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1.
Hydrogeochemical processes controlling surface water chemistry were examined in five small (<1.5 km 2) forested catchments that have contrasting bedrock lithologies of granite, and conglomerate, and are distributed in the southeast of Seto district, central Japan. Watersheds developed on these two bedrocks differ in their ability to neutralize atmospheric acid (pH ~4.5) deposition. The study was conducted to (1) characterize the hydrogeochemical processes controlling surface water chemistry, and (2) to elucidate acidification of spring and stream waters using data from three sampling campaigns conducted from August to October 2000. Stream and spring water solutes fall into two general groups according to concentration: alkaline, relatively high pH (5.2–7.7) and high cation concentrations (HCO 3 -, Cl -, base cations), and dilute, low pH (4.2–5.5) waters. Concentrations of trace metals (Al, Ba, Sr) showed a strong negative correlation with pH, suggesting the mobility of these metals in the dissolved load of catchments underlain by Tokai conglomerate. The strontium isotope ratio ( 87Sr/ 86Sr) of rock and soil, plant, precipitation, and surface water samples was used to identify different reservoirs within the ecosystem. Low Si concentrations in stream and spring waters from the conglomerate area, with a relatively high pool of SiO 2, >90 (wt%), suggest slow chemical weathering. The dissolved solute concentrations are generally of similar magnitude in stream waters within the catchments of similar bedrock lithology. The high inverse correlation ( r 2=0.72) between pH and SO 4 – concentrations and the high positive correlation ( r 2 =0.90) between Ba and SO 4 – concentrations in waters draining Tokai conglomerate suggest that barite (BaSO 4) is being dissolved in an acidic environment. The three catchments were identified as being sensitive to acidic deposition because the bedrock conglomerate provided little capacity to buffer acidic inputs. The soils from the granite area have a high cation-exchange capacity (CEC an average of 868 µmol/kg), and are nearly ten times greater than the soils from the conglomerate area. Because ion exchange, besides weathering, is the main source that counteracts soil acidification, the sensitivity to further acidification may increase.  相似文献   

2.
《Applied Geochemistry》2000,15(3):311-325
Barium/Sr and Ca/Sr ratios have been used to model the relative importance of different sources of stream water. Major and trace element concentrations together with 87Sr/86Sr ratios were measured in precipitation, soil water, groundwater and stream water in a small (9.4 km2) catchment in northern Sweden. The study catchment is drained by a first order stream and mainly covered with podzolized Quaternary till of granitic composition. It is underlain by a 1.8 Ga granite. A model with mixing equations used in an iterative mode was developed in order to separate the stream water into 3 subsurface components: soil water, shallow groundwater, and deep groundwater. Contributions from precipitation are thus not included in the model. This source may be significant for the stream water generation, but it does not interfere with the calculations of the relative contributions from the subsurface components. The results show that the deep groundwater constitutes between 5 and 20% of the subsurface water discharge into the stream water. The highest values of the deep groundwater fraction occur during base flow. Soil water dominates during snowmelt seasons, whereas during base flow it is the least important fraction. Soil water accounts for 10–100% of the subsurface water discharge into the stream water. Shallow groundwater accounts for up to 80% of the subsurface water discharge with the lowest values at peak discharge during snowmelt seasons and the highest values during base flow. The validity of the model was tested by comparing the measured 87Sr/86Sr ratios in the stream water with the 87Sr/86Sr ratios predicted by the model. There was a systematic difference between the measured and modelled 87Sr/86Sr ratios which suggests that the fraction of soil water is overestimated by the model, especially during spring flood. As a consequence of this overestimation of soil water the amount of shallow groundwater is probably underestimated during this period. However, it is concluded that the differences between measured and predicted values are relatively small, and that element ratios are potentially effective tracers for different subsurface water flowpaths in catchments.  相似文献   

