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1.
In the Suo-Nada area of the Seto Inland Sea, Japan, sedimentation rates and the sedimentary record of anthropogenic metal loads were determined by combining the Pb-210 dating technique with heavy metal analysis of the sediments. The sedimentation rates vary from 0.11 to 0.27 g cm–2 yr–1. Lower sedimentation rates were observed in the eastern part of the basin which is characterized by a bottom with sand and gravel, and fast tidal currents.Anthropogenic and natural loads of copper and zinc into the sediments are 34 and 326, and 65 and 375 ton yr–1, respectively. The anthropogenic loads are fairly low compared with those of the other main areas of sediment accumulation in the Seto Inland Sea. The highest level of zinc and copper pollution was observed in the western part of the basin because of waste discharge from an old and big ironworks outside basin since the early 1900's.  相似文献   

2.
The metal load into sediments and the change in the sedimentary environment of Osaka Bay in the Seto Inland Sea have been studied through geochemical analysis of core sediments, using both Pb-210 dating and a selective chemical leaching technique. Analytical results from a 6-m core of sediment show that copper and zinc pollution started in the late 1800's and the present enrichment ratios of copper and zinc, relative to background levels (20 mg kg–1 for Cu and 94 mg kg–1 for Zn), are 2.8 and 4.1, respectively. The present anthropogenic copper and zinc loads into Osaka Bay sediments, are 47 and 368 ton yr–1, while natural copper and zinc loads are 40 and 186 ton yr–1, respectively. Osaka Bay sediment at the present day is considered to be seriously polluted by zinc, now. The vertical profiles of copper and zinc in four successively separated fractions (10% acetic acid soluble fraction: F-HAC, 0.1M hydrochloric acid-soluble fraction: F-HCl, hydrogen peroxide-soluble fraction: F-H2O2 and hydrofluoric acid-soluble fraction: F-HF) from the core sediments indicate that enrichments of copper and zinc in the upper layer of the sediment are dependent on increases in the metal contents of the F-HAC, F-HCl and F-H2O2 fractions. Copper in F-HAC, and zinc in F-HAC and F-HCl, seem to be of anthropogenic origin.Results of sequential studies of the whole Seto Inland Sea can be summarized as follows: At the present time, the sedimentary loads of copper and zinc over the whole Seto Inland Sea area are 630 and 3,500 ton yr–1, respectively, while the natural and anthropogenic loads are 320 and 310 ton yr–1 for copper and 1,800 and 1,700 ton yr–1 for zinc, respectively.  相似文献   

3.
Sedimentation rates in ten sediment cores from Hiroshima Bay in the Seto Inland Sea of Japan were determined with the |2210|0Pb technique, and heavy metals were analyzed. The sedimentation rates vary from 0.18 to 0.33 g cm|2-2|0 yr|2-1|0. The highest sedimentation rates were observed in the northern part of the bay at the mouth of Ota River, while lower sedimentation rates not more than 0.20 g cm−2 yr−1 were observed at stations close to narrow water-ways, or where water depth was shallow. The contents of copper and zinc in the sediment cores began to increase around 1930 as a result of increased human activity, and have remained almost unchanged since 1970 possibly because of regulation of pollutant discharge. The natural background values of copper and zinc in the sediment of this bay range from 16 to 27 mgkg−1 and 70 to 105 mg kg−1, respectively. The total amounts of anthropogenic copper and zinc deposited in the sediments since about 1930 are estimated to be 0.5–2.7 ton km−2 and 2.2–14.5 ton km−2, respectively. At the present-day, the anthropogenic loads of copper and zinc to the sediments of the whole bay are 26 ton yr−1 and 183 ton yr−1, and these values constitute 39% and 48% of the total sedimentary loads at the present-day, respectively.  相似文献   

4.
Sedimentation rates were determined with the210Pb technique in six sediment cores from Harima Nada (Harima Sound), Seto Inland Sea. The rate of deposition varies from 0.11 g cm–2y–1 in the northern part to 0.33 g cm–2 y–1 in the southern part of the basin. A marked increase in copper and zinc content was observed above a depth in the core corresponding to about 1900 A.D. as a result of increasing human activities. Anthropogenic input of copper and zinc decreased slightly after 1970. Natural background levels of copper and zinc in the sediment in this sound are 11–16 ppm and 100–120 ppm, respectively. The total amounts of anthropogenic copper and zinc in the sediments were estimated to be 110–180g cm–2 and 610–1,280g cm–2, respectively. These values constitute 40–50% of the total sedimentary input of copper and zinc in the sediments since about 1900 A.D.  相似文献   

