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1.
城市群落大气污染源影响的空间结构及尺度特征 总被引：29，自引：1，他引：29
以迅速发展的城市群落-北京及周边区域为样本, 利用2003年冬季(2月)、夏季(8月)北京城市大气环境现场科学试验(BECAPEX, Beijing City Air Pollution Observation Experiment)建筑群边界层大气污染动力-化学过程观测资料以及相关的气象要素、卫星反演气溶胶光学厚度等综合资料, 进行“点-面”空间结构动力-统计合成分析, 剖析北京大城市及周边区域大气污染影响域的空间结构及多尺度特征. 结果表明, 冬、夏季不同污染排放源对大气污染成分特征的贡献率具有显著差异, 统计模型主成分分析结果亦表明, 冬季气溶胶颗粒物成分结构以SO2和NOx影响为主; 夏季粒子成分结构则以CO, NOx影响为主. 冬、夏季北京城区不同方位测点近地层大气动力、热力结构及建筑群上边界各类污染物种均具有“同位相”变化及其“影响域”空间尺度特征. 功率谱分析发现冬、夏季颗粒物浓度和大气风场动力结构的周期谱相吻合, 冬季以长周期为主, 夏季则多为短周期, 揭示出冬、夏季大气环流季节性尺度特征对大气污染变化周期特征的影响效应. 分析城市区域热力非均匀性特征, 可发现北京地区热岛多尺度效应与高层建筑群面积非均匀扩展特征存在相关关系. 城市大气动力、热力特征空间结构中城市边界层群筑群湍流尺度特征对城市大气污染多尺度特征具有重要影响. 晴空、稳定天气条件下MODIS气溶胶变分订正分析场和污染源追踪相关合成风矢场综合分析模型均表明, 冬季北京大气污染气溶胶颗粒物的排放源可远距离追溯到北京南部周边的河北、山东及天津等地更大尺度空间范围, 气溶胶指数高值区与北京及周边地区居民户数高值区(采暖面源)空间分布存在关联. 冬、夏季空气质点后向轨迹特征呈类似上述多尺度特征, 且描述出不同季节污染源空间分布的尺度特征差异, 城区大气污染周边源轨迹路径主体来自城市近郊固定工业面源或采暖面源, 且冬季周边污染源扩散输送距离较夏季呈更远的空间尺度, 上述结论描述出城市区域大气污染源影响和大气动力结构引起的多尺度空间影响域及季节性特征. 冬季TOMS气溶胶光学厚度高值区域位于北京地区并向南延伸, 且呈南北向带状分布, 可描述出周边地形分布对区域尺度大气污染源扩散的动力影响效应. 研究分析表明: 北京周边大地形“谷地”内冬季污染程度与南部周边地区的污染排放源密切相关; 北京及周边地区冬季的气溶胶光学厚度和日照时数的“反位相”变化特征显著, 冬季云量、雾日数与气溶胶呈区域尺度相关特征, 反映了该区域尺度气溶胶影响的局地气候效应. 另外, 流域面尺度的大气干、湿沉降分布对密云水库区域尺度空间水体的影响分析亦反映了夏季水、土、气多圈层污染源影响多尺度空间结构对密云水库水质影响的可能性. 相似文献
2.
