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1.
Methyl halides such as methyl chloride (CH3Cl) are known to be important carriers of halogen from the ocean to the atmosphere, and the halogens they release into the stratosphere by photolysis catalyze ozone depletion. Marine phytoplankton have been reported as a source of CH3Cl, but the effects of environmental temperature on the CH3Cl production by phytoplankton have not been investigated. In this study, we investigated the effects of temperature on the production of CH3Cl in the culture of a marine diatom, Phaeodactylum tricornutum CCMP 630, incubated at 10, 15, 20, 25, and 30 °C. CH3Cl concentrations in cultured samples were determined using purge and trap gas chromatograph–mass spectrometry. Phytoplankton growth was monitored by measuring the chlorophyll a concentrations. CH3Cl production was observed for several weeks at four different temperatures ranging from 10 to 25 °C. The CH3Cl production from P. tricornutum was increased with increasing temperature from 10 to 25 °C, and the maximum production rate for CH3Cl was 0.21~0.26 μmol (g chlorophyll a)?1 d?1 at 25 °C, which was several times higher than that at 10 °C (~0.03 μmol (g chlorophyll a)?1 d?1). The Arrhenius equation was successfully used to characterize the effects of temperature on the production rates of CH3Cl in the culture of P. tricornutum. Our results suggest that water temperature directly affects CH3Cl production derived from P. tricornutum and that water temperature would be a significant factor for estimating the emissions of CH3Cl from marine environments.  相似文献   

2.
The relationship between the radar reflectivity factor (Z) and the rainfall rate (R) is recalculated based on radar observations from 10 Doppler radars and hourly rainfall measurements at 6529 automatic weather stations over the Yangtze–Huaihe River basin. The data were collected by the National 973 Project from June to July 2013 for severe convective weather events. The Z–R relationship is combined with an empirical qr–R relationship to obtain a new Z–qr relationship, which is then used to correct the observational operator for radar reflectivity in the three-dimensional variational (3DVar) data assimilation system of the Weather Research and Forecasting (WRF) model to improve the analysis and prediction of severe convective weather over the Yangtze–Huaihe River basin. The performance of the corrected reflectivity operator used in the WRF 3DVar data assimilation system is tested with a heavy rain event that occurred over Jiangsu and Anhui provinces and the surrounding regions on 23 June 2013. It is noted that the observations for this event are not included in the calculation of the Z–R relationship. Three experiments are conducted with the WRF model and its 3DVar system, including a control run without the assimilation of reflectivity data and two assimilation experiments with the original and corrected reflectivity operators. The experimental results show that the assimilation of radar reflectivity data has a positive impact on the rainfall forecast within a few hours with either the original or corrected reflectivity operators, but the corrected reflectivity operator achieves a better performance on the rainfall forecast than the original operator. The corrected reflectivity operator extends the effective time of radar data assimilation for the prediction of strong reflectivity. The physical variables analyzed with the corrected reflectivity operator present more reasonable mesoscale structures than those obtained with the original reflectivity operator. This suggests that the new statistical Z–R relationship is more suitable for predicting severe convective weather over the Yangtze–Huaihe River basin than the Z–R relationships currently in use.  相似文献   

3.
The phenology of many ecological processes including pollination service is modulated by surface air temperature, making them potentially sensitive to climatic change. The Japanese hornfaced bee, Osmia cornifrons (Hymenoptera: Megachilidae), was introduced into the USA in the 1970s and has been used as a key pollinator of spring blooming fruit crops such as apple and blueberry. This study examined the effects of future climate change on three key phenological events of O. cornifrons: date for adult emergence (female and male) in spring, date for completion of egg and larval development, and duration for the development in the Eastern USA. We used daily temperature data obtained from 21 models in Coupled Model Intercomparison Project Phase 5 for 2006–2100 under the two future climate scenarios of Representative Concentration Pathways (RCPs 4.5 and 8.5). We estimated the Julian dates (JDs) of spring emergence and development of O. cornifrons using the phenological parameters derived from temperature-dependent biophysical models. The JDs for the bee emergence and development are projected to be significantly advanced in the Eastern USA under the RCP 4.5 and 8.5 scenarios. The number of days for bee development is projected to be longer in the southern region (+?0.57 days/decade) and shorter in the central (??0.27 days/decade) and northern (??0.65 days/decade) regions of the Eastern USA (all the p values <?0.01). The significantly longer duration of bee development under future climate change could pose a risk to the bee due to the longer period of being exposed to its pests. Implications for management of O. cornifrons population were discussed in this article.  相似文献   

