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1.
The deposition record of 137Cs was traced in the SE Black Sea sediments adjacent to the Coruh river mouth in comparison with the earlier studied chronology of 137Cs deposition in front of the Danube delta (NW Black Sea). In both cases, the 137Cs profiles showed two subsurface peaks attributable to maximum fallout of ‘bomb’ and Chernobyl radionuclides. The Coruh profile revealed a larger contribution of ‘bomb’ 137Cs in comparison with the Chernobyl input, suggesting different coverage of NW and SE Black Sea regions with the Chernobyl fallout. The 137Cs-derived dating showed that maximum deposition of particulate bound 137Cs in sediments adjacent to the Coruh river mouth was delayed for 14 yr relative to date of Chernobyl accident, reflecting a buffer effect of the watershed soils. This transit time is 3 times longer than in the Danube catchment area, indicating a difference in retention processes in these mountainous (Coruh) and lowland (Danube) river basins. The 137Cs profile in Coruh sediments showed penetration of 137Cs to much greater depth than would be expected from 137Cs fallout chronology, suggesting the sediment mixing rate of 1.3 cm2 yr−1. This value was used to evaluate deposition chronology of 137Cs, applying the model developed for pulse fallout case. Comparing the measured and modelled data has allowed differentiation of the flood-induced discharge of the 137Cs-containing suspended matter and the slower transit of eroded soil particles from the contaminated catchment areas. The obtained results may be used for the prediction of period when the pollutants, deposited over the river basins, can reach the Black Sea.  相似文献   

2.
The Kara Sea is one of the arctic marginal seas strongly influenced by fresh water and river suspension. The highly seasonal discharge by the two major rivers Yenisei and Ob induces seasonal changes in hydrography, sea surface temperature, ice cover, primary production and sedimentation. In order to obtain a seasonal pattern of sedimentation in the Kara Sea, sediment traps were deployed near the river mouth of the Yenisei (Yen) as well as in the central Kara Sea (Kara) within the framework of the German–Russian project “Siberian River run-off; SIRRO”. Two and a half years of time-series flux data were obtained between September 2000 and April 2003 and were analyzed for bulk components, amino acids, stable carbon and nitrogen isotopes as well as sterols and fatty acids.Sediment trap data show that much of the annual deposition occurred under ice cover, possibly enhanced by zooplanktonic activity and sediment resuspension. An early bloom of ice-associated algae in April/May occurred in the polynya area and may have been very important to sustain the life cycles of higher organisms after the light limitation of the winter months due to no/low insolation and ice cover. The strong river input dominated the months June–August in the southern part of the Kara Sea. The central Kara Sea had a much shorter productive period starting in August and was less affected by the river plumes. Despite different time-scales of sampling and trapping biases, total annual fluxes from traps were in the same order of magnitude as accumulation rates in surface sediments. Terrestrial organic carbon accumulation decreased from 10.7 to 0.3 g C m−2 a−1 from the riverine source to the central Kara Sea. Parallel to this, preservation of marine organic matter decreased from 10% to 2% of primary productivity which was probably related to decreasing rates of sedimentation.  相似文献   

3.
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4.
High-resolution stable oxygen isotope (δ18O on ostracod shells), XRF-scanning and bulk grain-size data obtained on a transect of 6 gravity cores from the continental slope in the northwestern Black Sea give new insight into the hydrological evolution of the Black Sea since the Last Glacial Maximum (LGM). Stable climatic conditions during the LGM were followed by a series of meltwater pulses between 18 and 15.5 kyr BP that resulted in temporary isotopic depletion of the Black Sea waters. Subsequently, steadily increasing δ18O values in all cores are mainly caused by isotopically enriched precipitation at the onset of the Allerød/Bølling warm period. A comparison of the major trends in δ18O at different water depths suggests evaporation-driven deep water formation since ∼14.5 kyr BP, while the two shallowest cores from 168 and 465 m water depth were under the influence of increased warming in the upper water column since 14.5 and 12.5 kyr BP, respectively. The core from 168 m depth seems to be additionally influenced by freshwater input of the Danube. This core provides a high-resolution record from the Younger Dryas/Allerød boundary and suggests that a NAO-like climate mode was governing the interannual variability in the run-off of the Danube, which implies that this climate mode has been a persistent climatic feature over central Europe. The inflow of saline Mediterranean waters occurs between 9 and 8 kyr BP, where a merging of all δ18O records signals an initial homogenisation of the water column.  相似文献   