Fernald前向积分法能否用于机载大气探测激光雷达气溶胶后向散射系数的反演一直是一个有争议的课题.本文利用青岛机载大气探测激光雷达实测数据、国外机载大气探测激光雷达实测数据和机载大气探测激光雷达模拟数据,对Fernald前向积分法应用于不同高度的机载大气探测激光雷达气溶胶后向散射系数反演的误差进行了定量分析,分析结果表明:飞机的飞行高度在3.5 km左右,标定值存在20%的误差时,离地面2 km的高度范围内反演得到的气溶胶后向散射系数的相对误差在12%以内,但在标定点附近相对误差可达20%;飞机飞行高度在7 km左右,当标定值存在100%的误差时,反演得到的气溶胶后向散射系数的相对误差大都在10%~15%之间,标定值存在400%的误差时,反演得到的气溶胶后向散射系数的相对误差大部分在15%~50%之间.本文从理论上对Fernald前向积分法应用于机载大气探测激光雷达气溶胶后向散射系数反演出现负值的原因进行了探讨.研究表明:Fernald前向积分法能够较准确地反演出中高空探测(4.5 km以上)机载大气探测激光雷达气溶胶后向散射系数,但应用于低空探测(4.5 km以下)机载大气探测激光雷达气溶胶后向散射系数反演时,反演误差较大甚至反演结果会出现负值. 相似文献
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本文利用中国科学院空间科学与应用研究中心的瑞利激光雷达首次观测到了平流层地形重力波活动的现象,并结合美国国家环境预报中心(NCEP)的全球预报系统(GFS)的风场数据分析了该地形重力波的基本参数.与惯性重力波相比较,地形重力波的密度扰动没有下传的相位,在同一高度上,其扰动相位保持不变.北京空间科学与应用研究中心瑞利激光雷达自2012年开始观测实验以来,已经观测到多起地形重力波活动事件.本文以2013年11月11日的观测数据为例,研究北京上空的地形重力波活动,并结合GFS风场数据分析了北京上平流层地形重力波的波长、传播方向、传播速度等参量.通过分析得到在2013年11月11日北京上空存在一列传播方向为北偏西52.4°,水平波长为5.5km,平均垂直波长约为6.0km的地形重力波. 相似文献
4.
EOF模型分析北京周边气溶胶影响域气候变化显著性特征 总被引：5，自引：0，他引：5
利用1979~2000年TOMS气溶胶光学厚度和华北地区气象站日照时数、雾日数、低云量等资料以及EOF模型综合统计分析方法,研究冬季北京及周边城市群落的气溶胶分布特征及其对区域气候的影响效应问题,重点探讨了北京周边区域气候EOF模型特征向量变化显著区与气溶胶影响效应的相关联系.分析多年平均冬季TOMS气溶胶光学厚度的区域分布,发现北京及其南部周边地区“马蹄型”大地形谷地内存在南北向带状大范围相对稳定的气溶胶浓度高值区空间分布;冬季气溶胶光学厚度在北京与周边地区存在高相关影响区,在此气溶胶相互影响显著区,冬季气溶胶光学厚度与雾日数、低云量呈年际变化“同位相”特征,表明特定区域大气环流背景下,北京及周边地区气溶胶变化对该地区低云量、雾日数的年际变化存在影响效应.进一步通过EOF模型特征分析,揭示出华北地区冬季日照时数减少、低云量和雾日数增多气候变化区及其长期演变趋势,尤其EOF模型第一特征向量中日照时数、雾日数及低云量变化显著区与其20世纪80~90年代偏差显著区近似重合,且这些变化特征显著区域均与北京周边南北向带状气溶胶光学厚度高值区及其高相关区呈对应关系;日照时数、雾日数、低云量EOF模型第一特征向量时间系数与区域平均气溶胶光学厚度年际变化呈“同位相”特征,且均呈长期演变上升趋势.EOF模型分析描述出北京南部周边地区冬季日照时数减少、低云量和雾日数增多的区域气候变化主体特征,揭示出区域气溶胶影响效应,即多年平均冬季气溶胶光学厚度高值区以及日照时数、低云量和雾日数EOF模型第一特征向量变化显著区均位于北京南部周边城市群落区域,上述相关分布特征揭示出北京南部周边城市群落影响域存在气溶胶气候效应区域性增强的变化趋势. 相似文献
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大气边界层研究进展 总被引：1，自引：0，他引：1
大气边界层对云和对流的发展、演变有重要作用.本文回顾了在大气边界层高度计算方法,边界层的时空分布特征、结构和发展机理,以及边界层参数化方案等方面的主要研究进展.大气边界层高度计算方法主要分为基于大气廓线观测数据计算和基于模式参数化方案计算两大类;大气边界层高度频率分布形态具有明显的日变化特征,并且稳定、中性和对流边界层高度的频率分布呈现出不同的Gamma分布特征;地面湿度状况对边界层发展影响明显,对于不同的下垫面热力性质和地形状况,大气边界层高度呈现出明显的空间差异,青藏高原边界层高度明显高于一般平原地区;在强烈的地面加热驱动下,对流边界层与残余层通过正反馈机制循环增长可以形成4000 m以上的超高大气边界层;研制大气边界层、浅对流以及云物理方案的统一参数化框架是未来数值预报模式的发展趋势. 相似文献
6.
