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1.
Deciduous forest covers vast areas of permafrost under severe dry climate in eastern Siberia. Understanding the water cycle in this forest ecosystem is quite important for climate projection. In this study, diurnal variations in isotopic compositions of atmospheric water vapour were observed in eastern Siberia with isotope analyses of precipitation, sap water of larch trees, soil water, and water in surface organic layer during the late summer periods of 2006, 2007, and 2008. In these years, the soil moisture content was considerably high due to unusually large amounts of summer rainfall and winter snowfall. The observed sap water δ18O ranged from ?17.9‰ to ?13.3‰, which was close to that of summer precipitation and soil water in the shallow layer, and represents that of transpired water vapour. On sunny days, as the air temperature and mixing ratio rose from predawn to morning, the atmospheric water vapour δ18O increased by 1‰ to 5‰ and then decreased by about 2‰ from morning to afternoon with the mixing ratio. On cloudy days, by contrast, the afternoon decrease in δ18O and the mixing ratio was not observed. These results show that water vapour that transpired from plants, with higher δ18O than the atmospheric water vapour, contributes to the increase in δ18O in the morning, whereas water vapour in the free atmosphere, with lower δ18O, contributes to the decrease in the afternoon on sunny days. The observed results reveal the significance of transpired water vapour, with relatively high δ18O, in the water cycle on a short diurnal time scale and confirm the importance of the recycling of precipitation through transpiration in continental forest environments such as the eastern Siberian taiga. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

2.
M. Z. Iqbal 《水文研究》2008,22(23):4609-4619
Oxygen and deuterium isotopes in precipitation were analysed to define local isotopic trends in Iowa, US. The area is far inland from an oceanic source and the observed averages of δ18O and δ D are ? 6·43‰ and ? 41·35‰ for Ames, ? 7·53‰ and ? 51·33‰ for Cedar Falls, and ? 6·01‰ and ? 38·19‰ for Iowa City, respectively. Although these data generally follow global trends, they are different when compared to a semi‐arid mid‐continental location in North Platt, Nebraska. The local meteoric water lines of Iowa are δ D = 7·68 δ18O + 8·0 for Ames, δ D = 7·62 δ18O + 6·07 for Cedar Falls, and δ D = 7·78 δ18O + 8·61 for Iowa City. The current Iowa study compares well with a study conducted in Ames, Iowa, 10 years earlier. The differences between Iowa and Nebraska studies are attributed to a variable climate across the northern Great Plains ranging from sub‐humid in the east to semi‐arid in the west. Iowa being further east in the region is more strongly influenced by a moist sub‐humid to humid climate fed by the tropical air stream from the Gulf of Mexico. The average d‐excess values are 10·06‰ for Ames, 8·92‰ for Cedar Falls and 9·92‰ for Iowa City. Eighty seven percent of the samples are within the global d‐excess range of 0‰ and 20‰. The results are similar to previous studies, including those by National Atmospheric Deposition Programs and International Atomic Energy Agency. It appears that the impact of recycled water or secondary evaporation on δ18O values of area precipitation is minimal. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