3.
The Yacoraite River and its tributaries run down the eastern slope of the Aguilar Range. It is one of the tributaries of the Rio Grande, located in Quebrada de Humahuaca, a UNESCO World Heritage site. The Aguilar underground mine (Pb–Ag–Zn) is located in the upper reaches of the Yacoraite River drainage basin. The aim of this work is to characterize the presence of heavy metals in water and sediments of the Yacoraite River and to identify their sources. The analysis shows the seasonal variation of heavy metals concentration in water and their relation with the World Health Organization (WHO) limits established for human consumption. The Yacoraite basin is naturally anomalous in some metals and some elements, such as As which is controlled by the chemical composition of regional lithology. During the wet season, Al, Co, Mo and Pb concentrations in water samples are higher than during the dry season; in addition, these metals are also higher than WHO limit values. High enrichment factors for Ba, Mo, Pb, Zn and Cd were found in Casa Grande stream, indicating the direct influence of the mining activities. Cd, Pb and Zn are present in the Aguilar ore minerals, such as sphalerite and galena. Sediments collected during the dry season show a drastic increase in the concentration of As, Pb, Ba, Zn, Cd and Mn. The Müller geo-accumulation index in Casa Grande indicates that it is a highly polluted stream. The concentrations of As, Pb, Ba, Zn, Cd are also high in Yacoraite River: Security Quality Guidelines indicates toxicity. A decrease in enrichment factors and geo-accumulation indices observed in sediments indicates the occurrence of precipitation/adsorption processes in the river to restore the equilibrium composition. Strict environmental controls in Aguilar Mine are necessary to avoid the uncontrolled input of toxic metals in Casa Grande stream and Yacoraite River.  相似文献   

4.
Headwater stream, draining from a rural catchment in NW Spain, was sampled during baseflow and storm-event conditions to investigate the temporal variability in dissolved and particulate Al, Fe, Mn, Cu and Zn concentrations and the role of discharge (Q), pH, dissolved organic carbon (DOC) and suspended sediment (SS) in the transport of dissolved and particulate metals. Under baseflow and storm-event conditions, concentrations of the five metals were highly variable. The results of this study reveal that all metal concentrations are correlated with SS. DOC and SS appeared to influence both the metal concentrations and the partitioning of metals between dissolved and particulate. The SS was a good predictor of particulate metal levels. Distribution coefficients (KD) were similar between metals (4.72–6.55) and did not change significantly as a function of discharge regime. Stepwise multiple linear regression analysis reveals that the most important variable to explain storm-event KD for Al and Fe is DOC. The positive relationships found between metals, in each fraction, indicate that these elements mainly come from the same source. Metal concentrations in the stream were relatively low.  相似文献   

5.
A field study was conducted to determine the effect of landscape spatial pattern and micro-topography on nutrient transfer via runoff from two catchments into Yuqiao Reservoir in north China. The surface runoff discharge was measured during rainfall events and water samples were analyzed in 2004 and 2005. The mean annual total nitrogen (TN) and total phosphorus (TP) exports per unit area from Caogezhuang catchment (C catchment) were 1.048 and 0.561 kg ha−1 year−1, respectively, while the TN and TP exports from Taohuasi catchment (T catchment) were 0.158 and 0.027 kg ha−1 year−1. In both catchments, village and vineyard shared the highest nutrient export ability due to the accumulated animal waste and heavy application of fertilizer and manure. In T catchment, the distance of village and vineyard was about 1,500 m away from the receiving water and in between were woodland and cropland. In the hydrological pathway, there were sink landscape structures of small stone dams, roadside swale, vegetated filter strip and dry ponds, which could detain water and nutrients. In C catchment, the distance between the village and the receiving water was about 200 m, and the hydrological pathway was compacted roads and ditches with no sink structures. It is suggested that the distance between the pollution source area and the receiving water and the micro-topographical features were the main factors to control the great difference in nutrient export rates.  相似文献   

6.
Transport and sediment–water partitioning of trace metals (Cr, Co, Fe, Pb, Cu, Ni, Zn, Cd) in acid mine drainage were studied in two creeks in the Kwangyang Au–Ag mine area, southern part of Korea. Chemical analysis of stream waters and the weak acid (0.1 N HCl) extraction, strong acid (HF–HNO3–HClO4) extraction, and sequential extraction of stream sediments were performed. Heavy metal pollution of sediments was higher in Chonam-ri creek than in Sagok-ri creek, because there is a larger source of base metal sulfides in the ores and waste dump upstream of Chonam-ri creek. The sediment–water distribution coefficients (K d) for metals in both creeks were dependent on the water pH and decreased in the order Pb ≈ Al > Cu > Mn > Zn > Co > Ni ≈ Cd. K d values for Al, Cu and Zn were very sensitive to changes in pH. The results of sequential extraction indicated that among non-residual fractions, Fe–Mn oxides are most important for retaining trace metals in the sediments. Therefore, the precipitation of Fe(–Mn) oxides due to pH increase in downstream sites plays an important role in regulating the concentrations of dissolved trace metals in both creeks. For Al, Co, Cu, Mn, Pb and Zn, the metal concentrations determined by 0.1 N HCl extraction (Korean Standard Method for Soil Pollution) were almost identical to the cumulative concentrations determined for the first three weakly-bound fractions (exchangeable + bound to carbonates + bound to Fe–Mn oxides) in the sequential extraction procedure. This suggests that 0.1 N HCl extraction can be effectively used to assess the environmentally available and/or bioavailable forms of trace metals in natural stream sediments.  相似文献   

