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1.
Lake Bonney, a permanently ice-covered Antarctic lake, has a middepth maximum N2O concentration of 41.6 micromoles N (>580,000% saturation with respect to the global average mixing ratio of N2O) in its east lobe, representing the highest level yet reported for a natural aquatic system. Atmospheric N2O over the lake was 45% above the global average, indicating that this lake is an atmospheric source of N2O. Apparent N2O production (ANP) was correlated with apparent oxygen utilization (AOU), and denitrification was not detectable, implying that nitrification is the primary source for this gas. The slope of a regression of ANP on AOU revealed that potential N2O production per unit of potential O2 consumed in the east lobe of Lake Bonney is at least two orders of magnitude greater than reported for the ocean. The maximum yield ratio for N2O [ANP/(NO2(-) + NO3-)] in Lake Bonney is 26% (i.e. 1 atom of N appears in N2O for every 3.9 atoms appearing in oxidized N), which exceeds previous reports for pelagic systems, being similar to values from reduced sediments. Areal N2O flux from the lake to the atmosphere is >200 times the areal flux reported for oceanic systems; most of this gas apparently enters the atmosphere through a small moat that occupies approximately 3% of the surface of the lake and exists for approximately 10 weeks in summer.  相似文献   

2.
Nitrogen (N) lost from farms, especially as the highly bioavailable dissolved inorganic form, may be damaging Australia's Great Barrier Reef (GBR). As sugarcane is the dominant cropping system in GBR catchments, its N management practises are coming under increasing scrutiny. This study measured dissolved inorganic N lost in surface runoff water and sugarcane productivity over 3 years. The experiment compared the conventional fertiliser N application rate to sugarcane (average 180kg N/ha/year) and a rate based on replacing N exported in the previous crop (average 94kg N/ha/year). Dissolved inorganic N losses in surface water were 72%, 48% and 66% lower in the three monitored years in the reduced N fertiliser treatment. There was no significant difference in sugarcane yield between the two fertiliser N treatments, nor any treatment difference in soil mineral N - both of these results are indicators of the sustainability of the lower fertiliser N applications.  相似文献   

3.
This study presents input–output budgets of total dissolved nitrogen (TDN), dissolved organic N (DON) and dissolved inorganic N (DIN) for a reservoir in a peatland catchment in the south Pennines (UK). This site receives high levels of atmospheric inorganic N deposition, in the range of 26 kg N ha?1 yr?1. The results show that the reservoir retains ~21 to 31% of the annual TDN input (8806 ± 741 kg N). Approximately 39 to 55% of DON (3782 ± 653 kg N) and 6 to 13% of DIN (5024 ± 349 kg N) were retained/processed. A long water retention time (104 days), average annual pH of 6.5, high concentrations of DIN in the reservoir water and a deep water column suggest that denitrification is potentially a key mechanism of N retention/removal. The results also demonstrate that DON is potentially photodegraded and utilized within the reservoir, particularly during the summer season when 58 to 80% of DON input (682 ± 241 kg N) was retained, and a net export of DIN (~34 kg N) was observed. The findings therefore suggest that DON may play a more crucial role in the biogeochemistry of peat‐dominated acid sensitive upland freshwater systems than previously thought. Reservoirs, impoundments and large lakes in peatland catchments may be important sites in mediating downstream N transport and speciation. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

4.
Studies worldwide have indicated that agricultural pollution is the main source of nitrogen and phosphorus (N and P) in surface waters. A systematic understanding of N and P sources and sinks in agricultural systems is important for selecting the appropriate remedial strategies to control nutrient losses and water pollution. Based on nationwide data and a long-term monitoring program in Southeast China, the nationwide spatial and temporal patterns of N and P losses and the relationships between such losses and N and P inputs and rainfall were analyzed. The results showed that the annual nutrient losses from agricultural systems in China strongly varied, and the N/P values ranged from 0.01 to 51.0, with a majority at approximately 0–20, and an arithmetic mean of 9.73; these values mostly overlap the suitable range of N/P (6–15) for red bloom algae.  相似文献   

