共查询到20条相似文献，搜索用时 609 毫秒
1.
冰晶产生的非催化触发机制研究 总被引：5，自引：2，他引：5
本文研究了用压缩空气爆破(薄膜爆破,激波管等)和火药爆炸非催化方法触发冰晶产生的作用机制。我们通过大量实验认为超声波和冲击波的作用不一定能够触发过冷水滴冻结,而超声速气流的绝热膨胀冷却作用则是触发冰晶产生的确切机制。然后设计了超声速气流发生装置并在过冷雾中进行触发冰晶产生的实验。结果表明,超声速气流(M=1.1)触发冰晶产生非常有效。阈温为-2℃。冰晶产生的临界压强为2.1atm,阈压随实验温度升高而增加,当总压超过阈压0.2—0.3atm时,冰晶大量产生。这些结果与超声速绝热膨胀理论相一致。 相似文献
2.
利用已有的二维雷暴云起、放电模式模拟了一次雷暴天气,并通过敏感性试验研究了冰核浓度变化对雷暴云动力、微物理及电过程的影响。结果表明：随着大气冰核浓度的增加,雷暴云发展提前,上升气流速度和下沉气流速度均呈现降低的趋势。大气冰核浓度提升有利于异质核化过程增强,冰晶在高温区大量生成,而同质核化过程被抑制,因此冰晶整体含量降低,引起低温区中霰粒含量降低和高温区中霰粒尺度降低。在非感应起电过程中,正极性非感应起电率逐渐减小,负极性非感应起电率逐渐增大。由于液态水含量随大气冰核浓度的增加逐渐降低,高温度冰晶携带电荷的极性由负转变为正的时间有所提前。在感应起电过程中,由于霰粒尺度减小及云滴的快速消耗,感应起电率极值逐渐降低。冰晶优先在高温区生成而带负电,不同大气冰核浓度下的雷暴云空间电荷结构在雷暴云发展初期均呈现负的偶极性电荷结构。在雷暴云旺盛期,随着冰核浓度增加,空间电荷结构由三极性转变为复杂四极性。在雷暴云消散阶段不同个例均呈现偶极性电荷结构,且随着冰核浓度的增加电荷密度值逐渐减小。 相似文献
3.
Paleoclimate simulations of the mid-Holocene (MH) and Last Glacial maximum (LGM) by the latest versions of the Flexible Global Ocean-Atmosphere-Land System model, Spectral Version 2 and Grid-point Version 2 (FGOALS-s2 and g2) are evaluated in this study. The MH is characterized by changes of insolation induced by orbital parameters, and the LGM is a glacial period with large changes in greenhouse gases, sea level and ice sheets. For the MH, both versions of FGOALS simulate reasonable responses to the changes of insolation, such as the enhanced summer monsoon in African-Asian regions. Model differences can be identified at regional and seasonal scales. The global annual mean surface air temperature (TAS) shows no significant change in FGOALS-s2, while FGOALS-g2 shows a global cooling of about 0.7 C that is related with a strong cooling during boreal winter. The amplitude of ENSO is weaker in FGOALS-g2, which agrees with proxy data. For the LGM, FGOALS-g2 captures the features of the cold and dry glacial climate, including a global cooling of 4.6 C and a decrease in precipitation by 10%. The ENSO is weaker at the LGM, with a tendency of stronger ENSO cold events. Sensitivity analysis shows that the Equilibrium Climate Sensitivity (ECS) estimated for FGOALS ranges between 4.23 C and 4.59 C. The sensitivity of precipitation to the changes of TAS is～2.3% C-1 , which agrees with previous studies. FGOALS-g2 shows better simulations of the Atlantic Meridional Overturning Circulation (AMOC) and African summer monsoon precipitation in the MH when compared with FGOALS-g1.0; however, it is hard to conclude any improvements for the LGM. 相似文献
4.