7.
In an attempt to delineate heavy metal contamination precincts and to evaluate the extent and degree of toxic levels, besides their possible sources, 38 water samples from Ankaleshwar Industrial Estate, south Gujarat, India were analyzed. By clutching geochemical analyses and GIS-based colour composites areas depicting anomalously high concentration of heavy metals (Mo, Zn, Pb, Ni, Co, Cd, etc.) in the groundwater were revealed. The multicomponent overlays in grey-scale facilitated in identifying situates of heavy metal ‘hot spots’, and lateral protuberances of the contamination plume around defile stretch of the main stream Amla Khadi flowing through the area. The multiple pollution plumes emerging from other parts of the area further coincide with effluent laden streams and small channels indicating industrial establishments as major sources of groundwater contamination. Influent nature of the streams, accelerated infiltration process, high mass influx and shallow groundwater table are the factors conducive for easy access of heavy metals to the phreatic aquifers affecting over 20 km2 area. On the basis of P/U ratios (concentration of metals in polluted water to unpolluted water), geogenic and anthropogenic sources have been identified. Very high levels of technogenic elements present in the ground water raise concerns about possible migration into food crops, as the area is an important horticultural locale and is highly cultivated.  相似文献   

8.
Rivers and their floodplains are dynamic systems, sediments are continually added to floodplain surfaces, while erosion and scour may remove sediments to be added to floodplains further downstream. When mining sediments were introduced into some catchments in Britain as ore deposits were exploited, river channels and floodplains were grossly polluted with metals. The legacy of this uncontrolled release of contaminants is apparent still, and contemporary channel deposits are enriched in metals. While the floodplains acted as a buffer to the dispersal of metals straight through the catchment, metals are still being released hundreds of years later as the floodplains are eroded and this secondary pollution of the river is a long-term problem.By studying a range of mining catchments, the effects of key variables on heavy metal dispersal in the fluvial environment can be assessed. As no single catchment displays the whole array of possible situations, a mosaic of case studies from several areas provides a good representation of potential conditions.  相似文献   

9.
About 6,400 water samples were collected from small catchments in northern Finland and Norway above 66° N latitude as a part of the Nordkalott Project carried out jointly by the Geological Surveys of Finland, Norway, and Sweden. Electrical conductivity (EC) was measured in situ and Ca, Mg, Sr, Ba, Na, K, Si, Fe, Mn, Al, and Zn concentrations were determined from filtered and acidified samples by the ICAP method. The relative abundance of mafic, ultramafic, and carbonate rock components in the catchments is the most influential factor controlling the EC values and the main cation concentrations (Ca, Mg, Sr). These components also determine the HCO3 alkalinity or acid-neutralizing capacity (ANC) of streamwater. In the northern coastal belt, Na is derived largely from airborne sea salts, but in the southwestern corner of the research area it may be derived partly from relict sea salts in sediments. The concentrations of Na, K, and Si do not depend solely on the lithological environment. Fe and, to a lesser extent, Mn and Al occur in the highest abundances in the low-lying, intensely paludified southern part of the area, suggesting that these metals tend to go into solution and are transported in complexed forms with dissolved and colloidic humic matter. The areal distribution patterns of the main cations (Ca, Mg, Sr) and of some heavy metals (Fe, Mn) in streamwater are fairly consistent with those of till and minerogenic stream sediments, although, in a statistical approach, only a few significant correlation coefficients were established.  相似文献   