5.
Nonpoint sources of nitrogen (N) and other nutrients are a major source of water pollution within the Chesapeake Bay watershed and other basins around the world. Human activities associated with agricultural practices can account for a large percentage of N loadings delivered to streams and rivers. This work aims to improve understanding of N transport from groundwater to surface waters, quantifying the principal hydrological processes driving water and N fluxes into and out of a headwater agricultural stream reach. The study site is a 175-m stream reach in a heavily cultivated 40-ha watershed in east-central Pennsylvania. This subwatershed is underlain by fractured shale bedrock, and receives most of its baseflow from groundwater, either by diffuse matrix discharge through the streambed or by localized discharge through riparian seeps. Samples of stream, seep, and shallow groundwater were collected approximately monthly under steady hydrologic conditions in 2017. Calculated matrix flow from hydraulic head and conductivity measurements paired with differential stream gauging was used to solve for the riparian seep flux using a mass balance approach. Riparian seep fluxes ranged from 45 to 217 m3/d, transporting 0.6–4.2 kg N d−1 of nitrate-N from the fractured bedrock aquifer to the stream. Hydrochemical data suggest that the stream is mainly disconnected from the underlying aquifer and that seeps supply essentially all water and N to the system. Seeps are likely sourced with N in nearby agricultural fields and accelerated through the system with shorter residence times than shallow groundwater. Water isotope data reinforced this notion. This study underscores the importance of agriculture as a source of N to ground and surface waters. Identifying source areas that are causing groundwater enrichment of N and seep areas where N discharges to streams is beneficial for developing N pollution mitigation strategies and implementing management practices that aim to reduce nutrient loads to the Chesapeake Bay.  相似文献   

6.
A study was made of the water chemistry, tissue nutrients and surface phosphatase activities of the 2-cm apices of three mosses in four upland streams in northern England, UK. This was part of a project to optimize methods for assessing nutrient fractions in environments with highly variable water chemistry. Aqueous N and P fractions showed the greatest variability followed by moss phosphatase activities, with nutrient composition of the shoot apices the least variable. There was no consistent pattern as to which aqueous N or P fraction was the most variable. The ratio between total inorganic N and total filtrable P ranged over three orders of magnitude in some streams. The interrelations between tissue N and P concentrations, tissue N:P ratio, phosphatase activities and aqueous variables showed:

(1) Significant +ve relationship between tissue N and aqueous NO3–N in some populations, but not between tissue P and aqueous P concentration;

(2) Significant +ve relationships between phosphatase activities and aqueous organic N, but none with aqueous organic P;

(3) Significant +ve relationships between phosphodiesterase:phosphomonoesterase activities and aqueous organic N;

(4) Significant −ve relationships between phosphatase activities and tissue P concentration;

(5) Significant +ve relationships between phosphatase activities and tissue N:P.

Both types of biological measurement are valuable for monitoring ambient nutrients in upland streams. Neither is clearly better than the other, so both should be included in surveys.  相似文献   


7.
The process of urbanization aggravates the endogenous pollution of urban lake sediment,and polluted sediment may seriously affect the quality of the water in lakes.At present,it is difficult to distinguish the difference between sediment that is heavily polluted by nitrogen(N)and phosphorus(P)when using an analysis based on a physicochemical index classification.The current study applied phospholipid fatty acid(PLFA)technology to further analyze the sediment characteristics from the perspective of microbiology.Surface sediment from five urban lakes that are heavily polluted with N and P in Wuhan were sampled.Statistical approaches were used to analyze the microbial community structure in the sampled sediment,and to determine the correlations between the microorganisms and physicochemical indices.The most severely polluted lake sediment had similar PLFA structures,the highest saturated fatty-acid content,and bacteria as the dominant microorganism.However,there were differences between the microbial biomass of the various sediment samples,which may have been related to the degree of N and P pollution.Analysis of the microbial diversity in the sediment samples indicated that the bacteria were experiencing starvation and nutrient pressure,which may have been due to the dissolved oxygen concentration of the heavily polluted lake sediment.A correlation analysis showed that the endogenous N and P had different effects on the microbes of the polluted sediment.A redundancy analysis(RDA)demonstrated that the N/P ratio had the greatest influence on the PLFA species,accounting for 83%of the cumulative interpretation.To effectively promote the role of sediment microorganisms on circulating elements,it is necessary to regulate the N/P ratio of the sediment to some extent.When the N/P ratio in sediment exceeds 6,N pollution should be prioritized.  相似文献   