3.
We characterize the precipitation and groundwater in a mountainous (peaks slightly above 3000 m a.s.l.), semi‐arid river basin in SE Spain in terms of the isotopes 18O and 2H. This basin, with an extension of about 7000 km2, is an ideal site for such a study because fronts from the Atlantic and the Mediterranean converge here. Much of the land is farmed and irrigated both by groundwater and runoff water collected in reservoirs. A total of approximately 100 water samples from precipitation and 300 from groundwater have been analysed. To sample precipitation we set up a network of 39 stations at different altitudes (800–1700 m a.s.l.), with which we were able to collect the rain and snowfall from 29 separate events between July 2005 and April 2007 and take monthly samples during the periods of maximum recharge of the aquifers. To characterize the groundwater we set up a control network of 43 points (23 springs and 20 wells) to sample every 3 months the main aquifers and both the thermal and non‐thermal groundwater. We also sampled two shallow‐water sites (a reservoir and a river). The isotope composition of the precipitation forms a local meteoric water line (LMWL) characterized by the equation δD = 7·72δ18O + 9·90, with mean values for δ18O and δD of − 10·28‰ and − 69·33‰, respectively, and 12·9‰ for the d‐excess value. To correlate the isotope composition of the rainfall water with groundwater we calculated the weighted local meteoric water line (WLMWL), characterized by the equation δD = 7·40δ18O + 7·24, which takes into account the quantity of water precipitated during each event. These values of (dδD/dδ18O)< 8 and d‐excess (δD–8δ18O)< 10 in each curve bear witness to the ‘amount effect’, an effect which is more manifest between May and September, when the ground temperature is higher. Other effects noted in the basin were those of altitude and the continental influence. The isotopic compositions of the groundwater are represented by the equation δD = 4·79δ18O − 18·64. The groundwater is richer in heavy isotopes than the rainfall, with mean values of − 8·48‰ for δ18O and − 59·27‰ for δD. The isotope enrichment processes detected include a higher rate of evaporation from detrital aquifers than from carbonate ones, the effects of recharging aquifers from irrigation return flow and/or from reservoirs' leakage and enrichment in δ18O from thermal water. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

4.
The hydrology of oxygen‐18 (18O) isotopes was monitored between 1995 and 1998 in the Allt a' Mharcaidh catchment in the Cairngorm Mountains, Scotland. Precipitation (mean δ18O=−7·69‰) exhibited strong seasonal variation in δ18O values over the study period, ranging from −2·47‰ in the summer to −20·93‰ in the winter months. As expected, such variation was substantially damped in stream waters, which had a mean and range of δ18O of −9·56‰ and −8·45 to −10·44‰, respectively. Despite this, oxygen‐18 proved a useful tracer and streamwater δ18O variations could be explained in terms of a two‐component mixing model, involving a seasonally variable δ18O signature in storm runoff, mixing with groundwater characterized by relatively stable δ18O levels. Variations in soil water δ18O implied the routing of depleted spring snowmelt and enriched summer rainfall into streamwaters, probably by near‐surface hydrological pathways in peaty soils. The relatively stable isotope composition of baseflows is consistent with effective mixing processes in shallow aquifers at the catchment scale. Examination of the seasonal variation in δ18O levels in various catchment waters provided a first approximation of mean residence times in the major hydrological stores. Preliminary estimates are 0·2–0·8 years for near‐surface soil water that contributes to storm runoff and 2 and >5 years for shallow and deeper groundwater, respectively. These 18O data sets provide further evidence that the influence of groundwater on the hydrology and hydrochemistry of upland catchments has been underestimated. Copyright © 2000 John Wiley & Sons, Ltd.  相似文献   

5.
P. Rodgers  C. Soulsby  S. Waldron 《水文研究》2005,19(11):2291-2307
δ18O measurements of precipitation and stream waters were used as a natural tracer to investigate hydrological pathways and residence times in the River Feshie, a complex mesoscale (231 km2) catchment in the Cairngorm Mountains of Scotland. Precipitation δ18O exhibited strong seasonal variation over the 2001–02 hydrological year, ranging from −6·9‰ in the summer, to −12·0‰ during winter snowfalls (mean δ18O −9·59‰). Although damped, this seasonality was reflected in stream water outputs at seven sampling sites in the catchment, allowing δ18O variations to be used to infer hydrological source areas. Thus, stream water δ18O was generally controlled by a seasonally variable storm flow end member, mixing with groundwater of more constant isotopic composition. Periodic regression analysis allowed the differences in this mixing process between monitoring subcatchments to be assessed more quantitatively to provide a preliminary estimate of mean stream water residence time. This demonstrated the importance of responsive hydrological pathways associated with peat and shallow alpine soils in the headwater subcatchments in producing seasonally variable runoff with short mean residence times (33–113 days). In contrast, other tributaries with more freely draining soils and larger groundwater storage in shallow aquifers provided more effective mixing of variable precipitation inputs, resulting in longer residence time estimates (178–445 days). The mean residence time of runoff leaving the Feshie catchment reflected an integration of these contrasting influences (110–200 days). These insights from δ18O measurements extend the hydrological understanding of the Feshie catchment gained from other hydrochemical tracers, and demonstrate the utility of isotope tracers in investigating hydrological processes at the mesoscale. Copyright © 2005 John Wiley & Sons, Ltd.  相似文献   