4.
According to the statistical shape–slope (μ–Λ) relationship observed for the first time by several 2D-Video-Distrometers (2DVD) in southern China, a constrained gamma (C-G) model was proposed for the retrieval of rain drop size distributions (DSDs) from Guangzhou S-band polarimetric radar observations. Two typical precipitation processes were selected to verify the accuracy of the retrieval scheme. The μ–Λ relationship: Λ = 0.0241μ2 + 0.867μ + 2.453 was obtained based on the 2DVD observation results from at Huizhou Longmen station, which is a very representative location in the area. Relying on the Guangzhou polarimetric radar measurements of radar reflectivity (ZHH) and differential reflectivity (ZDR), the gamma (Γ) size distribution parameters (N0, μ, and Λ) can be retrieved by the C-G model retrieval scheme. The results show that the Guangzhou polarimetric radar retrievals of DSDs were close to the 2DVD observations at Guangzhou Maofengshan station. The rain rate, mass mean diameter, and normalized intercept parameter of radar retrievals were in good agreement with the 2DVD observations, and the relative errors were less than 10%. The overall accuracy of the retrieval scheme was high. The retrieval scheme has established the relationship between the polarimetric radar measurements and gamma size distribution parameters. It will be helpful to in-depth research and application of the dual-polarization radar data in microphysical precipitation processes analysis, as well as convection-resolved numerical model data assimilation and prediction effect evaluation.  相似文献   

5.
The mechanisms driving changes in dominant plant species are the key for understanding how grassland ecosystems respond to climate change. In this study, we examined plant functional traits (morphological characteristics: plant height, leaf area, and leaf number; biomasses: aboveground, belowground, and total; and growth indices: root-to-shoot ratio, specific leaf area, and leaf mass ratio) of four zonal Stipa species (S. baicalensis, S. bungeana, S. grandis, and S. breviflora) from Inner Mongolian grassland in response to warming (control, +1.5, +2.0, +4.0, and +6.0?), changing precipitation (-30%, -15%, control, +15%, and +30%), and their combined effects via climate control chambers. The results showed that warming and changing precipitation had significant interactive effects, different from the accumulation of single-factor effects, on functional traits of Stipa species. The correlation and sensitivity of different plant functional traits to temperature and precipitation differed. Among the four species, the accumulation and variability of functional traits had greater partial correlation with precipitation than temperature, except for leaf number, leaf area, and specific leaf area, in S. breviflora, S. bungeana, and S. grandis. For S. baicalensis, the accumulation and variability of plant height, aboveground biomass, and root-to-shoot ratio only had significant partial correlation with precipitation. However, the variability of morphological characteristics, biomasses, and some growth indices, was more sensitive to temperature than precipitation in S. bungeana, S. grandis, and S. breviflora—except for aboveground biomass and plant height. These results reveal that precipitation is the key factor determining the growth and changes in plant functional traits in Stipa species, and that temperature mainly influences the quantitative fluctuations of the changes in functional traits.  相似文献   

6.
PM10 samples were collected to characterize the seasonal and annual trends of carbonaceous content in PM10 at an urban site of megacity Delhi, India from January 2010 to December 2017. Organic carbon (OC) and elemental carbon (EC) concentrations were quantified by thermal-optical transmission (TOT) method of PM10 samples collected at Delhi. The average concentrations of PM10, OC, EC and TCA (total carbonaceous aerosol) were 222?±?87 (range: 48.2–583.8 μg m?3), 25.6?±?14.0 (range: 4.2–82.5 μg m?3), 8.7?±?5.8 (range: 0.8–35.6 μg m?3) and 54.7?±?30.6 μg m?3 (range: 8.4–175.2 μg m?3), respectively during entire sampling period. The average secondary organic carbon (SOC) concentration ranged from 2.5–9.1 μg m?3 in PM10, accounting from 14 to 28% of total OC mass concentration of PM10. Significant seasonal variations were recorded in concentrations of PM10, OC, EC and TCA with maxima during winter and minima during monsoon seasons. In the present study, the positive linear trend between OC and EC were recorded during winter (R2?=?0.53), summer (R2?=?0.59) and monsoon (R2?=?0.78) seasons. This behaviour suggests the contribution of similar sources and common atmospheric processes in both the fractions. OC/EC weight ratio suggested that vehicular emissions, fossil fuel combustion and biomass burning could be the major sources of carbonaceous aerosols of PM10 at the megacity Delhi, India. Trajectory analysis indicates that the air mass approches to the sampling site is mainly from Indo Gangetic plain (IGP) region (Uttar Pradesh, Haryana and Punjab etc.), Thar desert, Afghanistan, Pakistan and surrounding areas.  相似文献   