5.
Sedimentary core samples were collected from Mikawa Bay and analyzed for organic C, N and P, carbohydrate and protein including amino acids. Sedimentation rates for each of the core samples were found to lie in the range of 0.21–0.24 g cm–2yr–1 by the210Pb method. Degradation rate constants of organic C, N and P, carbohydrate and protein including amino acids had ranges of 3.8–5.5, 4.7–5.9, 6.3–7.4, 5.7–6.8 and 3.9–6.8×10–2yr–1, respectively. The rate of degradation of organic matter in the sediment was also calculated and is discussed in relation to the flux of particulate organic matter to the surface of the sediment.  相似文献   

6.
Profiles of 210Pb and 239 + 240Pu from sediment cores collected throughout Massachusetts Bay (water depths of 36–192 m) are interpreted with the aid of a numerical sediment-mixing model to infer bioturbation depths, rates and processes. The nuclide data suggest extensive bioturbation to depths of 25–35 cm. Roughly half the cores have 210Pb and 239 + 240Pu profiles that decrease monotonically from the surface and are consistent with biodiffusive mixing. Bioturbation rates are reasonably well constrained by these profiles and vary from 0.7 to 40 cm2 yr−1. As a result of this extensive reworking, however, sediment ages cannot be accurately determined from these radionuclides and only upper limits on sedimentation rates (of 0.3 cm yr−1) can be inferred. The other half of the radionuclide profiles are characterized by subsurface maxima in each nuclide, which cannot be reproduced by biodiffusive mixing models. A numerical model is used to demonstrate that mixing caused by organisms that feed at the sediment surface and defecate below the surface can cause the subsurface maxima, as suggested by previous work. The deep penetration depths of excess 210Pb and 239 + 240Pu suggest either that the organisms release material over a range of >15 cm depth or that biodiffusive mixing mediated by other organisms is occurring at depth. Additional constraints from surficial sediment 234Th data suggest that in this half of the cores, the vast majority of the present-day flux of recent, nuclide-bearing material to these core sites is transported over a timescale of a month or more to a depth of a few centimeters below the sediment surface. As a consequence of the complex mixing processes, surface sediments include material spanning a range of ages and will not accurately record recent changes in contaminant deposition.  相似文献   

7.
Modern and Holocene muddy strata were studied along the shoreline adjacent to the Amazon river mouth using sedimentological, radiochemical, physical, and seismic methods. The present paper is a synthesis of the results, collected during the AmasSeds project, that is used to outline a regional shoreline sediment budget. Erosion of relict Amazon muds in southern Amapa supplies 106 tons yr–1 to the Amazon advective mud stream. Local rivers are sediment-poor (total suspended discharge ~ 1 × 106 tons yr–1), but form depositional sandflats on the shoreface downdrift of the river mouths. Mudflat accumulation in northern Amapa sequesters 106–107 tons yr–1 by tidal-flat aggradation, alongshore mudcape accretion, and sediment trapping by mangroves. The processes temporarily store 1.5 × 108 tons of Amazon mud in January–June.  相似文献   

8.
Undisturbed sediment cores were collected by a modified gravity corer from Funka Bay. The sedimentation rate is determined by both210Pb and pumice chronological methods. The sedimentation rates by210Pb method are concordant with those by pumice methods. The derived rate varies from 0.06 to 0.22 g cm–2 y–1, and an average is 0.09 g cm–2 y–1.  相似文献   