6.
A Lagrangian (Rayleigh) distillation model is used to track the evolution of stable isotopes in precipitation over mountainous terrain from the Pacific Coast of Canada to two alpine field sites in the Canadian Rocky Mountains. Precipitation δ18O at Vancouver constrains the model and air–mass back trajectories provide the water vapour pathway for 10 winter storm events. Isotopic values along storm pathways are modelled with a classical Rayleigh model that prescribes a linear decrease in temperature and pressure from initial to final conditions, and two models that account directly for orographic precipitation processes by: (i) applying an orographic rainfall model and (ii) using North American Regional Reanalysis data to calculate the change in vapour content along storm pathways. All models are significant predictors of snowpack δ18O, but the orographic model provides the best fit to precipitation‐weighted δ18O for each storm. The improvement in modelled δ18O by accounting for terrain along storm trajectories illustrates the need to account for orographically driven moisture loss when modelling vapour transport to ice core sites with mountainous upwind terrain. This finding is also applicable to isotopic studies of paleoaltimetry and source areas of groundwater recharge. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

7.
The δ2H and δ18O composition of 77 precipitation samples collected between January 2014 and April 2019 from two sites across the Guadalquivir Basin, SW Spain, were analysed. The first site is located in an urban area of Seville at 100 km distance to the Atlantic coast and the second site is located in a dune area of the Doñana National Park a few kilometres from the coast. Sampling was performed within intervals of at least 14 days if rain occurred but frequently intervals were longer according to the rainfall incidence. Samples from both sites are available for the period February 2016 to June 2018 with six samples containing identical rain events at both locations. Precipitation weighted averages and local meteoric water lines produced by weighting and non-weighting regression methods are presented for its use in hydrological applications. Results show a remarkably high variability in δ2H and δ18O values and precipitation weighted average d-excess values of 11.8‰ and 13‰ at the sites Plaza de España and Doñana, respectively. Temperature and amount effects were found to be weak. A significant influence of secondary evaporation for single rainfall events during summer was identified by enriched isotopic signatures with reduced d-excess values plotting close or below the global meteoric water line. Backward trajectory analysis of 115 days with daily rainfall above 3 mm yield a predominant Atlantic Ocean vapour source with negligible Mediterranean influence and therefore, d-excess variability is attributed to the different ocean surface conditions of relative humidity and sea surface temperature. Parallel sampling indicate very similar isotopic signatures at both sites and point to the existence of thermal effects of the Plaza de España site in Seville city during the summer season.  相似文献   

8.
Little is known about the spatial and temporal variability of the stable isotopic composition of precipitation in the North Atlantic and its relationship to the North Atlantic Oscillation (NAO) and anthropogenic climate change. The islands of the Azores archipelago are uniquely positioned in the middle of the North Atlantic Ocean to address this knowledge gap. A survey of spatial and temporal variability of the stable isotope composition of precipitation in Azores is discussed using newly presented analyses along with Global Network of Isotopes in Precipitation data. The collected precipitation samples yield a new local meteoric water line (δ2H = 7.1 * δ18O + 8.46) for the Azores region and the North Atlantic Ocean. The annual isotopic mean of precipitation shows a small range for the unweighted and precipitation mass‐weighted δ18O‐H2O values. Results show an inverse relation between the monthly δ18O‐H2O and the amount of precipitation, which increases in elevation and into the interior of the island. Higher amounts of precipitation (from convective storm systems) do not correspond to the most depleted values of stable isotopes in precipitation. Precipitation shows an orographic effect with depleted δ18O‐H2O values related to the Rayleigh effect. Monthly δ18O‐H2O values for individual precipitation sampling stations show little relationship to air temperature. Results show a local source of moisture during the summer with the characteristics of the first vapour condensate. The stable isotope composition of precipitation is strongly correlated to the NAO index, and δ18O‐H2O values show a statistically significantly trend towards enrichment since 1962 coincident with the increased air temperature and relative humidity due to climate change. Results are in line with observations of increasing sea surface temperature and relative humidity.  相似文献   