采用WRFV2.2中尺度数值模式对鄱阳湖地区200 km×200 km范围内,2009年11月5日00∶00至2009年11月6日12∶00不同高度的气象要素进行了数值模拟,得到了水平分辨率为1 km的鄱阳湖地区大气边界层风、温、湿度场和廓线分布的大气边界层物理特征.模拟结果发现:白天鄱阳湖面上空存在着冷岛效应并伴随湖风,而夜间湖面上空存在着热岛效应并伴随陆风,湖面与陆地之间最大温差可达6 ℃;同时地形以及下垫面类型对鄱阳湖区风场的分布具有很大影响,夜间存在一条东北西南走向的低空辐合带,白天逐渐消失;此外受风场和地形作用湖面上空的湿度分布也不均匀,白天湿度层厚度低而夜晚湿度层厚度高,湖中心右侧湿度值大于左侧湿度值.模拟结果能较好地反映鄱阳湖的大气边界层物理特征,有助于了解鄱阳湖地区区域气候的特点,以及由于地形、地理环境、地表特征所形成的不同高度上的风、温、湿的分布规律和大气边界层物理特征,为鄱阳湖地区局地天气预报、风能资源开发、环境保护等提供了科学依据. 相似文献
7.
一种基于卫星遥感AOT估算近地面颗粒物的方法 总被引：9，自引：0，他引：9
本文建立了一种基于卫星遥感AOT估算近地面颗粒物浓度的新方法.该方法考虑大气边界层厚度和近地面相对湿度的区域分布变化情况,基于大气边界层模式模拟结果和卫星遥感气溶胶光学厚度进行近地面颗粒物浓度估算.基于RAMS模拟结果和MODIS气溶胶光学厚度数据,利用该方法获得了华北地区近地面PM2.5质量浓度.并用研究区域中16个地面站点的颗粒物浓度监测数据对估算结果进行了评估.结果表明,遥感反演的近地面PM2.5与地面监测数据在趋势上基本一致,二者相关R2达到0.61.与此同时,又利用地面激光雷达和气象仪测量结果对MODIS气溶胶光学厚度数据进行了近地面颗粒物估算,并将估算的结果与新方法得到的估算结果进行了比较.比较结果表明,新方法获得的估算结果与地面监测数据具有更好的相关性,和常规方法相比,相关R2从0.32提高到0.62. 相似文献
8.
广州地区一次严重灰霾过程的垂直探测 总被引：3，自引：0，他引：3
利用激光雷达和微波辐射计在广州地区一次严重灰霾过程进行探测,采用小波变换协方差方法反演边界层高度,从热力和动力的角度分析边界层气象因子和能见度之间的关系.结果表明,边界层高度有明显的日变化过程,和地面能见度变化有很好的一致性.在清洁过程,边界层高度超过1 km,发生严重灰霾时,最高仅为500 m.50-100 m的温度梯度滞后30 h和能见度相关性更加显著,相关系数达到0.77.高层能见度（255 m）和下层稳定度有显著的负相关,清洁日负相关系数最大达-0.76,灰霾日负相关系数最大达-0.49.在相关的边界层气象因子中,地表通风系数和地面能见度成线性关系,相关系数最高,达0.88.边界层高度、地面风速、相对湿度和地面能见度的相关系数分别为0.76,0.67和-0.77.各气象因子之间具有较高的相关性.此次灰霾过程的主控气象因子为地表通风系数,在没有边界层高度探测的地区可利用地面能见度和风速估算边界层高度. 相似文献
9.