5.
Elemental (carbon and nitrogen) ratios and stable carbon and nitrogen isotope ratios (δ13C and δ15N) are examined in sediments and suspended particulate matter from Hudson Bay to study the influence of river inputs and autochthonous production on organic matter distribution. River-derived particulate organic matter (POM) is heterogeneous, nitrogen-poor and isotopically depleted, consistent with expectations for OM derived from terrestrial C3 vascular plant sources, and distinct from marine OM sources. Both δ13C and C/N source signatures seem to be transmitted to sediments with little or no modification, therefore making good tracers for terrigenous OM in Hudson Bay. They suggest progressively larger contributions from marine sources with distance from shore and secondarily from south to north, which broadly corresponds to the distribution of river inputs to Hudson Bay. Processes other than mixing of marine and terrigenous OM influence sedimentary δ15N values, including variability in the δ15N of phytoplankton in the Bay's surface waters due to differences in relative nitrate utilization, and post-production processes, which bring about an apparently constant 15N-enrichment between surface waters and underlying sediments. Variability in the δ15N of phytoplankton in the Bay's surface waters, in contrast, seems to be organized spatially with a pattern that suggests an inshore–offshore difference in surface water nitrogen conditions (open- vs. closed-system) and hence the δ15N value of phytoplankton. The δ15N patterns, supported by a simple nitrate box-model budget, suggest that in inshore regions of Hudson Bay, upwelling of deep, nutrient-rich waters replenishes surface nitrate, resulting in ‘open system’ conditions which tend to maintain nitrate δ15N at low and constant values, and these values are reflected in the sinking detritus. River inflow, which is constrained to inshore regions of Hudson Bay, appears to be a relatively minor source of nitrate compared to upwelling of deep waters. However, river inflow may contribute indirectly to enhanced inshore nutrient supply by supporting large-scale estuarine circulation and consequently entrainment and upwelling of deep water in this area. In contrast to previous proposals that Hudson Bay is oligotrophic because it receives too much fresh water (Dunbar, 1993), our results support most of the primary production being organized around the margin of the Bay, where river flow is constrained.  相似文献   

6.
The influence of riverine inputs on biogeochemical cycling and organic matter recycling in sediments on the continental shelf off the Rhône River mouth (NW Mediterranean Sea) was investigated by measuring sediment oxygen uptake rates using a combination of in situ and laboratory techniques. Four stations were investigated during two cruises in June 2001 and June 2002, with depths ranging from 9 to 192 m and over a distance to the Rhône River mouth ranging from 4 to 36 km. Diffusive oxygen uptake (DOU) rates were determined using an in situ sediment microprofiler and total oxygen uptake (TOU) rates were measured using sediment core incubations. There was good agreement between these two techniques which indicates that the non-diffusive fraction of the oxygen flux was minimal at the investigated stations. DOU rates ranged from 3.7±0.4 mmol O2 m−2 d−1 at the continental shelf break to 19.3±0.5 mmol O2 m−2 d−1 in front of the Rhône River mouth. Sediment oxygen uptake rates mostly decreased with increasing depth and with distance from the Rhône mouth. The highest oxygen uptake rate was observed at 63 m on the Rhône prodelta, corresponding to intense remineralization of organic matter. This oxygen uptake rate was much larger than expected for the increasing bathymetry, which indicates that biogeochemical cycles and benthic deposition are largely influenced by the Rhône River inputs. This functioning was also supported by the detailed spatial distribution of total organic carbon (TOC), total nitrogen (TN) and C/N atomic ratio in surficial sediments. Sediments of the Rhône prodelta are enriched in organic carbon (2–2.2%) relative to the continental shelf sediments (<1%) and showed C/N ratios exceeding Redfield stoichiometry for fresh marine organic matter. A positive exponential correlation was found between DOU and TOC contents (r2=0.98, n=4). South-westward of the Rhône River mouth, sediments contained highly degraded organic matter of both terrestrial and marine origin, due to direct inputs from the Rhône River, sedimentation of marine organic matter and organic material redeposition after resuspension events.  相似文献   

