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1.
Total ozone anomalies (deviation from the long-term mean) are created by anomalous circulation patterns. The dynamically produced ozone anomalies can be estimated from known circulation parameters in the layer between the tropopause and the middle stratosphere by means of statistics. Satellite observations of ozone anomalies can be compared with those expected from dynamics. Residual negative anomalies may be due to chemical ozone destruction. The statistics are derived from a 14 year data set of TOMS (Total Ozone Mapping Spectrometer January 1979-Dec. 1992) and corresponding 300 hPa geopotential (for the tropopause height) together with 30 hPa temperature (for stratospheric waves) at 60°N. The correlation coefficient for the linear multiple regression between total ozone (dependent variable) and the dynamical parameters (independent variables) is 0.88 for the zonal deviations in the winter of the Northern Hemisphere. Zonal means are also significantly dependent on circulation parameters, besides showing the known negative trend function of total ozone observed by TOMS. The significant linear trend for 60°N is 3 DU/year in the winter months taking into account the dependence on the dynamics between the tropopause region and the mid-stratosphere. The highest correlation coefficient for the monthly mean total ozone anomalies is reached in November with 0.94.  相似文献   

2.
The Global Ozone Monitoring Experiment (GOME) onboard the ERS-2 satellite has been in operation since July 1995. The Norwegian ground-based total ozone network has played an important role both in the main validation during the commissioning phase and in the validation of upgraded versions of the analysis algorithms of the instrument. The ground-based network consists of various spectrometer types (Dobson, Brewer, UV filter instruments). The validation of the second algorithm version used until January 1998 reveals a very good agreement between GOME and ground-based data at solar zenith angles <60° and deviations of GOME total ozone data from ground-based data of up to ±60 DU (∼20%) at zenith angles ≥60°. The deviations strongly depend on the season of the year, being negative in summer and positive in winter/spring, The deviations furthermore show a considerable scattering (up to ±25 DU in monthly average values of 5° SZA intervals), even in close spatial and temporal coincidence with ground-based measurements, especially in the high Arctic. The deviations are also dependent on the viewing geometry/ground pixel size with an additional negative offset for the large pixels used in the backswath mode and at solar zenith angles ≥85°, compared to forward-swath pixels.  相似文献   

3.
本文基于1979—2014年臭氧总量的卫星遥感数据,利用多元线性回归模型对臭氧总量数据序列进行模拟计算,考察了北太平洋上空臭氧总量长期变化趋势及其影响因素的作用.结果表明,北太平洋地区大气臭氧总量长期变化呈现减少趋势,但是减少速率随季节和纬度带表现出差异性,在各纬度带臭氧峰值季节臭氧下降趋势最为显著.在0°—15°N地区臭氧高值出现在夏秋季节并在8月达到峰值,峰值月份臭氧年均下降率约为0.2DU/a;15°—30°N亚热带地区臭氧高值出现在春夏季并在5月达到峰值,峰值月份臭氧年均下降速率约为0.22DU/a;而在30°—45°N中纬度地区臭氧高值出现在冬春季并在2月达到峰值,峰值月份臭氧年均下降率0.75DU/a.在臭氧分布年平均态基础上,影响臭氧总量分布变化的因素主要有臭氧损耗物质(EESC)、太阳辐射周期(Solar)、准两年振荡(QBO)和厄尔尼诺-南方涛动(ENSO)等.其中,EESC导致臭氧损耗效应随着纬度升高而增大,在从低到高的三个纬度带损耗最大值分别为11DU、16DU和66DU;Solar增强导致臭氧增加,在三个纬度带的增加效应最大值分别为16DU、17DU和19DU;QBO@10hPa和QBO@30hPa对臭氧影响幅度基本在±10DU内波动,只有QBO@10hPa对30°—45°N区域的影响作用达到14DU,值得注意的是QBO影响作用随着纬度变化存在相位差异,在0°—15°N区域臭氧变化与QBO呈现相同相位,而在15°—30°N和30°—45°N区域臭氧变化与QBO呈现相反相位;ENSO对各个纬度带臭氧影响幅度也在±10DU内,ENSO影响作用在不同纬度带也存在相位差异,臭氧总量变化在0°—15°N、15°—30°N区域与ENSO相位相反,在30°—45°N区域与ENSO相位一致.  相似文献   