东亚大陆及周边海域Moho界面深度分布和基本构造格局 总被引：30，自引：4，他引：30
基于中国大陆和周边相邻各国及邻近海域: 俄罗斯、哈萨克斯坦、日本、印度、巴基斯坦、菲律宾以及日本海、黄海、东海、南海、菲律宾海盆、太平洋及印度洋等地多年来所进行的人工源深部地震探测剖面及所取得的岩石圈结构和构造的结果, 并通过这些资料的分析与研究, 提出了以中国大陆及海域为核心的东亚大陆及海域Moho界面的二维结构分布特征. 依据莫霍(Moho)界面的埋深和起伏变化特征提出: 东亚地域可以划分为18条大小不一的梯度带, 18个地壳块体, 20个沉积盆地与拗陷地区. 这些块体本身的Moho界面深度变化相对平缓, 而不同块体之间却为Moho界面深度明显变化的边界. 基于东亚及周边地域Moho界面展布和块体分区与梯度带的分布特征, 对造山带与沉积盆地、断裂体系与裂谷、板块边界与海陆耦合及构造格局进行了论述. 相似文献
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11.
Aerosol can induce visibility reduction, affect radiation balance and modify cloud property on the environmental effect, and show the harmful effects on human health. Insight of aerosol becomes an integral task in the process of control measures for environmental pollution. The present study provided an analysis of temporal–spatial variations of aerosol optical depth (AOD) using the MOD04 level-2 in collection 6 (C6) with the deep blue retrieval algorithm from January 2005 to December 2015 over Yangtze River Delta (YRD) in China. The AOD validations between MODIS and Aerosol Robotic Network (AERONET) were estimated by the methods of regression, correlation. Then, the periodic features and trends of AOD and angstrom exponent (AE) were explored with the wavelet transformation (WT) procedure. Further, the variations of AOD and AE spatial distribution on multi-time scales (annual, monthly and season) were demonstrated. Meantime, the sources of AOD are discussed. It was found that the daily AOD from MODIS has a strong correlation relationship (slope?=?0.9838, r?=?0.84) with AERONET over YRD. The variations of both AOD and AE on time series have been distinct temporal periodic (12, 6 and 4 months) characteristics, and show the decreasing trends on annual and semi-annual periods. On annual, the AOD on spatial distribution is slowly declining from the northwest towards the southeast, and the AE on spatial distribution is gradually decreasing from the northwest to the southeast and from the land to the coast. The variations both inter-annual AOD and AE on spatial distribution show the inverse trends, respectively. On monthly, the means of AOD range from minimum 0.46 in January to maximum 0.90 in July, and the variations of spatial distribution mainly occur in the north parts of Yangtze River and some scattered areas with high terrain and south coast. The means of AE range from minimum 1.13 in October to maximum 1.58 in April, and the variations of spatial distribution are mainly found in the south of Henan, the north of Jiangsu, the coast belt and the riverside of Yangtze River and the high terrain regions. On seasonality, the means of AOD reaches its maximum 0.68 in summer and minimum 0.50 in winter, and the variations of spatial distribution mainly occur in the coast belt, the north parts of Hongze Lake and the south parts with high terrain. The means of AE reaches its maximum 1.48 in spring and minimum 1.25 in autumn, and the variations of spatial distribution were shown the similarity with that of monthly. 相似文献
12.
Vadimas Dudoitis Steigvilė Byčenkienė Kristina Plauškaitė Carlo Bozzetti Roman Fröhlich Genrik Mordas Vidmantas Ulevičius 《Acta Geophysica》2016,64(3):711-731
The aerosol chemical composition in air masses affected by large vegetation fires transported from the Kaliningrad region (Russia) and southeast regions (Belarus and Ukraine) during early spring (March 2014) was characterized at the remote background site of Preila, Lithuania. In this study, the chemical composition of the particulate matter was studied by high temporal resolution instruments, including an Aerosol Chemical Speciation Monitor (ACSM) and a seven-wavelength aethalo-meter. Air masses were transported from twenty to several hundred kilometres, arriving at the measurement station after approximately half a day of transport. The concentration-weighted trajectory analysis suggests that organic aerosol particles are mainly transported over the Baltic Sea and the continent (southeast of Belarus). Results show that a significant fraction of the vegetation burning organic aerosol is transformed into oxidised forms in less than a half-day. Biomass burning aerosol (BBOA) was quantified from the ACSM data using a positive matrix factorization (PMF) analysis, while its spatial distribution was evaluated using air mass clustering approach. 相似文献
13.