7.
Geochemical analysis of surface sediment samples collected in 2005 and 2006 was used to evaluate the potential sources of the organic matter present in sediments of southeast Poland's Solina Reservoir.Statistical analysis of sediment variables(carbon to nitrogen ratio, and the carbon 13 and nitrogen 15 isotope ratios) determined for the organic fraction indicated significant spatial variability with respect to sources of organic matter. A binary mixing model was developed from literature sources to predict the relative contributions of allochthonous and autochthonous production to sediment organic matter.Autochthonous production was shown to account for 60-75% of bulk sedimentation in the lacustrine parts of the reservoir, near the dam. In contrast, autochthonous production accounted for only 25% of sedimentation in the riverine zone receiving stream inputs. Statistical analysis identified the δ~(15)N of organic matter as the best predictor of the source of organic matter. Multiple regression analysis indicated that two water-quality variables(nitrate and dissolved silica) were significantly related to the δ~(15)N signature of organic matter. This led to a conclusion that limnetic nitrate and dissolved silica concentrations were regulating organic matter production in the Solina Reservoir.  相似文献   

8.
Recently, black carbon has been introduced as the form of carbon that may be separated from the biologically mediated carbon cycle thereby representing the non-bioavailable fraction of the estimated organic carbon. It has been speculated that the bioavailability of organic matter may be a limiting factor for the presence of active bacteria within the sediments. In order to address this question, marine sediments were collected from the Thracian Sea (Eastern Mediterranean), a complex system impacted by riverine inputs and Black Sea water masses. In addition to counts of total bacteria, we estimated the fraction of active bacteria by using a destaining step to the DAPI staining method. Black carbon was also estimated following the thermal oxidation method in order to determine the fraction of the refractory organic matter. The fraction of black carbon to total organic carbon varied from 16% to 53% indicating that black carbon constitutes a significant pool of sedimentary organic carbon in the Thracian sea. A fraction ranging from 18% to 97% was scored as nucleoid containing cells. We did not record any significant differences in the fraction of nucleoid-containing bacteria among sediment depths (P<0.05) indicating that there was no accumulation of dead bacterial cells with depth. The same was observed for the fraction of black carbon and bioavailable organic carbon with sediment depth (P<0.05) indicating that benthic consumers are not the key regulators of the organic matter pool in these sediments but have a minor effect. A possible reason for these observations and for the uncoupling between the active bacterial fraction and the bioavailability of organic matter could be (i) the presence of refractory components in the estimated bioavailable organic matter and (ii) the hydrological and geological complexity of the study area. The North Aegean marginal slopes are highly unstable experiencing frequent seismic events. These events are capable of inducing sediment transport from the upper slopes thus altering the entire sediment profile. On the other hand, the significant correlations that were recorded between nucleoid-containing cells and phytopigments (chlorophyll a, phaeopigments, chloroplastic pigment equivalents) at all sediment depths indicate that bacterial communities respond immediately to the deposited phytodetritus, using it as a primary source of carbon and energy. Our data suggests that the Thracian Sea sediments are by no means homogeneous and can best be described as a mosaic controlled by numerous local and regional environmental factors.  相似文献   

