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1.
A coupled meteorology and aerosol/chemistry model WRF-Chem(Weather Research and Forecast model coupled with Chemistry) was used to conduct a pair of simulations with present-day(PD) and preindustrial(PI) emissions over East Asia to examine the aerosol indirect effect on clouds.As a result of an increase in aerosols in January,the cloud droplet number increased by 650 cm-3 over the ocean and East China,400 cm-3 over Central and Southwest China,and less than 200 cm-3 over North China.The cloud liquid water path(LWP) increased by 40-60 g m-2 over the ocean and Southeast China and 30 g m-2 over Central China;the LWP increased less than 5 g m-2 or decreased by 5 g m-2 over North China.The effective radius(Re) decreased by more than 4 μm over Southwest,Central,and Southeast China and 2μm over North China.In July,variations in cloud properties were more uniform;the cloud droplet number increased by approximately 250-400 cm-3,the LWP increased by approximately 30-50 g m-2,and Re decreased by approximately 3 ?m over most regions of China.In response to cloud property changes from PI to PD,shortwave(SW) cloud radiative forcing strengthened by 30 W m-2 over the ocean and 10 W m-2 over Southeast China,and it weakened slightly by approximately 2-10 W m-2 over Central and Southwest China in January.In July,SW cloud radiative forcing strengthened by 15 W m-2 over Southeast and North China and weakened by 10 W m-2 over Central China.The different responses of SW cloud radiative forcing in different regions was related to cloud feedbacks and natural variability.  相似文献   

2.
To assess individual direct radiative effects of diverse aerosol species on a regional scale,the air quality modeling system RAMS-CMAQ(Regional Atmospheric Modeling System and Community Multiscale Air Quality) coupled with an aerosol optical properties/radiative transfer module was used to simulate the temporal and spatial distributions of their optical and radiative properties over East Asia throughout 2005.Annual and seasonal averaged aerosol direct radiative forcing(ADRF) of all important aerosols and individual components,such as sulfate,nitrate,ammonium,black carbon(BC),organic carbon(OC),and dust at top-of-atmosphere(TOA) in clear sky are analyzed.Analysis of the model results shows that the annual average ADRF of all important aerosols was in the range of 0 to-18 W m?2,with the maximum values mainly distributed over the Sichuan Basin.The direct radiative effects of sulfate,nitrate,and ammonium make up most of the total ADRF in East Asia,being concentrated mainly over North and Southeast China.The model domain is also divided into seven regions based on different administrative regions or countries to investigate detailed information about regional ADRF variations over East Asia.The model results show that the ADRFs of sulfate,ammonium,BC,and OC were stronger in summer and weaker in winter over most regions of East Asia,except over Southeast Asia.The seasonal variation in the ADRF of nitrate exhibited the opposite trend.A strong ADRF of dust mainly appeared in spring over Northwest China and Mongolia.  相似文献   

3.
The air quality model system RAMS (Regional Atmospheric Modeling System)-CMAQ (Models-3 Community Multi-scale Air Quality) coupled with an aerosol optical/radiative module was applied to investigate the impact of different aerosol mixing states (i.e., externally mixed, half externally and half internally mixed, and internally mixed) on radiative forcing in East Asia. The simulation results show that the aerosol optical depth (AOD) generally increased when the aerosol mixing state changed from externally mixed to internally mixed, while the single scattering albedo (SSA) decreased. Therefore, the scattering and absorption properties of aerosols can be significantly affected by the change of aerosol mixing states. Comparison of simulated and observed SSAs at five AERONET (Aerosol Robotic Network) sites suggests that SSA could be better estimated by considering aerosol particles to be internally mixed. Model analysis indicates that the impact of aerosol mixing state upon aerosol direct radiative forcing (DRF) is complex. Generally, the cooling effect of aerosols over East Asia are enhanced in the northern part of East Asia (Northern China, Korean peninsula, and the surrounding area of Japan) and are reduced in the southern part of East Asia (Sichuan Basin and Southeast China) by internal mixing process, and the variation range can reach 5 W m－2. The analysis shows that the internal mixing between inorganic salt and dust is likely the main reason that the cooling effect strengthens. Conversely, the internal mixture of anthropogenic aerosols, including sulfate, nitrate, ammonium, black carbon, and organic carbon, could obviously weaken the cooling effect.  相似文献   