4.
During the Arctic Tropospheric Ozone Chemistry (ARCTOC) campaigns at Ny-Ålesund, Spitsbergen, the role of halogens in the depletion of boundary layer ozone was investigated. In spring 1995 and 1996 up to 30 ppt bromine monoxide were found whenever ozone decreased from normal levels of about 40 ppb. Those main trace gases and others were specifically followed in the UV-VIS spectral region by differential optical absorption spectroscopy (DOAS) along light paths running between 20 and 475 m a.s.l. The daily variation of peroxy radicals closely followed the ozone photolysis rate J(O3(O1D)) in the absence of ozone depletion most of the time. However, during low ozone events this close correlation was no longer found because the measurement of radicals by chemical amplification (CA) turned out to be sensitive to peroxy radicals and ClOx. Large CA signals at night can sometimes definitely be assigned to ClOx and reached up to 2 ppt. Total bromine and iodine were both stripped quantitatively from air by active charcoal traps and measured after neutron activation of the samples. Total bromine increased from background levels of about 15 ppt to a maximum of 90 ppt during an event of complete ozone depletion. For the spring season a strong source of bromine is identified in the pack ice region according to back trajectories. Though biogenic emission sources cannot be completely ruled out, a primary activation of halogenides by various oxidants seems to initiate an efficient autocatalytic process, mainly driven by ozone and light, on ice and perhaps on aerosols. Halogenides residing on pack ice surfaces are continuously oxidised by hypohalogenous acids releasing bromine and chlorine into the air. During transport and especially above open water this air mixes with upper layer pristine air. As large quantities of bromine, often in the form of BrO, have been observed at polar sunrise also around Antarctica, its release seems to be a natural phenomenon. The source strength of bromine from halogen activation on the pack ice, as based on the measured inorganic bromine levels, averages about 1012 Br-atoms m−2 s−1 during sunlit periods in Arctic spring. The total source strength of inorganic bromine from sunlit polar regions may therefore amount to 30 kt y−1.  相似文献   

5.
The variations of total ozone at Alma-Ata (43°N, 76 °E) and ozone profiles obtained by balloon sounding at Tateno (36°N, 140°E), Wallops Island (38°N, 75°W) and Cagliari (39°N, 9°E) in the periods of Forbush decreases (FD) in galactic cosmic rays have been analysed. A decrease of total ozone was observed in the initial stage of the FD and an increase 10–11 days later. The average total deviations calculated using the superposed epoch method for 9 FD events are equal to 30 D. U. in the positive and to –18 D. U. in the negative phase. The changes of average ozone profiles, associated with 26 FD events, are more significant in the lower stratosphere and upper troposphere. The decrease of the partial ozone pressure at a height of 12–15 km is about 30 mb. These vertical variations of ozone coincide with the average changes of the respective temperature profiles. A cooling, on the average, of 3°C was observed at 12–15 km, and a heating of 4°C below this level.  相似文献   

6.
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7.
Changes in solar ultraviolet flux produce changes in ozone concentration in the upper stratosphere with associated radiative and dynamical effects. At low latitudes, the response of ozone mixing ratio to solar UV variations on the time scale of the solar rotation period is well characterized observationally. In addition, there is some provisional evidence for an ozone response at intermediate periods of 60-80 days. Current two-dimensional stratospheric models simulate the observed 27-day response amplitudes and phase lags with reasonable accuracy in the upper stratosphere. The observed response of total ozone on the 27-day time scale is also in approximate agreement with the same models although observed ozone sensitivities and phase lags are slightly larger than expected theoretically. Future studies of the 27-day response at higher latitudes and altitudes are needed to test more completely our understanding of the direct effects of solar UV variability on the middle atmosphere.  相似文献   

8.
Variations of the total electron content according to the index IONEX IGS in the period of preparation of the earthquake in Haiti (M7.9) on January 12, 2010, are considered. The situation is exceptional owing to the unique position of the island of Haiti relative to the structure of the ionosphere over the Caribbean Sea: the ionospheric region over Haiti is in the trough formed by the northern slope of the equatorial anomaly and additional maximum formed at latitudes of approximately 30° N within this longitudinal interval. Distortion of the shape of the equatorial anomaly, total decrease in the electron content in the equatorial anomaly a few days prior to the earthquake, increase in the electron concentration directly over the earthquake epicenter a few days prior to the earthquake, increase in the additional maximum at latitudes of ∼30° N, and formation of an additional maximum in the Southern Hemisphere in the region conjugated to the additional maximum in the Northern Hemisphere in the periods of its intensification are observed. The configuration of the equatorial anomaly is restored after the earthquake.  相似文献   