9.
The transformation of dissolved inorganic nitrogen (DIN) and soluble reactive phosphorous (SRP), and the release of dissolved organic and particulate N and P, were analyzed in two lake complexes (Uzlina–Isac and Puiu–Rosu–Rosulet) of the Danube Delta wetland during flood conditions in May and at low water level in September 2006. The Uzlina–Isac complex was hydrologically tightly-connected with the Danube River and was flushed with river-borne nutrients and organic matter. These lakes acted as effective transformers for nutrients and produced large amounts of fresh biomass, that promoted the excretion of dissolved organic N and P during active growth. Biomass breakdown created particulate matter (<0.45 μm), which was widely liberated during low flow in the fall. The Puiu–Rosu–Rosulet complex was characterized by a more distant position to the Danube and proximity to the Black Sea, and received dominantly transformed organic compounds from the flow-through water and vast vegetation cover. Due to reduced nutrient input, the internal production of organic biomass also was reduced in these more remote lakes. Total N and P export from the lake nearest to the shelf was governed by dominantly dissolved organic and particulate compounds (mean 58 and 82%, respectively). Overall, this survey found that these highly productive wetlands efficiently transform nutrients into a large pool of dissolved organic and particulate N and P. Hence, wetland lakes may behave widely as net sources of organic N and P to downstream waters and coastal marine systems.  相似文献   

10.
The Yellow River (YR) supplies a large amount of nutrients and fresh water to the northern Chinese marginal seas, and greatly influences the ecosystem and current patterns. The relocation of the YR outlet from the southern Yellow Sea (YS) to the Bohai Sea in 1855 was demonstrated using northern East China Sea (ECS) sediment characteristics. Both isotopic (δ13C, δ15N) signals and C/N ratios in the organic matter (OM) indicate that prior to 1750, the predominant source of OM to the sediments was terrestrial. The terrestrial influences continuously weakened until 1855, when the YR estuary moved; after 1855, the OM was characterized by oceanic sources. Major elements (Al, Ti, Fe, Mn) and trace elements (Ni, Cr, Cu, Pb) had a much closer association with Malan loess prior to 1855, as >90% of the YR sediment was loess-derived. These results reveal that the relocation of the YR induced significant changes in the current patterns of the northern China Seas in the last 250 years; however, more studies are needed to further examine these linkages.  相似文献   

11.
The molecular distribution and compound specific stable carbon and hydrogen isotope ratios were measured on solvent extractable hydrocarbons from the Late Paleoproterozoic McArthur River, or “Here's Your Chance” (HYC) Pb/Zn/Ag ore deposit in the Northern Territory of Australia. Five samples were collected from the McArthur River mine on a northeast–southwest transect in order to sample a gradient of hydrothermal alteration. One sample was taken from the unmineralized W-Fold Shale unit immediately below the HYC ore deposit. δD of n-alkanes, branched alkanes and bulk aromatic fractions were measured, and δ13C of n-alkanes, polynuclear aromatic hydrocarbons (PAHs) and bulk kerogen were measured to assess the isotopic effects of a varying degree of hydrothermal alteration on different components of HYC organic matter (OM). Relative to n-alkanes in Barney Creek Formation sediments that did not undergo mineralization, HYC n-alkanes are enriched in deuterium (D) by 50–60‰. This is likely to be a result of equilibrium hydrogen exchange during ore genesis with a highly D-enriched fluid that originated in an evaporitic basin. Trends with distance along the sample transect are ambiguous, but from the northernmost to southernmost point, n-alkanes are less D-enriched, and PAHs are less abundant and less 13C-enriched. This could be due to decreasing hydrothermal alteration effects, decreasing delivery of highly altered OM by the mineralizing fluid, or both. The carbon isotopic composition of HYC PAHs is inconsistent with a Barney Creek Fm source, but consistent with an origin in the underlying Wollogorang Formation. PAHs are 13C-depleted relative to n-alkanes, reflecting a kerogen source that was 13C-depleted compared to n-alkanes, typical for Precambrian sediments. PAHs are more 13C-depleted with increasing molecular weight and aromaticity, strengthening the case for a negative isotopic effect associated with aromatization in ancient sediments. Together, these data are consistent with a an ore deposition model in which fluids originated in an evaporitic deposit lower in the basin and interacted with metals and OM in the Tawallah Group at temperatures above 250 °C and a depth of ~ 6 km before ascending along a flower structure associated with the Emu Fault and cooling to 200 ± 20 °C before reaching Barney Creek sediments.  相似文献   