9.
Stable isotopic composition of precipitation as preserved in continental proxy climate archives (e.g., ice cores, lacustrine sediments, tree rings, groundwater, and organic matter) can sensitively record fluctuations in local meteorological variables. These are important natural climatic tracers to understand the atmospheric circulation patterns and hydrological cycle and to reconstruct past climate from archives. Precipitation was collected at Dokriani Glacier to understand the response of glaciers to climate change in the Garhwal Central Himalaya, Upper Ganga Basin. The local meteoric water line deviates from the global meteoric water line and is useful for the identification of moisture source in the region. The data suggest different clusters of isotopic signals, that is, summer (June–September) and winter (November–April); the mean values of δ18O, δD, and d ‰ during summer are ?13.03‰, ?84.49‰, and 19.78 ‰, respectively, whereas during winter, the mean values of δ18O, δD, and d ‰ are ?7.59‰, ?36.28‰, and 24.46 ‰, respectively. Backward wind trajectory analysis ascertains that the major source of precipitation during summer is from the Indian Summer Monsoon and during winter from the westerlies. Regression analysis has been carried out in order to establish interrelationship between the precipitation isotopic signatures and meteorological variables such as air temperature, relative humidity, and precipitation. Temperature and precipitation have good correlation with the isotopic signatures of precipitation with R2 values >.5, suggesting that both temperature and amount effects prevail in the study region. Multiple regression analysis found strong relationships for both the seasons. The relationship of deuterium excess with δ18O, relative humidity, and precipitation are significant for the winter season. No significant relationships of deuterium excess were found with other meteorological variables such as temperature and radiation. The correlation and regression analysis performed are significant and valuable for interpretation of processes in the hydrological cycle as well as for interpretation of palaeoclimate records from the region.  相似文献   

10.
The continuous real‐time analysis, at 30‐s intervals, of precipitation at an Australian tropical location revealed extreme and rapidly changing δ18O and δD values related to variations in moisture source areas, transport paths and precipitation histories. The range of δ18O (?19.6‰ to +2.6‰) and δD (?140‰ to +13‰) values from 5948 measurements of nine rain events over 15 days during an 8‐month period at a single location was comparable with the range measured in 1532 monthly samples from all seven Australian Global Network of Isotopes in Precipitation stations from 1962 to 2002. Extreme variations in δ18O (?8.7‰ to ?19.6‰) and δD (?54‰ to ?140‰) were recorded within a single 4‐h period. Real‐time stable isotope monitoring of precipitation at a high temporal resolution enables new and powerful tracer applications in climatology, hydrology, ecophysiology and palaeoclimatology. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