8.
Nitrogen (N) fertilization may profoundly affect soil microbial communities. In this study, a field fertilization experiment was conducted in temperate grassland in Inner Mongolia, China to examine the effect of N fertilization on soil microbial properties and the main factors related to the characteristics of soil microbial community. Soil microbial biomass carbon (MBC) and microbial functional diversity along an N gradient were measured over three months (June to August). The result showed that N fertilization significantly decreased MBC under high N treatment (N200, 200 kg N ha?1 y?1) compared with the control (N0, 0 kg N ha?1 y?1) in the three months. Microbial functional diversity in July and August were significantly increased by low N treatment (N50, 50 kg N ha?1 y?1). Among the three fertilization treatments, microbial functional diversity under N200 in the three months was significantly lower than that of N50. The decrease of MBC and functional diversity under N200 were mainly due to the significant decline of plant belowground biomass under high N treatment. The increase of functional diversity under N50 treatment was due to the higher plant aboveground biomass as a result of the higher soil moisture availability. This finding highlighted that the higher N fertilization (N200) was not suitable for the growth and improvement of functional diversity of the soil microbial community, and that site and plant community play an important role in regulating the characteristics of soil microbial community.  相似文献   

9.
More than 1000 feet of fine-textured, unsaturated zone core beneath nitrogen-fertilized and irrigated farmland was collected, leached and analyzed for nitrate-nitrogen. Fertility plots treated with 200, 300, and 400 Ibs N/acre/yr accumulated significant quantities of nitrate-nitrogen in the vadose zone below the crop rooting zone. The average nitrate-nitrogen concentration approximately doubled with each 100 lbs N/acre/yr increment above the 100 lbs N/ acre/ yr treatment. Nitrate loading estimates for the plots treated with 400 lbs N/ acre/ yr indicate that over 1200 lbs N/ acre was in the vadose zone beneath the crop rooting zone. In 15 years, the nitrate moved vertically at least 60 feet through these fine-textured, unsaturated sediments. As much as 600 lbs N/acre have accumulated in the vadose zone under independent corn producers'fields.
Vadose zone sampling is effective in predicting future non-point nitrate-contaminated areas.  相似文献   

10.
In Europe, computation of displacement demand for seismic assessment of existing buildings is essentially based on a simplified formulation of the N2 method as prescribed by Eurocode 8(EC8). However, a lack of accuracy of the N2 method in certain conditions has been pointed out by several studies. This paper addresses the assessment of effectiveness of the N2 method in seismic displacement demand determination in non-linear domain. The objective of this work is to investigate the accuracy of the N2 method through comparison with displacement demands computed using non-linear timehistory analysis(NLTHA). Results show that the original N2 method may lead to overestimation or underestimation of displacement demand predictions. This may affect results of mechanical model-based assessment of seismic vulnerability at an urban scale. Hence, the second part of this paper addresses an improvement of the N2 method formula by empirical evaluation of NLTHA results based on EC8 ground-classes. This task is formulated as a mathematical programming problem in which coefficients are obtained by minimizing the overall discrepancy between NLTHA and modified formula results. Various settings of the mathematical programming problem have been solved using a global optimization metaheuristic. An extensive comparison between the original N2 method formulation and optimized formulae highlights benefits of the strategy.  相似文献   

11.
The net anthropogenic nitrogen input(NANI) is an important nutrient source that causes eutrophication in water bodies. Understanding the spatio-temporal variation of NANI is important for regional environment assessment and management.This paper calculated NANI in the upper Yangtze River basin(YRB), upstream of the Three Gorges Dam(TGD), from1990 to 2012, and analyzed its spatio-temporal characteristics. Over the past 23 years of the study, the average annual NANI increased from 3200 kg N km~(-2) to 4931 kg N km~(-2). The major components were fertilizer N application, atmospheric N deposition,and net food and feed N import. In the northwest high mountainous region with a sparse population, the main component was atmospheric N deposition. Fertilizer N application and net food and feed N import were concentrated in the Chengdu Plain because of the high population density and large areas of farmland. This research found that NANI increased with rapid urbanization and increasing population. The Pearson correlation results illustrated that the spatial distributions of NANI and its major components were affected by land cover/use, agricultural GDP and total population. Increasing NANI has been the major cause of the degrading stream water quality over the past 20 years and is becoming a major threat to the water quality of the TGD reservoir.  相似文献   

