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1.
The paper focuses on the redistribution of aerosol particles (APs) during the artificial nucleation and subsequent growth of ice crystals in a supercooled cloud. A significant number of the supercooled cloud droplets during icing periods (seeding agents: C3H8, CO2) did not freeze as was presumed prior to the experiment but instead evaporated. The net mass flux of water vapour from the evaporating droplets to the nucleating ice crystals (Bergeron–Findeisen mechanism) led to the release of residual particles that simultaneously appeared in the interstitial phase. The strong decrease of the droplet residuals confirms the nucleation of ice particles on seeding germs without natural aerosol particles serving as ice nuclei. As the number of residual particles during the seedings did not drop to zero, other processes such as heterogeneous ice nucleation, spontaneous freezing, entrainment of supercooled droplets and diffusion to the created particle-free ice germs must have contributed to the experimental findings. During the icing periods, residual mass concentrations in the condensed phase dropped by a factor of 1.1–6.7, as compared to the unperturbed supercooled cloud. As the Bergeron–Findeisen process also occurs without artificial seeding in the atmosphere, this study demonstrated that the hydrometeors in mixed-phase clouds might be much cleaner than anticipated for the simple freezing process of supercooled droplets in tropospheric mid latitude clouds. 相似文献
2.
Summary A one-dimensional kinematic model is used to investigate the effects of silver iodide seeding in the region of a Cb cloud between isotherms of –8°C and –12°C. The agent interaction with cloud atmosphere is simulated by an improved microphysical model version which includes phoretic processes. The behaviour of the different agent types is investigated using the maximum values of agent mixing ratios and corresponding agent particle masses and radii.It is shown that the agent residence time in the seeding zone significantly depends on vertical velocity. The residence time is comparable to that previously reported. On the other side, the final graupel production decreases slightly when vertical velocity increases, while the corresponding graupel production is quite different for agents used. The main agent nucleation mechanisms are the Brownian coagulation of cloud droplets, inertial impact of cloud droplets and deposition nucleation.With 9 Figures 相似文献
3.
利用三维全弹性冰雹云模式,对2008年5月24日山东境内一次受高空冷涡影响的大范围冰雹天气过程进行模拟,分析了冰雹的形成机制和催化防雹机理。结果表明:该过程过冷雨水中心位于最大上升气流中心下方,不存在过冷雨累积区,过冷雨水含量最大值仅为4.9gm-3,但雹云中过冷雨水含量仍然丰富,对雹胚的形成及增长起着重要作用。雹胚以冻滴为主,冻滴胚来源于冰雪晶与过冷雨水碰撞冻结以及雨滴核化过程。冻滴形成后主要以碰并过冷雨水、云水增长。冻滴胚自动转化过程是冰雹数量、质量的主要来源;冰雹形成后,前期主要靠碰并冻滴、霰和过冷雨水增长,后期主要靠碰并过冷云水增长。催化试验表明,播撒57.5g催化剂足以通过"竞争"减雹50%以上,增加AgI剂量,防雹的同时能够兼顾增雨。催化剂用量为230g时,催化后液态降水有所增加,固态降水量及占总降水量的比例减少显著,特别是冰雹。AgI主要以凝华核的作用产生人工冰晶,冰晶凝华增长导致过冷云水、雨水含量降低。催化后雹胚特别是冻滴胚数量增多,对过冷云水、雨水的竞争增强;其平均尺度、质量的减小,降低了向冰雹的转化率。冰雹碰并过冷云水、雨水增长过程被减弱,导致冰雹总质量进一步减少,达到消雹目的。 相似文献
4.