10.
Atmospheric deposition of S in Sweden has decreased by some 80% over the last 15 a, resulting in a general reduction of SO4 concentrations in ground and surface water. This project, however, shows that artificial hydrological alteration in an acid wetland can reverse this trend and increase acidity and SO4 concentrations. The experiment involved the monitoring of two catchments in relatively virgin conditions. In one of the catchments, an experiment with intensive groundwater extraction from the bedrock was carried out. During the experiment, the runoff from the catchment decreased by 50%. Furthermore, the extraction of groundwater resulted in increased seasonal aeration of the centrally located wetland, leading to oxidation of reduced S bound to the soil layers of the wetland. The S changed to solute SO4, with a subsequent SO4 surge. Thus, the experiment resulted in an induced acidification of the wetland and runoff waters. The extraction of groundwater significantly increased the recharge of water from the overburden, glacial till and organic soils to groundwater in the bedrock, which in turn reduced the retention time in the bedrock aquifer. These changes resulted in the chemical signature of the groundwater in the bedrock becoming similar to those of the wetland. The findings revealed deterioration in the water quality in the bedrock due to increased concentrations of dissolved organic C and SO4, as well as a decrease in pH.  相似文献   

11.
The purpose of this study was to determine the levels of heavy metals namely cadmium (Cd), copper (Cu) and lead (Pb) in the five aquatic plants. For this purpose, the concentration of heavy metals were measured in water and in the five aquatic plant species, Lepironia articulata, Pandanus helicopus, Scirpus grossus, Cabomba furcata and Nelumbo nucifera, in 15 sites from Tasik Chini. The concentrations were different among the plant species as well as among the parts of plants. The highest concentration of heavy metals among the aquatic plants and plant parts was found in the roots of S. grossus. The concentrations of Cd in the leaves and stems of submerged aquatic plant, C. furcata, were higher than concentration of Cd in the leaves and stems of emergent aquatic plant and floating leaf plant. The concentration of Cu in the stem of C. furcata was greater than that in the leaf, while the concentration of Cd was more in the leaf than in the stem. The heavy metal contents of the aquatic plants were in descending order of Pb > Cu > Cd. The metal concentration quotient of leaves/roots and stems/roots (ML/MR and MS/MR) were calculated. The highest internal translocation was found in P. helicopus, while the lowest internal translocation was found in S. grossus.  相似文献   

12.
Steelmaking-coal waste rock placed in mountain catchments in the Elk Valley, British Columbia, Canada, drain constituents of interest (CIs) to surface water downgradient of the waste rock dumps. The role of groundwater in transporting CIs in the headwaters of mountain catchments is not well understood. This study characterizes the physical hydrogeology of a portion of a 10-km2 headwater catchment (West Line Creek) downgradient of a 2.7-km2 waste rock dump placed over a natural headwater valley-bottom groundwater system. The study site was instrumented with 13 monitoring wells. Drill core samples were collected to determine subsurface lithology and geotechnical properties. The groundwater system was characterized using field testing and water-level monitoring. The valley-bottom sediments were composed of unconsolidated glacial and meltwater successions (<64 m thick) deposited as a series of cut and fill structures overlying shale bedrock. An unconfined basal alluvial aquifer located above fractured bedrock was identified as the primary conduit for groundwater flow toward Line Creek (650 m from the toe of the dump). Discharge through the basal alluvial aquifer was estimated using the geometric mean hydraulic conductivity (±1 standard deviation). These calculations suggest groundwater discharge could account for approximately 15% (ranging from 2 to 60%) of the total water discharged from the watershed. The residence time from the base of the waste rock dump to Line Creek was estimated at <3 years. The groundwater system was defined as a snowmelt (i.e., nival) regime dominated by direct recharge (percolation of precipitation) across the catchment.  相似文献   

13.
金矿区河水和底泥中重金属含量分布与耦合关系   总被引：3，自引：1，他引：2  
河流中河水与底泥中重金属含量之间的关系对于河流污染防治意义重大。对某金矿区3种典型河流的河水与底泥中的重金属含量进行分析,发现4条河流均有超过国家标准限值的情况,河水中7种重金属元素均出现超标,Cr、As元素超标不严重;底泥中Hg、Pb、Cr、Cu、Zn超标,其中Hg超标最严重,河水和底泥中Hg最大超标倍数分别达到3099倍和244倍。河流中重金属主要赋存形态为沉积态,底泥的吸附解吸作用是河流底泥和河水中重金属沿程变化的主控因素;金矿区区域上河水和底泥中重金属很好地服从Langmuir等温吸附模式。矿业活动、地层岩性均会影响底泥对重金属的平均最大吸附容量,流径黄土区的双桥河平均最大吸附容量最大。研究结果为矿山河流污染防治与预警提供了参考依据。  相似文献   

