel (Ni), molybdenum (Mo), vanadium (V), total organic carbon (TOC), total nitrogen (TN) and total sulfur (TS) contents in surficial sediment collected from different water depths (30, 70, and 120?m) in three northern Chilean bays influenced by coastal upwelling and oxygen minimum zones (OMZs) were measured. Principal component analysis (PCA), cluster analysis, and Spearman?s rank correlation were used to identify the mechanisms responsible for the redox-sensitive metal accumulation. The content of redox-sensitive metals and organic components in sediment increased with increasing water column depth, whereas lithogenic metals decreased. In the Mejillones del Sur and Caldera bays, the enrichment factors of the redox-sensitive metals showed enrichment for all metals with depth. The Cd and V enrichments are mainly the product of biogenic flow to the seabed, and the Mo and Ni enrichments are due to preservation under low subsurface oxygen conditions. Sulfate reduction is not an important mechanism in the accumulation of redox-sensitive metals in the sediment of the three bays. The PCA showed that the behaviors of the redox-sensitive metals and organic components reflect differences in the effects of the OMZ in sediment along the coast of northern Chile, with a more intense OMZ in Mejillones del Sur bay and weaker OMZs in Caldera and Inglesa bays. However, the high degree of enrichment in redox-sensitive metals in Caldera Bay can be attributed to the intense activity of the mining industry near the bay, a situation that produces geochemical behavior similar to that observed in Mejillones del Sur Bay. 相似文献
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T. I. Moiseenko L. V. Razumovskii N. A. Gashkina A. V. Shevchenko V. L. Razumovskii A. S. Mashukov V. Yu. Khoroshavin 《Water Resources》2012,39(5):576-589
The results of studying four mountain lakes in different climatic zones (in regions of the Kola North and the Western Caucasus) are given. Original methods of paleoecological reconstruction developed by the authors have been used to characterize the main trends and rates in environmental changes at historical scale (by geochemical composition and diatom complexes in bottom sediment layers). Similar processes of modern water enrichment by metals (especially, Cd and Pb) have been determined in the examined lakes. Trends in changes in acid-base balance in The Kola North lakes since the late XIX century have been identified, reflecting the effect of transboundary transport of acid-forming substances from industrial Europe. Studies of diatom complexes in Caucasian lakes showed a rise in the mean annual temperature of lake water during the XX century supposedly by 1.5°C. 相似文献
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Sreenivasulu Ganugapenta Jayaraju Nadimikeri Sundara Raja Reddy Balam Chinnapolla Lakshmanna Ballari Rajasekhar Madiga Nirmala K Lakshmi Prasad Tella 《国际泥沙研究》2018,33(3):294-302
Sediment from twelve stations was sampled from the Tupilipalem Coast, southeast coast of India, and the presence of a set of heavy metals was established including iron (Fe), manganese (Mn), chromium (Cr), copper (Cu), nickel (Ni), lead (Pb), zinc (Zn) and cadmium (Cd). The heavy metals were assessed by factor analysis, the results of which showed positive and/or negative correlations among Fe, Mn, Cr, Cu, Ni, Pb, Zn, and Cd. Factor analysis also indicated that heavy metals in the sediments of the study area have different natural and anthropogenic sources. Similarly, a sediment pollution assessment was done using the Geoaccumulation Index (Igeo), Enrichment Factor (EF), and Pollution Load Index (PLI). The Geoaccumulation Index indicated that the surface sediment of the Tupilipalem Coast was extremely contaminated with Fe, Mn, Cr, Cu, Ni, Pb, and Zn. The calculation of enrichment factors showed a significant enrichment with respect to Pb, Zn, and Cd and a moderate enrichment with Cr, Cu, and Ni. The falling trend of average contents’ enrichment factors is Cd> Pb> Zn> Cu> Cr> Ni> Mn> Fe. The PLI values of the Cd show higher (>1) values due to the influence of distinct external sources like agricultural runoff, industrial activities, and other anthropogenic inputs. Ninety two percent of heavy metals under study showed the highest concentrations at station TP-5 where the Buckingham Canal and other agricultural and aquacultural effluents connect with the Bay of Bengal. This location is the second inlet which is periodically closed and it seemed that these parts of the study area are heavily affected by anthropogenic pollution. 相似文献
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K. Terytze 《洁净——土壤、空气、水》1993,21(1):8-20
For a wide variety of substances aquatic systems are the medium of origin, or sinks in a longer or shorter lasting stay or even in geological periods. For surface sediments of Berlin waters and their surroundings this paper describes the enrichment and distribution of heavy metals (SM), which have a high priority under international aspects and a marked capability to geoaccumulation. From the 25 metals investigated Hg, Pb, Cu, Cd and Zn are of anthropogenic origin, all others are of geochemical provenience and correspond to background values. Some metals (Hg, Cd, Ni, Co, Cu, Cr and Pb) have specific concentration profiles with increasing depth of water and sediment. The study of correlation of SM in sediments demonstrates generally a strong relation to macroelements and between some metals themselves. 相似文献
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Kurt Friese Gerald Schmidt Jorge Carvalho de Lena Dieter W. Zachmann 《Limnologica》2010,40(2):114-125
The artificial reservoir Lagoa da Pampulha in central Brazil has been increasingly affected by sediment deposition and pollution from urban and industrial sources. This study investigates water chemistry and heavy metal concentrations and their fractionation in the lake sediment using ICP-OES, ICP-MS, and XRD analyses. Fractionation analysis was done by sequential extraction under inert gas as well as after oxidation. The lake exhibits a permanent stratification with an oxygen-free hypolimnion below 2 m depth. Nutrient concentrations are enriched for phosphorous components (SRP, PO4). In the sediment it was not possible to detect oxygen. Carbon, sulfur, and most of the analyzed heavy metals are enriched in the top sediment layer with a pronounced downward decrease, indicating the presence of an anthropogenic influence. Statistical analysis, including correlations and a Principal Component Analysis (PCA) of depth-related total concentration data, helps to distinguish presumably anthropogenic heavy metals from geogenic components. Some samples with high element concentrations in the sediment also show elevated concentrations in their pore water. Analyses of element distribution between sediment and pore water suggest a strong bonding of heavy metals to the anoxic sediment. The trend towards elevated solubility in the pore water of oxidized samples is clear for most of the analyzed elements. Fractionation analysis reveals characteristic associations of selected elements to specific mineral bonding forms. In addition, it indicates that the behavior of heavy metals in the sediment is strongly influenced by organic substances. These substances provide buffering against oxidation, acidification, and metal release. The high nutrient loading causes reducing conditions in the lake sediment. These conditions trigger the accumulation of sediments rich in S2−, which stabilizes the fixation of heavy elements. In the future, care must be taken to reduce the supply of contaminants and to prevent the release of heavy metals from sediments dredged for remediation purposes. 相似文献