11.
The stable oxygen and hydrogen isotopic features of precipitation in Taiwan, an island located at the western Pacific monsoon area, are presented from nearly 3,500 samples collected during the past decade for 20 stations. Results demonstrate that moisture sources from diverse air masses with different isotopic signals are the main parameter in controlling the precipitation's isotope characteristics. The air mass from polar continental (Pc) region contributes the precipitation with high deuterium excess values (up to 23‰) and relatively enriched isotope compositions (e.g., ? 3.2‰ for δ18O) during the winter with prevailing northeasterly monsoon. By contrast, air masses from equatorial maritime (Em) and tropical maritime (Tm) supply the precipitation with low deuterium excess values (as low as about 7‰) and more depleted isotope values (e.g., ? 8.9‰ and ? 6.0‰ for δ18O of Tm and Em, respectively) during the summer with prevailing southwesterly monsoon. Thus seasonal differences in terms of δ18O, δD, and deuterium excess values are primarily influenced by the interactions among various precipitation sources. While these various air masses travel through Taiwan, secondary evaporation effects further modify the isotope characteristics of the inland precipitation, such as raindrop evaporation (reduces the deuterium excess of winter precipitation) and moisture recycling (increases the deuterium excess of summer precipitation). The semi-quantitative estimations in terms of evaluation for changes in the deuterium excess suggest that the raindrop evaporation fractions for winter precipitation range 7% to 15% and the proportions of recycling moisture in summer precipitation are less than 5%. Additionally, the isotopic altitude gradient in terms of δ18O for summer precipitation is ? 0.22‰/100 m, greater than ? 0.17‰/100 m of winter precipitation. The greater isotopic gradient in summer can be attributed to a higher temperature vs. altitude gradient relative to winter. The observed spatial and seasonal stable isotopic characteristics in Taiwan's precipitation not only contribute valuable information for regional monsoon research crossing the continent–ocean interface of East Asia, but also can serve as very useful database for local water resources management.  相似文献   

12.
Stable water isotopes (δ18O and δ2H) are an important source signature for understanding the hydrological cycle and altered climate regimes. However, the mechanisms underlying atmospheric water vapour isotopes in the northeast Qinghai‐Tibetan Plateau of central Asia remain poorly understood. This study initially investigated water vapour isotopic composition and its controls during the premonsoon and monsoon seasons. Isotopic compositions of water vapour and precipitation exhibited high variability across seasons, with the most negative average δ18O values of precipitation and the most positive δ18O values of water vapour found during the premonsoon periods. Temperature effect was significant during the premonsoon period but not the monsoon period. Both a higher slope and intercept of the local meteoric water line were found during the monsoon period as compared with in the premonsoon period, suggesting that raindrops have been experienced a greater kinetic fractionation process such as reevaporation below the cloud during the premonsoon periods. The δ2H and δ18O signatures in atmospheric water vapour tended to be depleted with the occurrence of precipitation events especially during the monsoon period and probably as a result of rainout processes. The monthly average contribution of evaporation from the lake to local precipitation was 35.2%. High d‐excess values of water vapour were influenced by the high proportion of local moisture mixing, as indicated by the gradually increasing relative humidity along westerly and Asian monsoon trajectories. The daily observation (observed ε) showed deviations from the equilibrium fractionation factors (calculated ε), implying that raindrops experienced substantial evaporative enrichment during their descent. The average fraction of raindrops reevaporation was estimated to be 16.4± 12.9%. These findings provide useful insights for understanding the interaction between water vapour and precipitation, moisture sources, and help in reconstructing the paleoclimate in the alpine regions.  相似文献   

13.
Characterization of stable isotope compositions (δ2H and δ18O) of surface water and groundwater in a catchment is critical for refining moisture sources and establishing modern isotope–elevation relationships for paleoelevation reconstructions. There is no consensus on the moisture sources of precipitation in the Yellow River source region during summer season. This study presents δ2H and δ18O data from 111 water samples collected from tributaries, mainstream, lakes, and groundwater across the Yellow River source region during summertime. Measured δ18O values of the tributaries range from ?13.5‰ to ?5.8‰ with an average of ?11.0‰. Measured δ18O values of the groundwater samples range from ?12.7‰ to ?10.5‰ with an average of ?11.9‰. The δ18O data of tributary waters display a northward increase of 1.66‰ per degree latitude. The δ18O data and d‐excess values imply that moisture sources of the Yellow River source region during summertime are mainly from the mixing of the Indian Summer Monsoon and the Westerlies, local water recycling, and subcloud evaporation. Analysis of tributary δ18O data from the Yellow River source region and streamwater and precipitation δ18O data from its surrounding areas leads to a best‐fit second‐order polynomial relationship between δ18O and elevation over a 4,600 m elevation range. A δ18O elevation gradient of ?1.6‰/km is also established using these data, and the gradient is in consistence with the δ18O elevation gradient of north and eastern plateau. Such relationships can be used for paleoelevation reconstructions in the Yellow River source region.  相似文献   