4.
在区域气候化学模式系统（RegCCMS）中,分别采用Hegg、Hansen、Ghan、Jones等4种云滴数浓度参数化方案,模拟研究了2003年10月硝酸盐气溶胶的浓度分布和第一间接气候效应,并对不同方案进行比较。结果表明,不同方案模拟的硝酸盐气溶胶分布大体上一致,主要集中在河南、山东、河北、四川等地,地面浓度最大值达18 μg/m3。Hegg、Hansen、Ghan、Jones等 4种云滴数浓度参数化方案计算得到的由硝酸盐气溶胶所造成的第一间接辐射强迫全国平均值分别为-148、-205、-161和-140 W/m2。4种方案模拟的硝酸盐气溶胶间接效应都表现为近地面气温下降,降水减少,其中Hansen方案的间接效应最强,Ghan、Hegg方案次之,Jones方案最弱。  相似文献   

5.
In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced by source emissions in 2006 and 2010 also reveals the sensitivity of the radiative effects to source emission.The results are shown as follows:(1) Compared with those in 2006,the annual average surface concentration of sulfate in 2010 decreased over central and eastern China with a range of-5 to 0 μg/m~3;the decrease of annual average aerosol optical depth of sulfate over East China varied from 0.04 to 0.08;the annual average surface concentrations of BC,OC and nitrate increased over central and eastern China with maximums of 10.90,11.52 and 12.50μg/m~3,respectively;the annual aerosol optical depths of BC,OC and nitrate increased over some areas of East China with extremes of 0.006,0.007 and 0.008,respectively.(2)For the regional average results in 2010,the radiative forcings of sulfate,BC,OC,nitrate and their total net radiative forcing at the top of the atmosphere over central and eastern China were-0.64,0.29,-0.41,-0.33 and-1.1 W/m~2,respectively.Compared with those in 2006,the radiative forcings of BC and OC in 2010 were both enhanced,while that of sulfate and the net radiative forcing were both weakened over East China mostly.(3)The reduction of the cooling effect of sulfate in 2010 produced a warmer surface air temperature over central and eastern China;the maximum value was 0.25 K.The cooling effect of nitrate was also slightly weakened.The warming effect of BC was enhanced over most of the areas in China,while the cooling effect of OC was enhanced over the similar area,particularly the area between Yangtze and Huanghe Rivers.The net radiative effect of the four anthropogenic aerosols generated the annual average reduction and the maximum reduction were-0.096 and-0.285 K,respectively,for the surface temperature in 2006,while in 2010 they were-0.063 and-0.256 K,respectively.In summary,the change in source emission lowered the cooling effect of anthropogenic aerosols,mainly because of the enhanced warming effect of BC and weakened cooling effect of scattering aerosols.  相似文献   

6.
东亚地区云和地表反照率对硫酸盐直接辐射强迫的影响   总被引：9，自引：3，他引：9  
王喜红  石广玉 《气象学报》2002,60(6):758-765
文中利用区域气候模式深入探讨了东亚地区云及地表反照率对硫酸盐直接辐射强迫的影响 ,同时定量估算了东亚地区云区气溶胶的直接辐射强迫 ,讨论了硫酸盐对地表和大气短波辐射平衡产生的不同影响。研究表明 :云对气溶胶的直接辐射强迫具有很强的减弱作用 ,这种减弱作用不仅取决于云覆盖份数 ,而且取决于云的光学厚度。就区域平均而言 ,文中模拟的东亚地区气溶胶直接辐射强迫为 - 0 .0 97W /m2 ,占总直接辐射强迫的 10 .4%左右。表明云对硫酸盐直接辐射具有很强的减弱作用 ,在估算其总的直接辐射强迫时 ,云区的贡献不可忽视。较高的地表反照率会减弱硫酸盐的直接辐射强迫 ,而较低地表反照率则会增加硫酸盐的辐射强迫。硫酸盐气溶胶对大气辐射平衡影响非常小 ,但对地表辐射平衡产生重要影响 ,影响程度与大气几乎一致。  相似文献   