During a series of substorm events on November 12 2004, the Neutral Atom Detector Unit(NUADU) flying onboard the TC-2 spacecraft observed, close to perigee, bright low-altitude Energetic Neutral Atom(ENA) emissions from both north and south poles. Through utilizing high temporal and spatial resolution data inversion techniques we present here a global view the associated processes of energetic ion deposition and injection at the uniquely high temporal resolution of a few minutes. It is demonstrated that the ENA emissions observed came mainly from the, low-altitude, high magnetic latitude polar region. Since precipitating ions follow magnetic field lines and have more chance to produce ENA emissions through charge exchange there.Therefore, the employment of a low-orbit satellite to record at high temporal and spatial resolution ENA image data is inferred to be the best way to monitor those dynamic ring current variations that occur during geomagnetic activity. 相似文献
14.
本研究收集整理了东亚地区一个黑碳气溶胶的排放源,并利用一个三维化学输送模式系统模拟研究了东亚地区春季黑碳气溶胶的输送和演变过程.黑碳气溶胶浓度的模拟值与地面观测站和观测船获取的监测值相比,模拟值与监测值具有良好的一致性,这表明本研究收集整理的黑碳气溶胶的排放量及其分布是基本合理的,模式系统较好地反映了黑碳气溶浓度的时空分布和变化趋势,再现了许多观测到的重要特征.模拟结果表明,东亚地区春季间隙性的长距离输送对于西北太平洋海域的黑碳气溶胶浓度分布具有非常重要的影响. 相似文献
15.
Ralph A.KAHN 《中国科学D辑(英文版)》2009,52(1):132-144
The Multiangle Imaging SpectroRadiometer (MISR) launched by NASA in late 1999 has a unique multiangle design, which points
nine cameras at fixed angles along the satellite flight track and collects reflected solar radiation simultaneously. This
design allows the retrieval of a rich dataset of particle abundance, shape and composition over both land and ocean. Some
of its capabilities have not been seen by any currently operating satellite aerosol sensors. Since MISR is sensitive to fine
particles, it provides a new data source to study the spatial and temporal characteristics of air quality over large geographical
regions. We first briefly introduce the MISR instrument, the retrieval and structure of MISR aerosol data, and then review
the applications of MISR aerosol data in various aspects of air quality research since its launch. These include the spatial
distributions of particle pollution events such as dust storms, wild fires, and urban pollution. Because of the high quality
of MISR aerosol data, they can be used as quantitative indicators of particle pollution levels. We review the current modeling
studies of surface level particle concentrations. Next, we introduce research results using MISR’s advanced data such as the
plume heights, and particle microphysical properties. In the discussion, we compare MISR research with current MODIS research
to the best of our ability as MODIS data have been more extensively explored by the Chinese scientific community. Finally,
we summarize the advantages and disadvantages of MISR data related to its applications to the air quality research. Given
the highly quantitative measurements and comprehensive aerosol information MISR can provide, we believe that it will provide
great values to advance our understanding of the particle air pollution in China.
Supported by Harvard-EPA Center on Particle Health Effects (Grant Nos. R-827353 and R-832416), NASA’s Climate and Radiation
Research and Analysis Program, the EOS-MISR Instrument Project and the National High Technology Research and Development Program
of China (Grant No. 2006AA06A305). 相似文献
16.
This study contains a comparative analysis of aerosol optical thickness (AOT) between numerical calculations obtained from
the Navy Aerosol Analysis and Prediction System (NAAPS) model and direct observations from the AERONET robotic network and
the Saharan Aerosol over WArsaw (SAWA) field campaign. AOT was calculated for 500 nm wavelength. The comparison shows underestimation
of the total aerosol optical thickness simulated by NAAPS. The correlation coefficients between model and observation oscillates
between 0.57 and 0.72. Results of seven-year (1998–2004) NAAPS simulation of aerosol components (sea salt, mineral dust, sulphate,
and smoke) show large temporal and spatial variability of the aerosol optical thickness over Europe. The least polluted region
is the Iberian Peninsula, while the highest aerosol burdens occurred in Central Europe, mostly due to anthropogenic sulphate
particles. Finally, the analysis of mineral dust transport shows frequent episodes of Saharan dust inflow over Central Europe.