14.
Metal concentrations from stream waters in two geological blocks in Northern Ireland were compared to determine the contributions of catchment characteristics and in-stream conditions. One block is composed of metamorphosed schist and unconsolidated glacial drift with peat or peaty podzol (mainly humic) soils, while the other block consists of tertiary basalt with brown earth and gley soils. Water samples were collected from 52 stream sites and analysed for iron (Fe), manganese (Mn) and aluminium (Al) as well as a range of other chemical determinands known to affect metal solubility. Densities of metal-rich ochre deposit were determined for stream bed stone samples. Higher conductivities and concentrations of bicarbonate, alkalinity, calcium and magnesium occurred on basalt than on schist. Despite higher Fe and Mn oxide concentrations in basalt-derived non-humic soils, stream water concentrations were much lower and ochre deposit densities only one-third of those on schist overlain by humic soils. Neither rock nor soil type predicted Al concentrations, but pH and dissolved oxygen did. Peat-generated acidity and the limited acid neutralising capacity of base-poor metamorphosed schist have resulted in elevated concentrations of metals and ochre deposit in surface waters.  相似文献   

15.
In this study the effect of anthropogenic discharges on the heavy metal content in the Potengi–Jundiai river system near the fast growing city of Natal, NE-Brazil, is investigated. Due to the multiple anthropogenic source character without any predominating anthropogenic heavy metal discharge the area of Natal may serve as a characteristic place for the study of the impact of the fast growing Brazilian cities on the environment. In general the sediments of the Rio Potengi–Jundiai river system in the studied area are not severely polluted. However, close to waste water drain pipes a characteristic anthropogenic heavy metal signature is visible in enhanced Zn, Pb, Cu and Cd values relative to reference elements such as Al and Fe. Sources are domestic and animal waste, combustion products and hydrocarbons. These heavy metals are probably mainly bound to organic matter. The elements Sn, Hg and Ag in part also belong to the anthropogenic heavy metal signature. The elements Cr, Ni and V are characteristic of weathering heavy minerals in crystalline rocks exposed in the catchment area of the river system and are not significantly added from anthropogenic sources. These heavy metals are most likely predominantly bound to oxides and represent the pristine geogenic background of the system. They can thus be used as reference elements to monitor incipient accumulation of Zn, Pb, Cu and Cd due to anthropogenic input. The element characteristics found here match with those found in other fast growing urban areas such as the Sao Paulo metropolitan area.  相似文献   

16.
《Applied Geochemistry》1997,12(2):203-211
The metal attenuation capacities of secondary acid mine water precipitates is dependent upon such factors as pH, ionic strength, the presence of competing ions, and tailings mineralogy. At the abandoned Spenceville Cu mine in Nevada County, California, approximately 6800 m3 of jarosite overburden and 28,000 m3 of hematite residue are potential sources of heavy metals loading to infiltrating surface waters. A column study was performed to assess the ability of the overburden and the residue to attenuate heavy metals from acidic mine drainage. The study information was needed as part of a remedial design for the abandoned mine, and was designed to simulate a worst-case scenario to examine the plausibility of backfilling a large open pit with the waste materials. Ten pore volumes of acidic mine drainage were allowed to pass through the materials, and the column effluents were analyzed for dissolved Fe, Al, Ca, Mg, Na, K, Mn, Cu, Zn, Pb and Ni using ICP-AES. The oxidation-reduction potential (Eh) was measured with a combination PtAg/AgCl electrode and also calculated from Fe(II) and Fe(III) measurements using the Nernst equation. Ion activities in solution and saturation index (SI) values for various solid phases were calculated using the geochemical speciation model MINTEQA2, and mineralogical compositions of fine (< 2 mm) and coarse ( > 2 mm) fractions were determined by XRD. Geochemical modeling of the column effluent compositions indicate that goethite, jarosite, jurbanite and gypsum are potential solid phases that may control metal solubilities in the column effluents. Excellent agreement was observed between the measured Eh values and those calculated from the activity ratio of Fe2+(aq) to Fe3+(aq). The large attenuation capacities for Cu and Zn exhibited by the jarosite overburden also suggest that solid solution substitution plays a large role in controlling metal concentrations in the pore waters. Relatively little metal attenuation, however, was provided by the hematite residue.  相似文献   