7.
The National Center for Atmospheric Research Community Atmosphere Model (version 3.5) coupled with the Morrison?CGettelman two-moment cloud microphysics scheme is employed to simulate the aerosol effects on clouds and precipitation in two numerical experiments, one representing present-day conditions (year?2000) and the other the pre-industrial conditions (year?1750) over East Asia by considering both direct and indirect aerosol effects. To isolate the aerosol effects, we used the same set of boundary conditions and only altered the aerosol emissions in both experiments. The simulated results show that the cloud microphysical properties are markedly affected by the increase in aerosols, especially for the column cloud droplet number concentration (DNC), liquid water path (LWP), and the cloud droplet effective radius (DER). With increased aerosols, DNC and LWP have been increased by 137% and 28%, respectively, while DER is reduced by 20%. Precipitation rates in East Asia and East China are reduced by 5.8% and 13%, respectively, by both the aerosol??s second indirect effect and the radiative forcing that enhanced atmospheric stability associated with the aerosol direct and first indirect effects. The significant reduction in summer precipitation in East Asia is also consistent with the weakening of the East Asian summer monsoon, resulting from the decreasing thermodynamic contrast between the Asian landmass and the surrounding oceans induced by the aerosol??s radiative effects. The increase in aerosols reduces the surface net shortwave radiative flux over the East Asia landmass, which leads to the reduction of the land surface temperature. With minimal changes in the sea surface temperature, hence, the weakening of the East Asian summer monsoon further enhances the reduction of summer precipitation over East Asia.  相似文献   

8.
在过去的20多年里,中外对硫酸盐气溶胶做了大量的研究,对它在大气中的排放、含量、光学特征和辐射强迫有了深入的认识;由于硝酸盐气溶胶在大气中平均含量比硫酸盐低很多,因此过去人们对硝酸盐的研究没有给予重视。然而,近年来的研究表明,硝酸盐气溶胶的散射性质在某些波段甚至强于硫酸盐;同时,由于未来对人为硫酸盐前体物的减排,硫酸盐气溶胶排放会大幅度减少,而硝酸盐气溶胶的排放却增长迅速,其在人为气溶胶中所占的比重越来越高,将会导致其在未来造成的辐射强迫有可能超过硫酸盐,使得其在地区范围内和季节尺度上成为重要的辐射强迫和气候影响因子。中国是硝酸盐气溶胶排放量较大的地区,硝酸盐对未来中国气候和气候变化的影响显得越来越重要。因此,就近年来有关硝酸盐气溶胶的排放和在大气中的浓度变化、光学厚度分布特征及其辐射强迫的研究进展做了回顾和介绍,并对其未来的研究做了展望。  相似文献   

9.
The authors used a high-resolution regional climate model(RegCM3) coupled with a chemistry/aerosol module to simulate East Asian climate in 2006 and to test the climatic impacts of aerosols on regionalscale climate.The direct radiative forcing and climatic effects of aerosols(dust,sulfate,black carbon,and organic carbon) were discussed.The results indicated that aerosols generally produced negative radiative forcing at the top-of-the-atmosphere(TOA) over most areas of East Asia.The radiative forcing induced by aerosols exhibited significant seasonal and regional variations,with the strongest forcing occurring in summer.The aerosol feedbacks on surface air temperature and precipitation were clear.Surface cooling dominated features over the East Asian continental areas,which varied in the approximate range of-0.5 to-2°C with the maximum up to-3-C in summer over the deserts of West China.The aerosols induced complicated variations of precipitation.Except in summer,the rainfall generally varied in the range of-1 to 1 mm d-1 over most areas of China.  相似文献   