层状云催化后过冷水分布与演变规律的数值模拟 总被引：4，自引：4，他引：4
在郭学良等(1999年)发展的层状云雨滴分档模式中加入冰晶繁生过程,模拟了碘化银和液态二氧化碳的催化效率以及催化后云中过冷水的分布与演变过程.结果表明:碘化银和液态二氧化碳在5200～5600 m高度上的催化效率相当,最大达到11.1%;液态二氧化碳在2600～3000 m高度层的催化效率明显增大,达到14.2%;模式云被催化后,云中云水含量在200 min都较未催化时增长0.05 g/m3以上,表现出云中过冷水被消耗后的恢复趋势;碘化银和液态二氧化碳对云体催化后,云中水汽含量减少0.5～2 g/m3,对过冷水的恢复作出贡献;催化过程使得模式云中雨滴浓度在210 rin时较未催化时减少73%,在240 min时较未催化时增加309%.得出了两点结论:(1)模式云被催化后,云中过冷水在200 rin表现出恢复趋势,云中水汽对过冷水的恢复过程作出了贡献;(2)在过冷水较多的区域播撒液态二氧化碳可以取得较好的催化效率. 相似文献
5.
含碘化银人工冰核检测问题 总被引：3，自引：0，他引：3
对中国人工影响天气中常用的几种碘化银催化剂的成核率做了比对，讨论了不同云室可能响应的主要冰核活化机制和混合云室检测误差来源，此外还给出了动态检测的尝试性结果。结果表明：碘化银类播云剂的检测除了应模拟冰核活化条件外，还应模拟冰核发生时的环境条件，当务之急是建造动态检测设备以取得更为接近实际的检测结果。 相似文献
6.
Mineral dust particles are known to be efficient ice nuclei in the atmosphere. Previous work has probed heterogeneous ice nucleation on various laboratory dust samples including Arizona Test Dust, kaolinite, montmorillonite, and illite as atmospheric dust surrogates. However, it has recently been suggested that NX illite may be a better representation of atmospheric dust. Hiranuma et al. (2015) performed a laboratory comparison for immersion ice nucleation on NX illite, but here we focus on depositional ice nucleation because of its importance in low temperature cirrus cloud formation. A Raman microscope setup was used to examine the ice-nucleating efficiency of NX illite. Organic coatings on the NX illite particles were also investigated using a mixture of 5 dicarboxylic acids (M5). The ratio of NX illite to M5 was varied from 1:10 to 100:1. It was found that NX illite efficiently nucleates ice with Sice = 1.07 ± 0.01 at ?47 °C, with Sice slightly increasing at lower temperatures. In contrast, pure M5 is a poorer ice nucleus with Sice = 1.30 ± 0.02 at ?40 °C, relatively independent of temperature. Further, it was found that M5 coatings on the order of several monolayers thick hindered the ice nucleating ability of NX illite. Optical images suggest that at colder temperatures (< ?50 °C) 1:1 NX illite:M5 particles and pure M5 particles nucleate ice depositionally, while at warmer temperatures (> ?50 °C) subsaturated immersion ice nucleation dominates. These experiments suggest that mineral dust particles may become less active towards ice nucleation as they age in the atmosphere. 相似文献
7.
三七炮弹是进行人工增雨和防雹作业所需碘化银催化剂的主要载体之一,炮弹中碘化银催化剂的成核率数据是人工影响天气作业设计和指挥中进行催化剂作业剂量测算的重要参考,因此,对人工影响天气业务中使用的三七炮弹的碘化银成核率进行检测非常重要。2013年11—12月中国气象局人工影响天气中心利用新建的1200 L等温云室和钢板式20 m3专用爆炸室等设备,对目前人工影响天气业务中使用的两个厂家三七炮弹 (样品1、样品2) 的碘化银成核率进行国内首次统一检测。检测结果表明:两厂家炮弹成核率检测结果的拟合值量级均为109~1012/(g·AgI)(检测温度-6℃至-20℃),样品2成核率明显高于样品1。将本次检测结果与国内历次三七炮弹检测结果相比发现,两样品在负温高温段的成核率值均高于以往检测结果,其中,在具有指示意义的-10℃下的成核率,两样品均比以往检测结果要高2~3个量级。不同检测实验中成核率检测结果存在较大差异的现状说明,采用同一平台开展成核率统一检测十分必要。 相似文献
8.