12.
High resolution OSL dating back to MIS 5e in the central Sea of Okhotsk   总被引：1，自引：0，他引：1  
Marine sediments contain important archives of past ocean and climate changes, but at high latitudes the absence of carbonate has prevented the construction of accurate chronological models. We have begun a study to (1) determine the accuracy of luminescence ages in deep-sea marine sediments, e.g. by comparison with marine oxygen isotope stratigraphy where possible, (2) describe changes in sedimentation rate through time, and (3) test whether it is possible to date back to marine isotope stage 5e (MIS 5e). We show here that optical dating of fine grains of quartz from the central Sea of Okhotsk is able to provide an accurate and precise chronology for the reconstruction of the palaeoceanic and palaeoclimatic environment at our site. The upper 6.5 m of the 18.42 m long core MR0604-PC07A is believed, based on its magnetic susceptibility and the oxygen isotope (δ18O) records to contain the last ～150 ka. Forty OSL samples were taken from this upper part of the core. The single-aliquot regenerative-dose (SAR) procedure is used for equivalent dose (De) determination. The luminescence characteristics of fine-grained quartz (4–11 μm) extracted from the core are described. The OSL signal is dominated by the fast component and a dose recovery test shows that we can accurately measure a known dose given in the laboratory prior to any heat treatment. Dose rates were determined using high-resolution gamma spectrometry, and vary between 0.4 and 1.6 Gy/ka. The OSL ages from this section lie between ～140 ka and ～15 ka and are in very good agreement with the δ18O stratigraphy up to MIS 5e. A clear change in sedimentation rate is identified: between ～139 and 110 ka, the sedimentation rate was ～0.09 m/ka, but then from ～110 to 15 ka, the sedimentation rate decreases to a constant value of ～0.04 m/ka. Our data confirm that OSL dating using widely distributed fine-grain quartz has great potential for dating deep-sea sediments. Because luminescence methods use clastic materials, they do not depend on the presence of biogenic carbonate. As a result it is now likely that we can establish a chronology in regions of the ocean that were previously undatable.  相似文献   

13.
Accumulation rates of marine and terrigenous organic carbon in the continental margin sediments off southwestern Taiwan were estimated from the measured concentrations and isotopic compositions of total organic carbon (TOC) and previously reported sedimentation rates. Surficial sediments were collected from the study area spanning from the narrow shelf near the Kaoping River mouth to the deep slope with depths reaching almost 3000 m. The average sediment loading of Kaoping River is 17 Mt/yr, which yields high sediment accumulation rates ranging from 0.08 to 1.44 g cm−2 yr−1 in the continental margin. About half of the discharged sediments were deposited on the margin within 120 km of the river mouth. Carbon isotopic compositions of terrestrial and marine end-members of organic matter were determined, respectively, based on suspended particulate matter (SPM) collected from three major rivers in the southwestern Taiwan and from an offshore station. All samples were analyzed for the TOC content and its isotopic composition (δ13Corg). The SPM samples were also analyzed for the total nitrogen (TN) content. TOC content in marine sediments ranges from 0.45% to 1.35% with the highest values on the upper slope near the Kaoping River mouth. The TOC/TN ratio of the SPM samples from the offshore station is 6.8±0.6, almost identical to the Redfield ratio, indicating their predominantly marine origin; their δ13Corg values are also typically marine with a mean of −21.5±0.3‰. The riverine SPM samples exhibit typical terrestrial δ13Corg values around −25‰. The δ13Corg values of surficial sediments range from −24.8‰ to −21.2‰, showing a distribution pattern influenced by inputs from the Kaoping River. The relative contributions from marine and terrestrial sources to sedimentary organic carbon were determined by the isotope mixing model with end-member compositions derived from the riverine and marine SPM. High fluvial sediment inputs lead to efficient trapping of organic carbon over a wide range of water depth in this continental margin. The marine organic accumulation rate ranges from 1.6 to 70 g C m−2 yr−1 with an area weighted mean of 4.2 g C m−2 yr−1, which is on a par with the mean terrestrial contribution and accounts for 2.3% of mean primary production. The depth-dependent accumulation rate of marine organic carbon can be simulated with a function involving primary productivity and mineral accumulation rate, which may be applicable to other continental margins with high sedimentation rates. Away from the nearshore area, the content of terrigenous organic carbon in surficial sediments decreases with distance from the river mouth, indicating its degradation in marine environments.  相似文献   