14.
Spatial and temporal variations of the isotopic composition of precipitation were investigated to better understand their controlling factors. Precipitation was collected from six locations in Hokkaido, Japan, and event‐based analyses were conducted for a period from March 2010 to February 2013. Relatively low δ values and a high d‐excess for annual averages were observed at three sites located along the Japan Sea compared to the three sites at Pacific Ocean side. Lower δ values in spring and fall and higher d‐excess in winter were observed for the region along the Japan Sea. In total, 264 precipitation events were identified. Precipitation originated predominantly from low‐pressure system (LPS) events, which were classified as northwest (LPS‐NW) and southeast (LPS‐SE) events according to the routes of the low‐pressure center, that passed northwest and southeast of Hokkaido, respectively. LPS‐SE events showed lower δ18O than LPS‐NW events, which is attributable to the lower δ18O of water vapor resulting from heavy rainfalls in the upstream region of the LPS air mass trajectories over the Pacific Ocean. This phenomenon observed in Hokkaido can be found in other midlatitude coastal regions and applied for hydrological, atmospheric, and paleoclimate studies. A characteristic spatial pattern was found in LPS‐NW events, in which lower δ18O was observed on the Japan Sea side than on the Pacific Ocean side in each season. This is likely due to the location of the sampling sites and their distance from the LPS: Precipitation with lower δ18O in the region along the Japan Sea occurs in a well‐developed cloud system near the low‐pressure center in cold and warm sectors of LPS, whereas precipitation with higher δ18O on the Pacific side mainly occurs in a warm sector away from the low‐pressure center. Air mass from the north does not always cause low δ in precipitation, and the precipitation process in the upstream region is another important factor controlling the isotopic composition of precipitation, other than the local temperature and precipitation amount.  相似文献   

15.
The stable isotope composition (18O and 2H) in the tropical precipitation collected from 18 locations throughout the Deduru Oya river basin in Sri Lanka, has been studied during August and September 2001, in order to characterize the isotopic composition of precipitation in the dry and intermediate climatic zones of Sri Lanka. The isotope compositions are described with respect to the distance from the coast and the altitude. The analyses show that δ18O vary from ? 5·11 to 1·39‰ and δD vary from ? 35·71 to 12·55‰. The d‐excess values range from ? 0·65 to 13·17 with an average value of ～7. Regression for the δ18O ? δD is y = 6·8x + 4·9 (R2 = 0·9) which is compatible with the precipitation in other tropical regions. The lower slope in the regression line and the lower d‐excess value indicate high temperature events which were possibly aided by concentration through successive evaporation within the atmosphere. The spatial variation of isotope composition indicates two different cloud contributions for the rain events, of which one may be linked to the Indian Ocean contribution and the other to the high altitude condensation. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