层状云降水效率通常较低,但却具有较高的云水资源开发潜力,是人工增雨作业的重要对象。随着中国南方地区生态改善、水库增蓄、抗旱等社会需求的增加,针对这些地区降水云系的人工增雨研究显得愈发重要。使用三维中尺度冷云催化模式,对2018年10月21日湖北省一次层状云飞机人工增雨作业过程进行了数值模拟研究,并将模拟结果与卫星、降水和机载云物理观测数据进行了对比。模式合理地模拟出了云和降水的主要宏、微观特征,观测和模拟结果均显示作业云区具有较好的冷云催化条件,在此基础上,按照实际作业中的飞机播撒轨迹,完整地模拟了此次催化作业过程。对数值模拟结果的分析表明:凝结冻结核化和凝华核化是碘化银催化剂的主要核化方式;90%以上碘化银粒子的局地活化比为0.01%—2%,平均活化比为0.07%—0.27%;云系降水是由冷云降水和暖云降水两种机制共同作用的结果,催化作业使两种降水机制均有增强,增雨效果明显;催化后4 h,整个评估区内的累计净增雨量为2.12×108 kg,局地增雨率为?51.1%—306.7%,区域平均增雨率为8.1%;催化作业也使部分地区出现减雨,主要是由于催化过程中的潜热释放引起过冷层动力场扰动,一部分云区的上升气流减弱,从而导致降水粒子的成长减弱,地面出现减雨;在过冷云区,碘化银核化使冰晶浓度升高,导致冰晶-雪、雪-霰的转化过程增强,雪、霰粒子总量增加,更多的雪、霰粒子从冷区落入暖区,在暖区上层产生更多的大雨滴,从而使暖区的云雨粒子碰并过程增强,最终地面降水增加,这是此次催化作业导致增雨的主要微物理链条。 相似文献
5.
Cirrus clouds related to transported dust layers were identified on 22 occasions with ground-based polarization lidar from December 2012 to February 2018 over Wuhan (30.5°N, 114.4°E), China. All the events occurred in spring and winter. Cirrus clouds were mostly located above 7.6 km on top of the aloft dust layers. In-cloud relative humidity with respect to ice (RHi) derived from water vapor Raman lidar as well as from ERA5 reanalysis data were used as criteria to determine the possible ice nucleation regimes. Corresponding to the two typical cases shown, the observed events can be classified into two categories: (1) category A (3 cases), in-cloud peak RHi ≥ 150%, indicating competition between heterogeneous nucleation and homogeneous nucleation; and (2) category B (19 cases), in-cloud peak RHi < 150%, revealing that only heterogeneous nucleation was involved. Heterogeneous nucleation generally took place during instances of cirrus cloud formation in the upper troposphere when advected dust particles were present. Although accompanying cloud-top temperatures ranged from –51.9°C to –30.4°C, dust-related heterogeneous nucleation contributed to primary ice nucleation in cirrus clouds by providing ice nucleating particle concentrations on the order of 10?3 L?1 to 102 L?1. Heterogeneous nucleation and subsequent crystal growth reduced the ambient RHi to be less than 150% by consuming water vapor and thus completely inhibited homogeneous nucleation. 相似文献
6.
Mineral dust particles are known to be efficient ice nuclei in the atmosphere. Previous work has probed heterogeneous ice nucleation on various laboratory dust samples including Arizona Test Dust, kaolinite, montmorillonite, and illite as atmospheric dust surrogates. However, it has recently been suggested that NX illite may be a better representation of atmospheric dust. Hiranuma et al. (2015) performed a laboratory comparison for immersion ice nucleation on NX illite, but here we focus on depositional ice nucleation because of its importance in low temperature cirrus cloud formation. A Raman microscope setup was used to examine the ice-nucleating efficiency of NX illite. Organic coatings on the NX illite particles were also investigated using a mixture of 5 dicarboxylic acids (M5). The ratio of NX illite to M5 was varied from 1:10 to 100:1. It was found that NX illite efficiently nucleates ice with Sice = 1.07 ± 0.01 at ?47 °C, with Sice slightly increasing at lower temperatures. In contrast, pure M5 is a poorer ice nucleus with Sice = 1.30 ± 0.02 at ?40 °C, relatively independent of temperature. Further, it was found that M5 coatings on the order of several monolayers thick hindered the ice nucleating ability of NX illite. Optical images suggest that at colder temperatures (< ?50 °C) 1:1 NX illite:M5 particles and pure M5 particles nucleate ice depositionally, while at warmer temperatures (> ?50 °C) subsaturated immersion ice nucleation dominates. These experiments suggest that mineral dust particles may become less active towards ice nucleation as they age in the atmosphere. 相似文献
7.