10.
The indirect radiative and climatic effects of sulfate and organic carbon aerosols over East Asia were investigated using a Regional Integrated Environment Model System (RIEMS) with an empirical aerosol-cloud parameterization.The first indirect radiative forcing was negative and ranged from-9-0 W m-2 in the domain.The maximum cooling,up to-9 W m-2,occurred in the Chongqing District in winter,whereas the cooling areas were larger during summer than in winter.Organic carbon (OC) aerosols were more abundant in winter than in summer,whereas the sulfate concentration during summer was much higher than during winter.The concentrations of sulfate and OC were comparable in winter,and sulfate played a dominant role in determining indirect radiative forcing in summer,whereas in winter,both sulfate and OC were important.The regional mean indirect radiative forcings were-0.73 W m-2 and-0.41 W m-2 in summer and winter,respectively.The surface cooling caused by indirect effects was more obvious in winter than that in summer.The ground temperature decreased by ～1.2 K in most areas of eastern China in winter,whereas in summer,the temperature decreased (～-1.5 K) in some regions,such as the Yangtze River region,but increased (～0.9 K) in the areas between the Yellow and Yangtze Rivers.In winter,the precipitation decreased by 0-6 mm in most areas of eastern China,but in summer,alternating bands of increasing (up to 80 mm) and decreasing (～-80 mm) precipitation appeared in eastern China.  相似文献   

11.
运用区域气候模式RegCM3耦合入一个化学过程,对东亚地区三类人为排放气溶胶（硫酸盐、黑碳和有机碳）的时空分布特征及其对夏季风环流的影响进行了数值模拟研究。模拟结果显示,气溶胶的引入会引起东亚地区夏季850 hPa风场发生改变,我国江淮以东洋面上空出现了一个气旋式距平环流中心,中心以西的偏北风气流将削弱东亚地区夏季西南季风。通过讨论春季中国地区气溶胶浓度与夏季东亚地区850 hPa经向风的时滞关系,以及夏季中国地区气溶胶浓度与同期东亚地区850 hPa经向风的关系,可以发现,春、夏季中国地区气溶胶浓度均与夏季东亚地区850 hPa经向风有很好的负相关关系,当春季中国北方和夏季中国南方地区气溶胶浓度增加时,中国东部地区夏季偏南季风减弱。这可能与气溶胶改变了大气层顶和地表的辐射强迫,进而引起了海陆气压差异和位势高度场的变化有关。  相似文献   

12.
Why Is the Climate Forcing of Sulfate Aerosols So Uncertain?   总被引：2，自引：0，他引：2  
l. IntroductionAlthough the aerosol has been recognized as an important factor which has innuence onthe past, present and future climate for a long time, it still has much uncertainty in assessingits climate forcing. The direct radiative forcing of sulfate aerosols has been estimated rangingfrom --0.3 W/ m2 to --0.9 W/ m2 in recent publications (Charlson et al., l992, Kiehl andBriegleb l993; Taylor and Penner 1994, Boucher and Anderson l995, Kieh1 and Rodhe l995;Chuang et al., l997, Penne…  相似文献   

13.
运用区域气候模式RegCM3耦合入一个化学过程,对东亚地区三类人为排放气溶胶（硫酸盐、黑碳和有机碳）的时空分布特征及其对夏季风环流的影响进行了数值模拟研究.模拟结果显示,气溶胶的引入会引起东亚地区夏季850 hPa风场发生改变,我国江淮以东洋面上空出现了一个气旋式距平环流中心,中心以西的偏北风气流将削弱东亚地区夏季西南季风.通过讨论春季中国地区气溶胶浓度与夏季东亚地区850 hPa经向风的时滞关系,以及夏季中国地区气溶胶浓度与同期东亚地区850 hPa经向风的关系,可以发现,春、夏季中国地区气溶胶浓度均与夏季东亚地区850hPa经向风有很好的负相关关系,当春季中国北方和夏季中国南方地区气溶胶浓度增加时,中国东部地区夏季偏南季风减弱.这可能与气溶胶改变了大气层顶和地表的辐射强迫,进而引起了海陆气压差异和位势高度场的变化有关.  相似文献   