17.
Morén  Ida  Mojarrad  Brian  Riml  Joakim  Wörman  Anders 《Hydrogeology Journal》2023,31(3):537-555

Hyporheic exchange flow (HEF) at the streambed–water interface (SWI) has been shown to impact the pattern and rate of discharging groundwater flow (GWF) and the consequential transport of heat, solutes and contaminants from the subsurface into streams. However, the control of geographic and hydromorphological catchment characteristics on GWF–HEF interactions is still not fully understood. Here, the spatial variability in flow characteristics in discharge zones was investigated and averaged over three spatial scales in five geographically different catchments in Sweden. Specifically, the deep GWF discharge velocity at the SWI was estimated using steady-state numerical models, accounting for the real multiscale topography and heterogeneous geology, while an analytical model, based on power spectral analysis of the streambed topography and statistical assessments of the stream hydraulics, was used to estimate the HEF. The modeling resulted in large variability in deep GWF and HEF velocities, both within and between catchments, and a regression analysis was performed to explain this observed variability by using a set of independent variables representing catchment topography and geology as well as local stream hydromorphology. Moreover, the HEF velocity was approximately two orders of magnitude larger than the deep GWF velocity in most of the investigated stream reaches, indicating significant potential to accelerate the deep GWF velocity and reduce the discharge areas. The greatest impact occurred in catchments with low average slope and in reaches close to the catchment outlet, where the deep GWF discharge velocity was generally low.

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18.
Globally, aquatic ecosystems are highly polluted with heavy metals arising from anthropogenic and terrigenous sources. The objective of this study was to investigate the pollution of stream sediments and possible sources of pollutants in Nakivubo Channel Kampala, Uganda. Stream sediments were collected and analysed for heavy metal concentration using flame atomic absorption spectrophotometer. The degree of pollution in Nakivubo channelized stream sediments for lead, cadmium, copper, zinc, manganese and iron was assessed using enrichment factor, geo-accumulation index and pollution load index. The results indicated that (1) the sediments have been polluted with lead, cadmium and zinc and have high anthropogenic influences; (2) the calculation of geo-accumulation index suggest that Nakivubo stream sediments have background concentration for copper, manganese and Fe (I geo ≤ 0); (3) factor analysis results reveal three sources of pollutants as explained by three factors (75.0 %); (i) mixed origin or retention phenomena of industrial and vehicular emissions; (ii) terrigenous and (iii) dual origin of zinc (vehicular and industrial). In conclusion, the co-precipitation (inclusion, occlusion and adsorption) of lead, cadmium and zinc with manganese and iron hydroxides, scavenging ability of other metals, very low dissolved oxygen and slightly acidic to slightly alkaline pH in stream water could account for the active accumulation of heavy metals in Nakivubo stream sediments. These phenomena may pose a risk of secondary water pollution under sediment disturbance and/or changes in the geo-chemistry of sediments.  相似文献   

19.
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20.
Environmental isotopes including \({\updelta }^{18}\)O, \({\updelta }^{2}\)H and \(^{3}\)H of precipitation, streams and springs were determined in the mountainous Bringi catchment of Kashmir Himalaya, dominated by carbonate lithology. The isotopic signature of winter precipitation is reflected in stream and spring water in late spring and is, therefore, representative of snow melting. The spring waters in September bear the enriched isotopic signatures of summer rainfall. The strong correlation (\(r^{2} = 0.97\)) between the isotopic composition of streams and springs indicates the streams and springs either share similar catchments or the springs are recharged by the streams. Chloride mass balance and isotopic mass balance studies suggest that the surface recharge component averages 337.35 m\(^{3}\)/s, which is about 75% of total stream discharge during the high flow period. Similarly, the contribution of surface water to groundwater recharge during the low flow period averages 7.5 m\(^{3}\)/s, which is about 18.6% of total stream flow. Furthermore, the mean residence time of the springs calculated from the tritium decay equation is very short (<1 year). The residence time is longer for Kongamnag and short for Achabalnag, which is further supported by dye testing.  相似文献   

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