Randolph D. Borys 《Journal of Atmospheric Chemistry》1989,9(1-3):169-185
Aerosol particles were collected on filters for studies of their ability to nucleate ice during the second Arctic Gas and Aerosol Sampling Program (AGASP-II) in April, 1986. The ice nuclei (IN) samples were collected from an aircraft at altitudes ranging from the surface to the vicinity of the tropopause in Arctic locations over Alaska, northern Canada and Greenland. Samples of other components of the aerosol were collected and measurements were made of other properties of the aerosol coincident in time with the IN samples. The IN filters were exposed to water saturation in a dynamic developing chamber at –15° C and –25° C. Ice crystals grew on the IN and were counted on the filters at discrete time intervals during the exposure period to determine the rate of ice nucleation and the final concentration of (IN). Results show that Arctic haze aerosol, identified by pollutant signatures, had lower IN concentrations, a lower IN to total aerosol fraction and slower ice nucleation rates than aerosol which had a chemical signature more indicative of the remote unpolluted troposphere. These observations suggest that the Arctic haze aerosol does not efficiently form ice in the arctic troposphere. This may be a factor contributing to the long-range transport of Arctic haze. 相似文献
8.
The microphysical model with the bulk water parameterization is applied to simulated both contact and deposition nucleation as well as the imersion freezing for unseeded cases and the cases immediately after seeding performed for the cold continental Cb clouds with small cloud droplets. The injection of agent AgI is performed in temperature region between –8°C and –12°C. The four groups of sensitivity experiments are executed.
With 14 Figures 相似文献
| a. | The Brownian coagulation of rain drops is the most important contact nucleation mechanism for seeded cases with great amount of rain drops. When cloud droplets mainly contribute to the liquid water content for seeded cases, the Brownian coagulation of cloud droplets is the primary nucleation mechanism while the inertial impact is the less effective contact nucleation mechanism; |
| b. | the mutual interdependence of contact and deposition nucleation mechanisms shows that the contact nucleation is more effective for graupel production than the deposition one for the temperature region considered in this model; |
| c. | the imersion freezing is the most important mechanism for all cases with significant amount of rain drops. It is more effective than the contact nucleation mechanism in unseeded cases with insufficient number of rain drops; |
| d. | the nucleation mechanisms are more sensitive to temperature changes than to pressure changes. |
9.
Stephan Mertes Alfons Schwarzenbck Paolo Laj Wolfram Wobrock Jean-Marc Pichon Giordano Orsi Jost Heintzenberg 《Atmospheric Research》2001,58(4)
A ground-based seeding experiment using carbon dioxide and propane sprayed from pressurized bottles was carried out under supercooled cloud conditions on a small spatial and short time scale. Water vapor deposition on the artificially generated dry ice and propane ice germs as the main ice formation process (nucleation and growth) is consistent with the experimental results. After nucleation, diffusional growth of the ice particles, partly at the expense of evaporating small droplets, was identified during the mixing of the seeding line with the ambient supercooled cloud. Within the seeding plume, ice water contents up to 80% of the total condensed water are observed, although the size of the formed ice particles did not exceed 25 μm. From the changes of the ice and supercooled liquid phase with time under mixed-phase conditions, liquid water content (LWC) evaporation, ice water content (IWC) formation, and ice crystal growth rates are estimated, which are not affected by the artificial nucleation process. Thus, these rates are assessed to be applicable for a growing ice phase of small ice particles in a young mixed-phase cloud, where other growth mechanisms, like riming or aggregation, are negligible. 相似文献
10.