7.
Ocean acidification increases the amount of dissolved inorganic carbon (DIC) available in seawater which can benefit photosynthesis in those algae that are currently carbon limited, leading to shifts in the structure and function of seaweed communities. Recent studies have shown that ocean acidification-driven shifts in seaweed community dominance will depend on interactions with other factors such as light and nutrients. The study of interactive effects of ocean acidification and warming can help elucidate the likely effects of climate change on marine primary producers. In this study, we investigated the ecophysiological responses of Cystoseira tamariscifolia (Hudson) Papenfuss. This large brown macroalga plays an important structural role in coastal Mediterranean communities. Algae were collected from both oligotrophic and ultraoligotrophic waters in southern Spain. They were then incubated in tanks at ambient (ca. 400–500 ppm) and high CO2 (ca. 1200–1300 ppm), and at 20 °C (ambient temperature) and 24 °C (ambient temperature +4 °C). Increased CO2 levels benefited the algae from both origins. Biomass increased in elevated CO2 treatments and was similar in algae from both origins. The maximal electron transport rate (ETRmax), used to estimate photosynthetic capacity, increased in ambient temperature/high CO2 treatments. The highest polyphenol content and antioxidant activity were observed in ambient temperature/high CO2 conditions in algae from both origins; phenol content was higher in algae from ultraoligotrophic waters (1.5–3.0%) than that from oligotrophic waters (1.0–2.2%). Our study shows that ongoing ocean acidification can be expected to increase algal productivity (ETRmax), boost antioxidant activity (EC 50 ), and increase production of photoprotective phenols. Cystoseira tamariscifolia collected from oligotrophic and ultraoligotrophic waters were able to benefit from increases in DIC at ambient temperatures. Warming, not acidification, may be the key stressor for this habitat as CO2 levels continue to rise.  相似文献   

8.
We evaluated the potential of polarimetric rainfall retrieval methods for the Tagaytay C-Band weather radar in the Philippines. For this purpose, we combined a method for fuzzy echo classification, an approach to extract and reconstruct the differential propagation phase, Φ DP , and a polarimetric self-consistency approach to calibrate horizontal and differential reflectivity. The reconstructed Φ DP was used to estimate path-integrated attenuation and to retrieve the specific differential phase, K DP . All related algorithms were transparently implemented in the Open Source radar processing software wradlib. Rainfall was then estimated from different variables: from re-calibrated reflectivity, from re-calibrated reflectivity that has been corrected for path-integrated attenuation, from the specific differential phase, and from a combination of reflectivity and specific differential phase. As an additional benchmark, rainfall was estimated by interpolating the rainfall observed by rain gauges. We evaluated the rainfall products for daily and hourly accumulations. For this purpose, we used observations of 16 rain gauges from a five-month period in the 2012 wet season. It turned out that the retrieval of rainfall from K DP substantially improved the rainfall estimation at both daily and hourly time scales. The measurement of reflectivity apparently was impaired by severe miscalibration while K DP was immune to such effects. Daily accumulations of rainfall retrieved from K DP showed a very low estimation bias and small random errors. Random scatter was, though, strongly present in hourly accumulations.  相似文献   