Sahana Paul A. Hazra U. K. De S. Bhar K. Goswami 《Journal of Atmospheric Chemistry》2006,53(2):155-168
Nucleation properties of different alcoholic solutions of Benzoin and Benzoin dust have been studied by varying the seeding temperature in a laboratory Cold Chamber. In the present study, three different alcoholic solutions are being used and these are due to the standard Ethyl alcohol, one higher alcohol i.e. Isopropyle alcohol and one lower alcohol i.e. Methyl alcohol. In addition, Benzil dust and droplets of Acetone and Chloroform have been used to examine if these agents have any ice nucleation ability. It has been observed that all alcoholic solutions of Benzoin have sufficient ice nucleation ability at the negative side of 0°C, with the maximum concentration occurring at −14.4°C. In case of Benzoin dust, the nucleation ability is better on the positive side of 0°C than the negative side. On the other hand, Benzil dust has insignificant nucleation ability and the droplets of two other agents have no nucleation ability at all.Considering the chemical as well as crystalline structure, one can conclude that the presence of OH group in the seeding molecule plays the central role in ice nucleation/hydrate crystal formation. In fact, a number of supplementary experiments like crystal growth in an incubator, XRD analysis and NMR study are performed to identify the nature of crystals formed by Benzoin dust above 0°C. One can conclude that these are hydrate crystals of Benzoin with water caging around Benzoin crystals. 相似文献
9.
Ines Hoog Subir K. Mitra Karoline Diehl Stephan Borrmann 《Journal of Atmospheric Chemistry》2007,57(1):73-84
In laboratory experiments the interactions of ammonia with ice crystals were studied within the temperature range between
0 and −20°C. In a first series of experiments dendritic ice crystals were grown from water vapor in presence of ammonia gas
in various concentrations between 4 and 400 ppbv. In a second series of experiments pure ice crystals were exposed to a humidified
ammonia–air mixture inside a horizontal flow tube. The influence of temperature, ammonia gas concentration (0.6, 1.5, and
10 ppmv), exposure time, and the presence of impurities such as sulfate on the ammonia uptake by the ice surface was investigated
by determining the ammonium content in the melt water of the ice crystals by ion chromatography. During the growth of ice
crystals significant amounts of ammonia (around 200 μg/l) were taken up even at small gas concentrations. In contrast, even
at high gas concentrations the uptake of ammonia by non-growing ice crystals was lower by approximately one order of magnitude.
The presence of sulfate on the ice surface affected an enhanced uptake of ammonia by a factor of 5–10. A model is presented
which describes the uptake of ammonia by ice considering the chemical processes occurring in the ice surface layer and simultaneous
diffusion of ammonia into bulk ice. Even the increased uptake of ammonia by growing ice is rather small compared to the uptake
by water droplets; thus, the major process for scavenging of ammonia from the atmosphere via the ice phase might not be the
direct uptake by ice crystals but the riming involving super-cooled droplets containing ammonia. 相似文献
10.
Aerosols emitted from volcanic activities and polluted mid-latitudes regions are efficiently transported over the Arctic during winter by the large-scale atmospheric circulation. These aerosols are highly acidic. The acid coating on ice nuclei, which are present among these aerosols, alters their ability to nucleate ice crystals. In this research, the effect of acid coating on deposition and contact ice nuclei on the Arctic cloud and radiation is evaluated for January 2007 using a regional climate model. Results show that the suppression of contact freezing by acid coating on ice nuclei leads to small changes of the cloud microstructure and has no significant effect on the cloud radiative forcing (CRF) at the top of the atmosphere when compared with the effect of the alteration of deposition ice nucleation by acid coating on deposition ice nuclei. There is a negative feedback by which the suppression of contact freezing leads to an increase of the ice crystal nucleation rate by deposition ice nucleation. As a result, the suppression of contact freezing leads to an increase of the cloud ice crystal concentration. Changes in the cloud liquid and ice water contents remain small and the CRF is not significantly modified. The alteration of deposition ice nucleation by acid coating on ice nuclei is dominant over the alteration of contact freezing. 相似文献
11.