14.
The main aim of this study was to estimate the influence of the seasonal variations of the Danube River particulate organic matter (POM) inputs on the Black Sea surface seawater POM and upper layer of sediments along the Romanian coast. Ratios of carbon ((13)C/(12)C) and nitrogen ((15)N/(14)N) stable isotopes allowed differentiating river and marine organic matter sources. Danube River POM presented significantly lower average values of delta(13)C (-27.52+/-0.88 per thousand) and delta(15)N (4.88+/-1.45 per thousand) than seawater POM (delta(13)C=-24.70+/-2.37 per thousand and delta(15)N=6.75+/-1.96 per thousand), whereas surface sediment presented average values similar to seawater POM (delta(13)C=-24.02+/-2.39 per thousand and delta(15)N=7.29+/-2.16 per thousand). Stable isotope values showed that the Danube River influence on marine ecosystems decreased from the North to the South of the Romanian coast. Strong seasonal variations of C and N isotopic signatures were observed in all compartments studied with generally higher values in spring when the river was flooding.  相似文献   

15.
Liu X  Xu L  Sun L  Liu F  Wang Y  Yan H  Liu Y  Luo Y  Huang J 《Marine pollution bulletin》2011,62(10):2205-2212
We reconstructed the first long-term (∼400 years) records of black carbon (BC) deposition flux from three ornithogenic sediment profiles, which were collected from three remote, isolated islets of the Xisha archipelago, South China Sea. The significant correlations between black carbon, organic matter and excess 210Pb suggested that black carbon was mainly derived from atmospheric deposition, and further enriched by plant-derived organic matter in sediments. During the past 400 years, the BC flux remained relatively low before the onset of 20th century; it started to increase from approximately 1900 AD, and peaked around the 1970s. In the recent 30 years, the BC flux seemed to display decreasing trend, very likely due to the change of energy structure and development of pollution control techniques. In comparison with marginal sea regions that are greatly impacted by anthropogenic activities, these pristine Xisha islands were not significantly influenced by black carbon of anthropogenic origin.  相似文献   