16.
The paper presents oxygen and hydrogen isotopes of 284 precipitation event samples systematically collected in Irkutsk, in the Baikal region (southeast Siberia), between June 2011 and April 2017. This is the first high-resolution dataset of stable isotopes of precipitation from this poorly studied region of continental Asia, which has a high potential for isotope-based palaeoclimate research. The dataset revealed distinct seasonal variations: relatively high δ18O (up to −4‰) and δD (up to −40‰) values characterize summer air masses, and lighter isotope composition (−41‰ for δ18O and −322‰ for δD) is characteristic of winter precipitation. Our results show that air temperature mainly affects the isotope composition of precipitation, and no significant correlations were obtained for precipitation amount and relative humidity. A new temperature dependence was established for weighted mean monthly precipitation: +0.50‰/°C (r2 = 0.83; p <.01; n = 55) for δ18O and +3.8‰/°C (r2 = 0.83, p < 0.01; n = 55) for δD. Secondary fractionation processes (e.g., contribution of recycled moisture) were identified mainly in summer from low d excess. Backward trajectories assessed with the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model indicate that precipitation with the lowest mean δ18O and δD values reaches Irkutsk in winter related to moisture transport from the Arctic. Precipitation originating from the west/southwest with the heaviest mean isotope composition reaches Irkutsk in summer, thus representing moisture transport across Eurasia. Generally, moisture transport from the west, that is, the Atlantic Ocean predominates throughout the year. A comparison of our new isotope dataset with simulation results using the European Centre/Hamburg version 5 (ECHAM5)-wiso climate model reveals a good agreement of variations in δ18O (r2 = 0.87; p <.01; n = 55) and air temperature (r2 = 0.99; p <.01; n = 71). However, the ECHAM5-wiso model fails to capture observed variations in d excess (r2 = 0.14; p < 0.01; n = 55). This disagreement can be partly explained by a model deficit of capturing regional hydrological processes associated with secondary moisture supply in summer.  相似文献   

17.
The local meteoric water line (LMWL), the functional relationship between locally measured values of δ18O and δ2H in precipitation, represents the isotopic composition of water entering hydrologic systems. The degree to which the LMWL departs from the global meteoric water line (GMWL), moreover, can reveal important information about meteoric sources of water (e.g. oceanic or terrestrial) and atmospheric conditions during transport. Here we characterize the isotopic composition of precipitation within an experimental watershed in the Western US that is subject to large topographic and seasonal gradients in precipitation. Interpreting the hydrometeorologic and spatial controls on precipitation, we constructed a seasonally weighted LMWL for southwestern Idaho that is expressed by the equation δ2H = 7.40 × δ18O ? 2.17. A seasonally weighted LMWL that is based on weighting isotopic concentrations by climatic precipitation volumes is novel, and we argue better represents the significant seasonality of precipitation in the region. The developed LMWL is considerably influenced by the semiarid climate experienced in southwest Idaho, yielding a slope and y‐intercept lower than the GMWL (δ2H = 8 × δ18O + 10). Moderate to strong correlations exist between the isotopic composition of precipitation from individual events and surface meteorologic variables, specifically surface air temperature, relative humidity, and precipitation amount. A strong negative correlation exists between the annual average isotopic composition of precipitation and elevation at individual collection sites, with a lapse rate of ?0.22‰/100 m. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

18.
Spatial and temporal variations of the isotopic composition of precipitation over Thailand were investigated. The local meteoric water line for Thailand deviates slightly from the global meteoric water line, with lower slopes (7.62 ± 0.07, 7.59 ± 0.08) and intercepts (6.42 ± 0.39, 6.22 ± 0.42) using ordinary and precipitation weighted methods. Differences in spatial and temporal δ18O distributions between the tropical monsoon and tropical savanna climate zones were found due to differing moisture source contributions and seasonal precipitation patterns. The temporal data reveals that the northeast monsoon rains originate from isotopically-enriched local moisture with isotope values of −9.36 to −0.09‰ (mean − 3.73 ± 0.42‰), whereas the southwest monsoon clouds had a more significant rainout effect from Rayleigh distillation, with isotope values of −9.56 to −1.78‰ (mean − 5.40 ± 0.38‰). The precipitation amount at each site was negatively correlated with δ18O (−0.24 to −3.20‰ per 100 mm, R2 = 0.1–0.9). Furthermore, δ18O was negatively correlated with geography (latitude, altitude) for the southwest monsoon periods, as expected based on other observed correlations. However, an inverse correlation was seen in the northeast monsoon due to differing moisture transportation as part of the continental effect. The correlation coefficient (R) was higher in the southwest monsoon (−0.84 for latitude effect, −0.64 for altitude effect) than the northeast monsoon (0.67 for latitude effect, 0.35 for altitude effect). The spatial pattern of isotopic composition reflects the southwest monsoon more clearly than the northeast monsoon, but the two monsoons also have a cancelling impact on orographic patterns. An agreement of the δ18O and deuterium excess (d-excess) was a negative correlation and found to reflect precipitation sources and re-evaporation processes. The d-excess was slightly higher for the northeast monsoon, bringing moisture from the Pacific Ocean and travelling across the continent before reaching the observed stations. By contrast, the d-excess was relatively lower for the Indian Ocean's moisture in the southwest monsoon.  相似文献   