9.
Trends in total column ozone have been analyzed in terms of the equatorial zonal wind. We used zonal monthly mean total ozone from Total Ozone Mapping Spectrometer (TOMS) and monthly mean zonal wind in the equatorial stratosphere at 30 hPa to define the phases of the quasi-biennial oscillation (QBO). Total column ozone trends have been assessed during the period 1979–2004, for both Hemispheres, and for each month, under three conditions considering, all the ozone dataset, ozone values during easterly phase and ozone values during westerly phase of the QBO. When the whole dataset is considered, negative trends are observed. From low to midlatitudes a zonal pattern is noticed with increasing negative values toward higher latitudes. When the data is filtered according to the QBO phase, statistically significant positive trends appear in the westerly case during January to May at low latitudes .The trend pattern in the case of the easterly phase presents more negative values.  相似文献   

10.
基于法国DEMETER卫星ISL探测器升轨数据,统计分析了2005—2009年全球37个Mw≥7.0级地震前后电离层电子浓度变化.结果发现,共有19个地震（51%）前观测到了较为明显的电子浓度异常扰动现象,其中大部分表现为异常增强;观测到的电子浓度异常现象一般出现在震前1~5天内,也有部分地震前出现两次及以上扰动现象.分析表明,在赤道和中低纬地区更容易观测到明显的电子浓度扰动,即异常震例基本发生在纬度±40°以内（18次）,更是以±20°内居多（13次）.此外,震源深度对电子浓度扰动的影响并不明显,而震级大小则与扰动幅度基本上呈正相关;震前出现的电子浓度异常有时会受到地磁活跃的共同影响,此时的扰动幅度一般较大.地震电离层扰动现象是复杂多变的,需要联合地基和天基手段共同观测,并从机理上加强研究.  相似文献   

11.
Summary The total ozone response to strong major geomagnetic storms (Ap≥60) in winter along the 50° N latitudinal circle is studied. The results add to the recent results of Laštovička et al. (1992) obtained for European middle latitudes (∼50°N) and to the results of Mlch (1994). A significant response of total ozone is only observed in winter under high solar activity/E-phase of QBO conditions (E-max) and seems to be caused by geomagnetic storm-induced changes of atmospheric dynamics. There are two sectors along latitude 50°N, which are sensitive to forcing by geomagnetic storms both in total ozone and the troposphere — north-eastern Atlantic-European and eastern Siberia-Aleutian sectors. The total ozone response under E-max conditions manifests itself mainly as a large decrease in the longitudinal variation of ozone after the storm, which means an increase of ozone in Europe. The observed effects in total ozone consist in redistribution, not production or loss of ozone.  相似文献   

12.
With a detailed chemistry scheme for the middle atmosphere up to 70 km which has been added to the 3-D Karlsruhe simulation model of the middle atmosphere (KASIMA), the effects of coupling chemistry and dynamics through ozone are studied for the middle atmosphere. An uncoupled version using an ozone climatology for determining heating rates and a coupled version using on-line ozone are compared in a 10-month integration with meteorological analyses for the winter 1992/93 as the lower boundary condition. Both versions simulate the meteorological situation satisfactorily, but exhibit a too cold lower stratosphere. The on-line ozone differs from the climatological data between 20 and 40 km by exhibiting too high ozone values, whereas in the lower mesosphere the ozone values are too low. The coupled model version is stable and differs only above 40 km significantly from the uncoupled version. Direct heating effects are identified to cause most of the differences. The well-known negative correlation between temperature and ozone is reproduced in the model. As a result, the coupled version slightly approaches the climatological ozone field. Further feedback effects are studied by using the on-line ozone field as a basis for an artificial climatology. For non-disturbed ozone conditions realistic monthly and zonally averaged ozone data are sufficient to determine the heating rates for modelling the middle atmosphere.  相似文献   