含水量对冰晶增长影响的风洞实验研究 总被引：1，自引：0，他引：1
用小型垂直过冷云风洞及其测试系统,使冰晶在自由悬浮的情况下生长。在实验温度为-5℃—15℃、含水量为0.5—2.0g/m~3的范围内,结果表明:在水面饱和条件下,冰晶的形状决定于所处的环境温度,含水量的大小对冰晶的基本形状没有影响,只是当含水量加大时,冰晶上会出现更加明显的碰冻增长的痕迹;冰晶的质量和速度增长的峰值和谷值温度分布与含水量的大小无关;随着含水量的增加,冰晶的质量和下落速度的增长会加快,但没有发现含水量的增加有加快冰晶2a轴增长的明显效果。 相似文献
11.
播撒碘化银粒子进行人工防雹的数值试验 总被引：16，自引：13，他引：16
本文在二维完全弹性冰雹云数值模式中，引入冰晶浓度和播撒物质AgI粒子的守恒方程，建立了一个二维催化模式，考虑了人工冰核的三种成核机制，即凝华核化（包含凝结—冻结核化）及与云、雨滴的接触冻结核化，模拟了几种不同冰雹云、不同催化方案下的人工防雹催化效果，指出了防雹的最佳催化方案和适宜催化作业的冰雹云条件。 相似文献
12.
Paolo Laj Andrea I. Flossmann Wolfram Wobrock Sandro Fuzzi Giordano Orsi Loretta Ricci Stephan Mertes Alfons Schwarzenbck Jost Heintzenberg Harry Ten Brink 《Atmospheric Research》2001,58(4):256
We investigated the partitioning of trace substances during the phase transition from supercooled to mixed-phase cloud induced by artificial seeding. Simultaneous determination of the concentrations of H2O2, NH3 and black carbon (BC) in both condensed and interstitial phases with high time resolution showed that the three species undergo different behaviour in the presence of a mixture of ice crystals and supercooled droplets. Both H2O2 and NH3 are efficiently scavenged by growing ice crystals, whereas BC stayed predominantly in the interstitial phase. In addition, the scavenging of H2O2 is driven by co-condensation with water vapour onto ice crystals while NH3 uptake into the ice phase is more efficient than co-condensation alone. The high solubility of NH4+ in the ice could explain this result. Finally, it appears that the H2O2–SO2 reaction is very slow in the ice phase with respect to the liquid phase. Our results are directly applicable for clouds undergoing limited riming. 相似文献
13.
层状云催化后过冷水分布与演变规律的数值模拟 总被引：4，自引：4，他引：4
在郭学良等(1999年)发展的层状云雨滴分档模式中加入冰晶繁生过程,模拟了碘化银和液态二氧化碳的催化效率以及催化后云中过冷水的分布与演变过程.结果表明:碘化银和液态二氧化碳在5200～5600 m高度上的催化效率相当,最大达到11.1%;液态二氧化碳在2600～3000 m高度层的催化效率明显增大,达到14.2%;模式云被催化后,云中云水含量在200 min都较未催化时增长0.05 g/m3以上,表现出云中过冷水被消耗后的恢复趋势;碘化银和液态二氧化碳对云体催化后,云中水汽含量减少0.5～2 g/m3,对过冷水的恢复作出贡献;催化过程使得模式云中雨滴浓度在210 rin时较未催化时减少73%,在240 min时较未催化时增加309%.得出了两点结论:(1)模式云被催化后,云中过冷水在200 rin表现出恢复趋势,云中水汽对过冷水的恢复过程作出了贡献;(2)在过冷水较多的区域播撒液态二氧化碳可以取得较好的催化效率. 相似文献
14.