引入一种新型冰晶异质核化方案, 基于二维雷暴云模式, 探讨雷暴云电过程对三种异质核化的响应。结果表明: 浸润核化是冰晶生成的最重要异质核化过程, 较高数浓度的冰晶消耗雷暴云内液态水含量, 抑制淞附过程, 导致霰粒子比含水量低, 表现为较强的负极性非感应起电率; 接触核化生成的冰晶量最少, 仅对雷暴云中下层3~5 km处的冰晶有贡献, 同时霰粒子数浓度较低, 导致该方案下的起电过程最弱; 沉积核化主要影响云砧处的冰晶, 有利于提高霰收集云滴的效率, 表现为极高的霰比含水量, 促进低温区非感应起电过程的发生。总体上来看, 三个方案下的电荷结构均由较复杂的多极性发展为偶极性。其中浸润方案中主正电荷区的抬升最明显, 而接触方案过低的冰晶分布高度与沉积方案过高的冰晶分布高度, 都直接导致了次正电荷区更快消散。 相似文献
12.
小型混合云室常用于自然冰核浓度的观测和人工冰核成核率的检测。使用表明:由于受云室容积、造雾方法和操作程序等因素的影响, 检测结果有很大差异, 难以相互比较。为提高检测数据的可信性, 设计并制作了15 L混合云室。云室由F22压缩机系统制冷, 最低能达到-28℃。为减小云室温度的波动, 在云室外围设计有装满乙二醇-水溶液的夹套。在溶液中, 安装了1个1 kW的电加热器, 接通后可使云室升温。在夹套外, 采用发泡技术形成约10 cm厚的绝热层, 以使云室与外界绝热。云室运行时, 可通过控制压缩机和电加热器得到实验温度。此外, 为拓宽检测冰核浓度的检测范围, 设计了玻璃片接取显微镜读数和糖盘接取目测读数两种可供选择使用的冰晶观测方法, 前者在冰晶浓度高时使用 (人工冰核), 后者在低浓度时使用 (自然冰核)。另一个重要改进是:先由一个超声雾化器产生常温雾, 而后使常温雾穿过一个低温狭缝进行预冷, 当雾温等于或低于云室温度后再进入云室。这一措施不仅避免了瞬时高度过饱和, 而且还减小了对云室温度的扰动。该云室在弹载催化剂成核率的改进实验中发挥了重要作用, 曾用它对多个人工冰核复合配方进行了检测和对比。结果表明:云室具有较好的稳定性和重复性, 整体性能优于以往的同类云室。这一结果是由于改进了提供过冷雾的设计和冰晶接取方法得到的。 相似文献
13.
为分析层状云垂直微物理结构,了解雷达参数特征,揭示降水机制,利用机载Ka波段云雷达和DMT（Droplet Measurement Technologies）粒子测量系统,针对2019年11月17日山东冷锋层状云系开展从云顶至云底的垂直探测。结果表明:观测云层由高层云（3100~4500 m高度）和雨层云（800 ~2600 m高度）两部分组成。高层云过冷水含量较低,平均值为0.0026 g·m-3,最大值为0.008 g·m-3,云内冰晶通过水汽凝华增长,平均浓度为8.2 L-1,最大直径为900 μm,平衡谱状态下冰晶浓度与雷达反射率因子具有较好相关性,相关系数最大为0.84。雨层云过冷水含量丰富,最大含水量为0.354 g·m-3,过冷水区平均雷达反射率因子为7.48 dBZ,多普勒速度为-2.3 m·s-1,速度谱宽为0.7 m·s-1;雨层云中上部以冰晶为主,下部为暖区融化粒子,冰晶通过凇附过程增长,平均浓度为208 L-1,最大直径为450 μm;雷达反射率因子随高度降低至1500 m不断增大,在1200~1500 m高度保持不变,1200 m高度以下减小,未出现明显0℃亮带,速度谱宽随高度降低增大。 相似文献
14.