16.
The fundamental assumption of 210Pb sediment dating is the stable flux of 210Pbex, which was derived from atmosphere and then transferred into sediments via lake water. When the sedimentation rate is relatively constant, the 210Pbex activity in sediments will be exponentially reduced with sedimentation age. 210Pbex in lake water is incorporated into sediments mainly via organic particulates. If the sedimentation flux of organic matter in lake water is suddenly increased, 210Pbex will be significantly deposited and then transferred into sediments. On the one hand such sudden purification effect is obviously unfit for the fundamental assumption of 210Pb dating; on the other hand, the sudden enhancement of 210Pbex flux would be indicative of the conspicuous variation of primary productivity of lake water. This problem will be discussed in accordance with the variation trend of 210Pbex in the vertical profile of recent sediments of Lake Chenghai, Yunnan Province. The sediment core was collected from the deep-water area of Lake Chenghai in June 1997. The vertical profile of 137Cs activity is characterized by a tree-peak pattern. This profile gave reliable ages, and also showed the stability of sediment accumulation in the recent ten years. The vertical profile of 210Pbex activity displays a specific distribution of peaks, and is similar to the vertical profile of Corg. This phenomenon seems to be related to the mechanism of constraining the transfer of 210Pbex into lake sediments. The average atomic ratios of Horg/Corg and Corg/Norg in Lake Chenghai sediments are 5.51 and 7.04, respectively, indicating that the organic matter was predominantly derived from the remains of endogenic algae. In terms of the three-stage evolutionary characteristics of organic matter in sediments, i.e., “deposition-de-composition-accumulation”, the sedimentation fluxes (F(Corg)) of organic carbon (Corg) since 1970 were calculated by modeling. The sedimentation fluxes of 210Pbex (F(210Pbex)) in different years display good synchronous relations with the sedimentation flux of organic carbon (F(Corg)), especially in the years of 1972–1974 and 1986–1989. The variation of F(Corg) led to the variation of F(210Pbex); the variation of F(210Pbex) reflects, to some extent, the historical variation of lake productivity.  相似文献   

17.
《Continental Shelf Research》2006,26(17-18):2260-2280
On October 3, 2002 Hurricane Lili made landfall on a previously studied region of the inner Louisiana shelf as a Category 2 storm with winds over 160 km/h. A week after the hurricane, major impacts of the storm were not evident in the water column except for the lower than expected inshore salinities (∼12 psu) for this time of year, which was characterized by low river discharge. Turbidity profiles were typical of those measured during previous investigations with suspended sediment concentrations >75 mg/L at inshore stations and <50 mg/L in surface waters and offshore. The implication is that the sediments resuspended during the hurricane settled soon after the storm passage. Water column particulate organic carbon (POC) concentrations ranged from 0.1 to over 2.0 mg/L, with the highest concentrations measured near the seabed and in the inshore portions of the study area. Suspended particles were characterized by low organic matter content (%POC of 0.5–2 wt%), low chlorophyll:POC ratios (Chl:POC<4 mg/g) and moderately elevated POC:particulate nitrogen ratios (POC:PN of 10–14 mol/mol), all suggesting their source was locally resuspended seabed sediment rather than from algal biomass or land-derived vascular plant detritus.Post hurricane sediment deposition throughout the study area resulted in a storm layer that ranged from <0.5 to 20 cm in thickness. In most locations sediment accumulation ranged from 3 to 10 cm. The storm deposits were generally composed of silty clays with a coarser, somewhat sandy 1–2 cm basal layer. Surface sediments from the storm layer were characterized by relatively high mineral surface areas (SA of 30–50 m2/g) and elevated OC contents (%OC of 1.0–2.0%). The dispersal of fine sediments following the hurricane resulted in marked changes in the SA and %OC values of surface sediments from offshore locations, which prior to the storm contained coarser, organic-poor particles (SA of 5–15 m2/g and %OC of 0.2–0.6%). The OC:SA and OC:N ratios of storm layer sediments ranged from 0.4 to 0.6 mg OC/m2 and from 10 to 12 mol/mol, respectively, and were comparable to those measured in surface sediments prior to the hurricane. Such similarities in the composition of the organic matter reinforce the idea that the source of the storm deposits was the finer fraction of resuspended seabed sediments, with little evidence for inputs from local land-derived sources or autochthonous algal production. Overall, the magnitude of sediment and organic matter deposition on the seabed after the storm greatly exceeded the annual inputs from the Atchafalaya River and coastal primary production. The combined effects of hurricane-driven erosion and post-storm deposition represent a major perturbation to the benthic community of the region, which is already subject to these types of disturbances due to the combined effects of peaks in river discharge and the passage of storm fronts.  相似文献   