12.
As an essential component of proteins and genetic material for all organisms, nitrogen (N) is one of the major limiting factors that control the dynamics, biodiversity and functioning of lacustrine wetlands, in which intensified N biogeochemical activities take place. Reactive N loaded into wetland ecosystems has been doubled due to various human activities, including industrial, agricultural activities and urbanization. The main driving mechanisms of N transport and transformation in lacustrine wetlands are categorized to pushing forces and pulling forces in this study. Geomorphology, wetland age, N concentrations, and temperature are the main pushing forces (passive forces); whereas water table variation, oxygen concentration, other elements availability, oxidation-reduction potential (Eh) and pH, and microorganisms are the predominant pulling forces (active forces). The direction and kinetic energy of reactions are determined by pulling forces and then are stimulated by pushing forces. These two types of forces are analyzed and discussed separately. Based on the analysis of driving mechanisms, possible solutions to wetland N pollutions are proposed at individual, regional and global scales, respectively. Additional research needs are addressed to obtain a thorough understanding of N transport and transformations in wetlands and to reduce detrimental impacts of excessive N on such fragile ecosystems.  相似文献   

13.
淀山湖、小兴凯湖和洱海分别处在不同的营养阶段,夏季都存在蓝藻水华现象,有效控制蓝藻水华应控氮还是控磷一直存在争议.本研究采用营养物加富生物测试的试验方法,研究和比较三个湖泊限制性营养元素(N和P)夏季对浮游藻类生长的刺激作用,并采用多因素方差分析和两两比较方法(LSD)检验试验结果的显著性.结果表明:淀山湖(TN/TP=10左右)、洱海(TN/TP=29左右)、小兴凯湖(TN/TP=9左右)在夏季分别表现出显著的氮响应、氮磷双重响应、氮响应;较低氮磷比的营养程度较高的湖泊(淀山湖和小兴凯湖)夏季应控制氮含量,若添加氮更容易引发蓝藻(微囊藻)水华,而高氮磷比的初期富营养化湖泊(洱海)夏季应同时控制氮磷含量,同时添加氮磷的交互作用容易引发蓝藻(微囊藻)水华.  相似文献   

14.
Increasing eutrophication in the coastal seas of China from 1970 to 2050   总被引：4，自引：0，他引：4  
We analyzed the potential for eutrophication in major seas around China: the Bohai Gulf, Yellow Sea and South China Sea. We model the riverine inputs of nitrogen (N), phosphorus (P) and silica (Si) to coastal seas from 1970 to 2050. Between 1970 and 2000 dissolved N and P inputs to the three seas increased by a factor of 2–5. In contrast, inputs of particulate N and P and dissolved Si, decreased due to damming of rivers. Between 2000 and 2050, the total N and P inputs increase further by 30–200%. Sewage is the dominant source of dissolved N and P in the Bohai Gulf, while agriculture is the primary source in the other seas. In the future, the ratios of Si to N and P decrease, which increases the risk of harmful algal blooms. Sewage treatment may reduce this risk in the Bohai Gulf, and agricultural management in the other seas.  相似文献   