9.
Atmospheric circulation epochs and climate changes   总被引：5，自引：0，他引：5  
The atmospheric circulation studies allow climate changes to be diagnosed and forecasted. Variations in occurrence frequencies of the atmospheric circulation forms W, E, and C (by the Vangengeim classification) and Z, M 1, and M 2 (by the Girs classification), which characterize climatic conditions in most of the Northern Hemisphere, are analyzed over a period of more than 100 years. It is shown that the occurrence frequency of the forms W, C, and M 1 continually decreased, while that of the forms E and Z increased, which indicates a significant change in atmospheric circulation in the Northern Hemisphere during the last century. The occurrence frequency of the forms C and Z demonstrates specific features at inter-decade time scales. Correlations are found between accumulated sums of anomalies of occurrence frequencies of the atmospheric circulation forms C, (W + E), Z, and (M 1 + M 2) and inter-decade variations of the Earth’s rotation. The causes of these relationships are discussed along with possibilities of their use for diagnosis of climatic variations in the Northern Hemisphere.  相似文献   

10.
The aim of this work is to obtain an index for predicting the probability of occurrence of zonda event at surface level from sounding data at Mendoza city, Argentine. To accomplish this goal, surface zonda wind events were previously found with an objective classification method (OCM) only considering the surface station values. Once obtained the dates and the onset time of each event, the prior closest sounding for each event was taken to realize a principal component analysis (PCA) that is used to identify the leading patterns of the vertical structure of the atmosphere previously to a zonda wind event. These components were used to construct the index model. For the PCA an entry matrix of temperature (T) and dew point temperature (Td) anomalies for the standard levels between 850 and 300 hPa was build. The analysis yielded six significant components with a 94 % of the variance explained and the leading patterns of favorable weather conditions for the development of the phenomenon were obtained. A zonda/non-zonda indicator c can be estimated by a logistic multiple regressions depending on the PCA component loadings, determining a zonda probability index \( \widehat{c} \) calculable from T and Td profiles and it depends on the climatological features of the region. The index showed 74.7 % efficiency. The same analysis was performed by adding surface values of T and Td from Mendoza Aero station increasing the index efficiency to 87.8 %. The results revealed four significantly correlated PCs with a major improvement in differentiating zonda cases and a reducing of the uncertainty interval.  相似文献   

11.
We investigated and evaluated the occurrence of fault zone tracer gases (CO2, He, Rn), volatile organohalogens (CH3Cl, CHCl3, CHBr3), alkanes and limonene in soil and nest gases of red wood ants (RWA) in comparison to ambient air, in a seismically active area. In this new approach, we compared RWA-free areas to RWA-areas by combining different investigation and analytical methods. In soil gas, the fault zone tracer gas Rn was surprisingly highly correlated to limonene, suggesting a combination of biotic production of limonene and abiotic degassing of Rn in a seismically active area; moderate correlations were found with trihalomethanes and other halocarbons. In RWA nests a variety of elevated concentrations of haloforms were found, while remaining below the atmospheric background values in RWA-free areas. The evidence of CHCl3 in RWA nests is the first record. Its average concentrations in nests of F. rufa and F. polyctena were up to 3 fold higher than atmospheric background and up to 28–70 fold higher compared to e.g. volcanic emissions being considered as one of its main geogenic sources. Thus, RWA nests could possibly be an additional source for CHCl3 liberation. Consequently, apart from RWA being bioindicators for seismically active degassing faults, they might also be used as bioindicators for CHCl3 formation in forest soils. Although we cannot yet differentiate between a geogenic/abiotic and a biotic formation. RWA nests will have to be reconsidered for halocarbon formation in future quantifications of geochemical cycles at global scale, since they impact organic soil chemistry through biotic and/or abiotic pathways. Therefore, further larger-scale research in different tectonic settings but also in well-known CHCl3 “hot spot” study areas such as the Klosterhede area (Denmark) should focus directly on gas sampling from confirmed active fault systems. Nests of other ant species should be addressed to compare seasonal, diurnal and nocturnal variations of degassing procedures in relation to earth tides, different geologic settings, and tectonic events such as earthquakes and on quantifying the fluxes to the atmosphere.  相似文献   