9.
A sulfur budget for the Black Sea anoxic zone   总被引：1，自引：0，他引：1  
A budget for the sulfur cycle in the Black Sea is proposed which incorporates specific biogeochemical process rates. The average sulfide production in the water column is estimated to be 30–50 Tg yr−1, occurring essentially in the layer between 500 and 2000 m. About 3.2–5.2 Tg sulfide yr−1 form during sulfate reduction in surface sediments of the anoxic zone. Total sulfur burial in anoxic sediments of 1 Tg yr−1 consists of 10–70% (ca. 40–50% is the average) water column formed (syngenetic) component, the rest being diagenetic pyrite. As a maximum, between 3 and 5 Tg yr−1 contribute sulfide to the bottom water or diffuse downward in the sediment. About 20–50 Tg yr−1 sulfide is oxidized mostly at the chemocline and about 10–20% of this amount (4.4–9.2 Tg yr−1) below the chemocline by the oxygen of the Lower Bosphorus Current. A model simulating the vertical distribution of sulfide in the Black Sea water column shows net consumption in the upper layers down to ca. 500 m, essentially due to oxidation at the chemocline, and net production down to the bottom. On the basis of the calculated budget anoxic conditions in the Black Sea are sustained by the balance between sulfide production in the anoxic water column and oxidation at the chemocline. On average the residence time of sulfide in the anoxic zone is about 90–150 yr, comparable to the water exchange time between oxic and anoxic zones. Hydrophysical control on the sulfur cycle appears to be the main factor regulating the extent of anoxic conditions in the Black Sea water column, rather than rates of biogeochemical processes.  相似文献   

10.
The detailed flow structure around a tical front in Hiuchi-Nada, Japan was observed with the use of ADCP (Acoustic Doppler Current Profiler). The surface convergence region is observed at the transition zone between vertically well mixed area and the stratified area. The surface divergence regions exist next to the surface convergence region. The strong downward current is estimated in the middle layer just below the surface convergence region. The maximum surface convergence and the maximum downward velocity in the middle layer are 1.0×10–4 s–1 and 0.12 cm s–1, respectively.  相似文献   

11.
The Bay of Concepcion (36°40′S; 73°02′W) is a semi-enclosed and shallow embayment in which biogeochemical processes are seasonally coupled to coastal upwelling during the austral spring and summer. The nutrient cycle in the bay is complex due to the combined effects of a pronounced O2 minimum layer and high nutrient concentrations both originating from subsurface equatorial water during coastal upwelling and a rapid rate of sediment nutrient recycling. The sediments are characterized by a high content of organic matter mainly due to the extremely high rates of phytoplankton production and deposition. During the upwelling period, a black flocculent layer frequently covers the sediment–water interface in the inner part of the bay where an extensive mat of Beggiatoa spp. develops. Three approaches are used to analyse the extent to which the benthic system recycles or retains nutrients at two stations, located at the centre (station C, St. C) and mouth (station B, St. B) of the bay for a 1-year period (March 1996–1997): (1) estimation of C and N remineralization rates based on SO42− reduction measurements, (2) calculation of C and N turnover rates using a diagenetic model applied to total organic carbon and total nitrogen vertical distributions and, (3) construction of C and N budgets from direct measurements of sedimentation (from a sediment trap) and estimates of the C and N burial rates. Depth-integrated SO42− reduction rates varied between 3.4 (winter) and 25.5 (summer) mmol m−2 d−1. Estimated C and N oxidation rates ranged between 7.9 and 87.8 mol C m−2 yr−1 and between 0.9 and 6.9 mol N m−2 yr−1, respectively. Each approach yielded minor differences in the C and N remineralization rates (and also minor differences between both studied stations), except when the kinetic model was applied to C and N distribution without including the presence of the flocculent layer. The rates of carbon oxidation and sulphate reduction were considerably higher than in other coastal sediments with similar depositional regime. The C and N burial rates were 2.23 and 0.21 (St. C) and 1.30 and 0.09 (St. B) mol m−2 yr−1, respectively. The C/N ratio of the buried fraction was ca. 10.6 at St. C and 14.4 at St. B. Because the observed differences in burial rates could not be ascribed to distinctive depositional (both stations have similar sediment accumulation rates) and oceanographic (similar O2 concentration and hydrography) conditions, differences may be due to in part spatial heterogeneity in the supply of organic matter. The degree of preservation of organic matter as plankton detritus and nitrogen accumulating bacterial biomass associated with Beggiatoa spp. at St. C may also be involved.  相似文献   