碘化银（AgI）类催化剂是人工影响天气外场试验和业务作业中使用最广泛的催化剂,其核化效率和核化机制在很大程度上影响催化效果。在总结美国、中国和欧洲多个国家利用云室和风洞研究AgI类催化剂的核化机制、核化阈温及成核率的室内实验成果的基础上,梳理利用室内实验成果发展的AgI数值催化模式,旨在为下一步优选新型高效AgI类催化剂和改进数值催化模式提供借鉴。AgI类催化剂核化机制包括凝华核化、接触冻结核化、凝结冻结核化和浸没冻结核化,其核化过程受大气温湿条件、催化剂粒子大小、成分等多种因素影响,并与催化剂粒子的燃烧溶液法、燃烧焰剂法和爆炸法等发生方式有关。目前国内外使用的AgI类催化剂含有不同成分,有多种催化剂粒子产生方式,催化剂粒子的核化机制和成核率有很大差异。将来应重点基于高性能云室和风洞,分析不同催化剂配方的核化机制和成核率,优选新型高效催化剂,改进AgI数值催化模式。 相似文献
15.
三维对流云催化数值模式人工冰晶参数化方案的改进与个例模拟试验 总被引：3，自引：0，他引：3
在中国科学院大气物理研究所的三维全弹性对流风暴云催化数值模式(简称为IAP-CSM3D)的基础上,对模式中催化部分的参数化方案进行了改进,推导出人工冰晶与其它粒子之间相互作用的微物理过程的参数化方程。改进后的模式将催化产生的人工冰晶单独作为预报量进行处理,把人工冰晶与自然冰晶区分开,且考虑的人工冰晶谱型为双参数粒子谱,使模式更符合实际。利用改进后的模式模拟了2005年7月8日发生在辽宁省朝阳市的一次冰雹云天气过程,着重分析了催化云人工冰晶的微物理过程、空间分布和谱型,以及对冰相降水粒子的贡献。数值试验表明,自然雹云模拟结果与观测事实相吻合,说明改进后的模式对冰雹云具有较可靠的模拟能力。模拟分析表明,冻滴是该例自然雹云冰雹胚胎的主要来源,对该冰雹云进行AgI催化可明显地减少降雹量,特别是在云中冰雹形成初期进行催化防雹效果最好,既可产生最大的防雹作业效果又不至于过度减少降雨量。催化减雹的主要原因是催化显著地减少了云中冻滴向冰雹胚胎的转化总量。进一步研究发现,人工冰晶在云的不同阶段对各种冰相降水粒子的贡献是不同的。人工冰晶对雪花总质量的贡献较小,对霰总质量的贡献有所增大,而对冻滴总质量的贡献较大。模拟的冰晶粒子谱可较好地反映出人工冰晶谱型较窄,浓度较大,尺度较小的特征。 相似文献
16.
不同云底温度雹云成雹机制及其引晶催化的数值研究 总被引：24，自引：1，他引：23
用二维准弹性冰雹云模式模拟了中国不同地区的冰雹云的成雹机制和人工引晶催化的效果,结果表明：强对流云中自然初始降水元的形成主要同云雨自动转化相关;云底温度较低的冰雹云的雹胚形成以云霰转化过程为主,暖云底的雹云则以雨霰转化为主。人工引晶的作用有三：（１）加强云中冰霰转化过程,雹胚过多争食防雹;（２）促进雨霰转化过程,使雹胚浓度增加,并且减少过冷雨滴,抑制冰雹碰冻过冷雨滴的增长;（３）使云的下部霰量增加,降低降水粒子的增长轨迹,阻碍霰雹的增长。多次催化有时比一次大剂量催化的防雹增雨效果好。 相似文献
17.