12.
As photosynthetically active radiation (PAR) variability and PAR estimating methods play an important role in climate change and ecological process research, PAR variation trends and broadband global solar radiation (R s ) ratios (PAR/R s ) in the North China Plain (NCP) are examined using in situ PAR and R s observed data for 2005 to 2011. The annual average PAR value found in the NCP is 22.9 mol m?2 d?1. The highest and lowest values were recorded at Changwu and Luancheng sites, respectively. The highest PAR/R s value was found in Jiaozhouwan due to large water vapor volumes present in this area. PAR/R s levels have increased in the NCP due to a decrease in fine aerosols and increase in water vapor concentration. From these analysis results, a parameterization model that can be applied to all sky conditions was checked. Empirical estimation model comparisons for obtaining PAR values indicate that model was least accurate when R s was used independently. When the model included R s, the clearness index (K s) and the solar zenith angle, the model estimated PAR values with acceptable accuracy. A parameterization model was constructed by considering K s and attenuation factors of PAR under clear weather conditions (ρ clear). The improved parameterization model more accurately predicts values for local sites and for various observation sites.  相似文献   

13.
Soil temperature (T s) and its thermal regime are the most important factors in plant growth, biological activities, and water movement in soil. Due to scarcity of the T s data, estimation of soil temperature is an important issue in different fields of sciences. The main objective of the present study is to investigate the accuracy of multivariate adaptive regression splines (MARS) and support vector machine (SVM) methods for estimating the T s. For this aim, the monthly mean data of the T s (at depths of 5, 10, 50, and 100 cm) and meteorological parameters of 30 synoptic stations in Iran were utilized. To develop the MARS and SVM models, various combinations of minimum, maximum, and mean air temperatures (T min, T max, T); actual and maximum possible sunshine duration; sunshine duration ratio (n, N, n/N); actual, net, and extraterrestrial solar radiation data (R s, R n, R a); precipitation (P); relative humidity (RH); wind speed at 2 m height (u 2); and water vapor pressure (Vp) were used as input variables. Three error statistics including root-mean-square-error (RMSE), mean absolute error (MAE), and determination coefficient (R 2) were used to check the performance of MARS and SVM models. The results indicated that the MARS was superior to the SVM at different depths. In the test and validation phases, the most accurate estimations for the MARS were obtained at the depth of 10 cm for T max, T min, T inputs (RMSE = 0.71 °C, MAE = 0.54 °C, and R 2 = 0.995) and for RH, V p, P, and u 2 inputs (RMSE = 0.80 °C, MAE = 0.61 °C, and R 2 = 0.996), respectively.  相似文献   

14.
A three-dimensional charge–discharge numerical model is used, in a semi-idealized mode, to simulate a thunder-storm cell. Characteristics of the graupel microphysics and vertical air motion associated with the lightning initiation are revealed, which could be useful in retrieving charge strength during lightning when no charge–discharge model is available. The results show that the vertical air motion at the lightning initiation sites (Wini) has a cubic polynomial correlation with the maximum updraft of the storm cell (Wcell-max), with the adjusted regression coefficient R2 of approximately 0.97. Meanwhile, the graupel mixing ratio at the lightning initiation sites (qg-ini) has a linear correlation with the maximum graupel mixing ratio of the storm cell (qg-cell-max) and the initiation height (zini), with the coefficients being 0.86 and 0.85, respectively. These linear correlations are more significant during the middle and late stages of lightning activity. A zero-charge zone, namely, the area with very low net charge density between the main positive and negative charge layers, appears above the area of qg-cell-max and below the upper edge of the graupel region, and is found to be an important area for lightning initiation. Inside the zero-charge zone, large electric intensity forms, and the ratio of qice (ice crystal mixing ratio) to qg (graupel mixing ratio) illustrates an exponential relationship to qg-ini. These relationships provide valuable clues to more accurately locating the high-risk area of lightning initiation in thunderstorms when only dual-polarization radar data or outputs from numerical models without charging/discharging schemes are available. The results can also help understand the environmental conditions at lightning initiation sites.  相似文献   