Further laboratory experiments of thunderstorm charging by ice crystal collisions with riming graupel pellets have led to results that may help account for a major difference between two independent studies reported earlier. The problem concerns values of the cloud liquid water content required to change the sign of graupel charging. The present work has noted and investigated differences in the techniques of cloud nucleation used in the two studies. In one set of measurements by Takahashi, ice crystals are nucleated continuously in a supercooled water droplet cloud, while in the other experiments by Jayaratne et al. and Saunders et al., the droplet cloud is nucleated only briefly. These two nucleation methods lead to differences in the mass of cloud particles collected on a sampling probe used to determine the liquid water content of the cloud. In the continuous nucleation case, the probe collects sufficient numbers of ice crystals to lead to a substantial overestimate of the cloud liquid water content. 相似文献
15.
冰晶核化对雷暴云微物理过程和起电影响的数值模拟研究 总被引：2，自引：0，他引：2
本文在已有的二维对流云模式中采用了一种与气溶胶有关的冰晶核化方案替代原有的冰晶核化经验公式, 并选取个例, 分别就两种方案进行了模拟对比试验。模拟结果表明:(1)新方案所得冰晶比含水量主要分布在-0.1~-7.6℃温区之间, 高于原方案所得的-50.1~-24.2℃温区;在整个雷暴云的发展过程中新方案冰晶的分布高度、温度区间以及最大浓度值均大于原方案。(2)在新方案中, 温度相对较高的过冷区产生大量冰晶, 其争食云中水汽抑制了云滴、雨滴的增长。此外, 与原方案相比, 霰增长受雨滴大幅减小的影响进一步得到限制, 导致生成的霰小于原方案, 且空间分布具有较大区别。(3)两方案在雷暴云初期形成的电荷结构不同;在发展旺盛与消散阶段新方案中电荷空间分布区域和电荷量均大于原方案, 此外, 在不同时刻主正电荷区和主负电荷区的中心高度存在差异。本文对云微物理过程及起电的分析为后继探讨气溶胶与雷暴云起放电过程、电荷结构之间的相互关系提供了有利条件。 相似文献
16.
含水量对冰晶增长影响的风洞实验研究 总被引：1，自引：0，他引：1
用小型垂直过冷云风洞及其测试系统,使冰晶在自由悬浮的情况下生长。在实验温度为-5℃—15℃、含水量为0.5—2.0g/m~3的范围内,结果表明:在水面饱和条件下,冰晶的形状决定于所处的环境温度,含水量的大小对冰晶的基本形状没有影响,只是当含水量加大时,冰晶上会出现更加明显的碰冻增长的痕迹;冰晶的质量和速度增长的峰值和谷值温度分布与含水量的大小无关;随着含水量的增加,冰晶的质量和下落速度的增长会加快,但没有发现含水量的增加有加快冰晶2a轴增长的明显效果。 相似文献
17.
18.
Theories to describe the structures and properties of ice surface were critically examined. Misconceptions were clarified in regard to treatment of the liquid-like layer that is expected to exist on the surface of an ice crystal below 0°C, 1 atm under equilibrium. It was shown that the pressure in the surface layer, not the surface free energy, is responsible for the formation of the liquid-like layer. Transformation of this layer into transitional liquid layer under ice-supersaturated conditions of the environment and the roles played by the latter layer in non-dendritic and dendritic growth of ice crystals were explained. 相似文献
19.
20.
A band of cooling that extends across mid-latitude Eurasia is identified in the wintertime surface air temperatures of the latest ECMWF reanalysis. This cooling is related to extreme warming around the Kara Sea through changes in the meridional temperature gradient. Surface temperatures in the Arctic have risen faster than those at lower latitudes, and as the Arctic warming increases, this north–south temperature gradient is weakened. This change in the meridional temperature gradient causes a decrease in the westerly winds that help maintain the mild European climate by transporting heat from the Atlantic. Since decreasing sea ice concentrations have been shown to be a driving factor in Arctic amplification, a singular value decomposition analysis is used to confirm the co-variability of the Arctic sea ice, including the Kara Sea, and the temperatures over the mid-latitude Eurasia. These findings suggest that decreasing sea ice concentrations can change the meridional temperature gradient and hence the large-scale atmospheric flow of the Northern Hemisphere. 相似文献