12.
Within the framework of the EU-funded BENGAL programme, the effects of seasonality on biogenic silica early diagenesis have been studied at the Porcupine Abyssal Plain (PAP), an abyssal locality located in the northeast Atlantic Ocean. Nine cruises were carried out between August 1996 and August 1998. Silicic acid (DSi) increased downward from 46.2 to 213 μM (mean of 27 profiles). Biogenic silica (BSi) decreased from ca. 2% near the sediment–water interface to <1% at depth. Benthic silicic acid fluxes as measured from benthic chambers were close to those estimated from non-linear DSi porewater gradients. Some 90% of the dissolution occurred within the top 5.5 cm of the sediment column, rather than at the sediment–water interface and the annual DSi efflux was close to 0.057 mol Si m−2 yr−1. Biogenic silica accumulation was close to 0.008 mol Si m−2 yr−1 and the annual opal delivery reconstructed from sedimentary fluxes, assuming steady state, was 0.065 mol Si m−2 yr−1. This is in good agreement with the mean annual opal flux determined from sediment trap samples, averaged over the last decade (0.062 mol Si m−2 yr−1). Thus ca. 12% of the opal flux delivered to the seafloor get preserved in the sediments. A simple comparison between the sedimentation rate and the dissolution rate in the uppermost 5.5 cm of the sediment column suggests that there should be no accumulation of opal in PAP sediments. However, by combining the BENGAL high sampling frequency with our experimental results on BSi dissolution, we conclude that non-steady state processes associated with the seasonal deposition of fresh biogenic particles may well play a fundamental role in the preservation of BSi in these sediments. This comes about though the way seasonal variability affects the quality of the biogenic matter reaching the seafloor. Hence it influences the intrinsic dissolution properties of the opal at the seafloor and also the part played by non-local mixing events by ensuring the rapid transport of BSi particles deep into the sediment to where saturation is reached.  相似文献   

13.
Sedimentation rates were determined for the northern Gulf of Mexico margin sediments at water depths ranging from 770 to 3560 m, using radiocarbon determinations of organic matter. Resulting sedimentation rates ranged from 3 to 15 cm/kyr, decreasing with increasing water depth. These rates agree with long-term sedimentation rates estimated previously using stratigraphic methods, and with estimates of sediment delivery rates by the Mississippi River to the northern Gulf of Mexico, but are generally higher by 1–2 orders of magnitude than those estimated by 210Pbxs methods. Near-surface slope sediments from 2737 m water depth in the Mississippi River fan were much older than the rest. They had minimum 14C ages of 16–27 kyr and δ13C values ranging from −24‰ to −26.5‰, indicating a terrestrial origin of organic matter. The sediments from this site were thus likely deposited by episodic mass wasting of slope sediment through the canyon, delineating the previously suggested main pathway of sediment and clay movement to abyssal Gulf sediments.  相似文献   

14.
 Recent sediment accumulation rates are 18–230 mg cm-2 yr-1 (0.02–0.2 cm yr-1) based on excess 210Pb activity profiles in the southwestern part of the East Sea (Sea of Japan). Assuming no mixing beneath surface mixed layers, 210Pb-derived sediment accumulation rates are 18–32 mg cm-2 yr-1 in the northern part of the Yamato Ridge and the Ulleung Basin, 29–136 mg cm-2 yr-1 in the Korea Plateau, and 230 mg cm-2 yr-1 in the southern shelf. These values generally agree with long-term sedimentation rates estimated from dated ash layers. Received: 6 October 1995 / Revision received: 31 May 1996  相似文献   

15.
The Role of Suspended Oyster Culture on Nitrogen Cycle in Hiroshima Bay   总被引：1，自引：0，他引：1  
The predominance of bivalves affects the cycle of materials in the coastal ecosystem. In the present study, the role of suspended oyster culture on the nitrogen cycle was demonstrated for the northern Hiroshima Bay. The nitrogen cycle was considered as two systems, (1) the primary production (PP) system and (2) the oyster culture (OC) system. The results show that about 26% of N productivity was supplied to process by cultured oysters in the OC system. This process varies seasonally due to the seasonal variations of PON, physiological activities and biomass of oysters. The N processing rates were found to be high in summer and low in winter. The biodeposition and excretion of N in the OC system are 3.0 and 2.1 ton N d–1, while the natural sedimentation rate and N regeneration in the PP system are 8.3 and 18.0 ton N d–1, which indicates that the PP system is a major system regenerating N in the water column. The release of total dissolved N from the bottom to the water column is about 8.3 ton N d–1. The amount of N harvested as oyster product was about 1.3 ton N d–1, which is about 10% of daily N loading in north Hiroshima Bay. According to the N cycle developed in the present study, the results suggest the significant role of suspended oyster culture on the nitrogen cycle in Hiroshima Bay. In addition, our results indicate that oyster production was efficiently harvested, suggesting that oyster culture could probably be used as a tool to remove N from Hiroshima Bay.  相似文献   