15.
Long-term variation of rainfall erosivity in Calabria (Southern Italy)   总被引：1，自引：0，他引：1  
The changes in rainfall erosivity have been investigated using the rainfall erosivity factor (R) proposed for USLE by Wischmeier and Smith (R W-S ) and some simplified indexes (the Fournier index modified by Arnoldus, F, a regional index spatial independent, R Fr , and a regional index spatial dependent, R Fs ) estimated by indirect approaches. The analysis has been carried out over 48 rainfall stations located in Calabria (Southern Italy) using data collected in the period 1936–2012 and divided in three sub-periods. The series of the erosivity indexes and of some precipitation variables have been analyzed for evidence of trends using standard methods. The simplified indexes suggested a general underestimation of the rainfall erosivity with respect to R W-S . The mean underestimation ranged between 23 and 54 % for R Fr and from 10 to 15 % for R Fs . Both the sign and the magnitude of the trends were different for the different stations depending on the variable and sub-period considered. In general, the erosivity increased during the period 1936–1955 (1st sub-period) and during the more recent sub-period (1992–2012, 3rd sub-period), whereas it decreased during 1958–1977 (2nd sub-period). The evidence of trends was generally higher for R W-S than for R Fr and R Fs . Focusing on the most recent sub-period (3rd sub-period), all the variables analyzed showed mainly increasing trends but with different magnitude. More particularly, R W-S showed a mean increment of 29 %; F, R Fr and R Fs increased by 11, 15 and 18 %, respectively; the maximum intensity of 0.5-h precipitation increased by 5 %; and the annual precipitation increased by 22 %. Consequently, it remains difficult to define which precipitation variable plays the dominant role in the temporal variation of rainfall erosivity in the region. However, the overall results suggest that the indexes estimated by indirect procedures (F, R Fr , and R Fs ) should be used with caution for climate change analysis, despite they are used for practical purposes considering they are based on easily available information.  相似文献   

16.
Although Brazil is predominantly a tropical country, frosts are observed with relative high frequency in the Center-Southern states of the country, affecting mainly agriculture, forestry, and human activities. Therefore, information about the frost climatology is of high importance for planning of these activities. Based on that, the aims of the present study were to develop monthly meteorological (F MET) and agronomic (F AGR) frost day models, based on minimum shelter air temperature (T MN), in order to characterize the temporal and spatial frost days variability in Center-Southern Brazil. Daily minimum air temperature data from 244 weather stations distributed across the study area were used, being 195 for developing the models and 49 for validating them. Multivariate regression models were obtained to estimate the monthly T MN, once the frost day models were based on this variable. All T MN regression models were statistically significant (p < 0.001), presenting adjusted R 2 between 0.69 and 0.90. Center-Southern Brazil is mainly hit by frosts from mid-fall (April) to mid-spring (October). The period from November to March is considered as frost-free, being very rare a frost day within that period. Monthly F MET and F AGR presented significant sigmoidal relationships with T MN (p < 0.0001), with adjusted R 2 above of 0.82. The residuals of the frost day models were random, which means that the sigmoidal models performed quite well for interpreting the frost day variability throughout the study area. The highlands of Santa Catarina, Rio Grande do Sul, São Paulo, and Minas Gerais had in average more than 25 and 13 frosts per year, respectively, for F MET and F AGR. The F MET and F AGR maps developed in this study for Center-Southern Brazil is a useful tool for farmers, foresters, and researchers, since they contribute to reduce frost spatial and temporal uncertainty, helping in planning project for strategic purposes. Furthermore, the monthly F MET and F AGR maps for this Brazilian region are the first zoning of these variables for the country.  相似文献   

17.
Estimation of ground heat flux from soil temperature over a bare soil   总被引：1，自引：0，他引：1  
Ground soil heat flux, G 0, is a difficult-to-measure but important component of the surface energy budget. Over the past years, many methods were proposed to estimate G 0; however, the application of these methods was seldom validated and assessed under different weather conditions. In this study, three popular models (force-restore, conduction-convection, and harmonic) and one widely used method (plate calorimetric), which had well performance in publications, were investigated using field data to estimate daily G 0 on clear, cloudy, and rainy days, while the gradient calorimetric method was regarded as the reference for assessing the accuracy. The results showed that harmonic model was well reproducing the G 0 curve for clear days, but it yielded large errors on cloudy and rainy days. The force-restore model worked well only under rainfall condition, but it was poor to estimate G 0 under rain-free conditions. On the contrary, the conduction-convection model was acceptable to determine G 0 under rain-free conditions, but it generated large errors on rainfall days. More importantly, the plate calorimetric method was the best to estimate G 0 under different weather conditions compared with the three models, but the performance of this method is affected by the placement depth of the heat flux plate. As a result, the heat flux plate was recommended to be buried as close as possible to the surface under clear condition. But under cloudy and rainy conditions, the plate placed at depth of around 0.075 m yielded G 0 well. Overall, the findings of this paper provide guidelines to acquire more accurate estimation of G 0 under different weather conditions, which could improve the surface energy balance in field.  相似文献   