19.
Utilising datasets from the Global Network of Isotopes in Precipitation of the International Atomic Energy Agency, and previous isotopic studies, we investigated δ18O spatial and temporal patterns in Chinese precipitation. Significantly positive relationships existed between precipitation δ18O and air temperature above the north of 35°N and in high altitude regions above 32°N. Significantly negative relationships between precipitation δ18O and the precipitation amount existed below south of 35°N. These temperature and precipitation effects became stronger with increasing altitude except in high altitude regions between 32°N and 35°N. The NCEP/NCAR reanalysis data from 1980 to 2004 showed that variations in spatial and seasonal wind fields at 700 hpa and total precipitable water from the ground to the top of the atmosphere were correlated with the monthly spatial distribution of precipitation δ18O. Basing on this relationship, we established quantitative correlations between the mean monthly precipitation δ18O and both latitude and temperature in different seasons. We found that spatial variations in precipitation δ18O could be described well using the Bowen–Wilkinson model and second‐order equations developed during the present study only in winter (from December to February). During the rest of the year, patterns were too complex to predict using simple models. The results suggest that it is difficult to demonstrate variations of precipitation δ18O throughout the year and for all regions of China using a single model. Moreover, the new models for the relationships among precipitation, latitude, and temperature were better able to depict the variations in precipitation δ18O than the Bowen–Wilkinson model. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

20.
Deuterium and oxygen‐18 are common environmental tracers in water used to investigate hydrological processes such as evaporation and groundwater recharge, and to trace moisture source. In this study, we collected event precipitation from 01 January 2010 to 28 February 2011 at a site in Changsha, Yangtze River Basin to estimate the influence of moisture source and atmospheric conditions on stable isotope compositions. The local meteoric water line, established as δD = (8.45 ± 0.13) δ18O + (17.7 ± 0.9) (r2 = 0.97, n = 189), had a higher slope and intercept than global meteoric water line. Temperature–δ18O exhibited complex correlations, with positive correlations during Nov.–Apr. superior to during Jun.–Sep., which was attributed to distinctive moisture sources, but vague the overall period; amount effect examined throughout the year. Linear regressions between δ18O and δD value in different precipitation event size classes revealed progressively decreasing slope and intercept values with decreasing precipitation amount and increasing vapour pressure deficit, indicating that small rainfall events (0–5 mm) were subject to secondary evaporation effects during rainwater descent. In contrast, snowfall and heavy precipitation events exhibited high slope and intercepts for the regression equation between δ18O and δD. High concentrations of heavy isotopes were associated with precipitation events sourced from remote westerly air masses, degenerated tropical marine air masses from the Bay of Bengal (BoB), and inland moisture in the pre‐monsoon period, as determined from backward trajectories assessed in the HYSPLIT model. Meanwhile, low concentrations of heavy isotopes were found to correspond with remote maritime moisture from BoB, the South China Sea, and the west Pacific at three different air pressures in summer monsoon and post‐monsoon using HYSPLIT and records of typhoon paths. These findings suggest that stable isotope compositions in precipitation events are closely associated with the meteorological conditions and respond sensitively to moisture source in subtropical monsoon climates. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

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