13.
A self-consistent method for daytime F-region modelling was applied to EISCAT observations during two periods comprising the very disturbed days 3 April 1992 and 10 April 1990. The observed strong Ne decrease at F2-layer heights originated from different physical mechanisms in the two cases. The negative F2-layer storm effect with an NmF2 decrease by a factor of 6.4 on 3 April 1992 was produced by enhanced electric fields (E 85 mV/m) and strong downward plasma drifts, but without any noticeable changes in thermos-pheric parameters. The increase of the O+ + N2 reaction rate resulted in a strong enrichment of the ionosphere with molecular ions even at F2-layer heights. The enhanced electric field produced a wide mid-latitude daytime trough on 03 April 1992 not usually observed during similar polarization jet events. The other strong negative storm effect on 10 April 1990 with a complete disappearance of the F2-layer maximum at the usual heights was attributed mainly to changes in neutral composition and temperature. A small value for the shape parameter S in the neutral temperature profile and a low neutral temperature at 120 km indicate strong cooling of the lower thermosphere. We propose that this cooling is due to increased nitric oxide concentration usually observed at these heights during geomagnetic storms.  相似文献   

14.
Summary Ozone observations made during 1964 and 1965 at nine Mediterranean, central and southeast European stations (latitudes 38–52°N, longitudes 9–23°E) reveal patterns of seasonal and shorter time-variations in total ozone as well as in vertical ozone distribution. During the winter-spring season, a significant increase (20%) of ozone occurs essentially simultaneously with the spring stratospheric warming, and is noticed at all stations.—Autocorrelation coefficients show that the total ozone on any day is strongly related to the total ozone of the preceding four days in summer or one or two days in winter-spring or autumn. Changes of total ozone in southeast Europe correlate closely with those in Mediterranean Europe, and less closely with those from north central Europe.—Power spectrum analysis detects the dependence of ozone changes on processes with periods longer than 6–8 days, and indicates a significant oscillation with a period of 14–15 days, perhaps a result of the direct influence of lower stratospheric circumhemispheric circulation. — Reliable vertical ozone soundings were not available from all stations. The mean vertical profiles at Arosa, Switzerland (47°N) and Belsk, Poland (51°) are very similar. More than 60% of the variability of the total ozone is contributed by changes in ozone concentration between 10 and 24 km; less than 10% is due to variations above 33 km. Changes in ozone partial pressure at different altitudes, and relationships of those changes to total ozone, indicates that a mean vertical ozone distribution may be described adequately by considering the ozone changes in four layers: a) the troposphere, b) the lower stratosphere up to 24 km, c) a transition layer from 24 km to a variable upper border at 33–37 km, and d) the layer above 33–37 km.Part of this paper was presented at the Ozone Seminar in Potsdam, Germany, 27 September 1966.  相似文献   

15.
Erythemally-weighted ultraviolet (UVery) levels measured over southern England, during anticyclonic weather between 30 April and 2 May, 1997, were almost 50 higher than normally expected for clear skies and were similar to mid-summer values for the first time since measurements began in 1990. Investigation of this episode suggests that a combination of both meteorological and chemical effects were responsible for generating record low ozone amounts for the time of year. Further, comparisons between the A band ultraviolet (315 to 400 nm wavelength) amounts, and radiative calculations confirm that the high UVery was primarily due to the reduction in total ozone. These results are contrasted with a similar period for 1998, in which near climatological ozone amounts were measured. The prospects for enhanced UVery levels in future years are briefly reviewed in the light of expected increases in stratospheric halogen levels and greenhouse gases.  相似文献   

16.
The spatial and temporal distribution of total ozone over India and its vertical distribution in theatmosphere during 1964–1969 was studied using Dobson spectrophotometer data at a network of six stations in India, Srinagar (34°N), New Delhi (28°N), Varanasi (24°N), Ahmedabad (23°N), Dum Dum (22°N), and Kodaikanal (10°N). The annual and seasonal variations show a clear phase-shift in the occurrence of the ozone maxima and minima as one proceeds from higher to lower latitudes in the tropics. In the northern stations (north of 25°N) the increase in total ozone during the course of the annual variation is caused by the fractional increase in all layers from the ground to 28 km, the main contribution coming from 10–24 km. Above 28 km the concentration changes roughly in accordance with photochemical production.In lower latitudes (south of 25°N) an increase in total ozone amount during the annual cycle is caused by a gradual increase in all the layers from the ground to 36 km above which the variation is negligible.  相似文献   