18.
以巢湖湖底有机碎屑为研究对象,基于对有机碎屑中总有机碳的测定,研究了利用好氧强化降解湖底有机碎屑.研究了有机碎屑的可生化性及好氧强化降解湖底有机碎屑的效果,并讨论了有机碎屑的浓度及曝气量对其降解效果的影响.结果说明,处理的有机碎屑具有较好的可生化性,在反应30 h左右,降解达到了平衡,总去除率达到了50.69%,降解速率常数K25为0.19 h-1.有机碎屑的浓度以及曝气量对降解效果具有一定的影响.强化好氧法与传统的对底泥处理的方法相比具有更快、更好的效果,为预防及治理水体黑臭现象提供了新的途径.  相似文献   

19.
To investigate the sources of particulate organic matter (POM) and the impact of Three Gorges Dam (TGD), two large lakes and erosion processes on determining the composition and flux of POM in low water discharge periods along the middle and lower Changjiang, suspended particulate samples were collected along the middle and lower reaches of the Changjiang (Yangtze River) in January 2008. Organic geochemistry of bulk sediment (particulate organic carbon, organic carbon to nitrogen molar ratio (C/N), stable carbon isotope (δ13C) and grain size) and biomarker of bulk sediment (lignin phenols) were measured to trace the sources of POM. The range of C/N ratios (6.4–8.9), δ13C (?24.3‰ – ?26.2‰) and lignin phenols concentration Λ8 (0.45 mg/100 mg OC‐2.00 mg/100 mg OC) of POM suggested that POM originated from the mixture of soil, plant tissue and autochthonous organic matter (OM) during the dry season. POM from lakes contained a higher portion of terrestrial OM than the mainstream, which was related to sand mining and hydropower erosion processes. A three end‐member model based on δ13C and Λ8 was performed. The results indicated that soil contributed approximately 50% of OM to the POM, which is the dominant OM source in most stations. POM composition was affected by total suspended matter (TSM) and grain size composition, and the direct OM input from two lakes and channel erosion induced OM. The lower TSM concentration in January 2008 was mainly caused by seasonal variations; the impact from the TGD in the dry season was relatively small. A box model indicated that more than 90% of the terrestrial OM transported by the Changjiang in January 2008 was from the middle and lower drainage basins. Channel erosion induced OM, and contributions from Poyang Lake were the major terrestrial OM sources in the dry season. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

20.
Total organic carbon (TOC) and biogenic silica (opal) content, elemental (C/N) and isotopic (δ13C, δ15N) composition of organic matter and the content of lipid biomarkers derived from both marine and terrestrial sources constrain relative contributions from marine productivity and continental erosion to surface sediments throughout coastal SE Alaska (54°N to 61°N). TOC and opal content are very high (up to 8% and 33% by weight, respectively) in fjords and inlets south of Icy Strait (∼58°N) and uniformly low at offshore sites to the south, and at both offshore and inland sites to the north (averaging 0.6±0.3% and 2.3±1.8%, respectively). TOC and opal mass accumulation rates (MARs, based on bulk density and 210Pb-derived sediment MAR) suggest dilution with terrigenous, inorganic detrital materials accounts for the low concentrations of both biogenic phases in sediments from the glacial tidewater fjords of Muir and Yakutat Bays but not elsewhere. C/N, δ13C, and δ15N indicate a dominant marine origin for organic matter deposited at most sites. This conclusion implicates elevated primary productivity in inland waters to the south with diatoms, based on opal results, being the dominant contributor. A very significant terrestrial organic fraction (25–50%) is contained in sediments deposited on the continental shelf to the north of 58°N. Hydrocarbon biomarkers indicate the terrestrial fraction in sediments from this region is represented by old organic matter (kerogen) likely contained within riverborne particles eroding from now heavily glaciated adjacent landscapes. In sediment to the south, the terrestrial fraction is traced to modern soil organic matter eroded from the now non-glaciated, heavily forested adjacent landscape. Our study provides a framework to guide future investigations of short- (anthropogenic) to long- (Holocene) term environmental and/or climate change in this region through down-core, stratigraphic analysis.  相似文献   

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