15.
Investigating factors controlling the temporal patterns of nitrogen (N) and dissolved organic carbon (DOC) exports on the basis of a comparative study of different land uses is beneficial for managing water resources, especially in agricultural watersheds. We focused our research on an agricultural watershed (AW) and a forested watershed (FW) located in the Shibetsu watershed of eastern Hokkaido, Japan, to investigate the temporal patterns of N and DOC exports and factors controlling those patterns at different timescales (inter‐annual, seasonal, and hydrological event scales). Results showed that the annual patterns of N and DOC exports significantly varied over time and were probably controlled by climate. Higher discharge volumes in 2003, a wet year, showed higher N and DOC loadings in both watersheds. However, this process was also regulated by land use associated with N inputs. Higher concentrations and loadings were shown in the agricultural watershed. At the seasonal scale, N and DOC exports in the AW and the FW were more likely controlled by sources associated with land use. The Total N (TN) and Nitrate‐N (NO3?‐N) had higher concentrations during snowmelt season in the AW, which may be attributed to manure application in late autumn or early winter in the agricultural watershed. Concentrations of TN, NO3?‐N, dissolved organic nitrogen (DON), and DOC showed higher values during the summer rainy season in the FW, related to higher litter decomposition during summer and autumn and the fertilizer application in the agricultural area during summer. Higher DOC concentrations and loadings were observed during the rainy season in the AW, which is probably attributed to higher DOC production related to temperature and microbial activity during summer and autumn in grasslands. Correlations between discharge and concentrations differed during different periods or in different watersheds, suggesting that weather discharge can adequately represent the fact that N export depends on N concentrations, discharge level, and other factors. The differing correlations between N/DOC concentrations and the Si concentration indicated that the N/DOC exports might occur along different flow paths during different periods. During baseflow, the high NO3?‐N exports were probably derived from deep groundwater and might have percolated from uplands during hydrological events. During hydrological events, NO3?‐N exports may occur along near‐surface flow paths and in deep groundwater, whereas DOC exports could be related to near‐surface flow paths. At the event scale, the relationships between discharge and concentrations of N and DOC were regulated by antecedent soil moisture (shallow groundwater condition) in each watershed. These results indicated that factors controlling N and DOC exports varied at different timescales in the Shibetsu area and that better management of manure application during winter in agricultural lands is urgently needed to control water pollution in streams. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

16.
The Apollo 11 soil breccias are samplers of the ancient lunar environment due to their history in the regolith and their efficient closure to addition of recent solar wind upon compaction. These breccias contain the lowest15N/14N isotopic ratio yet reported for any lunar sample (in fact, for any natural sample). This extends the range of variation of15N/14N of the solar wind to greater than 30%, from a δ15N of ?190‰ in the past to +120‰ at present. No mechanism is yet known that is capable of accounting for such a large change in the15N/14N ratio without producing a substantial concomitant change in the13C/12C ratio, although some sort of nuclear reaction in the sun appears to be required. Apollo 11 soil breccias and 15086 are all formed by meteoritic impacts which compact the lower regolith against the basement rock without much heating. Rock 15086 formed from the layer of regolith between 100 and 200 cm depth, as shown by the close agreement between the nitrogen content and isotopic ratios of 15086 and those of the Apollo 15 deep drill core. Cosmic ray exposure ages, based on spallation-produced15N, are 2.3 ± 0.4 b.y. for Apollo 11 breccias. This age is much greater than the estimate from cosmogenic21Ne, presumably due to diffusive loss of neon.  相似文献   

17.
激发态氮分子N*2在电离层F区中起着重要的作用,它使F区占主导地位的O+离子的损失率增大,从而使该区的电子浓度减少. 本文利用理论电离层数值模型,通过考虑与不考虑N*2的作用,对包括1990年6月、1997年5月、1998年5月以及2000年4月磁暴事件在内的时间区间的电离层响应情形进行模拟研究,并与实测结果进行对比. 结果表明,N*2对电离层电子浓度的影响在太阳活动高年非常明显,在太阳活动低年虽有些影响,但效果并不明显,其程度远不如高年. 在太阳活动高年,不仅是磁暴期间,在较宁静期间也必须考虑N*2的影响. 而且,在考虑N*2的作用时,还与激发态振动温度Tν有关,在采用Tν=Tn（其中Tn为背景中性大气的温度）的简化处理时,所得结果与观测结果的符合程度不如对Tν进行精确计算时所得的结果好. 模拟结果还表明,太阳活动高年,N*2作用的结果主要是使150km高度以上的F区电离层电子浓度减少,而对150km以下高度的电离层电子浓度则影响不大. 另外,N*2基本不影响F2层峰高hmF2的值.  相似文献   