16.
Rivers draining into the Gulf of Papua (GOP) from the Papua New Guinea mainland deliver approximately 340 × 106 t yr–1 of sediment to the marine environment. The terrestrially derived sediment contains 1.1 ± 0.2% particulate organic carbon with a carbon-isotope composition of –26.5 ± 0.2, and amounts to 3.7 ± 0.7 × 106 t yr–1. The carbon-isotope composition of sediments in the Gulf of Papua indicates that 40% of the sediment cover contains 75% or more terrestrially derived carbon. Suspended sediments that are transported beyond the delta complex of the Fly River are transported north and northwest, augmented by sediments from other rivers along the coast of the GOP. The carbon-isotope results suggest that a significant quantity of terrestrially derived sediment escapes from the GOP, either along the coastlines to east and west or into the deep ocean via the Moresby and Pandora troughs. Little sediment travels south onto the Great Barrier Reef shelf. Extrapolating the results from this study to the region of Oceania suggests a total flux of particulate organic carbon to the world's oceans from the islands of Oceania of ~ 90 × 106 t yr–1 or twice the flux of riverine POC from the major rivers of North America, South America, and Africa combined. While such a calculation must be considered illustrative only, the similar tectonic, geomorphologic, and climatic features of the islands of Oceania suggest that the calculation is unlikely to be grossly in error and that the rivers of Oceania therefore represent a major but poorly documented source of sediment and organic carbon to the global ocean.  相似文献   

17.
Sulfate reduction in deep coastal marine sediments   总被引：1，自引：0，他引：1  
Sulfate reduction rates in sediments of four deep stations in the Saguenay Fjord and the Laurentian Trough, Gulf of St. Lawrence, are among the lowest reported for the coastal environment. Maximum rates were 0.4–7.0 nmol cm−3 day−1. The low rates are due to relatively low sedimentation rates and continuously low temperatures. Regional differences in both integrated and maximum sulfate reduction rates in the sediment correlate with sediment trap measurements of sedimentation rate and organic carbon flux.Sulfate reduction accounts for the degradation of 5–26% of the estimated downward flux of organic matter to these sediments. Unlike the absolute rate of sulfate reduction, the relative proportion of the carbon flux that is degraded via sulfate reduction is not directly correlated with the sedimentation rate but is a function of organic matter composition, intensity of bioturbation, and the abundance of sub-oxic electron acceptors. Thus, the lowest proportion of carbon degradation via sulfate reduction occurred at a Gulf site, where a combination of low sedimentation and bioturbation rates allowed a long residence time for organic matter near the sediment surface and, in consequence, a low flux of labile carbon into the sulfate reduction zone. The highest proportion was observed at a station with a similar organic carbon flux but with higher rates of sedimentation and bioturbation. At a third site, with the highest rates of sulfate reduction as well as the highest rates of sedimentation and bioturbation, the contribution of sulfate reduction to organic matter degradation was only intermediate. This is attributable to the exhaustion of the supply of porewater sulfate. In deep coastal environments the proportion of organic matter degraded via sulfate reduction can be highly variable both spatially and temporally.  相似文献   