14.
吴蓬萍  韩志伟 《大气科学》2011,35(3):547-559
本文利用发展的RIEMS对硫酸盐气溶胶第一间接辐射强迫及其气候效应进行了研究.同卫星观测和其它模式模拟结果对比表明,RIEMS能比较好地模拟云和辐射过程.东亚地区硫酸盐气溶胶的第一间接辐射强迫为负并有明显的季节变化,各季节分别为:冬季-0.88 W/m2,春季-2.27 W/m2,夏季-2.41 W/m2,秋季-1.4...  相似文献   

15.
The air quality modeling system RAMS （Regional Atmospheric Modeling System）-CMAQ （Models-3 Community Multi-scale Air Quality） is developed to simulate the aerosol optical depth （AOD） and aerosol direct forcing （DF）. The aerosol-specific extinction, single scattering albedo, and asymmetry factor are parameterized based on Mie theory taking into account the aerosol size distribution, composition, refractive index, and water uptake of solution particles. A two-stream solar radiative model considers all gaseous molecular absorption, Rayleigh scattering, and aerosols and clouds. RAMSCMAQ is applied to simulate all major aerosol concentrations （e.g., sulfate, nitrate, ammonium, organic carbon, black carbon, fine soil, and sea salt） and AOD and DF over East Asia in 2005. To evaluate its performance, the simulated AOD values were compared with ground-based in situ measurements. The comparison shows that RAMSCMAQ performed well in most of the model domain and generally captured the observed variations. High AOD values （0.2-1.0） mainly appear in the Sichuan Basin as well as in central and southeastern China. The geographic distribution of DF generally follows the AOD distribution patterns, and the DF at the top-of-the-atmosphere is less than -25 and -20 W m^-2 in clear-sky and all-sky over the Sichuan Basin. Both AOD and DF exhibit seasonal variations with lower values in July and higher ones in January. The DF could obviously be impacted by high cloud fractions.  相似文献   

16.
本文应用WRF-Chem(Weather Research and Forecasting—Chemistry)模式研究中国东部地区气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)在天气尺度下的辐射强迫和对地面气温的影响。5个无明显降水时间段(2006年8月23～25日、2008年11月10～12日、2008年12月16～18日、2009年1月15～17日和2009年4月27～29日)的模拟显示,气溶胶浓度呈现显著的白天低,夜间高的日变化特征,且北方区域(29.8°～42.6°N,110.2°～120.3°E)平均PM2.5近地面浓度(40～80 μg m-3)高于南方区域(22.3°～29.9°N,109.7°～120.2°E,30～47 μg m-3)。气溶胶对地面2 m温度(地面气温)有明显的降温效果,在早上08:00(北京时,下同)和下午17:00左右最为显著,最高可降低约0.2～1 K,同时气溶胶的参与改善了模式对地面气温的模拟。本文还通过对2006年8月23～25日一次个例的模拟,定量分析了气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)的总天气效应(直接效应+间接效应)、直接效应和间接效应分别对到达地面的短波辐射和地面气温的影响。北方区域平均气溶胶直接效应所造成的短波辐射强迫要高于南方区域,分别为-11.3 W m-2和-5.8 W m-2,导致地面气温分别降低了0.074 K和0.039 K。南方区域平均气溶胶间接效应所产的短波辐射强迫高于北方区域,分别为-14.4 W m-2和-12.4 W m-2,引起的地面气温的改变分别为-0.094 K和-0.035 K。对于气溶胶组分,硫酸盐气溶胶的直接效应和间接效应的作用相当,其总效应在北方和南方区域平均短波辐射强迫分别为-7.0 W m-2和-10.5 W m-2,对地面气温的影响为-0.062 K和-0.074 K,而硝酸盐气溶胶的作用略小。黑碳气溶胶使得北方和南方区域平均到达地表的太阳短波辐射分别减少了6.5 W m-2和5.8 W m-2,而地表气温则分别增加了0.053 K和0.017 K,相比于间接效应,黑碳气溶胶的直接效应的影响更加显著。  相似文献   