18.
Urbanization has a substantial effect on urban meteorology. It can alter the atmospheric diffusion capability in urban areas and therefore affect pollutant concentrations. To study the effects of Hangzhou’s urban development in most recent decade on its urban meteorological characteristics and pollutant diffusion, 90 weather cases were simulated, covering 9 weather types, with the Nanjing University City Air Quality Prediction System and high-resolution surface-type data and urban construction data for 2000 and 2010. The results show that the most recent decade of urban development in Hangzhou substantially affected its urban meteorology. Specifically, the average urban wind speed decreased by 1.1 m s ?1; the average intensity of the heat island increased by 0.5°C; and the average urban relative humidity decreased by 9.7%. Based on one case for each of the nine weather types, the impact of urbanization on air pollution diffusion was investigated, revealing that the changes in the meteorological environment decreased the urban atmosphere’s diffusion capability, and therefore increased urban pollutant concentrations. For instance, the urban nitrogen oxides concentration increased by 2.1 μg m ?3 on average; the fine particulate matter (diameter of 2.5 μm or less; PM2.5) pollution concentration increased by 2.3 μg m ?3 on average; in highly urbanized areas, the PM2.5 concentration increased by 30 μg m ?3 and average visibility decreased by 0.2 km, with a maximum decrease of 1 km; the average number of daily hours of haze increased by 0.46 h; and the haze height lifted by 100–300 m. The “self-cleaning time” of pollutants increased by an average of 1.5 h.  相似文献   

19.
A new instrument (LOPAP: LOng Path liquid Absorption Photometer) for the sensitive detection of nitric acid (HNO3) in the atmosphere is described. HNO3 is sampled in a temperature controlled stripping coil mounted in an external sampling module to minimize sampling artefacts in sampling lines. After conversion into a strongly absorbing dye, HNO3 is detected in long path absorption in special Teflon® AF 2400 tubes used as liquid core wave guides. For the correction of some interferences, due to for example HONO and particle nitrate, two channels are used in series. The interferences from several potential interfering compounds including particle nitrate were quantified in the laboratory and in a large outdoor simulation chamber. With the exception of the interference caused by N2O5, which is quantitatively measured by the instrument, all tested interferences can be corrected under atmospheric conditions. Thus, in the instrument only the sum of N(V) from HNO3 and N2O5 is determined, which is expected to be a common problem of wet chemical HNO3 instruments. The instrument has a detection limit of 5–30 pptv for a time response of 6–2 min, respectively and was validated against the FTIR technique in a large outdoor simulation chamber. In addition, the applicability of the instrument was demonstrated in a field campaign.  相似文献   

20.
The angular momentum for ideal axisymmetric tropical cyclones on the f-plane is investigated with a focus on the total-volume integrated quantity. Budget analysis of the momentum equation at cylindrical coordinates shows that a tropical cyclone loses angular momentum during its development and mature stages due to the dynamical difference between the viscous inward-flow near the surface and the angular momentum conserving outward-flow aloft. The total relative angular momentum of a tropical cyclone, as a result, can be negative (i.e., implying anticyclonic rotation as a whole) despite intense cyclonic wind in the tropospheric layers. This anticyclonic rotation was measured in terms of the super-rotation ratio, the ratio of total relative angular momentum to the planetary angular momentum. Simulations with the numerical model of Weather Research and Forecasting (WRF) version 3.4.1 was found to be in favor of the theoretical angular-momentum budget analysis. It was revealed in the numerical simulations that the super-rotation ratio was negative, indicating a sub-rotation, as was predicted by analysis. The sub-rotation ratio was found to be less than one percent for typical tropical cyclones. To show the angular momentum decrease even in the decaying stage, numerical simulations where the thermal forcing by sea surface temperature switched off in the mature stage were carried out. In support of the angular momentum budget analysis, the results indicated that the angular momentum also decreases for a while soon after the forcing was eliminated.  相似文献   

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