18.
An array of five bottom-tethered moorings with 19 PARFLUX time-series sediment trap at three depths (1 and 2 km below the surface, and 0.7 km above the sea-floor) was deployed in the western Pacific sector of the Southern Ocean, along 170°W. The five stations were selected to sample settling particles in the main hydrological zones of the Southern Ocean. The sampling period spanned 425 days (November 28, 1996–January 23, 1998) and was divided into 13 or 21 synchronized time intervals. A total of 174 sequential samples were recovered and analyzed to estimate fluxes of total mass (TMF), organic carbon, carbonate, biogenic silica, and lithogenic particles. The fluxes of biogenic material were higher than anticipated, challenging the notion that the Southern Ocean is a low-productivity region. Organic carbon fluxes at 1 km depth within the Polar Frontal Zone and the Antarctic Zone were relatively uniform (1.7–2.3 g m−2 yr−1), and about twice the estimated ocean-wide average (ca. 1 g m−2 yr−1). Carbonate fluxes were also high and uniform between the Subantarctic Front and ca. 64°S (11–13 g m−2 yr−1). A large fraction of the carbonate flux in the Antarctic Zone was due to the presence of pteropod shells. Coccoliths were found only to the north of the Polar Front, and calcium carbonate became the dominant phase in the Subantarctic Zone. In contrast, carbonate particles were nearly absent near 64°S. Latitudinal variations in biogenic silica fluxes were substantial. The large opal flux (57 g m−2 yr−1) measured in the Antarctic Zone suggests that opal productivity in this region has been previously underestimated and helps to explain the high sedimentary opal accumulation often found south of the Polar Front. Unlike biogenic material, fluxes of lithogenic particles were among the lowest measured in the open-ocean (0.12–0.05 g m−2 yr−1), reflecting a very low dust input.  相似文献   

19.
The vertical distribution patterns of grain-size parameters, carbonate and organic carbon contents, and clay mineral abundances were examined in ten sediment cores from basins of the northern Aegean Sea. Sedimentation rates for Holocene deposition were determined on the basis of 11 14C datings and indirectly from the age of the lower sapropel S1; they were estimated at 14.9, 18.9–21.8 and 34.7 cm 103 year–1 for the North Skyros, Athos, and North Limnos basins respectively. The sedimentation rates decrease gradually towards the southern basins, as a consequence of the greater distance from sediment supply sources. Also, sedimentation rates appear to decrease from the last glacial to Holocene units. The clay minerals illite, smectite, kaolinite and chlorite were identified in the cores. Generally, illite is the predominant mineral, showing a north–south-decreasing trend, followed by smectite; both minerals have a terrigenous origin, and smectite occurrence is higher in basins located near Limnos Island where volcanic formations prevail. Terrigenous illite is abundant in the sapropel S1, exhibiting the highest content of all sedimentological units. High illite content is unusual in eastern Mediterranean sapropels. This pattern is attributed to the proximity of the N. Aegean Sea basins to Balkan and Turkish land sources. In general, sediment mass gravity flow processes coupled with seasonal deposition from nepheloid layers are the predominant sedimentation mechanisms in the N. Aegean basins. The relative sea-level stand, the proximity to terrigenous sources (rivers), the morphology of the N. Aegean basins (small dimensions, isolated, steep slopes), as well as seismic activity and strong bottom currents are probably the major factors controlling sedimentation in the region.  相似文献   

20.
Standing stocks and production rates of phytoplankton and planktonic copepods were investigated at 15 stations in the Inland Sea of Japan during four cruises in October–November 1979, January, April and June 1980. The overall mean of phytoplankton biomass was relatively constant during the study period, ranging from 2.3 mg chl.a m–3 in April to 3.6 mg chl.a m–3 in October–November. Primary production was low in January (mean: 90 mg C m–2 d–1), but higher than 375 mg C m–2 d–1 on the other occasions. Integrated annual primary production was 122 g C m–2 yr–1. In terms of carbon weight,Paracalanus parvus was the most important copepod species. The variation of the mean copepod biomass (range: 7.6 mg C m–3 in April to 20.2 mg C m–3 in June) was smaller than that of copepod production, which was estimated by the Ikeda-Motoda's physiological method. Copepod producion was low in cold seasons (0.6 and 0.9 mg C m–3 d–1 in January and April, respectively), and increased, following the elevation of primary production, to 4.9 mg C m–3 d–1 in June. Annual copepod production was 33.7 g C m–2 yr–1, of which herbivore (secondary) production was 26.4 g C m–2 yr–1 (21.7% of primary production). The ratios of pelagic planktivorous fish catch and total fish catch to the primary production were 0.82 and 1.8%, respectively, indicating very high efficiency in exploiting fishery resources in the Inland Sea of Japan.  相似文献   

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