云数值模拟是研究降雹过程和人工防雹试验的重要手段。利用三维冰雹云AgI催化模式,对北京1996年6月10日的一次降雹过程进行AgI不同催化高度、催化剂量和催化时间的系列催化模拟试验,并优选催化方案,为外场防雹设计和作业提供依据。在催化系列模拟中发现,不同催化高度的催化剂均在上升到-5℃高度后开始核化。在2.1~4.9 km高度范围内催化,AgI成核率比较高,防雹效果较好。核化的人工冰晶有效弥补了该高度上自然冰晶的不足。小剂量催化,可在减雹的同时增加部分降雨量,而大剂量催化,在减雹的同时会减少降雨。在催化时间、剂量和高度的系列催化试验中得出,采用在模拟的第15分钟在5 km高度附近播撒AgI,连续4次以5×106 kg-1的催化剂量进行催化,催化效果较好,可减少降雹量约60%,同时可避免降雨量的大幅减少。 相似文献
18.
将云滴冻结方案植入已有的二维雷暴云起、放电模式,结合一次山地雷暴个例,探讨了气溶胶浓度对雷暴云微物理过程、起电以及空间电荷结构的影响。结果表明:气溶胶浓度增加,云滴数目增多,尺度降低,雨滴含量减少;云滴冻结导致冰晶在低温区快速生长,冰晶数浓度增加,尺度减小,当气溶胶浓度高于1000 cm-3后小冰晶难以增长成大尺度的霰粒子,因此霰粒子数浓度先增加后急剧减少。此外,气溶胶浓度的大小不会影响雷暴云的电荷结构特征,但会对云内的起电强度产生明显的作用:当气溶胶浓度较低时,增加气溶胶浓度,更多的冰晶和霰粒子发生碰撞使得云内起电过程增强,空间电荷密度增加;当气溶胶浓度高于1000 cm-3后,少量的霰粒子和小冰晶的出现抑制了非感应起电过程,导致电荷密度降低。 相似文献
19.
减弱对流云降水的AgI催化原理的数值模拟研究 总被引：3，自引：0，他引：3
在对流云模式中增加了AgI两个预报量,耦合了考虑受水汽过饱度和温度影响的4种核化机制的AgI催化模块,使其具备了对AgI类催化剂的模拟能力,能够研究AgI类催化剂对对流云系统的影响。利用该模式对一次华南对流云降水过程进行了AgI催化数值模拟试验,对人工减缓对流云降水的可能性及原理进行了研究。模拟结果表明,在适当的时机对适当的部位进行大剂量的催化,可以减少总降水量,也可以减少最大降水中心的雨强。当催化浓度达到2×10~8 kg~(-1)时,可以减少32%的降水量,具备有效减缓对流云降水的可能性。大剂量催化后,大量的AgI粒子在冷区核化后,消耗了大量的过冷水。催化后霰粒子的落速和雨水的落速减小。催化阶段由于霰融化成雨水减少而使降水减弱。催化结束后在霰融化成雨水增多的情况下,雨水的蒸发大幅增加,从而导致了降水量的持续减少。AgI在模拟的强对流云中主要以受过饱和度影响的凝结冻结和催化剂长时间作用的浸没冻结这两种方式成核。研究所用催化方法在外场作业中具有技术可行性。 相似文献
20.
Abstract Past theoretical investigations have reported that observed peaks in the diffusional growth of ice crystals in the vicinity of ‐5 and ‐15°C could be qualitatively modelled assuming certain specific crystal properties. This study re‐examines the ice crystal diffusional growth model using more recently available observations of pertinent crystal parameters. The results, indicative of the growth of average crystals, imply a much weaker dependence of the diffusional mass growth rate on temperature in the range of ‐5 to ‐15°C. Extension of the model to include growth by accretion, also suggests that the mass of heavily rimed crystals is not very sensitive to the original crystal habit. The results of the calculations are compared with observed crystal sizes in cumulus clouds following seeding on three different days. The observations indicate that small crystals were continuously being produced as long as 15 min after seeding. In two cases, crystals much larger than those predicted by the model for any reasonable set of parameters suggest that crystal aggregation may have been occurring at a significant rate. 相似文献