There are about 20 days a year (4 days in May) when instantaneous AOT associated with mineral dust aerosol increases over
0.1. 相似文献
17.
The structure of the mid- and high-latitude ionosphere during the November 2004 storm event obtained from GPS observations 总被引：1，自引：1，他引：1
Andrzej Krankowski Irk I. Shagimuratov Lubomir W. Baran Galina Yakimova 《Acta Geophysica》2007,55(4):490-508
GPS data from the International GNSS Service (IGS) network were used to study the development of the severe geomagnetic storm
of November 7–12, 2004, in the total electron content (TEC) on a global scale. The TEC maps were produced for analyzing the
storm. For producing the maps over European and North American sectors, GPS measurements from more than 100 stations were
used. The dense network of GPS stations provided TEC measurements with a high temporal and spatial resolution. To present
the temporal and spatial variation of TEC during the storm, differential TEC maps relative to a quiet day (November 6, 2004)
were created.
The features of geomagnetic storm attributed to the complex development of ionospheric storm depend on latitude, longitude
and local time. The positive, as well as negative effects were detected in TEC variations as a consequence of the evolution
of the geomagnetic storm. The maximal effect was registered in the subauroral/auroral ionosphere during substorm activity
in the evening and night period. The latitudinal profiles obtained from TEC maps for Europe gave rise to the storm-time dynamic
of the ionospheric trough, which was detected on November 7 and 9 at latitudes below 50°N. In the report, features of the
response of TEC to the storm for European and North American sectors are analyzed. 相似文献
18.
In this study, monthly and annual Upper Blue Nile Basin rainfall data were analyzed to learn the rainfall statistics and its temporal and spatial distribution. Frequency analysis and spatial characterization of rainfall in the Upper Blue Nile Basin are presented. Frequency analysis was performed on monthly basin rainfall. Monthly basin average rainfall data were computed from a network of 32 gauges with varying lengths of records. Monthly rainfall probability distribution varies from month to month fitting Gamma‐2, Normal, Weibull and Log‐Normal distributions. The January, July, October and November basin rainfall fit the Gamma‐2 probability distribution. The February, June and December ones fit Weibull distribution. The March, April, May and August rainfall fit Normal distribution. The September rainfall fits Log‐Normal distribution. Upper Blue Nile Basin is relatively wet with a mean annual rainfall of 1423 mm (1960–2002) with a standard deviation of 125 mm. The annual rainfall has a Normal probability distribution. The 100‐year‐drought basin annual rainfall is 1132 mm and the 100‐year‐wet basin annual rainfall is 1745 mm. The dry season is from November through April. The wet season runs from June through September with 74% of the annual rainfall. October and May are transition months. Monthly and annual rainfalls for return periods 2‐, 5‐, 10‐, 25‐, 50‐ and 100‐year dry and wet patterns are presented. Spatial distribution of annual rainfall over the basin is mapped and shows high variation with the southern tip receiving as high as 2049 mm and the northeastern tip as low as 794 mm annual average rainfall. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献
19.
China has developed an airborne gravimetry system based on SINS/DGPS named SGA-WZ,the first system in which a strapdown inertial navigation system(SINS)has been used for airborne gravimetry in China.This gravity measurement system consists of a strap-down inertial navigation system and a differential global positioning system(DGPS).In April 2010,a flight test was carried out in Shandong Province of China to test the accuracy of this system.The test was designed to assess the repeatability and accuracy of the system.Two repeated flights and six grid flights were made.The flying altitude was about 400 m.The average flying speed was about 60 m/s,which corresponds to a spatial resolution of 4.8 km when using 160-s cutoff low-pass filter.This paper describes the data processing of the system.The evaluation of the internal precision is based on repeated flights and differences in crossover points.Gravity results in this test from the repeated flight lines show that the repeatability of the repeat lines is 1.6 mGal with a spatial resolution of 4.8 km,and the internal precision of grid flight data is3.2 mGal with a spatial resolution of 4.8 km.There are some systematic errors in the gravity results,which can be modeled using trigonometric function.After the systematic errors are compensated,the precision of grid flight data can be better than1 mGal. 相似文献