17.
中国地区春季沙尘气溶胶短波辐射气候效应数值模拟研究   总被引：1，自引：0，他引：1  
利用耦合了起沙模型(MEDM)的区域气候模式RegCM3,模拟研究了2000年春季中国地区沙尘气溶胶短波辐射气候效应。结果表明,春季中国沙尘气溶胶垂直负荷的大值区主要位于南疆盆地和阿拉善高原。引入沙尘气溶胶后,中国地区地表均出现负的辐射强迫,地面气温普遍降低,中低层(400 hPa层以下)大气温度则呈上升趋势。沙尘源区及其下游地区总云量及降水主要呈减少趋势,云量与降水的分布特征与空中流场的变化趋势一致性较好。  相似文献   

18.
中国地区气溶胶的辐射强迫及其气候响应试验   总被引：15，自引：3，他引：12  
胡荣明  石广玉 《大气科学》1998,22(6):917-525
根据国内测定的排放因子数据和国家、部委及各省市统计年鉴公布的排放源数据,得到的中国大陆的1°×1°网格精度的SO2的排放分布,计算了中国地区人为扰动气溶胶的辐射强迫。应用近期开发的二维能量平衡模式计算了由该种气溶胶所引起的中国地区地面温度变化。模式结果表明,最大辐射强迫和最大地面温度变化都集中在中国的沿海和四川地区。最大辐射强迫达3 W/m2。  相似文献   

19.
 The atmospheric general circulation model ECHAM-4 is coupled to a chemistry model to calculate sulfate mass distribution and the radiative forcing due to sulfate aerosol particles. The model simulates the main components of the hydrological cycle and, hence, it allows an explicit treatment of cloud transformation processes and precipitation scavenging. Two experiments are performed, one with pre-industrial and one with present-day sulfur emissions. In the pre-industrial emission scenario SO2 is oxidized faster to sulfate and the in-cloud oxidation via the reaction with ozone is more important than in the present-day scenario. The atmospheric sulfate mass due to anthropogenic emissions is estimated as 0.38 Tg sulfur. The radiative forcing due to anthropogenic sulfate aerosols is calculated diagnostically. The backscattering of shortwave radiation (direct effect) as well as the impact of sulfate aerosols on the cloud albedo (indirect effect) is estimated. The model predicts a direct forcing of −0.35 W m-2 and an indirect forcing of −0.76 W m-2. Over the continents of the Northern Hemisphere the direct forcing amounts to −0.64 W m-2. The geographical distribution of the direct and indirect effect is very different. Whereas the direct forcing is strongest over highly polluted continental regions, the indirect forcing over sea exceeds that over land. It is shown that forcing estimates based on monthly averages rather than on instantaneous sulfate pattern overestimate the indirect effect but have little effect on the direct forcing. Received: 16 October 1996/Accepted: 24 October 1996  相似文献   

20.
Summary Regional climate model (RegCM2) and sulfur transport model (NJUADMS) were combined to simulate the distribution of anthropogenic sulfate aerosol burden over China, where a look up table method was applied to illustrate sulfate formation from SO2-oxidation. Direct radiative forcing of sulfate aerosol was further estimated using the scheme suggested by Charlson et al (1991). Investigations show that the annual average total sulfate column over mainland China is 2.01mg/m2 with high value in East and Central areas (more than 7mg/m2). The annual average direct radiative forcing of China is about –0.85W/m2. The forcing can reach –7W/m2 in Central and East China during the winter season. Total sulfate column shows significant seasonal variations with winter maximum-summer minimum in the Southern part of China and spring maximum-autumn minimum in the northern part of China. Strong seasonal cycles of direct radiative forcing are also found due to the influence of total sulfate column, cloud, relative humidity and the reflectivity of underlying surfaceReceived May 16, 2001; accepted August 5, 2002 Published online: May 8, 2003  相似文献   

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