17.
我国上空平流层中微量气体的垂直分布和变化趋势   总被引：7，自引：0，他引：7       下载免费PDF全文
利用1992～2005年卤素掩星试验（HALOE）的观测资料分析了中国上空平流层的几种微量气体（NO, NO2, HF, HCl, CH4, H2O 和O3）混合比的垂直分布和变化趋势，以期为研究平流层的辐射和化学过程提供一些有用的数据. 文中除给出我国上空平流层各高度上平均的各种微量气体的含量外，还给出青藏高原上空这些微量气体的含量. 分析结果表明，平流层各种微量气体混合比的垂直分布有其不同的特征，在对流层上层到平流层底部各种微量气体的混合比分布和季节变化与平流层相比有明显的差异；分析结果还表明，这些微量气体的季节变化、准两年周期振荡和长期变化趋势都很明显，并且在平流层的不同高度上它们的变化趋势是不相同的. 在平流层中层，NO, NO2, HCl 和H2O 混合比在1998年以前都是增加而后则是明显下降的，但O3相反，在1998年以前明显减少，1998年后其减少的趋势不明显. 这表明，近年来平流层中层这些微量气体的减少使得它们对臭氧的破坏有所缓解. 但在平流层下层，臭氧的耗损仍然很明显.  相似文献   

18.
Energetic particle precipitation couples the solar wind to the Earth's atmosphere and indirectly to Earth's climate. Ionisation and dissociation increases, due to particle precipitation, create odd nitrogen (NOx) and odd hydrogen (HOX) in the upper atmosphere, which can affect ozone chemistry. The long-lived NOx can be transported downwards into the stratosphere, particularly during the polar winter. Thus, the impact of NOx is determined by both the initial ionisation production, which is a function of the particle flux and energy spectrum, as well as transport rates. In this paper, we use the Sodankylä Ion and Neurtal Chemistry (SIC) model to simulate the production of NOx from examples of the most representative particle flux and energy spectra available today of solar proton events (SPE), auroral energy electrons, and relativistic electron precipitation (REP). Large SPEs are found to produce higher initial NOx concentrations than long-lived REP events, which themselves produce higher initial NOx levels than auroral electron precipitation. Only REP microburst events were found to be insignificant in terms of generating NOx. We show that the Global Ozone Monitoring by Occultation of Stars (GOMOS) observations from the Arctic winter 2003–2004 are consistent with NOx generation by a combination of SPE, auroral altitude precipitation, and long-lived REP events.  相似文献   

19.
Using the data on solar proton fluxes measured on board the GOES satellites, the most powerful solar proton events (SPEs) of solar cycle 23 are selected, and ionization rates in the atmosphere in these periods at high latitudes of the Northern Hemisphere are calculated. Assuming that each ion pair formed at the retardation of solar protons in the atmosphere leads to the formation of 1.25 molecules of nitric oxide, 2.0 molecules of the OH radical, and one oxygen atom, changes in the content of ozone, nitrogen and other compounds were calculated using a photochemical model. The calculations showed that the strongest ionization and destruction of ozone was caused by SPEs that occurred on July 14, 2000; November 8, 2000; November 4, 2001; and October 28, 2003. The results can form the basis for compiling the catalog of changes in ionization and ozone in the atmosphere caused by solar proton activity.  相似文献   

20.
The results of three series of rocket measurements of mesospheric electric fields carried out under different geomagnetic conditions at polar and high middle latitudes are analysed. The measurements show a clear dependence of the vertical electric fields on geomagnetic activity at polar and high middle latitudes. The vertical electric fields in the lower mesosphere increase with the increase of geomagnetic indexes Kp and Kp. The simultaneous increase of the vertical electric field strength and ion conductivity was observed in the mesosphere during geomagnetic disturbances. This striking phenomenon was displayed most clearly during the solar proton events of October, 1989 accompanied by very strong geomagnetic storm (Kp = 8+). A possible mechanism of generation of the vertical electric fields in the mesosphere caused by gravitational sedimentation of charged aerosol particles is discussed. Simultaneous existence in the mesosphere of both the negative and positive multiply charged aerosol particles of different sizes is assumed for explanation of the observed V/m vertical electric fields and their behaviour under geomagnetically disturbed conditions.Paper Presented at the Second IAGA/ICMA (IAMAS) Workshop on Solar Activity Forcing of the Middle Atmosphere, Prague, August 1997  相似文献   

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