18.
The southwestern Adirondack region of New York receives among the highest rates of atmospheric nitrogen (N) deposition in the USA. Atmospheric N deposition to sensitive ecosystems, like the Adirondacks, may increase the acidification of soils through losses of exchangeable nutrient cations, and the acidification of surface waters associated with enhanced mobility of nitrate (NO3?). However, watershed attributes, including surficial terrestrial characteristics, in‐lake processing, and geological settings, have been found to complicate the relationships between atmospheric N deposition and N drainage losses. We studied two lake‐watersheds in the southwestern Adirondacks, Grass Pond and Constable Pond, which are located in close proximity (～26 km) and receive similarly high N deposition, but have contrasting watershed attributes (e.g. wetland area, geological settings). Since the difference in the influence of N deposition was minimal, we were able to examine both within‐ and between‐watershed influences of land cover, the contribution of glacial till groundwater inputs, and in‐lake processes on surface water chemistry with particular emphasis on N solutes and dissolved organic carbon (DOC). Monthly samples at seven inlets and one outlet of each lake were collected from May to October in 1999 and 2000. The concentrations of NO3? were high at the Grass Pond inlets, especially at two inlets, and NO3? was the major N solute at the Grass Pond inlets. The concentrations of likely weathering products (i.e. dissolved Si, Ca2+, Mg2+, Na+) as well as acid neutralizing capacity and pH values, were also particularly high at those two Grass Pond inlets, suggesting a large contribution of groundwater inputs. Dissolved organic N (DON) was the major N solute at the Constable Pond inlets. The higher concentrations of DON and DOC at the Constable Pond inlets were attributed to a large wetland area in the watershed. The DOC/DON ratios were also higher at the Constable Pond inlets, possibly due to a larger proportion of coniferous forest area. Although DON and DOC were strongly related, the stronger relationship of the proportion of wetland area with DOC suggests that additional factors regulate DON. The aggregated representation of watershed physical features (i.e. elevation, watershed area, mean topographic index, hypsometric‐analysis index) was not clearly related to the lake N and DOC chemistry. Despite distinctive differences in inlet N chemistry, NO3? and DON concentrations at the outlets of the two lakes were similar. The lower DOC/DON ratios at the lake outlets and at the inlets having upstream ponds suggest the importance of N processing and organic N sources within the lakes. Although an inverse relationship between NO3? and DOC/DON has been suggested to be indicative of a N deposition gradient, the existence of this relationship for sites that receive similar atmospheric N deposition suggest that the relationship between NO3? and the DOC/DON ratio is derived from environmental and physical factors. Our results suggest that, despite similar wet N deposition at the two watershed sites, N solutes entering lakes were strongly affected by hydrology associated with groundwater contribution and the presence of wetlands, whereas N solutes leaving lakes were strongly influenced by in‐lake processing. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

19.
鄱阳湖产银鱼的繁殖生物学   总被引：6，自引：1，他引：6  
陈国华  张本 《湖泊科学》1990,2(1):59-67
本文记述了鄱阳湖产太湖短吻银鱼(Neosalanx tangkahkeii taihuensis)、乔氏短吻银鱼(Neosalanx jordani)、雷氏银鱼(Reganisalanx brachyrostralis)等三种银鱼的成熟年龄、繁殖时期、生殖群体的体长、性比、生殖力、卵的特征等繁殖生物学资料,并记述了太湖短吻银鱼性腺成熟系数的周年变化、太湖短吻银鱼和乔氏短吻银鱼的产卵生态条件等。近二十年来鄱阳湖银鱼产量急剧下降的主要原因是产卵场遭到了严重破坏。银鱼生命周期仅一年,繁殖力强,认为加强繁殖保护、合理安排捕捞时间是恢复鄱阳湖银鱼资源的关键措施。  相似文献   

20.
进入湖泊中不同氮源氮稳定同位素值(δ15N)的差异和生物对氮稳定同位素的记忆作用,可以反映流域人类活动输入的污染物对生态系统的影响程度.本文调查了太湖4个湖湾(梅梁湾、贡湖湾、竺山湾和东太湖)中铜锈环棱螺(Bel-lamya aeruginosa)的δ15N值,结果表明环棱螺δ15N值的变幅为6.9‰～18.1‰,平均值为11.2‰,不同湖湾中环棱螺δ15N值差异极显著,从高到低依次为梅梁湾(17.7‰)、贡湖湾(13.2‰)、东太湖(10.2‰)和竺山湾(7.8‰).分析认为,梅梁湾和贡湖湾接纳较多的人类活动产生的污染物,其周边城市如无锡、常州等地的污水处理效率有待提高;竺山湾水体氮素主要来自于农业面源污染,需降低农田化肥的使用量.  相似文献   

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